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Spotlights on Recent JACS Publications pp 1–1 DOI: 10.1021/ja312637b |
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Engineered rRNA Enhances the Efficiency of Selenocysteine Incorporation during Translation Ross Thyer, Aleksandra Filipovska, and Oliver Rackham pp 2–5 DOI: 10.1021/ja3069177 Supporting Info |
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Synthesis of Monoclinic Potassium Niobate Nanowires That Are Stable at Room Temperature Seungwook Kim, Ju-Hyuck Lee, Jaeyeon Lee, Sang-Woo Kim, Myung Hwa Kim, Sungnam Park, Haegeun Chung, Yong-Il Kim, and Woong Kim pp 6–9 DOI: 10.1021/ja308209m Supporting Info |
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Core Values: Elucidating the Role of Seed Structure in the Synthesis of Symmetrically Branched Nanocrystals Christopher J. DeSantis and Sara E. Skrabalak pp 10–13 DOI: 10.1021/ja308456w Supporting Info |
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A Chemistry-Based Method To Detect Individual Telomere Length at a Single Chromosome Terminus Takumi Ishizuka, Yan Xu, and Makoto Komiyama pp 14–17 DOI: 10.1021/ja308481c Supporting Info |
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Enhanced Photoresponsive Ultrathin Graphitic-Phase C3N4 Nanosheets for Bioimaging Xiaodong Zhang, Xiao Xie, Hui Wang, Jiajia Zhang, Bicai Pan, and Yi Xie pp 18–21 DOI: 10.1021/ja308249k Supporting Info |
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A Binding Site for Nonsteroidal Anti-inflammatory Drugs in Fatty Acid Amide Hydrolase Laura Bertolacci, Elisa Romeo, Marina Veronesi, Paola Magotti, Clara Albani, Mauro Dionisi, Chiara Lambruschini, Rita Scarpelli, Andrea Cavalli, Marco De Vivo, Daniele Piomelli, and Gianpiero Garau pp 22–25 DOI: 10.1021/ja308733u Supporting Info |
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Synthesis and Structural Characterization of an Atom-Precise Bimetallic Nanocluster, Ag4Ni2(DMSA)4 Scott R. Biltek, Sukhendu Mandal, Ayusman Sen, Arthur C. Reber, Anthony F. Pedicini, and Shiv N. Khanna pp 26–29 DOI: 10.1021/ja308884s Supporting Info |
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Energetics of Zinc-Mediated Interactions in the Allosteric Pathways of Metal Sensor Proteins Dhruva K. Chakravorty, Trent M. Parker, Alfredo J. Guerra, C. David Sherrill, David P. Giedroc, and Kenneth M. Merz, Jr. pp 30–33 DOI: 10.1021/ja309170g Supporting Info |
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Electric Field-Induced Assembly of Monodisperse Polyhedral Metal–Organic Framework Crystals Nobuhiro Yanai, Melinda Sindoro, Jing Yan, and Steve Granick pp 34–37 DOI: 10.1021/ja309361d Supporting Info |
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Surface Plasmon Mediated Chemical Solution Deposition of Gold Nanoparticles on a Nanostructured Silver Surface at Room Temperature Jingjing Qiu, Yung-Chien Wu, Yi-Chung Wang, Mark H. Engelhard, Lisa McElwee-White, and Wei David Wei pp 38–41 DOI: 10.1021/ja309392x Supporting Info |
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Design of Pt–Pd Binary Superlattices Exploiting Shape Effects and Synergistic Effects for Oxygen Reduction Reactions Yijin Kang, Xingchen Ye, Jun Chen, Yun Cai, Rosa E. Diaz, Radoslav R. Adzic, Eric A. Stach, and Christopher B. Murray pp 42–45 DOI: 10.1021/ja3097527 Supporting Info |
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Highlightable Ca2+ Indicators for Live Cell Imaging Hiofan Hoi, Tomoki Matsuda, Takeharu Nagai, and Robert E. Campbell pp 46–49 DOI: 10.1021/ja310184a Supporting Info |
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Hydration of Terminal Alkynes Catalyzed by Water-Soluble Cobalt Porphyrin Complexes Tadashi Tachinami, Takuho Nishimura, Richiro Ushimaru, Ryoji Noyori, and Hiroshi Naka pp 50–53 DOI: 10.1021/ja310282t Supporting Info |
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Bioinspired Multifunctional Janus Particles for Droplet Manipulation Yuanjin Zhao, Hongcheng Gu, Zhuoying Xie, Ho Cheung Shum, Baoping Wang, and Zhongze Gu pp 54–57 DOI: 10.1021/ja310389w Supporting Info |
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N-Heterocyclic Carbene-Catalyzed Ireland–Coates Claisen Rearrangement: Synthesis of Functionalized β-Lactones Lisa Candish and David W. Lupton pp 58–61 DOI: 10.1021/ja310449k Supporting Info |
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A Photostable AIE Luminogen for Specific Mitochondrial Imaging and Tracking Chris Wai Tung Leung, Yuning Hong, Sijie Chen, Engui Zhao, Jacky Wing Yip Lam, and Ben Zhong Tang pp 62–65 DOI: 10.1021/ja310324q Supporting Info |
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Rh(III)-Catalyzed Regioselective Synthesis of Pyridines from Alkenes and α,β-Unsaturated Oxime Esters Jamie M. Neely and Tomislav Rovis pp 66–69 DOI: 10.1021/ja3104389 Supporting Info |
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Surface Display of a Redox Enzyme and its Site-Specific Wiring to Gold Electrodes Liron Amir, Stewart A. Carnally, Josep Rayo, Shaked Rosenne, Sarit Melamed Yerushalmi, Orr Schlesinger, Michael M. Meijler, and Lital Alfonta pp 70–73 DOI: 10.1021/ja310556n Supporting Info |
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A Supramolecular Cross-Linked Conjugated Polymer Network for Multiple Fluorescent Sensing Xiaofan Ji, Yong Yao, Jinying Li, Xuzhou Yan, and Feihe Huang pp 74–77 DOI: 10.1021/ja3108559 Supporting Info |
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Temporal Switching of Homo-FRET Pathways in Single-Chromophore Dimer Models of π-Conjugated Polymers Thomas Stangl, Sebastian Bange, Daniela Schmitz, Dominik Würsch, Sigurd Höger, Jan Vogelsang, and John M. Lupton pp 78–81 DOI: 10.1021/ja3108643 Supporting Info |
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Enantioselective Homocrotylboration of Aliphatic Aldehydes Hongkun Lin, Wenbo Pei, Hao Wang, Kendall N. Houk, and Isaac J. Krauss pp 82–85 DOI: 10.1021/ja311061n Supporting Info |
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Enantioselective Synthesis of Planar Chiral Ferrocenes via Palladium-Catalyzed Direct Coupling with Arylboronic Acids De-Wei Gao, Yan-Chao Shi, Qing Gu, Zheng-Le Zhao, and Shu-Li You pp 86–89 DOI: 10.1021/ja311082u Supporting Info |
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Selective Fluorescent Detection of RNA in Living Cells by Using Imidazolium-Based Cyclophane Bahareh Shirinfar, Nisar Ahmed, Yu Shin Park, Gun-Sik Cho, Il Seung Youn, Jin-Kwan Han, Hong Gil Nam, and Kwang S. Kim pp 90–93 DOI: 10.1021/ja3112274 Supporting Info |
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Stereoselective Access to Z and E Macrocycles by Ruthenium-Catalyzed Z-Selective Ring-Closing Metathesis and Ethenolysis Vanessa M. Marx, Myles B. Herbert, Benjamin K. Keitz, and Robert H. Grubbs pp 94–97 DOI: 10.1021/ja311241q Supporting Info |
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DNA Ligase-Mediated Translation of DNA Into Densely Functionalized Nucleic Acid Polymers Ryan Hili, Jia Niu, and David R. Liu pp 98–101 DOI: 10.1021/ja311331m Supporting Info |
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Thermodynamics of Anion−π Interactions in Aqueous Solution Paloma Arranz-Mascarós, Carla Bazzicalupi, Antonio Bianchi, Claudia Giorgi, Maria-Luz Godino-Salido, Maria-Dolores Gutiérrez-Valero, Rafael Lopez-Garzón, and Matteo Savastano pp 102–105 DOI: 10.1021/ja311389z Supporting Info |
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Controlled Spontaneous Emission of Single Molecules in a Two-Dimensional Photonic Band Gap Takahiro Kaji, Toshiki Yamada, Syoji Ito, Hiroshi Miyasaka, Rieko Ueda, Shin-ichiro Inoue, and Akira Otomo pp 106–109 DOI: 10.1021/ja3115357 Supporting Info |
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Topochemical Polymerization of Phenylacetylene Macrocycles: A New Strategy for the Preparation of Organic Nanorods Simon Rondeau-Gagné, Jules Roméo Néabo, Maude Desroches, Jérémie Larouche, Josée Brisson, and Jean-François Morin pp 110–113 DOI: 10.1021/ja3116422 Supporting Info |
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Dynamic or Nondynamic? Helical Trajectory in Hexabenzocoronene Nanotubes Biased by a Detachable Chiral Auxiliary Wei Zhang, Wusong Jin, Takanori Fukushima, Noriyuki Ishii, and Takuzo Aida pp 114–117 DOI: 10.1021/ja311738m Supporting Info |
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Iron Sulfide Catalyzed Redox/Condensation Cascade Reaction between 2-Amino/Hydroxy Nitrobenzenes and Activated Methyl Groups: A Straightforward Atom Economical Approach to 2-Hetaryl-benzimidazoles and -benzoxazoles Thanh Binh Nguyen, Ludmila Ermolenko, and Ali Al-Mourabit pp 118–121 DOI: 10.1021/ja311780a Supporting Info |
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Mechanical Identities of RNA and DNA Double Helices Unveiled at the Single-Molecule Level Elías Herrero-Galán, Maria Eugenia Fuentes-Perez, Carolina Carrasco, José M. Valpuesta, José L. Carrascosa, Fernando Moreno-Herrero, and J. Ricardo Arias-Gonzalez pp 122–131 DOI: 10.1021/ja3054755 Supporting Info |
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Ternary Electrocatalysts for Oxidizing Ethanol to Carbon Dioxide: Making Ir Capable of Splitting C–C Bond Meng Li, David A. Cullen, Kotaro Sasaki, Nebojsa S. Marinkovic, Karren More, and Radoslav R. Adzic pp 132–141 DOI: 10.1021/ja306384x Supporting Info |
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Mechanism of Homogeneous Reduction of CO2 by Pyridine: Proton Relay in Aqueous Solvent and Aromatic Stabilization Chern-Hooi Lim, Aaron M. Holder, and Charles B. Musgrave pp 142–154 DOI: 10.1021/ja3064809 Supporting Info |
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Formation of Nitrogen-Containing Polycyclic Cations by Gas-Phase and Intracluster Reactions of Acetylene with the Pyridinium and Pyrimidinium Ions Abdel-Rahman Soliman, Ahmed M. Hamid, Isaac Attah, Paul Momoh, and M. Samy El-Shall pp 155–166 DOI: 10.1021/ja3068116 Supporting Info |
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Exploring Key Orientations at Protein–Protein Interfaces with Small Molecule Probes Eunhwa Ko, Arjun Raghuraman, Lisa M. Perez, Thomas R. Ioerger, and Kevin Burgess pp 167–173 DOI: 10.1021/ja3067258 Supporting Info |
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Functional Imaging of Legumain in Cancer Using a New Quenched Activity-Based Probe Laura E. Edgington, Martijn Verdoes, Alberto Ortega, Nimali P. Withana, Jiyoun Lee, Salahuddin Syed, Michael H. Bachmann, Galia Blum, and Matthew Bogyo pp 174–182 DOI: 10.1021/ja307083b Supporting Info |
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ExBox: A Polycyclic Aromatic Hydrocarbon Scavenger Jonathan C. Barnes, Michal Juríček, Nathan L. Strutt, Marco Frasconi, Srinivasan Sampath, Marc A. Giesener, Psaras L. McGrier, Carson J. Bruns, Charlotte L. Stern, Amy A. Sarjeant, and J. Fraser Stoddart pp 183–192 DOI: 10.1021/ja307360n Supporting Info |
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DNA Mismatch Synthesis Complexes Provide Insights into Base Selectivity of a B Family DNA Polymerase Shuangluo Xia, Jimin Wang, and William H. Konigsberg pp 193–202 DOI: 10.1021/ja3079048 Supporting Info |
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Explaining the Highly Enantiomeric Photocyclodimerization of 2-Anthracenecarboxylate Bound to Human Serum Albumin Using Time-Resolved Anisotropy Studies Denis Fuentealba, Hanako Kato, Masaki Nishijima, Gaku Fukuhara, Tadashi Mori, Yoshihisa Inoue, and Cornelia Bohne pp 203–209 DOI: 10.1021/ja3081555 Supporting Info |
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Caulosegnins I–III: A Highly Diverse Group of Lasso Peptides Derived from a Single Biosynthetic Gene Cluster Julian D. Hegemann, Marcel Zimmermann, Xiulan Xie, and Mohamed A. Marahiel pp 210–222 DOI: 10.1021/ja308173b Supporting Info |
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Hydrogen Evolution from Pt/Ru-Coated p-Type WSe2 Photocathodes James R. McKone, Adam P. Pieterick, Harry B. Gray, and Nathan S. Lewis pp 223–231 DOI: 10.1021/ja308581g Supporting Info |
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Impact of Diradical Character on Two-Photon Absorption: Bis(acridine) Dimers Synthesized from an Allenic Precursor Kenji Kamada, Shin-ichi Fuku-en, Shu Minamide, Koji Ohta, Ryohei Kishi, Masayoshi Nakano, Hiroyuki Matsuzaki, Hiroshi Okamoto, Hiroyuki Higashikawa, Katsuya Inoue, Satoshi Kojima, and Yohsuke Yamamoto pp 232–241 DOI: 10.1021/ja308396a Supporting Info |
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Twisted Cyanines: A Non-Planar Fluorogenic Dye with Superior Photostability and its Use in a Protein-Based Fluoromodule Nathaniel I. Shank, Ha H. Pham, Alan S. Waggoner, and Bruce A. Armitage pp 242–251 DOI: 10.1021/ja308629w Supporting Info |
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Ion Pair Dynamics: Solvolyses of Chiral 1,3-Diarylallyl Carboxylates as a Case Study Konstantin Troshin and Herbert Mayr pp 252–265 DOI: 10.1021/ja308670g Supporting Info |
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Surface-Induced Hydrogelation Inhibits Platelet Aggregation Wenting Zheng, Jie Gao, Lijie Song, Chongyi Chen, Di Guan, Zhihong Wang, Zhibo Li, Deling Kong, and Zhimou Yang pp 266–271 DOI: 10.1021/ja308690y Supporting Info |
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Antioxidant β-Carotene Does Not Quench Singlet Oxygen in Mammalian Cells Gabriela N. Bosio, Thomas Breitenbach, Julieta Parisi, Miguel Reigosa, Frances H. Blaikie, Brian W. Pedersen, Elsa F. F. Silva, Daniel O. Mártire, and Peter R. Ogilby pp 272–279 DOI: 10.1021/ja308930a Supporting Info |
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Nickel-Catalyzed Cross Couplings of Benzylic Ammonium Salts and Boronic Acids: Stereospecific Formation of Diarylethanes via C–N Bond Activation Prantik Maity, Danielle M. Shacklady-McAtee, Glenn P. A. Yap, Eric R. Sirianni, and Mary P. Watson pp 280–285 DOI: 10.1021/ja3089422 Supporting Info |
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Streamlined Expressed Protein Ligation Using Split Inteins Miquel Vila-Perelló, Zhihua Liu, Neel H. Shah, John A. Willis, Juliana Idoyaga, and Tom W. Muir pp 286–292 DOI: 10.1021/ja309126m Supporting Info |
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Recyclable Thermoresponsive Polymer–Cellulase Bioconjugates for Biomass Depolymerization Katherine J. Mackenzie and Matthew B. Francis pp 293–300 DOI: 10.1021/ja309277v Supporting Info |
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Structure Enhancement Factor Relationships in Single Gold Nanoantennas by Surface-Enhanced Raman Excitation Spectroscopy Samuel L. Kleinman, Bhavya Sharma, Martin G. Blaber, Anne-Isabelle Henry, Nicholas Valley, R. Griffith Freeman, Michael J. Natan, George C. Schatz, and Richard P. Van Duyne pp 301–308 DOI: 10.1021/ja309300d Supporting Info |
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Profluorogenic Reductase Substrate for Rapid, Selective, and Sensitive Visualization and Detection of Human Cancer Cells that Overexpress NQO1 William C. Silvers, Bijeta Prasai, David H. Burk, Matthew L. Brown, and Robin L. McCarley pp 309–314 DOI: 10.1021/ja309346f Supporting Info |
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Description of Aromaticity in Porphyrinoids Judy I. Wu, Israel Fernández, and Paul v. R. Schleyer pp 315–321 DOI: 10.1021/ja309434t Supporting Info |
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Pipette–Surface Interaction: Current Enhancement and Intrinsic Force Richard W. Clarke, Alexander Zhukov, Owen Richards, Nicholas Johnson, Victor Ostanin, and David Klenerman pp 322–329 DOI: 10.1021/ja3094586 Supporting Info |
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Electrodeposition of Crystalline GaAs on Liquid Gallium Electrodes in Aqueous Electrolytes Eli Fahrenkrug, Junsi Gu, and Stephen Maldonado pp 330–339 DOI: 10.1021/ja309476x Supporting Info |
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Self-Assembled Antibody Multimers through Peptide Nucleic Acid Conjugation Stephanie A. Kazane, Jun Y. Axup, Chan Hyuk Kim, Mihai Ciobanu, Erik D. Wold, Sofia Barluenga, Benjamin A. Hutchins, Peter G. Schultz, Nicolas Winssinger, and Vaughn V. Smider pp 340–346 DOI: 10.1021/ja309505c Supporting Info |
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Self-Assembled Monolayers of n-Alkanethiols Suppress Hydrogen Evolution and Increase the Efficiency of Rechargeable Iron Battery Electrodes Souradip Malkhandi, Bo Yang, Aswin K. Manohar, G. K. Surya Prakash, and S. R. Narayanan pp 347–353 DOI: 10.1021/ja3095119 Supporting Info |
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Cascade of Reduced Speed and Accuracy after Errors in Enzyme-Free Copying of Nucleic Acid Sequences Kevin Leu, Eric Kervio, Benedikt Obermayer, Rebecca M. Turk-MacLeod, Caterina Yuan, Jesus-Mario Luevano, Jr., Eric Chen, Ulrich Gerland, Clemens Richert, and Irene A. Chen pp 354–366 DOI: 10.1021/ja3095558 Supporting Info |
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Thioflavin T as an Efficient Inducer and Selective Fluorescent Sensor for the Human Telomeric G-Quadruplex DNA Jyotirmayee Mohanty, Nilotpal Barooah, V. Dhamodharan, S. Harikrishna, P. I. Pradeepkumar, and Achikanath C. Bhasikuttan pp 367–376 DOI: 10.1021/ja309588h Supporting Info |
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Hydrophobic Enhancement of Dopa-Mediated Adhesion in a Mussel Foot Protein Wei Wei, Jing Yu, Christopher Broomell, Jacob N. Israelachvili, and J. Herbert Waite pp 377–383 DOI: 10.1021/ja309590f Supporting Info |
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Tailored Design of Multiple Nanoarchitectures in Metal-Cyanide Hybrid Coordination Polymers Ming Hu, Alexei A. Belik, Masataka Imura, and Yusuke Yamauchi pp 384–391 DOI: 10.1021/ja3096703 Supporting Info |
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Chemistry and Structure of a Host–Guest Relationship: The Power of NMR and X-ray Diffraction in Tandem Qi-Qiang Wang, Victor W. Day, and Kristin Bowman-James pp 392–399 DOI: 10.1021/ja3096762 Supporting Info |
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Mesomorphic [2]Rotaxanes: Sheltering Ionic Cores with Interlocking Components Natalie D. Suhan, Stephen J. Loeb, and S. Holger Eichhorn pp 400–408 DOI: 10.1021/ja309558p Supporting Info |
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Rational Design of Highly Sensitive Fluorescence Probes for Protease and Glycosidase Based on Precisely Controlled Spirocyclization Masayo Sakabe, Daisuke Asanuma, Mako Kamiya, Ryu J. Iwatate, Kenjiro Hanaoka, Takuya Terai, Tetsuo Nagano, and Yasuteru Urano pp 409–414 DOI: 10.1021/ja309688m Supporting Info |
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Effect of Metal Ions on the Reactions of the Cumyloxyl Radical with Hydrogen Atom Donors. Fine Control on Hydrogen Abstraction Reactivity Determined by Lewis Acid–Base Interactions Michela Salamone, Livia Mangiacapra, Gino A. DiLabio, and Massimo Bietti pp 415–423 DOI: 10.1021/ja309579t Supporting Info |
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Variable Pathways for Oxygen Atom Insertion into Metal–Carbon Bonds: The Case of Cp*W(O)2(CH2SiMe3) Jiajun Mei, Kurtis M. Carsch, Cody R. Freitag, T. Brent Gunnoe, and Thomas R. Cundari pp 424–435 DOI: 10.1021/ja309755g Supporting Info |
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Highly Selective, Facile NO2 Reduction to NO at Cryogenic Temperatures on Hydrogen Precovered Gold Ming Pan, Hyung Chul Ham, Wen-Yueh Yu, Gyeong S. Hwang, and C. Buddie Mullins pp 436–442 DOI: 10.1021/ja3096575 Supporting Info |
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Mechanistic Investigation of the Palladium-Catalyzed Synthesis of Allylic Silanes and Boronates from Allylic Alcohols Johanna M. Larsson and Kálmán J. Szabó pp 443–455 DOI: 10.1021/ja309860h Supporting Info |
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Mechanical Bond-Induced Radical Stabilization Hao Li, Zhixue Zhu, Albert C. Fahrenbach, Brett M. Savoie, Chenfeng Ke, Jonathan C. Barnes, Juying Lei, Yan-Li Zhao, Laura M. Lilley, Tobin J. Marks, Mark A. Ratner, and J. Fraser Stoddart pp 456–467 DOI: 10.1021/ja310060n Supporting Info |
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Rhodium(III)-Catalyzed N-Nitroso-Directed C–H Olefination of Arenes. High-Yield, Versatile Coupling under Mild Conditions Baoqing Liu, Yang Fan, Yang Gao, Chao Sun, Cheng Xu, and Jin Zhu pp 468–473 DOI: 10.1021/ja3099245 Supporting Info |
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Mechanistic Studies into Amine-Mediated Electrophilic Arene Borylation and Its Application in MIDA Boronate Synthesis Viktor Bagutski, Alessandro Del Grosso, Josue Ayuso Carrillo, Ian A. Cade, Matthew D. Helm, James R. Lawson, Paul J. Singleton, Sophia A. Solomon, Tommaso Marcelli, and Michael J. Ingleson pp 474–487 DOI: 10.1021/ja3100963 Supporting Info |
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Labile Cu(I) Catalyst/Spectator Cu(II) Species in Copper-Catalyzed C–C Coupling Reaction: Operando IR, in Situ XANES/EXAFS Evidence and Kinetic Investigations Chuan He, Guanghui Zhang, Jie Ke, Heng Zhang, Jeffrey T. Miller, Arthur J. Kropf, and Aiwen Lei pp 488–493 DOI: 10.1021/ja310111p Supporting Info |
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The Carbon Electrode in Nonaqueous Li–O2 Cells Muhammed M. Ottakam Thotiyl, Stefan A. Freunberger, Zhangquan Peng, and Peter G. Bruce pp 494–500 DOI: 10.1021/ja310258x Supporting Info |
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Orthogonal Self-Assembly in Folding Block Copolymers Nobuhiko Hosono, Martijn A. J. Gillissen, Yuanchao Li, Sergei S. Sheiko, Anja R. A. Palmans, and E. W. Meijer pp 501–510 DOI: 10.1021/ja310422w Supporting Info |
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Reductive Cleavage of Nitrite to Form Terminal Uranium Mono-Oxo Complexes Andrew J. Lewis, Patrick J. Carroll, and Eric J. Schelter pp 511–518 DOI: 10.1021/ja311057y Supporting Info |
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Access to the Akuammiline Family of Alkaloids: Total Synthesis of (+)-Scholarisine A Gregory L. Adams, Patrick J. Carroll, and Amos B. Smith, III pp 519–528 DOI: 10.1021/ja3111626 Supporting Info |
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Spotlights on Recent JACS Publications pp 529–529 DOI: 10.1021/ja3127147 |
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High Stability, High Activity Pt/ITO Oxygen Reduction Electrocatalysts Ying Liu and William E. Mustain pp 530–533 DOI: 10.1021/ja307635r Supporting Info |
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Conversion of Fe–NH2 to Fe–N2 with release of NH3 John S. Anderson, Marc-Etienne Moret, and Jonas C. Peters pp 534–537 DOI: 10.1021/ja307714m Supporting Info |
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Real-Time Observation of Tight Au–Au Bond Formation and Relevant Coherent Motion upon Photoexcitation of [Au(CN)2–] Oligomers Munetaka Iwamura, Koichi Nozaki, Satoshi Takeuchi, and Tahei Tahara pp 538–541 DOI: 10.1021/ja310004z Supporting Info |
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d-Amino Acids Boost the Selectivity and Confer Supramolecular Hydrogels of a Nonsteroidal Anti-Inflammatory Drug (NSAID) Jiayang Li, Yi Kuang, Yuan Gao, Xuewen Du, Junfeng Shi, and Bing Xu pp 542–545 DOI: 10.1021/ja310019x Supporting Info |
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Control of Crystallinity and Porosity of Covalent Organic Frameworks by Managing Interlayer Interactions Based on Self-Complementary π-Electronic Force Xiong Chen, Matthew Addicoat, Stephan Irle, Atsushi Nagai, and Donglin Jiang pp 546–549 DOI: 10.1021/ja3100319 Supporting Info |
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A Model of Smart G-Quadruplex Ligand Romain Haudecoeur, Loic Stefan, Franck Denat, and David Monchaud pp 550–553 DOI: 10.1021/ja310056y Supporting Info |
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Molecular Marriage through Partner Preferences in Covalent Cage Formation and Cage-to-Cage Transformation Koushik Acharyya, Sandip Mukherjee, and Partha Sarathi Mukherjee pp 554–557 DOI: 10.1021/ja310083p Supporting Info |
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Fullerene/Sulfur-Bridged Annulene Cocrystals: Two-Dimensional Segregated Heterojunctions with Ambipolar Transport Properties and Photoresponsivity Jing Zhang, Jiahui Tan, Zhiying Ma, Wei Xu, Guangyao Zhao, Hua Geng, Chong’an Di, Wenping Hu, Zhigang Shuai, Kamaljit Singh, and Daoben Zhu pp 558–561 DOI: 10.1021/ja310098k Supporting Info |
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Fine-Tuning Pore Size by Shifting Coordination Sites of Ligands and Surface Polarization of Metal–Organic Frameworks To Sharply Enhance the Selectivity for CO2 Liting Du, Zhiyong Lu, Kaiyuan Zheng, Junyi Wang, Xin Zheng, Yi Pan, Xiaozeng You, and Junfeng Bai pp 562–565 DOI: 10.1021/ja309992a Supporting Info |
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Visualizing the Perturbation of Cellular Cyclic di-GMP Levels in Bacterial Cells Chun Loong Ho, Kavin Shi Jie Chong, Jamila Akosua Oppong, Mary Lay Cheng Chuah, Suet Mien Tan, and Zhao-Xun Liang pp 566–569 DOI: 10.1021/ja310497x Supporting Info |
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Ultrasensitive Electroanalytical Tool for Detecting, Sizing, and Evaluating the Catalytic Activity of Platinum Nanoparticles Radhika Dasari, Donald A. Robinson, and Keith J. Stevenson pp 570–573 DOI: 10.1021/ja310614x Supporting Info |
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Sequential Photo-oxidation of Methanol to Methyl Formate on TiO2(110) Katherine R. Phillips, Stephen C. Jensen, Martin Baron, Shao-Chun Li, and Cynthia M. Friend pp 574–577 DOI: 10.1021/ja3106797 Supporting Info |
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Superomniphobic Surfaces for Effective Chemical Shielding Shuaijun Pan, Arun K. Kota, Joseph M. Mabry, and Anish Tuteja pp 578–581 DOI: 10.1021/ja310517s Supporting Info |
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Total Synthesis of (±)-Bisabosqual A Christopher W. am Ende, Zhou Zhou, and Kathlyn A. Parker pp 582–585 DOI: 10.1021/ja3108577 Supporting Info |
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Fullerene Crystals with Bimodal Pore Architectures Consisting of Macropores and Mesopores Lok Kumar Shrestha, Yusuke Yamauchi, Jonathan P. Hill, Kun’ichi Miyazawa, and Katsuhiko Ariga pp 586–589 DOI: 10.1021/ja3108752 Supporting Info |
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Exploiting the Modularity of Ion-Paired Chiral Ligands for Palladium-Catalyzed Enantioselective Allylation of Benzofuran-2(3H)-ones Kohsuke Ohmatsu, Mitsunori Ito, Tomoatsu Kunieda, and Takashi Ooi pp 590–593 DOI: 10.1021/ja312125a Supporting Info |
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Diametric Stereocontrol in Dynamic Catalytic Reduction of Racemic Acyl Phosphonates: Divergence from α-Keto Ester Congeners Michael T. Corbett and Jeffrey S. Johnson pp 594–597 DOI: 10.1021/ja310980q Supporting Info |
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Thermochemistry of Zeolitic Imidazolate Frameworks of Varying Porosity James T. Hughes, Thomas D. Bennett, Anthony K. Cheetham, and Alexandra Navrotsky pp 598–601 DOI: 10.1021/ja311237m Supporting Info |
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Top-Down Preparation of Self-Supporting Supramolecular Polymeric Membranes Using Highly Selective Photocyclic Aromatization of Cis–Cisoid Helical Poly(phenylacetylene)s in the Membrane State Lijia Liu, Takeshi Namikoshi, Yu Zang, Toshiki Aoki, Shingo Hadano, Yunosuke Abe, Ikuya Wasuzu, Toyokazu Tsutsuba, Masahiro Teraguchi, and Takashi Kaneko pp 602–605 DOI: 10.1021/ja3113214 Supporting Info |
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Shape Control from Thermodynamic Growth Conditions: The Case of hcp Ruthenium Hourglass Nanocrystals John Watt, Chenlong Yu, Shery L. Y. Chang, Soshan Cheong, and Richard D. Tilley pp 606–609 DOI: 10.1021/ja311366k Supporting Info |
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X-ray Spectroscopic Observation of an Interstitial Carbide in NifEN-Bound FeMoco Precursor Kyle M. Lancaster, Yilin Hu, Uwe Bergmann, Markus W. Ribbe, and Serena DeBeer pp 610–612 DOI: 10.1021/ja309254g Supporting Info |
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Noncovalent Tailoring of the Binding Pocket of Self-Assembled Cages by Remote Bulky Ancillary Groups Yu Fang, Takashi Murase, Sota Sato, and Makoto Fujita pp 613–615 DOI: 10.1021/ja311373f Supporting Info |
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Palladium-Catalyzed C–H Activation/Cross-Coupling of Pyridine N-Oxides with Nonactivated Secondary Alkyl Bromides Bin Xiao, Zhao-Jing Liu, Lei Liu, and Yao Fu pp 616–619 DOI: 10.1021/ja3113752 Supporting Info |
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Iron(II) Bromide-Catalyzed Intramolecular C–H Bond Amination [1,2]-Shift Tandem Reactions of Aryl Azides Quyen Nguyen, Tuyen Nguyen, and Tom G. Driver pp 620–623 DOI: 10.1021/ja3113565 Supporting Info |
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Nickel-Catalyzed Carbon–Carbon Bond-Forming Reactions of Unactivated Tertiary Alkyl Halides: Suzuki Arylations Susan L. Zultanski and Gregory C. Fu pp 624–627 DOI: 10.1021/ja311669p Supporting Info |
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Catalytic Enantioselective Cyclization and C3-Fluorination of Polyenes Nikki A. Cochrane, Ha Nguyen, and Michel R. Gagne pp 628–631 DOI: 10.1021/ja3116795 Supporting Info |
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Bromine Radical-Mediated Sequential Radical Rearrangement and Addition Reaction of Alkylidenecyclopropanes Takashi Kippo, Kanako Hamaoka, and Ilhyong Ryu pp 632–635 DOI: 10.1021/ja311821h Supporting Info |
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A Tunable Class of Chiral Cp Ligands for Enantioselective Rhodium(III)-Catalyzed C–H Allylations of Benzamides Baihua Ye and Nicolai Cramer pp 636–639 DOI: 10.1021/ja311956k Supporting Info |
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Photoalignment Layers for Liquid Crystals from the Di-π-methane Rearrangement Jason R. Cox, Jeffrey H. Simpson, and Timothy M. Swager pp 640–643 DOI: 10.1021/ja312090p Supporting Info |
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Enantioselective Total Synthesis of Hyperforin Brian A. Sparling, David C. Moebius, and Matthew D. Shair pp 644–647 DOI: 10.1021/ja312150d Supporting Info |
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Bi-reforming of Methane from Any Source with Steam and Carbon Dioxide Exclusively to Metgas (CO–2H2) for Methanol and Hydrocarbon Synthesis George A. Olah, Alain Goeppert, Miklos Czaun, and G. K. Surya Prakash pp 648–650 DOI: 10.1021/ja311796n Supporting Info |
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First Observation of a Kondo Resonance for a Stable Neutral Pure Organic Radical, 1,3,5-Triphenyl-6-oxoverdazyl, Adsorbed on the Au(111) Surface Jie Liu, Hironari Isshiki, Keiichi Katoh, Takaumi Morita, Brian, K. Breedlove, Masahiro Yamashita, and Tadahiro Komeda pp 651–658 DOI: 10.1021/ja303510g Supporting Info |
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Regioselective Aliphatic Carbon–Carbon Bond Cleavage by a Model System of Relevance to Iron-Containing Acireductone Dioxygenase Caleb J. Allpress, Katarzyna Grubel, Ewa Szajna-Fuller, Atta M. Arif, and Lisa M. Berreau pp 659–668 DOI: 10.1021/ja3038189 Supporting Info |
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High-Affinity, Small-Molecule Peptidomimetic Inhibitors of MLL1/WDR5 Protein–Protein Interaction Hacer Karatas, Elizabeth C. Townsend, Fang Cao, Yong Chen, Denzil Bernard, Liu Liu, Ming Lei, Yali Dou, and Shaomeng Wang pp 669–682 DOI: 10.1021/ja306028q Supporting Info |
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Anionic Substituent Control of the Electronic Structure of Aromatic Nitrenes Nathan J. Rau, Emily A. Welles, and Paul G. Wenthold pp 683–690 DOI: 10.1021/ja306364z Supporting Info |
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Control of Intermolecular Bonds by Deposition Rates at Room Temperature: Hydrogen Bonds versus Metal Coordination in Trinitrile Monolayers Thomas Sirtl, Stefan Schlögl, Atena Rastgoo-Lahrood, Jelena Jelic, Subhadip Neogi, Michael Schmittel, Wolfgang M. Heckl, Karsten Reuter, and Markus Lackinger pp 691–695 DOI: 10.1021/ja306834a Supporting Info |
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Single-Step Rapid Assembly of DNA Origami Nanostructures for Addressable Nanoscale Bioreactors Yanming Fu, Dongdong Zeng, Jie Chao, Yanqiu Jin, Zhao Zhang, Huajie Liu, Di Li, Hongwei Ma, Qing Huang, Kurt V. Gothelf, and Chunhai Fan pp 696–702 DOI: 10.1021/ja3076692 Supporting Info |
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A One-Pot Three-Component Radiochemical Reaction for Rapid Assembly of 125I-Labeled Molecular Probes Ran Yan, Kerstin Sander, Eva Galante, Vineeth Rajkumar, Adam Badar, Mathew Robson, Ethaar El-Emir, Mark F. Lythgoe, R. Barbara Pedley, and Erik Årstad pp 703–709 DOI: 10.1021/ja307926g Supporting Info |
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Ionization state of l-Phenylalanine at the Air–Water Interface Elizabeth C. Griffith and Veronica Vaida pp 710–716 DOI: 10.1021/ja308089n Supporting Info |
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Calculation of Vibrational Shifts of Nitrile Probes in the Active Site of Ketosteroid Isomerase upon Ligand Binding Joshua P. Layfield and Sharon Hammes-Schiffer pp 717–725 DOI: 10.1021/ja3084384 Supporting Info |
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Phonon Scattering through a Local Anisotropic Structural Disorder in the Thermoelectric Solid Solution Cu2Zn1–xFexGeSe4 Wolfgang G. Zeier, Yanzhong Pei, Gregory Pomrehn, Tristan Day, Nicholas Heinz, Christophe P. Heinrich, G. Jeffrey Snyder, and Wolfgang Tremel pp 726–732 DOI: 10.1021/ja308627v Supporting Info |
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Mammalian Frataxin Controls Sulfur Production and Iron Entry during de Novo Fe4S4 Cluster Assembly Florent Colin, Alain Martelli, Martin Clémancey, Jean-Marc Latour, Serge Gambarelli, Laura Zeppieri, Catherine Birck, Adeline Page, Hélène Puccio, and Sandrine Ollagnier de Choudens pp 733–740 DOI: 10.1021/ja308736e Supporting Info |
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Development of a Robust Model System of FRET using Base Surrogates Tethering Fluorophores for Strict Control of Their Position and Orientation within DNA Duplex Tomohiro Kato, Hiromu Kashida, Hideo Kishida, Hiroyuki Yada, Hiroshi Okamoto, and Hiroyuki Asanuma pp 741–750 DOI: 10.1021/ja309279w Supporting Info |
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Nickel-Catalyzed Reductive Conjugate Addition to Enones via Allylnickel Intermediates Ruja Shrestha, Stephanie C. M. Dorn, and Daniel J. Weix pp 751–762 DOI: 10.1021/ja309176h Supporting Info |
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Lithium–Sulfur Battery Cathode Enabled by Lithium–Nitrile Interaction Juchen Guo, Zichao Yang, Yingchao Yu, Héctor D. Abruña, and Lynden A. Archer pp 763–767 DOI: 10.1021/ja309435f Supporting Info |
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Nanoscale Stabilization of New Phases in the PbTe–Sb2Te3 System: PbmSb2nTem+3n Nanocrystals Ronald B. Soriano, Indika U. Arachchige, Christos D. Malliakas, Jinsong Wu, and Mercouri G. Kanatzidis pp 768–774 DOI: 10.1021/ja309626q Supporting Info |
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High-Affinity Manganese Coordination by Human Calprotectin Is Calcium-Dependent and Requires the Histidine-Rich Site Formed at the Dimer Interface Joshua A. Hayden, Megan Brunjes Brophy, Lisa S. Cunden, and Elizabeth M. Nolan pp 775–787 DOI: 10.1021/ja3096416 Supporting Info |
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Mechanism-based Inhibition Reveals Transitions between Two Conformational States in the Action of Lysine 5,6-Aminomutase: A Combination of Electron Paramagnetic Resonance Spectroscopy, Electron Nuclear Double Resonance Spectroscopy, and Density Functional Theory Study Yung-Han Chen, Amarendra N. Maity, Perry A. Frey, and Shyue-Chu Ke pp 788–794 DOI: 10.1021/ja309603a Supporting Info |
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Assignment of Pterin Deaminase Activity to an Enzyme of Unknown Function Guided by Homology Modeling and Docking Hao Fan, Daniel S. Hitchcock, Ronald D. Seidel, II, Brandan Hillerich, Henry Lin, Steven C. Almo, Andrej Sali, Brian K. Shoichet, and Frank M. Raushel pp 795–803 DOI: 10.1021/ja309680b Supporting Info |
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Methane Reacts with Heteropolyacids Chemisorbed on Silica to Produce Acetic Acid under Soft Conditions Miao Sun, Edy Abou-Hamad, Aaron J. Rossini, Jizhe Zhang, Anne Lesage, Haibo Zhu, Jeremie Pelletier, Lyndon Emsley, Valerie Caps, and Jean-Marie Basset pp 804–810 DOI: 10.1021/ja309966j Supporting Info |
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Cationic, Neutral, and Anionic Allyl Magnesium Compounds: Unprecedented Ligand Conformations and Reactivity Toward Unsaturated Hydrocarbons Crispin Lichtenberg, Thomas P. Spaniol, Ilja Peckermann, Timothy P. Hanusa, and Jun Okuda pp 811–821 DOI: 10.1021/ja310112e Supporting Info |
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Interplay between Structure and Relaxations in Perfluorosulfonic Acid Proton Conducting Membranes Guinevere A. Giffin, Gregory M. Haugen, Steven J. Hamrock, and Vito Di Noto pp 822–834 DOI: 10.1021/ja3099799 Supporting Info |
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General Methodology of Using Oil-in-Water and Water-in-Oil Emulsions for Coiling Nanofilaments Liyong Chen, Suzhu Yu, Hong Wang, Jun Xu, Cuicui Liu, Wen Han Chong, and Hongyu Chen pp 835–843 DOI: 10.1021/ja310405d Supporting Info |
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Synthesis, Electronic Structure, Molecular Packing/Morphology Evolution, and Carrier Mobilities of Pure Oligo-/Poly(alkylthiophenes) Lei Zhang, Nicholas S. Colella, Feng Liu, Stephan Trahan, Jayanta K. Baral, H. Henning Winter, Stefan C. B. Mannsfeld, and Alejandro L. Briseno pp 844–854 DOI: 10.1021/ja3104796 Supporting Info |
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Fluorescence Coupling for Direct Imaging of Electrocatalytic Heterogeneity Joshua P. Guerrette, Stephen J. Percival, and Bo Zhang pp 855–861 DOI: 10.1021/ja310401b Supporting Info |
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Light-Harvesting and Ultrafast Energy Migration in Porphyrin-Based Metal–Organic Frameworks Ho-Jin Son, Shengye Jin, Sameer Patwardhan, Sander J. Wezenberg, Nak Cheon Jeong, Monica So, Christopher E. Wilmer, Amy A. Sarjeant, George C. Schatz, Randall Q. Snurr, Omar K. Farha, Gary P. Wiederrecht, and Joseph T. Hupp pp 862–869 DOI: 10.1021/ja310596a Supporting Info |
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Spherical Assemblies from π-Conjugated Alternating Copolymers: Toward Optoelectronic Colloidal Crystals Taeko Adachi, Liang Tong, Junpei Kuwabara, Takaki Kanbara, Akinori Saeki, Shu Seki, and Yohei Yamamoto pp 870–876 DOI: 10.1021/ja3106626 Supporting Info |
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Tandem-Layered Quantum Dot Solar Cells: Tuning the Photovoltaic Response with Luminescent Ternary Cadmium Chalcogenides Pralay K. Santra and Prashant V. Kamat pp 877–885 DOI: 10.1021/ja310737m Supporting Info |
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Universal Transients in Polymer and Ionic Transition Metal Complex Light-Emitting Electrochemical Cells Stephan van Reenen, Takeo Akatsuka, Daniel Tordera, Martijn Kemerink, and Henk J. Bolink pp 886–891 DOI: 10.1021/ja3107803 Supporting Info |
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Anion−π Interactions: Generality, Binding Strength, and Structure De-Xian Wang and Mei-Xiang Wang pp 892–897 DOI: 10.1021/ja310834w Supporting Info |
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Unveiling the Reactivity of Propargylic Hydroperoxides under Gold Catalysis Benito Alcaide, Pedro Almendros, M. Teresa Quirós, Ramón López, María I. Menéndez, and Aleksandra Sochacka-Ćwikła pp 898–905 DOI: 10.1021/ja3108966 Supporting Info |
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Generation of Oxygen Vacancies at a Au/TiO2 Perimeter Interface during CO Oxidation Detected by in Situ Electrical Conductance Measurement Yasushi Maeda, Yasuo Iizuka, and Masanori Kohyama pp 906–909 DOI: 10.1021/ja310999c Supporting Info |
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Y3MnAu5: Three Distinctive d-Metal Functions in an Intergrown Cluster Phase Saroj L. Samal, Abhishek Pandey, David C. Johnston, and John D. Corbett pp 910–917 DOI: 10.1021/ja3110208 Supporting Info |
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A Structural Diagnostics Diagram for Metallofullerenes Encapsulating Metal Carbides and Nitrides Sachiko Maki, Eiji Nishibori, Ikuya Terauchi, Masayuki Ishihara, Shinobu Aoyagi, Makoto Sakata, Masaki Takata, Hisashi Umemoto, Takashi Inoue, and Hisanori Shinohara pp 918–923 DOI: 10.1021/ja311070v Supporting Info |
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Synthesis of N3′-P5′-linked Phosphoramidate DNA by Nonenzymatic Template-Directed Primer Extension Shenglong Zhang, Na Zhang, J. Craig Blain, and Jack W. Szostak pp 924–932 DOI: 10.1021/ja311164j Supporting Info |
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Acid-Active Cell-Penetrating Peptides for in Vivo Tumor-Targeted Drug Delivery Erlei Jin, Bo Zhang, Xuanrong Sun, Zhuxian Zhou, Xinpeng Ma, Qihang Sun, Jianbin Tang, Youqing Shen, Edward Van Kirk, William J. Murdoch, and Maciej Radosz pp 933–940 DOI: 10.1021/ja311180x Supporting Info |
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Mechanistic Studies on the Metal-Free Activation of Dihydrogen by Antiaromatic Pentarylboroles Adrian Y. Houghton, Virve A. Karttunen, Cheng Fan, Warren E. Piers, and Heikki M. Tuononen pp 941–947 DOI: 10.1021/ja311842r Supporting Info |
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Correction to “Affinity-Based Probes Based on Type II Kinase Inhibitors” Pratistha Ranjitkar, B. Gayani K. Perera, Danielle L. Swaney, Sanjay B. Hari, Eric T. Larson, Ratika Krishnamurty, Ethan A. Merritt, Judit Villén, and Dustin J. Maly pp 948–948 DOI: 10.1021/ja3120967 |
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Spotlights on Recent JACS Publications pp 949–950 DOI: 10.1021/ja400349a |
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Poly(3-alkyltellurophene)s Are Solution-Processable Polyheterocycles Ashlee A. Jahnke, Brandon Djukic, Theresa M. McCormick, Ester Buchaca Domingo, Christoph Hellmann, Yunjeong Lee, and Dwight S. Seferos pp 951–954 DOI: 10.1021/ja309404j Supporting Info |
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Energy Transfer from Quantum Dots to Metal–Organic Frameworks for Enhanced Light Harvesting Shengye Jin, Ho-Jin Son, Omar K. Farha, Gary P. Wiederrecht, and Joseph T. Hupp pp 955–958 DOI: 10.1021/ja3097114 Supporting Info |
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Two [4Fe-4S] Clusters Containing Radical SAM Enzyme SkfB Catalyze Thioether Bond Formation during the Maturation of the Sporulation Killing Factor Leif Flühe, Olaf Burghaus, Beata M. Wieckowski, Tobias W. Giessen, Uwe Linne, and Mohamed A. Marahiel pp 959–962 DOI: 10.1021/ja310542g Supporting Info |
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Enhancing Proton Conduction in a Metal–Organic Framework by Isomorphous Ligand Replacement SiRim Kim, Karl W. Dawson, Benjamin S. Gelfand, Jared M. Taylor, and George K. H. Shimizu pp 963–966 DOI: 10.1021/ja310675x Supporting Info |
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Evidence for Metal–Ligand Cooperation in a Pd–PNF Pincer-Catalyzed Cross-Coupling Adam Scharf, Israel Goldberg, and Arkadi Vigalok pp 967–970 DOI: 10.1021/ja310782k Supporting Info |
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Simple Branched Sulfur–Olefins as Chiral Ligands for Rh-Catalyzed Asymmetric Arylation of Cyclic Ketimines: Highly Enantioselective Construction of Tetrasubstituted Carbon Stereocenters Hui Wang, Tao Jiang, and Ming-Hua Xu pp 971–974 DOI: 10.1021/ja3110818 Supporting Info |
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Anomalous High Ionic Conductivity of Nanoporous β-Li3PS4 Zengcai Liu, Wujun Fu, E. Andrew Payzant, Xiang Yu, Zili Wu, Nancy J. Dudney, Jim Kiggans, Kunlun Hong, Adam J. Rondinone, and Chengdu Liang pp 975–978 DOI: 10.1021/ja3110895 Supporting Info |
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Free Energy Relationships in the Electrical Double Layer over Single-Layer Graphene Jennifer L. Achtyl, Ivan V. Vlassiouk, Pasquale F. Fulvio, Shannon M. Mahurin, Sheng Dai, and Franz M. Geiger pp 979–981 DOI: 10.1021/ja3120899 Supporting Info |
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Reactant Vibrational Excitations Are More Effective than Translational Energy in Promoting an Early-Barrier Reaction F + H2O → HF + OH Jun Li, Bin Jiang, and Hua Guo pp 982–985 DOI: 10.1021/ja311159j Supporting Info |
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Origin of the Tunable Open-Circuit Voltage in Ternary Blend Bulk Heterojunction Organic Solar Cells Robert A. Street, Daniel Davies, Petr P. Khlyabich, Beate Burkhart, and Barry C. Thompson pp 986–989 DOI: 10.1021/ja3112143 |
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Anomalous Isosteric Enthalpy of Adsorption of Methane on Zeolite-Templated Carbon Nicholas P. Stadie, Maxwell Murialdo, Channing C. Ahn, and Brent Fultz pp 990–993 DOI: 10.1021/ja311415m Supporting Info |
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Iridium-Catalyzed Enantioselective Allylic Vinylation James Y. Hamilton, David Sarlah, and Erick M. Carreira pp 994–997 DOI: 10.1021/ja311422z Supporting Info |
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Organized Self-Assembly of Janus Micromotors with Hydrophobic Hemispheres Wei Gao, Allen Pei, Xiaomiao Feng, Camille Hennessy, and Joseph Wang pp 998–1001 DOI: 10.1021/ja311455k Supporting Info |
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Rate Dispersion in the Biexciton Decay of CdSe/ZnS Nanoparticles from Multiple Population-Period Transient Spectroscopy Kalyanasis Sahu, Haorui Wu, and Mark A. Berg pp 1002–1005 DOI: 10.1021/ja3112109 Supporting Info |
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Free-Radical-Mediated [2 + 2 + 1] Cycloaddition of Acetylenes, Amidines, and CO Leading to Five-Membered α,β-Unsaturated Lactams Takahide Fukuyama, Nao Nakashima, Takuma Okada, and Ilhyong Ryu pp 1006–1008 DOI: 10.1021/ja312654q Supporting Info |
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Single Molecule Dynamics at a Mechanically Controllable Break Junction in Solution at Room Temperature Tatsuya Konishi, Manabu Kiguchi, Mai Takase, Fumika Nagasawa, Hideki Nabika, Katsuyoshi Ikeda, Kohei Uosaki, Kosei Ueno, Hiroaki Misawa, and Kei Murakoshi pp 1009–1014 DOI: 10.1021/ja307821u Supporting Info |
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On the Formation and Properties of Interstrand DNA–DNA Cross-Links Forged by Reaction of an Abasic Site with the Opposing Guanine Residue of 5′-CAp Sequences in Duplex DNA Kevin M. Johnson, Nathan E. Price, Jin Wang, Mostafa I. Fekry, Sanjay Dutta, Derrick R. Seiner, Yinsheng Wang, and Kent S. Gates pp 1015–1025 DOI: 10.1021/ja308119q Supporting Info |
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Concepts for Stereoselective Acrylate Insertion Boris Neuwald, Lucia Caporaso, Luigi Cavallo, and Stefan Mecking pp 1026–1036 DOI: 10.1021/ja3101787 Supporting Info |
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The Single Crystal X-ray Structure of β-Hematin DMSO Solvate Grown in the Presence of Chloroquine, a β-Hematin Growth-Rate Inhibitor Johandie Gildenhuys, Tanya le Roex, Timothy J. Egan, and Katherine A. de Villiers pp 1037–1047 DOI: 10.1021/ja308741e Supporting Info |
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Profiling Genome-Wide Chromatin Methylation with Engineered Posttranslation Apparatus within Living Cells Rui Wang, Kabirul Islam, Ying Liu, Weihong Zheng, Haiping Tang, Nathalie Lailler, Gil Blum, Haiteng Deng, and Minkui Luo pp 1048–1056 DOI: 10.1021/ja309412s Supporting Info |
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Using TiO2 as a Conductive Protective Layer for Photocathodic H2 Evolution Brian Seger, Thomas Pedersen, Anders B. Laursen, Peter C. K. Vesborg, Ole Hansen, and Ib Chorkendorff pp 1057–1064 DOI: 10.1021/ja309523t Supporting Info |
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An Ionic Liquid Dependent Mechanism for Base Catalyzed β-Elimination Reactions from QM/MM Simulations Caley Allen, Somisetti V. Sambasivarao, and Orlando Acevedo pp 1065–1072 DOI: 10.1021/ja3098614 Supporting Info |
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Oxygen Atom Transfer and Oxidative Water Incorporation in Cuboidal Mn3MOn Complexes Based on Synthetic, Isotopic Labeling, and Computational Studies Jacob S. Kanady, Jose L. Mendoza-Cortes, Emily Y. Tsui, Robert J. Nielsen, William A. Goddard, III, and Theodor Agapie pp 1073–1082 DOI: 10.1021/ja310022p Supporting Info |
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Impact of Metal and Anion Substitutions on the Hydrogen Storage Properties of M-BTT Metal–Organic Frameworks Kenji Sumida, David Stück, Lorenzo Mino, Jeng-Da Chai, Eric D. Bloch, Olena Zavorotynska, Leslie J. Murray, Mircea Dincă, Sachin Chavan, Silvia Bordiga, Martin Head-Gordon, and Jeffrey R. Long pp 1083–1091 DOI: 10.1021/ja310173e Supporting Info |
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Observation of a Distinct Surface Molecular Orientation in Films of a High Mobility Conjugated Polymer Torben Schuettfort, Lars Thomsen, and Christopher R. McNeill pp 1092–1101 DOI: 10.1021/ja310240q Supporting Info |
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Six-Color Time-Resolved Förster Resonance Energy Transfer for Ultrasensitive Multiplexed Biosensing Daniel Geißler, Stefan Stufler, Hans-Gerd Löhmannsröben, and Niko Hildebrandt pp 1102–1109 DOI: 10.1021/ja310317n Supporting Info |
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Gas-Phase Azide Functionalization of Carbon Eric D. Stenehjem, Vadim R. Ziatdinov, T. Daniel P. Stack, and Christopher E. D. Chidsey pp 1110–1116 DOI: 10.1021/ja310410d |
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Direct and Real-Time Observation of Rotary Movement of a DNA Nanomechanical Device Arivazhagan Rajendran, Masayuki Endo, Kumi Hidaka, and Hiroshi Sugiyama pp 1117–1123 DOI: 10.1021/ja310454k Supporting Info |
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Iron L-Edge X-ray Absorption Spectroscopy of Oxy-Picket Fence Porphyrin: Experimental Insight into Fe–O2 Bonding Samuel A. Wilson, Thomas Kroll, Richard A. Decreau, Rosalie K. Hocking, Marcus Lundberg, Britt Hedman, Keith O. Hodgson, and Edward I. Solomon pp 1124–1136 DOI: 10.1021/ja3103583 Supporting Info |
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Dithieno[3,2-c:2′,3′-e]-2,7-diketophosphepin: A Unique Building Block for Multifunctional π-Conjugated Materials Xiaoming He, Javier Borau-Garcia, Alva Y. Y. Woo, Simon Trudel, and Thomas Baumgartner pp 1137–1147 DOI: 10.1021/ja310680x Supporting Info |
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Enhanced Brightness Emission-Tuned Nanoparticles from Heterodifunctional Polyfluorene Building Blocks Christoph S. Fischer, Moritz C. Baier, and Stefan Mecking pp 1148–1154 DOI: 10.1021/ja311497e Supporting Info |
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Biosynthetic Multitasking Facilitates Thalassospiramide Structural Diversity in Marine Bacteria Avena C. Ross, Ying Xu, Liang Lu, Roland D. Kersten, Zongze Shao, Abdulaziz M. Al-Suwailem, Pieter C. Dorrestein, Pei-Yuan Qian, and Bradley S. Moore pp 1155–1162 DOI: 10.1021/ja3119674 Supporting Info |
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Correction to A Biomimetic Route for Construction of the [4 + 2] and [3 + 2] Core Skeletons of Dimeric Pyrrole–Imidazole Alkaloids and Asymmetric Synthesis of Ageliferins Xiao Wang, Xiaolei Wang, Xianghui Tan, Jianming Lu, Kevin W. Cormier, Zhiqiang Ma, and Chuo Chen pp 1163–1163 DOI: 10.1021/ja311681x |
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Spotlights on Recent JACS Publications pp 1165–1166 DOI: 10.1021/ja400709t |
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The Li-Ion Rechargeable Battery: A Perspective John B. Goodenough and Kyu-Sung Park pp 1167–1176 DOI: 10.1021/ja3091438 |
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Protein Structure in the Gas Phase: The Influence of Side-Chain Microsolvation Stephan Warnke, Gert von Helden, and Kevin Pagel pp 1177–1180 DOI: 10.1021/ja308528d Supporting Info |
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In-Situ Crystallization Route to Nanorod-Aggregated Functional ZSM-5 Microspheres Bin Li, Bo Sun, Xufang Qian, Wei Li, Zhangxiong Wu, Zhenkun Sun, Minghua Qiao, Mikel Duke, and Dongyuan Zhao pp 1181–1184 DOI: 10.1021/ja309194z Supporting Info |
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Steric Pressure between Membrane-Bound Proteins Opposes Lipid Phase Separation Christine S. Scheve, Paul A. Gonzales, Noor Momin, and Jeanne C. Stachowiak pp 1185–1188 DOI: 10.1021/ja3099867 Supporting Info |
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Spatial Organization of Lipid Phases in Micropatterned Polymer-Supported Membranes Friedrich Roder, Oliver Birkholz, Oliver Beutel, Dirk Paterok, and Jacob Piehler pp 1189–1192 DOI: 10.1021/ja310186g Supporting Info |
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A Water-Stable Metal–Organic Framework with Highly Acidic Pores for Proton-Conducting Applications Jared M. Taylor, Karl W. Dawson, and George K. H. Shimizu pp 1193–1196 DOI: 10.1021/ja310435e Supporting Info |
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Phosphine Quenching of Cyanine Dyes as a Versatile Tool for Fluorescence Microscopy Joshua C. Vaughan, Graham T. Dempsey, Eileen Sun, and Xiaowei Zhuang pp 1197–1200 DOI: 10.1021/ja3105279 Supporting Info |
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Can Boron and Nitrogen Co-doping Improve Oxygen Reduction Reaction Activity of Carbon Nanotubes? Yu Zhao, Lijun Yang, Sheng Chen, Xizhang Wang, Yanwen Ma, Qiang Wu, Yufei Jiang, Weijin Qian, and Zheng Hu pp 1201–1204 DOI: 10.1021/ja310566z Supporting Info |
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The Energetic Difference between Synthesis of Correct and Incorrect Base Pairs Accounts for Highly Accurate DNA Replication Andrew C. Olson, Jennifer N. Patro, Milan Urban, and Robert D. Kuchta pp 1205–1208 DOI: 10.1021/ja309866m Supporting Info |
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Synthesis of (−)-Neothiobinupharidine Daniel J. Jansen and Ryan A. Shenvi pp 1209–1212 DOI: 10.1021/ja310778t Supporting Info |
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Single-Layer Single-Crystalline SnSe Nanosheets Lun Li, Zhong Chen, Ying Hu, Xuewen Wang, Ting Zhang, Wei Chen, and Qiangbin Wang pp 1213–1216 DOI: 10.1021/ja3108017 Supporting Info |
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Mechanism of Hydrogenolysis of an Iridium–Methyl Bond: Evidence for a Methane Complex Intermediate Jesús Campos, Sabuj Kundu, Dale R. Pahls, Maurice Brookhart, Ernesto Carmona, and Thomas R. Cundari pp 1217–1220 DOI: 10.1021/ja310982v Supporting Info |
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Ni-Catalyzed Direct Carboxylation of Benzyl Halides with CO2 Thierry León, Arkaitz Correa, and Ruben Martin pp 1221–1224 DOI: 10.1021/ja311045f Supporting Info |
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Iridium-Catalyzed Hydrosilylative Reduction of Glucose to Hexane(s) Matthew P. McLaughlin, Laura L. Adduci, Jennifer J. Becker, and Michel R. Gagné pp 1225–1227 DOI: 10.1021/ja3110494 Supporting Info |
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A Powerful Aluminum Catalyst for the Synthesis of Highly Functional Organic Carbonates Christopher J. Whiteoak, Nicola Kielland, Victor Laserna, Eduardo C. Escudero-Adán, Eddy Martin, and Arjan W. Kleij pp 1228–1231 DOI: 10.1021/ja311053h Supporting Info |
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C2-Symmetric Cyclic Selenium-Catalyzed Enantioselective Bromoaminocyclization Feng Chen, Chong Kiat Tan, and Ying-Yeung Yeung pp 1232–1235 DOI: 10.1021/ja311202e Supporting Info |
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Pd(II)-Catalyzed Enantioselective C–H Activation/C–O Bond Formation: Synthesis of Chiral Benzofuranones Xiu-Fen Cheng, Yan Li, Yi-Ming Su, Feng Yin, Jian-Yong Wang, Jie Sheng, Harit U. Vora, Xi-Sheng Wang, and Jin-Quan Yu pp 1236–1239 DOI: 10.1021/ja311259x Supporting Info |
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Application of N-Halogeno-N-sodiobenzenesulfonamide Reagents to the Selective Detection of 5-Methylcytosine in DNA Sequences Tianlu Wang, Tingting Hong, Tun Tang, Qianqian Zhai, Xiwen Xing, Wuxiang Mao, Xiaolong Zheng, Liang Xu, Jinjun Wu, Xiaocheng Weng, Shaoru Wang, Tian Tian, Bifeng Yuan, Bing Huang, Lin Zhuang, and Xiang Zhou pp 1240–1243 DOI: 10.1021/ja311229n Supporting Info |
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Highly Selective Catalyst-Dependent Competitive 1,2-C→C, -O→C, and -N→C Migrations from β-Methylene-β-silyloxy-β-amido-α-diazoacetates Xichen Xu, Yu Qian, Peter Y. Zavalij, and Michael P. Doyle pp 1244–1247 DOI: 10.1021/ja311392m Supporting Info |
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C(sp3)–F Bond Activation of CF3-Substituted Anilines with Catalytically Generated Silicon Cations: Spectroscopic Evidence for a Hydride-Bridged Ru–S Dimer in the Catalytic Cycle Timo Stahl, Hendrik F. T. Klare, and Martin Oestreich pp 1248–1251 DOI: 10.1021/ja311398j Supporting Info |
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MOFs Under Pressure: The Reversible Compression of a Single Crystal Kevin J. Gagnon, Christine M. Beavers, and Abraham Clearfield pp 1252–1255 DOI: 10.1021/ja311613p Supporting Info |
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Growing Crystalline Chalcogenidoarsenates in Surfactants: From Zero-Dimensional Cluster to Three-Dimensional Framework Wei-Wei Xiong, Eashwer Umesh Athresh, Yu Ting Ng, Junfeng Ding, Tom Wu, and Qichun Zhang pp 1256–1259 DOI: 10.1021/ja3116179 Supporting Info |
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Reconstitution of Biosynthetic Machinery for Indole-Diterpene Paxilline in Aspergillus oryzae Koichi Tagami, Chengwei Liu, Atsushi Minami, Motoyoshi Noike, Tetsuya Isaka, Shuhei Fueki, Yoshihiro Shichijo, Hiroaki Toshima, Katsuya Gomi, Tohru Dairi, and Hideaki Oikawa pp 1260–1263 DOI: 10.1021/ja3116636 Supporting Info |
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Mn-Catalyzed Aromatic C–H Alkenylation with Terminal Alkynes Bingwei Zhou, Hui Chen, and Congyang Wang pp 1264–1267 DOI: 10.1021/ja311689k Supporting Info |
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Chiral Anion Phase-Transfer Catalysis Applied to the Direct Enantioselective Fluorinative Dearomatization of Phenols Robert J. Phipps and F. Dean Toste pp 1268–1271 DOI: 10.1021/ja311798q Supporting Info |
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A New Nanobiocatalytic System Based on Allosteric Effect with Dramatically Enhanced Enzymatic Performance Liang-Bing Wang, You-Cheng Wang, Rong He, Awei Zhuang, Xiaoping Wang, Jie Zeng, and J. G. Hou pp 1272–1275 DOI: 10.1021/ja3120136 Supporting Info |
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Highly Active Ruthenium Metathesis Catalysts Exhibiting Unprecedented Activity and Z-Selectivity Lauren E. Rosebrugh, Myles B. Herbert, Vanessa M. Marx, Benjamin K. Keitz, and Robert H. Grubbs pp 1276–1279 DOI: 10.1021/ja311916m Supporting Info |
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Transition between Collective Behaviors of Micromotors in Response to Different Stimuli Wentao Duan, Ran Liu, and Ayusman Sen pp 1280–1283 DOI: 10.1021/ja3120357 Supporting Info |
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Cation Modules as Building Blocks Forming Supramolecular Assemblies with Planar Receptor–Anion Complexes Bin Dong, Tsuneaki Sakurai, Yoshihito Honsho, Shu Seki, and Hiromitsu Maeda pp 1284–1287 DOI: 10.1021/ja312214a Supporting Info |
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Energetic Basis of Uncoupling Folding from Binding for an Intrinsically Disordered Protein Igor Drobnak, Natalie De Jonge, Sarah Haesaerts, Gorazd Vesnaver, Remy Loris, and Jurij Lah pp 1288–1294 DOI: 10.1021/ja305081b Supporting Info |
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Unraveling the Pathway of Gold(I)-Catalyzed Olefin Hydrogenation: An Ionic Mechanism Aleix Comas-Vives and Gregori Ujaque pp 1295–1305 DOI: 10.1021/ja305630z Supporting Info |
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Quantum-Mechanical Analysis of the Energetic Contributions to π Stacking in Nucleic Acids versus Rise, Twist, and Slide Trent M. Parker, Edward G. Hohenstein, Robert M. Parrish, Nicholas V. Hud, and C. David Sherrill pp 1306–1316 DOI: 10.1021/ja3063309 Supporting Info |
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The Backbone Dynamics of the Amyloid Precursor Protein Transmembrane Helix Provides a Rationale for the Sequential Cleavage Mechanism of γ-Secretase Oxana Pester, Paul J. Barrett, Daniel Hornburg, Philipp Hornburg, Rasmus Pröbstle, Simon Widmaier, Christoph Kutzner, Milena Dürrbaum, Aphrodite Kapurniotu, Charles R. Sanders, Christina Scharnagl, and Dieter Langosch pp 1317–1329 DOI: 10.1021/ja3112093 Supporting Info |
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Fluoroketone Inhibition of Ca2+-Independent Phospholipase A2 through Binding Pocket Association Defined by Hydrogen/Deuterium Exchange and Molecular Dynamics Yuan-Hao Hsu, Denis Bucher, Jian Cao, Sheng Li, Sheng-Wei Yang, George Kokotos, Virgil L. Woods, Jr, J. Andrew McCammon, and Edward A. Dennis pp 1330–1337 DOI: 10.1021/ja306490g |
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A General Mechanism for the Copper- and Silver-Catalyzed Olefin Aziridination Reactions: Concomitant Involvement of the Singlet and Triplet Pathways Lourdes Maestre, W. M. C. Sameera, M. Mar Díaz-Requejo, Feliu Maseras, and Pedro J. Pérez pp 1338–1348 DOI: 10.1021/ja307229e Supporting Info |
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III–V Nanocrystals Capped with Molecular Metal Chalcogenide Ligands: High Electron Mobility and Ambipolar Photoresponse Wenyong Liu, Jong-Soo Lee, and Dmitri V. Talapin pp 1349–1357 DOI: 10.1021/ja308200f Supporting Info |
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Multidimensional Magic Angle Spinning NMR Spectroscopy for Site-Resolved Measurement of Proton Chemical Shift Anisotropy in Biological Solids Guangjin Hou, Sivakumar Paramasivam, Si Yan, Tatyana Polenova, and Alexander J. Vega pp 1358–1368 DOI: 10.1021/ja3084972 Supporting Info |
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Small-molecule Binding to the DNA Minor Groove Is Mediated by a Conserved Water Cluster DengGuo Wei, W David Wilson, and Stephen Neidle pp 1369–1377 DOI: 10.1021/ja308952y |
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Reversible and Cyclical Transformations between Solid and Hollow Nanostructures in Confined Reactions of Manganese Oxide and Silica within Nanosized Spheres Tae-Lin Ha, Jin Goo Kim, Soo Min Kim, and In Su Lee pp 1378–1385 DOI: 10.1021/ja309142j Supporting Info |
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Large-Scale Production of Edge-Selectively Functionalized Graphene Nanoplatelets via Ball Milling and Their Use as Metal-Free Electrocatalysts for Oxygen Reduction Reaction In-Yup Jeon, Hyun-Jung Choi, Sun-Min Jung, Jeong-Min Seo, Min-Jung Kim, Liming Dai, and Jong-Beom Baek pp 1386–1393 DOI: 10.1021/ja3091643 Supporting Info |
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Besting Vitamin E: Sidechain Substitution is Key to the Reactivity of Naphthyridinol Antioxidants in Lipid Bilayers Bo Li, Jitendra R. Harjani, Nicholas S. Cormier, Hasam Madarati, Jeffrey Atkinson, Gonzalo Cosa, and Derek A. Pratt pp 1394–1405 DOI: 10.1021/ja309153x Supporting Info |
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Enzyme Molecules as Nanomotors Samudra Sengupta, Krishna K. Dey, Hari S. Muddana, Tristan Tabouillot, Michael E. Ibele, Peter J. Butler, and Ayusman Sen pp 1406–1414 DOI: 10.1021/ja3091615 Supporting Info |
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Folding and Binding of an Intrinsically Disordered Protein: Fast, but Not ‘Diffusion-Limited’ Joseph M. Rogers, Annette Steward, and Jane Clarke pp 1415–1422 DOI: 10.1021/ja309527h Supporting Info |
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Living Unimodal Growth of Polyion Complex Vesicles via Two-Dimensional Supramolecular Polymerization Yasutaka Anraku, Akihiro Kishimura, Yuichi Yamasaki, and Kazunori Kataoka pp 1423–1429 DOI: 10.1021/ja3096587 Supporting Info |
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Synthesis and Characterization of Quarteranthene: Elucidating the Characteristics of the Edge State of Graphene Nanoribbons at the Molecular Level Akihito Konishi, Yasukazu Hirao, Kouzou Matsumoto, Hiroyuki Kurata, Ryohei Kishi, Yasuteru Shigeta, Masayoshi Nakano, Kazuya Tokunaga, Kenji Kamada, and Takashi Kubo pp 1430–1437 DOI: 10.1021/ja309599m Supporting Info |
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Nanoparticle Adhesion to the Cell Membrane and Its Effect on Nanoparticle Uptake Efficiency Anna Lesniak, Anna Salvati, Maria J. Santos-Martinez, Marek W. Radomski, Kenneth A. Dawson, and Christoffer Åberg pp 1438–1444 DOI: 10.1021/ja309812z Supporting Info |
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Interaction of Cisplatin with Adenine and Guanine: A Combined IRMPD, MS/MS, and Theoretical Study Barbara Chiavarino, Maria Elisa Crestoni, Simonetta Fornarini, Debora Scuderi, and Jean-Yves Salpin pp 1445–1455 DOI: 10.1021/ja309857d Supporting Info |
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Mechanism and Origins of Ligand-Controlled Selectivities in [Ni(NHC)]-Catalyzed Intramolecular (5 + 2) Cycloadditions and Homo-Ene Reactions: A Theoretical Study Xin Hong, Peng Liu, and K. N. Houk pp 1456–1462 DOI: 10.1021/ja309873z Supporting Info |
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Stereoselective Rh2(S-IBAZ)4-Catalyzed Cyclopropanation of Alkenes, Alkynes, and Allenes: Asymmetric Synthesis of Diacceptor Cyclopropylphosphonates and Alkylidenecyclopropanes Vincent N. G. Lindsay, Dominic Fiset, Philipp J. Gritsch, Soula Azzi, and André B. Charette pp 1463–1470 DOI: 10.1021/ja3099728 Supporting Info |
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Mechanism and the Origins of Stereospecificity in Copper-Catalyzed Ring Expansion of Vinyl Oxiranes: A Traceless Dual Transition-Metal-Mediated Process Thomas J. L. Mustard, Daniel J. Mack, Jon T. Njardarson, and Paul Ha-Yeon Cheong pp 1471–1475 DOI: 10.1021/ja310065z Supporting Info |
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Direct STM Elucidation of the Effects of Atomic-Level Structure on Pt(111) Electrodes for Dissolved CO Oxidation Junji Inukai, Donald A. Tryk, Takahiro Abe, Mitsuru Wakisaka, Hiroyuki Uchida, and Masahiro Watanabe pp 1476–1490 DOI: 10.1021/ja309886p Supporting Info |
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Single Molecule Characterization of the Interactions between Amyloid-β Peptides and the Membranes of Hippocampal Cells Priyanka Narayan, Kristina A. Ganzinger, James McColl, Laura Weimann, Sarah Meehan, Seema Qamar, John A. Carver, Mark R. Wilson, Peter St. George-Hyslop, Christopher M. Dobson, and David Klenerman pp 1491–1498 DOI: 10.1021/ja3103567 Supporting Info |
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Engineering Catalytic Contacts and Thermal Stability: Gold/Iron Oxide Binary Nanocrystal Superlattices for CO Oxidation Yijin Kang, Xingchen Ye, Jun Chen, Liang Qi, Rosa E. Diaz, Vicky Doan-Nguyen, Guozhong Xing, Cherie R. Kagan, Ju Li, Raymond J. Gorte, Eric A. Stach, and Christopher B. Murray pp 1499–1505 DOI: 10.1021/ja310427u Supporting Info |
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Heterogeneous Ceria Catalyst with Water-Tolerant Lewis Acidic Sites for One-Pot Synthesis of 1,3-Diols via Prins Condensation and Hydrolysis Reactions Yehong Wang, Feng Wang, Qi Song, Qin Xin, Shutao Xu, and Jie Xu pp 1506–1515 DOI: 10.1021/ja310498c Supporting Info |
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A New Strategy for Intracellular Delivery of Enzyme Using Mesoporous Silica Nanoparticles: Superoxide Dismutase Yi-Ping Chen, Chien-Tsu Chen, Yann Hung, Chih-Ming Chou, Tsang-Pai Liu, Ming-Ren Liang, Chao-Tsen Chen, and Chung-Yuan Mou pp 1516–1523 DOI: 10.1021/ja3105208 Supporting Info |
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Two-Dimensional Mesoporous Carbon Nanosheets and Their Derived Graphene Nanosheets: Synthesis and Efficient Lithium Ion Storage Yin Fang, Yingying Lv, Renchao Che, Haoyu Wu, Xuehua Zhang, Dong Gu, Gengfeng Zheng, and Dongyuan Zhao pp 1524–1530 DOI: 10.1021/ja310849c Supporting Info |
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Confounding the Paradigm: Peculiarities of Amyloid Fibril Nucleation Dimo Kashchiev, Raffaela Cabriolu, and Stefan Auer pp 1531–1539 DOI: 10.1021/ja311228d |
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Spiroketal Formation and Modification in Avermectin Biosynthesis Involves a Dual Activity of AveC Peng Sun, Qunfei Zhao, Futao Yu, Hua Zhang, Zhuhua Wu, Yinyan Wang, Yan Wang, Qinglin Zhang, and Wen Liu pp 1540–1548 DOI: 10.1021/ja311339u Supporting Info |
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Mechanistic Investigation of Oxidative Mannich Reaction with tert-Butyl Hydroperoxide. The Role of Transition Metal Salt Maxim O. Ratnikov and Michael P. Doyle pp 1549–1557 DOI: 10.1021/ja3113559 Supporting Info |
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Moderating Strain without Sacrificing Reactivity: Design of Fast and Tunable Noncatalyzed Alkyne–Azide Cycloadditions via Stereoelectronically Controlled Transition State Stabilization Brian Gold, Gregory B. Dudley, and Igor V. Alabugin pp 1558–1569 DOI: 10.1021/ja3114196 Supporting Info |
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Viologen-Mediated Assembly of and Sensing with Carboxylatopillar[5]arene-Modified Gold Nanoparticles Hui Li, Dai-Xiong Chen, Yu-Long Sun, Yue Bing Zheng, Li-Li Tan, Paul S. Weiss, and Ying-Wei Yang pp 1570–1576 DOI: 10.1021/ja3115168 Supporting Info |
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Bare-Minimum Fluorous Mixture Synthesis of a Stereoisomer Library of 4,8,12-Trimethylnonadecanols and Predictions of NMR Spectra of Saturated Oligoisoprenoid Stereoisomers Edmund A.-H. Yeh, Eveline Kumli, Krishnan Damodaran, and Dennis P. Curran pp 1577–1584 DOI: 10.1021/ja311606u Supporting Info |
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Simplifying Nickel(0) Catalysis: An Air-Stable Nickel Precatalyst for the Internally Selective Benzylation of Terminal Alkenes Eric A. Standley and Timothy F. Jamison pp 1585–1592 DOI: 10.1021/ja3116718 Supporting Info |
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I-Motif-Programmed Functionalization of DNA Nanocircles Tao Li and Michael Famulok pp 1593–1599 DOI: 10.1021/ja3118224 Supporting Info |
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A Pd(0)-Mediated Indole (Macro)cyclization Reaction Steven P. Breazzano, Yam B. Poudel, and Dale L. Boger pp 1600–1606 DOI: 10.1021/ja3121394 Supporting Info |
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Understanding the High Photocatalytic Activity of (B, Ag)-Codoped TiO2 under Solar-Light Irradiation with XPS, Solid-State NMR, and DFT Calculations Ningdong Feng, Qiang Wang, Anmin Zheng, Zhengfeng Zhang, Jie Fan, Shang-Bin Liu, Jean-Paul Amoureux, and Feng Deng pp 1607–1616 DOI: 10.1021/ja312205c Supporting Info |
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Transforming Thymidine into a Magnetic Resonance Imaging Probe for Monitoring Gene Expression Amnon Bar-Shir, Guanshu Liu, Yajie Liang, Nirbhay N. Yadav, Michael T. McMahon, Piotr Walczak, Sridhar Nimmagadda, Martin G. Pomper, Keri A. Tallman, Marc M. Greenberg, Peter C.M. van Zijl, Jeff W.M. Bulte, and Assaf A. Gilad pp 1617–1624 DOI: 10.1021/ja312353e Supporting Info |
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Correction to How Lipid Unsaturation, Peroxyl Radical Partitioning, and Chromanol Lipophilic Tail Affect the Antioxidant Activity of α-Tocopherol: Direct Visualization via High-Throughput Fluorescence Studies Conducted with Fluorogenic α-Tocopherol Analogues Katerina Krumova, Sayuri Friedland, and Gonzalo Cosa pp 1625–1625 DOI: 10.1021/ja400143q |
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Benzimidazole and Related Ligands for Cu-Catalyzed Azide–Alkyne Cycloaddition Valentin O. Rodionov, Stanislav I. Presolski, Sean Gardinier, Yeon-Hee Lim, and M. G. Finn pp 1626–1626 DOI: 10.1021/ja400176a |
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Spotlights on Recent JACS Publications pp 1627–1628 DOI: 10.1021/ja400789q |
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The Revolution and Evolution of Shotgun Proteomics for Large-Scale Proteome Analysis John R. Yates, III pp 1629–1640 DOI: 10.1021/ja3094313 |
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Dynamic Nuclear Polarization of Sedimented Solutes Enrico Ravera, Björn Corzilius, Vladimir K. Michaelis, Camilla Rosa, Robert G. Griffin, Claudio Luchinat, and Ivano Bertini pp 1641–1644 DOI: 10.1021/ja312553b Supporting Info |
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Multiplexed Protease Activity Assay for Low-Volume Clinical Samples Using Droplet-Based Microfluidics and Its Application to Endometriosis Chia-Hung Chen, Miles A. Miller, Aniruddh Sarkar, Michael T. Beste, Keith B. Isaacson, Douglas A. Lauffenburger, Linda G. Griffith, and Jongyoon Han pp 1645–1648 DOI: 10.1021/ja307866z Supporting Info |
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Nanoscale Coating of LiMO2 (M = Ni, Co, Mn) Nanobelts with Li+-Conductive Li2TiO3: Toward Better Rate Capabilities for Li-Ion Batteries Jun Lu, Qing Peng, Weiyang Wang, Caiyun Nan, Lihong Li, and Yadong Li pp 1649–1652 DOI: 10.1021/ja308717z Supporting Info |
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On/Off Photoswitching in a Cyanide-Bridged {Fe2Co2} Magnetic Molecular Square Abhishake Mondal, Yanling Li, Mannan Seuleiman, Miguel Julve, Loïc Toupet, Marylise Buron-Le Cointe, and Rodrigue Lescouëzec pp 1653–1656 DOI: 10.1021/ja3087467 Supporting Info |
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Label-Free SERS Monitoring of Chemical Reactions Catalyzed by Small Gold Nanoparticles Using 3D Plasmonic Superstructures Wei Xie, Bernd Walkenfort, and Sebastian Schlücker pp 1657–1660 DOI: 10.1021/ja309074a Supporting Info |
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Real-Time Detection of Telomerase Activity Using the Exponential Isothermal Amplification of Telomere Repeat Assay Leilei Tian and Yossi Weizmann pp 1661–1664 DOI: 10.1021/ja309198j Supporting Info |
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Induced Axial Chirality in Biocatalytic Asymmetric Ketone Reduction Rubén Agudo, Gheorghe-Doru Roiban, and Manfred T. Reetz pp 1665–1668 DOI: 10.1021/ja3092517 Supporting Info |
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Small-Molecule Inducer of β Cell Proliferation Identified by High-Throughput Screening Weijun Shen, Matthew S. Tremblay, Vishal A. Deshmukh, Weidong Wang, Christophe M. Filippi, George Harb, You-qing Zhang, Anwesh Kamireddy, Janine E Baaten, Qihui Jin, Tom Wu, Jonathan G. Swoboda, Charles Y. Cho, Jing Li, Bryan A. Laffitte, Peter McNamara, Richard Glynne, Xu Wu, Ann E. Herman, and Peter G. Schultz pp 1669–1672 DOI: 10.1021/ja309304m Supporting Info |
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Lewis Acid-Promoted Ketene–Alkene [2 + 2] Cycloadditions Christopher M. Rasik and M. Kevin Brown pp 1673–1676 DOI: 10.1021/ja3103007 Supporting Info |
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Nanoscience of an Ancient Pigment Darrah Johnson-McDaniel, Christopher A. Barrett, Asma Sharafi, and Tina T. Salguero pp 1677–1679 DOI: 10.1021/ja310587c Supporting Info |
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Size-Dependent Assemblies of Nanoparticle Mixtures in Thin Films Joseph Kao, Peter Bai, J. Matthew Lucas, A. Paul Alivisatos, and Ting Xu pp 1680–1683 DOI: 10.1021/ja3107912 Supporting Info |
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Direct Electrodeposition of Crystalline Silicon at Low Temperatures Junsi Gu, Eli Fahrenkrug, and Stephen Maldonado pp 1684–1687 DOI: 10.1021/ja310897r Supporting Info |
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High-Resolution Heteronuclear Multidimensional NMR of Proteins in Living Insect Cells Using a Baculovirus Protein Expression System Jumpei Hamatsu, Daniel O’Donovan, Takashi Tanaka, Takahiro Shirai, Yuichiro Hourai, Tsutomu Mikawa, Teppei Ikeya, Masaki Mishima, Wayne Boucher, Brian O. Smith, Ernest D. Laue, Masahiro Shirakawa, and Yutaka Ito pp 1688–1691 DOI: 10.1021/ja310928u Supporting Info |
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Stabilization of Ruthenium Sensitizers to TiO2 Surfaces through Cooperative Anchoring Groups Douglas G. Brown, Phil A. Schauer, Javier Borau-Garcia, Brandon R. Fancy, and Curtis P. Berlinguette pp 1692–1695 DOI: 10.1021/ja310965h Supporting Info |
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Tin Clathrates with the Type II Structure Marion C. Schäfer and Svilen Bobev pp 1696–1699 DOI: 10.1021/ja3112934 Supporting Info |
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Glucose Sensing via Aggregation and the Use of “Knock-Out” Binding To Improve Selectivity Yan-Jun Huang, Wen-Juan Ouyang, Xin Wu, Zhao Li, John S. Fossey, Tony D. James, and Yun-Bao Jiang pp 1700–1703 DOI: 10.1021/ja311442x Supporting Info |
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A Super-Reduced Diferrous [2Fe–2S] Cluster Antonia Albers, Serhiy Demeshko, Kevin Pröpper, Sebastian Dechert, Eckhard Bill, and Franc Meyer pp 1704–1707 DOI: 10.1021/ja311563y Supporting Info |
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Electrochemically Mediated Atom Transfer Radical Polymerization on Nonconducting Substrates: Controlled Brush Growth through Catalyst Diffusion Bin Li, Bo Yu, Wilhelm T. S. Huck, Weimin Liu, and Feng Zhou pp 1708–1710 DOI: 10.1021/ja3116197 Supporting Info |
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Exploiting Specific Interactions toward Next-Generation Polymeric Drug Transporters Sebastian Wieczorek, Eberhard Krause, Steffen Hackbarth, Beate Röder, Anna K. H. Hirsch, and Hans G. Börner pp 1711–1714 DOI: 10.1021/ja311895z Supporting Info |
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Electron-Deficient η1-Indenyl,η3-allylpalladium(II) Complexes Stabilized by Fluxional Non-covalent Interactions Christophe Werlé, Mustapha Hamdaoui, Corinne Bailly, Xavier-Frédéric Le Goff, Lydia Brelot, and Jean-Pierre Djukic pp 1715–1718 DOI: 10.1021/ja312003q Supporting Info |
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Nb–Nb Interactions Define the Charge Density Wave Structure of 2H-NbSe2 Christos D. Malliakas and Mercouri G. Kanatzidis pp 1719–1722 DOI: 10.1021/ja3120554 Supporting Info |
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Mixed Valency in Hydrogen Bonded ‘Dimers of Dimers’ Luke A. Wilkinson, Laura McNeill, Anthony J. H. M. Meijer, and Nathan J. Patmore pp 1723–1726 DOI: 10.1021/ja312176x Supporting Info |
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Charge Separation Promoted Activation of Molecular Oxygen by Neutral Gold Clusters Alex P. Woodham, Gerard Meijer, and André Fielicke pp 1727–1730 DOI: 10.1021/ja312223t Supporting Info |
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Thiophene-Fused Bisdehydro[12]annulene That Undergoes Transannular Alkyne Cycloaddition by Either Light or Heat Aiko Fukazawa, Hiroya Oshima, Yoshihito Shiota, Shouya Takahashi, Kazunari Yoshizawa, and Shigehiro Yamaguchi pp 1731–1734 DOI: 10.1021/ja3126849 Supporting Info |
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Investigation of Fungal Iterative Polyketide Synthase Functions Using Partially Assembled Intermediates Zhizeng Gao, Jingjing Wang, Amy K. Norquay, Kangjian Qiao, Yi Tang, and John C. Vederas pp 1735–1738 DOI: 10.1021/ja4001823 Supporting Info |
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Characterization of Streptonigrin Biosynthesis Reveals a Cryptic Carboxyl Methylation and an Unusual Oxidative Cleavage of a N–C Bond Fei Xu, Dekun Kong, Xinyi He, Zhang Zhang, Mo Han, Xinqiang Xie, Peng Wang, Hairong Cheng, Meifeng Tao, Liping Zhang, Zixin Deng, and Shuangjun Lin pp 1739–1748 DOI: 10.1021/ja3069243 Supporting Info |
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Non-ribosomal Propeptide Precursor in Nocardicin A Biosynthesis Predicted from Adenylation Domain Specificity Dependent on the MbtH Family Protein NocI Jeanne M. Davidsen, David M. Bartley, and Craig A. Townsend pp 1749–1759 DOI: 10.1021/ja307710d Supporting Info |
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Atomistic Theory of Ostwald Ripening and Disintegration of Supported Metal Particles under Reaction Conditions Runhai Ouyang, Jin-Xun Liu, and Wei-Xue Li pp 1760–1771 DOI: 10.1021/ja3087054 Supporting Info |
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How Do Disorder, Reorganization, and Localization Influence the Hole Mobility in Conjugated Copolymers? Sebastian T. Hoffmann, Frank Jaiser, Anna Hayer, Heinz Bässler, Thomas Unger, Stavros Athanasopoulos, Dieter Neher, and Anna Köhler pp 1772–1782 DOI: 10.1021/ja308820j Supporting Info |
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Strategy for Dual-Analyte Luciferin Imaging: In Vivo Bioluminescence Detection of Hydrogen Peroxide and Caspase Activity in a Murine Model of Acute Inflammation Genevieve C. Van de Bittner, Carolyn R. Bertozzi, and Christopher J. Chang pp 1783–1795 DOI: 10.1021/ja309078t Supporting Info |
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One-Pot versus Sequential Reactions in the Self-Assembly of Gigantic Nanoscale Polyoxotungstates Jing Gao, Jun Yan, Sebastian Beeg, De-Liang Long, and Leroy Cronin pp 1796–1805 DOI: 10.1021/ja309237x Supporting Info |
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Fluorine Substituents Reduce Charge Recombination and Drive Structure and Morphology Development in Polymer Solar Cells Andrew C. Stuart, John R. Tumbleston, Huaxing Zhou, Wentao Li, Shubin Liu, Harald Ade, and Wei You pp 1806–1815 DOI: 10.1021/ja309289u Supporting Info |
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Inhibition of IspH, a [4Fe–4S]2+ Enzyme Involved in the Biosynthesis of Isoprenoids via the Methylerythritol Phosphate Pathway Karnjapan Janthawornpong, Sergiy Krasutsky, Philippe Chaignon, Michel Rohmer, C. Dale Poulter, and Myriam Seemann pp 1816–1822 DOI: 10.1021/ja309557s Supporting Info |
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Oxygen Switch in Visible-Light Photoredox Catalysis: Radical Additions and Cyclizations and Unexpected C–C-Bond Cleavage Reactions Shaoqun Zhu, Arindam Das, Lan Bui, Hanjun Zhou, Dennis P. Curran, and Magnus Rueping pp 1823–1829 DOI: 10.1021/ja309580a Supporting Info |
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Reevaluation of the d-Amino Acid Compatibility with the Elongation Event in Translation Tomoshige Fujino, Yuki Goto, Hiroaki Suga, and Hiroshi Murakami pp 1830–1837 DOI: 10.1021/ja309570x Supporting Info |
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SrFe0.5Ru0.5O2: Square-Planar Ru2+ in an Extended Oxide Fabio Denis Romero, Steven J. Burr, John E. McGrady, Diego Gianolio, Giannantonio Cibin, and Michael A. Hayward pp 1838–1844 DOI: 10.1021/ja309798e Supporting Info |
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Single-Molecule Catalysis Mapping Quantifies Site-Specific Activity and Uncovers Radial Activity Gradient on Single 2D Nanocrystals Nesha May Andoy, Xiaochun Zhou, Eric Choudhary, Hao Shen, Guokun Liu, and Peng Chen pp 1845–1852 DOI: 10.1021/ja309948y Supporting Info |
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Quantification of the Effect of Conformational Restriction on Supramolecular Effective Molarities Harry Adams, Elena Chekmeneva, Christopher A. Hunter, Maria Cristina Misuraca, Cristina Navarro, and Simon M. Turega pp 1853–1863 DOI: 10.1021/ja310221t Supporting Info |
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Covalency in Metal–Oxygen Multiple Bonds Evaluated Using Oxygen K-edge Spectroscopy and Electronic Structure Theory Stefan G. Minasian, Jason M. Keith, Enrique R. Batista, Kevin S. Boland, Joseph A. Bradley, Scott R. Daly, Stosh A. Kozimor, Wayne W. Lukens, Richard L. Martin, Dennis Nordlund, Gerald T. Seidler, David K. Shuh, Dimosthenis Sokaras, Tolek Tyliszczak, Gregory L. Wagner, Tsu-Chein Weng, and Ping Yang pp 1864–1871 DOI: 10.1021/ja310223b Supporting Info |
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Laboratory Evolution of Enantiocomplementary Candida antarctica Lipase B Mutants with Broad Substrate Scope Qi Wu, Pankaj Soni, and Manfred T. Reetz pp 1872–1881 DOI: 10.1021/ja310455t Supporting Info |
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Interplay between Drying and Stability of a TIM Barrel Protein: A Combined Simulation–Experimental Study Payel Das, Divya Kapoor, Kevin T. Halloran, Ruhong Zhou, and C. Robert Matthews pp 1882–1890 DOI: 10.1021/ja310544t Supporting Info |
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Enantioselective Formal Aza-Diels–Alder Reactions of Enones with Cyclic Imines Catalyzed by Primary Aminothioureas Mathieu P. Lalonde, Meredeth A. McGowan, Naomi S. Rajapaksa, and Eric N. Jacobsen pp 1891–1894 DOI: 10.1021/ja310718f Supporting Info |
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Multisite Prenylation of 4-Substituted Tryptophans by Dimethylallyltryptophan Synthase Jeffrey D. Rudolf, Hong Wang, and C. Dale Poulter pp 1895–1902 DOI: 10.1021/ja310734n Supporting Info |
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Electronic and Structural Effects of Stepwise Borylation and Quaternization on Borirene Aromaticity Holger Braunschweig, Alexander Damme, Rian D. Dewhurst, Sundargopal Ghosh, Thomas Kramer, Bernd Pfaffinger, Krzysztof Radacki, and Alfredo Vargas pp 1903–1911 DOI: 10.1021/ja3110126 Supporting Info |
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Size- and Orientation-Selective Si Nanowire Growth: Thermokinetic Effects of Nanoscale Plasma Chemistry Hamid Mehdipour and Kostya (Ken) Ostrikov pp 1912–1918 DOI: 10.1021/ja3110279 Supporting Info |
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Optimized Phospholipid Bilayer Nanodiscs Facilitate High-Resolution Structure Determination of Membrane Proteins Franz Hagn, Manuel Etzkorn, Thomas Raschle, and Gerhard Wagner pp 1919–1925 DOI: 10.1021/ja310901f Supporting Info |
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Semiconductor@Metal–Organic Framework Core–Shell Heterostructures: A Case of ZnO@ZIF-8 Nanorods with Selective Photoelectrochemical Response Wen-wen Zhan, Qin Kuang, Jian-zhang Zhou, Xiang-jian Kong, Zhao-xiong Xie, and Lan-sun Zheng pp 1926–1933 DOI: 10.1021/ja311085e Supporting Info |
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Smart Mesoporous SiO2 Nanoparticles for the DNAzyme-Induced Multiplexed Release of Substrates Zhanxia Zhang, Dora Balogh, Fuan Wang, and Itamar Willner pp 1934–1940 DOI: 10.1021/ja311385y Supporting Info |
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Synthesis of Ag Nanocubes 18–32 nm in Edge Length: The Effects of Polyol on Reduction Kinetics, Size Control, and Reproducibility Yi Wang, Yiqun Zheng, Cheng Zhi Huang, and Younan Xia pp 1941–1951 DOI: 10.1021/ja311503q Supporting Info |
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Counterintuitive Mechanisms of the Addition of Hydrogen and Simple Olefins to Heavy Group 13 Alkene Analogues Christine A. Caputo, Juha Koivistoinen, Jani Moilanen, Jessica N. Boynton, Heikki M. Tuononen, and Philip P. Power pp 1952–1960 DOI: 10.1021/ja3116789 Supporting Info |
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Atomic Level Resolution of Dye Regeneration in the Dye-Sensitized Solar Cell Kiyoshi C. D. Robson, Ke Hu, Gerald J. Meyer, and Curtis P. Berlinguette pp 1961–1971 DOI: 10.1021/ja311640f Supporting Info |
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The Dynamics of Dendrimers by NMR Relaxation: Interpretation Pitfalls Luiz F. Pinto, Juan Correa, Manuel Martin-Pastor, Ricardo Riguera, and Eduardo Fernandez-Megia pp 1972–1977 DOI: 10.1021/ja311908n Supporting Info |
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Chemoselectivity in the Reductive Elimination from High Oxidation State Palladium Complexes – Scrambling Mechanism Uncovered Mads C. Nielsen, Eirik Lyngvi, and Franziska Schoenebeck pp 1978–1985 DOI: 10.1021/ja312047b Supporting Info |
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Dialkoxybithiazole: A New Building Block for Head-to-Head Polymer Semiconductors Xugang Guo, Jordan Quinn, Zhihua Chen, Hakan Usta, Yan Zheng, Yu Xia, Jonathan W. Hennek, Rocío Ponce Ortiz, Tobin J. Marks, and Antonio Facchetti pp 1986–1996 DOI: 10.1021/ja3120532 Supporting Info |
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Combined Experimental and Theoretical Study on the Reductive Cleavage of Inert C–O Bonds with Silanes: Ruling out a Classical Ni(0)/Ni(II) Catalytic Couple and Evidence for Ni(I) Intermediates Josep Cornella, Enrique Gómez-Bengoa, and Ruben Martin pp 1997–2009 DOI: 10.1021/ja311940s Supporting Info |
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Spotlights on Recent JACS Publications pp 2011–2012 DOI: 10.1021/ja4011749 |
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Strongly Coupled Inorganic/Nanocarbon Hybrid Materials for Advanced Electrocatalysis Yongye Liang, Yanguang Li, Hailiang Wang, and Hongjie Dai pp 2013–2036 DOI: 10.1021/ja3089923 |
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Engineering Bacterial Two-Component System PmrA/PmrB to Sense Lanthanide Ions Haihua Liang, Xin Deng, Mike Bosscher, Quanjiang Ji, Mark P. Jensen, and Chuan He pp 2037–2039 DOI: 10.1021/ja312032c Supporting Info |
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Fused Dithienogermolodithiophene Low Band Gap Polymers for High-Performance Organic Solar Cells without Processing Additives Hongliang Zhong, Zhe Li, Florent Deledalle, Elisa Collado Fregoso, Munazza Shahid, Zhuping Fei, Christian B. Nielsen, Nir Yaacobi-Gross, Stephan Rossbauer, Thomas D. Anthopoulos, James R. Durrant, and Martin Heeney pp 2040–2043 DOI: 10.1021/ja311700u Supporting Info |
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Colocalized Delivery of Adjuvant and Antigen Using Nanolipoprotein Particles Enhances the Immune Response to Recombinant Antigens Nicholas O. Fischer, Amy Rasley, Michele Corzett, Mona H. Hwang, Paul D. Hoeprich, and Craig D. Blanchette pp 2044–2047 DOI: 10.1021/ja3063293 Supporting Info |
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Electrocatalytic Water Oxidation with a Copper(II) Polypeptide Complex Ming-Tian Zhang, Zuofeng Chen, Peng Kang, and Thomas J. Meyer pp 2048–2051 DOI: 10.1021/ja3097515 Supporting Info |
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A Molecular Platinum Cluster Junction: A Single-Molecule Switch Linda A. Zotti, Edmund Leary, Maria Soriano, Juan Carlos Cuevas, and Juan Jose Palacios pp 2052–2055 DOI: 10.1021/ja3100116 Supporting Info |
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Liposome–Quantum Dot Complexes Enable Multiplexed Detection of Attomolar DNAs without Target Amplification Juan Zhou, Qiang-xin Wang, and Chun-yang Zhang pp 2056–2059 DOI: 10.1021/ja3110329 Supporting Info |
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Termini of Bottom-Up Fabricated Graphene Nanoribbons Leopold Talirz, Hajo Söde, Jinming Cai, Pascal Ruffieux, Stephan Blankenburg, Rached Jafaar, Reinhard Berger, Xinliang Feng, Klaus Müllen, Daniele Passerone, Roman Fasel, and Carlo A. Pignedoli pp 2060–2063 DOI: 10.1021/ja311099k Supporting Info |
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A Nonribosomal Peptide Synthetase-Derived Iron(III) Complex from the Pathogenic Fungus Aspergillus fumigatus Wen-Bing Yin, Joshua A. Baccile, Jin Woo Bok, Yiming Chen, Nancy P. Keller, and Frank C. Schroeder pp 2064–2067 DOI: 10.1021/ja311145n Supporting Info |
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Control of Diastereoselectivity for Iridium-Catalyzed Allylation of a Prochiral Nucleophile with a Phosphate Counterion Wenyong Chen and John F. Hartwig pp 2068–2071 DOI: 10.1021/ja311363a Supporting Info |
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DNAzyme Footprinting: Detecting Protein–Aptamer Complexation on Surfaces by Blocking DNAzyme Cleavage Activity Yulin Chen and Robert M. Corn pp 2072–2075 DOI: 10.1021/ja311367t Supporting Info |
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A Rechargeable Li–O2 Battery Using a Lithium Nitrate/N,N-Dimethylacetamide Electrolyte Wesley Walker, Vincent Giordani, Jasim Uddin, Vyacheslav S. Bryantsev, Gregory V. Chase, and Dan Addison pp 2076–2079 DOI: 10.1021/ja311518s Supporting Info |
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Redox Mediator Effect on Water Oxidation in a Ruthenium-Based Chromophore–Catalyst Assembly Michael R. Norris, Javier J. Concepcion, Daniel P. Harrison, Robert A. Binstead, Dennis L. Ashford, Zhen Fang, Joseph L. Templeton, and Thomas J. Meyer pp 2080–2083 DOI: 10.1021/ja311645d Supporting Info |
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Formation of [3]Catenanes from 10 Precursors via Multicomponent Coordination-Driven Self-Assembly of Metallarectangles Shijun Li, Jianying Huang, Timothy R. Cook, J. Bryant Pollock, Hyunuk Kim, Ki-Whan Chi, and Peter J. Stang pp 2084–2087 DOI: 10.1021/ja3118812 Supporting Info |
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Substrate-Initiated Synthesis of Cell-Penetrating Poly(disulfide)s Eun-Kyoung Bang, Giulio Gasparini, Guillaume Molinard, Aurélien Roux, Naomi Sakai, and Stefan Matile pp 2088–2091 DOI: 10.1021/ja311961k Supporting Info |
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Iridium-Catalyzed [3 + 2] Annulation of Cyclic N-Sulfonyl Ketimines with 1,3-Dienes via C–H Activation Takahiro Nishimura, Yusuke Ebe, and Tamio Hayashi pp 2092–2095 DOI: 10.1021/ja311968d Supporting Info |
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Thermally Persistent Fluorosulfonyl Nitrene and Unexpected Formation of the Fluorosulfonyl Radical Xiaoqing Zeng, Helmut Beckers, and Helge Willner pp 2096–2099 DOI: 10.1021/ja312073w Supporting Info |
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Catalytic Asymmetric Protonation of Silyl Ketene Imines Joyram Guin, Georgy Varseev, and Benjamin List pp 2100–2103 DOI: 10.1021/ja312141b Supporting Info |
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Bifunctional Ruthenium(II) Hydride Complexes with Pendant Strong Lewis Acid Moieties: Structure, Dynamics, and Cooperativity Thomas G. Ostapowicz, Carina Merkens, Markus Hölscher, Jürgen Klankermayer, and Walter Leitner pp 2104–2107 DOI: 10.1021/ja3119477 Supporting Info |
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When Electron Transfer Meets Electron Transport in Redox-Active Molecular Nanojunctions Marion Janin, Jalal Ghilane, and Jean-Christophe Lacroix pp 2108–2111 DOI: 10.1021/ja3122125 Supporting Info |
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Selective Cell Death by Photochemically Induced pH Imbalance in Cancer Cells Xiling Yue, Ciceron O. Yanez, Sheng Yao, and Kevin D. Belfield pp 2112–2115 DOI: 10.1021/ja3122312 Supporting Info |
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Iridium-Catalyzed Intermolecular Asymmetric Hydroheteroarylation of Bicycloalkenes Christo S. Sevov and John F. Hartwig pp 2116–2119 DOI: 10.1021/ja312360c Supporting Info |
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Accessing Long-Lived Nuclear Spin Order by Isotope-Induced Symmetry Breaking Michael C. D. Tayler and Malcolm H. Levitt pp 2120–2123 DOI: 10.1021/ja312227h Supporting Info |
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Palladium-Catalyzed Picolinamide-Directed Alkylation of Unactivated C(sp3)–H Bonds with Alkyl Iodides Shu-Yu Zhang, Gang He, William A. Nack, Yingsheng Zhao, Qiong Li, and Gong Chen pp 2124–2127 DOI: 10.1021/ja312277g Supporting Info |
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Time-Resolved Radiation Chemistry: Photoelectron Imaging of Transient Negative Ions of Nucleobases Margaret A. Yandell, Sarah B. King, and Daniel M. Neumark pp 2128–2131 DOI: 10.1021/ja312414y |
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Dinuclear Bis-Propagators for the Stereoselective Living Coordinative Chain Transfer Polymerization of Propene Jia Wei, Wonseok Hwang, Wei Zhang, and Lawrence R. Sita pp 2132–2135 DOI: 10.1021/ja312463f Supporting Info |
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On-Surface Azide–Alkyne Cycloaddition on Cu(111): Does It “Click” in Ultrahigh Vacuum? Fabian Bebensee, Christian Bombis, Sundar-Raja Vadapoo, Jacob R. Cramer, Flemming Besenbacher, Kurt V. Gothelf, and Trolle R. Linderoth pp 2136–2139 DOI: 10.1021/ja312303a Supporting Info |
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Copper-Catalyzed Enantioselective Allyl–Allyl Cross-Coupling Valentín Hornillos, Manuel Pérez, Martín Fañanás-Mastral, and Ben L. Feringa pp 2140–2143 DOI: 10.1021/ja312487r Supporting Info |
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Stereochemical Control of Polymorph Transitions in Nanoscale Reactors Qi Jiang, Chunhua Hu, and Michael D. Ward pp 2144–2147 DOI: 10.1021/ja312511v Supporting Info |
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Cooperative Supramolecular Polymerization Driven by Metallophilic Pd···Pd Interactions María José Mayoral, Christina Rest, Vladimir Stepanenko, Jennifer Schellheimer, Rodrigo Q. Albuquerque, and Gustavo Fernández pp 2148–2151 DOI: 10.1021/ja312628g Supporting Info |
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Chiral Selective Transmembrane Transport of Amino Acids through Artificial Channels Lei Chen, Wen Si, Liang Zhang, Gangfeng Tang, Zhan-Ting Li, and Jun-Li Hou pp 2152–2155 DOI: 10.1021/ja312704e Supporting Info |
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Supramolecular Switching between Flat Sheets and Helical Tubules Triggered by Coordination Interaction Suyong Shin, Sunhee Lim, Yongju Kim, Taehoon Kim, Tae-Lim Choi, and Myongsoo Lee pp 2156–2159 DOI: 10.1021/ja400160j Supporting Info |
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Twisted Tethered Tolanes: Unanticipated Long-Lived Phosphorescence at 77 K Sebastian Menning, Maximilian Krämer, Benjamin A. Coombs, Frank Rominger, Andrew Beeby, Andreas Dreuw, and Uwe H. F. Bunz pp 2160–2163 DOI: 10.1021/ja400416r Supporting Info |
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Binding of Serotonin to Lipid Membranes Günther H. Peters, Chunhua Wang, Nicolaj Cruys-Bagger, Gustavo F. Velardez, Jesper J. Madsen, and Peter Westh pp 2164–2171 DOI: 10.1021/ja306681d Supporting Info |
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Asymmetric Ligand Binding Facilitates Conformational Transitions in Pentameric Ligand-Gated Ion Channels David Mowrey, Mary Hongying Cheng, Lu Tian Liu, Dan Willenbring, Xinghua Lu, Troy Wymore, Yan Xu, and Pei Tang pp 2172–2180 DOI: 10.1021/ja307275v Supporting Info |
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Sequence Effects on Peptide Assembly Characteristics Observed by Using Scanning Tunneling Microscopy Xiaobo Mao, Yuanyuan Guo, Yin Luo, Lin Niu, Lei Liu, Xiaojing Ma, Huibin Wang, Yanlian Yang, Guanghong Wei, and Chen Wang pp 2181–2187 DOI: 10.1021/ja307198u Supporting Info |
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An Atomistic Model for Assembly of Transmembrane Domain of T cell Receptor Complex Satyan Sharma and André H. Juffer pp 2188–2197 DOI: 10.1021/ja308413e Supporting Info |
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A Unified Electrocatalytic Description of the Action of Inhibitors of Nickel Carbon Monoxide Dehydrogenase Vincent C.-C. Wang, Mehmet Can, Elizabeth Pierce, Stephen W. Ragsdale, and Fraser A. Armstrong pp 2198–2206 DOI: 10.1021/ja308493k Supporting Info |
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Using Self-Organization To Control Morphology in Molecular Photovoltaics Seok Ju Kang, Seokhoon Ahn, Jong Bok Kim, Christine Schenck, Anna M. Hiszpanski, Seokjoon Oh, Theanne Schiros, Yueh-Lin Loo, and Colin Nuckolls pp 2207–2212 DOI: 10.1021/ja308628z Supporting Info |
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A Generic Approach for the Synthesis of Dimer Nanoclusters and Asymmetric Nanoassemblies Yongxing Hu and Yugang Sun pp 2213–2221 DOI: 10.1021/ja309501s Supporting Info |
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Ruthenium-Mediated C–H Functionalization of Pyridine: The Role of Vinylidene and Pyridylidene Ligands David G. Johnson, Jason M. Lynam, Neetisha S. Mistry, John M. Slattery, Robert J. Thatcher, and Adrian C. Whitwood pp 2222–2234 DOI: 10.1021/ja3097256 Supporting Info |
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Long-Loop G-Quadruplexes Are Misfolded Population Minorities with Fast Transition Kinetics in Human Telomeric Sequences Deepak Koirala, Chiran Ghimire, Christopher Bohrer, Yuta Sannohe, Hiroshi Sugiyama, and Hanbin Mao pp 2235–2241 DOI: 10.1021/ja309668t Supporting Info |
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Productive Chemical Interaction between a Bacterial Microcolony Couple Is Enhanced by Periodic Relocation Chang Kyu Byun, Hyundoo Hwang, Woon Sun Choi, Toshiyuki Yaguchi, Jiwoon Park, Dasol Kim, Robert J. Mitchell, Taesung Kim, Yoon-Kyoung Cho, and Shuichi Takayama pp 2242–2247 DOI: 10.1021/ja3094923 Supporting Info |
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Formation Pathway for LTA Zeolite Crystals Synthesized via a Charge Density Mismatch Approach Min Bum Park, Yoorim Lee, Anmin Zheng, Feng-Shou Xiao, Christopher P. Nicholas, Gregory J. Lewis, and Suk Bong Hong pp 2248–2255 DOI: 10.1021/ja309831e Supporting Info |
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Proton-Conductive Magnetic Metal–Organic Frameworks, {NR3(CH2COOH)}[MaIIMbIII(ox)3]: Effect of Carboxyl Residue upon Proton Conduction Hisashi O̅kawa, Masaaki Sadakiyo, Teppei Yamada, Mitsuhiko Maesato, Masaaki Ohba, and Hiroshi Kitagawa pp 2256–2262 DOI: 10.1021/ja309968u Supporting Info |
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Structural Insights into a Unique Inhibitor Binding Pocket in Kinesin Spindle Protein Venkatasubramanian Ulaganathan, Sandeep K. Talapatra, Oliver Rath, Andrew Pannifer, David D. Hackney, and Frank Kozielski pp 2263–2272 DOI: 10.1021/ja310377d Supporting Info |
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Size-Dependent Dissociation of Carbon Monoxide on Cobalt Nanoparticles Anders Tuxen, Sophie Carenco, Mahati Chintapalli, Cheng-Hao Chuang, Carlos Escudero, Elzbieta Pach, Peng Jiang, Ferenc Borondics, Brandon Beberwyck, A. Paul Alivisatos, Geoff Thornton, Way-Faung Pong, Jinghua Guo, Ruben Perez, Flemming Besenbacher, and Miquel Salmeron pp 2273–2278 DOI: 10.1021/ja3105889 |
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Tetrahalide Complexes of the [U(NR)2]2+ Ion: Synthesis, Theory, and Chlorine K-Edge X-ray Absorption Spectroscopy Liam P. Spencer, Ping Yang, Stefan G. Minasian, Robert E. Jilek, Enrique R. Batista, Kevin S. Boland, James M. Boncella, Steven D. Conradson, David L. Clark, Trevor W. Hayton, Stosh A. Kozimor, Richard L. Martin, Molly M. MacInnes, Angela C. Olson, Brian L. Scott, David K. Shuh, and Marianne P. Wilkerson pp 2279–2290 DOI: 10.1021/ja310575j Supporting Info |
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Reconciling the Roles of Kinetic and Thermodynamic Factors in Membrane–Protein Insertion James C. Gumbart, Ivan Teo, Benoît Roux, and Klaus Schulten pp 2291–2297 DOI: 10.1021/ja310777k Supporting Info |
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Impact of Regiochemistry and Isoelectronic Bridgehead Substitution on the Molecular Shape and Bulk Organization of Narrow Bandgap Chromophores Gregory C. Welch, Ronald C. Bakus, II, Simon J. Teat, and Guillermo C. Bazan pp 2298–2305 DOI: 10.1021/ja310694t Supporting Info |
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Covalently Functionalized Double-Walled Carbon Nanotubes Combine High Sensitivity and Selectivity in the Electrical Detection of Small Molecules Jia Huang, Allen L. Ng, Yanmei Piao, Chien-Fu Chen, Alexander A. Green, Chuan-Fu Sun, Mark C. Hersam, Cheng S. Lee, and YuHuang Wang pp 2306–2312 DOI: 10.1021/ja310844u Supporting Info |
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Ditopic Ambiphilicity of an Anionic Dimetalloborylene Complex Holger Braunschweig, Alexander Damme, Rian D. Dewhurst, Thomas Kramer, Sebastian Östreicher, Krzysztof Radacki, and Alfredo Vargas pp 2313–2320 DOI: 10.1021/ja310895w Supporting Info |
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Nanoscale Mechanism of Molecular Transport through the Nuclear Pore Complex As Studied by Scanning Electrochemical Microscopy Jiyeon Kim, Anahita Izadyar, Nikoloz Nioradze, and Shigeru Amemiya pp 2321–2329 DOI: 10.1021/ja311080j Supporting Info |
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Tunable Biomimetic Chalcogels with Fe4S4 Cores and [SnnS2n+2]4–(n = 1, 2, 4) Building Blocks for Solar Fuel Catalysis Yurina Shim, Benjamin D. Yuhas, Scott M. Dyar, Amanda L. Smeigh, Alexios P. Douvalis, Michael R. Wasielewski, and Mercouri G. Kanatzidis pp 2330–2337 DOI: 10.1021/ja311310k Supporting Info |
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Critical Role of Alkyl Chain Branching of Organic Semiconductors in Enabling Solution-Processed N-Channel Organic Thin-Film Transistors with Mobility of up to 3.50 cm2 V–1 s–1 Fengjiao Zhang, Yunbin Hu, Torben Schuettfort, Chong-an Di, Xike Gao, Christopher R. McNeill, Lars Thomsen, Stefan C. B. Mannsfeld, Wei Yuan, Henning Sirringhaus, and Daoben Zhu pp 2338–2349 DOI: 10.1021/ja311469y Supporting Info |
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Structural Factors Controlling the Spin–Spin Exchange Coupling: EPR Spectroscopic Studies of Highly Asymmetric Trityl–Nitroxide Biradicals Yangping Liu, Frederick A. Villamena, Antal Rockenbauer, Yuguang Song, and Jay L. Zweier pp 2350–2356 DOI: 10.1021/ja311571v Supporting Info |
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Mechanism of Copper(I)/TEMPO-Catalyzed Aerobic Alcohol Oxidation Jessica M. Hoover, Bradford L. Ryland, and Shannon S. Stahl pp 2357–2367 DOI: 10.1021/ja3117203 Supporting Info |
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Step Flow Versus Mosaic Film Growth in Hexagonal Boron Nitride Jiong Lu, Pei Shan Emmeline Yeo, Yi Zheng, Hai Xu, Chee Kwan Gan, Michael B. Sullivan, A.H. Castro Neto, and Kian Ping Loh pp 2368–2373 DOI: 10.1021/ja3117735 Supporting Info |
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Time-Resolved Observation of Chiral-Index-Selective Wrapping on Single-Walled Carbon Nanotube with Non-Aromatic Polysilane Woojung Chung, Kazuyuki Nobusawa, Hironari Kamikubo, Mikio Kataoka, Michiya Fujiki, and Masanobu Naito pp 2374–2383 DOI: 10.1021/ja311799m Supporting Info |
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Correction to Nickel-Silicide Colloid Prepared under Mild Conditions as a Versatile Ni Precursor for More Efficient CO2 Reforming of CH4 Catalysts David Baudouin, Kaï Chung Szeto, Pierre Laurent, Aimery De Mallmann, Bernard Fenet, Laurent Veyre, Uwe Rodemerck, Christophe Copéret, and Chloé Thieuleux pp 2384–2384 DOI: 10.1021/ja400426p |
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Spotlights on Recent JACS Publications pp 2385–2386 DOI: 10.1021/ja401254p |
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Fluorescent Proteins: Shine on, You Crazy Diamond Peter Dedecker, Frans C. De Schryver, and Johan Hofkens pp 2387–2402 DOI: 10.1021/ja309768d |
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Photoinduced Electron Transfer of DNA/Ag Nanoclusters Modulated by G-Quadruplex/Hemin Complex for the Construction of Versatile Biosensors Libing Zhang, Jinbo Zhu, Shaojun Guo, Tao Li, Jing Li, and Erkang Wang pp 2403–2406 DOI: 10.1021/ja3089857 Supporting Info |
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Sizing by Weighing: Characterizing Sizes of Ultrasmall-Sized Iron Oxide Nanocrystals Using MALDI-TOF Mass Spectrometry Byung Hyo Kim, Kwangsoo Shin, Soon Gu Kwon, Youngjin Jang, Hyun-Seok Lee, Hyunjae Lee, Samuel Woojoo Jun, Jisoo Lee, Sang Yun Han, Yong-Hyeon Yim, Dae-Hyeong Kim, and Taeghwan Hyeon pp 2407–2410 DOI: 10.1021/ja310030c Supporting Info |
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An Exceptionally Simple Strategy for DNA-Functionalized Up-Conversion Nanoparticles as Biocompatible Agents for Nanoassembly, DNA Delivery, and Imaging Le-Le Li, Peiwen Wu, Kevin Hwang, and Yi Lu pp 2411–2414 DOI: 10.1021/ja310432u Supporting Info |
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An Arsenical–Maleimide for the Generation of New Targeted Biochemical Reagents Aparna Sapra and Colin Thorpe pp 2415–2418 DOI: 10.1021/ja310553h Supporting Info |
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Cleavage of DNA by Proton-Coupled Electron Transfer to a Photoexcited, Hydrated Ru(II) 1,10-Phenanthroline-5,6-dione Complex Steven A. Poteet, Marek B. Majewski, Zachary S. Breitbach, Cynthia A. Griffith, Shreeyukta Singh, Daniel W. Armstrong, Michael O. Wolf, and Frederick M. MacDonnell pp 2419–2422 DOI: 10.1021/ja3106863 Supporting Info |
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A Locked Nucleic Acid-Based Nanocrawler: Designed and Reversible Movement Detected by Multicolor Fluorescence I. Kira Astakhova, Karol Pasternak, Meghan A. Campbell, Pankaj Gupta, and Jesper Wengel pp 2423–2426 DOI: 10.1021/ja311250w Supporting Info |
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Facile Large-Scale Synthesis of Monodisperse Mesoporous Silica Nanospheres with Tunable Pore Structure Kun Zhang, Lang-Lang Xu, Jin-Gang Jiang, Nathalie Calin, Koon-Fung Lam, San-Jun Zhang, Hai-Hong Wu, Guang-Dong Wu, Bélen Albela, Laurent Bonneviot, and Peng Wu pp 2427–2430 DOI: 10.1021/ja3116873 Supporting Info |
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Inner-Sphere Electron-Transfer Single Iodide Mechanism for Dye Regeneration in Dye-Sensitized Solar Cells Jiwon Jeon, William A. Goddard, III, and Hyungjun Kim pp 2431–2434 DOI: 10.1021/ja311714a Supporting Info |
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How “Hollow” Are Hollow Nanoparticles? Paul Podsiadlo, Soon Gu Kwon, Bonil Koo, Byeongdu Lee, Vitali B. Prakapenka, Przemyslaw Dera, Kirill K. Zhuravlev, Galyna Krylova, and Elena V. Shevchenko pp 2435–2438 DOI: 10.1021/ja311926r Supporting Info |
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Homopolar Dihydrogen Bonding in Alkali Metal Amidoboranes: Crystal Engineering of Low-Dimensional Molecular Materials David J. Wolstenholme, Jenna Flogeras, Franklin N. Che, Andreas Decken, and G. Sean McGrady pp 2439–2442 DOI: 10.1021/ja311778k Supporting Info |
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Dynamic DNA Assemblies Mediated by Binding-Induced DNA Strand Displacement Feng Li, Hongquan Zhang, Zhixin Wang, Xukun Li, Xing-Fang Li, and X. Chris Le pp 2443–2446 DOI: 10.1021/ja311990w Supporting Info |
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Efficient Self-Assembly in Water of Long Noncovalent Polymers by Nucleobase Analogues Brian J. Cafferty, Isaac Gállego, Michael C. Chen, Katherine I. Farley, Ramon Eritja, and Nicholas V. Hud pp 2447–2450 DOI: 10.1021/ja312155v Supporting Info |
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Site-Specific Immobilization of Single-Walled Carbon Nanotubes onto Single and One-Dimensional DNA Origami Anshuman Mangalum, Masudur Rahman, and Michael L. Norton pp 2451–2454 DOI: 10.1021/ja312191a Supporting Info |
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Tetragonal and Helical Morphologies from Polyferrocenylsilane Block Polyelectrolytes via Ionic Self-Assembly Rumman Ahmed, Sanjib K. Patra, Ian W. Hamley, Ian Manners, and Charl F. J. Faul pp 2455–2458 DOI: 10.1021/ja312318d Supporting Info |
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Regio- and Enantioselective Synthesis of Pyrrolidines Bearing a Quaternary Center by Palladium-Catalyzed Asymmetric [3 + 2] Cycloaddition of Trimethylenemethanes Barry M. Trost, Tom M. Lam, and Melissa A. Herbage pp 2459–2461 DOI: 10.1021/ja312351s Supporting Info |
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π-Conjugated Nickel Bis(dithiolene) Complex Nanosheet Tetsuya Kambe, Ryota Sakamoto, Ken Hoshiko, Kenji Takada, Mariko Miyachi, Ji-Heun Ryu, Sono Sasaki, Jungeun Kim, Kazuo Nakazato, Masaki Takata, and Hiroshi Nishihara pp 2462–2465 DOI: 10.1021/ja312380b Supporting Info |
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Redox-Controlled Selective Docking in a [2]Catenane Host Gokhan Barin, Marco Frasconi, Scott M. Dyar, Julien Iehl, Onur Buyukcakir, Amy A. Sarjeant, Raanan Carmieli, Ali Coskun, Michael R. Wasielewski, and J. Fraser Stoddart pp 2466–2469 DOI: 10.1021/ja3125004 Supporting Info |
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Late-Stage Deoxyfluorination of Alcohols with PhenoFluor Filippo Sladojevich, Sophie I. Arlow, Pingping Tang, and Tobias Ritter pp 2470–2473 DOI: 10.1021/ja3125405 Supporting Info |
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Efficient Asymmetric Synthesis of P-Chiral Phosphine Oxides via Properly Designed and Activated Benzoxazaphosphinine-2-oxide Agents Zhengxu S. Han, Navneet Goyal, Melissa A. Herbage, Joshua D. Sieber, Bo Qu, Yibo Xu, Zhibin, Li, Jonathan T. Reeves, Jean-Nicolas Desrosiers, Shengli Ma, Nelu Grinberg, Heewon Lee, Hari P. R. Mangunuru, Yongda Zhang, Dhileep Krishnamurthy, Bruce Z. Lu, Jinhua J. Song, Guijun Wang, and Chris H. Senanayake pp 2474–2477 DOI: 10.1021/ja312352p Supporting Info |
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Unstabilized Azomethine Ylides for the Stereoselective Synthesis of Substituted Piperidines, Tropanes, and Azabicyclo[3.1.0] Systems Michael A. Ischay, Michael K. Takase, Robert G. Bergman, and Jonathan A. Ellman pp 2478–2481 DOI: 10.1021/ja312311k Supporting Info |
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Prediction of Catalyst and Substrate Performance in the Enantioselective Propargylation of Aliphatic Ketones by a Multidimensional Model of Steric Effects Kaid C. Harper, Sarah C. Vilardi, and Matthew S. Sigman pp 2482–2485 DOI: 10.1021/ja4001807 Supporting Info |
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Oxidation of Carbene-Stabilized Diarsenic: Diarsene Dications and Diarsenic Radical Cations Mariham Y. Abraham, Yuzhong Wang, Yaoming Xie, Robert J. Gilliard, Jr., Pingrong Wei, Brian J. Vaccaro, Michael K. Johnson, Henry F. Schaefer, III, Paul v. R. Schleyer, and Gregory H. Robinson pp 2486–2488 DOI: 10.1021/ja400219d Supporting Info |
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Post-Polyketide Synthase Steps in Iso-migrastatin Biosynthesis, Featuring Tailoring Enzymes with Broad Substrate Specificity Ming Ma, Thomas Kwong, Si-Kyu Lim, Jianhua Ju, Jeremy R. Lohman, and Ben Shen pp 2489–2492 DOI: 10.1021/ja4002635 Supporting Info |
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Two Reversible σ-Bond Metathesis Pathways for Boron–Palladium Bond Formation: Selective Synthesis of Isomeric Five-Coordinate Borylpalladium Complexes Naohiro Kirai, Jun Takaya, and Nobuharu Iwasawa pp 2493–2496 DOI: 10.1021/ja400294m Supporting Info |
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1,3,5-Triazine as a Modular Scaffold for Covalent Inhibitors with Streamlined Target Identification Ranjan Banerjee, Nicholas J. Pace, Douglas R. Brown, and Eranthie Weerapana pp 2497–2500 DOI: 10.1021/ja400427e Supporting Info |
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A Catalytic Enantioselective Tandem Allylation Strategy for Rapid Terpene Construction: Application to the Synthesis of Pumilaside Aglycon Grace E. Ferris, Kai Hong, Ian A. Roundtree, and James P. Morken pp 2501–2504 DOI: 10.1021/ja400506j Supporting Info |
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Catalytic Hydrotrifluoromethylation of Unactivated Alkenes Satoshi Mizuta, Stefan Verhoog, Keary M. Engle, Tanatorn Khotavivattana, Miriam O’Duill, Katherine Wheelhouse, Gerasimos Rassias, Maurice Médebielle, and Véronique Gouverneur pp 2505–2508 DOI: 10.1021/ja401022x Supporting Info |
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Heavy-Enzyme Kinetic Isotope Effects on Proton Transfer in Alanine Racemase Michael D. Toney, Joan Nieto Castro, and Trevor A. Addington pp 2509–2511 DOI: 10.1021/ja3101243 Supporting Info |
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Fast Protein Motions Are Coupled to Enzyme H-Transfer Reactions Christopher R. Pudney, Andrew Guerriero, Nicola J. Baxter, Linus O. Johannissen, Jonathan P. Waltho, Sam Hay, and Nigel S. Scrutton pp 2512–2517 DOI: 10.1021/ja311277k Supporting Info |
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Structure of a Glycomimetic Ligand in the Carbohydrate Recognition Domain of C-type Lectin DC-SIGN. Structural Requirements for Selectivity and Ligand Design Michel Thépaut, Cinzia Guzzi, Ieva Sutkeviciute, Sara Sattin, Renato Ribeiro-Viana, Norbert Varga, Eric Chabrol, Javier Rojo, Anna Bernardi, Jesus Angulo, Pedro M. Nieto, and Franck Fieschi pp 2518–2529 DOI: 10.1021/ja3053305 Supporting Info |
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Characterization of [4Fe-4S] Cluster Vibrations and Structure in Nitrogenase Fe Protein at Three Oxidation Levels via Combined NRVS, EXAFS, and DFT Analyses Devrani Mitra, Simon J. George, Yisong Guo, Saeed Kamali, Stephen Keable, John W. Peters, Vladimir Pelmenschikov, David A. Case, and Stephen P. Cramer pp 2530–2543 DOI: 10.1021/ja307027n Supporting Info |
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Drug Delivery with a Calixpyrrole–trans-Pt(II) Complex Grazia Cafeo, Grazia Carbotti, Angela Cuzzola, Marina Fabbi, Silvano Ferrini, Franz H. Kohnke, Georgia Papanikolaou, Maria Rosaria Plutino, Camillo Rosano, and Andrew J. P. White pp 2544–2551 DOI: 10.1021/ja307791j Supporting Info |
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Copper-Mediated Fluorination of Arylboronate Esters. Identification of a Copper(III) Fluoride Complex Patrick S. Fier, Jingwei Luo, and John F. Hartwig pp 2552–2559 DOI: 10.1021/ja310909q Supporting Info |
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Distinct CCK-2 Receptor Conformations Associated with β-Arrestin-2 Recruitment or Phospholipase-C Activation Revealed by a Biased Antagonist Rémi Magnan, Chantal Escrieut, Véronique Gigoux, Kavita De, Pascal Clerc, Fan Niu, Joelle Azema, Bernard Masri, Arnau Cordomi, Michel Baltas, Irina G. Tikhonova, and Daniel Fourmy pp 2560–2573 DOI: 10.1021/ja308784w Supporting Info |
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Hydrophobic Molecules Infiltrating into the Poly(ethylene glycol) Domain of the Core/Shell Interface of a Polymeric Micelle: Evidence Obtained with Anomalous Small-Angle X-ray Scattering Yusuke Sanada, Isamu Akiba, Kazuo Sakurai, Kouichi Shiraishi, Masayuki Yokoyama, Efstratios Mylonas, Noboru Ohta, Naoto Yagi, Yuya Shinohara, and Yoshiyuki Amemiya pp 2574–2582 DOI: 10.1021/ja308965j Supporting Info |
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CO Self-Promoting Oxidation on Nanosized Gold Clusters: Triangular Au3 Active Site and CO Induced O–O Scission Chunyan Liu, Yingzi Tan, Sisi Lin, Hui Li, Xiaojun Wu, Lei Li, Yong Pei, and Xiao Cheng Zeng pp 2583–2595 DOI: 10.1021/ja309460v Supporting Info |
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Catalytic DNAs That Harness Violet Light To Repair Thymine Dimers in a DNA Substrate Adam Barlev and Dipankar Sen pp 2596–2603 DOI: 10.1021/ja309638j Supporting Info |
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Quantum Chemical Calculations with the Inclusion of Nonspecific and Specific Solvation: Asymmetric Transfer Hydrogenation with Bifunctional Ruthenium Catalysts Pavel A. Dub and Takao Ikariya pp 2604–2619 DOI: 10.1021/ja3097674 Supporting Info |
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Different Nature of the Interactions between Anions and HAT(CN)6: From Reversible Anion−π Complexes to Irreversible Electron-Transfer Processes (HAT(CN)6 = 1,4,5,8,9,12-Hexaazatriphenylene) Gemma Aragay, Antonio Frontera, Vega Lloveras, José Vidal-Gancedo, and Pablo Ballester pp 2620–2627 DOI: 10.1021/ja309960m Supporting Info |
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Directly Probing the Effects of Ions on Hydration Forces at Interfaces Jason I. Kilpatrick, Siu-Hong Loh, and Suzanne P. Jarvis pp 2628–2634 DOI: 10.1021/ja310255s Supporting Info |
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Copper(I)-Catalyzed Borylative exo-Cyclization of Alkenyl Halides Containing Unactivated Double Bond Koji Kubota, Eiji Yamamoto, and Hajime Ito pp 2635–2640 DOI: 10.1021/ja3104582 Supporting Info |
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Controlling Crystal Polymorphism in Organic-Free Synthesis of Na-Zeolites Miguel Maldonado, Matthew D. Oleksiak, Sivadinarayana Chinta, and Jeffrey D. Rimer pp 2641–2652 DOI: 10.1021/ja3105939 Supporting Info |
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Enantioselective Liquid–Liquid Extractions of Underivatized General Amino Acids with a Chiral Ketone Extractant Haofei Huang, Raju Nandhakumar, Misun Choi, Zhishan Su, and Kwan Mook Kim pp 2653–2658 DOI: 10.1021/ja3105945 Supporting Info |
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Effective Optical Faraday Rotations of Semiconductor EuS Nanocrystals with Paramagnetic Transition-Metal Ions Yasuchika Hasegawa, Masashi Maeda, Takayuki Nakanishi, Yoshihiro Doi, Yukio Hinatsu, Koji Fujita, Katsuhisa Tanaka, Hitoshi Koizumi, and Koji Fushimi pp 2659–2666 DOI: 10.1021/ja3106253 Supporting Info |
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Molecular Recognition of Complex-Type Biantennary N-Glycans by Protein Receptors: a Three-Dimensional View on Epitope Selection by NMR Ana Ardá, Pilar Blasco, Daniel Varón Silva, Volker Schubert, Sabine André, Marta Bruix, F. Javier Cañada, Hans-Joachim Gabius, Carlo Unverzagt, and Jesús Jiménez-Barbero pp 2667–2675 DOI: 10.1021/ja3104928 Supporting Info |
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Sensitizing Curium Luminescence through an Antenna Protein To Investigate Biological Actinide Transport Mechanisms Manuel Sturzbecher-Hoehne, Christophe Goujon, Gauthier J.-P. Deblonde, Anne B. Mason, and Rebecca J. Abergel pp 2676–2683 DOI: 10.1021/ja310957f Supporting Info |
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Formation of Diverse Supercrystals from Self-Assembly of a Variety of Polyhedral Gold Nanocrystals Ching-Wen Liao, Yeh-Sheng Lin, Kaushik Chanda, Yen-Fang Song, and Michael H. Huang pp 2684–2693 DOI: 10.1021/ja311008r Supporting Info |
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Principles of Sustained Enzymatic Hydrogen Oxidation in the Presence of Oxygen – The Crucial Influence of High Potential Fe–S Clusters in the Electron Relay of [NiFe]-Hydrogenases Rhiannon M. Evans, Alison Parkin, Maxie M. Roessler, Bonnie J. Murphy, Hope Adamson, Michael J. Lukey, Frank Sargent, Anne Volbeda, Juan C. Fontecilla-Camps, and Fraser A. Armstrong pp 2694–2707 DOI: 10.1021/ja311055d Supporting Info |
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Supramolecular Organization and Magnetic Properties of Mesogen-Hybridized Mixed-Valent Manganese Single Molecule Magnets [MnIII8MnIV4O12(Lx,y,z-CB)16(H2O)4] Emmanuel Terazzi, Guillaume Rogez, Jean-Louis Gallani, and Bertrand Donnio pp 2708–2722 DOI: 10.1021/ja311190a Supporting Info |
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Five Discrete Multinuclear Metal-Organic Assemblies from One Ligand: Deciphering the Effects of Different Templates Imogen A. Riddell, Yana R. Hristova, Jack K. Clegg, Christopher S. Wood, Boris Breiner, and Jonathan R. Nitschke pp 2723–2733 DOI: 10.1021/ja311285b Supporting Info |
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Freezing of Water Next to Solid Surfaces Probed by Infrared–Visible Sum Frequency Generation Spectroscopy Emmanuel Anim-Danso, Yu Zhang, Azar Alizadeh, and Ali Dhinojwala pp 2734–2740 DOI: 10.1021/ja311648q |
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Heterogeneous Catalysts Need Not Be so “Heterogeneous”: Monodisperse Pt Nanocrystals by Combining Shape-Controlled Synthesis and Purification by Colloidal Recrystallization Yijin Kang, Meng Li, Yun Cai, Matteo Cargnello, Rosa E. Diaz, Thomas R. Gordon, Noah L. Wieder, Radoslav R. Adzic, Raymond J. Gorte, Eric A. Stach, and Christopher B. Murray pp 2741–2747 DOI: 10.1021/ja3116839 Supporting Info |
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Structural Complexity Meets Transport and Magnetic Anisotropy in Single Crystalline Ln30Ru4Sn31 (Ln = Gd, Dy) Devin C. Schmitt, Neel Haldolaarachchige, Joseph Prestigiacomo, Amar Karki, David P. Young, Shane Stadler, Rongying Jin, and Julia Y. Chan pp 2748–2758 DOI: 10.1021/ja311779t Supporting Info |
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Self-Assembled Nanoscale DNA–Porphyrin Complex for Artificial Light Harvesting Jakob G. Woller, Jonas K. Hannestad, and Bo Albinsson pp 2759–2768 DOI: 10.1021/ja311828v Supporting Info |
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From Yellow to Black: Dramatic Changes between Cerium(IV) and Plutonium(IV) Molybdates Justin N. Cross, Patrick M. Duncan, Eric M. Villa, Matthew J. Polinski, Jean-Marie Babo, Evgeny V. Alekseev, Corwin H. Booth, and Thomas E. Albrecht-Schmitt pp 2769–2775 DOI: 10.1021/ja311910h Supporting Info |
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Crystal and Magnetic Structures and Physical Properties of a New Pyroxene NaMnGe2O6 Synthesized under High Pressure Jinguang Cheng, Wei Tian, Jianshi Zhou, Vincent M. Lynch, Hugo Steinfink, Arumugam Manthiram, Andrew F. May, Vasile O. Garlea, Joerg C. Neuefeind, and Jiaqiang Yan pp 2776–2786 DOI: 10.1021/ja312038g |
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Anomalous Manganese Activation of a Pyrophosphate Cathode in Sodium Ion Batteries: A Combined Experimental and Theoretical Study Chan Sun Park, Heejin Kim, Rana A. Shakoor, Eunjeong Yang, Soo Yeon Lim, Ramazan Kahraman, Yousung Jung, and Jang Wook Choi pp 2787–2792 DOI: 10.1021/ja312044k Supporting Info |
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Bimetallic Cyanide-Bridged Coordination Polymers as Lithium Ion Cathode Materials: Core@Shell Nanoparticles with Enhanced Cyclability Daisuke Asakura, Carissa H. Li, Yoshifumi Mizuno, Masashi Okubo, Haoshen Zhou, and Daniel R. Talham pp 2793–2799 DOI: 10.1021/ja312160v Supporting Info |
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Efficient Two-Electron Reduction of Dioxygen to Hydrogen Peroxide with One-Electron Reductants with a Small Overpotential Catalyzed by a Cobalt Chlorin Complex Kentaro Mase, Kei Ohkubo, and Shunichi Fukuzumi pp 2800–2808 DOI: 10.1021/ja312199h Supporting Info |
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Strong Correlation between Molecular Configurations and Charge-Transfer Processes Probed at the Single-Molecule Level by Surface-Enhanced Raman Scattering Emiliano Cortés, Pablo G. Etchegoin, Eric C. Le Ru, Alejandro Fainstein, María E. Vela, and Roberto C. Salvarezza pp 2809–2815 DOI: 10.1021/ja312236y |
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High-Resolution Insight into G-Overhang Architecture Robert Hänsel, Frank Löhr, Lukáš Trantirek, and Volker Dötsch pp 2816–2824 DOI: 10.1021/ja312403b Supporting Info |
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Temperature-Independent Catalytic Two-Electron Reduction of Dioxygen by Ferrocenes with a Copper(II) Tris[2-(2-pyridyl)ethyl]amine Catalyst in the Presence of Perchloric Acid Dipanwita Das, Yong-Min Lee, Kei Ohkubo, Wonwoo Nam, Kenneth D. Karlin, and Shunichi Fukuzumi pp 2825–2834 DOI: 10.1021/ja312523u Supporting Info |
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Cis–Trans Amide Bond Rotamers in β-Peptoids and Peptoids: Evaluation of Stereoelectronic Effects in Backbone and Side Chains Jonas S. Laursen, Jens Engel-Andreasen, Peter Fristrup, Pernille Harris, and Christian A. Olsen pp 2835–2844 DOI: 10.1021/ja312532x Supporting Info |
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Free Fructose Is Conformationally Locked Emilio J. Cocinero, Alberto Lesarri, Patricia Écija, Álvaro Cimas, Benjamin G. Davis, Francisco J. Basterretxea, José A. Fernández, and Fernando Castaño pp 2845–2852 DOI: 10.1021/ja312393m Supporting Info |
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Inhibition of Tau Filament Formation by Conformational Modulation Elias Akoury, Michal Gajda, Marcus Pickhardt, Jacek Biernat, Pornsuwan Soraya, Christian Griesinger, Eckhard Mandelkow, and Markus Zweckstetter pp 2853–2862 DOI: 10.1021/ja312471h Supporting Info |
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Correction to Cell-Selective Biological Activity of Rhodium Metalloinsertors Correlates with Subcellular Localization Alexis C. Komor, Curtis J. Schneider, Alyson G. Weidmann, and Jacqueline K. Barton pp 2863–2863 DOI: 10.1021/ja400471q |
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Correction to “Design and Characterization of Programmable DNA Nanotubes” Paul W. K. Rothemund, Axel Ekani-Nkodo, Nick Papadakis, Ashish Kumar, Deborah Kuchnir Fygenson, and Erik Winfree pp 2864–2864 DOI: 10.1021/ja400841u Supporting Info |
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Spotlights on Recent JACS Publications pp 2865–2866 DOI: 10.1021/ja401646m |
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On Terminal Alkynes That Can React with Active-Site Cysteine Nucleophiles in Proteases Reggy Ekkebus, Sander I. van Kasteren, Yogesh Kulathu, Arjen Scholten, Ilana Berlin, Paul P. Geurink, Annemieke de Jong, Soenita Goerdayal, Jacques Neefjes, Albert J. R. Heck, David Komander, and Huib Ovaa pp 2867–2870 DOI: 10.1021/ja309802n Supporting Info |
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Mapping Molecular Perturbations by a New Form of Two-Dimensional Spectroscopy E̅riks Kupče and Ray Freeman pp 2871–2874 DOI: 10.1021/ja310107e Supporting Info |
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Conjugation-Induced Fluorescent Labeling of Proteins and Polymers Using Dithiomaleimides Mathew P. Robin, Paul Wilson, Anne B. Mabire, Jenny K. Kiviaho, Jeffery E. Raymond, David M. Haddleton, and Rachel K. O’Reilly pp 2875–2878 DOI: 10.1021/ja3105494 Supporting Info |
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Site-Specific and Regiospecific Installation of Methylarginine Analogues into Recombinant Histones and Insights into Effector Protein Binding Daniel D. Le, Arianna T. Cortesi, Samuel A. Myers, Alma L. Burlingame, and Danica Galonić Fujimori pp 2879–2882 DOI: 10.1021/ja3108214 Supporting Info |
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Selective Tumor Cell Targeting by the Disaccharide Moiety of Bleomycin Zhiqiang Yu, Ryan M. Schmaltz, Trevor C. Bozeman, Rakesh Paul, Michael J. Rishel, Krystal S. Tsosie, and Sidney M. Hecht pp 2883–2886 DOI: 10.1021/ja311090e Supporting Info |
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Fluorescent Probes Reveal a Minimal Ligase Recognition Motif in the Prokaryotic Ubiquitin-like Protein from Mycobacterium tuberculosis Denis Smirnov, Abhinav Dhall, Kalkena Sivanesam, Rudy J. Sharar, and Champak Chatterjee pp 2887–2890 DOI: 10.1021/ja311376h Supporting Info |
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Effective Palladium-Catalyzed Hydroxycarbonylation of Aryl Halides with Substoichiometric Carbon Monoxide Signe Korsager, Rolf H. Taaning, and Troels Skrydstrup pp 2891–2894 DOI: 10.1021/ja3114032 Supporting Info |
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Raman Spectra of Interchanging β-Lactamase Inhibitor Intermediates on the Millisecond Time Scale Hossein Heidari Torkabadi, Tao Che, Jingjing Shou, Sivaprakash Shanmugam, Michael W. Crowder, Robert A. Bonomo, Marianne Pusztai-Carey, and Paul R. Carey pp 2895–2898 DOI: 10.1021/ja311440p Supporting Info |
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Hyperstability and Substrate Promiscuity in Laboratory Resurrections of Precambrian β-Lactamases Valeria A. Risso, Jose A. Gavira, Diego F. Mejia-Carmona, Eric A. Gaucher, and Jose M. Sanchez-Ruiz pp 2899–2902 DOI: 10.1021/ja311630a Supporting Info |
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Activatable Rotor for Quantifying Lysosomal Viscosity in Living Cells Lu Wang, Yi Xiao, Wenming Tian, and Liezheng Deng pp 2903–2906 DOI: 10.1021/ja311688g Supporting Info |
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Supramolecular Nanostructures Formed by Anticancer Drug Assembly Andrew G. Cheetham, Pengcheng Zhang, Yi-an Lin, Lye Lin Lock, and Honggang Cui pp 2907–2910 DOI: 10.1021/ja3115983 Supporting Info |
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Mallard Blue: A High-Affinity Selective Heparin Sensor That Operates in Highly Competitive Media Stephen M. Bromfield, Anna Barnard, Paola Posocco, Maurizio Fermeglia, Sabrina Pricl, and David K. Smith pp 2911–2914 DOI: 10.1021/ja311734d Supporting Info |
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Toward Understanding the Catalytic Synergy in the Design of Bimetallic Molecular Sieves for Selective Aerobic Oxidations Rebecca M. Leithall, Vasudev N. Shetti, Sara Maurelli, Mario Chiesa, Enrica Gianotti, and Robert Raja pp 2915–2918 DOI: 10.1021/ja3119064 Supporting Info |
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Minimal Peptide Motif for Non-covalent Peptide–Heparin Hydrogels Robert Wieduwild, Mikhail Tsurkan, Karolina Chwalek, Priyanka Murawala, Mirko Nowak, Uwe Freudenberg, Christoph Neinhuis, Carsten Werner, and Yixin Zhang pp 2919–2922 DOI: 10.1021/ja312022u Supporting Info |
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A Low-Overpotential Potassium–Oxygen Battery Based on Potassium Superoxide Xiaodi Ren and Yiying Wu pp 2923–2926 DOI: 10.1021/ja312059q Supporting Info |
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Synthesis and Activity of Biomimetic Biofilm Disruptors Thomas Böttcher, Ilana Kolodkin-Gal, Roberto Kolter, Richard Losick, and Jon Clardy pp 2927–2930 DOI: 10.1021/ja3120955 Supporting Info |
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Nano-Encrypted Morse Code: A Versatile Approach to Programmable and Reversible Nanoscale Assembly and Disassembly Ngo Yin Wong, Hang Xing, Li Huey Tan, and Yi Lu pp 2931–2934 DOI: 10.1021/ja3122284 Supporting Info |
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High-Field 13C Dynamic Nuclear Polarization with a Radical Mixture Vladimir K. Michaelis, Albert A. Smith, Björn Corzilius, Olesya Haze, Timothy M. Swager, and Robert G. Griffin pp 2935–2938 DOI: 10.1021/ja312265x Supporting Info |
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An Anodic Method for Covalent Attachment of Molecules to Electrodes through an Ethynyl Linkage Matthew V. Sheridan, Kevin Lam, and William E. Geiger pp 2939–2942 DOI: 10.1021/ja312405h Supporting Info |
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Site-Specific Interaction between α-Synuclein and Membranes Probed by NMR-Observed Methionine Oxidation Rates Alexander S. Maltsev, Jue Chen, Rodney L. Levine, and Ad Bax pp 2943–2946 DOI: 10.1021/ja312415q Supporting Info |
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Synthesis of Primary and Secondary Alkylboronates through Site-Selective C(sp3)–H Activation with Silica-Supported Monophosphine–Ir Catalysts Soichiro Kawamorita, Ryo Murakami, Tomohiro Iwai, and Masaya Sawamura pp 2947–2950 DOI: 10.1021/ja3126239 Supporting Info |
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Superconducting Phases in Potassium-Intercalated Iron Selenides Tianping Ying, Xiaolong Chen, Gang Wang, Shifeng Jin, Xiaofang Lai, Tingting Zhou, Han Zhang, Shijie Shen, and Wanyan Wang pp 2951–2954 DOI: 10.1021/ja312705x Supporting Info |
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Silver-Mediated Trifluoromethylation–Iodination of Arynes Yuwen Zeng, Laijun Zhang, Yanchuan Zhao, Chuanfa Ni, Jingwei Zhao, and Jinbo Hu pp 2955–2958 DOI: 10.1021/ja312711c Supporting Info |
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RCA Strands as Scaffolds To Create Nanoscale Shapes by a Few Staple Strands Yinzhou Ma, Hongning Zheng, Cuie Wang, Qin Yan, Jie Chao, Chunhai Fan, and Shou-Jun Xiao pp 2959–2962 DOI: 10.1021/ja400102s Supporting Info |
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Enantioselective Synthesis of Atropisomeric Benzamides through Peptide-Catalyzed Bromination Kimberly T. Barrett and Scott J. Miller pp 2963–2966 DOI: 10.1021/ja400082x Supporting Info |
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Molecular Imprinting of Luminescent Vesicles Supratim Banerjee and Burkhard König pp 2967–2970 DOI: 10.1021/ja4001568 Supporting Info |
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Modulating Cocaine Vaccine Potency through Hapten Fluorination Xiaoqing Cai, Kyoji Tsuchikama, and Kim D. Janda pp 2971–2974 DOI: 10.1021/ja400356g Supporting Info |
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Dynamic Nuclear Polarization Enhanced Natural Abundance 17O Spectroscopy Frédéric Blanc, Luke Sperrin, David A. Jefferson, Shane Pawsey, Melanie Rosay, and Clare P. Grey pp 2975–2978 DOI: 10.1021/ja4004377 Supporting Info |
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A Genetically Encoded AND Gate for Cell-Targeted Metabolic Labeling of Proteins Alborz Mahdavi, Thomas H. Segall-Shapiro, Songzi Kou, Granton A. Jindal, Kevin G. Hoff, Shirley Liu, Mohsen Chitsaz, Rustem F. Ismagilov, Jonathan J. Silberg, and David A. Tirrell pp 2979–2982 DOI: 10.1021/ja400448f Supporting Info |
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Highly Enantioselective Construction of Trifluoromethylated All-Carbon Quaternary Stereocenters via Nickel-Catalyzed Friedel–Crafts Alkylation Reaction Jian-Rong Gao, Hao Wu, Bin Xiang, Wu-Bin Yu, Liang Han, and Yi-Xia Jia pp 2983–2986 DOI: 10.1021/ja400650m Supporting Info |
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Toward a Silicon Version of Metathesis: From Schrock-Type Titanium Silylidenes to Silatitanacyclobutenes Vladimir Ya. Lee, Shinji Aoki, Taka Yokoyama, Satoru Horiguchi, Akira Sekiguchi, Heinz Gornitzka, Jing-Dong Guo, and Shigeru Nagase pp 2987–2990 DOI: 10.1021/ja401072j Supporting Info |
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Reactivity of Atomic Oxygen Radical Anions Bound to Titania and Zirconia Nanoparticles in the Gas Phase: Low-Temperature Oxidation of Carbon Monoxide Jia-Bi Ma, Bo Xu, Jing-Heng Meng, Xiao-Nan Wu, Xun-Lei Ding, Xiao-Na Li, and Sheng-Gui He pp 2991–2998 DOI: 10.1021/ja311695t Supporting Info |
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ATPase Active-Site Electrostatic Interactions Control the Global Conformation of the 100 kDa SecA Translocase Dorothy M. Kim, Haiyan Zheng, Yuanpeng J. Huang, Gaetano T. Montelione, and John F. Hunt pp 2999–3010 DOI: 10.1021/ja306361q Supporting Info |
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Controlled Integration of Gold Nanoparticles and Organic Fluorophores Using Synthetically Modified MS2 Viral Capsids Stacy L. Capehart, Michael P. Coyle, Jeff E. Glasgow, and Matthew B. Francis pp 3011–3016 DOI: 10.1021/ja3078472 Supporting Info |
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Giant Ising-Type Magnetic Anisotropy in Trigonal Bipyramidal Ni(II) Complexes: Experiment and Theory Renaud Ruamps, Rémi Maurice, Luke Batchelor, Martial Boggio-Pasqua, Régis Guillot, Anne Laure Barra, Junjie Liu, El-Eulmi Bendeif, Sébastien Pillet, Stephen Hill, Talal Mallah, and Nathalie Guihéry pp 3017–3026 DOI: 10.1021/ja308146e Supporting Info |
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Three-Mode Electrochemical Sensing of Ultralow MicroRNA Levels Mahmoud Labib, Nasrin Khan, Shahrokh M. Ghobadloo, Jenny Cheng, John Paul Pezacki, and Maxim V. Berezovski pp 3027–3038 DOI: 10.1021/ja308216z Supporting Info |
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Supramolecular Architectures with π-Acidic 3,6-Bis(2-pyridyl)-1,2,4,5-tetrazine Cavities: Role of Anion−π Interactions in the Remarkable Stability of Fe(II) Metallacycles in Solution Helen T. Chifotides, Ian D. Giles, and Kim R. Dunbar pp 3039–3055 DOI: 10.1021/ja3082473 Supporting Info |
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Contrasting Photophysical Properties of Star-Shaped vs Linear Perylene Diimide Complexes Christopher M. Pochas, Kurt A. Kistler, Hajime Yamagata, Spiridoula Matsika, and Frank C. Spano pp 3056–3066 DOI: 10.1021/ja3087449 Supporting Info |
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It Is the Outside That Counts: Chemical and Physical Control of Dynamic Surfaces Sarah M. Brosnan, Andrew H. Brown, and Valerie Sheares Ashby pp 3067–3072 DOI: 10.1021/ja308080g Supporting Info |
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Strong Effects of Cluster Size and Air Exposure on Oxygen Reduction and Carbon Oxidation Electrocatalysis by Size-Selected Ptn (n ≤ 11) on Glassy Carbon Electrodes Sebastian Proch, Mark Wirth, Henry S. White, and Scott L. Anderson pp 3073–3086 DOI: 10.1021/ja309868z Supporting Info |
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Temperature Sculpting in Yoctoliter Volumes Joseph E. Reiner, Joseph W. F. Robertson, Daniel L. Burden, Lisa K. Burden, Arvind Balijepalli, and John J. Kasianowicz pp 3087–3094 DOI: 10.1021/ja309892e Supporting Info |
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Visible Light-Driven O2 Reduction by a Porphyrin–Laccase System Theodore Lazarides, Igor V. Sazanovich, A. Jalila Simaan, Maria Chrisanthi Kafentzi, Milan Delor, Yasmina Mekmouche, Bruno Faure, Marius Réglier, Julia A. Weinstein, Athanassios G. Coutsolelos, and Thierry Tron pp 3095–3103 DOI: 10.1021/ja309969s Supporting Info |
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Oriented Protein Immobilization using Covalent and Noncovalent Chemistry on a Thiol-Reactive Self-Reporting Surface Dorothee Wasserberg, Carlo Nicosia, Eldrich E. Tromp, Vinod Subramaniam, Jurriaan Huskens, and Pascal Jonkheijm pp 3104–3111 DOI: 10.1021/ja3102133 Supporting Info |
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Evidence for Cardiolipin Binding Sites on the Membrane-Exposed Surface of the Cytochrome bc1 Clement Arnarez, Jean-Pierre Mazat, Juan Elezgaray, Siewert-J Marrink, and Xavier Periole pp 3112–3120 DOI: 10.1021/ja310577u Supporting Info |
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Hydroxyl Ion Addition to One-Electron Oxidized Thymine: Unimolecular Interconversion of C5 to C6 OH-Adducts Amitava Adhikary, Anil Kumar, Alicia N. Heizer, Brian J. Palmer, Venkata Pottiboyina, Yong Liang, Stanislaw F. Wnuk, and Michael D. Sevilla pp 3121–3135 DOI: 10.1021/ja310650n Supporting Info |
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Microfluidic Screening of Electrophoretic Mobility Shifts Elucidates Riboswitch Binding Function Kelly Karns, Jacob M. Vogan, Qian Qin, Scott F. Hickey, Stephen C. Wilson, Ming C. Hammond, and Amy E. Herr pp 3136–3143 DOI: 10.1021/ja310742m Supporting Info |
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Genetically Encoded Copper(I) Reporters with Improved Response for Use in Imaging Jun Liu, Jason Karpus, Seraphine V. Wegner, Peng R. Chen, and Chuan He pp 3144–3149 DOI: 10.1021/ja3106779 Supporting Info |
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Hydrophobic Interaction Drives Surface-Assisted Epitaxial Assembly of Amyloid-like Peptides Seung-gu Kang, Tien Huynh, Zhen Xia, Yi Zhang, Haiping Fang, Guanghong Wei, and Ruhong Zhou pp 3150–3157 DOI: 10.1021/ja310989u Supporting Info |
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Effect of Doping on the Magnetostructural Ordered Phase of Iron Arsenides: A Comparative Study of the Resistivity Anisotropy in Doped BaFe2As2 with Doping into Three Different Sites Shigeyuki Ishida, Masamichi Nakajima, Tian Liang, Kunihiro Kihou, Chul-Ho Lee, Akira Iyo, Hiroshi Eisaki, Teruhisa Kakeshita, Yasuhide Tomioka, Toshimitsu Ito, and Shin-ichi Uchida pp 3158–3163 DOI: 10.1021/ja311174e |
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Unusual Negative Photochromism via a Short-Lived Imidazolyl Radical of 1,1′-Binaphthyl-Bridged Imidazole Dimer Sayaka Hatano, Takeru Horino, Atsuhiro Tokita, Toyoji Oshima, and Jiro Abe pp 3164–3172 DOI: 10.1021/ja311344u Supporting Info |
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Fully Convergent Chemical Synthesis of Ester Insulin: Determination of the High Resolution X-ray Structure by Racemic Protein Crystallography Michal Avital-Shmilovici, Kalyaneswar Mandal, Zachary P. Gates, Nelson B. Phillips, Michael A. Weiss, and Stephen B. H. Kent pp 3173–3185 DOI: 10.1021/ja311408y Supporting Info |
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Cis–Trans Isomerizations of Proline Residues Are Key to Bradykinin Conformations Nicholas A. Pierson, Liuxi Chen, David H. Russell, and David E. Clemmer pp 3186–3192 DOI: 10.1021/ja3114505 Supporting Info |
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Evidence for Metal–Surface Interactions and Their Role in Stabilizing Well-Defined Immobilized Ru–NHC Alkene Metathesis Catalysts Manoja K. Samantaray, Johan Alauzun, David Gajan, Santosh Kavitake, Ahmad Mehdi, Laurent Veyre, Moreno Lelli, Anne Lesage, Lyndon Emsley, Christophe Copéret, and Chloé Thieuleux pp 3193–3199 DOI: 10.1021/ja311722k Supporting Info |
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Surface Facet of Palladium Nanocrystals: A Key Parameter to the Activation of Molecular Oxygen for Organic Catalysis and Cancer Treatment Ran Long, Keke Mao, Xiaodong Ye, Wensheng Yan, Yaobing Huang, Jianyong Wang, Yao Fu, Xisheng Wang, Xiaojun Wu, Yi Xie, and Yujie Xiong pp 3200–3207 DOI: 10.1021/ja311739v Supporting Info |
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Quantum Dots as Templates for Self-Assembly of Photoswitchable Polymers: Small, Dual-Color Nanoparticles Capable of Facile Photomodulation Sebastián A. Díaz, Luciana Giordano, Julio C. Azcárate, Thomas M. Jovin, and Elizabeth A. Jares-Erijman pp 3208–3217 DOI: 10.1021/ja3117813 |
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Microfluidic Mixing Triggered by an External LED Illumination Anna Venancio-Marques, Fanny Barbaud, and Damien Baigl pp 3218–3223 DOI: 10.1021/ja311837r Supporting Info |
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Diniobium Inverted Sandwich Complexes with μ-η6:η6-Arene Ligands: Synthesis, Kinetics of Formation, and Electronic Structure Thomas L. Gianetti, Grégory Nocton, Stefan G. Minasian, Neil C. Tomson, A. L. David Kilcoyne, Stosh A. Kozimor, David K. Shuh, Tolek Tyliszczak, Robert G. Bergman, and John Arnold pp 3224–3236 DOI: 10.1021/ja311966h Supporting Info |
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Zwitterions and Unobserved Intermediates in Organocatalytic Diels–Alder Reactions of Linear and Cross-Conjugated Trienamines Arne Dieckmann, Martin Breugst, and K. N. Houk pp 3237–3242 DOI: 10.1021/ja312043g Supporting Info |
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Total Syntheses of Lyconadins A–C Takuya Nishimura, Aditya K. Unni, Satoshi Yokoshima, and Tohru Fukuyama pp 3243–3247 DOI: 10.1021/ja312065m Supporting Info |
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Picosecond Binding of the His Ligand to Four-Coordinate Heme in Cytochrome c′: A One-Way Gate for Releasing Proximal NO Byung-Kuk Yoo, Isabelle Lamarre, Jean-Louis Martin, Colin R. Andrew, and Michel Negrerie pp 3248–3254 DOI: 10.1021/ja312140f |
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Filming the Birth of Molecules and Accompanying Solvent Rearrangement Jae Hyuk Lee, Michael Wulff, Savo Bratos, Jakob Petersen, Laurent Guerin, Jean-Claude Leicknam, Marco Cammarata, Qingyu Kong, Jeongho Kim, Klaus B. Møller, and Hyotcherl Ihee pp 3255–3261 DOI: 10.1021/ja312513w Supporting Info |
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Iodine (I2) as a Janus-Faced Ligand in Organometallics Andrey Yu. Rogachev and Roald Hoffmann pp 3262–3275 DOI: 10.1021/ja312584u Supporting Info |
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Fragmentation Energetics of Clusters Relevant to Atmospheric New Particle Formation Bryan R. Bzdek, Joseph W. DePalma, Douglas P. Ridge, Julia Laskin, and Murray V. Johnston pp 3276–3285 DOI: 10.1021/ja3124509 Supporting Info |
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Comparison of High-Spin and Low-Spin Nonheme FeIII–OOH Complexes in O–O Bond Homolysis and H-Atom Abstraction Reactivities Lei V. Liu, Seungwoo Hong, Jaeheung Cho, Wonwoo Nam, and Edward I. Solomon pp 3286–3299 DOI: 10.1021/ja400183g Supporting Info |
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Correction to Improved Ruthenium Catalysts for Z-Selective Olefin Metathesis Benjamin K. Keitz, Koji Endo, Paresma R. Patel, Myles B. Herbert, and Robert H. Grubbs pp 3300–3300 DOI: 10.1021/ja3119288 Supporting Info |
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Spotlights on Recent JACS Publications pp 3301–3302 DOI: 10.1021/ja401902h |
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Retention or Inversion in Stereospecific Nickel-Catalyzed Cross-Coupling of Benzylic Carbamates with Arylboronic Esters: Control of Absolute Stereochemistry with an Achiral Catalyst Michael R. Harris, Luke E. Hanna, Margaret A. Greene, Curtis E. Moore, and Elizabeth R. Jarvo pp 3303–3306 DOI: 10.1021/ja311783k Supporting Info |
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Nickel-Catalyzed Cross-Couplings of Benzylic Pivalates with Arylboroxines: Stereospecific Formation of Diarylalkanes and Triarylmethanes Qi Zhou, Harathi D. Srinivas, Srimoyee Dasgupta, and Mary P. Watson pp 3307–3310 DOI: 10.1021/ja312087x Supporting Info |
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Reactions of All Escherichia coli Lytic Transglycosylases with Bacterial Cell Wall Mijoon Lee, Dusan Hesek, Leticia I. Llarrull, Elena Lastochkin, Hualiang Pi, Bill Boggess, and Shahriar Mobashery pp 3311–3314 DOI: 10.1021/ja309036q Supporting Info |
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Nitrogen-Doped Fullerene as a Potential Catalyst for Hydrogen Fuel Cells Feng Gao, Guang-Lin Zhao, Shizhong Yang, and James J. Spivey pp 3315–3318 DOI: 10.1021/ja309042m Supporting Info |
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Controlling Formation of Single-Molecule Junctions by Electrochemical Reduction of Diazonium Terminal Groups Thomas Hines, Ismael Díez-Pérez, Hisao Nakamura, Tomomi Shimazaki, Yoshihiro Asai, and Nongjian Tao pp 3319–3322 DOI: 10.1021/ja3106434 Supporting Info |
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Chiral Gold Complex-Catalyzed Hetero-Diels–Alder Reaction of Diazenes: Highly Enantioselective and General for Dienes Bin Liu, Kang-Nan Li, Shi-Wei Luo, Jian-Zhou Huang, Huan Pang, and Liu-Zhu Gong pp 3323–3326 DOI: 10.1021/ja3110472 Supporting Info |
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Ruthenium Hydride-Promoted Dienyl Isomerization: Access to Highly Substituted 1,3-Dienes Joseph R. Clark, Justin R. Griffiths, and Steven T. Diver pp 3327–3330 DOI: 10.1021/ja4011207 Supporting Info |
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Simple and Highly Z-Selective Ruthenium-Based Olefin Metathesis Catalyst Giovanni Occhipinti, Fredrik R. Hansen, Karl W. Törnroos, and Vidar R. Jensen pp 3331–3334 DOI: 10.1021/ja311505v Supporting Info |
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Reversible Assembly of Stacked Membrane Nanodiscs with Reduced Dimensionality and Variable Periodicity Paul A. Beales, Nienke Geerts, Krishna K. Inampudi, Hideki Shigematsu, Corey J. Wilson, and T. Kyle Vanderlick pp 3335–3338 DOI: 10.1021/ja311561d Supporting Info |
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Synthesis of Nanostructured and Biofunctionalized Water-in-Oil Droplets as Tools for Homing T Cells Ilia Platzman, Jan-Willi Janiesch, and Joachim Pius Spatz pp 3339–3342 DOI: 10.1021/ja311588c Supporting Info |
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Iron(II)-Catalyzed Intramolecular Aminohydroxylation of Olefins with Functionalized Hydroxylamines Guan-Sai Liu, Yong-Qiang Zhang, Yong-An Yuan, and Hao Xu pp 3343–3346 DOI: 10.1021/ja311923z Supporting Info |
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A Dynamic Combinatorial Approach for the Analysis of Weak Carbohydrate/Aromatic Complexes: Dissecting Facial Selectivity in CH/π Stacking Interactions Andrés G. Santana, Ester Jiménez-Moreno, Ana M. Gómez, Francisco Corzana, Carlos González, Gonzalo Jiménez-Oses, Jesus Jiménez-Barbero, and Juan Luis Asensio pp 3347–3350 DOI: 10.1021/ja3120218 Supporting Info |
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Enhanced Dipole Moments in Trimetallic Nitride Template Endohedral Metallofullerenes with the Pentalene Motif Jianyuan Zhang, Daniel W. Bearden, Tim Fuhrer, Liaosa Xu, Wujun Fu, Tianming Zuo, and Harry C. Dorn pp 3351–3354 DOI: 10.1021/ja312045t Supporting Info |
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Efficient and Stereoselective Nitration of Mono- and Disubstituted Olefins with AgNO2 and TEMPO Soham Maity, Srimanta Manna, Sujoy Rana, Togati Naveen, Arijit Mallick, and Debabrata Maiti pp 3355–3358 DOI: 10.1021/ja311942e Supporting Info |
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A Prodrug Resistance Mechanism Is Involved in Colibactin Biosynthesis and Cytotoxicity Carolyn A. Brotherton and Emily P. Balskus pp 3359–3362 DOI: 10.1021/ja312154m Supporting Info |
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Ordering a Dynamic Protein Via a Small-Molecule Stabilizer Ningkun Wang, Chinmay Y. Majmudar, William C. Pomerantz, Jessica K. Gagnon, Jack D. Sadowsky, Jennifer L. Meagher, Taylor K. Johnson, Jeanne A. Stuckey, Charles L. Brooks, III, James A. Wells, and Anna K. Mapp pp 3363–3366 DOI: 10.1021/ja3122334 Supporting Info |
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Membrane-Dependent Modulation of the mTOR Activator Rheb: NMR Observations of a GTPase Tethered to a Lipid-Bilayer Nanodisc Mohammad T. Mazhab-Jafari, Christopher B. Marshall, Peter B. Stathopulos, Yoshihiro Kobashigawa, Vuk Stambolic, Lewis E. Kay, Fuyuhiko Inagaki, and Mitsuhiko Ikura pp 3367–3370 DOI: 10.1021/ja312508w Supporting Info |
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Chiral Recognition and Kinetic Resolution of Aromatic Amines via Supramolecular Chiral Nanocapsules in Nonpolar Solvents Toshiyuki Kida, Takuya Iwamoto, Haruyasu Asahara, Tomoaki Hinoue, and Mitsuru Akashi pp 3371–3374 DOI: 10.1021/ja312367k Supporting Info |
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Iridium-Catalyzed C–H Borylation of Cyclopropanes Carl W. Liskey and John F. Hartwig pp 3375–3378 DOI: 10.1021/ja400103p Supporting Info |
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Mechanism of Electrolyte-Induced Brightening in Single-Wall Carbon Nanotubes Juan G. Duque, Laura Oudjedi, Jared J. Crochet, Sergei Tretiak, Brahim Lounis, Stephen K. Doorn, and Laurent Cognet pp 3379–3382 DOI: 10.1021/ja4001757 Supporting Info |
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Charge Transfer Dynamics between Photoexcited CdS Nanorods and Mononuclear Ru Water-Oxidation Catalysts Huan-Wei Tseng, Molly B. Wilker, Niels H. Damrauer, and Gordana Dukovic pp 3383–3386 DOI: 10.1021/ja400178g Supporting Info |
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Palladium(0)-Catalyzed Alkynylation of C(sp3)–H Bonds Jian He, Masayuki Wasa, Kelvin S. L. Chan, and Jin-Quan Yu pp 3387–3390 DOI: 10.1021/ja400648w Supporting Info |
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Simultaneous Occurrence of Three Different Valence Tautomers in meso-Vinylruthenium-Modified Zinc Porphyrin Radical Cations Jing Chen, Evelyn Wuttke, Walther Polit, Thomas Exner, and Rainer F. Winter pp 3391–3394 DOI: 10.1021/ja400673c Supporting Info |
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Twisted Aspirin Crystals Xiaoyan Cui, Andrew L. Rohl, Alexander Shtukenberg, and Bart Kahr pp 3395–3398 DOI: 10.1021/ja400833r |
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Migration Insertion Polymerization (MIP) of Cyclopentadienyldicarbonyldiphenylphosphinopropyliron (FpP): A New Concept for Main Chain Metal-Containing Polymers (MCPs) Xiaosong Wang, Kai Cao, Yibo Liu, Brian Tsang, and Sean Liew pp 3399–3402 DOI: 10.1021/ja400755e Supporting Info |
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A Transition Metal Lewis Acid/Base Triad System for Cooperative Substrate Binding Oscar Tutusaus, Chengbao Ni, and Nathaniel K. Szymczak pp 3403–3406 DOI: 10.1021/ja400962h Supporting Info |
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Photo- and Thermal-Induced Multistructural Transformation of 2-Phenylazolyl Chelate Boron Compounds Ying-Li Rao, Hazem Amarne, Leanne D. Chen, Matthew L. Brown, Nicholas J. Mosey, and Suning Wang pp 3407–3410 DOI: 10.1021/ja400917r Supporting Info |
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Catalytic Enantioselective Epoxidation of Tertiary Allylic and Homoallylic Alcohols José Luis Olivares-Romero, Zhi Li, and Hisashi Yamamoto pp 3411–3413 DOI: 10.1021/ja401182a Supporting Info |
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Isolation and X-ray Crystal Structures of Triarylphosphine Radical Cations Xiaobo Pan, Xiaoyu Chen, Tao Li, Yizhi Li, and Xinping Wang pp 3414–3417 DOI: 10.1021/ja4012113 Supporting Info |
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Hierarchical Assembly of Collagen Peptide Triple Helices into Curved Disks and Metal Ion-Promoted Hollow Spheres David E. Przybyla, Charles M. Rubert Pérez, Jeremy Gleaton, Vikas Nandwana, and Jean Chmielewski pp 3418–3422 DOI: 10.1021/ja307651e Supporting Info |
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Oxidation of Adenosine and Inosine: The Chemistry of 8-Oxo-7,8-dihydropurines, Purine Iminoquinones, and Purine Quinones as Observed by Ultrafast Spectroscopy Denis I. Nilov, Dmitry Y. Komarov, Maxim S. Panov, Kanykey E. Karabaeva, Andrey S. Mereshchenko, Alexander N. Tarnovsky, and R. Marshall Wilson pp 3423–3438 DOI: 10.1021/ja3068148 Supporting Info |
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Low-Temperature Processed Ga-Doped ZnO Coatings from Colloidal Inks Enrico Della Gaspera, Marco Bersani, Michela Cittadini, Massimo Guglielmi, Diego Pagani, Rodrigo Noriega, Saahil Mehra, Alberto Salleo, and Alessandro Martucci pp 3439–3448 DOI: 10.1021/ja307960z Supporting Info |
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Sequence-Selective Detection of Double-Stranded DNA Sequences Using Pyrrole–Imidazole Polyamide Microarrays Ishwar Singh, Christian Wendeln, Alasdair W. Clark, Jonathan M. Cooper, Bart Jan Ravoo, and Glenn A. Burley pp 3449–3457 DOI: 10.1021/ja309677h Supporting Info |
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Experimental and Theoretical Investigation of Molybdenum Carbide and Nitride as Catalysts for Ammonia Decomposition Weiqing Zheng, Thomas P. Cotter, Payam Kaghazchi, Timo Jacob, Benjamin Frank, Klaus Schlichte, Wei Zhang, Dang Sheng Su, Ferdi Schüth, and Robert Schlögl pp 3458–3464 DOI: 10.1021/ja309734u |
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Simultaneous Detection of ATP and GTP by Covalently Linked Fluorescent Ribonucleopeptide Sensors Shun Nakano, Masatora Fukuda, Tomoki Tamura, Reiko Sakaguchi, Eiji Nakata, and Takashi Morii pp 3465–3473 DOI: 10.1021/ja3097652 Supporting Info |
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In Vitro and Mechanistic Studies of an Antiamyloidogenic Self-Assembled Cyclic d,l-α-Peptide Architecture Michal Richman, Sarah Wilk, Marina Chemerovski, Sebastian K. T. S. Wärmländer, Anna Wahlström, Astrid Gräslund, and Shai Rahimipour pp 3474–3484 DOI: 10.1021/ja310064v Supporting Info |
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Recycling Nicotinamide. The Transition-State Structure of Human Nicotinamide Phosphoribosyltransferase Emmanuel S. Burgos, Mathew J. Vetticatt, and Vern L. Schramm pp 3485–3493 DOI: 10.1021/ja310180c Supporting Info |
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Photochemical Water Oxidation by Crystalline Polymorphs of Manganese Oxides: Structural Requirements for Catalysis David M. Robinson, Yong Bok Go, Michelle Mui, Graeme Gardner, Zhijuan Zhang, Daniel Mastrogiovanni, Eric Garfunkel, Jing Li, Martha Greenblatt, and G. Charles Dismukes pp 3494–3501 DOI: 10.1021/ja310286h Supporting Info |
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An Organometallic Building Block Approach To Produce a Multidecker 4f Single-Molecule Magnet Jennifer J. Le Roy, Matthew Jeletic, Serge I. Gorelsky, Ilia Korobkov, Liviu Ungur, Liviu F. Chibotaru, and Muralee Murugesu pp 3502–3510 DOI: 10.1021/ja310642h Supporting Info |
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Selective Extraction of N2 from Air by Diarylimine Iron Complexes Erika R. Bartholomew, Emily C. Volpe, Peter T. Wolczanski, Emil B. Lobkovsky, and Thomas R. Cundari pp 3511–3527 DOI: 10.1021/ja311021u Supporting Info |
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A Dynamic Structural Model of Expanded RNA CAG Repeats: A Refined X-ray Structure and Computational Investigations Using Molecular Dynamics and Umbrella Sampling Simulations Ilyas Yildirim, HaJeung Park, Matthew D. Disney, and George C. Schatz pp 3528–3538 DOI: 10.1021/ja3108627 Supporting Info |
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Thiolates Chemically Induce Redox Activation of BTZ043 and Related Potent Nitroaromatic Anti-Tuberculosis Agents Rohit Tiwari, Garrett C. Moraski, Viktor Krchňák, Patricia A. Miller, Mariangelli Colon-Martinez, Eliza Herrero, Allen G. Oliver, and Marvin J. Miller pp 3539–3549 DOI: 10.1021/ja311058q Supporting Info |
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Efficient General Procedure To Access a Diversity of Gold(0) Particles and Gold(I) Phosphine Complexes from a Simple HAuCl4 Source. Localization of Homogeneous/Heterogeneous System’s Interface and Field-Emission Scanning Electron Microscopy Study Sergey S. Zalesskiy, Alexander E. Sedykh, Alexey S. Kashin, and Valentine P. Ananikov pp 3550–3559 DOI: 10.1021/ja311258e Supporting Info |
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Catalytic Dehydrogenative Borylation of Terminal Alkynes by a SiNN Pincer Complex of Iridium Chun-I Lee, Jia Zhou, and Oleg V. Ozerov pp 3560–3566 DOI: 10.1021/ja311682c Supporting Info |
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Synthesis and Application of an Environmentally Insensitive Cy3-Based Arsenical Fluorescent Probe To Identify Adaptive Microbial Responses Involving Proximal Dithiol Oxidation Na Fu, Dian Su, John R. Cort, Baowei Chen, Yijia Xiong, Wei-Jun Qian, Allan E. Konopka, Diana J. Bigelow, and Thomas C. Squier pp 3567–3575 DOI: 10.1021/ja3117284 Supporting Info |
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Steering On-Surface Polymerization with Metal-Directed Template Tao Lin, Xue Song Shang, Jinne Adisoejoso, Pei Nian Liu, and Nian Lin pp 3576–3582 DOI: 10.1021/ja311890n Supporting Info |
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An Efficient and Faithful in Vitro Replication System for Threose Nucleic Acid Hanyang Yu, Su Zhang, Matthew R. Dunn, and John C. Chaput pp 3583–3591 DOI: 10.1021/ja3118703 Supporting Info |
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Chiral Sum Frequency Generation for In Situ Probing Proton Exchange in Antiparallel β-Sheets at Interfaces Li Fu, Dequan Xiao, Zhuguang Wang, Victor S. Batista, and Elsa C. Y. Yan pp 3592–3598 DOI: 10.1021/ja3119527 Supporting Info |
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Expanding the Chemical Structure Space of Opto-Electronic Molecular Materials: Unprecedented Push–Pull Chromophores by Reaction of a Donor-Substituted Tetracyanofulvene with Electron-Rich Alkynes Govindasamy Jayamurugan, Oliver Dumele, Jean-Paul Gisselbrecht, Corinne Boudon, W. Bernd Schweizer, Bruno Bernet, and François Diederich pp 3599–3606 DOI: 10.1021/ja312084s Supporting Info |
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High-Resolution Zero-Field NMR J-Spectroscopy of Aromatic Compounds John W. Blanchard, Micah P. Ledbetter, Thomas Theis, Mark C. Butler, Dmitry Budker, and Alexander Pines pp 3607–3612 DOI: 10.1021/ja312239v Supporting Info |
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Direct Observation of the Ion-Pair Dynamics at a Protein–DNA Interface by NMR Spectroscopy Kurtis M. Anderson, Alexandre Esadze, Mariappan Manoharan, Rafael Brüschweiler, David G. Gorenstein, and Junji Iwahara pp 3613–3619 DOI: 10.1021/ja312314b Supporting Info |
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Interdigitated Hydrogen Bonds: Electrophile Activation for Covalent Capture and Fluorescence Turn-On Detection of Cyanide Junyong Jo, András Olasz, Chun-Hsing Chen, and Dongwhan Lee pp 3620–3632 DOI: 10.1021/ja312313f Supporting Info |
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Isolation of a Mixed Valence Diiron Hydride: Evidence for a Spectator Hydride in Hydrogen Evolution Catalysis Wenguang Wang, Mark J. Nilges, Thomas B. Rauchfuss, and Matthias Stein pp 3633–3639 DOI: 10.1021/ja312458f Supporting Info |
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Mapping the Nucleotide Binding Site of Uncoupling Protein 1 Using Atomic Force Microscopy Rong Zhu, Anne Rupprecht, Andreas Ebner, Thomas Haselgrübler, Hermann J. Gruber, Peter Hinterdorfer, and Elena E. Pohl pp 3640–3646 DOI: 10.1021/ja312550k Supporting Info |
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White Light from a Single-Emitter Light-Emitting Electrochemical Cell Shi Tang, Junyou Pan, Herwig A. Buchholz, and Ludvig Edman pp 3647–3652 DOI: 10.1021/ja312548b |
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Preparation, Structure, and Electrochemistry of Layered Polyanionic Hydroxysulfates: LiMSO4OH (M = Fe, Co, Mn) Electrodes for Li-Ion Batteries Chinmayee V. Subban, Mohamed Ati, Gwenaëlle Rousse, Artem M. Abakumov, Gustaaf Van Tendeloo, Raphaël Janot, and Jean-Marie Tarascon pp 3653–3661 DOI: 10.1021/ja3125492 Supporting Info |
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Mechanistic Studies of the Oxygen Evolution Reaction Mediated by a Nickel–Borate Thin Film Electrocatalyst D. Kwabena Bediako, Yogesh Surendranath, and Daniel G. Nocera pp 3662–3674 DOI: 10.1021/ja3126432 Supporting Info |
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Photoresponsive Retinal-Modified Silk–Elastin Copolymer Zhongyuan Sun, Guokui Qin, Xiaoxia Xia, Mark Cronin-Golomb, Fiorenzo G. Omenetto, and David L. Kaplan pp 3675–3679 DOI: 10.1021/ja312647n Supporting Info |
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Surface-Induced Orientation Control of CuPc Molecules for the Epitaxial Growth of Highly Ordered Organic Crystals on Graphene Kai Xiao, Wan Deng, Jong K. Keum, Mina Yoon, Ivan V. Vlassiouk, Kendal W. Clark, An-Ping Li, Ivan I. Kravchenko, Gong Gu, Edward A. Payzant, Bobby G. Sumpter, Sean C. Smith, James F. Browning, and David B. Geohegan pp 3680–3687 DOI: 10.1021/ja3125096 Supporting Info |
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Surface-Enhanced Infrared Absorption Using Individual Cross Antennas Tailored to Chemical Moieties Lisa V. Brown, Ke Zhao, Nicholas King, Heidar Sobhani, Peter Nordlander, and Naomi J. Halas pp 3688–3695 DOI: 10.1021/ja312694g Supporting Info |
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Reduced Native State Stability in Crowded Cellular Environment Due to Protein–Protein Interactions Ryuhei Harada, Naoya Tochio, Takanori Kigawa, Yuji Sugita, and Michael Feig pp 3696–3701 DOI: 10.1021/ja3126992 Supporting Info |
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Extremely Long Nonradiative Relaxation of Photoexcited Graphane Is Greatly Accelerated by Oxidation: Time-Domain Ab Initio Study Tammie R. Nelson and Oleg V. Prezhdo pp 3702–3710 DOI: 10.1021/ja400033g |
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Structure and Chemistry of the Heteronuclear Oxo-Cluster [VPO4]•+: A Model System for the Gas-Phase Oxidation of Small Hydrocarbons Nicolas Dietl, Torsten Wende, Kai Chen, Ling Jiang, Maria Schlangen, Xinhao Zhang, Knut R. Asmis, and Helmut Schwarz pp 3711–3721 DOI: 10.1021/ja400198y Supporting Info |
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Sorption-Induced Structural Transition of Zeolitic Imidazolate Framework-8: A Hybrid Molecular Simulation Study Liling Zhang, Zhongqiao Hu, and Jianwen Jiang pp 3722–3728 DOI: 10.1021/ja401129h Supporting Info |
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Correction to “Nature’s Polyoxometalate Chemistry: X-ray structure of the Mo Storage Protein Loaded with Discrete Polynuclear Mo–O Clusters” Björn Kowalewski, Juliane Poppe, Ulrike Demmer, Eberhard Warkentin, Thomas Dierks, Ulrich Ermler, and Klaus Schneider pp 3729–3729 DOI: 10.1021/ja311281g Supporting Info |
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Correction to “Palladium-Catalyzed Chemo- and Enantioselective Oxidation of Allylic Esters and Carbonates” Barry M. Trost, Jeffery Richardson, and Kelvin Yong pp 3730–3730 DOI: 10.1021/ja312194k Supporting Info |
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Spotlights on Recent JACS Publications pp 3731–3732 DOI: 10.1021/ja4023122 |
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Stable Hydrogen Evolution from CdS-Modified CuGaSe2 Photoelectrode under Visible-Light Irradiation Makoto Moriya, Tsutomu Minegishi, Hiromu Kumagai, Masao Katayama, Jun Kubota, and Kazunari Domen pp 3733–3735 DOI: 10.1021/ja312653y Supporting Info |
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Unveiling Chemical Reactivity and Structural Transformation of Two-Dimensional Layered Nanocrystals Jae Hyo Han, Sujeong Lee, Dongwon Yoo, Jae-Hyun Lee, Sohee Jeong, Jin-Gyu Kim, and Jinwoo Cheon pp 3736–3739 DOI: 10.1021/ja309744c Supporting Info |
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Palladium-Catalyzed Direct Arylation of Methyl Sulfoxides with Aryl Halides Tiezheng Jia, Ana Bellomo, Kawtar EL Baina, Spencer D. Dreher, and Patrick J. Walsh pp 3740–3743 DOI: 10.1021/ja4009776 Supporting Info |
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Selective Growth of Dual-Color-Emitting Heterogeneous Microdumbbells Composed of Organic Charge-Transfer Complexes Yi Long Lei, Liang Sheng Liao, and Shuit Tong Lee pp 3744–3747 DOI: 10.1021/ja3114278 Supporting Info |
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Target-Responsive “Sweet” Hydrogel with Glucometer Readout for Portable and Quantitative Detection of Non-Glucose Targets Ling Yan, Zhi Zhu, Yuan Zou, Yishun Huang, Dewen Liu, Shasha Jia, Dunming Xu, Min Wu, Yu Zhou, Shuang Zhou, and Chaoyong James Yang pp 3748–3751 DOI: 10.1021/ja3114714 Supporting Info |
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Analysis and Refactoring of the A-74528 Biosynthetic Pathway Jay T. Fitzgerald, Louise K. Charkoudian, Katharine R. Watts, and Chaitan Khosla pp 3752–3755 DOI: 10.1021/ja311579s Supporting Info |
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Modular Pyridine Synthesis from Oximes and Enals through Synergistic Copper/Iminium Catalysis Ye Wei and Naohiko Yoshikai pp 3756–3759 DOI: 10.1021/ja312346s Supporting Info |
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Cu-Catalyzed Multicomponent Polymerization To Synthesize a Library of Poly(N-sulfonylamidines) In-Hwan Lee, Hyunseok Kim, and Tae-Lim Choi pp 3760–3763 DOI: 10.1021/ja312592e Supporting Info |
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In Situ Visualization of Self-Assembly of Charged Gold Nanoparticles Yuzi Liu, Xiao-Min Lin, Yugang Sun, and Tijana Rajh pp 3764–3767 DOI: 10.1021/ja312620e Supporting Info |
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Atomically Dispersed Au–(OH)x Species Bound on Titania Catalyze the Low-Temperature Water-Gas Shift Reaction Ming Yang, Lawrence F. Allard, and Maria Flytzani-Stephanopoulos pp 3768–3771 DOI: 10.1021/ja312646d Supporting Info |
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Organocatalytic C–H Bond Arylation of Aldehydes to Bis-heteroaryl Ketones Qiao Yan Toh, Andrew McNally, Silvia Vera, Nico Erdmann, and Matthew J. Gaunt pp 3772–3775 DOI: 10.1021/ja400051d Supporting Info |
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Tuning the Moenomycin Pharmacophore To Enable Discovery of Bacterial Cell Wall Synthesis Inhibitors Christian M. Gampe, Hirokazu Tsukamoto, Emma H. Doud, Suzanne Walker, and Daniel Kahne pp 3776–3779 DOI: 10.1021/ja4000933 Supporting Info |
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Quantitative Analysis of the Coverage Density of Br– Ions on Pd{100} Facets and Its Role in Controlling the Shape of Pd Nanocrystals Hsin-Chieh Peng, Shuifen Xie, Jinho Park, Xiaohu Xia, and Younan Xia pp 3780–3783 DOI: 10.1021/ja400301k Supporting Info |
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Bimetallic Coordination Insertion Polymerization of Unprotected Polar Monomers: Copolymerization of Amino Olefins and Ethylene by Dinickel Bisphenoxyiminato Catalysts Madalyn R. Radlauer, Aya K. Buckley, Lawrence M. Henling, and Theodor Agapie pp 3784–3787 DOI: 10.1021/ja4004816 Supporting Info |
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Modular Access to Complex Prodiginines: Total Synthesis of (+)-Roseophilin via its 2-Azafulvene Prototropisomer James H. Frederich and Patrick G. Harran pp 3788–3791 DOI: 10.1021/ja400473v Supporting Info |
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A Polar Copper–Boron One-Electron σ-Bond Marc-Etienne Moret, Limei Zhang, and Jonas C. Peters pp 3792–3795 DOI: 10.1021/ja4006578 Supporting Info |
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Successive C–C Coupling of Dienes to Vicinally Dioxygenated Hydrocarbons: Ruthenium Catalyzed [4 + 2] Cycloaddition across the Diol, Hydroxycarbonyl, or Dione Oxidation Levels Laina M. Geary, Ben W. Glasspoole, Mary M. Kim, and Michael J. Krische pp 3796–3799 DOI: 10.1021/ja400691t Supporting Info |
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Synthesis of Gold Hexagonal Bipyramids Directed by Planar-Twinned Silver Triangular Nanoprisms Michelle L. Personick, Mark R. Langille, Jinsong Wu, and Chad A. Mirkin pp 3800–3803 DOI: 10.1021/ja400794q Supporting Info |
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Dinitrogen Reduction via Photochemical Activation of Heteroleptic Tris(cyclopentadienyl) Rare-Earth Complexes Megan E. Fieser, Jefferson E. Bates, Joseph W. Ziller, Filipp Furche, and William J. Evans pp 3804–3807 DOI: 10.1021/ja400664s Supporting Info |
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From a Remarkable Manifestation of Polar Effects in a Radical Fragmentation to the Convergent Synthesis of Highly Functionalized Ketones Laurent Debien and Samir Z. Zard pp 3808–3811 DOI: 10.1021/ja400831w Supporting Info |
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A Folding-Based Approach for the Luminescent Detection of a Short RNA Hairpin Cristina Penas, Elena Pazos, José L. Mascareñas, and M. Eugenio Vázquez pp 3812–3814 DOI: 10.1021/ja400270a Supporting Info |
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Patchy Supramolecules as Versatile Tools To Probe Hydrophobicity in Nanoglobular Systems Luis M. Negrón, Yazmary Meléndez-Contés, and José M. Rivera pp 3815–3817 DOI: 10.1021/ja401373h Supporting Info |
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Carbonyl Sulfide Hydrolase from Thiobacillus thioparus Strain THI115 Is One of the β-Carbonic Anhydrase Family Enzymes Takahiro Ogawa, Keiichi Noguchi, Masahiko Saito, Yoshiko Nagahata, Hiromi Kato, Akashi Ohtaki, Hiroshi Nakayama, Naoshi Dohmae, Yasuhiko Matsushita, Masafumi Odaka, Masafumi Yohda, Hiroshi Nyunoya, and Yoko Katayama pp 3818–3825 DOI: 10.1021/ja307735e Supporting Info |
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Utilizing Redox-Mediated Bergman Cyclization toward the Development of Dual-Action Metalloenediyne Therapeutics Sarah E. Lindahl, Hyunsoo Park, Maren Pink, and Jeffrey M. Zaleski pp 3826–3833 DOI: 10.1021/ja308190q Supporting Info |
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Measurement of Electron Transfer through Cytochrome P450 Protein on Nanopillars and the Effect of Bound Substrates John E. Jett, David Lederman, Lance A. Wollenberg, Debin Li, Darcy R. Flora, Christopher D. Bostick, Timothy S. Tracy, and Peter M. Gannett pp 3834–3840 DOI: 10.1021/ja309104g Supporting Info |
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Oxo-Functionalization and Reduction of the Uranyl Ion through Lanthanide-Element Bond Homolysis: Synthetic, Structural, and Bonding Analysis of a Series of Singly Reduced Uranyl–Rare Earth 5f1-4fn Complexes Polly L. Arnold, Emmalina Hollis, Gary S. Nichol, Jason B. Love, Jean-Christophe Griveau, Roberto Caciuffo, Nicola Magnani, Laurent Maron, Ludovic Castro, Ahmed Yahia, Samuel O. Odoh, and Georg Schreckenbach pp 3841–3854 DOI: 10.1021/ja308993g Supporting Info |
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Enzymatic Single-Molecule Kinetic Isotope Effects Christopher R. Pudney, Richard S. K. Lane, Alistair J. Fielding, Steven W. Magennis, Sam Hay, and Nigel S. Scrutton pp 3855–3864 DOI: 10.1021/ja309286r Supporting Info |
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The Dynamic Structure of α-Synuclein Multimers Thomas Gurry, Orly Ullman, Charles K. Fisher, Iva Perovic, Thomas Pochapsky, and Collin M. Stultz pp 3865–3872 DOI: 10.1021/ja310518p Supporting Info |
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Pseudo-Single-Crystal Electrochemistry on Polycrystalline Electrodes: Visualizing Activity at Grains and Grain Boundaries on Platinum for the Fe2+/Fe3+ Redox Reaction Barak D. B. Aaronson, Chang-Hui Chen, Hongjiao Li, Marc T. M. Koper, Stanley C. S. Lai, and Patrick R. Unwin pp 3873–3880 DOI: 10.1021/ja310632k Supporting Info |
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Asymmetric Catalysis at the Mesoscale: Gold Nanoclusters Embedded in Chiral Self-Assembled Monolayer as Heterogeneous Catalyst for Asymmetric Reactions Elad Gross, Jack H. Liu, Selim Alayoglu, Matthew A. Marcus, Sirine C. Fakra, F. Dean Toste, and Gabor A. Somorjai pp 3881–3886 DOI: 10.1021/ja310640b Supporting Info |
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Introducing Copper as Catalyst for Oxidative Alkane Dehydrogenation Ana Conde, Laia Vilella, David Balcells, M. Mar Díaz-Requejo, Agustí Lledós, and Pedro J. Pérez pp 3887–3896 DOI: 10.1021/ja310866k Supporting Info |
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Low-Potential Sodium Insertion in a NASICON-Type Structure through the Ti(III)/Ti(II) Redox Couple P. Senguttuvan, G. Rousse, M. E. Arroyo y de Dompablo, Hervé Vezin, J.-M. Tarascon, and M. R. Palacín pp 3897–3903 DOI: 10.1021/ja311044t Supporting Info |
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Oxidative Thymine Mutation in DNA: Water-Wire-Mediated Proton-Coupled Electron Transfer Robert N. Barnett, Joshy Joseph, Uzi Landman, and Gary B. Schuster pp 3904–3914 DOI: 10.1021/ja311282k Supporting Info |
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A Metal–Metal Bond in the Light-Induced State of [NiFe] Hydrogenases with Relevance to Hydrogen Evolution Mario Kampa, Maria-Eirini Pandelia, Wolfgang Lubitz, Maurice van Gastel, and Frank Neese pp 3915–3925 DOI: 10.1021/ja3115899 Supporting Info |
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Steady-State Catalytic Wave-Shapes for 2-Electron Reversible Electrocatalysts and Enzymes Vincent Fourmond, Carole Baffert, Kateryna Sybirna, Thomas Lautier, Abbas Abou Hamdan, Sébastien Dementin, Philippe Soucaille, Isabelle Meynial-Salles, Hervé Bottin, and Christophe Léger pp 3926–3938 DOI: 10.1021/ja311607s Supporting Info |
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Heterogeneous Electron Transfer from Dye-Sensitized Nanocrystalline TiO2 to [Co(bpy)3]3+: Insights Gained from Impedance Spectroscopy Yeru Liu, James R. Jennings, Shaik M. Zakeeruddin, Michael Grätzel, and Qing Wang pp 3939–3952 DOI: 10.1021/ja311743m Supporting Info |
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Between Superexchange and Hopping: An Intermediate Charge-Transfer Mechanism in Poly(A)-Poly(T) DNA Hairpins Nicolas Renaud, Yuri A. Berlin, Frederick D. Lewis, and Mark A. Ratner pp 3953–3963 DOI: 10.1021/ja3113998 Supporting Info |
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Enantioselective Synthesis of Multisubstituted Biaryl Skeleton by Chiral Phosphoric Acid Catalyzed Desymmetrization/Kinetic Resolution Sequence Keiji Mori, Yuki Ichikawa, Manato Kobayashi, Yukihiro Shibata, Masahiro Yamanaka, and Takahiko Akiyama pp 3964–3970 DOI: 10.1021/ja311902f Supporting Info |
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Si–H Activation in an Iridium Nitrido Complex—A Mechanistic and Theoretical Study Daniel Sieh and Peter Burger pp 3971–3982 DOI: 10.1021/ja311905h Supporting Info |
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Structural Determinants of Specific Lipid Binding to Potassium Channels Markus Weingarth, Alexander Prokofyev, Elwin A. W. van der Cruijsen, Deepak Nand, Alexandre M. J. J. Bonvin, Olaf Pongs, and Marc Baldus pp 3983–3988 DOI: 10.1021/ja3119114 Supporting Info |
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Efficient and Regioselective Ruthenium-catalyzed Hydro-aminomethylation of Olefins Lipeng Wu, Ivana Fleischer, Ralf Jackstell, and Matthias Beller pp 3989–3996 DOI: 10.1021/ja312271c Supporting Info |
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Insights into the Interplay of Lewis and Brønsted Acid Catalysts in Glucose and Fructose Conversion to 5-(Hydroxymethyl)furfural and Levulinic Acid in Aqueous Media Vinit Choudhary, Samir H. Mushrif, Christopher Ho, Andrzej Anderko, Vladimiros Nikolakis, Nebojsa S. Marinkovic, Anatoly I. Frenkel, Stanley I. Sandler, and Dionisios G. Vlachos pp 3997–4006 DOI: 10.1021/ja3122763 Supporting Info |
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Nitrite Reduction Mediated by Heme Models. Routes to NO and HNO? Julie L. Heinecke, Chosu Khin, Jose Clayston Melo Pereira, Sebastián A. Suárez, Alexei V. Iretskii, Fabio Doctorovich, and Peter C. Ford pp 4007–4017 DOI: 10.1021/ja312092x Supporting Info |
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Acid-Induced Mechanism Change and Overpotential Decrease in Dioxygen Reduction Catalysis with a Dinuclear Copper Complex Dipanwita Das, Yong-Min Lee, Kei Ohkubo, Wonwoo Nam, Kenneth D. Karlin, and Shunichi Fukuzumi pp 4018–4026 DOI: 10.1021/ja312256u Supporting Info |
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Mechanism of Assembly of the Dimanganese-Tyrosyl Radical Cofactor of Class Ib Ribonucleotide Reductase: Enzymatic Generation of Superoxide Is Required for Tyrosine Oxidation via a Mn(III)Mn(IV) Intermediate Joseph A. Cotruvo, Jr., Troy A. Stich, R. David Britt, and JoAnne Stubbe pp 4027–4039 DOI: 10.1021/ja312457t Supporting Info |
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Reversible Switching from Antiferro- to Ferromagnetic Behavior by Solvent-Mediated, Thermally-Induced Phase Transitions in a Trimorphic MOF-Based Magnetic Sponge System Mario Wriedt, Andrey A. Yakovenko, Gregory J. Halder, Andrey V. Prosvirin, Kim R. Dunbar, and Hong-Cai Zhou pp 4040–4050 DOI: 10.1021/ja312347p Supporting Info |
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Stepwise Construction of an Iron-Substituted Rigid-Rod Molecular Wire: Targeting a Tetraferra–Tetracosa–Decayne Franziska Lissel, Thomas Fox, Olivier Blacque, Walther Polit, Rainer F. Winter, Koushik Venkatesan, and Heinz Berke pp 4051–4060 DOI: 10.1021/ja400078c Supporting Info |
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Improving the Second-Order Nonlinear Optical Response of Fluorescent Proteins: The Symmetry Argument Evelien De Meulenaere, Ngan Nguyen Bich, Marc de Wergifosse, Kristof Van Hecke, Luc Van Meervelt, Jozef Vanderleyden, Benoît Champagne, and Koen Clays pp 4061–4069 DOI: 10.1021/ja400098b Supporting Info |
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Comprehensive Insights into the Structural and Chemical Changes in Mixed-Anion FeOF Electrodes by Using Operando PDF and NMR Spectroscopy Kamila M. Wiaderek, Olaf J. Borkiewicz, Elizabeth Castillo-Martínez, Rosa Robert, Nathalie Pereira, Glenn G. Amatucci, Clare P. Grey, Peter J. Chupas, and Karena W. Chapman pp 4070–4078 DOI: 10.1021/ja400229v Supporting Info |
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Universal Method for Protein Immobilization on Chemically Functionalized Germanium Investigated by ATR-FTIR Difference Spectroscopy Jonas Schartner, Jörn Güldenhaupt, Bastian Mei, Matthias Rögner, Martin Muhler, Klaus Gerwert, and Carsten Kötting pp 4079–4087 DOI: 10.1021/ja400253p Supporting Info |
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The “Catalytic Nitrosyl Effect”: NO Bending Boosting the Efficiency of Rhenium Based Alkene Hydrogenations Yanfeng Jiang, Birgitta Schirmer, Olivier Blacque, Thomas Fox, Stefan Grimme, and Heinz Berke pp 4088–4102 DOI: 10.1021/ja400135d Supporting Info |
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Azaaldol Condensation of a Lithium Enolate Solvated by N,N,N′,N′-Tetramethylethylenediamine: Dimer-Based 1,2-Addition to Imines Timothy S. De Vries, Angela M. Bruneau, Lara R. Liou, Hariharaputhiran Subramanian, and David B. Collum pp 4103–4109 DOI: 10.1021/ja400345c Supporting Info |
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Accordion-like Oscillation of Contracted and Stretched Helices of Polyacetylenes Synchronized with the Restricted Rotation of Side Chains Yoshiaki Yoshida, Yasuteru Mawatari, Asahi Motoshige, Ranko Motoshige, Toshifumi Hiraoki, Manfred Wagner, Klaus Müllen, and Masayoshi Tabata pp 4110–4116 DOI: 10.1021/ja4004987 Supporting Info |
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General Approach for Preparing Epidithiodioxopiperazines from Trioxopiperazine Precursors: Enantioselective Total Syntheses of (+)- and (−)-Gliocladine C, (+)-Leptosin D, (+)-T988C, (+)-Bionectin A, and (+)-Gliocladin A John E. DeLorbe, David Horne, Richard Jove, Steven M. Mennen, Sangkil Nam, Fang-Li Zhang, and Larry E. Overman pp 4117–4128 DOI: 10.1021/ja400315y Supporting Info |
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Transformation from Kinetically into Thermodynamically Controlled Self-Organization of Complex Helical Columns with 3D Periodicity Assembled from Dendronized Perylene Bisimides Virgil Percec, Hao-Jan Sun, Pawaret Leowanawat, Mihai Peterca, Robert Graf, Hans W. Spiess, Xiangbing Zeng, Goran Ungar, and Paul A. Heiney pp 4129–4148 DOI: 10.1021/ja400639q Supporting Info |
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Platinum-Modulated Cobalt Nanocatalysts for Low-Temperature Aqueous-Phase Fischer–Tropsch Synthesis Hang Wang, Wu Zhou, Jin-Xun Liu, Rui Si, Geng Sun, Meng-Qi Zhong, Hai-Yan Su, Hua-Bo Zhao, Jose A. Rodriguez, Stephen J. Pennycook, Juan-Carlos Idrobo, Wei-Xue Li, Yuan Kou, and Ding Ma pp 4149–4158 DOI: 10.1021/ja400771a Supporting Info |
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Correction to “EPR Spectroscopic Studies of the Fe–S Clusters in the O2-Tolerant [NiFe]-Hydrogenase Hyd-1 from Escherichia coli and Characterization of the Unique [4Fe–3S] Cluster by HYSCORE” Maxie M. Roessler, Rhiannon M. Evans, Rosalind A. Davies, Jeffrey Harmer, and Fraser A. Armstrong pp 4159–4159 DOI: 10.1021/ja312695k |
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Correction to “Combining Electron-Neutral Building Blocks with Intramolecular ‘Conformational Locks’ Affords Stable, High-Mobility P- and N-Channel Polymer Semiconductors” Hui Huang, Zhihua Chen, Rocio Ponce Ortiz, Christopher Newman, Hakan Usta, Sylvia Lou, Jangdae Youn, Yong-Young Noh, Kang-Jun Baeg, Lin X. Chen, Antonio Facchetti, and Tobin J. Marks pp 4160–4160 DOI: 10.1021/ja400834j |
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Spotlights on Recent JACS Publications pp 4161–4162 DOI: 10.1021/ja402559v |
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Synthesis and Properties of Two Cationic Narrow Band Gap Conjugated Polyelectrolytes Zachary B. Henson, Yuan Zhang, Thuc-Quyen Nguyen, Jung Hwa Seo, and Guillermo C. Bazan pp 4163–4166 DOI: 10.1021/ja400140d Supporting Info |
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Palladium-Catalyzed 1,4-Difunctionalization of Butadiene To Form Skipped Polyenes Matthew S. McCammant, Longyan Liao, and Matthew S. Sigman pp 4167–4170 DOI: 10.1021/ja3110544 Supporting Info |
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Structures and Comparative Characterization of Biosynthetic Gene Clusters for Cyanosporasides, Enediyne-Derived Natural Products from Marine Actinomycetes Amy L. Lane, Sang-Jip Nam, Takashi Fukuda, Kazuya Yamanaka, Christopher A. Kauffman, Paul R. Jensen, William Fenical, and Bradley S. Moore pp 4171–4174 DOI: 10.1021/ja311065v Supporting Info |
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Nonlinear Scaling of Surface Water Diffusion with Bulk Water Viscosity of Crowded Solutions John M. Franck, John A. Scott, and Songi Han pp 4175–4178 DOI: 10.1021/ja3112912 Supporting Info |
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Biocompatible, Functional Spheres Based on Oxidative Coupling Assembly of Green Tea Polyphenols Zhenhua Chen, Caihong Wang, Junze Chen, and Xudong Li pp 4179–4182 DOI: 10.1021/ja311374b Supporting Info |
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Extending the Limits of Precision Polymer Synthesis: Giant Polyphenylene Dendrimers in the Megadalton Mass Range Approaching Structural Perfection Thi-Thanh-Tam Nguyen, Martin Baumgarten, Ali Rouhanipour, Hans Joachim Räder, Ingo Lieberwirth, and Klaus Müllen pp 4183–4186 DOI: 10.1021/ja311430r Supporting Info |
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An Experimentally Observed Trimetallofullerene Sm3@Ih-C80: Encapsulation of Three Metal Atoms in a Cage without a Nonmetallic Mediator Wei Xu, Lai Feng, Matteo Calvaresi, Jia Liu, Yang Liu, Ben Niu, Zujin Shi, Yongfu Lian, and Francesco Zerbetto pp 4187–4190 DOI: 10.1021/ja400490u Supporting Info |
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A Homogeneous Chemiluminescent Immunoassay Method Hashem Akhavan-Tafti, Dean G. Binger, John J. Blackwood, Ying Chen, Richard S. Creager, Renuka de Silva, Robert A. Eickholt, Jose E. Gaibor, Richard S. Handley, Kenneth P. Kapsner, Senja K. Lopac, Michael E. Mazelis, Terri L. McLernon, James D. Mendoza, Bruce H. Odegaard, Sarada G. Reddy, Michael Salvati, Barry A. Schoenfelner, Nir Shapir, Katherine R. Shelly, Jeff C. Todtleben, Guoping Wang, and Wenhua Xie pp 4191–4194 DOI: 10.1021/ja312039k Supporting Info |
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MOF-Supported Selective Ethylene Dimerization Single-Site Catalysts through One-Pot Postsynthetic Modification Jerome Canivet, Sonia Aguado, Yves Schuurman, and David Farrusseng pp 4195–4198 DOI: 10.1021/ja312120x Supporting Info |
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Monodisperse and Inorganically Capped Sn and Sn/SnO2 Nanocrystals for High-Performance Li-Ion Battery Anodes Kostiantyn Kravchyk, Loredana Protesescu, Maryna I. Bodnarchuk, Frank Krumeich, Maksym Yarema, Marc Walter, Christoph Guntlin, and Maksym V. Kovalenko pp 4199–4202 DOI: 10.1021/ja312604r Supporting Info |
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Nanoscopic Cylindrical Dual Concentric and Lengthwise Block Brush Terpolymers as Covalent Preassembled High-Resolution and High-Sensitivity Negative-Tone Photoresist Materials Guorong Sun, Sangho Cho, Corrie Clark, Stanislav V. Verkhoturov, Michael J. Eller, Ang Li, Adriana Pavía-Jiménez, Emile A. Schweikert, James W. Thackeray, Peter Trefonas, and Karen L. Wooley pp 4203–4206 DOI: 10.1021/ja3126382 Supporting Info |
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Ionic Liquid as an Efficient Modulator on Artificial Enzyme System: Toward the Realization of High-Temperature Catalytic Reactions Youhui Lin, Andong Zhao, Yu Tao, Jinsong Ren, and Xiaogang Qu pp 4207–4210 DOI: 10.1021/ja400280f Supporting Info |
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Synthesis and Optical Properties of Stable Gallafluorene Derivatives: Investigation of Their Emission via Triplet States Takuya Matsumoto, Kazuo Tanaka, and Yoshiki Chujo pp 4211–4214 DOI: 10.1021/ja400287y Supporting Info |
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Designing a Deep-Ultraviolet Nonlinear Optical Material with a Large Second Harmonic Generation Response Hongping Wu, Hongwei Yu, Zhihua Yang, Xueling Hou, Xin Su, Shilie Pan, Kenneth R. Poeppelmeier, and James M. Rondinelli pp 4215–4218 DOI: 10.1021/ja400500m Supporting Info |
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Visible Light Driven Water Splitting in a Molecular Device with Unprecedentedly High Photocurrent Density Yan Gao, Xin Ding, Jianhui Liu, Lei Wang, Zhongkai Lu, Lin Li, and Licheng Sun pp 4219–4222 DOI: 10.1021/ja400402d Supporting Info |
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Total Synthesis of 6-Deoxyerythronolide B via C–C Bond-Forming Transfer Hydrogenation Xin Gao, Sang Kook Woo, and Michael J. Krische pp 4223–4226 DOI: 10.1021/ja4008722 Supporting Info |
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A Simple and Universal Gel Permeation Chromatography Technique for Precise Molecular Weight Characterization of Well-Defined Poly(ionic liquid)s Hongkun He, Mingjiang Zhong, Brian Adzima, David Luebke, Hunaid Nulwala, and Krzysztof Matyjaszewski pp 4227–4230 DOI: 10.1021/ja4012645 Supporting Info |
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Enantioselective Total Synthesis of Plectosphaeroic Acid B Salman Y. Jabri and Larry E. Overman pp 4231–4234 DOI: 10.1021/ja401423j Supporting Info |
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Mechanistic Insights on the ortho-Hydroxylation of Aromatic Compounds by Non-heme Iron Complex: A Computational Case Study on the Comparative Oxidative Ability of Ferric-Hydroperoxo and High-Valent FeIV═O and FeV═O Intermediates Azaj Ansari, Abhishek Kaushik, and Gopalan Rajaraman pp 4235–4249 DOI: 10.1021/ja307077f Supporting Info |
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Indirect Dynamics in a Highly Exoergic Substitution Reaction Jochen Mikosch, Jiaxu Zhang, Sebastian Trippel, Christoph Eichhorn, Rico Otto, Rui Sun, Wibe A. de Jong, Matthias Weidemüller, William L. Hase, and Roland Wester pp 4250–4259 DOI: 10.1021/ja308042v |
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Correlation Between Structural, Spectroscopic, and Reactivity Properties Within a Series of Structurally Analogous Metastable Manganese(III)–Alkylperoxo Complexes Michael K. Coggins, Vlad Martin-Diaconescu, Serena DeBeer, and Julie A. Kovacs pp 4260–4272 DOI: 10.1021/ja308915x Supporting Info |
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Coverage- and Temperature-Controlled Isomerization of an Imine Derivative on Au(111) Cornelius Gahl, Daniel Brete, Felix Leyssner, Matthias Koch, Erik R. McNellis, Johannes Mielke, Robert Carley, Leonhard Grill, Karsten Reuter, Petra Tegeder, and Martin Weinelt pp 4273–4281 DOI: 10.1021/ja309330e |
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Charge Photogeneration in Donor–Acceptor Conjugated Materials: Influence of Excess Excitation Energy and Chain Length Raphael Tautz, Enrico Da Como, Christian Wiebeler, Giancarlo Soavi, Ines Dumsch, Nils Fröhlich, Giulia Grancini, Sybille Allard, Ullrich Scherf, Giulio Cerullo, Stefan Schumacher, and Jochen Feldmann pp 4282–4290 DOI: 10.1021/ja309252a Supporting Info |
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Negative Ion Photoelectron Spectroscopy Confirms the Prediction that (CO)5 and (CO)6 Each Has a Singlet Ground State Xiaoguang Bao, David A. Hrovat, Weston Thatcher Borden, and Xue-Bin Wang pp 4291–4298 DOI: 10.1021/ja4005128 Supporting Info |
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Solvent and Pressure Effects on the Motions of Encapsulated Guests: Tuning the Flexibility of a Supramolecular Host Jeffrey S. Mugridge, Achim Zahl, Rudi van Eldik, Robert G. Bergman, and Kenneth N. Raymond pp 4299–4306 DOI: 10.1021/ja309949q Supporting Info |
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Probing the Magic Numbers of Aluminum–Magnesium Cluster Anions and Their Reactivity toward Oxygen Zhixun Luo, Cameron J. Grover, Arthur C. Reber, Shiv N. Khanna, and A. W. Castleman, Jr. pp 4307–4313 DOI: 10.1021/ja310467n Supporting Info |
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Guest Packing Motifs within a Supramolecular Nanocapsule and a Covalent Analogue Simin Liu, David H. Russell, Nathanael F. Zinnel, and Bruce C. Gibb pp 4314–4324 DOI: 10.1021/ja310741q Supporting Info |
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Differentiation of CC vs CXC Chemokine Dimers with GAG Octasaccharide Binding Partners: An Ion Mobility Mass Spectrometry Approach Youjin Seo, Armann Andaya, Christian Bleiholder, and Julie A. Leary pp 4325–4332 DOI: 10.1021/ja310915m Supporting Info |
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Proline Editing: A General and Practical Approach to the Synthesis of Functionally and Structurally Diverse Peptides. Analysis of Steric versus Stereoelectronic Effects of 4-Substituted Prolines on Conformation within Peptides Anil K. Pandey, Devan Naduthambi, Krista M. Thomas, and Neal J. Zondlo pp 4333–4363 DOI: 10.1021/ja3109664 Supporting Info |
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Proline Primed Helix Length as a Modulator of the Nuclear Receptor–Coactivator Interaction Sascha Fuchs, Hoang D. Nguyen, Trang T. P. Phan, Matthew F. Burton, Lidia Nieto, Ingrid J. de Vries-van Leeuwen, Andrea Schmidt, Monireh Goodarzifard, Stijn M. Agten, Rolf Rose, Christian Ottmann, Lech-Gustav Milroy, and Luc Brunsveld pp 4364–4371 DOI: 10.1021/ja311748r Supporting Info |
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The Prolyl Isomerase SlyD Is a Highly Efficient Enzyme but Decelerates the Conformational Folding of a Client Protein Gabriel Zoldák, Anne-Juliane Geitner, and Franz X. Schmid pp 4372–4379 DOI: 10.1021/ja311775a |
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Bicontinuous Zeolite Polymer Composite Membranes Prepared via Float Casting Ina Kiesow, Dawid Marczewski, Lutz Reinhardt, Marcel Mühlmann, Mario Possiwan, and Werner A. Goedel pp 4380–4388 DOI: 10.1021/ja311785f |
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Electrostatically Driven Second-Sphere Ligand Switch between High and Low Reorganization Energy Forms of Native Cytochrome c Damián Alvarez-Paggi, María A. Castro, Verónica Tórtora, Laura Castro, Rafael Radi, and Daniel H. Murgida pp 4389–4397 DOI: 10.1021/ja311786b Supporting Info |
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Understanding the Role of Defect Sites in Glucan Hydrolysis on Surfaces Oz M. Gazit and Alexander Katz pp 4398–4402 DOI: 10.1021/ja311918z Supporting Info |
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Structural Principles of RNA Catalysis in a 2′–5′ Lariat-Forming Ribozyme Teresa Carlomagno, Irene Amata, Luca Codutti, Melanie Falb, Jörg Fohrer, Pawel Masiewicz, and Bernd Simon pp 4403–4411 DOI: 10.1021/ja311868t Supporting Info |
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Iron Pyrite Thin Films Synthesized from an Fe(acac)3 Ink Sean Seefeld, Moritz Limpinsel, Yu Liu, Nima Farhi, Amanda Weber, Yanning Zhang, Nicholas Berry, Yon Joo Kwon, Craig L. Perkins, John C. Hemminger, Ruqian Wu, and Matt Law pp 4412–4424 DOI: 10.1021/ja311974n Supporting Info |
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Reactivity Models of Hydrogen Activation by Frustrated Lewis Pairs: Synergistic Electron Transfers or Polarization by Electric Field? Tibor András Rokob, Imre Bakó, András Stirling, Andrea Hamza, and Imre Pápai pp 4425–4437 DOI: 10.1021/ja312387q Supporting Info |
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Precise Sequence Control in Linear and Cyclic Copolymers of 2,5-Bis(2-thienyl)pyrrole and Aniline by DNA-Programmed Assembly Wen Chen and Gary B. Schuster pp 4438–4449 DOI: 10.1021/ja312507z Supporting Info |
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Dendrite-Free Lithium Deposition via Self-Healing Electrostatic Shield Mechanism Fei Ding, Wu Xu, Gordon L. Graff, Jian Zhang, Maria L. Sushko, Xilin Chen, Yuyan Shao, Mark H. Engelhard, Zimin Nie, Jie Xiao, Xingjiang Liu, Peter V. Sushko, Jun Liu, and Ji-Guang Zhang pp 4450–4456 DOI: 10.1021/ja312241y Supporting Info |
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EcdGHK Are Three Tailoring Iron Oxygenases for Amino Acid Building Blocks of the Echinocandin Scaffold Wei Jiang, Ralph A. Cacho, Grace Chiou, Neil K. Garg, Yi Tang, and Christopher T. Walsh pp 4457–4466 DOI: 10.1021/ja312572v Supporting Info |
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Visible Light Photocatalysis with c-WO3–x/WO3×H2O Nanoheterostructures In Situ Formed in Mesoporous Polycarbosilane-Siloxane Polymer Mahdi Seifollahi Bazarjani, Mirabbos Hojamberdiev, Koji Morita, Gangqiang Zhu, Gennady Cherkashinin, Claudia Fasel, Thomas Herrmann, Hergen Breitzke, Aleksander Gurlo, and Ralf Riedel pp 4467–4475 DOI: 10.1021/ja3126678 Supporting Info |
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Formation and Healing of Vacancies in Graphene Chemical Vapor Deposition (CVD) Growth Lu Wang, Xiuyun Zhang, Helen L.W. Chan, Feng Yan, and Feng Ding pp 4476–4482 DOI: 10.1021/ja312687a Supporting Info |
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Stereodivergent SN2@P Reactions of Borane Oxazaphospholidines: Experimental and Theoretical Studies Hester Zijlstra, Thierry León, Abel de Cózar, Célia Fonseca Guerra, Daniel Byrom, Antoni Riera, Xavier Verdaguer, and F. Matthias Bickelhaupt pp 4483–4491 DOI: 10.1021/ja400208t Supporting Info |
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High-Temperature and Pressure-Induced Ferroelectricity in Hydrogen-Bonded Supramolecular Crystals of Anilic Acids and 2,3-Di(2-pyridinyl)pyrazine Sachio Horiuchi, Reiji Kumai, and Yoshinori Tokura pp 4492–4500 DOI: 10.1021/ja400318v Supporting Info |
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Monolayered Nanodots of Transition Metal Oxides Keisuke Nakamura, Yuya Oaki, and Hiroaki Imai pp 4501–4508 DOI: 10.1021/ja400443a Supporting Info |
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Formation of Guanine-6-sulfonate from 6-Thioguanine and Singlet Oxygen: A Combined Theoretical and Experimental Study Xiaoran Zou, Hongmei Zhao, Youqing Yu, and Hongmei Su pp 4509–4515 DOI: 10.1021/ja400483j Supporting Info |
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Ordered Mesoporous Cobalt Oxide as Highly Efficient Oxygen Evolution Catalyst Jonathan Rosen, Gregory S. Hutchings, and Feng Jiao pp 4516–4521 DOI: 10.1021/ja400555q Supporting Info |
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Chemical Noise Produced by Equilibrium Adsorption/Desorption of Surface Pyridine at Au–Ag–Au Bimetallic Atom-Scale Junctions Studied by Fluctuation Spectroscopy Tai-Wei Hwang, Sean P. Branagan, and Paul W. Bohn pp 4522–4528 DOI: 10.1021/ja400567j Supporting Info |
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Self-Recognition of Structurally Identical, Rod-Shaped Macroions with Different Central Metal Atoms during Their Assembly Process Panchao Yin, Jin Zhang, Tao Li, Xiaobing Zuo, Jian Hao, Anna Marie Warner, Soma Chattopadhyay, Tomohiro Shibata, Yongge Wei, and Tianbo Liu pp 4529–4536 DOI: 10.1021/ja400656j Supporting Info |
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Suppression of Tumor Growth by Designed Dimeric Epidithiodiketopiperazine Targeting Hypoxia-Inducible Transcription Factor Complex Ramin Dubey, Michael D. Levin, Lajos Z. Szabo, Csaba F. Laszlo, Swati Kushal, Jason B. Singh, Philip Oh, Jan E. Schnitzer, and Bogdan Z. Olenyuk pp 4537–4549 DOI: 10.1021/ja400805b Supporting Info |
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π-Conjugated Heterotriangulene Macrocycles by Solution and Surface-supported Synthesis toward Honeycomb Networks Florian Schlütter, Frédéric Rossel, Milan Kivala, Volker Enkelmann, Jean-Paul Gisselbrecht, Pascal Ruffieux, Roman Fasel, and Klaus Müllen pp 4550–4557 DOI: 10.1021/ja400857g Supporting Info |
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Asymmetric Dearomatizing Spirolactonization of Naphthols Catalyzed by Spirobiindane-Based Chiral Hypervalent Iodine Species Toshifumi Dohi, Naoko Takenaga, Tomofumi Nakae, Yosuke Toyoda, Mikio Yamasaki, Motoo Shiro, Hiromichi Fujioka, Akinobu Maruyama, and Yasuyuki Kita pp 4558–4566 DOI: 10.1021/ja401074u Supporting Info |
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Gemcitabine–Coumarin–Biotin Conjugates: A Target Specific Theranostic Anticancer Prodrug Sukhendu Maiti, Nayoung Park, Ji Hye Han, Hyun Mi Jeon, Jae Hong Lee, Sankarprasad Bhuniya, Chulhun Kang, and Jong Seung Kim pp 4567–4572 DOI: 10.1021/ja401350x Supporting Info |
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Correction to “Small-Molecule Inducer of β Cell Proliferation Identified by High-Throughput Screening” Weijun Shen, Matthew S. Tremblay, Vishal A. Deshmukh, Weidong Wang, Christophe M. Filippi, George Harb, You-qing Zhang, Anwesh Kamireddy, Janine E. Baaten, Qihui Jin, Tom Wu, Jonathan G. Swoboda, Eric C. Peters, Charles Y. Cho, Jing Li, Bryan A. Laffitte, Peter McNamara, Richard Glynne, Xu Wu, Ann E. Herman, and Peter G. Schultz pp 4573–4573 DOI: 10.1021/ja401118g |
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Spotlights on Recent JACS Publications pp 4575–4575 DOI: 10.1021/ja402799z |
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Highly Enantioselective Rhodium-Catalyzed [2+2+2] Cycloaddition of Diynes to Sulfonimines Muriel Amatore, David Lebœuf, Max Malacria, Vincent Gandon, and Corinne Aubert pp 4576–4579 DOI: 10.1021/ja309301n Supporting Info |
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Caged Mono- and Divalent Ligands for Light-Assisted Disruption of PDZ Domain-Mediated Interactions Matthieu Sainlos, Wendy S. Iskenderian-Epps, Nelson B. Olivier, Daniel Choquet, and Barbara Imperiali pp 4580–4583 DOI: 10.1021/ja309870q Supporting Info |
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Ligand Conjugation of Chemically Exfoliated MoS2 Stanley S. Chou, Mrinmoy De, Jaemyung Kim, Segi Byun, Conner Dykstra, Jin Yu, Jiaxing Huang, and Vinayak P. Dravid pp 4584–4587 DOI: 10.1021/ja310929s Supporting Info |
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The Isolation of [Pd{OC(O)H}(H)(NHC)(PR3)] (NHC = N-Heterocyclic Carbene) and Its Role in Alkene and Alkyne Reductions Using Formic Acid Julie Broggi, Václav Jurčík, Olivier Songis, Albert Poater, Luigi Cavallo, Alexandra M. Z. Slawin, and Catherine S. J. Cazin pp 4588–4591 DOI: 10.1021/ja311087c Supporting Info |
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Direct Measurement of Electron Transfer through a Hydrogen Bond between Single Molecules Tomoaki Nishino, Nobuhiko Hayashi, and Phuc T. Bui pp 4592–4595 DOI: 10.1021/ja311463b Supporting Info |
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Artificial Z-Scheme Constructed with a Supramolecular Metal Complex and Semiconductor for the Photocatalytic Reduction of CO2 Keita Sekizawa, Kazuhiko Maeda, Kazunari Domen, Kazuhide Koike, and Osamu Ishitani pp 4596–4599 DOI: 10.1021/ja311541a Supporting Info |
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The Critical Role of Phosphate in Vanadium Phosphate Oxide for the Catalytic Activation and Functionalization of n-Butane to Maleic Anhydride Mu-Jeng Cheng and William A. Goddard, III pp 4600–4603 DOI: 10.1021/ja3115746 Supporting Info |
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Lab in a Tube: Ultrasensitive Detection of MicroRNAs at the Single-Cell Level and in Breast Cancer Patients Using Quadratic Isothermal Amplification Ruixue Duan, Xiaolei Zuo, Shutao Wang, Xiyun Quan, Dongliang Chen, Zhifei Chen, Lei Jiang, Chunhai Fan, and Fan Xia pp 4604–4607 DOI: 10.1021/ja311313b Supporting Info |
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Impact of Molecular Clustering inside Nanopores on Desorption Processes Manuel Tsotsalas, Pavel Hejcik, Kenji Sumida, Ziya Kalay, Shuhei Furukawa, and Susumu Kitagawa pp 4608–4611 DOI: 10.1021/ja312115x Supporting Info |
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Postsynthesis Modification of a Porous Coordination Polymer by LiCl To Enhance H+ Transport Satoshi Horike, Yusuke Kamitsubo, Munehiro Inukai, Tomohiro Fukushima, Daiki Umeyama, Tomoya Itakura, and Susumu Kitagawa pp 4612–4615 DOI: 10.1021/ja3122872 Supporting Info |
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The Fumagillin Biosynthetic Gene Cluster in Aspergillus fumigatus Encodes a Cryptic Terpene Cyclase Involved in the Formation of β-trans-Bergamotene Hsiao-Ching Lin, Yit-Heng Chooi, Sourabh Dhingra, Wei Xu, Ana M. Calvo, and Yi Tang pp 4616–4619 DOI: 10.1021/ja312503y Supporting Info |
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Redox-Activated Manganese-Based MR Contrast Agent Galen S. Loving, Shreya Mukherjee, and Peter Caravan pp 4620–4623 DOI: 10.1021/ja312610j Supporting Info |
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Role of Sodium Doping in Lead Chalcogenide Thermoelectrics Jiaqing He, Li-Dong Zhao, Jin-Cheng Zheng, Jeff W. Doak, Haijun Wu, Hui-Qiong Wang, Yeseul Lee, Chris Wolverton, Mercouri G. Kanatzidis, and Vinayak P. Dravid pp 4624–4627 DOI: 10.1021/ja312562d Supporting Info |
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Re/Mg Bimetallic Tandem Catalysis for [4+2] Annulation of Benzamides and Alkynes via C-H/N-H Functionalization Qiuzheng Tang, Dexin Xia, Xiqing Jin, Qing Zhang, Xiao-Qiang Sun, and Congyang Wang pp 4628–4631 DOI: 10.1021/ja400020e Supporting Info |
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Forming Cross-Linked Peptidoglycan from Synthetic Gram-Negative Lipid II Matthew D. Lebar, Tania J. Lupoli, Hirokazu Tsukamoto, Janine M. May, Suzanne Walker, and Daniel Kahne pp 4632–4635 DOI: 10.1021/ja312510m Supporting Info |
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Detection of Living Anionic Species in Polymerization Reactions Using Hyperpolarized NMR Youngbok Lee, Gyu Seong Heo, Haifeng Zeng, Karen L. Wooley, and Christian Hilty pp 4636–4639 DOI: 10.1021/ja4001008 Supporting Info |
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Silver-Catalyzed Radical Aminofluorination of Unactivated Alkenes in Aqueous Media Zhaodong Li, Liyan Song, and Chaozhong Li pp 4640–4643 DOI: 10.1021/ja400124t Supporting Info |
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Imaging of Nonuniform Motion of Single DNA Molecules Reveals the Kinetics of Varying-Field Isotachophoresis Shengquan Liu, Bailin Zhao, Dapeng Zhang, Cuiping Li, and Hailin Wang pp 4644–4647 DOI: 10.1021/ja400126b Supporting Info |
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Mild Copper-Mediated Fluorination of Aryl Stannanes and Aryl Trifluoroborates Yingda Ye and Melanie S. Sanford pp 4648–4651 DOI: 10.1021/ja400300g Supporting Info |
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Transannulation of 1-Sulfonyl-1,2,3-triazoles with Heterocumulenes Stepan Chuprakov, Sen Wai Kwok, and Valery V. Fokin pp 4652–4655 DOI: 10.1021/ja400350c Supporting Info |
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Linear Side Chains in Benzo[1,2-b:4,5-b′]dithiophene–Thieno[3,4-c]pyrrole-4,6-dione Polymers Direct Self-Assembly and Solar Cell Performance Clément Cabanetos, Abdulrahman El Labban, Jonathan A. Bartelt, Jessica D. Douglas, William R. Mateker, Jean M. J. Fréchet, Michael D. McGehee, and Pierre M. Beaujuge pp 4656–4659 DOI: 10.1021/ja400365b Supporting Info |
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Synthesis of Large Dendrimers with the Dimensions of Small Viruses Jongdoo Lim, Mauri Kostiainen, Jan Maly, Viviana C. P. da Costa, Onofrio Annunziata, Giovanni M. Pavan, and Eric E. Simanek pp 4660–4663 DOI: 10.1021/ja400432e Supporting Info |
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Metal Ions To Control the Morphology of Semiconductor Nanoparticles: Copper Selenide Nanocubes Wenhua Li, Reza Zamani, Maria Ibáñez, Doris Cadavid, Alexey Shavel, Joan Ramon Morante, Jordi Arbiol, and Andreu Cabot pp 4664–4667 DOI: 10.1021/ja400472m Supporting Info |
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Alkane C–H Insertion by Aryne Intermediates with a Silver Catalyst Sang Young Yun, Kung-Pern Wang, Nam-Kyu Lee, Phani Mamidipalli, and Daesung Lee pp 4668–4671 DOI: 10.1021/ja400477r Supporting Info |
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Uncovering the Mechanism of the Ag(I)/Persulfate-Catalyzed Cross-Coupling Reaction of Arylboronic Acids and Heteroarenes Niki R. Patel and Robert A. Flowers, II pp 4672–4675 DOI: 10.1021/ja400712g Supporting Info |
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A GTP Affinity Probe for Proteomics Highlights Flexibility in Purine Nucleotide Selectivity Elizabeth A. George Cisar, Nhan Nguyen, and Hugh Rosen pp 4676–4679 DOI: 10.1021/ja400839e Supporting Info |
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A New Strategy for Efficient Synthesis of Medium and Large Ring Lactones without High Dilution or Slow Addition Wanxiang Zhao, Zigang Li, and Jianwei Sun pp 4680–4683 DOI: 10.1021/ja400883q Supporting Info |
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Photoclickable Dendritic Molecular Glue: Noncovalent-to-Covalent Photochemical Transformation of Protein Hybrids Noriyuki Uchida, Kou Okuro, Yamato Niitani, Xiao Ling, Takayuki Ariga, Michio Tomishige, and Takuzo Aida pp 4684–4687 DOI: 10.1021/ja401059w Supporting Info |
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A New Nanotechnology Technique for Determining Drug Efficacy Using Targeted Plasmonically Enhanced Single Cell Imaging Spectroscopy Lauren A. Austin, Bin Kang, and Mostafa A. El-Sayed pp 4688–4691 DOI: 10.1021/ja4011145 Supporting Info |
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Catalytic Asymmetric Diaziridination Lennart Lykke, Kim Søholm Halskov, Bjørn Dreiø Carlsen, Victor X. Chen, and Karl Anker Jørgensen pp 4692–4695 DOI: 10.1021/ja401150m Supporting Info |
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Application of In Situ-Generated Rh-Bound Trimethylenemethane Variants to the Synthesis of 3,4-Fused Pyrroles Erica E. Schultz and Richmond Sarpong pp 4696–4699 DOI: 10.1021/ja401380d Supporting Info |
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Building Biologics by Chemical Synthesis: Practical Preparation of Di- and Triantennary N-Linked Glycoconjugates Maciej A. Walczak, Joji Hayashida, and Samuel J. Danishefsky pp 4700–4703 DOI: 10.1021/ja401385v Supporting Info |
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A Nanospheric Polyhydrido Copper Cluster of Elongated Triangular Orthobicupola Array: Liberation of H2 from Solar Energy Rajendra S. Dhayal, Jian-Hong Liao, Yan-Ru Lin, Ping-Kuei Liao, Samia Kahlal, Jean-Yves Saillard, and C. W. Liu pp 4704–4707 DOI: 10.1021/ja401576s Supporting Info |
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Synthesis of Substituted Pyridines from Cascade [1 + 5] Cycloaddition of Isonitriles to N-Formylmethyl-Substituted Enamides, Aerobic Oxidative Aromatization, and Acyl Transfer Reaction Chuan-Hu Lei, De-Xian Wang, Liang Zhao, Jieping Zhu, and Mei-Xiang Wang pp 4708–4711 DOI: 10.1021/ja401701x Supporting Info |
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N-Heterocyclic Carbene Ligands as Modulators of Luminescence in Three-Coordinate Gold(I) Complexes with Spectacular Quantum Yields Renso Visbal, Isaura Ospino, José M. López-de-Luzuriaga, Antonio Laguna, and M. Concepción Gimeno pp 4712–4715 DOI: 10.1021/ja401523x Supporting Info |
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Rhodium-Catalyzed Conversion of Furans to Highly Functionalized Pyrroles Brendan T. Parr, Samantha A. Green, and Huw M. L. Davies pp 4716–4718 DOI: 10.1021/ja401386z Supporting Info |
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Synthesis and Self-Assembly of Photonic Materials from Nanocrystalline Titania Sheets Jian Zhu, Jinguo Wang, Fujian Lv, Shengxiong Xiao, Colin Nuckolls, and Hexing Li pp 4719–4721 DOI: 10.1021/ja401334j Supporting Info |
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Formation of a Bifunctional Redox System Using Electrochemical Reduction of Platinum in Ferrocene Based Ionic Liquid and Its Reactivity with Aryldiazonium Jalal Ghilane and Jean-Christophe Lacroix pp 4722–4728 DOI: 10.1021/ja310889z |
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Native States of Fast-Folding Proteins Are Kinetic Traps Alex Dickson and Charles L. Brooks, III pp 4729–4734 DOI: 10.1021/ja311077u Supporting Info |
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Dynamics of Site Switching in DNA Polymerase Rajan Lamichhane, Svitlana Y. Berezhna, Joshua P. Gill, Edwin Van der Schans, and David P. Millar pp 4735–4742 DOI: 10.1021/ja311641b Supporting Info |
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A Theoretical Investigation on the Mechanism and Stereochemical Course of the Addition of (E)-2-Butenyltrimethylsilane to Acetaldehyde by Electrophilic and Nucleophilic Activation Larry M. Wolf and Scott E. Denmark pp 4743–4756 DOI: 10.1021/ja311889v Supporting Info |
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Tailor-Made Highly Luminescent and Ambipolar Transporting Organic Mixed Stacked Charge-Transfer Crystals: An Isometric Donor–Acceptor Approach Sang Kyu Park, Shinto Varghese, Jong H. Kim, Seong-Jun Yoon, Oh Kyu Kwon, Byeong-Kwan An, Johannes Gierschner, and Soo Young Park pp 4757–4764 DOI: 10.1021/ja312197b Supporting Info |
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A Supramolecular Janus Hyperbranched Polymer and Its Photoresponsive Self-Assembly of Vesicles with Narrow Size Distribution Yong Liu, Chunyang Yu, Haibao Jin, Binbin Jiang, Xinyuan Zhu, Yongfeng Zhou, Zhongyuan Lu, and Deyue Yan pp 4765–4770 DOI: 10.1021/ja3122608 Supporting Info |
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Synthetic Control Over Photoinduced Electron Transfer in Phosphorescence Zinc Sensors Hana Woo, Somin Cho, Yejee Han, Weon-Sik Chae, Dae-Ro Ahn, Youngmin You, and Wonwoo Nam pp 4771–4787 DOI: 10.1021/ja3123202 Supporting Info |
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Phosphoryl Transfer by Protein Kinase A Is Captured in a Crystal Lattice Adam C. Bastidas, Michael S. Deal, Jon M. Steichen, Yurong Guo, Jian Wu, and Susan S. Taylor pp 4788–4798 DOI: 10.1021/ja312237q Supporting Info |
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Multifunctional Mesoporous Silica-Coated Graphene Nanosheet Used for Chemo-Photothermal Synergistic Targeted Therapy of Glioma Yi Wang, Kaiyuan Wang, Jianfeng Zhao, Xingang Liu, Juan Bu, Xueying Yan, and Rongqin Huang pp 4799–4804 DOI: 10.1021/ja312221g Supporting Info |
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Simultaneous Discrimination of Diameter, Handedness, and Metallicity of Single-Walled Carbon Nanotubes with Chiral Diporphyrin Nanocalipers Gang Liu, Feng Wang, Songpol Chaunchaiyakul, Yukie Saito, Ajoy K. Bauri, Takahide Kimura, Yuji Kuwahara, and Naoki Komatsu pp 4805–4814 DOI: 10.1021/ja312519s Supporting Info |
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Probing the Unique Dehydration-Induced Structural Modifications in Cancer Cell DNA Using Surface Enhanced Raman Spectroscopy Sajanlal R. Panikkanvalappil, Megan A. Mackey, and Mostafa A. El-Sayed pp 4815–4821 DOI: 10.1021/ja400187b Supporting Info |
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Effects of the Protein Environment on the Spectral Properties of Tryptophan Radicals in Pseudomonas aeruginosa Azurin Caterina Bernini, Tadeusz Andruniów, Massimo Olivucci, Rebecca Pogni, Riccardo Basosi, and Adalgisa Sinicropi pp 4822–4833 DOI: 10.1021/ja400464n Supporting Info |
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Multiple Shape Transformations of Composite Hydrogel Sheets Héloïse Thérien-Aubin, Zi Liang Wu, Zhihong Nie, and Eugenia Kumacheva pp 4834–4839 DOI: 10.1021/ja400518c Supporting Info |
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Absorption of CO2 and CS2 into the Hofmann-Type Porous Coordination Polymer: Electrostatic versus Dispersion Interactions Milind Madhusudan Deshmukh, Masaaki Ohba, Susumu Kitagawa, and Shigeyoshi Sakaki pp 4840–4849 DOI: 10.1021/ja400537f Supporting Info |
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Axially Engineered Metal–Insulator Phase Transition by Graded Doping VO2 Nanowires Sangwook Lee, Chun Cheng, Hua Guo, Kedar Hippalgaonkar, Kevin Wang, Joonki Suh, Kai Liu, and Junqiao Wu pp 4850–4855 DOI: 10.1021/ja400658u Supporting Info |
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On the Existence of Designer Magnetic Superatoms Xinxing Zhang, Yi Wang, Haopeng Wang, Alane Lim, Gerd Gantefoer, Kit H. Bowen, J. Ulises Reveles, and Shiv N. Khanna pp 4856–4861 DOI: 10.1021/ja400830z Supporting Info |
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Synthesis and Electronic Structure of Bis(imino)pyridine Iron Metallacyclic Intermediates in Iron-Catalyzed Cyclization Reactions Jordan M. Hoyt, Kevin T. Sylvester, Scott P. Semproni, and Paul J. Chirik pp 4862–4877 DOI: 10.1021/ja400895j Supporting Info |
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Origins of 1,6-Stereoinduction in Torquoselective 6π Electrocyclizations Ashay Patel, Gregg A. Barcan, Ohyun Kwon, and K. N. Houk pp 4878–4883 DOI: 10.1021/ja400882y Supporting Info |
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Helix-Forming Propensity of Aliphatic Urea Oligomers Incorporating Noncanonical Residue Substitution Patterns Nagendar Pendem, Céline Douat, Paul Claudon, Michel Laguerre, Sabine Castano, Bernard Desbat, Dominique Cavagnat, Eric Ennifar, Brice Kauffmann, and Gilles Guichard pp 4884–4892 DOI: 10.1021/ja401151v Supporting Info |
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Improving the Charge Transport in Self-Assembled Monolayer Field-Effect Transistors: From Theory to Devices Christof M. Jäger, Thomas Schmaltz, Michael Novak, Artoem Khassanov, Alexei Vorobiev, Matthias Hennemann, Andreas Krause, Hanno Dietrich, Dirk Zahn, Andreas Hirsch, Marcus Halik, and Timothy Clark pp 4893–4900 DOI: 10.1021/ja401320n Supporting Info |
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Spotlights on Recent JACS Publications pp 4901–4901 DOI: 10.1021/ja402888z |
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The Functional Model Complex [Fe2(BPMP)(OPr)(NO)2](BPh4)2 Provides Insight into the Mechanism of Flavodiiron NO Reductases Sheng Zheng, Timothy C. Berto, Eric W. Dahl, Melissa B. Hoffman, Amy L. Speelman, and Nicolai Lehnert pp 4902–4905 DOI: 10.1021/ja309782m Supporting Info |
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RNA-Based Fluorescent Biosensors for Live Cell Imaging of Second Messengers Cyclic di-GMP and Cyclic AMP-GMP Colleen A. Kellenberger, Stephen C. Wilson, Jade Sales-Lee, and Ming C. Hammond pp 4906–4909 DOI: 10.1021/ja311960g Supporting Info |
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Radiation-Induced Formation of Chlorine Oxides and Their Potential Role in the Origin of Martian Perchlorates Yong S. Kim, Kellie P. Wo, Surajit Maity, Sushil K. Atreya, and Ralf I. Kaiser pp 4910–4913 DOI: 10.1021/ja3122922 Supporting Info |
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High Thermoelectric Properties of n-Type AgBiSe2 Lin Pan, David Bérardan, and Nita Dragoe pp 4914–4917 DOI: 10.1021/ja312474n Supporting Info |
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Effects of Microcomplexity on Hydrophobic Hydration in Amphiphiles Ming-Liang Tan, Joseph R. Cendagorta, and Toshiko Ichiye pp 4918–4921 DOI: 10.1021/ja312504q Supporting Info |
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Hybridization of Phenylthiolate- and Methylthiolate-Adatom Species at Low Coverage on the Au(111) Surface Petro Maksymovych, Dan C. Sorescu, Oleksandr Voznyy, and John T. Yates, Jr. pp 4922–4925 DOI: 10.1021/ja4000905 Supporting Info |
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Full-Range Intracellular pH Sensing by an Aggregation-Induced Emission-Active Two-Channel Ratiometric Fluorogen Sijie Chen, Yuning Hong, Yang Liu, Jianzhao Liu, Chris W. T. Leung, Min Li, Ryan T. K. Kwok, Engui Zhao, Jacky W. Y. Lam, Yong Yu, and Ben Zhong Tang pp 4926–4929 DOI: 10.1021/ja400337p Supporting Info |
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A Large-Molecular-Weight Polyanion, Synthesized via Ring-Opening Metathesis Polymerization, as a Lubricant for Human Articular Cartilage Michel Wathier, Benjamin A. Lakin, Prashant N. Bansal, Stephanie S. Stoddart, Brian D. Snyder, and Mark W. Grinstaff pp 4930–4933 DOI: 10.1021/ja400695h Supporting Info |
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Regioselective and Stereospecific Copper-Catalyzed Aminoboration of Styrenes with Bis(pinacolato)diboron and O-Benzoyl-N,N-dialkylhydroxylamines Naoki Matsuda, Koji Hirano, Tetsuya Satoh, and Masahiro Miura pp 4934–4937 DOI: 10.1021/ja4007645 Supporting Info |
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H–H and Si–H Bond Addition to Fe≡NNR2 Intermediates Derived from N2 Daniel L. M. Suess and Jonas C. Peters pp 4938–4941 DOI: 10.1021/ja400836u Supporting Info |
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A Golden Ring: Molecular Gold Carbido Complexes Elliot S. Borren, Anthony F. Hill, Rong Shang, Manab Sharma, and Anthony C. Willis pp 4942–4945 DOI: 10.1021/ja400128h Supporting Info |
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Separation of Precise Compositions of Noble Metal Clusters Protected with Mixed Ligands Yoshiki Niihori, Miku Matsuzaki, Thalappil Pradeep, and Yuichi Negishi pp 4946–4949 DOI: 10.1021/ja4009369 Supporting Info |
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Reactions of the Three AmpD Enzymes of Pseudomonas aeruginosa Weilie Zhang, Mijoon Lee, Dusan Hesek, Elena Lastochkin, Bill Boggess, and Shahriar Mobashery pp 4950–4953 DOI: 10.1021/ja400970n Supporting Info |
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Irreversible Network Transformation in a Dynamic Porous Host Catalyzed by Sulfur Dioxide Sihai Yang, Leifeng Liu, Junliang Sun, K. Mark Thomas, Andrew J. Davies, Michael W. George, Alexander J. Blake, Adrian H. Hill, Andrew N. Fitch, Chiu C. Tang, and Martin Schröder pp 4954–4957 DOI: 10.1021/ja401061m Supporting Info |
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Transition-Metal-Free BF3-Mediated Regioselective Direct Alkylation and Arylation of Functionalized Pyridines Using Grignard or Organozinc Reagents Quan Chen, Xavier Mollat du Jourdin, and Paul Knochel pp 4958–4961 DOI: 10.1021/ja401146v Supporting Info |
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Multifunctional Dendronized Peptide Polymer Platform for Safe and Effective siRNA Delivery Hanxiang Zeng, Hannah C. Little, Timothy N. Tiambeng, Gregory A. Williams, and Zhibin Guan pp 4962–4965 DOI: 10.1021/ja400986u Supporting Info |
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Heterobimetallic Carbene Complexes by a Single-Step Site-Selective Metalation of a Tricarbene Ligand Ramananda Maity, Hannah Koppetz, Alexander Hepp, and F. Ekkehardt Hahn pp 4966–4969 DOI: 10.1021/ja401546h Supporting Info |
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Pd-Catalyzed Asymmetric β-Hydride Elimination en Route to Chiral Allenes Ian T. Crouch, Robynne K. Neff, and Doug E. Frantz pp 4970–4973 DOI: 10.1021/ja401606e Supporting Info |
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Stoichiometric Metal-Free Reduction of CO in Syn-Gas Roman Dobrovetsky and Douglas W. Stephan pp 4974–4977 DOI: 10.1021/ja401492s Supporting Info |
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Passive Tumor Targeting of Renal-Clearable Luminescent Gold Nanoparticles: Long Tumor Retention and Fast Normal Tissue Clearance Jinbin Liu, Mengxiao Yu, Chen Zhou, Shengyang Yang, Xuhui Ning, and Jie Zheng pp 4978–4981 DOI: 10.1021/ja401612x Supporting Info |
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Tracing the Interstitial Carbide of the Nitrogenase Cofactor during Substrate Turnover Jared A. Wiig, Chi Chung Lee, Yilin Hu, and Markus W. Ribbe pp 4982–4983 DOI: 10.1021/ja401698d Supporting Info |
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Controlled Catalyst Transfer Polycondensation and Surface-Initiated Polymerization of a p-Phenyleneethynylene-Based Monomer Songsu Kang, Robert J. Ono, and Christopher W. Bielawski pp 4984–4987 DOI: 10.1021/ja401740m Supporting Info |
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Salen Promoted Enantioselective Nazarov Cyclizations of Activated and Unactivated Dienones Gerri E. Hutson, Yunus E. Türkmen, and Viresh H. Rawal pp 4988–4991 DOI: 10.1021/ja401908m Supporting Info |
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Directing Group Enhanced Carbonylative Ring Expansions of Amino-Substituted Cyclopropanes: Rhodium-Catalyzed Multicomponent Synthesis of N-Heterobicyclic Enones Megan H. Shaw, Ekaterina Y. Melikhova, Daniel P. Kloer, William G. Whittingham, and John F. Bower pp 4992–4995 DOI: 10.1021/ja401936c Supporting Info |
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A Bioorthogonal Ligation Enabled by Click Cycloaddition of o-Quinolinone Quinone Methide and Vinyl Thioether Qiang Li, Ting Dong, Xiaohui Liu, and Xiaoguang Lei pp 4996–4999 DOI: 10.1021/ja401989p Supporting Info |
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Electrochemical C–H Amination: Synthesis of Aromatic Primary Amines via N-Arylpyridinium Ions Tatsuya Morofuji, Akihiro Shimizu, and Jun-ichi Yoshida pp 5000–5003 DOI: 10.1021/ja402083e Supporting Info |
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A Cyclic Germadicarbene (“Germylone”) from Germyliumylidene Yun Xiong, Shenglai Yao, Gengwen Tan, Shigeyoshi Inoue, and Matthias Driess pp 5004–5007 DOI: 10.1021/ja402477w Supporting Info |
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A Redox Responsive, Fluorescent Supramolecular Metallohydrogel Consists of Nanofibers with Single-Molecule Width Ye Zhang, Bei Zhang, Yi Kuang, Yuan Gao, Junfeng Shi, Xi Xiang Zhang, and Bing Xu pp 5008–5011 DOI: 10.1021/ja402490j Supporting Info |
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DNA-Mediated Assembly of Protein Heterodimers on Membrane Surfaces Michael P. Coyle, Qian Xu, Samantha Chiang, Matthew B. Francis, and Jay T. Groves pp 5012–5016 DOI: 10.1021/ja3101215 Supporting Info |
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Bulges in G-Quadruplexes: Broadening the Definition of G-Quadruplex-Forming Sequences Vineeth Thachappilly Mukundan and Anh Tuân Phan pp 5017–5028 DOI: 10.1021/ja310251r Supporting Info |
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A General Strategy for Biocompatible, High-Effective Upconversion Nanocapsules Based on Triplet–Triplet Annihilation Qian Liu, Baoru Yin, Tianshe Yang, Yongchao Yang, Zhen Shen, Ping Yao, and Fuyou Li pp 5029–5037 DOI: 10.1021/ja3104268 Supporting Info |
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Liquid Cell Transmission Electron Microscopy Study of Platinum Iron Nanocrystal Growth and Shape Evolution Hong-Gang Liao and Haimei Zheng pp 5038–5043 DOI: 10.1021/ja310612p Supporting Info |
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Membrane Orientation of Gαiβ1γ2 and Gβ1γ2 Determined via Combined Vibrational Spectroscopic Studies Pei Yang, Andrew Boughton, Kristoff T. Homan, John J. G. Tesmer, and Zhan Chen pp 5044–5051 DOI: 10.1021/ja3116026 Supporting Info |
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Brønsted Acid-Promoted C–H Bond Cleavage via Electron Transfer from Toluene Derivatives to a Protonated Nonheme Iron(IV)-Oxo Complex with No Kinetic Isotope Effect Jiyun Park, Yong-Min Lee, Wonwoo Nam, and Shunichi Fukuzumi pp 5052–5061 DOI: 10.1021/ja311662w Supporting Info |
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Cations Bind Only Weakly to Amides in Aqueous Solutions Halil I. Okur, Jaibir Kherb, and Paul S. Cremer pp 5062–5067 DOI: 10.1021/ja3119256 Supporting Info |
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Multifunctional Envelope-Type Mesoporous Silica Nanoparticles for Tumor-Triggered Targeting Drug Delivery Jing Zhang, Zhe-Fan Yuan, Ya Wang, Wei-Hai Chen, Guo-Feng Luo, Si-Xue Cheng, Ren-Xi Zhuo, and Xian-Zheng Zhang pp 5068–5073 DOI: 10.1021/ja312004m Supporting Info |
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Control of Intrachain Charge Transfer in Model Systems for Block Copolymer Photovoltaic Materials Kerr Johnson, Ya-Shih Huang, Sven Huettner, Michael Sommer, Martin Brinkmann, Rhiannon Mulherin, Dorota Niedzialek, David Beljonne, Jenny Clark, Wilhelm T. S. Huck, and Richard H. Friend pp 5074–5083 DOI: 10.1021/ja3121247 Supporting Info |
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Recycling and Imaging of Nuclear Singlet Hyperpolarization Giuseppe Pileio, Sean Bowen, Christoffer Laustsen, Michael C. D. Tayler, Joseph T. Hill-Cousins, Lynda J. Brown, Richard C. D. Brown, Jan H. Ardenkjaer-Larsen, and Malcolm H. Levitt pp 5084–5088 DOI: 10.1021/ja312333v Supporting Info |
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[H(OXeF2)n][AsF6] and [FXeII(OXeIVF2)n][AsF6] (n = 1, 2): Examples of Xenon(IV) Hydroxide Fluoride and Oxide Fluoride Cations and the Crystal Structures of [F3Xe---FH][Sb2F11] and [H5F4][SbF6]·2[F3Xe---FH][Sb2F11] David S. Brock, Hélène P. A. Mercier, and Gary J. Schrobilgen pp 5089–5104 DOI: 10.1021/ja312493j Supporting Info |
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Solid-State NMR on Bacterial Cells: Selective Cell Wall Signal Enhancement and Resolution Improvement using Dynamic Nuclear Polarization Hiroki Takahashi, Isabel Ayala, Michel Bardet, Gaël De Paëpe, Jean-Pierre Simorre, and Sabine Hediger pp 5105–5110 DOI: 10.1021/ja312501d Supporting Info |
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Charge-Dependent Dynamics of a Polyelectrolyte Dendrimer and Its Correlation with Invasive Water Bin Wu, Yun Liu, Xin Li, Eugene Mamontov, Alexander I. Kolesnikov, Souleymane O. Diallo, Changwoo Do, Lionel Porcar, Kunlun Hong, Sean C. Smith, Li Liu, Gregory S. Smith, Takeshi Egami, and Wei-Ren Chen pp 5111–5117 DOI: 10.1021/ja3125959 |
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Dynamics in the Interior of AOT Lamellae Investigated with Two-Dimensional Infrared Spectroscopy S. K. Karthick Kumar, A. Tamimi, and Michael D. Fayer pp 5118–5126 DOI: 10.1021/ja312676e |
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Cleavage of Ether, Ester, and Tosylate C(sp3)–O Bonds by an Iridium Complex, Initiated by Oxidative Addition of C–H Bonds. Experimental and Computational Studies Sabuj Kundu, Jongwook Choi, David Y. Wang, Yuriy Choliy, Thomas J. Emge, Karsten Krogh-Jespersen, and Alan S. Goldman pp 5127–5143 DOI: 10.1021/ja312464b Supporting Info |
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Hydrogen-Incorporated TiS2 Ultrathin Nanosheets with Ultrahigh Conductivity for Stamp-Transferrable Electrodes Chenwen Lin, Xiaojiao Zhu, Jun Feng, Changzheng Wu, Shuanglin Hu, Jing Peng, Yuqiao Guo, Lele Peng, Jiyin Zhao, Jianliu Huang, Jinlong Yang, and Yi Xie pp 5144–5151 DOI: 10.1021/ja400041f Supporting Info |
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High-Performance Tellurium-Free Thermoelectrics: All-Scale Hierarchical Structuring of p-Type PbSe–MSe Systems (M = Ca, Sr, Ba) Yeseul Lee, Shih-Han Lo, John Androulakis, Chun-I Wu, Li-Dong Zhao, Duck-Young Chung, Timothy P. Hogan, Vinayak P. Dravid, and Mercouri G. Kanatzidis pp 5152–5160 DOI: 10.1021/ja400069s Supporting Info |
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A Set of de Novo Designed Parallel Heterodimeric Coiled Coils with Quantified Dissociation Constants in the Micromolar to Sub-nanomolar Regime Franziska Thomas, Aimee L. Boyle, Antony J. Burton, and Derek N. Woolfson pp 5161–5166 DOI: 10.1021/ja312310g Supporting Info |
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Bioinspired Water-Enhanced Mechanical Gradient Nanocomposite Films That Mimic the Architecture and Properties of the Squid Beak Justin D. Fox, Jeffrey R. Capadona, Paul D. Marasco, and Stuart J. Rowan pp 5167–5174 DOI: 10.1021/ja4002713 Supporting Info |
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Unimolecular Photoconversion of Multicolor Luminescence on Hierarchical Self-Assemblies Liangliang Zhu, Xin Li, Quan Zhang, Xing Ma, Menghuan Li, Huacheng Zhang, Zhong Luo, Hans Ågren, and Yanli Zhao pp 5175–5182 DOI: 10.1021/ja400456h Supporting Info |
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Liquid Crystal Reorientation Induced by Aptamer Conformational Changes Patrick S. Noonan, Richard H. Roberts, and Daniel K. Schwartz pp 5183–5189 DOI: 10.1021/ja400619k Supporting Info |
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Microsolvation of LiI and CsI in Water: Anion Photoelectron Spectroscopy and ab initio Calculations Ren-Zhong Li, Cheng-Wen Liu, Yi Qin Gao, Hong Jiang, Hong-Guang Xu, and Wei-Jun Zheng pp 5190–5199 DOI: 10.1021/ja4006942 Supporting Info |
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Asymmetric Organocatalytic Thio-Diels–Alder Reactions via Trienamine Catalysis Hao Jiang, David Cruz Cruz, Yang Li, Vibeke Henriette Lauridsen, and Karl Anker Jørgensen pp 5200–5207 DOI: 10.1021/ja4007244 Supporting Info |
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Energetics of Adsorbed CH3 on Pt(111) by Calorimetry Eric M. Karp, Trent L. Silbaugh, and Charles T. Campbell pp 5208–5211 DOI: 10.1021/ja400899p |
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Photocatalytic Cross-Coupling of Methanol and Formaldehyde on a Rutile TiO2(110) Surface Qing Yuan, Zongfang Wu, Yuekang Jin, Lingshun Xu, Feng Xiong, Yunsheng Ma, and Weixin Huang pp 5212–5219 DOI: 10.1021/ja400978r |
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Structural Zn(II) Implies a Switch from Fully Cooperative to Partly Downhill Folding in Highly Homologous Proteins Maddalena Palmieri, Gaetano Malgieri, Luigi Russo, Ilaria Baglivo, Sabrina Esposito, Fortuna Netti, Annarita Del Gatto, Ivan de Paola, Laura Zaccaro, Paolo V. Pedone, Carla Isernia, Danilo Milardi, and Roberto Fattorusso pp 5220–5228 DOI: 10.1021/ja4009562 Supporting Info |
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Spotlights on Recent JACS Publications pp 5229–5229 DOI: 10.1021/ja403242v |
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Tunable and Switchable Dielectric Constant in an Amphidynamic Crystal Wen Zhang, Heng-Yun Ye, Robert Graf, Hans W. Spiess, Ye-Feng Yao, Run-Qiang Zhu, and Ren-Gen Xiong pp 5230–5233 DOI: 10.1021/ja3110335 Supporting Info |
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Probing the Mechanism of Cyanobacterial Aldehyde Decarbonylase Using a Cyclopropyl Aldehyde Bishwajit Paul, Debasis Das, Benjamin Ellington, and E. Neil G. Marsh pp 5234–5237 DOI: 10.1021/ja3115949 Supporting Info |
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Quantitative Exploration of Electron Transfer in a Single Noncovalent Supramolecular Assembly Phuc T. Bui, Tomoaki Nishino, Yojiro Yamamoto, and Hiroshi Shiigi pp 5238–5241 DOI: 10.1021/ja312019p Supporting Info |
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Intramolecular Oxyallyl–Carbonyl (3 + 2) Cycloadditions Elizabeth H. Krenske, Shuzhong He, Jian Huang, Yunfei Du, K. N. Houk, and Richard P. Hsung pp 5242–5245 DOI: 10.1021/ja312459b Supporting Info |
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Efficient Isomerization of Glucose to Fructose over Zeolites in Consecutive Reactions in Alcohol and Aqueous Media Shunmugavel Saravanamurugan, Marta Paniagua, Juan A. Melero, and Anders Riisager pp 5246–5249 DOI: 10.1021/ja400097f Supporting Info |
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Interfacial Energy Conversion in RuII Polypyridyl-Derivatized Oligoproline Assemblies on TiO2 Da Ma, Stephanie E. Bettis, Kenneth Hanson, Maria Minakova, Leila Alibabaei, William Fondrie, Derek M. Ryan, Garegin A. Papoian, Thomas J. Meyer, Marcey L. Waters, and John M. Papanikolas pp 5250–5253 DOI: 10.1021/ja312143h Supporting Info |
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A DNAzyme-Gold Nanoparticle Probe for Uranyl Ion in Living Cells Peiwen Wu, Kevin Hwang, Tian Lan, and Yi Lu pp 5254–5257 DOI: 10.1021/ja400150v Supporting Info |
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Single Particle Detection by Area Amplification: Single Wall Carbon Nanotube Attachment to a Nanoelectrode Jun Hui Park, Scott N. Thorgaard, Bo Zhang, and Allen J. Bard pp 5258–5261 DOI: 10.1021/ja4000917 Supporting Info |
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Double Helices of a Pyridine-Appended Zinc Chlorophyll Derivative Yoshinao Shinozaki, Gary Richards, Keizo Ogawa, Akihito Yamano, Kazuaki Ohara, Kentaro Yamaguchi, Shin-ichiro Kawano, Kentaro Tanaka, Yasuyuki Araki, Takehiko Wada, and Joe Otsuki pp 5262–5265 DOI: 10.1021/ja400493e Supporting Info |
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Photoluminescent Gold–Copper Nanoparticle Alloys with Composition-Tunable Near-Infrared Emission Christopher M. Andolina, Andrew C. Dewar, Ashley M. Smith, Lauren E. Marbella, Michael J. Hartmann, and Jill E. Millstone pp 5266–5269 DOI: 10.1021/ja400569u Supporting Info |
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Nylon-3 Polymers with Selective Antifungal Activity Runhui Liu, Xinyu Chen, Zvi Hayouka, Saswata Chakraborty, Shaun P. Falk, Bernard Weisblum, Kristyn S. Masters, and Samuel H. Gellman pp 5270–5273 DOI: 10.1021/ja4006404 Supporting Info |
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Histone Modification via Rapid Cleavage of C4′-Oxidized Abasic Sites in Nucleosome Core Particles Chuanzheng Zhou, Jonathan T. Sczepanski, and Marc M. Greenberg pp 5274–5277 DOI: 10.1021/ja400915w Supporting Info |
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Steric-Hindrance-Driven Shape Transition in PbS Quantum Dots: Understanding Size-Dependent Stability Hyekyoung Choi, Jae-Hyeon Ko, Yong-Hyun Kim, and Sohee Jeong pp 5278–5281 DOI: 10.1021/ja400948t Supporting Info |
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Photothermal Colloid Antibodies for Shape-Selective Recognition and Killing of Microorganisms Josef Borovička, William J. Metheringham, Leigh A. Madden, Christopher D. Walton, Simeon D. Stoyanov, and Vesselin N. Paunov pp 5282–5285 DOI: 10.1021/ja400781f Supporting Info |
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Palladium-Catalyzed Intermolecular Dehydrogenative Aminohalogenation of Alkenes under Molecular Oxygen: An Approach to Brominated Enamines Xiaochen Ji, Huawen Huang, Wanqing Wu, and Huanfeng Jiang pp 5286–5289 DOI: 10.1021/ja401034g Supporting Info |
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Intein-Triggered Artificial Protein Hydrogels That Support the Immobilization of Bioactive Proteins Miguel Ramirez, Dongli Guan, Victor Ugaz, and Zhilei Chen pp 5290–5293 DOI: 10.1021/ja401075s Supporting Info |
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Complementary Helicity Interchange of Optically Switchable Supramolecular-Enantiomeric Helicenes with (−)-Gel-Sol-(+)-Gel Transition Ternary Logic Chien-Tien Chen, Chien-Hsiang Chen, and Tiow-Gan Ong pp 5294–5297 DOI: 10.1021/ja401214t Supporting Info |
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Electrophilic Fragment-Based Design of Reversible Covalent Kinase Inhibitors Rand M. Miller, Ville O. Paavilainen, Shyam Krishnan, Iana M. Serafimova, and Jack Taunton pp 5298–5301 DOI: 10.1021/ja401221b Supporting Info |
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Transmembrane Halogen-Bonding Cascades Andreas Vargas Jentzsch and Stefan Matile pp 5302–5303 DOI: 10.1021/ja4013276 Supporting Info |
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Controlled Synthesis of Highly Crystalline MoS2 Flakes by Chemical Vapor Deposition Xinsheng Wang, Hongbin Feng, Yongmin Wu, and Liying Jiao pp 5304–5307 DOI: 10.1021/ja4013485 Supporting Info |
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Nickel-Catalyzed Direct Alkylation of C–H Bonds in Benzamides and Acrylamides with Functionalized Alkyl Halides via Bidentate-Chelation Assistance Yoshinori Aihara and Naoto Chatani pp 5308–5311 DOI: 10.1021/ja401344e Supporting Info |
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Nickel(II) Dithiocarbamate Complexes Containing Sulforhodamine B as Fluorescent Probes for Selective Detection of Nitrogen Dioxide Yan Yan, Saarangan Krishnakumar, Huan Yu, Srinivas Ramishetti, Lih-Wen Deng, Suhua Wang, Leaf Huang, and Dejian Huang pp 5312–5315 DOI: 10.1021/ja401555y Supporting Info |
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Highly Diastereo- and Enantioselective Allylboration of Aldehydes using α-Substituted Allyl/Crotyl Pinacol Boronic Esters via in Situ Generated Borinic Esters Jack L.-Y. Chen, Helen K. Scott, Matthew J. Hesse, Christine L. Willis, and Varinder K. Aggarwal pp 5316–5319 DOI: 10.1021/ja401564z Supporting Info |
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Tension Sensing Nanoparticles for Mechano-Imaging at the Living/Nonliving Interface Yang Liu, Kevin Yehl, Yoshie Narui, and Khalid Salaita pp 5320–5323 DOI: 10.1021/ja401494e Supporting Info |
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Asymmetric Total Synthesis of (−)-Amphidinolide V through Effective Combinations of Catalytic Transformations Ivan Volchkov and Daesung Lee pp 5324–5327 DOI: 10.1021/ja401717b Supporting Info |
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Mechanochemical Synthesis of Chemically Stable Isoreticular Covalent Organic Frameworks Bishnu P. Biswal, Suman Chandra, Sharath Kandambeth, Binit Lukose, Thomas Heine, and Rahul Banerjee pp 5328–5331 DOI: 10.1021/ja4017842 Supporting Info |
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Copper-Catalyzed Electrophilic Carbofunctionalization of Alkynes to Highly Functionalized Tetrasubstituted Alkenes Marcos G. Suero, Elliott D. Bayle, Beatrice S. L. Collins, and Matthew J. Gaunt pp 5332–5335 DOI: 10.1021/ja401840j Supporting Info |
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Molecularly Imprinted Polymer-Based Catalytic Micromotors for Selective Protein Transport Jahir Orozco, Allan Cortés, Guanzhi Cheng, Sirilak Sattayasamitsathit, Wei Gao, Xiaomiao Feng, Yufeng Shen, and Joseph Wang pp 5336–5339 DOI: 10.1021/ja4018545 Supporting Info |
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Enantio- and Diastereoselective Synthesis of N-Acetyl Dihydrotetrafibricin Methyl Ester Philippe Nuhant and William R. Roush pp 5340–5343 DOI: 10.1021/ja401918r Supporting Info |
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Dramatic Effect of Furanose C2′ Substitution on Structure and Stability: Directing the Folding of the Human Telomeric Quadruplex with a Single Fluorine Atom Nerea Martín-Pintado, Maryam Yahyaee-Anzahaee, Glen F. Deleavey, Guillem Portella, Modesto Orozco, Masad J. Damha, and Carlos González pp 5344–5347 DOI: 10.1021/ja401954t Supporting Info |
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Azaphosphatranes as Structurally Tunable Organocatalysts for Carbonate Synthesis from CO2 and Epoxides Bastien Chatelet, Lionel Joucla, Jean-Pierre Dutasta, Alexandre Martinez, Kai C. Szeto, and Véronique Dufaud pp 5348–5351 DOI: 10.1021/ja402053d Supporting Info |
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Synthesis and Spectroscopic and Computational Characterization of the Chalcogenido-Substituted Analogues of the Uranyl Ion, [OUE]2+ (E = S, Se) Jessie L. Brown, Skye Fortier, Guang Wu, Nikolas Kaltsoyannis, and Trevor W. Hayton pp 5352–5355 DOI: 10.1021/ja402068j Supporting Info |
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Enantioselective Iron-Catalyzed Azidation of β-Keto Esters and Oxindoles Qing-Hai Deng, Tim Bleith, Hubert Wadepohl, and Lutz H. Gade pp 5356–5359 DOI: 10.1021/ja402082p Supporting Info |
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The Marriage of Metallacycle Transfer Chemistry with Suzuki–Miyaura Cross-Coupling To Give Main Group Element-Containing Conjugated Polymers Gang He, Le Kang, William Torres Delgado, Olena Shynkaruk, Michael J. Ferguson, Robert McDonald, and Eric Rivard pp 5360–5363 DOI: 10.1021/ja402242z Supporting Info |
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A Coupling of Benzamides and Donor/Acceptor Diazo Compounds To Form γ-Lactams via Rh(III)-Catalyzed C–H Activation Todd K. Hyster, Kyle E. Ruhl, and Tomislav Rovis pp 5364–5367 DOI: 10.1021/ja402274g Supporting Info |
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Visible-Light-Induced Oxygenation of Benzene by the Triplet Excited State of 2,3-Dichloro-5,6-dicyano-p-benzoquinone Kei Ohkubo, Atsushi Fujimoto, and Shunichi Fukuzumi pp 5368–5371 DOI: 10.1021/ja402303k Supporting Info |
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Stacking Variants and Superconductivity in the Bi–O–S System W. Adam Phelan, David C. Wallace, Kathryn E. Arpino, James R. Neilson, Kenneth J. Livi, Che R. Seabourne, Andrew J. Scott, and Tyrel M. McQueen pp 5372–5374 DOI: 10.1021/ja4011767 Supporting Info |
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Fabrication of CaFe2O4/TaON Heterojunction Photoanode for Photoelectrochemical Water Oxidation Eun Sun Kim, Naoyuki Nishimura, Ganesan Magesh, Jae Young Kim, Ji-Wook Jang, Hwichan Jun, Jun Kubota, Kazunari Domen, and Jae Sung Lee pp 5375–5383 DOI: 10.1021/ja308723w Supporting Info |
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A Dual Anchoring Strategy for the Localization and Activation of Artificial Metalloenzymes Based on the Biotin–Streptavidin Technology Jeremy M. Zimbron, Tillmann Heinisch, Maurus Schmid, Didier Hamels, Elisa S. Nogueira, Tilman Schirmer, and Thomas R. Ward pp 5384–5388 DOI: 10.1021/ja309974s Supporting Info |
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Direct Modulation of Microtubule Stability Contributes to Anthracene General Anesthesia Daniel J. Emerson, Brian P. Weiser, John Psonis, Zhengzheng Liao, Olena Taratula, Ashley Fiamengo, Xiaozhao Wang, Keizo Sugasawa, Amos B. Smith, III, Roderic G. Eckenhoff, and Ivan J. Dmochowski pp 5389–5398 DOI: 10.1021/ja311171u Supporting Info |
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Cyclic Denaturation and Renaturation of Double-Stranded DNA by Redox-State Switching of DNA Intercalators Shahida N. Syed, Holger Schulze, Daniel Macdonald, Jason Crain, Andrew R. Mount, and Till T. Bachmann pp 5399–5407 DOI: 10.1021/ja311873t Supporting Info |
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Expanding the Scope of Replicable Unnatural DNA: Stepwise Optimization of a Predominantly Hydrophobic Base Pair Thomas Lavergne, Mélissa Degardin, Denis A. Malyshev, Henry T. Quach, Kirandeep Dhami, Phillip Ordoukhanian, and Floyd E. Romesberg pp 5408–5419 DOI: 10.1021/ja312148q Supporting Info |
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Stability of Single- and Few-Molecule Junctions of Conjugated Diamines M. Teresa González, Adrián Díaz, Edmund Leary, Raúl García, M. Ángeles Herranz, Gabino Rubio-Bollinger, Nazario Martín, and Nicolás Agraït pp 5420–5426 DOI: 10.1021/ja312392q Supporting Info |
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Transformation of Metal–Organic Framework to Polymer Gel by Cross-Linking the Organic Ligands Preorganized in Metal–Organic Framework Takumi Ishiwata, Yuki Furukawa, Kouta Sugikawa, Kenta Kokado, and Kazuki Sada pp 5427–5432 DOI: 10.1021/ja3125614 Supporting Info |
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TRAP Display: A High-Speed Selection Method for the Generation of Functional Polypeptides Takahiro Ishizawa, Takashi Kawakami, Patrick C. Reid, and Hiroshi Murakami pp 5433–5440 DOI: 10.1021/ja312579u Supporting Info |
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[Co(bpy)3]3+/2+ and [Co(phen)3]3+/2+ Electron Mediators for Overall Water Splitting under Sunlight Irradiation Using Z-Scheme Photocatalyst System Yasuyoshi Sasaki, Hideki Kato, and Akihiko Kudo pp 5441–5449 DOI: 10.1021/ja400238r Supporting Info |
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Millifluidics for Time-resolved Mapping of the Growth of Gold Nanostructures Katla Sai Krishna, Chelliah V. Navin, Sanchita Biswas, Varshni Singh, Kyungmin Ham, G. Lisa Bovenkamp, Chandra S. Theegala, Jeffery T. Miller, James J. Spivey, and Challa S. S. R. Kumar pp 5450–5456 DOI: 10.1021/ja400434c Supporting Info |
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A General Method for Constructing Atomic-Resolution RNA Ensembles using NMR Residual Dipolar Couplings: The Basis for Interhelical Motions Revealed Loïc Salmon, Gavin Bascom, Ioan Andricioaei, and Hashim M. Al-Hashimi pp 5457–5466 DOI: 10.1021/ja400920w Supporting Info |
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Total Synthesis and Complete Structural Assignment of Yaku’amide A Takefumi Kuranaga, Yusuke Sesoko, Komei Sakata, Naoya Maeda, Atsushi Hayata, and Masayuki Inoue pp 5467–5474 DOI: 10.1021/ja401457h Supporting Info |
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Spotlights on Recent JACS Publications pp 5475–5476 DOI: 10.1021/ja403480m |
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The Supramolecular Chemistry of β-Sheets Pin-Nan Cheng, Johnny D. Pham, and James S. Nowick pp 5477–5492 DOI: 10.1021/ja3088407 |
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Discovery of Face-Centered-Cubic Ruthenium Nanoparticles: Facile Size-Controlled Synthesis Using the Chemical Reduction Method Kohei Kusada, Hirokazu Kobayashi, Tomokazu Yamamoto, Syo Matsumura, Naoya, Sumi, Katsutoshi Sato, Katsutoshi Nagaoka, Yoshiki Kubota, and Hiroshi Kitagawa pp 5493–5496 DOI: 10.1021/ja311261s Supporting Info |
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Direct Observation of a Metastable Crystal Phase of LixFePO4 under Electrochemical Phase Transition Yuki Orikasa, Takehiro Maeda, Yukinori Koyama, Haruno Murayama, Katsutoshi Fukuda, Hajime Tanida, Hajime Arai, Eiichiro Matsubara, Yoshiharu Uchimoto, and Zempachi Ogumi pp 5497–5500 DOI: 10.1021/ja312527x Supporting Info |
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Emergence of Glass-like Behavior in Markov State Models of Protein Folding Dynamics Jeffrey K. Weber, Robert L. Jack, and Vijay S. Pande pp 5501–5504 DOI: 10.1021/ja4002663 Supporting Info |
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Combining Gold and Photoredox Catalysis: Visible Light-Mediated Oxy- and Aminoarylation of Alkenes Basudev Sahoo, Matthew N. Hopkinson, and Frank Glorius pp 5505–5508 DOI: 10.1021/ja400311h Supporting Info |
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Molecular Mechanism of Polyacrylate Helix Sense Switching across Its Free Energy Landscape Adriana Pietropaolo and Tamaki Nakano pp 5509–5512 DOI: 10.1021/ja4002508 Supporting Info |
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Inducing Rapid Cellular Response on RGD-Binding Threaded Macromolecular Surfaces Ji-Hun Seo, Sachiro Kakinoki, Yuuki Inoue, Tetsuji Yamaoka, Kazuhiko Ishihara, and Nobuhiko Yui pp 5513–5516 DOI: 10.1021/ja400817q Supporting Info |
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Enhanced Electrogenerated Chemiluminescence in Thermoresponsive Microgels Florent Pinaud, Lorenzo Russo, Sandra Pinet, Isabelle Gosse, Valérie Ravaine, and Neso Sojic pp 5517–5520 DOI: 10.1021/ja401011j Supporting Info |
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Efficient Electrocatalytic Oxidation of Formic Acid Using Au@Pt Dendrimer-Encapsulated Nanoparticles Ravikumar Iyyamperumal, Liang Zhang, Graeme Henkelman, and Richard M. Crooks pp 5521–5524 DOI: 10.1021/ja4010305 Supporting Info |
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Determination of Specific Binding Interactions at l-Cystine Crystal Surfaces with Chemical Force Microscopy Trinanjana Mandal and Michael D. Ward pp 5525–5528 DOI: 10.1021/ja401309d Supporting Info |
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Efficient Tandem and Triple-Junction Polymer Solar Cells Weiwei Li, Alice Furlan, Koen H. Hendriks, Martijn M. Wienk, and René A. J. Janssen pp 5529–5532 DOI: 10.1021/ja401434x Supporting Info |
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C–N Bond Cleavage of Anilines by a (Salen)ruthenium(VI) Nitrido Complex Wai-Lun Man, Jianhui Xie, Yi Pan, William W. Y. Lam, Hoi-Ki Kwong, Kwok-Wa Ip, Shek-Man Yiu, Kai-Chung Lau, and Tai-Chu Lau pp 5533–5536 DOI: 10.1021/ja401553d Supporting Info |
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Hydrocarbon-Soluble Nanocatalysts with No Bulk Phase: Coplanar, Two-Coordinate Arrays of the Base Metals Jeffrey Camacho-Bunquin, Michael J. Ferguson, and Jeffrey M. Stryker pp 5537–5540 DOI: 10.1021/ja401579x Supporting Info |
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Enhancing Raman Scattering without Plasmons: Unprecedented Sensitivity Achieved by TiO2 Shell-Based Resonators Ivano Alessandri pp 5541–5544 DOI: 10.1021/ja401666p Supporting Info |
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Evaporation-Induced Buckling and Fission of Microscale Droplet Interface Bilayers Jonathan B. Boreyko, Prachya Mruetusatorn, Stephen A. Sarles, Scott T. Retterer, and C. Patrick Collier pp 5545–5548 DOI: 10.1021/ja4019435 Supporting Info |
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Hierarchically Structured Nanoporous Poly(Ionic Liquid) Membranes: Facile Preparation and Application in Fiber-Optic pH Sensing Qiang Zhao, Mingjie Yin, A. Ping Zhang, Simon Prescher, Markus Antonietti, and Jiayin Yuan pp 5549–5552 DOI: 10.1021/ja402100r Supporting Info |
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Enantioselective Ketone Hydroacylation Using Noyori’s Transfer Hydrogenation Catalyst Stephen K. Murphy and Vy M. Dong pp 5553–5556 DOI: 10.1021/ja4021974 Supporting Info |
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Copper-Catalyzed Diastereoselective Arylation of Tryptophan Derivatives: Total Synthesis of (+)-Naseseazines A and B Madeleine E. Kieffer, Kangway V. Chuang, and Sarah E. Reisman pp 5557–5560 DOI: 10.1021/ja4023557 Supporting Info |
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Stable Tetraaryldiphosphine Radical Cation and Dication Xiaobo Pan, Yuanting Su, Xiaoyu Chen, Yue Zhao, Yizhi Li, Jinglin Zuo, and Xinping Wang pp 5561–5564 DOI: 10.1021/ja402492u Supporting Info |
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Carbamoyl Anion Addition to N-Sulfinyl Imines: Highly Diastereoselective Synthesis of α-Amino Amides Jonathan T. Reeves, Zhulin Tan, Melissa A. Herbage, Zhengxu S. Han, Maurice A. Marsini, Zhibin Li, Guisheng Li, Yibo Xu, Keith R. Fandrick, Nina C. Gonnella, Scot Campbell, Shengli Ma, Nelu Grinberg, Heewon Lee, Bruce Z. Lu, and Chris H. Senanayake pp 5565–5568 DOI: 10.1021/ja402647m Supporting Info |
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Scalable and Effective Enrichment of Semiconducting Single-Walled Carbon Nanotubes by a Dual Selective Naphthalene-Based Azo Dispersant Ashok Kumar Sundramoorthy, Sara Mesgari, Jing Wang, Raj Kumar, Mahasin Alam Sk., Siew Hooi Yeap, Qing Zhang, Siu Kwan Sze, Kok Hwa Lim, and Mary B. Chan-Park pp 5569–5581 DOI: 10.1021/ja312282g Supporting Info |
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Mechanistic Study of the Diels–Alder Reaction of Paramagnetic Endohedral Metallofullerene: Reaction of La@C82 with 1,2,3,4,5-Pentamethylcyclopentadiene Satoru Sato, Yutaka Maeda, Jing-Dong Guo, Michio Yamada, Naomi Mizorogi, Shigeru Nagase, and Takeshi Akasaka pp 5582–5587 DOI: 10.1021/ja309763f Supporting Info |
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Plasmonic Harvesting of Light Energy for Suzuki Coupling Reactions Feng Wang, Chuanhao Li, Huanjun Chen, Ruibin Jiang, Ling-Dong Sun, Quan Li, Jianfang Wang, Jimmy C. Yu, and Chun-Hua Yan pp 5588–5601 DOI: 10.1021/ja310501y Supporting Info |
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The Essential Role of Stacking Adenines in a Two-Base-Pair RNA Kissing Complex William Stephenson, Papa Nii Asare-Okai, Alan A. Chen, Sean Keller, Rachel Santiago, Scott A. Tenenbaum, Angel E. Garcia, Daniele Fabris, and Pan T. X. Li pp 5602–5611 DOI: 10.1021/ja310820h Supporting Info |
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Toehold-Mediated Nonenzymatic DNA Strand Displacement As a Platform for DNA Genotyping Dmitriy A. Khodakov, Anastasia S. Khodakova, Adrian Linacre, and Amanda V. Ellis pp 5612–5619 DOI: 10.1021/ja310991r Supporting Info |
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Colocalization of the Ganglioside GM1 and Cholesterol Detected by Secondary Ion Mass Spectrometry Mónica M. Lozano, Zhao Liu, Eva Sunnick, Andreas Janshoff, Krishna Kumar, and Steven G. Boxer pp 5620–5630 DOI: 10.1021/ja310831m Supporting Info |
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Characterization of Metastable Intermediates Formed in the Reaction between a Mn(II) Complex and Dioxygen, Including a Crystallographic Structure of a Binuclear Mn(III)–Peroxo Species Michael K. Coggins, Xianru Sun, Yeonju Kwak, Edward I. Solomon, Elena Rybak-Akimova, and Julie A. Kovacs pp 5631–5640 DOI: 10.1021/ja311166u Supporting Info |
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A General Protocol for Determining the Structures of Molecularly Ordered but Noncrystalline Silicate Frameworks Darren H. Brouwer, Sylvian Cadars, Juergen Eckert, Zheng Liu, Osamu Terasaki, and Bradley F. Chmelka pp 5641–5655 DOI: 10.1021/ja311649m Supporting Info |
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Aromatic Sulfonyl Fluorides Covalently Kinetically Stabilize Transthyretin to Prevent Amyloidogenesis while Affording a Fluorescent Conjugate Neil P. Grimster, Stephen Connelly, Aleksandra Baranczak, Jiajia Dong, Larissa B. Krasnova, K. Barry Sharpless, Evan T. Powers, Ian A. Wilson, and Jeffery W. Kelly pp 5656–5668 DOI: 10.1021/ja311729d Supporting Info |
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Alkylation of Gold Surface by Treatment with C18H37HgOTs and Anodic Hg Stripping Malgorzata Mucha, Eva Kaletová, Anna Kohutová, Frank Scholz, Elizabeth S. Stensrud, Ivan Stibor, Lubomír Pospíšil, Florian von Wrochem, and Josef Michl pp 5669–5677 DOI: 10.1021/ja3117125 Supporting Info |
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Chain-Reaction Anion Exchange between Metal–Organic Cages Shucong Ma, Maarten M. J. Smulders, Yana R. Hristova, Jack K. Clegg, Tanya K. Ronson, Salvatore Zarra, and Jonathan R. Nitschke pp 5678–5684 DOI: 10.1021/ja311882h Supporting Info |
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Carrier Generation in Multicomponent Wide-Bandgap Oxides: InGaZnO4 Altynbek Murat, Alexander U. Adler, Thomas O. Mason, and Julia E. Medvedeva pp 5685–5692 DOI: 10.1021/ja311955g |
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Generating Long Supramolecular Pathways with a Continuous Density of States by Physically Linking Conjugated Molecules via Their End Groups Roozbeh Shokri, Marie-Agnés Lacour, Thibaut Jarrosson, Jean-Pierre Lère-Porte, Françoise Serein-Spirau, Karinne Miqueu, Jean-Marc Sotiropoulos, François Vonau, Dominique Aubel, Marion Cranney, Günter Reiter, and Laurent Simon pp 5693–5698 DOI: 10.1021/ja311964b |
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Mechanistic Insights into Ring-Opening and Decarboxylation of 2-Pyrones in Liquid Water and Tetrahydrofuran Mei Chia, M. Ali Haider, Gerald Pollock, III, George A. Kraus, Matthew Neurock, and James A. Dumesic pp 5699–5708 DOI: 10.1021/ja312075r Supporting Info |
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Controllable Drug Release and Simultaneously Carrier Decomposition of SiO2-Drug Composite Nanoparticles Silu Zhang, Zhiqin Chu, Chun Yin, Chunyuan Zhang, Ge Lin, and Quan Li pp 5709–5716 DOI: 10.1021/ja3123015 Supporting Info |
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Ring-Opening Metathesis Polymerization with the Second Generation Hoveyda–Grubbs Catalyst: An Efficient Approach toward High-Purity Functionalized Macrocyclic Oligo(cyclooctene)s Anton Blencowe and Greg G. Qiao pp 5717–5725 DOI: 10.1021/ja312418z Supporting Info |
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On the Magnetic and Spectroscopic Properties of High-Valent Mn3CaO4 Cubanes as Structural Units of Natural and Artificial Water-Oxidizing Catalysts Vera Krewald, Frank Neese, and Dimitrios A. Pantazis pp 5726–5739 DOI: 10.1021/ja312552f Supporting Info |
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Cation−π Interactions As Lipid-Specific Anchors for Phosphatidylinositol-Specific Phospholipase C Cédric Grauffel, Boqian Yang, Tao He, Mary F. Roberts, Anne Gershenson, and Nathalie Reuter pp 5740–5750 DOI: 10.1021/ja312656v Supporting Info |
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Conformational Disorder Enhances Electron Transfer Through Alkyl Monolayers: Ferrocene on Conductive Diamond Rose E. Ruther, Qiang Cui, and Robert J. Hamers pp 5751–5761 DOI: 10.1021/ja312680p Supporting Info |
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Hyperconjugative Interactions in Permethylated Siloxanes and Ethers: The Nature of the SiO Bond Frank Weinhold and Robert West pp 5762–5767 DOI: 10.1021/ja312222k Supporting Info |
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Mechanisms of Halogen-Based Covalent Self-Assembly on Metal Surfaces Jonas Björk, Felix Hanke, and Sven Stafström pp 5768–5775 DOI: 10.1021/ja400304b Supporting Info |
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Membrane-Proximal Domain of a Disintegrin and Metalloprotease-17 Represents the Putative Molecular Switch of Its Shedding Activity Operated by Protein-disulfide Isomerase Stefan Düsterhöft, Sascha Jung, Chien-Wen Hung, Andreas Tholey, Frank D. Sönnichsen, Joachim Grötzinger, and Inken Lorenzen pp 5776–5781 DOI: 10.1021/ja400340u Supporting Info |
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H3O2 Bridging Ligand in a Metal–Organic Framework. Insight into the Aqua-Hydroxo↔Hydroxyl Equilibrium: A Combined Experimental and Theoretical Study Richard F. D’Vries, Victor A. de la Peña-O’Shea, Natalia Snejko, Marta Iglesias, Enrique Gutiérrez-Puebla, and M. Angeles Monge pp 5782–5792 DOI: 10.1021/ja4005046 Supporting Info |
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Enhancing Catalytic Performance of Palladium in Gold and Palladium Alloy Nanoparticles for Organic Synthesis Reactions through Visible Light Irradiation at Ambient Temperatures Sarina Sarina, Huaiyong Zhu, Esa Jaatinen, Qi Xiao, Hongwei Liu, Jianfeng Jia, Chao Chen, and Jian Zhao pp 5793–5801 DOI: 10.1021/ja400527a Supporting Info |
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Structural Changes in Cytochrome c Oxidase Induced by Binding of Sodium and Calcium Ions: An ATR-FTIR Study Amandine Maréchal, Masayo Iwaki, and Peter R. Rich pp 5802–5807 DOI: 10.1021/ja4005706 Supporting Info |
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Oxyanion Hole Stabilization by C–H···O Interaction in a Transition State—A Three-Point Interaction Model for Cinchona Alkaloid-Catalyzed Asymmetric Methanolysis of meso-Cyclic Anhydrides Hui Yang and Ming Wah Wong pp 5808–5818 DOI: 10.1021/ja4005893 Supporting Info |
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Accounting for Conformational Variability in Protein–Ligand Docking with NMR-Guided Rescoring Lars Skjærven, Luca Codutti, Andrea Angelini, Manuela Grimaldi, Dorota Latek, Peter Monecke, Matthias K. Dreyer, and Teresa Carlomagno pp 5819–5827 DOI: 10.1021/ja4007468 Supporting Info |
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Quantifying Functional Group Interactions That Determine Urea Effects on Nucleic Acid Helix Formation Emily J. Guinn, Jeffrey J. Schwinefus, Hyo Keun Cha, Joseph L. McDevitt, Wolf E. Merker, Ryan Ritzer, Gregory W. Muth, Samuel W. Engelsgjerd, Kathryn E. Mangold, Perry J. Thompson, Michael J. Kerins, and M. Thomas Record, Jr. pp 5828–5838 DOI: 10.1021/ja400965n Supporting Info |
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Extein Residues Play an Intimate Role in the Rate-Limiting Step of Protein Trans-Splicing Neel H. Shah, Ertan Eryilmaz, David Cowburn, and Tom W. Muir pp 5839–5847 DOI: 10.1021/ja401015p Supporting Info |
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Z-Selective Ethenolysis with a Ruthenium Metathesis Catalyst: Experiment and Theory Hiroshi Miyazaki, Myles B. Herbert, Peng Liu, Xiaofei Dong, Xiufang Xu, Benjamin K. Keitz, Thay Ung, Garik Mkrtumyan, K. N. Houk, and Robert H. Grubbs pp 5848–5858 DOI: 10.1021/ja4010267 Supporting Info |
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Small-Molecule Binding Sites on Proteins Established by Paramagnetic NMR Spectroscopy Jia-Ying Guan, Peter H. J. Keizers, Wei-Min Liu, Frank Löhr, Simon P. Skinner, Edwin A. Heeneman, Harald Schwalbe, Marcellus Ubbink, and Gregg Siegal pp 5859–5868 DOI: 10.1021/ja401323m Supporting Info |
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From Sphere to Multipod: Thermally Induced Transitions of CdSe Nanocrystals Studied by Molecular Dynamics Simulations Zhaochuan Fan, Anil O. Yalcin, Frans D. Tichelaar, Henny W. Zandbergen, Elise Talgorn, Arjan J. Houtepen, Thijs J. H. Vlugt, and Marijn A. van Huis pp 5869–5876 DOI: 10.1021/ja401406q Supporting Info |
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meta-Selective C–H Bond Alkylation with Secondary Alkyl Halides Nora Hofmann and Lutz Ackermann pp 5877–5884 DOI: 10.1021/ja401466y Supporting Info |
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An Effective Strategy for Exploring Unknown Metabolic Pathways by Genome Mining Dorianne A. Castillo, Mariya D. Kolesnikova, and Seiichi P. T. Matsuda pp 5885–5894 DOI: 10.1021/ja401535g Supporting Info |
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Influence of Active Site Location on Catalytic Activity in de Novo-Designed Zinc Metalloenzymes Melissa L. Zastrow and Vincent L. Pecoraro pp 5895–5903 DOI: 10.1021/ja401537t Supporting Info |
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Phosphonated Trityl Probes for Concurrent in Vivo Tissue Oxygen and pH Monitoring Using Electron Paramagnetic Resonance-Based Techniques Ilirian Dhimitruka, Andrey A. Bobko, Timothy D. Eubank, Denis A. Komarov, and Valery V. Khramtsov pp 5904–5910 DOI: 10.1021/ja401572r Supporting Info |
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Dynamic Evolving Two-Component Supramolecular Gels—Hierarchical Control over Component Selection in Complex Mixtures William Edwards and David K. Smith pp 5911–5920 DOI: 10.1021/ja4017107 Supporting Info |
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Controlling the Effective Surface Area and Pore Size Distribution of sp2 Carbon Materials and Their Impact on the Capacitance Performance of These Materials Long Zhang, Xi Yang, Fan Zhang, Guankui Long, Tengfei Zhang, Kai Leng, Yawei Zhang, Yi Huang, Yanfeng Ma, Mingtao Zhang, and Yongsheng Chen pp 5921–5929 DOI: 10.1021/ja402552h Supporting Info |
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Correction to “Inducible Biosynthetic Nanoscaffolds as Recruitment Platforms for Detecting Molecular Target Interactions inside Living Cells” Sangkyu Lee, Jae-Seok Ha, Seung-Goo Lee, and Tae K. Kim pp 5930–5930 DOI: 10.1021/ja400541t |
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Correction to “Catalytic Mechanism of Cytochrome P450 for 5′-Hydroxylation of Nicotine: Fundamental Reaction Pathways and Stereoselectivity Dongmei Li, Xiaoqin Huang, Keli Han, and Chang-Guo Zhan pp 5931–5931 DOI: 10.1021/ja4021099 |
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Correction to “Fluoroketone Inhibition of Ca2+-Independent Phospholipase A2 through Binding Pocket Association Defined by Hydrogen/Deuterium Exchange and Molecular Dynamics” Yuan-Hao Hsu, Denis Bucher, Jian Cao, Sheng Li, Sheng-Wei Yang, George Kokotos, Virgil L. Woods, Jr., J. Andrew McCammon, and Edward A. Dennis pp 5932–5932 DOI: 10.1021/ja4023623 |
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Spotlights on Recent JACS Publications pp 5933–5933 DOI: 10.1021/ja403755u |
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Investigation of SSEA-4 Binding Protein in Breast Cancer Cells Ting-Chun Hung, Chih-Wei Lin, Tsui-Ling Hsu, Chung-Yi Wu, and Chi-Huey Wong pp 5934–5937 DOI: 10.1021/ja312210c Supporting Info |
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Quantitating the Lattice Strain Dependence of Monolayer Pt Shell Activity toward Oxygen Reduction Xiaoming Wang, Yuki Orikasa, Yuki Takesue, Hideo Inoue, Masashi Nakamura, Taketoshi Minato, Nagahiro Hoshi, and Yoshiharu Uchimoto pp 5938–5941 DOI: 10.1021/ja312382h Supporting Info |
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Spin Transitions in Fe(II) Metallogrids Modulated by Substituents, Counteranions, and Solvents Yi-Tong Wang, Shu-Tao Li, Shu-Qi Wu, Ai-Li Cui, De-Zhong Shen, and Hui-Zhong Kou pp 5942–5945 DOI: 10.1021/ja312622c Supporting Info |
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A Perfluoroaryl-Cysteine SNAr Chemistry Approach to Unprotected Peptide Stapling Alexander M. Spokoyny, Yekui Zou, Jingjing J. Ling, Hongtao Yu, Yu-Shan Lin, and Bradley L. Pentelute pp 5946–5949 DOI: 10.1021/ja400119t Supporting Info |
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Integration of Gold Nanoparticles into Bilayer Structures via Adaptive Surface Chemistry Hee-Young Lee, Sun Hae Ra Shin, Ludmila L. Abezgauz, Sean A. Lewis, Aaron M. Chirsan, Dganit D. Danino, and Kyle J. M. Bishop pp 5950–5953 DOI: 10.1021/ja400225n Supporting Info |
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Optically Selective Two-Photon Uncaging of Glutamate at 900 nm Jeremy P. Olson, Hyung-Bae Kwon, Kevin T. Takasaki, Chiayu Q. Chiu, Michael J. Higley, Bernardo L. Sabatini, and Graham C. R. Ellis-Davies pp 5954–5957 DOI: 10.1021/ja4019379 Supporting Info |
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Cu2Ge(S3–xSex) Colloidal Nanocrystals: Synthesis, Characterization, and Composition-Dependent Band Gap Engineering Chi Yang, Bin Zhou, Shu Miao, Chunyan Yang, Bing Cai, Wen-Hua Zhang, and Xin Xu pp 5958–5961 DOI: 10.1021/ja400452t Supporting Info |
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Metabolic Perturbation of an Essential Pathway: Evaluation of a Glycine Precursor of Coenzyme A Michael Rothmann, MinJin Kang, Reymundo Villa, Ioanna Ntai, James J. La Clair, Neil L. Kelleher, Eli Chapman, and Michael D. Burkart pp 5962–5965 DOI: 10.1021/ja400795m Supporting Info |
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Real-Time Evaluation of Binding Mechanisms in Multivalent Interactions: A Surface Plasmon Resonance Kinetic Approach Eva Maria Munoz, Juan Correa, Ricardo Riguera, and Eduardo Fernandez-Megia pp 5966–5969 DOI: 10.1021/ja400951g Supporting Info |
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A Previously Unrecognized Kanosamine Biosynthesis Pathway in Bacillus subtilis Natasha D. Vetter, David M. Langill, Shazia Anjum, Julie Boisvert-Martel, Rajendra C. Jagdhane, Egiroh Omene, Hongyan Zheng, Karin E. van Straaten, Isaac Asiamah, Ed S. Krol, David A. R. Sanders, and David R. J. Palmer pp 5970–5973 DOI: 10.1021/ja4010255 Supporting Info |
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Charge Transport in Photoswitchable Dimethyldihydropyrene-Type Single-Molecule Junctions Diego Roldan, Veerabhadrarao Kaliginedi, Saioa Cobo, Viliam Kolivoska, Christophe Bucher, Wenjing Hong, Guy Royal, and Thomas Wandlowski pp 5974–5977 DOI: 10.1021/ja401484j Supporting Info |
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Magnitude and Origin of the Enhanced Basicity of the Catalytic Glutamate of Triosephosphate Isomerase M. Merced Malabanan, Lucia Nitsch-Velasquez, Tina L. Amyes, and John P. Richard pp 5978–5981 DOI: 10.1021/ja401504w Supporting Info |
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Stepwise Transformation of the Molecular Building Blocks in a Porphyrin-Encapsulating Metal–Organic Material Zhenjie Zhang, Lukasz Wojtas, Mohamed Eddaoudi, and Michael J. Zaworotko pp 5982–5985 DOI: 10.1021/ja4015666 Supporting Info |
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Salt-Free Reducing Reagent of Bis(trimethylsilyl)cyclohexadiene Mediates Multielectron Reduction of Chloride Complexes of W(VI) and W(IV) Hayato Tsurugi, Hiromasa Tanahashi, Haruka Nishiyama, Waldemar Fegler, Teruhiko Saito, Andreas Sauer, Jun Okuda, and Kazushi Mashima pp 5986–5989 DOI: 10.1021/ja401589a Supporting Info |
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Light-Driven Linear Helical Supramolecular Polymer Formed by Molecular-Recognition-Directed Self-Assembly of Bis(p-sulfonatocalix[4]arene) and Pseudorotaxane Ruyi Sun, Chenming Xue, Xiang Ma, Min Gao, He Tian, and Quan Li pp 5990–5993 DOI: 10.1021/ja4016952 Supporting Info |
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Correlated Electrochemical and Optical Tracking of Discrete Collision Events Stephen E. Fosdick, Morgan J. Anderson, Elizabeth G. Nettleton, and Richard M. Crooks pp 5994–5997 DOI: 10.1021/ja401864k Supporting Info |
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Single-Layer MoS2-Based Nanoprobes for Homogeneous Detection of Biomolecules Changfeng Zhu, Zhiyuan Zeng, Hai Li, Fan Li, Chunhai Fan, and Hua Zhang pp 5998–6001 DOI: 10.1021/ja4019572 Supporting Info |
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Diced Electrophoresis Gel Assay for Screening Enzymes with Specified Activities Toru Komatsu, Kenjiro Hanaoka, Alexander Adibekian, Kentaro Yoshioka, Takuya Terai, Tasuku Ueno, Mitsuyasu Kawaguchi, Benjamin F. Cravatt, and Tetsuo Nagano pp 6002–6005 DOI: 10.1021/ja401792d Supporting Info |
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Modular Stitching To Image Single-Molecule DNA Transport Juan Guan, Bo Wang, Sung Chul Bae, and Steve Granick pp 6006–6009 DOI: 10.1021/ja4020138 Supporting Info |
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Structural Characterization and Oxidation Reactivity of a Nickel(II) Acylperoxo Complex Jun Nakazawa, Shota Terada, Masaki Yamada, and Shiro Hikichi pp 6010–6013 DOI: 10.1021/ja4020277 Supporting Info |
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Hydroxyproline-Free Single Composition ABC Collagen Heterotrimer Abhishek A. Jalan, Borries Demeler, and Jeffrey D. Hartgerink pp 6014–6017 DOI: 10.1021/ja402187t Supporting Info |
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Stoichiometric C═O Bond Oxidative Addition of Benzophenone by a Discrete Radical Intermediate To Form a Cobalt(I) Carbene Seth L. Marquard, Mark W. Bezpalko, Bruce M. Foxman, and Christine M. Thomas pp 6018–6021 DOI: 10.1021/ja4022683 Supporting Info |
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Macroscale Lateral Alignment of Semiconductor Nanorods into Freestanding Thin Films Tie Wang, Xirui Wang, Derek LaMontagne, Zhongwu Wang, and Y. Charles Cao pp 6022–6025 DOI: 10.1021/ja402539f Supporting Info |
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Synthesis of Z-(Pinacolato)allylboron and Z-(Pinacolato)alkenylboron Compounds through Stereoselective Catalytic Cross-Metathesis Elizabeth T. Kiesewetter, Robert V. O’Brien, Elsie C. Yu, Simon J. Meek, Richard R. Schrock, and Amir H. Hoveyda pp 6026–6029 DOI: 10.1021/ja403188t Supporting Info |
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β-Arylation of Carboxamides via Iron-Catalyzed C(sp3)–H Bond Activation Rui Shang, Laurean Ilies, Arimasa Matsumoto, and Eiichi Nakamura pp 6030–6032 DOI: 10.1021/ja402806f Supporting Info |
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High Catalytic Rates for Hydrogen Production Using Nickel Electrocatalysts with Seven-Membered Cyclic Diphosphine Ligands Containing One Pendant Amine Michael P. Stewart, Ming-Hsun Ho, Stefan Wiese, Mary Lou Lindstrom, Colleen E. Thogerson, Simone Raugei, R. Morris Bullock, and Monte L. Helm pp 6033–6046 DOI: 10.1021/ja400181a Supporting Info |
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Capture and Quality Control Mechanisms for Adenosine-5′-triphosphate Binding Li Li, Susan A. Martinis, and Zaida Luthey-Schulten pp 6047–6055 DOI: 10.1021/ja308044w Supporting Info |
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Site-Selective Doping Effect in AMn3V4O12 (A = Na+, Ca2+, and La3+) Shoubao Zhang, Takashi Saito, Masaichiro Mizumaki, Wei-tin Chen, Takenori Tohyama, and Yuichi Shimakawa pp 6056–6060 DOI: 10.1021/ja308851f |
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Performance Improvement of Nanocatalysts by Promoter-Induced Defects in the Support Material: Methanol Synthesis over Cu/ZnO:Al Malte Behrens, Stefan Zander, Patrick Kurr, Nikolas Jacobsen, Jürgen Senker, Gregor Koch, Thorsten Ressler, Richard W. Fischer, and Robert Schlögl pp 6061–6068 DOI: 10.1021/ja310456f Supporting Info |
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The Copper Active Site of CBM33 Polysaccharide Oxygenases Glyn R. Hemsworth, Edward J. Taylor, Robbert Q. Kim, Rebecca C. Gregory, Sally J. Lewis, Johan P. Turkenburg, Alison Parkin, Gideon J. Davies, and Paul H. Walton pp 6069–6077 DOI: 10.1021/ja402106e Supporting Info |
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Detergent Release Prolongs the Lifetime of Native-like Membrane Protein Conformations in the Gas-Phase Antoni J. Borysik, Dominic J. Hewitt, and Carol V. Robinson pp 6078–6083 DOI: 10.1021/ja401736v Supporting Info |
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Enthalpic Signature of Methonium Desolvation Revealed in a Synthetic Host–Guest System Based on Cucurbit[7]uril Yi Wang, Jason R. King, Pan Wu, Daniel L. Pelzman, David N. Beratan, and Eric J. Toone pp 6084–6091 DOI: 10.1021/ja311327v Supporting Info |
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A Comprehensive Mathematical Model for Three-Body Binding Equilibria Eugene F. Douglass, Jr., Chad J. Miller, Gerson Sparer, Harold Shapiro, and David A. Spiegel pp 6092–6099 DOI: 10.1021/ja311795d Supporting Info |
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Suppression of Intersite Charge Transfer in Charge-Disproportionated Perovskite YCu3Fe4O12 Hidenobu Etani, Ikuya Yamada, Kenya Ohgushi, Naoaki Hayashi, Yoshihiro Kusano, Masaichiro Mizumaki, Jungeun Kim, Naruki Tsuji, Ryoji Takahashi, Norimasa Nishiyama, Toru Inoue, Tetsuo Irifune, and Mikio Takano pp 6100–6106 DOI: 10.1021/ja312015j Supporting Info |
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CO Chemisorption and Dissociation at High Coverages during CO Hydrogenation on Ru Catalysts Brett T. Loveless, Corneliu Buda, Matthew Neurock, and Enrique Iglesia pp 6107–6121 DOI: 10.1021/ja311848e |
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Probing Hydrogen Bond Energies by Mass Spectrometry Hai-Feng Su, Lan Xue, Yun-Hua Li, Shui-Chao Lin, Yi-Mei Wen, Rong-Bin Huang, Su-Yuan Xie, and Lan-Sun Zheng pp 6122–6129 DOI: 10.1021/ja312133k Supporting Info |
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Pyrolysis Pathways of Sulfonated Polyethylene, an Alternative Carbon Fiber Precursor Jarod M. Younker, Tomonori Saito, Marcus A. Hunt, Amit K. Naskar, and Ariana Beste pp 6130–6141 DOI: 10.1021/ja3121845 Supporting Info |
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Understanding the Mechanism of the Asymmetric Propargylation of Aldehydes Promoted by 1,1′-Bi-2-naphthol-Derived Catalysts Matthew N. Grayson and Jonathan M. Goodman pp 6142–6148 DOI: 10.1021/ja3122137 Supporting Info |
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Pressure Modulation of Ras–Membrane Interactions and Intervesicle Transfer Shobhna Kapoor, Alexander Werkmüller, Roger S. Goody, Herbert Waldmann, and Roland Winter pp 6149–6156 DOI: 10.1021/ja312671j Supporting Info |
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Ultrathin 2D Coordination Polymer Nanosheets by Surfactant-Mediated Synthesis Sebastian C. Junggeburth, Leo Diehl, Stephan Werner, Viola Duppel, Wilfried Sigle, and Bettina V. Lotsch pp 6157–6164 DOI: 10.1021/ja312567v Supporting Info |
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Mapping the Thermal Behavior of DNA Origami Nanostructures Xixi Wei, Jeanette Nangreave, Shuoxing Jiang, Hao Yan, and Yan Liu pp 6165–6176 DOI: 10.1021/ja4000728 Supporting Info |
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Isomerization of Terminal Epoxides by a [Pd–H] Catalyst: A Combined Experimental and Theoretical Mechanistic Study Devendra J. Vyas, Evgeny Larionov, Céline Besnard, Laure Guénée, and Clément Mazet pp 6177–6183 DOI: 10.1021/ja400325w Supporting Info |
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Genetically Encoded Multispectral Labeling of Proteins with Polyfluorophores on a DNA Backbone Vijay Singh, Shenliang Wang, and Eric T. Kool pp 6184–6191 DOI: 10.1021/ja4004393 Supporting Info |
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Enzyme-Like Catalysis via Ternary Complex Mechanism: Alkoxy-Bridged Dinuclear Cobalt Complex Mediates Chemoselective O-Esterification over N-Amidation Yukiko Hayashi, Stefano Santoro, Yuki Azuma, Fahmi Himo, Takashi Ohshima, and Kazushi Mashima pp 6192–6199 DOI: 10.1021/ja400367h Supporting Info |
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Expanded Halogen-Bonded Anion Organic Networks with Star-Shaped Iodoethynyl-Substituted Molecules: From Corrugated 2D Hexagonal Lattices to Pyrite-Type 2-Fold Interpenetrated Cubic Lattices Julien Lieffrig, Olivier Jeannin, and Marc Fourmigué pp 6200–6210 DOI: 10.1021/ja400740v Supporting Info |
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Precision Templating with DNA of a Virus-like Particle with Peptide Nanostructures Yves Ruff, Tyson Moyer, Christina J. Newcomb, Borries Demeler, and Samuel I. Stupp pp 6211–6219 DOI: 10.1021/ja4008003 Supporting Info |
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Single-Electron Induces Double-Reaction by Charge Delocalization Kai Huang, Lydie Leung, Tingbin Lim, Zhanyu Ning, and John C. Polanyi pp 6220–6225 DOI: 10.1021/ja400612c Supporting Info |
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Competition of Charge- versus Radical-Directed Fragmentation of Gas-Phase Protonated Cysteine Sulfinyl Radicals Chasity B. Love, Lei Tan, Joseph S. Francisco, and Yu Xia pp 6226–6233 DOI: 10.1021/ja4008744 Supporting Info |
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Silver Nanoassemblies Constructed from Boranephosphonate DNA Subhadeep Roy, Magdalena Olesiak, Shiying Shang, and Marvin H. Caruthers pp 6234–6241 DOI: 10.1021/ja400898s Supporting Info |
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Comprehensive Experimental and Computational Analysis of Binding Energy Hot Spots at the NF-κB Essential Modulator/IKKβ Protein–Protein Interface Mary S. Golden, Shaun M. Cote, Marianna Sayeg, Brandon S. Zerbe, Elizabeth A. Villar, Dmitri Beglov, Stephen L. Sazinsky, Rosina M. Georgiadis, Sandor Vajda, Dima Kozakov, and Adrian Whitty pp 6242–6256 DOI: 10.1021/ja400914z Supporting Info |
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Mechanistic Study of Stepwise Methylisocyanide Coupling and C–H Activation Mediated by a Low-Valent Main Group Molecule Zachary D. Brown, Petra Vasko, Jeremy D. Erickson, James C. Fettinger, Heikki M. Tuononen, and Philip P. Power pp 6257–6261 DOI: 10.1021/ja4003553 Supporting Info |
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Diversity-oriented Synthesis of Inner Core Oligosaccharides of the Lipopolysaccharide of Pathogenic Gram-negative Bacteria You Yang, Shunsuke Oishi, Christopher E. Martin, and Peter H. Seeberger pp 6262–6271 DOI: 10.1021/ja401164s Supporting Info |
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Total Synthesis of Daptomycin by Cyclization via a Chemoselective Serine Ligation Hiu Yung Lam, Yinfeng Zhang, Han Liu, Jianchao Xu, Clarence T. T. Wong, Ci Xu, and Xuechen Li pp 6272–6279 DOI: 10.1021/ja4012468 Supporting Info |
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Effects of Pendant Ligand Binding Affinity on Chain Transfer for 1-Hexene Polymerization Catalyzed by Single-Site Zirconium Amine Bis-Phenolate Complexes D. Keith Steelman, Silei Xiong, Paul D. Pletcher, Erin Smith, Jeffrey M. Switzer, Grigori A. Medvedev, W. Nicholas Delgass, James M. Caruthers, and Mahdi M. Abu-Omar pp 6280–6288 DOI: 10.1021/ja401474v Supporting Info |
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Rational Design of Fatty Acid Amide Hydrolase Inhibitors That Act by Covalently Bonding to Two Active Site Residues Katerina Otrubova, Monica Brown, Michael S. McCormick, Gye W. Han, Scott T. O’Neal, Benjamin F. Cravatt, Raymond C. Stevens, Aron H. Lichtman, and Dale L. Boger pp 6289–6299 DOI: 10.1021/ja4014997 Supporting Info |
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Electron Transport via Cytochrome C on Si–H Surfaces: Roles of Fe and Heme Nadav Amdursky, Israel Pecht, Mordechai Sheves, and David Cahen pp 6300–6306 DOI: 10.1021/ja4015474 Supporting Info |
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Adsorption and Orientation of the Physiological Extracellular Peptide Glutathione Disulfide on Surface Functionalized Colloidal Alumina Particles Fabian Meder, Henrik Hintz, Yvonne Koehler, Maike M. Schmidt, Laura Treccani, Ralf Dringen, and Kurosch Rezwan pp 6307–6316 DOI: 10.1021/ja401590c Supporting Info |
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Electrophilic Aromatic Substitutions of Aryltrifluoroborates with Retention of the BF3– Group: Quantification of the Activating and Directing Effects of the Trifluoroborate Group Guillaume Berionni, Varvara Morozova, Maximilian Heininger, Peter Mayer, Paul Knochel, and Herbert Mayr pp 6317–6324 DOI: 10.1021/ja4017655 Supporting Info |
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Room Temperature Phosphorescence of Metal-Free Organic Materials in Amorphous Polymer Matrices Dongwook Lee, Onas Bolton, Byoung Choul Kim, Ji Ho Youk, Shuichi Takayama, and Jinsang Kim pp 6325–6329 DOI: 10.1021/ja401769g |
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“Texas-Sized” Molecular Boxes: Building Blocks for the Construction of Anion-Induced Supramolecular Species via Self-Assembly Han-Yuan Gong, Brett M. Rambo, Vincent M. Lynch, Karin M. Keller, and Jonathan L. Sessler pp 6330–6337 DOI: 10.1021/ja401893w Supporting Info |
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A Selective Turn-On Fluorescent Sensor for Sulfur Mustard Simulants Vinod Kumar and Eric V. Anslyn pp 6338–6344 DOI: 10.1021/ja401845e Supporting Info |
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The Interaction of Fluoride with Fluorogenic Ureas: An ON1–OFF–ON2 Response Valeria Amendola, Greta Bergamaschi, Massimo Boiocchi, Luigi Fabbrizzi, and Lorenzo Mosca pp 6345–6355 DOI: 10.1021/ja4019786 Supporting Info |
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Helicity-Selective Photoreaction of Single-Walled Carbon Nanotubes with Organosulfur Compounds in the Presence of Oxygen Yutaka Maeda, Junki Higo, Yuri Amagai, Jun Matsui, Kei Ohkubo, Yusuke Yoshigoe, Masahiro Hashimoto, Kazuhiro Eguchi, Michio Yamada, Tadashi Hasegawa, Yoshinori Sato, Jing Zhou, Jing Lu, Tokuji Miyashita, Shunichi Fukuzumi, Tatsuya Murakami, Kazuyuki Tohji, Shigeru Nagase, and Takeshi Akasaka pp 6356–6362 DOI: 10.1021/ja402199n Supporting Info |
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Pushing Extended p-Quinodimethanes to the Limit: Stable Tetracyano-oligo(N-annulated perylene)quinodimethanes with Tunable Ground States Zebing Zeng, Masatoshi Ishida, José L. Zafra, Xiaojian Zhu, Young Mo Sung, Nina Bao, Richard D. Webster, Byung Sun Lee, Run-Wei Li, Wangdong Zeng, Yuan Li, Chunyan Chi, Juan T. López Navarrete, Jun Ding, Juan Casado, Dongho Kim, and Jishan Wu pp 6363–6371 DOI: 10.1021/ja402467y Supporting Info |
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Adsorption of Small Organic Molecules on Graphene Petr Lazar, František Karlický, Petr Jurečka, Mikuláš Kocman, Eva Otyepková, Klára Šafářová, and Michal Otyepka pp 6372–6377 DOI: 10.1021/ja403162r Supporting Info |
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Correction to “Water Oxidation Electrocatalyzed by an Efficient Mn3O4/CoSe2 Nanocomposite” Min-Rui Gao, Yun-Fei Xu, Jun Jiang, Ya-Rong Zheng, and Shu-Hong Yu pp 6378–6378 DOI: 10.1021/ja4021815 |
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Spotlights on Recent JACS Publications pp 6379–6379 DOI: 10.1021/ja403997e |
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Redox-Linked Changes to the Hydrogen-Bonding Network of Ribonucleotide Reductase β2 Adam R. Offenbacher, Ellen C. Minnihan, JoAnne Stubbe, and Bridgette A. Barry pp 6380–6383 DOI: 10.1021/ja3032949 Supporting Info |
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Tolerance of Base Pair Size and Shape in Postlesion DNA Synthesis Hailey L. Gahlon, W. Bernd Schweizer, and Shana J. Sturla pp 6384–6387 DOI: 10.1021/ja311434s Supporting Info |
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A Mononuclear Non-Heme Manganese(IV)–Oxo Complex Binding Redox-Inactive Metal Ions Junying Chen, Yong-Min Lee, Katherine M. Davis, Xiujuan Wu, Mi Sook Seo, Kyung-Bin Cho, Heejung Yoon, Young Jun Park, Shunichi Fukuzumi, Yulia N. Pushkar, and Wonwoo Nam pp 6388–6391 DOI: 10.1021/ja312113p Supporting Info |
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Controlled pH Stability and Adjustable Cellular Uptake of Mixed-Charge Nanoparticles Pramod P. Pillai, Sabil Huda, Bartlomiej Kowalczyk, and Bartosz A. Grzybowski pp 6392–6395 DOI: 10.1021/ja4001272 Supporting Info |
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A CatalyCEST MRI Contrast Agent That Detects the Enzyme-Catalyzed Creation of a Covalent Bond Dina V. Hingorani, Edward A. Randtke, and Mark D. Pagel pp 6396–6398 DOI: 10.1021/ja400254e Supporting Info |
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A Switchable Surface Enables Visualization of Single DNA Hybridization Events with Atomic Force Microscopy Gary R. Abel, Jr., Eric A. Josephs, Norman Luong, and Tao Ye pp 6399–6402 DOI: 10.1021/ja401036t Supporting Info |
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Intermediate-Range Structure of Self-Assembled Cobalt-Based Oxygen-Evolving Catalyst Christopher L. Farrow, D. Kwabena Bediako, Yogesh Surendranath, Daniel G. Nocera, and Simon J. L. Billinge pp 6403–6406 DOI: 10.1021/ja401276f Supporting Info |
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Metastable Liquid Crystal as Time-Responsive Reaction Medium: Aging-Induced Dual Enantioselective Control Yasuhiro Ishida, Yuki Matsuoka, Yukiko Kai, Kuniyo Yamada, Kenta Nakagawa, Toru Asahi, and Kazuhiko Saigo pp 6407–6410 DOI: 10.1021/ja4016556 Supporting Info |
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Tunable Anisotropic Thermal Expansion of a Porous Zinc(II) Metal–Organic Framework Ilne Grobler, Vincent J. Smith, Prashant M. Bhatt, Simon A. Herbert, and Leonard J. Barbour pp 6411–6414 DOI: 10.1021/ja401671p Supporting Info |
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Chemoselective Metal-Free Aerobic Alcohol Oxidation in Lignin Alireza Rahimi, Ali Azarpira, Hoon Kim, John Ralph, and Shannon S. Stahl pp 6415–6418 DOI: 10.1021/ja401793n Supporting Info |
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Catalytic, Enantioselective, Intramolecular Carbosulfenylation of Olefins Scott E. Denmark and Alex Jaunet pp 6419–6422 DOI: 10.1021/ja401867b Supporting Info |
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Direct Measurement of Sequential Folding Pathway and Energy Landscape of Human Telomeric G-quadruplex Structures Wei Li, Xi-Miao Hou, Peng-Ye Wang, Xu-Guang Xi, and Ming Li pp 6423–6426 DOI: 10.1021/ja4019176 Supporting Info |
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Mechanistic Study of the Oxidative Coupling of Styrene with 2-Phenylpyridine Derivatives Catalyzed by Cationic Rhodium(III) via C–H Activation Mikaël Brasse, Juan Cámpora, Jonathan A. Ellman, and Robert G. Bergman pp 6427–6430 DOI: 10.1021/ja401561q Supporting Info |
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Fractal Etching of Graphene Dechao Geng, Bin Wu, Yunlong Guo, Birong Luo, Yunzhou Xue, Jianyi Chen, Gui Yu, and Yunqi Liu pp 6431–6434 DOI: 10.1021/ja402224h Supporting Info |
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Geminal Tetraauration of Acetonitrile: Hemilabile-Phosphine-Stabilized Au8Ag4 Cluster Compounds Xiao-Li Pei, Yang Yang, Zhen Lei, and Quan-Ming Wang pp 6435–6437 DOI: 10.1021/ja402352c Supporting Info |
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Rate-Determining Water-Assisted O–O Bond Cleavage of an FeIII-OOH Intermediate in a Bio-inspired Nonheme Iron-Catalyzed Oxidation Williamson N. Oloo, Andrew J. Fielding, and Lawrence Que, Jr. pp 6438–6441 DOI: 10.1021/ja402759c Supporting Info |
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Nine-Step Enantioselective Total Synthesis of (−)-Vincorine Benjamin D. Horning and David W. C. MacMillan pp 6442–6445 DOI: 10.1021/ja402933s Supporting Info |
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C–H Bond Activation by Radical Ion Pairs Derived from R3P/Al(C6F5)3 Frustrated Lewis Pairs and N2O Gabriel Ménard, Jillian A. Hatnean, Hugh J. Cowley, Alan J. Lough, Jeremy M. Rawson, and Douglas W. Stephan pp 6446–6449 DOI: 10.1021/ja402964h Supporting Info |
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A Synthetic Receptor for Asymmetric Dimethyl Arginine Lindsey I. James, Joshua E. Beaver, Natalie W. Rice, and Marcey L. Waters pp 6450–6455 DOI: 10.1021/ja307907p Supporting Info |
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A Mechanistic Model for Amorphous Protein Aggregation of Immunoglobulin-like Domains Madeleine B. Borgia, Adrian A. Nickson, Jane Clarke, and Michael J. Hounslow pp 6456–6464 DOI: 10.1021/ja308852b Supporting Info |
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Reactions of a Cationic Geminal Zr+/P Pair with Small Molecules Xin Xu, Gerald Kehr, Constantin G. Daniliuc, and Gerhard Erker pp 6465–6476 DOI: 10.1021/ja3110076 Supporting Info |
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A (3 + 3)-Dimensional “Hypercubic” Oxide-Ionic Conductor: Type II Bi2O3–Nb2O5 Chris D. Ling, Siegbert Schmid, Peter E. R. Blanchard, Vaclav Petříček, Garry J. McIntyre, Neeraj Sharma, Andrey Maljuk, Aleksey A. Yaremchenko, Vladislav V. Kharton, Matthias Gutmann, and Ray L. Withers pp 6477–6484 DOI: 10.1021/ja3109328 Supporting Info |
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On the Influence of Water on the Electronic Structure of Firefly Oxyluciferin Anions from Absorption Spectroscopy of Bare and Monohydrated Ions in Vacuo Kristian Støchkel, Christian Nygaard Hansen, Jørgen Houmøller, Lisbeth Munksgaard Nielsen, Kelvin Anggara, Mathieu Linares, Patrick Norman, Fernando Nogueira, Oleg V. Maltsev, Lukas Hintermann, Steen Brøndsted Nielsen, Panče Naumov, and Bruce F. Milne pp 6485–6493 DOI: 10.1021/ja311400t Supporting Info |
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Rattle-Structured Multifunctional Nanotheranostics for Synergetic Chemo-/Radiotherapy and Simultaneous Magnetic/Luminescent Dual-Mode Imaging Wenpei Fan, Bo Shen, Wenbo Bu, Feng Chen, Kuaile Zhao, Shengjian Zhang, Liangping Zhou, Weijun Peng, Qingfeng Xiao, Huaiyong Xing, Jianan Liu, Dalong Ni, Qianjun He, and Jianlin Shi pp 6494–6503 DOI: 10.1021/ja312225b Supporting Info |
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Epitope-distal Effects Accompany the Binding of Two Distinct Antibodies to Hepatitis B Virus Capsids Jessica Z. Bereszczak, Rebecca J. Rose, Esther van Duijn, Norman R. Watts, Paul T. Wingfield, Alasdair C. Steven, and Albert J. R. Heck pp 6504–6512 DOI: 10.1021/ja402023x Supporting Info |
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Enhanced Catalytic Four-Electron Dioxygen (O2) and Two-Electron Hydrogen Peroxide (H2O2) Reduction with a Copper(II) Complex Possessing a Pendant Ligand Pivalamido Group Saya Kakuda, Ryan L. Peterson, Kei Ohkubo, Kenneth D. Karlin, and Shunichi Fukuzumi pp 6513–6522 DOI: 10.1021/ja3125977 Supporting Info |
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Free-Standing, Single-Monomer-Thick Two-Dimensional Polymers through Covalent Self-Assembly in Solution Kangkyun Baek, Gyeongwon Yun, Youngkook Kim, Dongwoo Kim, Raghunandan Hota, Ilha Hwang, Dan Xu, Young Ho Ko, Gil Ho Gu, Ju Hyung Suh, Chan Gyung Park, Bong June Sung, and Kimoon Kim pp 6523–6528 DOI: 10.1021/ja4002019 Supporting Info |
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Labeling Proteins with Fluorophore/Thioamide Förster Resonant Energy Transfer Pairs by Combining Unnatural Amino Acid Mutagenesis and Native Chemical Ligation Rebecca F. Wissner, Solongo Batjargal, Colin M. Fadzen, and E. James Petersson pp 6529–6540 DOI: 10.1021/ja4005943 Supporting Info |
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Differential Role of the Protein Matrix on the Binding of a Catalytic Aspartate to Mg2+ vs Ca2+: Application to Ribonuclease H C. Satheesan Babu, Todor Dudev, and Carmay Lim pp 6541–6548 DOI: 10.1021/ja4006095 Supporting Info |
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Supramolecular Autoregulation Francisco Rodríguez-Llansola and E. W. Meijer pp 6549–6553 DOI: 10.1021/ja4006833 Supporting Info |
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A Selective Blocking Method To Control the Overgrowth of Pt on Au Nanorods John Fennell, Dongsheng He, Anicetus Muche Tanyi, Andrew J. Logsdail, Roy L. Johnston, Z. Y. Li, and Sarah L. Horswell pp 6554–6561 DOI: 10.1021/ja4003475 Supporting Info |
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Bicyclic Peptide Ligands Pulled out of Cysteine-Rich Peptide Libraries Shiyu Chen, Inmaculada Rentero Rebollo, Sergey A. Buth, Julia Morales-Sanfrutos, Jeremy Touati, Petr G. Leiman, and Christian Heinis pp 6562–6569 DOI: 10.1021/ja400461h Supporting Info |
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3-Trimethylsilylcyclobutylidene. The γ-Effect of Silicon on Carbenes Xavier Creary pp 6570–6578 DOI: 10.1021/ja400747u Supporting Info |
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Electrophilicities of Benzaldehyde-Derived Iminium Ions: Quantification of the Electrophilic Activation of Aldehydes by Iminium Formation Roland Appel, Saloua Chelli, Takahiro Tokuyasu, Konstantin Troshin, and Herbert Mayr pp 6579–6587 DOI: 10.1021/ja401106x Supporting Info |
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Mechanism and Origins of Selectivity in Ru(II)-Catalyzed Intramolecular (5+2) Cycloadditions and Ene Reactions of Vinylcyclopropanes and Alkynes from Density Functional Theory Xin Hong, Barry M. Trost, and K. N. Houk pp 6588–6600 DOI: 10.1021/ja4012657 Supporting Info |
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Synthesis, Electrochemistry, and Photophysics of a Family of Phlorin Macrocycles That Display Cooperative Fluoride Binding Allen J. Pistner, Daniel A. Lutterman, Michael J. Ghidiu, Ying-Zhong Ma, and Joel Rosenthal pp 6601–6607 DOI: 10.1021/ja401391z Supporting Info |
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A Facile Strategy To Design Zeolite L Crystals with Tunable Morphology and Surface Architecture Alexandra I. Lupulescu, Manjesh Kumar, and Jeffrey D. Rimer pp 6608–6617 DOI: 10.1021/ja4015277 Supporting Info |
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A Detailed Study of Acetate-Assisted C–H Activation at Palladium(IV) Centers Ansis Maleckis, Jeff W. Kampf, and Melanie S. Sanford pp 6618–6625 DOI: 10.1021/ja401557m Supporting Info |
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Photoinduced and Thermal Denitrogenation of Bulky Triazoline Crystals: Insights into Solid-to-Solid Transformation Denisse de Loera, Antoine Stopin, and Miguel A. Garcia-Garibay pp 6626–6632 DOI: 10.1021/ja401577p Supporting Info |
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Mechanism of Alkoxy Groups Substitution by Grignard Reagents on Aromatic Rings and Experimental Verification of Theoretical Predictions of Anomalous Reactions Gonzalo Jiménez-Osés, Anthony J. Brockway, Jared T. Shaw, and K. N. Houk pp 6633–6642 DOI: 10.1021/ja4015937 Supporting Info |
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Permanent Fixing or Reversible Trapping and Release of DNA Micropatterns on a Gold Nanostructure Using Continuous-Wave or Femtosecond-Pulsed Near-Infrared Laser Light Tatsuya Shoji, Junki Saitoh, Noboru Kitamura, Fumika Nagasawa, Kei Murakoshi, Hiroaki Yamauchi, Syoji Ito, Hiroshi Miyasaka, Hajime Ishihara, and Yasuyuki Tsuboi pp 6643–6648 DOI: 10.1021/ja401657j Supporting Info |
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Striped, Ellipsoidal Particles by Controlled Assembly of Diblock Copolymers Se Gyu Jang, Debra J. Audus, Daniel Klinger, Daniel V. Krogstad, Bumjoon J. Kim, Alexandre Cameron, Sang-Woo Kim, Kris T. Delaney, Su-Mi Hur, Kato L. Killops, Glenn H. Fredrickson, Edward J. Kramer, and Craig J. Hawker pp 6649–6657 DOI: 10.1021/ja4019447 Supporting Info |
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Theoretical Exploration of the Mechanism of Riboflavin Formation from 6,7-Dimethyl-8-ribityllumazine: Nucleophilic Catalysis, Hydride Transfer, Hydrogen Atom Transfer, or Nucleophilic Addition? Martin Breugst, Albert Eschenmoser, and K. N. Houk pp 6658–6668 DOI: 10.1021/ja402099f Supporting Info |
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Seed-Mediated Growth of Shape-Controlled Wurtzite CdSe Nanocrystals: Platelets, Cubes, and Rods Katherine P. Rice, Aaron E. Saunders, and Mark P. Stoykovich pp 6669–6676 DOI: 10.1021/ja402240m Supporting Info |
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The Cinchona Primary Amine-Catalyzed Asymmetric Epoxidation and Hydroperoxidation of α,β-Unsaturated Carbonyl Compounds with Hydrogen Peroxide Olga Lifchits, Manuel Mahlau, Corinna M. Reisinger, Anna Lee, Christophe Farès, Iakov Polyak, Gopinadhanpillai Gopakumar, Walter Thiel, and Benjamin List pp 6677–6693 DOI: 10.1021/ja402058v Supporting Info |
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Photophysical Properties of Self-Assembled Multinuclear Platinum Metallacycles with Different Conformational Geometries Jun-Sheng Chen, Guang-Jiu Zhao, Timothy R. Cook, Ke-Li Han, and Peter J. Stang pp 6694–6702 DOI: 10.1021/ja402421w Supporting Info |
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Electron-Rich N-Heterocyclic Silylene (NHSi)–Iron Complexes: Synthesis, Structures, and Catalytic Ability of an Isolable Hydridosilylene–Iron Complex Burgert Blom, Stephan Enthaler, Shigeyoshi Inoue, Elisabeth Irran, and Matthias Driess pp 6703–6713 DOI: 10.1021/ja402480v Supporting Info |
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The Role of Arene–Arene Interactions in the Folding of ortho-Phenylenes Sanyo M. Mathew, James T. Engle, Christopher J. Ziegler, and C. Scott Hartley pp 6714–6722 DOI: 10.1021/ja4026006 Supporting Info |
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Spotlights on Recent JACS Publications pp 6723–6723 DOI: 10.1021/ja404289d |
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Integrated Materials Design of Organic Semiconductors for Field-Effect Transistors Jianguo Mei, Ying Diao, Anthony L. Appleton, Lei Fang, and Zhenan Bao pp 6724–6746 DOI: 10.1021/ja400881n |
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Enantioselective Thiourea-Catalyzed Intramolecular Cope-Type Hydroamination Adam R. Brown, Christopher Uyeda, Carolyn A. Brotherton, and Eric N. Jacobsen pp 6747–6749 DOI: 10.1021/ja402893z Supporting Info |
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Probing Carbon Nanotube–Surfactant Interactions with Two-Dimensional DOSY NMR Tejas A. Shastry, Adam J. Morris-Cohen, Emily A. Weiss, and Mark C. Hersam pp 6750–6753 DOI: 10.1021/ja312235n Supporting Info |
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N–N Bond Cleavage of Hydrazines with a Multiproton-Responsive Pincer-Type Iron Complex Kazuki Umehara, Shigeki Kuwata, and Takao Ikariya pp 6754–6757 DOI: 10.1021/ja3122944 Supporting Info |
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Atomic Resolution Imaging of Grain Boundary Defects in Monolayer Chemical Vapor Deposition-Grown Hexagonal Boron Nitride Ashley L. Gibb, Nasim Alem, Jian-Hao Chen, Kristopher J. Erickson, Jim Ciston, Abhay Gautam, Martin Linck, and Alex Zettl pp 6758–6761 DOI: 10.1021/ja400637n Supporting Info |
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Low-Temperature Reactivity of Zn+ Ions Confined in ZSM-5 Zeolite toward Carbon Monoxide Oxidation: Insight from in Situ DRIFT and ESR Spectroscopy Guodong Qi, Jun Xu, Jihu Su, Jiafu Chen, Xiumei Wang, and Feng Deng pp 6762–6765 DOI: 10.1021/ja400757c Supporting Info |
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Characterizing the Protonation State of Cytosine in Transient G·C Hoogsteen Base Pairs in Duplex DNA Evgenia N. Nikolova, Garrett B. Goh, Charles L. Brooks, III, and Hashim M. Al-Hashimi pp 6766–6769 DOI: 10.1021/ja400994e Supporting Info |
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Spirobis(pentagerma[1.1.1]propellane): A Stable Tetraradicaloid Yuki Ito, Vladimir Ya. Lee, Heinz Gornitzka, Catharina Goedecke, Gernot Frenking, and Akira Sekiguchi pp 6770–6773 DOI: 10.1021/ja401650q Supporting Info |
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Sequential C–H Functionalization Reactions for the Enantioselective Synthesis of Highly Functionalized 2,3-Dihydrobenzofurans Hengbin Wang, Gang Li, Keary M. Engle, Jin-Quan Yu, and Huw M. L. Davies pp 6774–6777 DOI: 10.1021/ja401731d Supporting Info |
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Nanoscale Growth and Patterning of Inorganic Oxides Using DNA Nanostructure Templates Sumedh P. Surwade, Feng Zhou, Bryan Wei, Wei Sun, Anna Powell, Christina O’Donnell, Peng Yin, and Haitao Liu pp 6778–6781 DOI: 10.1021/ja401785h Supporting Info |
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Fluorophore Labeling of Native FKBP12 by Ligand-Directed Tosyl Chemistry Allows Detection of Its Molecular Interactions in Vitro and in Living Cells Tomonori Tamura, Yoshiyuki Kioi, Takayuki Miki, Shinya Tsukiji, and Itaru Hamachi pp 6782–6785 DOI: 10.1021/ja401956b Supporting Info |
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Size-, Mass-, and Density-Controlled Preparation of TiO2 Nanoparticles in a Spherical Coordination Template Tatsuya Ichijo, Sota Sato, and Makoto Fujita pp 6786–6789 DOI: 10.1021/ja4019995 Supporting Info |
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Direct Calorimetric Measurement of Enthalpy of Adsorption of Carbon Dioxide on CD-MOF-2, a Green Metal–Organic Framework Di Wu, Jeremiah J. Gassensmith, Douglas Gouvêa, Sergey Ushakov, J. Fraser Stoddart, and Alexandra Navrotsky pp 6790–6793 DOI: 10.1021/ja402315d |
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Crystal Structure of the Complex between Prokaryotic Ubiquitin-like Protein and Its Ligase PafA Jonas Barandun, Cyrille L. Delley, Nenad Ban, and Eilika Weber-Ban pp 6794–6797 DOI: 10.1021/ja4024012 Supporting Info |
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Anisotropic Self-Assembly of Gold Nanoparticle Grafted with Polyisoprene and Polystyrene Having Symmetric Polymer Composition Tatsuhiro Nakano, Daisuke Kawaguchi, and Yushu Matsushita pp 6798–6801 DOI: 10.1021/ja402412q Supporting Info |
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Catalytic Asymmetric Synthesis of Pyrroloindolines via a Rhodium(II)-Catalyzed Annulation of Indoles Jillian E. Spangler and Huw M. L. Davies pp 6802–6805 DOI: 10.1021/ja4025337 Supporting Info |
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Synthesis of Atactic and Isotactic Poly(1,2-glycerol carbonate)s: Degradable Polymers for Biomedical and Pharmaceutical Applications Heng Zhang and Mark W. Grinstaff pp 6806–6809 DOI: 10.1021/ja402558m Supporting Info |
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Chiral Dienes as “Ligands” for Borane-Catalyzed Metal-Free Asymmetric Hydrogenation of Imines Yongbing Liu and Haifeng Du pp 6810–6813 DOI: 10.1021/ja4025808 Supporting Info |
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Ruthenium-Catalyzed Intramolecular Hydrocarbamoylation of Allylic Formamides: Convenient Access to Chiral Pyrrolidones Nicolas Armanino and Erick M. Carreira pp 6814–6817 DOI: 10.1021/ja4026787 Supporting Info |
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On the Effect of a Single Solvent Molecule on the Charge-Transfer Band of a Donor–Acceptor Anion Jørgen Houmøller, Marius Wanko, Kristian Støchkel, Angel Rubio, and Steen Brøndsted Nielsen pp 6818–6821 DOI: 10.1021/ja4025275 Supporting Info |
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Spontaneous Partition of Carbon Nanotubes in Polymer-Modified Aqueous Phases Constantine Y Khripin, Jeffrey A. Fagan, and Ming Zheng pp 6822–6825 DOI: 10.1021/ja402762e Supporting Info |
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Polycarbonates Derived from Glucose via an Organocatalytic Approach Koichiro Mikami, Alexander T. Lonnecker, Tiffany P. Gustafson, Nathanael F. Zinnel, Pei-Jing Pai, David H. Russell, and Karen L. Wooley pp 6826–6829 DOI: 10.1021/ja402319m Supporting Info |
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Enantioselective Redox-Relay Oxidative Heck Arylations of Acyclic Alkenyl Alcohols using Boronic Acids Tian-Sheng Mei, Erik W. Werner, Alexander J. Burckle, and Matthew S. Sigman pp 6830–6833 DOI: 10.1021/ja402916z Supporting Info |
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Self-Adjustable Crystalline Inorganic Nanocoils Peng-peng Wang, Yong Yang, Jing Zhuang, and Xun Wang pp 6834–6837 DOI: 10.1021/ja403065z Supporting Info |
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Selective Detection of Allosteric Phosphatase Inhibitors Ralf Schneider, Claudia Beumer, Jeffrey R. Simard, Christian Grütter, and Daniel Rauh pp 6838–6841 DOI: 10.1021/ja4030484 Supporting Info |
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A Hybrid Soft Solar Cell Based on the Mycobacterial Porin MspA Linked to a Sensitizer–Viologen Diad Ayomi S. Perera, Navaneetha K. Subbaiyan, Mausam Kalita, Sebastian O. Wendel, Thilani N. Samarakoon, Francis D’Souza, and Stefan H. Bossmann pp 6842–6845 DOI: 10.1021/ja403090x Supporting Info |
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A Hydrophobic Surface Is Essential To Inhibit the Aggregation of a Tau-Protein-Derived Hexapeptide Jing Zheng, Arya M. Baghkhanian, and James S. Nowick pp 6846–6852 DOI: 10.1021/ja310817d Supporting Info |
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Bilayer Thickness Mismatch Controls Domain Size in Model Membranes Frederick A. Heberle, Robin S. Petruzielo, Jianjun Pan, Paul Drazba, Norbert Kučerka, Robert F. Standaert, Gerald W. Feigenson, and John Katsaras pp 6853–6859 DOI: 10.1021/ja3113615 Supporting Info |
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Polymorph-Specific Kinetics and Thermodynamics of β-Amyloid Fibril Growth Wei Qiang, Kevin Kelley, and Robert Tycko pp 6860–6871 DOI: 10.1021/ja311963f Supporting Info |
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Helicity as a Steric Force: Stabilization and Helicity-Dependent Reversion of Colored o-Quinonoid Intermediates of Helical Chromenes Jarugu Narasimha Moorthy, Susovan Mandal, Arindam Mukhopadhyay, and Subhas Samanta pp 6872–6884 DOI: 10.1021/ja312027c Supporting Info |
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Structure and Stability of SnO2 Nanocrystals and Surface-Bound Water Species Hsiu-Wen Wang, David J. Wesolowski, Thomas E. Proffen, Lukas Vlcek, Wei Wang, Lawrence F. Allard, Alexander I. Kolesnikov, Mikhail Feygenson, Lawrence M. Anovitz, and Rick L. Paul pp 6885–6895 DOI: 10.1021/ja312030e Supporting Info |
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Metal–Organic Framework Luminescence in the Yellow Gap by Codoping of the Homoleptic Imidazolate ∞3[Ba(Im)2] with Divalent Europium Jens-Christoph Rybak, Michael Hailmann, Philipp R. Matthes, Alexander Zurawski, Jörn Nitsch, Andreas Steffen, Joachim G. Heck, Claus Feldmann, Stefan Götzendörfer, Jürgen Meinhardt, Gerhard Sextl, Holger Kohlmann, Stefan J. Sedlmaier, Wolfgang Schnick, and Klaus Müller-Buschbaum pp 6896–6902 DOI: 10.1021/ja3121718 Supporting Info |
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Photosystem II Does Not Possess a Simple Excitation Energy Funnel: Time-Resolved Fluorescence Spectroscopy Meets Theory Yutaka Shibata, Shunsuke Nishi, Keisuke Kawakami, Jian-Ren Shen, and Thomas Renger pp 6903–6914 DOI: 10.1021/ja312586p Supporting Info |
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Molecular Solution Approach To Synthesize Electronic Quality Cu2ZnSnS4 Thin Films Wenbing Yang, Hsin-Sheng Duan, Kitty C. Cha, Chia-Jung Hsu, Wan-Ching Hsu, Huanping Zhou, Brion Bob, and Yang Yang pp 6915–6920 DOI: 10.1021/ja312678c Supporting Info |
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EPR and FTIR Analysis of the Mechanism of H2 Activation by [FeFe]-Hydrogenase HydA1 from Chlamydomonas reinhardtii David W. Mulder, Michael W. Ratzloff, Eric M. Shepard, Amanda S. Byer, Seth M. Noone, John W. Peters, Joan B. Broderick, and Paul W. King pp 6921–6929 DOI: 10.1021/ja4000257 Supporting Info |
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Thermal Stability of Li2B12H12 and its Role in the Decomposition of LiBH4 Mark P. Pitt, Mark Paskevicius, David H. Brown, Drew A. Sheppard, and Craig E. Buckley pp 6930–6941 DOI: 10.1021/ja400131b Supporting Info |
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Concentration-Dependent Supramolecular Engineering of Hydrogen-Bonded Nanostructures at Surfaces: Predicting Self-Assembly in 2D Artur Ciesielski, Paweł J. Szabelski, Wojciech Rżysko, Andrea Cadeddu, Timothy R. Cook, Peter J. Stang, and Paolo Samorì pp 6942–6950 DOI: 10.1021/ja4002025 Supporting Info |
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The Effect and Role of Carbon Atoms in Poly(β-amino ester)s for DNA Binding and Gene Delivery Corey J. Bishop, Tiia-Maaria Ketola, Stephany Y. Tzeng, Joel C. Sunshine, Arto Urtti, Helge Lemmetyinen, Elina Vuorimaa-Laukkanen, Marjo Yliperttula, and Jordan J. Green pp 6951–6957 DOI: 10.1021/ja4002376 Supporting Info |
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Intra- and Intermolecular Charge Transfer in Aggregates of Tetrathiafulvalene-Triphenylmethyl Radical Derivatives in Solution Judith Guasch, Luca Grisanti, Manuel Souto, Vega Lloveras, José Vidal-Gancedo, Imma Ratera, Anna Painelli, Concepció Rovira, and Jaume Veciana pp 6958–6967 DOI: 10.1021/ja400281b Supporting Info |
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Ultrafast Infrared Spectroscopy on Channelrhodopsin-2 Reveals Efficient Energy Transfer from the Retinal Chromophore to the Protein Mirka-Kristin Neumann-Verhoefen, Karsten Neumann, Christian Bamann, Ionela Radu, Joachim Heberle, Ernst Bamberg, and Josef Wachtveitl pp 6968–6976 DOI: 10.1021/ja400554y |
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Macromolecular Amplification of Binding Response in Superaptamer Hydrogels Wei Bai, Nicholas A. Gariano, and David A. Spivak pp 6977–6984 DOI: 10.1021/ja400576p Supporting Info |
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PNA-Peptide Assembly in a 3D DNA Nanocage at Room Temperature Justin D. Flory, Sandip Shinde, Su Lin, Yan Liu, Hao Yan, Giovanna Ghirlanda, and Petra Fromme pp 6985–6993 DOI: 10.1021/ja400762c Supporting Info |
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Rhodium–Carbon Bond Energies in Tp′Rh(CNneopentyl)(CH2X)H: Quantifying Stabilization Effects in M–C Bonds Yunzhe Jiao, Meagan E. Evans, James Morris, William W. Brennessel, and William D. Jones pp 6994–7004 DOI: 10.1021/ja400966y Supporting Info |
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Are Halogen Bonded Structures Electrostatically Driven? Anthony J. Stone pp 7005–7009 DOI: 10.1021/ja401420w Supporting Info |
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Mononuclear Single-Molecule Magnets: Tailoring the Magnetic Anisotropy of First-Row Transition-Metal Complexes Silvia Gomez-Coca, Eduard Cremades, Núria Aliaga-Alcalde, and Eliseo Ruiz pp 7010–7018 DOI: 10.1021/ja4015138 Supporting Info |
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Identification of a Cyclic Nucleotide as a Cryptic Intermediate in Molybdenum Cofactor Biosynthesis Bradley M. Hover, Anna Loksztejn, Anthony A. Ribeiro, and Kenichi Yokoyama pp 7019–7032 DOI: 10.1021/ja401781t Supporting Info |
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Impact of Preferential Indium Nucleation on Electrical Conductivity of Vapor–Liquid–Solid Grown Indium–Tin Oxide Nanowires Gang Meng, Takeshi Yanagida, Kazuki Nagashima, Hideto Yoshida, Masaki Kanai, Annop Klamchuen, Fuwei Zhuge, Yong He, Sakon Rahong, Xiaodong Fang, Seiji Takeda, and Tomoji Kawai pp 7033–7038 DOI: 10.1021/ja401926u Supporting Info |
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Quantitative Understanding of Guest Binding Enables the Design of Complex Host–Guest Behavior Maarten M. J. Smulders, Salvatore Zarra, and Jonathan R. Nitschke pp 7039–7046 DOI: 10.1021/ja402084x Supporting Info |
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Cooperative Adsorption of Lipoprotein Phospholipids, Triglycerides, and Cholesteryl Esters Are a Key Factor in Nonspecific Adsorption from Blood Plasma to Antifouling Polymer Surfaces Gesine Gunkel and Wilhelm T. S. Huck pp 7047–7052 DOI: 10.1021/ja402126t Supporting Info |
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Substrate-Assisted and Nucleophilically Assisted Catalysis in Bovine α1,3-Galactosyltransferase. Mechanistic Implications for Retaining Glycosyltransferases Hansel Gómez, José M. Lluch, and Laura Masgrau pp 7053–7063 DOI: 10.1021/ja4024447 Supporting Info |
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Theory of Polymer–Nanopore Interactions Refined Using Molecular Dynamics Simulations Arvind Balijepalli, Joseph W. F. Robertson, Joseph E. Reiner, John J. Kasianowicz, and Richard W. Pastor pp 7064–7072 DOI: 10.1021/ja4026193 |
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The Activation Mechanism of Ru–Indenylidene Complexes in Olefin Metathesis César A. Urbina-Blanco, Albert Poater, Tomas Lebl, Simone Manzini, Alexandra M. Z. Slawin, Luigi Cavallo, and Steven P. Nolan pp 7073–7079 DOI: 10.1021/ja402700p Supporting Info |
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Correction to “Temperature-Dependent Spin Crossover in Neuronal Nitric Oxide Synthase Bound with the Heme-Coordinating Thioether Inhibitors” Tzanko Doukov, Huiying Li, Ajay Sharma, Jeffrey D. Martell, S. Michael Soltis, Richard B. Silverman, and Thomas L. Poulos pp 7080–7080 DOI: 10.1021/ja3105472 |
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Spotlights on Recent JACS Publications pp 7081–7081 DOI: 10.1021/ja404575r |
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2-Bromopalmitate Analogues as Activity-Based Probes To Explore Palmitoyl Acyltransferases Baohui Zheng, Michael DeRan, Xinyan Li, Xuebin Liao, Masaki Fukata, and Xu Wu pp 7082–7085 DOI: 10.1021/ja311416v Supporting Info |
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Transition-Metal-Free Direct Arylation: Synthesis of Halogenated 2-Amino-2′-hydroxy-1,1′-biaryls and Mechanism by DFT Calculations Hongyin Gao, Daniel H. Ess, Muhammed Yousufuddin, and László Kürti pp 7086–7089 DOI: 10.1021/ja400897u Supporting Info |
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Selective Cavitand-Mediated Endocytosis of Targeted Imaging Agents into Live Cells Yoo-Jin Ghang, Michael P. Schramm, Fan Zhang, Roger A. Acey, Clement N. David, Emma H. Wilson, Yinsheng Wang, Quan Cheng, and Richard J. Hooley pp 7090–7093 DOI: 10.1021/ja401273g Supporting Info |
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Chemical Synthesis of the Lantibiotic Lacticin 481 Reveals the Importance of Lanthionine Stereochemistry Patrick J. Knerr and Wilfred A. van der Donk pp 7094–7097 DOI: 10.1021/ja4014024 Supporting Info |
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CuTe Nanocrystals: Shape and Size Control, Plasmonic Properties, and Use as SERS Probes and Photothermal Agents Wenhua Li, Reza Zamani, Pilar Rivera Gil, Beatriz Pelaz, Maria Ibáñez, Doris Cadavid, Alexey Shavel, Ramon A. Alvarez-Puebla, Wolfgang J. Parak, Jordi Arbiol, and Andreu Cabot pp 7098–7101 DOI: 10.1021/ja401428e Supporting Info |
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Asymmetric Induction via Short-Lived Chiral Enolates with a Chiral C–O Axis Tomoyuki Yoshimura, Keisuke Tomohara, and Takeo Kawabata pp 7102–7105 DOI: 10.1021/ja4018122 Supporting Info |
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Structural Characterization and Unusual Reactivity of Oxosulfido-Mo(V) Compounds: Implications for the Structure and Electronic Description of the Very Rapid Form of Xanthine Oxidase Victor W. L. Ng, Jonathan M. White, and Charles G. Young pp 7106–7109 DOI: 10.1021/ja4022057 Supporting Info |
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Magnetic Differentiation of Pyrogallol[4]arene Tubular and Capsular Frameworks Harshita Kumari, Cindi L. Dennis, Andrew V. Mossine, Carol A. Deakyne, and Jerry L. Atwood pp 7110–7113 DOI: 10.1021/ja402496x |
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Long-Chain Terminal Alcohols through Catalytic CO Hydrogenation Yizhi Xiang, Véronique Chitry, Peter Liddicoat, Peter Felfer, Julie Cairney, Simon Ringer, and Norbert Kruse pp 7114–7117 DOI: 10.1021/ja402512r Supporting Info |
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Improving Carbon Nitride Photocatalysis by Supramolecular Preorganization of Monomers Menny Shalom, Sahika Inal, Christian Fettkenhauer, Dieter Neher, and Markus Antonietti pp 7118–7121 DOI: 10.1021/ja402521s Supporting Info |
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Rhodium(III)-Catalyzed Indazole Synthesis by C–H Bond Functionalization and Cyclative Capture Yajing Lian, Robert G. Bergman, Luke D. Lavis, and Jonathan A. Ellman pp 7122–7125 DOI: 10.1021/ja402761p Supporting Info |
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Catalytic Enantioselective Carbon Insertion into the β-Vinyl C–H Bond of Cyclic Enones Sung Il Lee, Geum-Sook Hwang, and Do Hyun Ryu pp 7126–7129 DOI: 10.1021/ja402873b Supporting Info |
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Synthetic Control of FePtM Nanorods (M = Cu, Ni) To Enhance the Oxygen Reduction Reaction Huiyuan Zhu, Sen Zhang, Shaojun Guo, Dong Su, and Shouheng Sun pp 7130–7133 DOI: 10.1021/ja403041g Supporting Info |
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Construction of a Chiral Quaternary Carbon Center by Catalytic Asymmetric Alkylation of 2-Arylcyclohexanones under Phase-Transfer Conditions Taichi Kano, Yumi Hayashi, and Keiji Maruoka pp 7134–7137 DOI: 10.1021/ja403340r Supporting Info |
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Uncovering the Enzymes that Catalyze the Final Steps in Oxytetracycline Biosynthesis Peng Wang, Ghader Bashiri, Xue Gao, Michael R. Sawaya, and Yi Tang pp 7138–7141 DOI: 10.1021/ja403516u Supporting Info |
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Oxidative Addition of a Strained C–C Bond onto Electron-Rich Rhodium(I) at Room Temperature Yusuke Masuda, Maki Hasegawa, Makoto Yamashita, Kyoko Nozaki, Naoki Ishida, and Masahiro Murakami pp 7142–7145 DOI: 10.1021/ja403461f Supporting Info |
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Unraveling the Enigmatic Mechanism of l-Asparaginase II with QM/QM Calculations Diana S. Gesto, Nuno M. F. S. A. Cerqueira, Pedro A. Fernandes, and Maria J. Ramos pp 7146–7158 DOI: 10.1021/ja310165u Supporting Info |
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Contact Line Motion on Nanorough Surfaces: A Thermally Activated Process Melanie Ramiasa, John Ralston, Renate Fetzer, Rossen Sedev, Doris M. Fopp-Spori, Christoph Morhard, Claudia Pacholski, and Joachim P. Spatz pp 7159–7171 DOI: 10.1021/ja3104846 Supporting Info |
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Molecular-level Insight into Unusual Low Pressure CO2 Affinity in Pillared Metal–Organic Frameworks Nicholas C. Burtch, Himanshu Jasuja, David Dubbeldam, and Krista S. Walton pp 7172–7180 DOI: 10.1021/ja310770c Supporting Info |
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Turning a Kinase Deoxyribozyme into a Sensor Simon A. McManus and Yingfu Li pp 7181–7186 DOI: 10.1021/ja311850u Supporting Info |
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Solution-Based Single Molecule Imaging of Surface-Immobilized Conjugated Polymers Paul A. Dalgarno, Christopher A. Traina, J. Carlos Penedo, Guillermo C. Bazan, and Ifor D. W. Samuel pp 7187–7193 DOI: 10.1021/ja311874f Supporting Info |
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Nonheme Iron-Mediated Amination of C(sp3)–H Bonds. Quinquepyridine-Supported Iron-Imide/Nitrene Intermediates by Experimental Studies and DFT Calculations Yungen Liu, Xiangguo Guan, Ella Lai-Ming Wong, Peng Liu, Jie-Sheng Huang, and Chi-Ming Che pp 7194–7204 DOI: 10.1021/ja3122526 Supporting Info |
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Biosynthetic Pathway for the Epipolythiodioxopiperazine Acetylaranotin in Aspergillus terreus Revealed by Genome-Based Deletion Analysis Chun-Jun Guo, Hsu-Hua Yeh, Yi-Ming Chiang, James F. Sanchez, Shu-Ling Chang, Kenneth S. Bruno, and Clay C. C. Wang pp 7205–7213 DOI: 10.1021/ja3123653 Supporting Info |
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Direct Observation of the Formation of Surfactant Micelles under Nonisothermal Conditions by Synchrotron SAXS Grethe Vestergaard Jensen, Reidar Lund, Jérémie Gummel, Michael Monkenbusch, Theyencheri Narayanan, and Jan Skov Pedersen pp 7214–7222 DOI: 10.1021/ja312469n Supporting Info |
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Diastereomeric Spirooxindoles as Highly Potent and Efficacious MDM2 Inhibitors Yujun Zhao, Liu Liu, Wei Sun, Jianfeng Lu, Donna McEachern, Xiaoqin, Li, Shanghai Yu, Denzil Bernard, Philippe Ochsenbein, Vincent Ferey, Jean-Christophe Carry, Jeffrey R. Deschamps, Duxin Sun, and Shaomeng Wang pp 7223–7234 DOI: 10.1021/ja3125417 Supporting Info |
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Highly Enantioselective Zirconium-Catalyzed Cyclization of Aminoalkenes Kuntal Manna, William C. Everett, George Schoendorff, Arkady Ellern, Theresa L. Windus, and Aaron D. Sadow pp 7235–7250 DOI: 10.1021/ja4000189 Supporting Info |
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Low-Temperature Mechanisms for the Formation of Substituted Azanaphthalenes through Consecutive CN and C2H Additions to Styrene and N-Methylenebenzenamine: A Theoretical Study Alexander Landera and Alexander M. Mebel pp 7251–7263 DOI: 10.1021/ja400227q Supporting Info |
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Spontaneous Multielectron Transfer from the Surfaces of PbS Quantum Dots to Tetracyanoquinodimethane Kathryn E. Knowles, Michał Malicki, Radha Parameswaran, Laura C. Cass, and Emily A. Weiss pp 7264–7271 DOI: 10.1021/ja4003074 Supporting Info |
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Huge Enhancement in Two-Photon Photoluminescence of Au Nanoparticle Clusters Revealed by Single-Particle Spectroscopy Zhenping Guan, Nengyue Gao, Xiao-Fang Jiang, Peiyan Yuan, Fei Han, and Qing-Hua Xu pp 7272–7277 DOI: 10.1021/ja400364f Supporting Info |
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Molecular Insights into Clathrate Hydrate Nucleation at an Ice–Solution Interface Payman Pirzadeh and Peter G. Kusalik pp 7278–7287 DOI: 10.1021/ja400521e Supporting Info |
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High-Affinity DNA Base Analogs as Supramolecular, Nanoscale Promoters of Macroscopic Adhesion Cyrus A. Anderson, Amanda R. Jones, Ellen M. Briggs, Eric J. Novitsky, Darrell W. Kuykendall, Nancy R. Sottos, and Steven C. Zimmerman pp 7288–7295 DOI: 10.1021/ja4005283 Supporting Info |
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Stochastic Voyages into Uncharted Chemical Space Produce a Representative Library of All Possible Drug-Like Compounds Aaron M. Virshup, Julia Contreras-García, Peter Wipf, Weitao Yang, and David N. Beratan pp 7296–7303 DOI: 10.1021/ja401184g Supporting Info |
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α-Diazo-β-ketonitriles: Uniquely Reactive Substrates for Arene and Alkene Cyclopropanation Roger R. Nani and Sarah E. Reisman pp 7304–7311 DOI: 10.1021/ja401610p Supporting Info |
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Sulfur(IV)-Mediated Transformations: From Ylide Transfer to Metal-Free Arylation of Carbonyl Compounds Xueliang Huang, Mahendra Patil, Christophe Farès, Walter Thiel, and Nuno Maulide pp 7312–7323 DOI: 10.1021/ja4017683 Supporting Info |
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A Singlet Biradicaloid Zinc Compound and Its Nonradical Counterpart Amit Pratap Singh, Prinson P. Samuel, Herbert W. Roesky, Martin C. Schwarzer, Gernot Frenking, Navdeep S. Sidhu, and Birger Dittrich pp 7324–7329 DOI: 10.1021/ja402351x Supporting Info |
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Ligand-Free Palladium-Mediated Site-Specific Protein Labeling Inside Gram-Negative Bacterial Pathogens Jie Li, Shixian Lin, Jie Wang, Shang Jia, Maiyun Yang, Ziyang Hao, Xiaoyu Zhang, and Peng R. Chen pp 7330–7338 DOI: 10.1021/ja402424j Supporting Info |
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Studies on the Himbert Intramolecular Arene/Allene Diels–Alder Cycloaddition. Mechanistic Studies and Expansion of Scope to All-Carbon Tethers Yvonne Schmidt, Jonathan K. Lam, Hung V. Pham, K. N. Houk, and Christopher D. Vanderwal pp 7339–7348 DOI: 10.1021/ja4025963 Supporting Info |
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Dissociation or Cyclization: Options for a Triad of Radicals Released from Oxime Carbamates Roy T. McBurney and John C. Walton pp 7349–7354 DOI: 10.1021/ja402833w Supporting Info |
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Aqueous Copper-Mediated Living Polymerization: Exploiting Rapid Disproportionation of CuBr with Me6TREN Qiang Zhang, Paul Wilson, Zaidong Li, Ronan McHale, Jamie Godfrey, Athina Anastasaki, Christopher Waldron, and David M. Haddleton pp 7355–7363 DOI: 10.1021/ja4026402 Supporting Info |
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High Thermoelectric Performance via Hierarchical Compositionally Alloyed Nanostructures Li-Dong Zhao, Shiqiang Hao, Shih-Han Lo, Chun-I Wu, Xiaoyuan Zhou, Yeseul Lee, Hao Li, Kanishka Biswas, Timothy P. Hogan, Ctirad Uher, C. Wolverton, Vinayak P. Dravid, and Mercouri G. Kanatzidis pp 7364–7370 DOI: 10.1021/ja403134b Supporting Info |
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Combinatorial Generation of Complexity by Redox Enzymes in the Chaetoglobosin A Biosynthesis Kan’ichiro Ishiuchi, Takehito Nakazawa, Fumitoshi Yagishita, Takashi Mino, Hiroshi Noguchi, Kinya Hotta, and Kenji Watanabe pp 7371–7377 DOI: 10.1021/ja402828w Supporting Info |
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Initial Light Soaking Treatment Enables Hole Transport Material to Outperform Spiro-OMeTAD in Solid-State Dye-Sensitized Solar Cells Lei Yang, Bo Xu, Dongqin Bi, Haining Tian, Gerrit Boschloo, Licheng Sun, Anders Hagfeldt, and Erik M. J. Johansson pp 7378–7385 DOI: 10.1021/ja403344s Supporting Info |
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Correction to Theoretical Insights into Pyridinium-Based Photoelectrocatalytic Reduction of CO2 John A. Keith and Emily A. Carter pp 7386–7386 DOI: 10.1021/ja402838u |
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Correction to “Reactivity of Metallic Nitride Endohedral Metallofullerene Anions: Electrochemical Synthesis of a Lu3N@Ih-C80 Derivative” Fang-Fang Li, Antonio Rodríguez-Fortea, Josep M. Poblet, and Luis Echegoyen pp 7387–7387 DOI: 10.1021/ja403288d |
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Spotlights on Recent JACS Publications pp 7389–7389 DOI: 10.1021/ja404838j |
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A Simple Fluorescence Method for pKa Determination in RNA and DNA Reveals Highly Shifted pKa’s Jennifer L. Wilcox and Philip C. Bevilacqua pp 7390–7393 DOI: 10.1021/ja3125299 Supporting Info |
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Preparation and Exceptional Lithium Anodic Performance of Porous Carbon-Coated ZnO Quantum Dots Derived from a Metal–Organic Framework Seung Jae Yang, Seunghoon Nam, Taehoon Kim, Ji Hyuk Im, Haesol Jung, Jong Hun Kang, Sungun Wi, Byungwoo Park, and Chong Rae Park pp 7394–7397 DOI: 10.1021/ja311550t Supporting Info |
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Development of Metal–Organic Nanotubes Exhibiting Low-Temperature, Reversible Exchange of Confined “Ice Channels” Daniel K. Unruh, Kyle Gojdas, Anna Libo, and Tori Z. Forbes pp 7398–7401 DOI: 10.1021/ja400303f Supporting Info |
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The Mechanism of Carbon Dioxide Adsorption in an Alkylamine-Functionalized Metal–Organic Framework Nora Planas, Allison L. Dzubak, Roberta Poloni, Li-Chiang Lin, Alison McManus, Thomas M. McDonald, Jeffrey B. Neaton, Jeffrey R. Long, Berend Smit, and Laura Gagliardi pp 7402–7405 DOI: 10.1021/ja4004766 Supporting Info |
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Stereochemistry of Reductions Catalyzed by Methyl-Epimerizing Ketoreductase Domains of Polyketide Synthases Young-Ok You, Chaitan Khosla, and David E. Cane pp 7406–7409 DOI: 10.1021/ja4014776 Supporting Info |
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Mechanism-Based Design of a Photoactivatable Firefly Luciferase Jingyi Zhao, Shixian Lin, Yong Huang, Jing Zhao, and Peng R. Chen pp 7410–7413 DOI: 10.1021/ja4013535 Supporting Info |
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Organocatalytic Aryl–Aryl Bond Formation: An Atroposelective [3,3]-Rearrangement Approach to BINAM Derivatives Gong-Qiang Li, Hongyin Gao, Craig Keene, Michael Devonas, Daniel H. Ess, and László Kürti pp 7414–7417 DOI: 10.1021/ja401709k Supporting Info |
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Addressable Carbene Anchors for Gold Surfaces Aleksandr V. Zhukhovitskiy, Michael G. Mavros, Troy Van Voorhis, and Jeremiah A. Johnson pp 7418–7421 DOI: 10.1021/ja401965d Supporting Info |
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Fuzzy Liquid Analysis by an Array of Nonspecifically Interacting Reagents: The Taste of Fluorescence Pekka E. Hänninen, Joonas J. Siivonen, Pave I. Väisänen, Satu A. Tiittanen, Mirva M. Lehmusto, Timo Teimonen, Niklas Törnkvist, Mari A. Sandell, Antti J. Knaapila, Paul Mundill, and Harri J. Härmä pp 7422–7425 DOI: 10.1021/ja401726d Supporting Info |
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Involvement and Unusual Substrate Specificity of a Prolyl Oligopeptidase in Class III Lanthipeptide Maturation Ginka H. Völler, Bartlomiej Krawczyk, Paul Ensle, and Roderich D. Süssmuth pp 7426–7429 DOI: 10.1021/ja402296m Supporting Info |
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Real-Time Detection of Isothermal Amplification Reactions with Thermostable Catalytic Hairpin Assembly Yu (Sherry) Jiang, Bingling Li, John N. Milligan, Sanchita Bhadra, and Andrew D. Ellington pp 7430–7433 DOI: 10.1021/ja4023978 Supporting Info |
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Chiral Conflict among Different Helicenes Suppresses Formation of One Enantiomorph in 2D Crystallization Johannes Seibel, Oliver Allemann, Jay S. Siegel, and Karl-Heinz Ernst pp 7434–7437 DOI: 10.1021/ja402012j Supporting Info |
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Superprotonic Conductivity in a Highly Oriented Crystalline Metal–Organic Framework Nanofilm Gang Xu, Kazuya Otsubo, Teppei Yamada, Shun Sakaida, and Hiroshi Kitagawa pp 7438–7441 DOI: 10.1021/ja402727d Supporting Info |
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Catalytic Asymmetric Reductive Acyl Cross-Coupling: Synthesis of Enantioenriched Acyclic α,α-Disubstituted Ketones Alan H. Cherney, Nathaniel T. Kadunce, and Sarah E. Reisman pp 7442–7445 DOI: 10.1021/ja402922w Supporting Info |
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Evolution of Ordered Metal Chalcogenide Architectures through Chemical Transformations Jessy B. Rivest, Raffaella Buonsanti, Teresa E. Pick, Lina Zhu, Eunhee Lim, Cesar Clavero, Eric Schaible, Brett A. Helms, and Delia J. Milliron pp 7446–7449 DOI: 10.1021/ja403071w Supporting Info |
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Completely Regioselective Direct C–H Functionalization of Benzo[b]thiophenes Using a Simple Heterogeneous Catalyst Dan-Tam D. Tang, Karl D. Collins, and Frank Glorius pp 7450–7453 DOI: 10.1021/ja403130g Supporting Info |
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Luminescent Cell-Penetrating Pentadecanuclear Lanthanide Clusters Dominique T. Thielemann, Anna T. Wagner, Esther Rösch, Dominik K. Kölmel, Joachim G. Heck, Birgit Rudat, Marco Neumaier, Claus Feldmann, Ute Schepers, Stefan Bräse, and Peter W. Roesky pp 7454–7457 DOI: 10.1021/ja403539t Supporting Info |
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Complex Archimedean Tiling Self-Assembled from DNA Nanostructures Fei Zhang, Yan Liu, and Hao Yan pp 7458–7461 DOI: 10.1021/ja4035957 Supporting Info |
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Mechanism and Selectivity of Bioinspired Cinchona Alkaloid Derivatives Catalyzed Asymmetric Olefin Isomerization: A Computational Study Xiao-Song Xue, Xin Li, Ao Yu, Chen Yang, Chan Song, and Jin-Pei Cheng pp 7462–7473 DOI: 10.1021/ja309133z Supporting Info |
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Drug Uptake Pathways of Multidrug Transporter AcrB Studied by Molecular Simulations and Site-Directed Mutagenesis Experiments Xin-Qiu Yao, Nobuhiro Kimura, Satoshi Murakami, and Shoji Takada pp 7474–7485 DOI: 10.1021/ja310548h Supporting Info |
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Large Enhancements of Thermopower and Carrier Mobility in Quantum Dot Engineered Bulk Semiconductors Yuanfeng Liu, Pranati Sahoo, Julien P. A. Makongo, Xiaoyuan Zhou, Sung-Joo Kim, Hang Chi, Ctirad Uher, Xiaoqing Pan, and Pierre F. P. Poudeu pp 7486–7495 DOI: 10.1021/ja311059m |
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Mechanistic Insights into the Bifunctional Non-Heme Iron Oxygenase Carbapenem Synthase by Active Site Saturation Mutagenesis Ryan M. Phelan and Craig A. Townsend pp 7496–7502 DOI: 10.1021/ja311078s Supporting Info |
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Toward the Molecular Mechanism(s) by Which EGCG Treatment Remodels Mature Amyloid Fibrils Fernando L. Palhano, Jiyong Lee, Neil P. Grimster, and Jeffery W. Kelly pp 7503–7510 DOI: 10.1021/ja3115696 Supporting Info |
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Conversion of Metallic Single-Walled Carbon Nanotube Networks to Semiconducting through Electrochemical Ornamentation Darya Asheghali, Pornnipa Vichchulada, and Marcus D. Lay pp 7511–7522 DOI: 10.1021/ja311721g |
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Tocopherol Activity Correlates with Its Location in a Membrane: A New Perspective on the Antioxidant Vitamin E Drew Marquardt, Justin A. Williams, Norbert Kučerka, Jeffrey Atkinson, Stephen R. Wassall, John Katsaras, and Thad A. Harroun pp 7523–7533 DOI: 10.1021/ja312665r Supporting Info |
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Structure–Function Paradigm in Human Myoglobin: How a Single-Residue Substitution Affects NO Reactivity at Low pO2 Mariano Andrea Scorciapino, Enrico Spiga, Alessandra Vezzoli, Simona Mrakic-Sposta, Rosaria Russo, Bruno Fink, Mariano Casu, Maristella Gussoni, and Matteo Ceccarelli pp 7534–7544 DOI: 10.1021/ja400213t Supporting Info |
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Large-Scale Screening of Zeolite Structures for CO2 Membrane Separations Jihan Kim, Mahmoud Abouelnasr, Li-Chiang Lin, and Berend Smit pp 7545–7552 DOI: 10.1021/ja400267g Supporting Info |
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Solvent and H/D Isotope Effects on the Proton Transfer Pathways in Heteroconjugated Hydrogen-Bonded Phenol-Carboxylic Acid Anions Observed by Combined UV–vis and NMR Spectroscopy Benjamin Koeppe, Jing Guo, Peter M. Tolstoy, Gleb S. Denisov, and Hans-Heinrich Limbach pp 7553–7566 DOI: 10.1021/ja400611x Supporting Info |
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Pd(II)-Catalyzed ortho- or meta-C–H Olefination of Phenol Derivatives Hui-Xiong Dai, Gang Li, Xing-Guo Zhang, Antonia F. Stepan, and Jin-Quan Yu pp 7567–7571 DOI: 10.1021/ja400659s Supporting Info |
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High-Throughput Optimization of Ir-Catalyzed C–H Borylation: A Tutorial for Practical Applications Sean M. Preshlock, Behnaz Ghaffari, Peter E. Maligres, Shane W. Krska, Robert E. Maleczka, Jr., and Milton R. Smith, III pp 7572–7582 DOI: 10.1021/ja400295v Supporting Info |
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Mg2+ Binds to the Surface of Thymidylate Synthase and Affects Hydride Transfer at the Interior Active Site Zhen Wang, Paul J. Sapienza, Thelma Abeysinghe, Calvin Luzum, Andrew L. Lee, Janet S. Finer-Moore, Robert M. Stroud, and Amnon Kohen pp 7583–7592 DOI: 10.1021/ja400761x Supporting Info |
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Chemoselective Pd-Catalyzed Oxidation of Polyols: Synthetic Scope and Mechanistic Studies Kevin Chung, Steven M. Banik, Antonio G. De Crisci, David M. Pearson, Timothy R. Blake, Johan V. Olsson, Andrew J. Ingram, Richard N. Zare, and Robert M. Waymouth pp 7593–7602 DOI: 10.1021/ja4008694 Supporting Info |
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Dual-Responsive Surfaces Modified with Phenylboronic Acid-Containing Polymer Brush To Reversibly Capture and Release Cancer Cells Hongliang Liu, Yingying Li, Kang Sun, Junbing Fan, Pengchao Zhang, Jingxin Meng, Shutao Wang, and Lei Jiang pp 7603–7609 DOI: 10.1021/ja401000m Supporting Info |
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Homologous Critical Behavior in the Molecular Frameworks Zn(CN)2 and Cd(imidazolate)2 Ines E. Collings, Andrew B. Cairns, Amber L. Thompson, Julia E. Parker, Chiu C. Tang, Matthew G. Tucker, Jadna Catafesta, Claire Levelut, Julien Haines, Vladimir Dmitriev, Philip Pattison, and Andrew L. Goodwin pp 7610–7620 DOI: 10.1021/ja401268g Supporting Info |
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Exploiting High Pressures to Generate Porosity, Polymorphism, And Lattice Expansion in the Nonporous Molecular Framework Zn(CN)2 Saul H. Lapidus, Gregory J. Halder, Peter J. Chupas, and Karena W. Chapman pp 7621–7628 DOI: 10.1021/ja4012707 Supporting Info |
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Rationale for the Higher Reactivity of Interfacial Sites in Methanol Decomposition on Au13/TiO2(110) Sampyo Hong and Talat S. Rahman pp 7629–7635 DOI: 10.1021/ja4010738 Supporting Info |
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Asymmetric Growth in Polyelectrolyte Multilayers Ramy A. Ghostine, Marie Z. Markarian, and Joseph B. Schlenoff pp 7636–7646 DOI: 10.1021/ja401318m Supporting Info |
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Mechanism and Selectivity of Rhodium-Catalyzed 1:2 Coupling of Aldehydes and Allenes Genping Huang, Marcin Kalek, and Fahmi Himo pp 7647–7659 DOI: 10.1021/ja4014166 Supporting Info |
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Tunable Rare-Earth fcu-MOFs: A Platform for Systematic Enhancement of CO2 Adsorption Energetics and Uptake Dong-Xu Xue, Amy J. Cairns, Youssef Belmabkhout, Lukasz Wojtas, Yunling Liu, Mohamed H. Alkordi, and Mohamed Eddaoudi pp 7660–7667 DOI: 10.1021/ja401429x Supporting Info |
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Using VIPT-Jump to Distinguish Between Different Folding Mechanisms: Application to BBL and a Trpzip Chun-Wei Lin, Robert M. Culik, and Feng Gai pp 7668–7673 DOI: 10.1021/ja401473m Supporting Info |
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Reversible Near-Infrared Fluorescent Probe Introducing Tellurium to Mimetic Glutathione Peroxidase for Monitoring the Redox Cycles between Peroxynitrite and Glutathione in Vivo Fabiao Yu, Peng Li, Bingshuai Wang, and Keli Han pp 7674–7680 DOI: 10.1021/ja401360a Supporting Info |
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Role of Hydrophobic Interactions in the Encounter Complex Formation of the Plastocyanin and Cytochrome f Complex Revealed by Paramagnetic NMR Spectroscopy Sandra Scanu, Johannes M. Foerster, G. Matthias Ullmann, and Marcellus Ubbink pp 7681–7692 DOI: 10.1021/ja4015452 Supporting Info |
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Mechanism-Based Triarylphosphine-Ester Probes for Capture of Endogenous RSNOs Uthpala Seneviratne, Luiz C. Godoy, John S. Wishnok, Gerald N. Wogan, and Steven R. Tannenbaum pp 7693–7704 DOI: 10.1021/ja401565w Supporting Info |
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Sensing of Carboxylate Drugs in Urine by a Supramolecular Sensor Array Yuanli Liu, Tsuyoshi Minami, Ryuhei Nishiyabu, Zhuo Wang, and Pavel Anzenbacher, Jr. pp 7705–7712 DOI: 10.1021/ja4015748 Supporting Info |
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Protein Scaffold-Activated Protein Trans-Splicing in Mammalian Cells Daniel F. Selgrade, Jason J. Lohmueller, Florian Lienert, and Pamela A. Silver pp 7713–7719 DOI: 10.1021/ja401689b Supporting Info |
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An Efficient System for Heterologous Expression of Secondary Metabolite Genes in Aspergillus nidulans Yi-Ming Chiang, C. Elizabeth Oakley, Manmeet Ahuja, Ruth Entwistle, Aric Schultz, Shu-Lin Chang, Calvin T. Sung, Clay C. C. Wang, and Berl R. Oakley pp 7720–7731 DOI: 10.1021/ja401945a Supporting Info |
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Matrix Isolation Studies of Carbonic Acid—The Vapor Phase above the β-Polymorph Jürgen Bernard, Roland G. Huber, Klaus R. Liedl, Hinrich Grothe, and Thomas Loerting pp 7732–7737 DOI: 10.1021/ja4020925 Supporting Info |
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Structure and Flexibility of Nanoscale Protein Cages Designed by Symmetric Self-Assembly Yen-Ting Lai, Kuang-Lei Tsai, Michael R. Sawaya, Francisco J. Asturias, and Todd O. Yeates pp 7738–7743 DOI: 10.1021/ja402277f Supporting Info |
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Polymer Microcapsules with Programmable Active Release Alireza Abbaspourrad, Nick J. Carroll, Shin-Hyun Kim, and David A. Weitz pp 7744–7750 DOI: 10.1021/ja401960f Supporting Info |
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Catalytic CO2 Activation Assisted by Rhenium Hydride/B(C6F5)3 Frustrated Lewis Pairs—Metal Hydrides Functioning as FLP Bases Yanfeng Jiang, Olivier Blacque, Thomas Fox, and Heinz Berke pp 7751–7760 DOI: 10.1021/ja402381d Supporting Info |
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Sub-nanomolar Detection of Prostate-Specific Membrane Antigen in Synthetic Urine by Synergistic, Dual-Ligand Phage Kritika Mohan, Keith C. Donavan, Jessica A. Arter, Reginald M. Penner, and Gregory A. Weiss pp 7761–7767 DOI: 10.1021/ja4028082 Supporting Info |
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Experimental and Theoretical Comparison of Gas Desorption Energies on Metallic and Semiconducting Single-Walled Carbon Nanotubes Lynn Mandeltort, De-Li Chen, Wissam A. Saidi, J. Karl Johnson, Milton W. Cole, and John T. Yates, Jr. pp 7768–7776 DOI: 10.1021/ja402928s |
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Insertion of CO2 and COS into Bi–C Bonds: Reactivity of a Bismuth NCN Pincer Complex of an Oxyaryl Dianionic Ligand, [2,6-(Me2NCH2)2C6H3]Bi(C6H2tBu2O) Douglas R. Kindra, Ian J. Casely, Megan E. Fieser, Joseph W. Ziller, Filipp Furche, and William J. Evans pp 7777–7787 DOI: 10.1021/ja403133f Supporting Info |
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Correction to “Uncovering the Mechanism of the Ag(I)/Persulfate-Catalyzed Cross-Coupling Reaction of Arylboronic Acids and Heteroarenes” Niki R. Patel and Robert A. Flowers, II pp 7788–7788 DOI: 10.1021/ja402937c Supporting Info |
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Spotlights on Recent JACS Publications pp 7789–7790 DOI: 10.1021/ja404975y |
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Labeling Lysine Acetyltransferase Substrates with Engineered Enzymes and Functionalized Cofactor Surrogates Chao Yang, Jiaqi Mi, You Feng, Liza Ngo, Tielong Gao, Leilei Yan, and Yujun George Zheng pp 7791–7794 DOI: 10.1021/ja311636b Supporting Info |
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Effective Mercury Sorption by Thiol-Laced Metal–Organic Frameworks: in Strong Acid and the Vapor Phase Ka-Kit Yee, Nele Reimer, Jie Liu, Sum-Yin Cheng, Shek-Man Yiu, Jens Weber, Norbert Stock, and Zhengtao Xu pp 7795–7798 DOI: 10.1021/ja400212k Supporting Info |
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Charged Gold Nanoparticles with Essentially Zero Serum Protein Adsorption in Undiluted Fetal Bovine Serum Avinash K. Murthy, Robert J. Stover, William G. Hardin, Robert Schramm, Golay D. Nie, Sai Gourisankar, Thomas M. Truskett, Konstantin V. Sokolov, and Keith P. Johnston pp 7799–7802 DOI: 10.1021/ja400701c Supporting Info |
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Resonant Photocurrent Generation in Dye-Sensitized Periodically Nanostructured Photoconductors by Optical Field Confinement Effects M. Anaya, M. E. Calvo, J. M. Luque-Raigón, and H. Míguez pp 7803–7806 DOI: 10.1021/ja401096k Supporting Info |
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Convenient Detection of Pd(II) by a Metal–Organic Framework with Sulfur and Olefin Functions Jun He, Meiqin Zha, Jieshun Cui, Matthias Zeller, Allen D. Hunter, Shek-Man Yiu, Shuit-Tong Lee, and Zhengtao Xu pp 7807–7810 DOI: 10.1021/ja401479j Supporting Info |
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Real-Time Observation of Crystal Evaporation in a Metal Phosphate at High Temperature Sung-Yoon Chung, Young-Min Kim, Si-Young Choi, and Jin-Gyu Kim pp 7811–7814 DOI: 10.1021/ja401753u Supporting Info |
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Silica Encapsulation of Fluorescent Nanodiamonds for Colloidal Stability and Facile Surface Functionalization Ambika Bumb, Susanta K. Sarkar, Neil Billington, Martin W. Brechbiel, and Keir C. Neuman pp 7815–7818 DOI: 10.1021/ja4016815 Supporting Info |
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Highly Enantioselective Simmons–Smith Fluorocyclopropanation of Allylic Alcohols via the Halogen Scrambling Strategy of Zinc Carbenoids Louis-Philippe B. Beaulieu, Jakob F. Schneider, and André B. Charette pp 7819–7822 DOI: 10.1021/ja402393w Supporting Info |
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Efficient Metal-Free Electrocatalysts for Oxygen Reduction: Polyaniline-Derived N- and O-Doped Mesoporous Carbons Rafael Silva, Damien Voiry, Manish Chhowalla, and Tewodros Asefa pp 7823–7826 DOI: 10.1021/ja402450a Supporting Info |
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Mechanistic Insights into the LsrK Kinase Required for Autoinducer-2 Quorum Sensing Activation Jie Zhu, Mark S. Hixon, Daniel Globisch, Gunnar F. Kaufmann, and Kim D. Janda pp 7827–7830 DOI: 10.1021/ja4024989 Supporting Info |
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Terminal Olefins to Linear α,β-Unsaturated Ketones: Pd(II)/Hypervalent Iodine Co-catalyzed Wacker Oxidation–Dehydrogenation Marinus A. Bigi and M. Christina White pp 7831–7834 DOI: 10.1021/ja402651q Supporting Info |
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Colloidal Synthesis of Cu2SnSe3 Tetrapod Nanocrystals Jianjun Wang, Ajay Singh, Pai Liu, Shalini Singh, Claudia Coughlan, Yina Guo, and Kevin M Ryan pp 7835–7838 DOI: 10.1021/ja403083p Supporting Info |
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Formation of Colloidal Molecules Induced by Alternating-Current Electric Fields Fuduo Ma, David T. Wu, and Ning Wu pp 7839–7842 DOI: 10.1021/ja403172p Supporting Info |
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n→π* Interactions of Amides and Thioamides: Implications for Protein Stability Robert W. Newberry, Brett VanVeller, Ilia A. Guzei, and Ronald T. Raines pp 7843–7846 DOI: 10.1021/ja4033583 Supporting Info |
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Collective Activation of MRI Agents via Encapsulation and Disease-Triggered Release Mathieu L. Viger, Jagadis Sankaranarayanan, Caroline de Gracia Lux, Minnie Chan, and Adah Almutairi pp 7847–7850 DOI: 10.1021/ja403167p Supporting Info |
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Copper-Catalyzed Highly Enantioselective Cyclopentannulation of Indoles with Donor–Acceptor Cyclopropanes Hu Xiong, Hao Xu, Saihu Liao, Zuowei Xie, and Yong Tang pp 7851–7854 DOI: 10.1021/ja4042127 Supporting Info |
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Electronic Measurements of Single-Molecule Processing by DNA Polymerase I (Klenow Fragment) Tivoli J. Olsen, Yongki Choi, Patrick C. Sims, O. Tolga Gul, Brad L. Corso, Chengjun Dong, William A. Brown, Philip G. Collins, and Gregory A. Weiss pp 7855–7860 DOI: 10.1021/ja311603r Supporting Info |
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Electronic Measurements of Single-Molecule Catalysis by cAMP-Dependent Protein Kinase A Patrick C. Sims, Issa S. Moody, Yongki Choi, Chengjun Dong, Mariam Iftikhar, Brad L. Corso, O. Tolga Gul, Philip G. Collins, and Gregory A. Weiss pp 7861–7868 DOI: 10.1021/ja311604j Supporting Info |
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Highly Potent Inhibitors of Quorum Sensing in Staphylococcus aureus Revealed Through a Systematic Synthetic Study of the Group-III Autoinducing Peptide Yftah Tal-Gan, Danielle M. Stacy, Mary K. Foegen, David W. Koenig, and Helen E. Blackwell pp 7869–7882 DOI: 10.1021/ja3112115 Supporting Info |
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Restricted State Selection in Fluorescent Protein Förster Resonance Energy Transfer Thomas A. Masters, Richard J. Marsh, Daven A. Armoogum, Nick Nicolaou, Banafshé Larijani, and Angus J. Bain pp 7883–7890 DOI: 10.1021/ja312230b Supporting Info |
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Reduced Enthalpy of Metal Hydride Formation for Mg–Ti Nanocomposites Produced by Spark Discharge Generation Anca Anastasopol, Tobias V. Pfeiffer, Joost Middelkoop, Ugo Lafont, Roger J. Canales-Perez, Andreas Schmidt-Ott, Fokko M. Mulder, and Stephan W.H. Eijt pp 7891–7900 DOI: 10.1021/ja3123416 |
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Tracking the Formation of a Polynuclear Co16 Complex and Its Elimination and Substitution Reactions by Mass Spectroscopy and Crystallography Yue-Qiao Hu, Ming-Hua Zeng, Kun Zhang, Sheng Hu, Fu-Fang Zhou, and Mohamedally Kurmoo pp 7901–7908 DOI: 10.1021/ja3123784 Supporting Info |
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Cation Size Mismatch and Charge Interactions Drive Dopant Segregation at the Surfaces of Manganite Perovskites Wonyoung Lee, Jeong Woo Han, Yan Chen, Zhuhua Cai, and Bilge Yildiz pp 7909–7925 DOI: 10.1021/ja3125349 Supporting Info |
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Gold-Catalyzed Cycloisomerization of 1,6-Diyne Carbonates and Esters to 2,4a-Dihydro-1H-fluorenes Weidong Rao, Ming Joo Koh, Dan Li, Hajime Hirao, and Philip Wai Hong Chan pp 7926–7932 DOI: 10.1021/ja4032727 Supporting Info |
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Biodegradable Core–Shell Carriers for Simultaneous Encapsulation of Synergistic Actives Maike Windbergs, Yuanjin Zhao, John Heyman, and David A. Weitz pp 7933–7937 DOI: 10.1021/ja401422r Supporting Info |
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Peptide Crystal Simulations Reveal Hidden Dynamics Pawel A. Janowski, David S. Cerutti, James Holton, and David A. Case pp 7938–7948 DOI: 10.1021/ja401382y Supporting Info |
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Coordination Chemistry of Disilylated Stannylenes with Group 10 d10 Transition Metals: Silastannene vs Stannylene Complexation Henning Arp, Christoph Marschner, Judith Baumgartner, Patrick Zark, and Thomas Müller pp 7949–7959 DOI: 10.1021/ja401548d Supporting Info |
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p-Stilbazole Moieties As Artificial Base Pairs for Photo-Cross-Linking of DNA Duplex Hiromu Kashida, Tetsuya Doi, Takumi Sakakibara, Takamitsu Hayashi, and Hiroyuki Asanuma pp 7960–7966 DOI: 10.1021/ja401835j Supporting Info |
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DNA Branch Migration Reactions Through Photocontrollable Toehold Formation Fujian Huang, Mingxu You, Da Han, Xiangling Xiong, Haojun Liang, and Weihong Tan pp 7967–7973 DOI: 10.1021/ja4018495 Supporting Info |
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Self-Assembly of Amphiphilic Plasmonic Micelle-Like Nanoparticles in Selective Solvents Jie He, Xinglu Huang, Yan-Chun Li, Yijing Liu, Taarika Babu, Maria A. Aronova, Shouju Wang, Zhongyuan Lu, Xiaoyuan Chen, and Zhihong Nie pp 7974–7984 DOI: 10.1021/ja402015s Supporting Info |
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Surface Composition Tuning of Au–Pt Bimetallic Nanoparticles for Enhanced Carbon Monoxide and Methanol Electro-oxidation Jin Suntivich, Zhichuan Xu, Christopher E. Carlton, Junhyung Kim, Binghong Han, Seung Woo Lee, Nicéphore Bonnet, Nicola Marzari, Lawrence F. Allard, Hubert A. Gasteiger, Kimberly Hamad-Schifferli, and Yang Shao-Horn pp 7985–7991 DOI: 10.1021/ja402072r Supporting Info |
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Single Molecule Force Spectroscopy Reveals That Iron Is Released from the Active Site of Rubredoxin by a Stochastic Mechanism Peng Zheng, Shin-ichi J. Takayama, A. Grant Mauk, and Hongbin Li pp 7992–8000 DOI: 10.1021/ja402150q Supporting Info |
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Quantum Mechanics/Molecular Mechanics Modeling of Regioselectivity of Drug Metabolism in Cytochrome P450 2C9 Richard Lonsdale, Kerensa T. Houghton, Jolanta Żurek, Christine M. Bathelt, Nicolas Foloppe, Marcel J. de Groot, Jeremy N. Harvey, and Adrian J. Mulholland pp 8001–8015 DOI: 10.1021/ja402016p Supporting Info |
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Size Specifically High Activity of Ru Nanoparticles for Hydrogen Oxidation Reaction in Alkaline Electrolyte Junya Ohyama, Takuma Sato, Yuta Yamamoto, Shigeo Arai, and Atsushi Satsuma pp 8016–8021 DOI: 10.1021/ja4021638 Supporting Info |
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Interplay between 1,3-Butadien-1,4-diyl and 2-Buten-1,4-dicarbene Derivatives: The Quest for Nucleophilic Carbenes Gebhard Haberhauer and Rolf Gleiter pp 8022–8030 DOI: 10.1021/ja4020937 Supporting Info |
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Pyrrole-Fused Azacoronene Family: The Influence of Replacement with Dialkoxybenzenes on the Optical and Electronic Properties in Neutral and Oxidized States Masayoshi Takase, Tomoyuki Narita, Wataru Fujita, Motoko S. Asano, Tohru Nishinaga, Hiroaki Benten, Kenji Yoza, and Klaus Müllen pp 8031–8040 DOI: 10.1021/ja402371f Supporting Info |
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Non-uniform Velocity of Homogeneous DNA in a Uniform Electric Field: Consequence of Electric-Field-Induced Slow Dissociation of Highly Stable DNA–Counterion Complexes Michael U. Musheev, Mirzo Kanoatov, and Sergey N. Krylov pp 8041–8046 DOI: 10.1021/ja402257x Supporting Info |
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(De)Lithiation Mechanism of Li/SeSx (x = 0–7) Batteries Determined by in Situ Synchrotron X-ray Diffraction and X-ray Absorption Spectroscopy Yanjie Cui, Ali Abouimrane, Jun Lu, Trudy Bolin, Yang Ren, Wei Weng, Chengjun Sun, Victor A. Maroni, Steve M. Heald, and Khalil Amine pp 8047–8056 DOI: 10.1021/ja402597g Supporting Info |
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In Situ Modification of Plain Liposomes with Lipidated Coiled Coil Forming Peptides Induces Membrane Fusion Frank Versluis, Jens Voskuhl, Bartjan van Kolck, Harshal Zope, Marien Bremmer, Tjerk Albregtse, and Alexander Kros pp 8057–8062 DOI: 10.1021/ja4031227 Supporting Info |
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Beyond Classical Reactivity Patterns: Shifting from 1,4- to 1,6-Additions in Regio- and Enantioselective Organocatalyzed Vinylogous Reactions of Olefinic Lactones with Enals and 2,4-Dienals Luca Dell’Amico, Łukasz Albrecht, Tricia Naicker, Pernille H. Poulsen, and Karl Anker Jørgensen pp 8063–8070 DOI: 10.1021/ja4029928 Supporting Info |
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Preparation and Reactions of Enantiomerically Pure α-Functionalized Grignard Reagents Peter J. Rayner, Peter O’Brien, and Richard A. J. Horan pp 8071–8077 DOI: 10.1021/ja4033956 Supporting Info |
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Amino Acid Substitution in the Active Site of DNA Polymerase β Explains the Energy Barrier of the Nucleotidyl Transfer Reaction Vinod K. Batra, Lalith Perera, Ping Lin, David D. Shock, William A. Beard, Lars C. Pedersen, Lee G. Pedersen, and Samuel H. Wilson pp 8078–8088 DOI: 10.1021/ja403842j Supporting Info |
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Advances in Magnetic Resonance: From Stem Cells to Catalytic Surfaces Lyndon Emsley pp 8089–8091 DOI: 10.1021/ja404269a |
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Spotlights on Recent JACS Publications pp 8092–8092 DOI: 10.1021/ja404976q |
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GenK-Catalyzed C-6′ Methylation in the Biosynthesis of Gentamicin: Isolation and Characterization of a Cobalamin-Dependent Radical SAM Enzyme Hak Joong Kim, Reid M. McCarty, Yasushi Ogasawara, Yung-nan Liu, Steven O. Mansoorabadi, Jake LeVieux, and Hung-wen Liu pp 8093–8096 DOI: 10.1021/ja312641f Supporting Info |
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Graphene Oxide Nanosheet with High Proton Conductivity Mohammad Razaul Karim, Kazuto Hatakeyama, Takeshi Matsui, Hiroshi Takehira, Takaaki Taniguchi, Michio Koinuma, Yasumichi Matsumoto, Tomoyuki Akutagawa, Takayoshi Nakamura, Shin-ichiro Noro, Teppei Yamada, Hiroshi Kitagawa, and Shinya Hayami pp 8097–8100 DOI: 10.1021/ja401060q Supporting Info |
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Enantioselective Bromoaminocyclization of Allyl N-Tosylcarbamates Catalyzed by a Chiral Phosphine–Sc(OTf)3 Complex Deshun Huang, Xiaoqin Liu, Lijun Li, Yudong Cai, Weigang Liu, and Yian Shi pp 8101–8104 DOI: 10.1021/ja4010877 Supporting Info |
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Role of Dimerization Efficiency of Transmembrane Domains in Activation of Fibroblast Growth Factor Receptor 3 Pavel E. Volynsky, Anton A. Polyansky, Gulfia N. Fakhrutdinova, Eduard V. Bocharov, and Roman G. Efremov pp 8105–8108 DOI: 10.1021/ja4011942 Supporting Info |
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Enhanced Photoluminescence of Sulfur-Bridged Organic Chromophores Peter R. Christensen, Jeffrey K. Nagle, Aini Bhatti, and Michael O. Wolf pp 8109–8112 DOI: 10.1021/ja401383q Supporting Info |
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Catalytic Activation of Carbohydrates as Formaldehyde Equivalents for Stetter Reaction with Enones Junmin Zhang, Chong Xing, Bhoopendra Tiwari, and Yonggui Robin Chi pp 8113–8116 DOI: 10.1021/ja401511r Supporting Info |
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[2Fe-2S]-Ferredoxin Binds Directly to Cysteine Desulfurase and Supplies an Electron for Iron–Sulfur Cluster Assembly but Is Displaced by the Scaffold Protein or Bacterial Frataxin Jin Hae Kim, Ronnie O. Frederick, Nichole M. Reinen, Andrew T. Troupis, and John L. Markley pp 8117–8120 DOI: 10.1021/ja401950a Supporting Info |
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Odd–Even Effect in the Elastic Modulii of α,ω-Alkanedicarboxylic Acids Manish Kumar Mishra, Sunil Varughese, Upadrasta Ramamurty, and Gautam R. Desiraju pp 8121–8124 DOI: 10.1021/ja402290h Supporting Info |
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Cp*Rh-Based Heterometallic Metallarectangles: Size-Dependent Borromean Link Structures and Catalytic Acyl Transfer Sheng-Li Huang, Yue-Jian Lin, T. S. Andy Hor, and Guo-Xin Jin pp 8125–8128 DOI: 10.1021/ja402630g Supporting Info |
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Broadly Applicable Methodology for the Rapid and Dosable Small Molecule-Mediated Regulation of Transcription Factors in Human Cells Matthew D. Shoulders, Lisa M. Ryno, Christina B. Cooley, Jeffery W. Kelly, and R. Luke Wiseman pp 8129–8132 DOI: 10.1021/ja402756p Supporting Info |
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Enantioselective, Desymmetrizing Bromolactonization of Alkynes Michael Wilking, Christian Mück-Lichtenfeld, Constantin G. Daniliuc, and Ulrich Hennecke pp 8133–8136 DOI: 10.1021/ja402910d Supporting Info |
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Fabrication of Supported Cuprous Sites at Low Temperatures: An Efficient, Controllable Strategy Using Vapor-Induced Reduction Wen-Juan Jiang, Yu Yin, Xiao-Qin Liu, Xiao-Qian Yin, Yao-Qi Shi, and Lin-Bing Sun pp 8137–8140 DOI: 10.1021/ja4030269 Supporting Info |
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A Five-Coordinate Nickel(II) Fluoroalkyl Complex as a Precursor to a Spectroscopically Detectable Ni(III) Species Cheng-Pan Zhang, Huan Wang, Axel Klein, Christian Biewer, Kathrin Stirnat, Yoshitaka Yamaguchi, Long Xu, Valente Gomez-Benitez, and David A. Vicic pp 8141–8144 DOI: 10.1021/ja4030462 Supporting Info |
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Dis-assembly of a Benzylic CF3 Group Mediated by a Niobium(III) Imido Complex Thomas L. Gianetti, Robert G. Bergman, and John Arnold pp 8145–8148 DOI: 10.1021/ja4033007 Supporting Info |
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Differential Impact of β and γ Residue Preorganization on α/β/γ-Peptide Helix Stability in Water Young-Hee Shin, David E. Mortenson, Kenneth A. Satyshur, Katrina T. Forest, and Samuel H. Gellman pp 8149–8152 DOI: 10.1021/ja403319q Supporting Info |
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Reaction of HppE with Substrate Analogues: Evidence for Carbon–Phosphorus Bond Cleavage by a Carbocation Rearrangement Wei-chen Chang, Steven O. Mansoorabadi, and Hung-wen Liu pp 8153–8156 DOI: 10.1021/ja403441x Supporting Info |
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Iridium-Catalyzed Borylation of Secondary Benzylic C–H Bonds Directed by a Hydrosilane Seung Hwan Cho and John F. Hartwig pp 8157–8160 DOI: 10.1021/ja403462b Supporting Info |
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Catalytic Asymmetric Oxidation of N-Sulfonyl Imines with Hydrogen Peroxide–Trichloroacetonitrile System Daisuke Uraguchi, Ryosuke Tsutsumi, and Takashi Ooi pp 8161–8164 DOI: 10.1021/ja403491j Supporting Info |
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Chameleon Behavior of a Newly Synthesized Scandium Nitrilimine Derivative Jiaxiang Chu, Christos E. Kefalidis, Laurent Maron, Xuebing Leng, and Yaofeng Chen pp 8165–8168 DOI: 10.1021/ja403387v Supporting Info |
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Enantioselective Functionalization of Indoles and Pyrroles via an in Situ-Formed Spiro Intermediate Chun-Xiang Zhuo, Qing-Feng Wu, Qiang Zhao, Qing-Long Xu, and Shu-Li You pp 8169–8172 DOI: 10.1021/ja403535a Supporting Info |
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Extreme Oxatriquinanes: Structural Characterization of α-Oxyoxonium Species with Extraordinarily Long Carbon–Oxygen Bonds Gorkem Gunbas, William L. Sheppard, James C. Fettinger, Marilyn M. Olmstead, and Mark Mascal pp 8173–8176 DOI: 10.1021/ja4032715 Supporting Info |
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Synthesis of Telechelic Olefin Polymers via Catalyzed Chain Growth on Multinuclear Alkylene Zinc Compounds Haruyuki Makio, Takashi Ochiai, Jun-ichi Mohri, Kouji Takeda, Toshiyuki Shimazaki, Yoko Usui, Sadahiko Matsuura, and Terunori Fujita pp 8177–8180 DOI: 10.1021/ja403626g Supporting Info |
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Quantifying the Structural Changes of Perfluorosulfonated Acid Ionomer upon Reaction with Hydroxyl Radicals Lida Ghassemzadeh and Steven Holdcroft pp 8181–8184 DOI: 10.1021/ja4037466 Supporting Info |
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Mn2(2,5-disulfhydrylbenzene-1,4-dicarboxylate): A Microporous Metal–Organic Framework with Infinite (−Mn–S−)∞ Chains and High Intrinsic Charge Mobility Lei Sun, Tomoyo Miyakai, Shu Seki, and Mircea Dincă pp 8185–8188 DOI: 10.1021/ja4037516 Supporting Info |
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“Flex-Activated” Mechanophores: Using Polymer Mechanochemistry To Direct Bond Bending Activation Michael B. Larsen and Andrew J. Boydston pp 8189–8192 DOI: 10.1021/ja403757p Supporting Info |
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A Highly Diastereo- and Enantioselective Synthesis of Tetrahydroquinolines: Quaternary Stereogenic Center Inversion and Functionalization Chaosheng Luo and Yong Huang pp 8193–8196 DOI: 10.1021/ja4040945 Supporting Info |
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Highly Stereoselective Olefin Cyclopropanation of Diazooxindoles Catalyzed by a C2-Symmetric Spiroketal Bisphosphine/Au(I) Complex Zhong-Yan Cao, Xiaoming Wang, Chen Tan, Xiao-Li Zhao, Jian Zhou, and Kuiling Ding pp 8197–8200 DOI: 10.1021/ja4040895 Supporting Info |
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Generation of Rhodium(I) Carbenes from Ynamides and Their Reactions with Alkynes and Alkenes Renhe Liu, Gabrielle N. Winston-McPherson, Zhong-Yue Yang, Xin Zhou, Wangze Song, Ilia A. Guzei, Xiufang Xu, and Weiping Tang pp 8201–8204 DOI: 10.1021/ja4047069 Supporting Info |
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Aerobic Dehydrogenation of Cyclohexanone to Cyclohexenone Catalyzed by Pd(DMSO)2(TFA)2: Evidence for Ligand-Controlled Chemoselectivity Tianning Diao, Doris Pun, and Shannon S. Stahl pp 8205–8212 DOI: 10.1021/ja4031648 Supporting Info |
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Aerobic Dehydrogenation of Cyclohexanone to Phenol Catalyzed by Pd(TFA)2/2-Dimethylaminopyridine: Evidence for the Role of Pd Nanoparticles Doris Pun, Tianning Diao, and Shannon S. Stahl pp 8213–8221 DOI: 10.1021/ja403165u Supporting Info |
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Ribozyme-Based Transfer RNA Switches for Post-transcriptional Control of Amino Acid Identity in Protein Synthesis Athanasios Saragliadis and Jörg S. Hartig pp 8222–8226 DOI: 10.1021/ja311107p Supporting Info |
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Discovery of Picomolar ABL Kinase Inhibitors Equipotent for Wild Type and T315I Mutant via Structure-Based de Novo Design Hwangseo Park, Seunghee Hong, Jinhee Kim, and Sungwoo Hong pp 8227–8237 DOI: 10.1021/ja311756u Supporting Info |
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Long-Term Fluorescent Cellular Tracing by the Aggregates of AIE Bioconjugates Zhengke Wang, Sijie Chen, Jacky W. Y. Lam, Wei Qin, Ryan T. K. Kwok, Ni Xie, Qiaoling Hu, and Ben Zhong Tang pp 8238–8245 DOI: 10.1021/ja312581r Supporting Info |
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Charge-Controlled Switchable CO2 Capture on Boron Nitride Nanomaterials Qiao Sun, Zhen Li, Debra J. Searles, Ying Chen, Gaoqing (Max) Lu, and Aijun Du pp 8246–8253 DOI: 10.1021/ja400243r Supporting Info |
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Metal–Metal Quadruple Bonds Supported by 5-Ethynylthiophene-2-carboxylato Ligands: Preparation, Molecular and Electronic Structures, Photoexcited State Dynamics, and Application as Molecular Synthons Samantha E. Brown-Xu, Malcolm H. Chisholm, Christopher B. Durr, and Thomas F. Spilker pp 8254–8259 DOI: 10.1021/ja400508u Supporting Info |
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Application of the Molecular Interaction Volume Model (MIVM) to Calcium-Based Liquid Alloys of Systems Forming High-Melting Intermetallics Sophie Poizeau and Donald R. Sadoway pp 8260–8265 DOI: 10.1021/ja4013886 |
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Isomer-Selective Detection of Hydrogen-Bond Vibrations in the Protonated Water Hexamer Nadja Heine, Matias R. Fagiani, Mariana Rossi, Torsten Wende, Giel Berden, Volker Blum, and Knut R. Asmis pp 8266–8273 DOI: 10.1021/ja401359t Supporting Info |
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Partial Base Flipping Is Sufficient for Strand Slippage near DNA Duplex Termini Nilesh K. Banavali pp 8274–8282 DOI: 10.1021/ja401573j Supporting Info |
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WGS Catalysis and In Situ Studies of CoO1–x, PtCon/Co3O4, and PtmCom′/CoO1–x Nanorod Catalysts Shiran Zhang, Jun-jun Shan, Yuan Zhu, Anatoly I. Frenkel, Anitha Patlolla, Weixin Huang, Seog Joon Yoon, Lei Wang, Hideto Yoshida, Seiji Takeda, and Franklin (Feng) Tao pp 8283–8293 DOI: 10.1021/ja401967y Supporting Info |
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Magic Angle Spinning NMR Structure Determination of Proteins from Pseudocontact Shifts Jianping Li, Kala Bharath Pilla, Qingfeng Li, Zhengfeng Zhang, Xuncheng Su, Thomas Huber, and Jun Yang pp 8294–8303 DOI: 10.1021/ja4021149 Supporting Info |
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Redox Activity and Two-Step Valence Tautomerism in a Family of Dinuclear Cobalt Complexes with a Spiroconjugated Bis(dioxolene) Ligand Kerwyn G. Alley, Giordano Poneti, Peter S. D. Robinson, Ayman Nafady, Boujemaa Moubaraki, Jade B. Aitken, Simon C. Drew, Chris Ritchie, Brendan F. Abrahams, Rosalie K. Hocking, Keith S. Murray, Alan M. Bond, Hugh H. Harris, Lorenzo Sorace, and Colette Boskovic pp 8304–8323 DOI: 10.1021/ja4021155 Supporting Info |
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Quantification of Nitrate−π Interactions and Selective Transport of Nitrate Using Calix[4]pyrroles with Two Aromatic Walls Louis Adriaenssens, Carolina Estarellas, Andreas Vargas Jentzsch, Marta Martinez Belmonte, Stefan Matile, and Pablo Ballester pp 8324–8330 DOI: 10.1021/ja4021793 Supporting Info |
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Distance Dependent Electron Transfer at TiO2 Interfaces Sensitized with Phenylene Ethynylene Bridged RuII–Isothiocyanate Compounds Patrik G. Johansson, Andrew Kopecky, Elena Galoppini, and Gerald J. Meyer pp 8331–8341 DOI: 10.1021/ja402193f Supporting Info |
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Cooperative Self-Assembly of Discoid Dimers: Hierarchical Formation of Nanostructures with a pH Switch M. Tassilo Fenske, Wolfgang Meyer-Zaika, Hans-Gert Korth, Henning Vieker, Andrey Turchanin, and Carsten Schmuck pp 8342–8349 DOI: 10.1021/ja4025148 Supporting Info |
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Large-Scale Aqueous Synthesis of Fluorescent and Biocompatible Silicon Nanoparticles and Their Use as Highly Photostable Biological Probes Yiling Zhong, Fei Peng, Feng Bao, Siyi Wang, Xiaoyuan Ji, Liu Yang, Yuanyuan Su, Shuit-Tong Lee, and Yao He pp 8350–8356 DOI: 10.1021/ja4026227 Supporting Info |
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Direct Detection of RDX Vapor Using a Conjugated Polymer Network Deepti Gopalakrishnan and William R. Dichtel pp 8357–8362 DOI: 10.1021/ja402668e Supporting Info |
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Liquid-Phase Syntheses and Material Properties of Two-Dimensional Nanocrystals of Rare Earth–Selenium Compound Containing Planar Se Layers: RESe2 Nanosheets and RE4O4Se3 Nanoplates Jun Gu, Ze-Qiong Zhao, Yi Ding, Hong-Liang Chen, Ya-Wen Zhang, and Chun-Hua Yan pp 8363–8371 DOI: 10.1021/ja4028583 Supporting Info |
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Reversible Intercalation of Hexagonal Boron Nitride with Brønsted Acids Nina I. Kovtyukhova, Yuanxi Wang, Ruitao Lv, Mauricio Terrones, Vincent H. Crespi, and Thomas E. Mallouk pp 8372–8381 DOI: 10.1021/ja403197h Supporting Info |
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Photoisomerization Quantum Yield of Azobenzene-Modified DNA Depends on Local Sequence Yunqi Yan, Xin Wang, Jennifer I. L. Chen, and David S. Ginger pp 8382–8387 DOI: 10.1021/ja403249u Supporting Info |
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The Elusive Structure of Pd2(dba)3. Examination by Isotopic Labeling, NMR Spectroscopy, and X-ray Diffraction Analysis: Synthesis and Characterization of Pd2(dba-Z)3 Complexes Anant R. Kapdi, Adrian C. Whitwood, David C. Williamson, Jason M. Lynam, Michael J. Burns, Thomas J. Williams, Alan J. Reay, Jordan Holmes, and Ian J. S. Fairlamb pp 8388–8399 DOI: 10.1021/ja403259c Supporting Info |
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Overcoming Compound Fluorescence in the FLiK Screening Assay with Red-Shifted Fluorophores Ralf Schneider, Anne Gohla, Jeffrey R. Simard, Dharmendra B. Yadav, Zhizhou Fang, Willem A. L. van Otterlo, and Daniel Rauh pp 8400–8408 DOI: 10.1021/ja403074j Supporting Info |
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Growth Intermediates for CVD Graphene on Cu(111): Carbon Clusters and Defective Graphene Tianchao Niu, Miao Zhou, Jialin Zhang, Yuanping Feng, and Wei Chen pp 8409–8414 DOI: 10.1021/ja403583s Supporting Info |
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Chemical Tailoring of Teicoplanin with Site-Selective Reactions Tejas P. Pathak and Scott J. Miller pp 8415–8422 DOI: 10.1021/ja4038998 Supporting Info |
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Carbon Monoxide Induced Reductive Elimination of Disulfide in an N-Heterocyclic Carbene (NHC)/ Thiolate Dinitrosyl Iron Complex (DNIC) Randara Pulukkody, Samuel J. Kyran, Ryan D. Bethel, Chung-Hung Hsieh, Michael B. Hall, Donald J. Darensbourg, and Marcetta Y. Darensbourg pp 8423–8430 DOI: 10.1021/ja403916v Supporting Info |
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Spotlights on Recent JACS Publications pp 8431–8431 DOI: 10.1021/ja405586p |
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Water Oxidation and Oxygen Monitoring by Cobalt-Modified Fluorine-Doped Tin Oxide Electrodes Caleb A. Kent, Javier J. Concepcion, Christopher J. Dares, Daniel A. Torelli, Adam J. Rieth, Andrew S. Miller, Paul G. Hoertz, and Thomas J. Meyer pp 8432–8435 DOI: 10.1021/ja400616a Supporting Info |
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Copper-Promoted Sandmeyer Trifluoromethylation Reaction Jian-Jun Dai, Chi Fang, Bin Xiao, Jun Yi, Jun Xu, Zhao-Jing Liu, Xi Lu, Lei Liu, and Yao Fu pp 8436–8439 DOI: 10.1021/ja404217t Supporting Info |
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Controlled Formation of Carbon Nanotube Junctions via Linker-Induced Assembly in Aqueous Solution Matteo Palma, Wei Wang, Erika Penzo, Julian Brathwaite, Ming Zheng, James Hone, Colin Nuckolls, and Shalom J. Wind pp 8440–8443 DOI: 10.1021/ja4018072 Supporting Info |
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Stepwise Pore Size Reduction of Ordered Nanoporous Silica Materials at Angstrom Precision Siddharth Jambhrunkar, Meihua Yu, Jie Yang, Jun Zhang, Abhijit Shrotri, Liliana Endo-Munoz, Joël Moreau, Gaoqing Lu, and Chengzhong Yu pp 8444–8447 DOI: 10.1021/ja402463h Supporting Info |
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On-Surface Formation of One-Dimensional Polyphenylene through Bergman Cyclization Qiang Sun, Chi Zhang, Zhiwen Li, Huihui Kong, Qinggang Tan, Aiguo Hu, and Wei Xu pp 8448–8451 DOI: 10.1021/ja404039t Supporting Info |
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An Advanced Ni–Fe Layered Double Hydroxide Electrocatalyst for Water Oxidation Ming Gong, Yanguang Li, Hailiang Wang, Yongye Liang, Justin Z. Wu, Jigang Zhou, Jian Wang, Tom Regier, Fei Wei, and Hongjie Dai pp 8452–8455 DOI: 10.1021/ja4027715 Supporting Info |
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Copolymerization of Epoxides with Carbon Dioxide Catalyzed by Iron–Corrole Complexes: Synthesis of a Crystalline Copolymer Koji Nakano, Kazuki Kobayashi, Takahiro Ohkawara, Hideyuki Imoto, and Kyoko Nozaki pp 8456–8459 DOI: 10.1021/ja4028633 Supporting Info |
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Oxidative Heck Vinylation for the Synthesis of Complex Dienes and Polyenes Jared H. Delcamp, Paul E. Gormisky, and M. Christina White pp 8460–8463 DOI: 10.1021/ja402891m Supporting Info |
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Molecular Design toward Efficient Polymer Solar Cells with High Polymer Content Deping Qian, Wei Ma, Zhaojun Li, Xia Guo, Shaoqing Zhang, Long Ye, Harald Ade, Zhan’ao Tan, and Jianhui Hou pp 8464–8467 DOI: 10.1021/ja402971d Supporting Info |
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Anion-Dependent Self-Assembly of Near-Infrared Luminescent 24- and 32-Metal Cd–Ln Complexes with Drum-like Architectures Xiaoping Yang, Desmond Schipper, Richard A. Jones, Lauren A. Lytwak, Bradley J. Holliday, and Shaoming Huang pp 8468–8471 DOI: 10.1021/ja4031243 Supporting Info |
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DNA Catalysis of a Normally Disfavored RNA Hydrolysis Reaction Darren J. Parker, Ying Xiao, John M. Aguilar, and Scott K. Silverman pp 8472–8475 DOI: 10.1021/ja4032488 Supporting Info |
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Template Control over Dimerization and Guest Selectivity of Interpenetrated Coordination Cages Sabrina Freye, Reent Michel, Dietmar Stalke, Martin Pawliczek, Holm Frauendorf, and Guido H. Clever pp 8476–8479 DOI: 10.1021/ja403184a Supporting Info |
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Sterically Controlled, Palladium-Catalyzed Intermolecular Amination of Arenes Ruja Shrestha, Paramita Mukherjee, Yichen Tan, Zachary C. Litman, and John F. Hartwig pp 8480–8483 DOI: 10.1021/ja4032677 Supporting Info |
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Solution-Processed and High-Performance Organic Solar Cells Using Small Molecules with a Benzodithiophene Unit Jiaoyan Zhou, Yi Zuo, Xiangjian Wan, Guankui Long, Qian Zhang, Wang Ni, Yongsheng Liu, Zhi Li, Guangrui He, Chenxi Li, Bin Kan, Miaomiao Li, and Yongsheng Chen pp 8484–8487 DOI: 10.1021/ja403318y Supporting Info |
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C2′-OH of Amphotericin B Plays an Important Role in Binding the Primary Sterol of Human Cells but Not Yeast Cells Brandon C. Wilcock, Matthew M. Endo, Brice E. Uno, and Martin D. Burke pp 8488–8491 DOI: 10.1021/ja403255s Supporting Info |
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Effect of Protons on the Redox Chemistry of Colloidal Zinc Oxide Nanocrystals Carolyn N. Valdez, Miles Braten, Ashley Soria, Daniel R. Gamelin, and James M. Mayer pp 8492–8495 DOI: 10.1021/ja4035945 Supporting Info |
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Freezing and Melting of Salt Hydrates Next to Solid Surfaces Probed by Infrared–Visible Sum Frequency Generation Spectroscopy Emmanuel Anim-Danso, Yu Zhang, and Ali Dhinojwala pp 8496–8499 DOI: 10.1021/ja403437c Supporting Info |
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Total Synthesis of (±)-Gelsemoxonine Stefan Diethelm and Erick M. Carreira pp 8500–8503 DOI: 10.1021/ja403823n Supporting Info |
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Asymmetric N-Heterocyclic Carbene Catalyzed Addition of Enals to Nitroalkenes: Controlling Stereochemistry via the Homoenolate Reactivity Pathway To Access δ-Lactams Nicholas A. White, Daniel A. DiRocco, and Tomislav Rovis pp 8504–8507 DOI: 10.1021/ja403847e Supporting Info |
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A Ru−η6-Arene Complex as a C-Based Lewis Acid in the Activation of Hydrogen and Hydrogenation Catalysis Michael P. Boone and Douglas W. Stephan pp 8508–8511 DOI: 10.1021/ja403912n Supporting Info |
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[3,3]-Sigmatropic Rearrangement versus Carbene Formation in Gold-Catalyzed Transformations of Alkynyl Aryl Sulfoxides: Mechanistic Studies and Expanded Reaction Scope Biao Lu, Yuxue Li, Youliang Wang, Donald H. Aue, Yingdong Luo, and Liming Zhang pp 8512–8524 DOI: 10.1021/ja401343p Supporting Info |
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In Situ X-ray Absorption Spectroscopy Investigation of a Bifunctional Manganese Oxide Catalyst with High Activity for Electrochemical Water Oxidation and Oxygen Reduction Yelena Gorlin, Benedikt Lassalle-Kaiser, Jesse D. Benck, Sheraz Gul, Samuel M. Webb, Vittal K. Yachandra, Junko Yano, and Thomas F. Jaramillo pp 8525–8534 DOI: 10.1021/ja3104632 Supporting Info |
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Thermally Active Hybridization Drives the Crystallization of DNA-Functionalized Nanoparticles Ting I. N. G. Li, Rastko Sknepnek, and Monica Olvera de la Cruz pp 8535–8541 DOI: 10.1021/ja312644h Supporting Info |
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Characterizing the Membrane-Bound State of Cytochrome P450 3A4: Structure, Depth of Insertion, and Orientation Javier L. Baylon, Ivan L. Lenov, Stephen G. Sligar, and Emad Tajkhorshid pp 8542–8551 DOI: 10.1021/ja4003525 Supporting Info |
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Site-Specific Growth of Au–Pd Alloy Horns on Au Nanorods: A Platform for Highly Sensitive Monitoring of Catalytic Reactions by Surface Enhancement Raman Spectroscopy Jianfeng Huang, Yihan Zhu, Ming Lin, Qingxiao Wang, Lan Zhao, Yang Yang, Ke Xin Yao, and Yu Han pp 8552–8561 DOI: 10.1021/ja4004602 Supporting Info |
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Interactions of the Human Telomere Sequence with the Nanocavity of the α-Hemolysin Ion Channel Reveal Structure-Dependent Electrical Signatures for Hybrid Folds Na An, Aaron M. Fleming, and Cynthia J. Burrows pp 8562–8570 DOI: 10.1021/ja400973m Supporting Info |
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Sub-10 nm Fe3O4@Cu2–xS Core–Shell Nanoparticles for Dual-Modal Imaging and Photothermal Therapy Qiwei Tian, Junqing Hu, Yihan Zhu, Rujia Zou, Zhigang Chen, Shiping Yang, Runwei Li, Qianqian Su, Yu Han, and Xiaogang Liu pp 8571–8577 DOI: 10.1021/ja4013497 Supporting Info |
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Base-Catalyzed Bifunctional Addition to Amides and Imides at Low Temperature. A New Pathway for Carbonyl Hydrogenation Jeremy M. John, Satoshi Takebayashi, Nupur Dabral, Mark Miskolzie, and Steven H. Bergens pp 8578–8584 DOI: 10.1021/ja401294q Supporting Info |
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Function of the Diiron Cluster of Escherichia coli Class Ia Ribonucleotide Reductase in Proton-Coupled Electron Transfer Bigna Wörsdörfer, Denise A. Conner, Kenichi Yokoyama, Jovan Livada, Mohammad Seyedsayamdost, Wei Jiang, Alexey Silakov, JoAnne Stubbe, J. Martin Bollinger, Jr., and Carsten Krebs pp 8585–8593 DOI: 10.1021/ja401342s Supporting Info |
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One-Step Hydrothermal Synthesis of Manganese-Containing MFI-Type Zeolite, Mn–ZSM-5, Characterization, and Catalytic Oxidation of Hydrocarbons Yongtao Meng, Homer C. Genuino, Chung-Hao Kuo, Hui Huang, Sheng-Yu Chen, Lichun Zhang, Angelo Rossi, and Steven L. Suib pp 8594–8605 DOI: 10.1021/ja4013936 Supporting Info |
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Photooxidation of Ammonia on TiO2 as a Source of NO and NO2 under Atmospheric Conditions Mulu A. Kebede, Mychel E. Varner, Nicole K. Scharko, R. Benny Gerber, and Jonathan D. Raff pp 8606–8615 DOI: 10.1021/ja401846x |
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Understanding Molecular Motor Walking along a Microtubule: A Themosensitive Asymmetric Brownian Motor Driven by Bubble Formation Noriyoshi Arai, Kenji Yasuoka, Takahiro Koishi, Toshikazu Ebisuzaki, and Xiao Cheng Zeng pp 8616–8624 DOI: 10.1021/ja402014u Supporting Info |
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Carbocations Generated under Stable Conditions by Ionization of Matrix-Isolated Radicals: The Allyl and Benzyl Cations Vladimir Mišić, Krzysztof Piech, and Thomas Bally pp 8625–8631 DOI: 10.1021/ja401890m Supporting Info |
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Interaction of Tricationic Corroles with Single/Double Helix of Homopolymeric Nucleic Acids and DNA Alessandro D’Urso, Sara Nardis, Giuseppe Pomarico, Maria Elena Fragalà, Roberto Paolesse, and Roberto Purrello pp 8632–8638 DOI: 10.1021/ja4023539 Supporting Info |
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One-Dimensional Random Walk of a Synthetic Small Molecule Toward a Thermodynamic Sink Araceli G. Campaña, David A. Leigh, and Urszula Lewandowska pp 8639–8645 DOI: 10.1021/ja402382n Supporting Info |
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Nonprecious-Metal-Assisted Photochemical Hydrogen Production from ortho-Phenylenediamine Takeshi Matsumoto, Ho-Chol Chang, Masanori Wakizaka, Sho Ueno, Atsushi Kobayashi, Akira Nakayama, Tetsuya Taketsugu, and Masako Kato pp 8646–8654 DOI: 10.1021/ja4025116 Supporting Info |
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Stimuli Responsive Hybrid Magnets: Tuning the Photoinduced Spin-Crossover in Fe(III) Complexes Inserted into Layered Magnets Miguel Clemente-León, Eugenio Coronado, Maurici López-Jordà, João C. Waerenborgh, Cédric Desplanches, Hongfeng Wang, Jean-François Létard, Andreas Hauser, and Antoine Tissot pp 8655–8667 DOI: 10.1021/ja402674x Supporting Info |
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Understanding the Mechanisms of Cobalt-Catalyzed Hydrogenation and Dehydrogenation Reactions Guoqi Zhang, Kalyan V. Vasudevan, Brian L. Scott, and Susan K. Hanson pp 8668–8681 DOI: 10.1021/ja402679a Supporting Info |
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Nonadiabatic Dynamics of Positive Charge during Photocatalytic Water Splitting on GaN(10-10) Surface: Charge Localization Governs Splitting Efficiency Alexey V. Akimov, James T. Muckerman, and Oleg V. Prezhdo pp 8682–8691 DOI: 10.1021/ja4029395 Supporting Info |
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Insights into the Mechanism of Peptide Cyclodehydrations Achieved through the Chemoenzymatic Generation of Amide Derivatives Kyle L. Dunbar and Douglas A. Mitchell pp 8692–8701 DOI: 10.1021/ja4029507 Supporting Info |
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Quaternizing Diboranes(4): Highly Divergent Outcomes and an Inorganic Wagner–Meerwein Rearrangement Holger Braunschweig, Alexander Damme, Rian D. Dewhurst, Thomas Kramer, Thomas Kupfer, Krzysztof Radacki, Eva Siedler, Alexandra Trumpp, Katharina Wagner, and Christine Werner pp 8702–8707 DOI: 10.1021/ja403037k Supporting Info |
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Role of Solvent on Nonenzymatic Peptide Bond Formation Mechanisms and Kinetic Isotope Effects Katarzyna Świderek, Iñaki Tuñón, Sergio Martí, Vicent Moliner, and Juan Bertrán pp 8708–8719 DOI: 10.1021/ja403038t Supporting Info |
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Synthesis and Characterization of Patronite Form of Vanadium Sulfide on Graphitic Layer Chandra Sekhar Rout, Byeong-Hwan Kim, Xiaodong Xu, Jieun Yang, Hu Young Jeong, Dorj Odkhuu, Noejung Park, Jaephil Cho, and Hyeon Suk Shin pp 8720–8725 DOI: 10.1021/ja403232d Supporting Info |
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Metathesis Reactions of a Manganese Borylene Complex with Polar Heteroatom–Carbon Double Bonds: A Pathway to Previously Inaccessible Carbene Complexes Jürgen Bauer, Holger Braunschweig, Alexander Damme, Jose Oscar Carlos, Jimenez-Halla, Thomas Kramer, Krzysztof Radacki, Rong Shang, Eva Siedler, and Qing Ye pp 8726–8734 DOI: 10.1021/ja403389w Supporting Info |
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Transient Access to the Protein Interior: Simulation versus NMR Filip Persson and Bertil Halle pp 8735–8748 DOI: 10.1021/ja403405d Supporting Info |
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Ligand-Dependent Activation and Deactivation of the Human Adenosine A2A Receptor Jianing Li, Amanda L. Jonsson, Thijs Beuming, John C. Shelley, and Gregory A. Voth pp 8749–8759 DOI: 10.1021/ja404391q Supporting Info |
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Correction to “A Single-Component Liquid-Phase Hydrogen Storage Material” Wei Luo, Patrick G. Campbell, Lev N. Zakharov, and Shih-Yuan Liu pp 8760–8760 DOI: 10.1021/ja4039399 Supporting Info |
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Correction to “Quantification of the Effect of Conformational Restriction on Supramolecular Effective Molarities” Harry Adams, Elena Chekmeneva, Christopher A. Hunter, Maria Cristina Misuraca, Cristina Navarro, and Simon M. Turega pp 8761–8761 DOI: 10.1021/ja404462f |
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Spotlights on Recent JACS Publications pp 8763–8763 DOI: 10.1021/ja4058597 |
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Natural Product and Material Chemistries—Separated Forever? Horst Kunz and Klaus Müllen pp 8764–8769 DOI: 10.1021/ja309186q |
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Leukocyte-Mimicking Stem Cell Delivery via in Situ Coating of Cells with a Bioactive Hyperbranched Polyglycerol Jae Hyun Jeong, John J. Schmidt, Richie E. Kohman, Andrew T. Zill, Ross J. DeVolder, Cartney E. Smith, Mei-Hsiu Lai, Artem Shkumatov, Tor W. Jensen, Lawrence G. Schook, Steven C. Zimmerman, and Hyunjoon Kong pp 8770–8773 DOI: 10.1021/ja400636d Supporting Info |
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Facile B–H Bond Activation of Borane by Stable Carbenoid Species Hadrien Heuclin, Samuel Y.-F. Ho, Xavier F. Le Goff, Cheuk-Wai So, and Nicolas Mézailles pp 8774–8777 DOI: 10.1021/ja401763c Supporting Info |
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Stereoengineering of Poly(1,3-methylenecyclohexane) via Two-State Living Coordination Polymerization of 1,6-Heptadiene Kaitlyn E. Crawford and Lawrence R. Sita pp 8778–8781 DOI: 10.1021/ja402262x Supporting Info |
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Trifluoromethanesulfonyl Hypervalent Iodonium Ylide for Copper-Catalyzed Trifluoromethylthiolation of Enamines, Indoles, and β-Keto Esters Yu-Dong Yang, Ayaka Azuma, Etsuko Tokunaga, Mikio Yamasaki, Motoo Shiro, and Norio Shibata pp 8782–8785 DOI: 10.1021/ja402455f Supporting Info |
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Structure of Au15(SR)13 and Its Implication for the Origin of the Nucleus in Thiolated Gold Nanoclusters De-en Jiang, Steven H. Overbury, and Sheng Dai pp 8786–8789 DOI: 10.1021/ja402680c Supporting Info |
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Charge Carrier Dynamics of Vapor-Deposited Small-Molecule/Fullerene Organic Solar Cells Angela Y. Chang, Yi-Hong Chen, Hao-Wu Lin, Li-Yen Lin, Ken-Tsung Wong, and Richard D. Schaller pp 8790–8793 DOI: 10.1021/ja403056y Supporting Info |
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Pyramidanes Vladimir Ya. Lee, Yuki Ito, Akira Sekiguchi, Heinz Gornitzka, Olga A. Gapurenko, Vladimir I. Minkin, and Ruslan M. Minyaev pp 8794–8797 DOI: 10.1021/ja403173e Supporting Info |
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Selective Conversion of CO2 to CO with High Efficiency Using an Inexpensive Bismuth-Based Electrocatalyst John L. DiMeglio and Joel Rosenthal pp 8798–8801 DOI: 10.1021/ja4033549 Supporting Info |
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RhIII/CuII-Cocatalyzed Synthesis of 1H-Indazoles through C–H Amidation and N–N Bond Formation Da-Gang Yu, Mamta Suri, and Frank Glorius pp 8802–8805 DOI: 10.1021/ja4033555 Supporting Info |
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Microporous Aluminophosphate Nanosheets and Their Nanomorphic Zeolite Analogues Tailored by Hierarchical Structure-Directing Amines Yongbeom Seo, Sungjune Lee, Changbum Jo, and Ryong Ryoo pp 8806–8809 DOI: 10.1021/ja403580j Supporting Info |
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Rare Earth Metal-Mediated Group-Transfer Polymerization: From Defined Polymer Microstructures to High-Precision Nano-Scaled Objects Ning Zhang, Stephan Salzinger, Benedikt S. Soller, and Bernhard Rieger pp 8810–8813 DOI: 10.1021/ja4036175 Supporting Info |
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Surface Control of Alkyl Chain Conformations and 2D Chiral Amplification Nadine Hauptmann, Katharina Scheil, Thiruvancheril G. Gopakumar, Franziska L. Otte, Christian Schütt, Rainer Herges, and Richard Berndt pp 8814–8817 DOI: 10.1021/ja4036187 Supporting Info |
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Expulsion of Ions from Hydrophobic Hydration Shells Blake M. Rankin and Dor Ben-Amotz pp 8818–8821 DOI: 10.1021/ja4036303 Supporting Info |
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Metal-Cluster-Sensitized Solar Cells. A New Class of Thiolated Gold Sensitizers Delivering Efficiency Greater Than 2% Yong-Siou Chen, Hyunbong Choi, and Prashant V. Kamat pp 8822–8825 DOI: 10.1021/ja403807f Supporting Info |
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Chemistry at the Alkyne–Carbene Intersection: A Metallacyclobutene−η3-Vinylcarbene Equilibration Joseph M. O’Connor, Kim K. Baldridge, Carmen L. Vélez, Arnold L. Rheingold, and Curtis E. Moore pp 8826–8829 DOI: 10.1021/ja4039483 Supporting Info |
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Synthesis, Characterization, and Heterobimetallic Cooperation in a Titanium–Chromium Catalyst for Highly Branched Polyethylenes Shaofeng Liu, Alessandro Motta, Massimiliano Delferro, and Tobin J. Marks pp 8830–8833 DOI: 10.1021/ja4039505 Supporting Info |
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Naphthodithiophene–Naphthobisthiadiazole Copolymers for Solar Cells: Alkylation Drives the Polymer Backbone Flat and Promotes Efficiency Itaru Osaka, Takeshi Kakara, Noriko Takemura, Tomoyuki Koganezawa, and Kazuo Takimiya pp 8834–8837 DOI: 10.1021/ja404064m Supporting Info |
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A Mononuclear Non-Heme High-Spin Iron(III)–Hydroperoxo Complex as an Active Oxidant in Sulfoxidation Reactions Yun Mi Kim, Kyung-Bin Cho, Jaeheung Cho, Binju Wang, Chunsen Li, Sason Shaik, and Wonwoo Nam pp 8838–8841 DOI: 10.1021/ja404152q Supporting Info |
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A π-Conjugated System with Flexibility and Rigidity That Shows Environment-Dependent RGB Luminescence Chunxue Yuan, Shohei Saito, Cristopher Camacho, Stephan Irle, Ichiro Hisaki, and Shigehiro Yamaguchi pp 8842–8845 DOI: 10.1021/ja404198h Supporting Info |
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Sulfonyl 3-Alkynyl Pantetheinamides as Mechanism-Based Cross-Linkers of Acyl Carrier Protein Dehydratase Fumihiro Ishikawa, Robert W. Haushalter, D. John Lee, Kara Finzel, and Michael D. Burkart pp 8846–8849 DOI: 10.1021/ja4042059 Supporting Info |
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An Efficient Rh/O2 Catalytic System for Oxidative C–H Activation/Annulation: Evidence for Rh(I) to Rh(III) Oxidation by Molecular Oxygen Guoying Zhang, Lei Yang, Yanyu Wang, Yinjun Xie, and Hanmin Huang pp 8850–8853 DOI: 10.1021/ja404414q Supporting Info |
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Enantioselective Palladium-Catalyzed Diamination of Alkenes Using N-Fluorobenzenesulfonimide Erica L. Ingalls, Paul A. Sibbald, Werner Kaminsky, and Forrest E. Michael pp 8854–8856 DOI: 10.1021/ja4043406 Supporting Info |
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A Frontier Orbital Study with ab Initio Molecular Dynamics of the Effects of Solvation on Chemical Reactivity: Solvent-Induced Orbital Control in FeO-Activated Hydroxylation Reactions Leonardo Bernasconi and Evert Jan Baerends pp 8857–8867 DOI: 10.1021/ja311144d Supporting Info |
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Electrogenerated Chemiluminescence of Solutions, Films, and Nanoparticles of Dithienylbenzothiadiazole-Based Donor–Acceptor–Donor Red Fluorophore. Fluorescence Quenching Study of Organic Nanoparticles Mei Shen, Xu-Hui Zhu, and Allen J. Bard pp 8868–8873 DOI: 10.1021/ja312189k Supporting Info |
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Noise Characteristics of Nanoscaled Redox-Cycling Sensors: Investigations Based on Random Walks Enno Kätelhön, Kay J. Krause, Pradyumna S. Singh, Serge G. Lemay, and Bernhard Wolfrum pp 8874–8881 DOI: 10.1021/ja3121313 Supporting Info |
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Noninteracting, Vicinal Frustrated P/B-Lewis Pair at the Norbornane Framework: Synthesis, Characterization, and Reactions Muhammad Sajid, Gerald Kehr, Thomas Wiegand, Hellmut Eckert, Christian Schwickert, Rainer Pöttgen, Allan Jay P. Cardenas, Timothy H. Warren, Roland Fröhlich, Constantin G. Daniliuc, and Gerhard Erker pp 8882–8895 DOI: 10.1021/ja400338e Supporting Info |
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Fe3–xTixO4 Nanoparticles as Tunable Probes of Microbial Metal Oxidation Juan Liu, Carolyn I. Pearce, Chongxuan Liu, Zheming Wang, Liang Shi, Elke Arenholz, and Kevin M. Rosso pp 8896–8907 DOI: 10.1021/ja4015343 |
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Adenosine Triphosphate Hydrolysis Mechanism in Kinesin Studied by Combined Quantum-Mechanical/Molecular-Mechanical Metadynamics Simulations Matthew J. McGrath, I.-F. Will Kuo, Shigehiko Hayashi, and Shoji Takada pp 8908–8919 DOI: 10.1021/ja401540g Supporting Info |
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Direct Observation of RecBCD Helicase as Single-Stranded DNA Translocases Cinya Chung and Hung-Wen Li pp 8920–8925 DOI: 10.1021/ja401626t Supporting Info |
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Ambient-Processable High Capacitance Hafnia-Organic Self-Assembled Nanodielectrics Ken Everaerts, Jonathan D. Emery, Deep Jariwala, Hunter J. Karmel, Vinod K. Sangwan, Pradyumna L. Prabhumirashi, Michael L. Geier, Julian J. McMorrow, Michael J. Bedzyk, Antonio Facchetti, Mark C. Hersam, and Tobin J. Marks pp 8926–8939 DOI: 10.1021/ja4019429 Supporting Info |
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Nanoporous Metal Oxides with Tunable and Nanocrystalline Frameworks via Conversion of Metal–Organic Frameworks Tae Kyung Kim, Kyung Joo Lee, Jae Yeong Cheon, Jae Hwa Lee, Sang Hoon Joo, and Hoi Ri Moon pp 8940–8946 DOI: 10.1021/ja401869h Supporting Info |
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Temperature-Sensitive Transitions below LCST in Amphiphilic Dendritic Assemblies: Host–Guest Implications Jack M. Fuller, Krishna R. Raghupathi, Rajasekhar R. Ramireddy, Ayyagari V. Subrahmanyam, Volkan Yesilyurt, and S. Thayumanavan pp 8947–8954 DOI: 10.1021/ja402019c Supporting Info |
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Theoretical Study of Reactivity of Ge(II)-hydride Compound: Comparison with Rh(I)-Hydride Complex and Prediction of Full Catalytic Cycle by Ge(II)-hydride Nozomi Takagi and Shigeyoshi Sakaki pp 8955–8965 DOI: 10.1021/ja402039b Supporting Info |
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Magnetoluminescent Light Switches – Dual Modality in DNA Detection Eric D. Smolensky, Katie L. Peterson, Evan A. Weitz, Cutler Lewandowski, and Valérie C. Pierre pp 8966–8972 DOI: 10.1021/ja402107x |
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Regioselective Covalent Immobilization of Recombinant Antibody-Binding Proteins A, G, and L for Construction of Antibody Arrays Jin-soo Seo, Sungwon Lee, and C. Dale Poulter pp 8973–8980 DOI: 10.1021/ja402447g Supporting Info |
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Nitrogen-Doped Graphene Nanoplatelets from Simple Solution Edge-Functionalization for n-Type Field-Effect Transistors Dong Wook Chang, Eun Kwang Lee, Eun Yeob Park, Hojeong Yu, Hyun-Jung Choi, In-Yup Jeon, Gyung-Joo Sohn, Dongbin Shin, Noejung Park, Joon Hak Oh, Liming Dai, and Jong-Beom Baek pp 8981–8988 DOI: 10.1021/ja402555n Supporting Info |
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How Do Liquid Mixtures Solubilize Insoluble Gelators? Self-Assembly Properties of Pyrenyl-Linker-Glucono Gelators in Tetrahydrofuran–Water Mixtures Ni Yan, Zhiyan Xu, Kevin K. Diehn, Srinivasa R. Raghavan, Yu Fang, and Richard G. Weiss pp 8989–8999 DOI: 10.1021/ja402560n Supporting Info |
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Overcoming Product Inhibition in Catalysis of the Intramolecular Schmidt Reaction Hashim F. Motiwala, Charlie Fehl, Sze-Wan Li, Erin Hirt, Patrick Porubsky, and Jeffrey Aubé pp 9000–9009 DOI: 10.1021/ja402848c Supporting Info |
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Direct Observation of Photodissociation Products from Phenylperoxyl Radicals Isolated in the Gas Phase Alan T. Maccarone, Benjamin B. Kirk, Christopher S. Hansen, Thomas M. Griffiths, Seth Olsen, Adam J. Trevitt, and Stephen J. Blanksby pp 9010–9014 DOI: 10.1021/ja402610s Supporting Info |
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Photoinduced Charge Transfer and Acetone Sensitivity of Single-Walled Carbon Nanotube–Titanium Dioxide Hybrids Mengning Ding, Dan C. Sorescu, and Alexander Star pp 9015–9022 DOI: 10.1021/ja402887v Supporting Info |
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Proton-Coupled Electron Transfer Cleavage of Heavy-Atom Bonds in Electrocatalytic Processes. Cleavage of a C–O Bond in the Catalyzed Electrochemical Reduction of CO2 Cyrille Costentin, Samuel Drouet, Guillaume Passard, Marc Robert, and Jean-Michel Savéant pp 9023–9031 DOI: 10.1021/ja4030148 Supporting Info |
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Were Reactions of Triplet Silylenes Observed? Monica Kosa, Miriam Karni, and Yitzhak Apeloig pp 9032–9040 DOI: 10.1021/ja403068r Supporting Info |
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Electrochemistry and Electrogenerated Chemiluminescence of Three Phenanthrene Derivatives, Enhancement of Radical Stability, and Electrogenerated Chemiluminescence Efficiency by Substituent Groups Honglan Qi, Yu-Han Chen, Chien-Hong Cheng, and Allen J. Bard pp 9041–9049 DOI: 10.1021/ja403166s Supporting Info |
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Low-Temperature, Bottom-Up Synthesis of Graphene via a Radical-Coupling Reaction Lang Jiang, Tianchao Niu, Xiuqiang Lu, Huanli Dong, Wei Chen, Yunqi Liu, Wenping Hu, and Daoben Zhu pp 9050–9054 DOI: 10.1021/ja4031825 Supporting Info |
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Modular Synthesis of Amphiphilic Janus Glycodendrimers and Their Self-Assembly into Glycodendrimersomes and Other Complex Architectures with Bioactivity to Biomedically Relevant Lectins Virgil Percec, Pawaret Leowanawat, Hao-Jan Sun, Oleg Kulikov, Christopher D. Nusbaum, Tam M. Tran, Annabelle Bertin, Daniela A. Wilson, Mihai Peterca, Shaodong Zhang, Neha P. Kamat, Kevin Vargo, Diana Moock, Eric D. Johnston, Daniel A. Hammer, Darrin J. Pochan, Yingchao Chen, Yoann M. Chabre, Tze C. Shiao, Milan Bergeron-Brlek, Sabine André, René Roy, Hans-J. Gabius, and Paul A. Heiney pp 9055–9077 DOI: 10.1021/ja403323y Supporting Info |
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Direct Detection and Reactivity of the Short-Lived Phenyloxenium Ion Patrick J. Hanway, Jiadan Xue, Ujjal Bhattacharjee, Maeia J. Milot, Zhu Ruixue, David Lee Phillips, and Arthur H. Winter pp 9078–9082 DOI: 10.1021/ja403370k Supporting Info |
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Functional-Group-Tolerant, Nickel-Catalyzed Cross-Coupling Reaction for Enantioselective Construction of Tertiary Methyl-Bearing Stereocenters Hanna M. Wisniewska, Elizabeth C. Swift, and Elizabeth R. Jarvo pp 9083–9090 DOI: 10.1021/ja4034999 Supporting Info |
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A Mechanistic Rationale for the 9-Amino(9-deoxy)epi Cinchona Alkaloids Catalyzed Asymmetric Reactions via Iminium Ion Activation of Enones Antonio Moran, Alex Hamilton, Carles Bo, and Paolo Melchiorre pp 9091–9098 DOI: 10.1021/ja404784t Supporting Info |
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Investigating the Multiple Roles of Polyvinylpyrrolidone for a General Methodology of Oxide Encapsulation Hang Sun, Jiating He, Jiangyan Wang, Shuang-Yuan Zhang, Cuicui Liu, Thirumany Sritharan, Subodh Mhaisalkar, Ming-Yong Han, Dan Wang, and Hongyu Chen pp 9099–9110 DOI: 10.1021/ja4035335 Supporting Info |
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Redox-Based Control of the Transformation and Activation of siRNA Complexes in Extracellular Environments Using Ferrocenyl Lipids Burcu S. Aytar, John P. E. Muller, Yukishige Kondo, Yeshayahu Talmon, Nicholas L. Abbott, and David M. Lynn pp 9111–9120 DOI: 10.1021/ja403546b |
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Small, Highly Active DNAs That Hydrolyze DNA Hongzhou Gu, Kazuhiro Furukawa, Zasha Weinberg, Daniel F. Berenson, and Ronald R. Breaker pp 9121–9129 DOI: 10.1021/ja403585e Supporting Info |
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A Coupled Protein and Probe Engineering Approach for Selective Inhibition and Activity-Based Probe Labeling of the Caspases Junpeng Xiao, Petr Broz, Aaron W. Puri, Edgar Deu, Montse Morell, Denise M. Monack, and Matthew Bogyo pp 9130–9138 DOI: 10.1021/ja403521u Supporting Info |
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Coupling Protein Engineering with Probe Design To Inhibit and Image Matrix Metalloproteinases with Controlled Specificity Montse Morell, Thinh Nguyen Duc, Amanda L. Willis, Salahuddin Syed, Jiyoun Lee, Edgar Deu, Yang Deng, Junpeng Xiao, Benjamin E. Turk, Jason R. Jessen, Stephen J. Weiss, and Matthew Bogyo pp 9139–9148 DOI: 10.1021/ja403523p Supporting Info |
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Kinetic Mechanism of Translocation and dNTP Binding in Individual DNA Polymerase Complexes Kate R. Lieberman, Joseph M. Dahl, Ai H. Mai, Ashley Cox, Mark Akeson, and Hongyun Wang pp 9149–9155 DOI: 10.1021/ja403640b Supporting Info |
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Opposing Auxiliary Conformations Produce the Same Torquoselectivity in an Oxazolidinone-Directed Nazarov Cyclization Bernard L. Flynn, Narasimhulu Manchala, and Elizabeth H. Krenske pp 9156–9163 DOI: 10.1021/ja4036434 Supporting Info |
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A Structure-Based Model of Energy Transfer Reveals the Principles of Light Harvesting in Photosystem II Supercomplexes Doran I. G. Bennett, Kapil Amarnath, and Graham R. Fleming pp 9164–9173 DOI: 10.1021/ja403685a Supporting Info |
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Chirality Control for in Situ Preparation of Gold Nanoparticle Superstructures Directed by a Coordinatable Organogelator Liangliang Zhu, Xin Li, Shaojue Wu, Kim Truc Nguyen, Hong Yan, Hans Ågren, and Yanli Zhao pp 9174–9180 DOI: 10.1021/ja403722t Supporting Info |
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A Self-Calibrating Bipartite Viscosity Sensor for Mitochondria Zhigang Yang, Yanxia He, Jae-Hong Lee, Nayoung Park, Myungkoo Suh, Weon-Sik Chae, Jianfang Cao, Xiaojun Peng, Hyosung Jung, Chulhun Kang, and Jong Seung Kim pp 9181–9185 DOI: 10.1021/ja403851p Supporting Info |
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Enhanced Electron-Transfer Reactivity of Nonheme Manganese(IV)–Oxo Complexes by Binding Scandium Ions Heejung Yoon, Yong-Min Lee, Xiujuan Wu, Kyung-Bin Cho, Ritimukta Sarangi, Wonwoo Nam, and Shunichi Fukuzumi pp 9186–9194 DOI: 10.1021/ja403965h Supporting Info |
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Theoretical Study of Interfacial Electron Transfer from Reduced Anatase TiO2(101) to Adsorbed O2 Ye-Fei Li and Annabella Selloni pp 9195–9199 DOI: 10.1021/ja404044t Supporting Info |
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Formation and Characterization of a Molecule–Metal–Molecule Bridge in Real Space Florian Albrecht, Mathias Neu, Christina Quest, Ingmar Swart, and Jascha Repp pp 9200–9203 DOI: 10.1021/ja404084p Supporting Info |
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Photoreaction of a Hydroxyalkyphenone with the Membrane of Polymersomes: A Versatile Method To Generate Semipermeable Nanoreactors Mariana Spulber, Adrian Najer, Katharina Winkelbach, Olfa Glaied, Marcus Waser, Uwe Pieles, Wolfgang Meier, and Nico Bruns pp 9204–9212 DOI: 10.1021/ja404175x Supporting Info |
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Synthesis and Conformational Dynamics of the Reported Structure of Xylopyridine A Robert-André F. Rarig, Mai N. Tran, and David M. Chenoweth pp 9213–9219 DOI: 10.1021/ja404737q Supporting Info |
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Correction to “Quantifying Functional Group Interactions That Determine Urea Effects on Nucleic Acid Helix Formation” Emily J. Guinn, Jeffrey J. Schwinefus, Hyo Keun Cha, Joseph L. McDevitt, Wolf E. Merker, Ryan Ritzer, Gregory W. Muth, Samuel W. Engelsgjerd, Kathryn E. Mangold, Perry J. Thompson, Michael J. Kerins, and M. Thomas Record, Jr. pp 9220–9220 DOI: 10.1021/ja404053h |
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Spotlights on Recent JACS Publications pp 9221–9221 DOI: 10.1021/ja4060405 |
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Dynamic Combinatorial Libraries: From Exploring Molecular Recognition to Systems Chemistry Jianwei Li, Piotr Nowak, and Sijbren Otto pp 9222–9239 DOI: 10.1021/ja402586c |
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Covalently Patterned Graphene Surfaces by a Force-Accelerated Diels–Alder Reaction Shudan Bian, Amy M. Scott, Yang Cao, Yong Liang, Sílvia Osuna, K. N. Houk, and Adam B. Braunschweig pp 9240–9243 DOI: 10.1021/ja4042077 Supporting Info |
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Bifunctional Unnatural Sialic Acids for Dual Metabolic Labeling of Cell-Surface Sialylated Glycans Lianshun Feng, Senlian Hong, Jie Rong, Qiancheng You, Peng Dai, Rongbing Huang, Yanhong Tan, Weiyao Hong, Can Xie, Jing Zhao, and Xing Chen pp 9244–9247 DOI: 10.1021/ja402326z Supporting Info |
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Creating Protein-Imprinted Self-Assembled Monolayers with Multiple Binding Sites and Biocompatible Imprinted Cavities Xianfeng Zhang, Xuezhong Du, Xuan Huang, and Zhongpeng Lv pp 9248–9251 DOI: 10.1021/ja402423r Supporting Info |
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Catalytic Enantioselective One-pot Aminoborylation of Aldehydes: A Strategy for Construction of Nonracemic α-Amino Boronates Kai Hong and James P. Morken pp 9252–9254 DOI: 10.1021/ja402569j Supporting Info |
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Pd-Catalyzed Asymmetric Allylic Alkylation of Pyrazol-5-ones with Allylic Alcohols: The Role of the Chiral Phosphoric Acid in C–O Bond Cleavage and Stereocontrol Zhong-Lin Tao, Wen-Quan Zhang, Dian-Feng Chen, Arafate Adele, and Liu-Zhu Gong pp 9255–9258 DOI: 10.1021/ja402740q Supporting Info |
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Measurement of Active Site Ionization Equilibria in the 670 kDa Proteasome Core Particle Using Methyl-TROSY NMR Algirdas Velyvis and Lewis E. Kay pp 9259–9262 DOI: 10.1021/ja403091c Supporting Info |
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Postsynthetic Modification of Dicarbene-Derived Metallacycles via Photochemical [2 + 2] Cycloaddition Ying-Feng Han, Guo-Xin Jin, and F. Ekkehardt Hahn pp 9263–9266 DOI: 10.1021/ja4032067 Supporting Info |
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Nanostructured Nickel Phosphide as an Electrocatalyst for the Hydrogen Evolution Reaction Eric J. Popczun, James R. McKone, Carlos G. Read, Adam J. Biacchi, Alex M. Wiltrout, Nathan S. Lewis, and Raymond E. Schaak pp 9267–9270 DOI: 10.1021/ja403440e Supporting Info |
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Rh-Catalyzed (5+2) Cycloadditions of 3-Acyloxy-1,4-enynes and Alkynes: Computational Study of Mechanism, Reactivity, and Regioselectivity Xiufang Xu, Peng Liu, Xing-zhong Shu, Weiping Tang, and K. N. Houk pp 9271–9274 DOI: 10.1021/ja4036785 Supporting Info |
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Sensitization of p-GaP with CdSe Quantum Dots: Light-Stimulated Hole Injection Zhijie Wang, Anisha Shakya, Junsi Gu, Shichen Lian, and Stephen Maldonado pp 9275–9278 DOI: 10.1021/ja403701p Supporting Info |
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Cobalt-Catalyzed Ortho Alkylation of Aromatic Imines with Primary and Secondary Alkyl Halides Ke Gao and Naohiko Yoshikai pp 9279–9282 DOI: 10.1021/ja403759x Supporting Info |
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Enantioselective Synthesis of Cyclobutanes via Sequential Rh-catalyzed Bicyclobutanation/Cu-catalyzed Homoconjugate Addition Robert Panish, Srinivasa R. Chintala, David T. Boruta, Yinzhi Fang, Michael T. Taylor, and Joseph M. Fox pp 9283–9286 DOI: 10.1021/ja403811t Supporting Info |
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Evidence of Pressure Enhanced CO2 Storage in ZIF-8 Probed by FTIR Spectroscopy Yue Hu, Zhenxian Liu, Jun Xu, Yining Huang, and Yang Song pp 9287–9290 DOI: 10.1021/ja403635b Supporting Info |
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Bioinspired Total Synthesis of Bolivianine: A Diels– Alder/Intramolecular Hetero-Diels–Alder Cascade Approach Changchun Yuan, Biao Du, Li Yang, and Bo Liu pp 9291–9294 DOI: 10.1021/ja4040335 Supporting Info |
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Dynamic Amphiphile Libraries To Screen for the “Fragrant” Delivery of siRNA into HeLa Cells and Human Primary Fibroblasts Charlotte Gehin, Javier Montenegro, Eun-Kyoung Bang, Ana Cajaraville, Shota Takayama, Hisaaki Hirose, Shiroh Futaki, Stefan Matile, and Howard Riezman pp 9295–9298 DOI: 10.1021/ja404153m Supporting Info |
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The Structure of the Mercury Transporter MerF in Phospholipid Bilayers: A Large Conformational Rearrangement Results from N-Terminal Truncation George J. Lu, Ye Tian, Nemil Vora, Francesca M. Marassi, and Stanley J. Opella pp 9299–9302 DOI: 10.1021/ja4042115 Supporting Info |
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Iridium-Catalyzed, Intermolecular Hydroetherification of Unactivated Aliphatic Alkenes with Phenols Christo S. Sevov and John F. Hartwig pp 9303–9306 DOI: 10.1021/ja4052153 Supporting Info |
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In silico Design of Supramolecules from Their Precursors: Odd–Even Effects in Cage-Forming Reactions Kim E. Jelfs, Edward G. B. Eden, Jamie L. Culshaw, Stephen Shakespeare, Edward O. Pyzer-Knapp, Hugh P. G. Thompson, John Bacsa, Graeme M. Day, Dave J. Adams, and Andrew I. Cooper pp 9307–9310 DOI: 10.1021/ja404253j Supporting Info |
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Supersaturation-Dependent Surface Structure Evolution: From Ionic, Molecular to Metallic Micro/Nanocrystals Hai-xin Lin, Zhi-chao Lei, Zhi-yuan Jiang, Chang-ping Hou, De-yu Liu, Min-min Xu, Zhong-qun Tian, and Zhao-xiong Xie pp 9311–9314 DOI: 10.1021/ja404371k Supporting Info |
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Chemical Modification-Assisted Bisulfite Sequencing (CAB-Seq) for 5-Carboxylcytosine Detection in DNA Xingyu Lu, Chun-Xiao Song, Keith Szulwach, Zhipeng Wang, Payton Weidenbacher, Peng Jin, and Chuan He pp 9315–9317 DOI: 10.1021/ja4044856 Supporting Info |
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Pd-Catalyzed Chemoselective Catellani Ortho-Arylation of Iodopyrroles: Rapid Total Synthesis of Rhazinal Xianwei Sui, Rui Zhu, Gencheng Li, Xinna Ma, and Zhenhua Gu pp 9318–9321 DOI: 10.1021/ja404494u Supporting Info |
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Pd(II)-Catalyzed Phosphorylation of Aryl C–H Bonds Chen-Guo Feng, Mengchun Ye, Kai-Jiong Xiao, Suhua Li, and Jin-Quan Yu pp 9322–9325 DOI: 10.1021/ja404526x Supporting Info |
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A Highly Active Phosphine–Borane Organocatalyst for the Reduction of CO2 to Methanol Using Hydroboranes Marc-André Courtemanche, Marc-André Légaré, Laurent Maron, and Frédéric-Georges Fontaine pp 9326–9329 DOI: 10.1021/ja404585p Supporting Info |
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Concurrent Cationic Vinyl-Addition and Ring-Opening Copolymerization Using B(C6F5)3 as a Catalyst: Copolymerization of Vinyl Ethers and Isobutylene Oxide via Crossover Propagation Reactions Arihiro Kanazawa, Shokyoku Kanaoka, and Sadahito Aoshima pp 9330–9333 DOI: 10.1021/ja404616c Supporting Info |
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Cryptocaryols A and B: Total Syntheses, Stereochemical Revision, Structure Elucidation, and Structure–Activity Relationship Yanping Wang and George A. O’Doherty pp 9334–9337 DOI: 10.1021/ja404401f Supporting Info |
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Total Synthesis of (−)-Nakadomarin A Simone Bonazzi, Bichu Cheng, Joseph S. Wzorek, and David A. Evans pp 9338–9341 DOI: 10.1021/ja404673s Supporting Info |
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Copper-Catalyzed, Directing Group-Assisted Fluorination of Arene and Heteroarene C–H Bonds Thanh Truong, Kristine Klimovica, and Olafs Daugulis pp 9342–9345 DOI: 10.1021/ja4047125 Supporting Info |
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A Pentacoordinate Boron-Containing π-Electron System with Cl–B–Cl Three-Center Four-Electron Bonds Chuandong Dou, Shohei Saito, and Shigehiro Yamaguchi pp 9346–9349 DOI: 10.1021/ja404724f Supporting Info |
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Cu-Catalyzed Mild C(sp2)–H Functionalization Assisted by Carboxylic Acids en Route to Hydroxylated Arenes Joan Gallardo-Donaire and Ruben Martin pp 9350–9353 DOI: 10.1021/ja4047894 Supporting Info |
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Catalyzing Pyramidal Inversion: Configurational Lability of P-Stereogenic Phosphines via Single Electron Oxidation Kyle D. Reichl, Daniel H. Ess, and Alexander T. Radosevich pp 9354–9357 DOI: 10.1021/ja404943x Supporting Info |
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Enantioselective Intramolecular Aldehyde α-Alkylation with Simple Olefins: Direct Access to Homo-Ene Products Robert J. Comito, Fernanda G. Finelli, and David W. C. MacMillan pp 9358–9361 DOI: 10.1021/ja4047312 Supporting Info |
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‘Multicopy Multivalent’ Glycopolymer-Stabilized Gold Nanoparticles as Potential Synthetic Cancer Vaccines Alison L. Parry, Natasha A. Clemson, James Ellis, Stefan S. R. Bernhard, Benjamin G. Davis, and Neil R. Cameron pp 9362–9365 DOI: 10.1021/ja4046857 Supporting Info |
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Crystalline Arrays of Pairs of Molecular Rotors: Correlated Motion, Rotational Barriers, and Space-Inversion Symmetry Breaking Due to Conformational Mutations Cyprien Lemouchi, Konstantinos Iliopoulos, Leokadiya Zorina, Sergey Simonov, Pawel Wzietek, Thomas Cauchy, Antonio Rodríguez-Fortea, Enric Canadell, Jiřı́ Kaleta, Josef Michl, Denis Gindre, Michael Chrysos, and Patrick Batail pp 9366–9376 DOI: 10.1021/ja4044517 Supporting Info |
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Allosteric Activation of the Par-6 PDZ via a Partial Unfolding Transition Dustin S. Whitney, Francis C. Peterson, Evgenii L. Kovrigin, and Brian F. Volkman pp 9377–9383 DOI: 10.1021/ja400092a Supporting Info |
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Insights into the Mechanism by Which Interferon-γ Basic Amino Acid Clusters Mediate Protein Binding to Heparan Sulfate Els Saesen, Stéphane Sarrazin, Cédric Laguri, Rabia Sadir, Damien Maurin, Aline Thomas, Anne Imberty, and Hugues Lortat-Jacob pp 9384–9390 DOI: 10.1021/ja4000867 Supporting Info |
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Retinal Conformation Governs pKa of Protonated Schiff Base in Rhodopsin Activation Shengshuang Zhu, Michael F. Brown, and Scott E. Feller pp 9391–9398 DOI: 10.1021/ja4002986 Supporting Info |
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Mechanistic Insights into C–H Amination via Dicopper Nitrenes Mae Joanne B. Aguila, Yosra M. Badiei, and Timothy H. Warren pp 9399–9406 DOI: 10.1021/ja400879m Supporting Info |
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Photoswitching of Enzyme Activity by Laser-Induced pH-Jump Stefanie Kohse, Antje Neubauer, Alexandra Pazidis, Stefan Lochbrunner, and Udo Kragl pp 9407–9411 DOI: 10.1021/ja400700x Supporting Info |
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Efficacy of Base-Modification on Target Binding of Small Molecule DNA Aptamers Yuri Imaizumi, Yuuya Kasahara, Hiroto Fujita, Shunsuke Kitadume, Hiroaki Ozaki, Tamaki Endoh, Masayasu Kuwahara, and Naoki Sugimoto pp 9412–9419 DOI: 10.1021/ja4012222 Supporting Info |
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Irreversibility and Hysteresis in Redox Molecular Conduction Junctions Agostino Migliore and Abraham Nitzan pp 9420–9432 DOI: 10.1021/ja401336u Supporting Info |
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The Electronic Nature of Terminal Oxo Ligands in Transition-Metal Complexes: Ambiphilic Reactivity of Oxorhenium Species Jessica L. Smeltz, Cassandra P. Lilly, Paul D. Boyle, and Elon A. Ison pp 9433–9441 DOI: 10.1021/ja401390v Supporting Info |
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Substrate Water Exchange for the Oxygen Evolving Complex in PSII in the S1, S2, and S3 States Per E. M. Siegbahn pp 9442–9449 DOI: 10.1021/ja401517e Supporting Info |
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Binding Motif of Terminal Alkynes on Gold Clusters Prasenjit Maity, Shinjiro Takano, Seiji Yamazoe, Tomonari Wakabayashi, and Tatsuya Tsukuda pp 9450–9457 DOI: 10.1021/ja401798z Supporting Info |
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Highly Selective Quantum Sieving of D2 from H2 by a Metal–Organic Framework As Determined by Gas Manometry and Infrared Spectroscopy Stephen A. FitzGerald, Christopher J. Pierce, Jesse L. C. Rowsell, Eric D. Bloch, and Jarad A. Mason pp 9458–9464 DOI: 10.1021/ja402103u Supporting Info |
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The Role of Ligands on the Equilibria Between Functional States of a G Protein-Coupled Receptor Tae Hun Kim, Ka Young Chung, Aashish Manglik, Alexandar L. Hansen, Ron O. Dror, Thomas J. Mildorf, David E. Shaw, Brian K. Kobilka, and R. Scott Prosser pp 9465–9474 DOI: 10.1021/ja404305k Supporting Info |
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Simple and Sustainable Iron-Catalyzed Aerobic C–H Functionalization of N,N-Dialkylanilines Maxim O. Ratnikov, Xinfang Xu, and Michael P. Doyle pp 9475–9479 DOI: 10.1021/ja402479r Supporting Info |
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Ultrathin and Ultralong Single-Crystal Platinum Nanowire Assemblies with Highly Stable Electrocatalytic Activity Bao Yu Xia, Hao Bin Wu, Ya Yan, Xiong Wen (David) Lou, and Xin Wang pp 9480–9485 DOI: 10.1021/ja402955t Supporting Info |
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Adducts of Nitrous Oxide and N-Heterocyclic Carbenes: Syntheses, Structures, and Reactivity Alexander G. Tskhovrebov, Basile Vuichoud, Euro Solari, Rosario Scopelliti, and Kay Severin pp 9486–9492 DOI: 10.1021/ja4030287 Supporting Info |
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Uncovering a Dynamically Formed Substrate Access Tunnel in Carbon Monoxide Dehydrogenase/Acetyl-CoA Synthase Po-hung Wang, Maurizio Bruschi, Luca De Gioia, and Jochen Blumberger pp 9493–9502 DOI: 10.1021/ja403110s Supporting Info |
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Synthesis of Tetragonal and Orthorhombic Polymorphs of Hf3N4 by High-Pressure Annealing of a Prestructured Nanocrystalline Precursor Ashkan Salamat, Andrew L. Hector, Benjamin M. Gray, Simon A. J. Kimber, Pierre Bouvier, and Paul F. McMillan pp 9503–9511 DOI: 10.1021/ja403368b |
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Enantioselective Synthesis of (Z)- and (E)-2-Methyl-1,5-anti-Pentenediols via an Allene Hydroboration–Double-Allylboration Reaction Sequence Ming Chen and William R. Roush pp 9512–9517 DOI: 10.1021/ja4033633 Supporting Info |
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New Functional Handle for Use as a Self-Reporting Contrast and Delivery Agent in Nanomedicine Mathew P. Robin, Anne B. Mabire, Joanne C. Damborsky, Elizabeth S. Thom, Ursula H. Winzer-Serhan, Jeffery E. Raymond, and Rachel K. O’Reilly pp 9518–9524 DOI: 10.1021/ja403587c Supporting Info |
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Electron-Withdrawing Trifluoromethyl Groups in Combination with Hydrogen Bonds in Polyols: Brønsted Acids, Hydrogen-Bond Catalysts, and Anion Receptors Alireza Shokri, Xue-Bin Wang, and Steven R. Kass pp 9525–9530 DOI: 10.1021/ja4036384 Supporting Info |
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A Quasi-Quantum Well Sensitized Solar Cell with Accelerated Charge Separation and Collection Keyou Yan, Lixia Zhang, Jianhang Qiu, Yongcai Qiu, Zonglong Zhu, Jiannong Wang, and Shihe Yang pp 9531–9539 DOI: 10.1021/ja403756s Supporting Info |
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Boosting the Ambipolar Performance of Solution-Processable Polymer Semiconductors via Hybrid Side-Chain Engineering Junghoon Lee, A-Reum Han, Hojeong Yu, Tae Joo Shin, Changduk Yang, and Joon Hak Oh pp 9540–9547 DOI: 10.1021/ja403949g Supporting Info |
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A New Family of Nucleophiles for Photoinduced, Copper-Catalyzed Cross-Couplings via Single-Electron Transfer: Reactions of Thiols with Aryl Halides Under Mild Conditions (O °C) Christopher Uyeda, Yichen Tan, Gregory C. Fu, and Jonas C. Peters pp 9548–9552 DOI: 10.1021/ja404050f Supporting Info |
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Magnetocaloric Effect in AlFe2B2: Toward Magnetic Refrigerants from Earth-Abundant Elements Xiaoyan Tan, Ping Chai, Corey M. Thompson, and Michael Shatruk pp 9553–9557 DOI: 10.1021/ja404107p Supporting Info |
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Correction to Completely β-Selective Glycosylation Using 3,6-O-(o-Xylylene)-Bridged Axial-Rich Glucosyl Fluoride Yasunori Okada, Noriaki Asakura, Masafumi Bando, Yoshiki Ashikaga, and Hidetoshi Yamada pp 9558–9558 DOI: 10.1021/ja4050746 |
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Spotlights on Recent JACS Publications pp 9559–9559 DOI: 10.1021/ja406233h |
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A 13C Labeling Strategy Reveals a Range of Aromatic Side Chain Motion in Calmodulin Vignesh Kasinath, Kathleen G. Valentine, and A. Joshua Wand pp 9560–9563 DOI: 10.1021/ja4001129 Supporting Info |
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Singlet Oxygen Generation by the Genetically Encoded Tag miniSOG Rubén Ruiz-González, Aitziber L. Cortajarena, Sara H. Mejias, Montserrat Agut, Santi Nonell, and Cristina Flors pp 9564–9567 DOI: 10.1021/ja4020524 Supporting Info |
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Ligand-Stabilized Au13Cux (x = 2, 4, 8) Bimetallic Nanoclusters: Ligand Engineering to Control the Exposure of Metal Sites Huayan Yang, Yu Wang, Jing Lei, Lei Shi, Xiaohu Wu, Ville Mäkinen, Shuichao Lin, Zichao Tang, Jian He, Hannu Häkkinen, Lansun Zheng, and Nanfeng Zheng pp 9568–9571 DOI: 10.1021/ja402249s Supporting Info |
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Template-Free Synthesis of Hierarchical Porous Metal–Organic Frameworks Yanfeng Yue, Zhen-An Qiao, Pasquale F. Fulvio, Andrew J. Binder, Chengcheng Tian, Jihua Chen, Kimberly M. Nelson, Xiang Zhu, and Sheng Dai pp 9572–9575 DOI: 10.1021/ja402694f Supporting Info |
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Nanoemulsion Contrast Agents with Sub-picomolar Sensitivity for Xenon NMR Todd K. Stevens, R. Matthew Ramirez, and Alexander Pines pp 9576–9579 DOI: 10.1021/ja402885q Supporting Info |
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N–N Bond Cleavage of Mid-Valent Ta(IV) Hydrazido and Hydrazidium Complexes Relevant to the Schrock Cycle for Dinitrogen Fixation Andrew J. Keane, Peter Y. Zavalij, and Lawrence R. Sita pp 9580–9583 DOI: 10.1021/ja402804k Supporting Info |
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Direct Optical Determination of Interfacial Transport Barriers in Molecular Tunnel Junctions Jerry A. Fereiro, Richard L. McCreery, and Adam Johan Bergren pp 9584–9587 DOI: 10.1021/ja403123a Supporting Info |
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Anti-Markovnikov Hydroamination of Alkenes Catalyzed by an Organic Photoredox System Tien M. Nguyen and David A. Nicewicz pp 9588–9591 DOI: 10.1021/ja4031616 Supporting Info |
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Intermetallic NaAu2 as a Heterogeneous Catalyst for Low-Temperature CO Oxidation Chaoxian Xiao, Lin-Lin Wang, Raghu V. Maligal-Ganesh, Volodymyr Smetana, Holly Walen, Patricia A. Thiel, Gordon J. Miller, Duane D. Johnson, and Wenyu Huang pp 9592–9595 DOI: 10.1021/ja403175c Supporting Info |
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Fine-Tuning the Single-Molecule Magnet Properties of a [Dy(III)-Radical]2 Pair Elisabeth M. Fatila, Mathieu Rouzières, Michael C. Jennings, Alan J. Lough, Rodolphe Clérac, and Kathryn E. Preuss pp 9596–9599 DOI: 10.1021/ja403794d Supporting Info |
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Practical Selective Hydrogenation of α-Fluorinated Esters with Bifunctional Pincer-Type Ruthenium(II) Catalysts Leading to Fluorinated Alcohols or Fluoral Hemiacetals Takashi Otsuka, Akihiro Ishii, Pavel A. Dub, and Takao Ikariya pp 9600–9603 DOI: 10.1021/ja403852e Supporting Info |
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Co-Catalyzed Cross-Coupling of Alkyl Halides with Tertiary Alkyl Grignard Reagents Using a 1,3-Butadiene Additive Takanori Iwasaki, Hiroaki Takagawa, Surya P. Singh, Hitoshi Kuniyasu, and Nobuaki Kambe pp 9604–9607 DOI: 10.1021/ja404285b Supporting Info |
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Photoassisted Synthesis of Enantiopure Alkaloid Mimics Possessing Unprecedented Polyheterocyclic Cores N.N. Bhuvan Kumar, Olga A. Mukhina, and Andrei G. Kutateladze pp 9608–9611 DOI: 10.1021/ja4042109 Supporting Info |
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A Remote Lewis Acid Trigger Dramatically Accelerates Biaryl Reductive Elimination from a Platinum Complex Allegra L. Liberman-Martin, Robert G. Bergman, and T. Don Tilley pp 9612–9615 DOI: 10.1021/ja404339u Supporting Info |
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Asymmetric Silver “Nanocarrot” Structures: Solution Synthesis and Their Asymmetric Plasmonic Resonances Hongyan Liang, David Rossouw, Haiguang Zhao, Scott K. Cushing, Honglong Shi, Andreas Korinek, Hongxing Xu, Federico Rosei, Wenzhong Wang, Nianqiang Wu, Gianluigi A. Botton, and Dongling Ma pp 9616–9619 DOI: 10.1021/ja404345s Supporting Info |
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A Highly Chemoselective and Practical Alkynylation of Thiols Reto Frei and Jérôme Waser pp 9620–9623 DOI: 10.1021/ja4044196 Supporting Info |
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Spectral Tuning in Halorhodopsin: The Chloride Pump Photoreceptor Rhitankar Pal, Sivakumar Sekharan, and Victor S. Batista pp 9624–9627 DOI: 10.1021/ja404600z Supporting Info |
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Folding of a Linear Array of α-Amino Acids within a Helical Aromatic Oligoamide Frame Mayumi Kudo, Victor Maurizot, Brice Kauffmann, Aya Tanatani, and Ivan Huc pp 9628–9631 DOI: 10.1021/ja404656z Supporting Info |
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Storage of Hydrogen Spin Polarization in Long-Lived 13C2 Singlet Order and Implications for Hyperpolarized Magnetic Resonance Imaging Yesu Feng, Thomas Theis, Xiaofei Liang, Qiu Wang, Pei Zhou, and Warren S. Warren pp 9632–9635 DOI: 10.1021/ja404936p Supporting Info |
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Interception and Characterization of Alkyl and Acyl Complexes in Rhodium-Catalyzed Hydroformylation of Styrene Eleanor R. Nelsen and Clark R. Landis pp 9636–9639 DOI: 10.1021/ja404799m Supporting Info |
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G-Quadruplex DNA as a Molecular Target for Induced Synthetic Lethality in Cancer Cells Keith I. E. McLuckie, Marco Di Antonio, Heather Zecchini, Jian Xian, Carlos Caldas, Ben-Fillippo Krippendorff, David Tannahill, Christopher Lowe, and Shankar Balasubramanian pp 9640–9643 DOI: 10.1021/ja404868t Supporting Info |
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End-On Orientation of Semiconducting Polymers in Thin Films Induced by Surface Segregation of Fluoroalkyl Chains Jusha Ma, Kazuhito Hashimoto, Tomoyuki Koganezawa, and Keisuke Tajima pp 9644–9647 DOI: 10.1021/ja4051179 Supporting Info |
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The Length of the Calmodulin Linker Determines the Extent of Transient Interdomain Association and Target Affinity Nicholas J. Anthis and G. Marius Clore pp 9648–9651 DOI: 10.1021/ja4051422 Supporting Info |
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High Toughness, High Conductivity Ion Gels by Sequential Triblock Copolymer Self-Assembly and Chemical Cross-Linking Yuanyan Gu, Sipei Zhang, Luca Martinetti, Keun Hyung Lee, Lucas D. McIntosh, C. Daniel Frisbie, and Timothy P. Lodge pp 9652–9655 DOI: 10.1021/ja4051394 Supporting Info |
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Aldehydes and Ketones Form Intermediate π Complexes with the Gilman Reagent, Me2CuLi, at Low Temperatures in Tetrahydrofuran Steven H. Bertz, Richard A. Hardin, and Craig A. Ogle pp 9656–9658 DOI: 10.1021/ja404105u Supporting Info |
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Gold Nanorod@Chiral Mesoporous Silica Core–shell Nanoparticles with Unique Optical Properties Wenjing Liu, Zhening Zhu, Ke Deng, Zhengtao Li, Yunlong Zhou, Huibin Qiu, Yan Gao, Shunai Che, and Zhiyong Tang pp 9659–9664 DOI: 10.1021/ja312327m Supporting Info |
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Spectroscopic Studies of the Mononuclear Non-Heme FeII Enzyme FIH: Second-Sphere Contributions to Reactivity Kenneth M. Light, John A. Hangasky, Michael J. Knapp, and Edward I. Solomon pp 9665–9674 DOI: 10.1021/ja312571m Supporting Info |
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Discovery of Small-Molecule Modulators of the Sonic Hedgehog Pathway Giannina I. Schaefer, José R. Perez, Jeremy R. Duvall, Benjamin Z. Stanton, Alykhan F. Shamji, and Stuart L. Schreiber pp 9675–9680 DOI: 10.1021/ja400034k Supporting Info |
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Gas Phase Acidity Measurement of Local Acidic Groups in Multifunctional Species: Controlling the Binding Sites in Hydroxycinnamic Acids Andres Guerrero, Tomas Baer, Antonio Chana, Javier González, and Juan Z. Dávalos pp 9681–9690 DOI: 10.1021/ja400571r Supporting Info |
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Selective Nucleic Acid Capture with Shielded Covalent Probes Jeffrey R. Vieregg, Hosea M. Nelson, Brian M. Stoltz, and Niles A. Pierce pp 9691–9699 DOI: 10.1021/ja4009216 Supporting Info |
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Two Pathways for Electrocatalytic Oxidation of Hydrogen by a Nickel Bis(diphosphine) Complex with Pendant Amines in the Second Coordination Sphere Jenny Y. Yang, Stuart E. Smith, Tianbiao Liu, William G. Dougherty, Wesley A. Hoffert, W. Scott Kassel, M. Rakowski DuBois, Daniel L. DuBois, and R. Morris Bullock pp 9700–9712 DOI: 10.1021/ja400705a Supporting Info |
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Immunological Evaluation of a Synthetic Clostridium difficile Oligosaccharide Conjugate Vaccine Candidate and Identification of a Minimal Epitope Christopher E. Martin, Felix Broecker, Matthias A. Oberli, Julia Komor, Jochen Mattner, Chakkumkal Anish, and Peter H. Seeberger pp 9713–9722 DOI: 10.1021/ja401410y Supporting Info |
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Engineering Hydrophobic Protein–Carbohydrate Interactions to Fine-Tune Monoclonal Antibodies Xiaojie Yu, Kavitha Baruah, David J. Harvey, Snezana Vasiljevic, Dominic S. Alonzi, Byeong-Doo Song, Matthew K. Higgins, Thomas A. Bowden, Christopher N. Scanlan, and Max Crispin pp 9723–9732 DOI: 10.1021/ja4014375 Supporting Info |
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Toward a Lithium–“Air” Battery: The Effect of CO2 on the Chemistry of a Lithium–Oxygen Cell Hyung-Kyu Lim, Hee-Dae Lim, Kyu-Young Park, Dong-Hwa Seo, Hyeokjo Gwon, Jihyun Hong, William A. Goddard, III, Hyungjun Kim, and Kisuk Kang pp 9733–9742 DOI: 10.1021/ja4016765 Supporting Info |
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Thermodynamics of HIV-1 Reverse Transcriptase in Action Elucidates the Mechanism of Action of Non-Nucleoside Inhibitors Guillaume Bec, Benoit Meyer, Marie-Aline Gerard, Jessica Steger, Katja Fauster, Philippe Wolff, Dominique Burnouf, Ronald Micura, Philippe Dumas, and Eric Ennifar pp 9743–9752 DOI: 10.1021/ja4018418 Supporting Info |
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First-Principles Calculation of Dielectric Response in Molecule-Based Materials Henry M. Heitzer, Tobin J. Marks, and Mark A. Ratner pp 9753–9759 DOI: 10.1021/ja401904d Supporting Info |
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Specificity Profiling of Protein Phosphatases toward Phosphoseryl and Phosphothreonyl Peptides Qing Xiao, Rinrada Luechapanichkul, Yujing Zhai, and Dehua Pei pp 9760–9767 DOI: 10.1021/ja401692t Supporting Info |
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Divin: A Small Molecule Inhibitor of Bacterial Divisome Assembly Ye-Jin Eun, Maoquan Zhou, Daniela Kiekebusch, Susan Schlimpert, Rishi R. Trivedi, Somenath Bakshi, Zhou Zhong, Taylor A. Wahlig, Martin Thanbichler, and Douglas B. Weibel pp 9768–9776 DOI: 10.1021/ja404640f Supporting Info |
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Photoswitching Azo Compounds in Vivo with Red Light Subhas Samanta, Andrew A. Beharry, Oleg Sadovski, Theresa M. McCormick, Amirhossein Babalhavaeji, Vince Tropepe, and G. Andrew Woolley pp 9777–9784 DOI: 10.1021/ja402220t Supporting Info |
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Relative Stability of Different DNA Guanine Quadruplex Stem Topologies Derived Using Large-Scale Quantum-Chemical Computations Jiří Šponer, Arnošt Mládek, Naďa Špačková, Xiaohui Cang, Thomas E. Cheatham, III, and Stefan Grimme pp 9785–9796 DOI: 10.1021/ja402525c Supporting Info |
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Divergence between Organometallic and Single-Electron-Transfer Mechanisms in Copper(II)-Mediated Aerobic C–H Oxidation Alison M. Suess, Mehmed Z. Ertem, Christopher J. Cramer, and Shannon S. Stahl pp 9797–9804 DOI: 10.1021/ja4026424 Supporting Info |
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Glutathione-Triggered “Off–On” Release of Anticancer Drugs from Dendrimer-Encapsulated Gold Nanoparticles Xinyu Wang, Xiaopan Cai, Jingjing Hu, Naimin Shao, Fei Wang, Qiang Zhang, Jianru Xiao, and Yiyun Cheng pp 9805–9810 DOI: 10.1021/ja402903h Supporting Info |
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Surface-Induced Diastereomeric Complex Formation of a Nucleoside at the Liquid/Solid Interface: Stereoselective Recognition and Preferential Adsorption Zongxia Guo, Inge De Cat, Bernard Van Averbeke, Elke Ghijsens, Jianbin Lin, Hong Xu, Guojie Wang, Freek J. M. Hoeben, Željko Tomović, Roberto Lazzaroni, David Beljonne, E. W. Meijer, Albertus P. H. J. Schenning, and Steven De Feyter pp 9811–9819 DOI: 10.1021/ja402914m Supporting Info |
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Nanomolar E-Selectin Antagonists with Prolonged Half-Lives by a Fragment-Based Approach Jonas Egger, Céline Weckerle, Brian Cutting, Oliver Schwardt, Said Rabbani, Katrin Lemme, and Beat Ernst pp 9820–9828 DOI: 10.1021/ja4029582 Supporting Info |
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Improved Performances of Nanosilicon Electrodes Using the Salt LiFSI: A Photoelectron Spectroscopy Study Bertrand Philippe, Rémi Dedryvère, Mihaela Gorgoi, Håkan Rensmo, Danielle Gonbeau, and Kristina Edström pp 9829–9842 DOI: 10.1021/ja403082s Supporting Info |
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Real-Time Observation of the Formation of Excited Radical Ions in Bimolecular Photoinduced Charge Separation: Absence of the Marcus Inverted Region Explained Marius Koch, Arnulf Rosspeintner, Katrin Adamczyk, Bernhard Lang, Jens Dreyer, Erik T. J. Nibbering, and Eric Vauthey pp 9843–9848 DOI: 10.1021/ja403481v Supporting Info |
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N/S-Heterocyclic Contaminant Removal from Fuels by the Mesoporous Metal–Organic Framework MIL-100: The Role of the Metal Ion Ben Van de Voorde, Mohammed Boulhout, Frederik Vermoortele, Patricia Horcajada, Denise Cunha, Ji Sun Lee, Jong-San Chang, Emma Gibson, Marco Daturi, Jean-Claude Lavalley, Alexandre Vimont, Isabelle Beurroies, and Dirk E. De Vos pp 9849–9856 DOI: 10.1021/ja403571z Supporting Info |
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Completing the Series of +2 Ions for the Lanthanide Elements: Synthesis of Molecular Complexes of Pr2+, Gd2+, Tb2+, and Lu2+ Matthew R. MacDonald, Jefferson E. Bates, Joseph W. Ziller, Filipp Furche, and William J. Evans pp 9857–9868 DOI: 10.1021/ja403753j Supporting Info |
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A Cyanine-Modified Nanosystem for in Vivo Upconversion Luminescence Bioimaging of Methylmercury Yi Liu, Min Chen, Tianye Cao, Yun Sun, Chunyan Li, Qian Liu, Tianshe Yang, Liming Yao, Wei Feng, and Fuyou Li pp 9869–9876 DOI: 10.1021/ja403798m Supporting Info |
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Structural and Energetic Basis of Carbohydrate–Aromatic Packing Interactions in Proteins Wentao Chen, Sebastian Enck, Joshua L. Price, David L. Powers, Evan T. Powers, Chi-Huey Wong, H. Jane Dyson, and Jeffery W. Kelly pp 9877–9884 DOI: 10.1021/ja4040472 Supporting Info |
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Drug-Induced Conformational and Dynamical Changes of the S31N Mutant of the Influenza M2 Proton Channel Investigated by Solid-State NMR Jonathan K. Williams, Daniel Tietze, Jun Wang, Yibing Wu, William F. DeGrado, and Mei Hong pp 9885–9897 DOI: 10.1021/ja4041412 Supporting Info |
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AgNa(VO2F2)2: A Trioxovanadium Fluoride with Unconventional Electrochemical Properties Martin D. Donakowski, Arno Görne, John T. Vaughey, and Kenneth R. Poeppelmeier pp 9898–9906 DOI: 10.1021/ja404189t Supporting Info |
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Dephosphorylation of d-Peptide Derivatives to Form Biofunctional, Supramolecular Nanofibers/Hydrogels and Their Potential Applications for Intracellular Imaging and Intratumoral Chemotherapy Jiayang Li, Yuan Gao, Yi Kuang, Junfeng Shi, Xuewen Du, Jie Zhou, Huaimin Wang, Zhimou Yang, and Bing Xu pp 9907–9914 DOI: 10.1021/ja404215g Supporting Info |
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A Ratiometric Two-Photon Fluorescent Probe Reveals Reduction in Mitochondrial H2S Production in Parkinson’s Disease Gene Knockout Astrocytes Sung Keun Bae, Cheol Ho Heo, Dong Joo Choi, Debabrata Sen, Eun-Hye Joe, Bong Rae Cho, and Hwan Myung Kim pp 9915–9923 DOI: 10.1021/ja404004v Supporting Info |
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Toward Directionally Controlled Molecular Motions and Kinetic Intra- and Intermolecular Self-Sorting: Threading Processes of Nonsymmetric Wheel and Axle Components Arturo Arduini, Rocco Bussolati, Alberto Credi, Andrea Secchi, Serena Silvi, Monica Semeraro, and Margherita Venturi pp 9924–9930 DOI: 10.1021/ja404270c Supporting Info |
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A Study of Dinitro-bis-1,2,4-triazole-1,1′-diol and Derivatives: Design of High-Performance Insensitive Energetic Materials by the Introduction of N-Oxides Alexander A. Dippold and Thomas M. Klapötke pp 9931–9938 DOI: 10.1021/ja404164j Supporting Info |
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AAAA-DDDD Quadruple Hydrogen-Bond Arrays Featuring NH···N and CH···N Hydrogen Bonds David A. Leigh, Craig C. Robertson, Alexandra M. Z. Slawin, and Patrick I. T. Thomson pp 9939–9943 DOI: 10.1021/ja404504m Supporting Info |
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A Highly Specific Fluorescent Probe for Hypochlorous Acid and Its Application in Imaging Microbe-Induced HOCl Production Qingling Xu, Kyung-Ah Lee, Songyi Lee, Kyung Mi Lee, Won-Jae Lee, and Juyoung Yoon pp 9944–9949 DOI: 10.1021/ja404649m Supporting Info |
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Retraction of “Cooperative Melting in Caged Dimers of Rigid Small Molecule-DNA Hybrids” Brian R. Stepp, Julianne M. Gibbs-Davis, Dorothea L. F. Koh, and SonBinh T. Nguyen pp 9950–9950 DOI: 10.1021/ja403724b |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 9951–9951 DOI: 10.1021/ja406272c |
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Crystal Engineering: From Molecule to Crystal Gautam R. Desiraju pp 9952–9967 DOI: 10.1021/ja403264c |
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N,C-Capped Dipeptides with Selectivity for Mycobacterial Proteasome over Human Proteasomes: Role of S3 and S1 Binding Pockets Gang Lin, Tamutenda Chidawanyika, Christopher Tsu, Thulasi Warrier, Julien Vaubourgeix, Christopher Blackburn, Kenneth Gigstad, Michael Sintchak, Lawrence Dick, and Carl Nathan pp 9968–9971 DOI: 10.1021/ja400021x Supporting Info |
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Liquid Crystal-Based Emulsions for Synthesis of Spherical and Non-Spherical Particles with Chemical Patches Frédéric Mondiot, Xiaoguang Wang, Juan J. de Pablo, and Nicholas L. Abbott pp 9972–9975 DOI: 10.1021/ja4022182 Supporting Info |
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Electrostatic Modulation of Aromatic Rings via Explicit Solvation of Substituents Kamila B. Muchowska, Catherine Adam, Ioulia K. Mati, and Scott L. Cockroft pp 9976–9979 DOI: 10.1021/ja402566w Supporting Info |
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Mutational Analysis of 48G7 Reveals that Somatic Hypermutation Affects Both Antibody Stability and Binding Affinity Sophie B. Sun, Shiladitya Sen, Nam-Jung Kim, Thomas J. Magliery, Peter G. Schultz, and Feng Wang pp 9980–9983 DOI: 10.1021/ja402927u Supporting Info |
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Design and Preparation of a Core–Shell Metal–Organic Framework for Selective CO2 Capture Tao Li, Jeanne E. Sullivan, and Nathaniel L. Rosi pp 9984–9987 DOI: 10.1021/ja403008j Supporting Info |
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Aluminum–Ligand Cooperative N–H Bond Activation and an Example of Dehydrogenative Coupling Thomas W. Myers and Louise A. Berben pp 9988–9990 DOI: 10.1021/ja4032874 Supporting Info |
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Importance of Acid–Base Equilibrium in Electrocatalytic Oxidation of Formic Acid on Platinum Jiyong Joo, Taro Uchida, Angel Cuesta, Marc T. M. Koper, and Masatoshi Osawa pp 9991–9994 DOI: 10.1021/ja403578s Supporting Info |
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Large-Scale Synthesis of Transition-Metal-Doped TiO2 Nanowires with Controllable Overpotential Bin Liu, Hao Ming Chen, Chong Liu, Sean C. Andrews, Chris Hahn, and Peidong Yang pp 9995–9998 DOI: 10.1021/ja403761s Supporting Info |
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Stereodirection of an α-Ketoester at Sub-molecular Sites on Chirally Modified Pt(111): Heterogeneous Asymmetric Catalysis Vincent Demers-Carpentier, Anton M. H. Rasmussen, Guillaume Goubert, Lara Ferrighi, Yi Dong, Jean-Christian Lemay, Federico Masini, Yang Zeng, Bjørk Hammer, and Peter H. McBreen pp 9999–10002 DOI: 10.1021/ja403955k Supporting Info |
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Revisiting the Chemistry of the Actinocenes [(η8-C8H8)2An] (An = U, Th) with Neutral Lewis Bases. Access to the Bent Sandwich Complexes [(η8-C8H8)2An(L)] with Thorium (L = py, 4,4′-bipy, tBuNC, R4phen) Jean-Claude Berthet, Pierre Thuéry, Nicolas Garin, Jean-Pierre Dognon, Thibault Cantat, and Michel Ephritikhine pp 10003–10006 DOI: 10.1021/ja4036626 Supporting Info |
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Dodecaamide Cages: Organic 12-Arm Building Blocks for Supramolecular Chemistry Jamie L. Culshaw, Ge Cheng, Marc Schmidtmann, Tom Hasell, Ming Liu, Dave J. Adams, and Andrew I. Cooper pp 10007–10010 DOI: 10.1021/ja403987j Supporting Info |
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Chiral Structure of Thiolate-Protected 28-Gold-Atom Nanocluster Determined by X-ray Crystallography Chenjie Zeng, Tao Li, Anindita Das, Nathaniel L. Rosi, and Rongchao Jin pp 10011–10013 DOI: 10.1021/ja404058q Supporting Info |
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Development of a High-Throughput Screen and Its Use in the Discovery of Streptococcus pneumoniae Immunoglobulin A1 Protease Inhibitors Amanda L. Garner, Jessica L. Fullagar, Joshua A. Day, Seth M. Cohen, and Kim D. Janda pp 10014–10017 DOI: 10.1021/ja404180x Supporting Info |
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Self-Assembled Containers Based on Extended Tetrathiafulvalene Sébastien Bivaud, Sébastien Goeb, Vincent Croué, Paul I. Dron, Magali Allain, and Marc Sallé pp 10018–10021 DOI: 10.1021/ja404072w Supporting Info |
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Catalytic Ketyl-Olefin Cyclizations Enabled by Proton-Coupled Electron Transfer Kyle T. Tarantino, Peng Liu, and Robert R. Knowles pp 10022–10025 DOI: 10.1021/ja404342j Supporting Info |
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Organocatalytic Oxyamination of Azlactones: Kinetic Resolution of Oxaziridines and Asymmetric Synthesis of Oxazolin-4-ones Shunxi Dong, Xiaohua Liu, Yin Zhu, Peng He, Lili Lin, and Xiaoming Feng pp 10026–10029 DOI: 10.1021/ja404379n Supporting Info |
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Self-Sufficient and Exclusive Oxygenation of Methane and Its Source Materials with Oxygen to Methanol via Metgas Using Oxidative Bi-reforming George A. Olah, G. K. Surya Prakash, Alain Goeppert, Miklos Czaun, and Thomas Mathew pp 10030–10031 DOI: 10.1021/ja405439c |
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Synthesis of Highly Cis, Syndiotactic Polymers via Ring-Opening Metathesis Polymerization Using Ruthenium Metathesis Catalysts Lauren E. Rosebrugh, Vanessa M. Marx, Benjamin K. Keitz, and Robert H. Grubbs pp 10032–10035 DOI: 10.1021/ja405559y Supporting Info |
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Catalytic Epoxidation Activity of Keplerate Polyoxomolybdate Nanoball toward Aqueous Suspension of Olefins under Mild Aerobic Conditions Abdolreza Rezaeifard, Reza Haddad, Maasoumeh Jafarpour, and Mohammad Hakimi pp 10036–10039 DOI: 10.1021/ja405852s Supporting Info |
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Molecular Crowding Enhanced ATPase Activity of the RNA Helicase eIF4A Correlates with Compaction of Its Quaternary Structure and Association with eIF4G Sabine R. Akabayov, Barak Akabayov, Charles C. Richardson, and Gerhard Wagner pp 10040–10047 DOI: 10.1021/ja404404h Supporting Info |
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Theoretical Prediction and Experimental Realization of New Stable Inorganic Materials Using the Inverse Design Approach Andriy Zakutayev, Xiuwen Zhang, Arpun Nagaraja, Liping Yu, Stephan Lany, Thomas O. Mason, David S. Ginley, and Alex Zunger pp 10048–10054 DOI: 10.1021/ja311599g Supporting Info |
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Crowders Perturb the Entropy of RNA Energy Landscapes to Favor Folding Duncan Kilburn, Joon Ho Roh, Reza Behrouzi, Robert M. Briber, and Sarah A. Woodson pp 10055–10063 DOI: 10.1021/ja4030098 Supporting Info |
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Energy-Level Matching of Fe(III) Ions Grafted at Surface and Doped in Bulk for Efficient Visible-Light Photocatalysts Min Liu, Xiaoqing Qiu, Masahiro Miyauchi, and Kazuhito Hashimoto pp 10064–10072 DOI: 10.1021/ja401541k Supporting Info |
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Graphene Nanoelectrodes: Fabrication and Size-Dependent Electrochemistry Bo Zhang, Lixin Fan, Huawei Zhong, Yuwen Liu, and Shengli Chen pp 10073–10080 DOI: 10.1021/ja402456b Supporting Info |
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Heck Coupling of Olefins to Mixed Methyl/Thienyl Monolayers on Si(111) Surfaces Leslie E. O’Leary, Michael J. Rose, Tina X. Ding, Erik Johansson, Bruce S. Brunschwig, and Nathan S. Lewis pp 10081–10090 DOI: 10.1021/ja402495e Supporting Info |
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Insight into Magnetite’s Redox Catalysis from Observing Surface Morphology during Oxidation Shu Nie, Elena Starodub, Matteo Monti, David A. Siegel, Lucía Vergara, Farid El Gabaly, Norman C. Bartelt, Juan de la Figuera, and Kevin F. McCarty pp 10091–10098 DOI: 10.1021/ja402599t Supporting Info |
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Screening for Enhanced Triacetic Acid Lactone Production by Recombinant Escherichia coli Expressing a Designed Triacetic Acid Lactone Reporter Shuang-Yan Tang, Shuai Qian, Olubolaji Akinterinwa, Christopher S. Frei, Joseph A. Gredell, and Patrick C. Cirino pp 10099–10103 DOI: 10.1021/ja402654z Supporting Info |
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Solvent-Dependent Switch of Helical Main-Chain Chirality in Sergeants-and-Soldiers-Type Poly(quinoxaline-2,3-diyl)s: Effect of the Position and Structures of the “Sergeant” Chiral Units on the Screw-Sense Induction Yuuya Nagata, Tetsuya Yamada, Takumi Adachi, Yuto Akai, Takeshi Yamamoto, and Michinori Suginome pp 10104–10113 DOI: 10.1021/ja403391m Supporting Info |
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Single Sublattice Endotaxial Phase Separation Driven by Charge Frustration in a Complex Oxide Antoine Demont, Ruth Sayers, Maria A. Tsiamtsouri, Simon Romani, Philip A. Chater, Hongjun Niu, Carlos Martí-Gastaldo, Zhongling Xu, Zengqiang Deng, Yohann Bréard, Michael F. Thomas, John B. Claridge, and Matthew J. Rosseinsky pp 10114–10123 DOI: 10.1021/ja403611s Supporting Info |
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Highly Stable, Anion Conductive, Comb-Shaped Copolymers for Alkaline Fuel Cells Nanwen Li, Yongjun Leng, Michael A. Hickner, and Chao-Yang Wang pp 10124–10133 DOI: 10.1021/ja403671u |
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Dispersion Forces and Counterintuitive Steric Effects in Main Group Molecules: Heavier Group 14 (Si–Pb) Dichalcogenolate Carbene Analogues with Sub-90° Interligand Bond Angles Brian D. Rekken, Thomas M. Brown, James C. Fettinger, Felicitas Lips, Heikki M. Tuononen, Rolfe H. Herber, and Philip P. Power pp 10134–10148 DOI: 10.1021/ja403802a Supporting Info |
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Monoclinic Sr1–xNaxSiO3–0.5x: New Superior Oxide Ion Electrolytes Preetam Singh and John B. Goodenough pp 10149–10154 DOI: 10.1021/ja4042737 Supporting Info |
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Modulation of the Intrinsic Helix Propensity of an Intrinsically Disordered Protein Reveals Long-Range Helix–Helix Interactions Vytautas Iešmantavičius, Malene Ringkjøbing Jensen, Valéry Ozenne, Martin Blackledge, Flemming M. Poulsen, and Magnus Kjaergaard pp 10155–10163 DOI: 10.1021/ja4045532 Supporting Info |
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Isolation and First Total Synthesis of PM050489 and PM060184, Two New Marine Anticancer Compounds María Jesús Martín, Laura Coello, Rogelio Fernández, Fernando Reyes, Alberto Rodríguez, Carmen Murcia, María Garranzo, Cristina Mateo, Francisco Sánchez-Sancho, Santiago Bueno, Carlos de Eguilior, Andrés Francesch, Simon Munt, and Carmen Cuevas pp 10164–10171 DOI: 10.1021/ja404578u Supporting Info |
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Modulation of In-Membrane Receptor Clustering upon Binding of Multivalent Ligands Anna Grochmal, Elena Ferrero, Lilia Milanesi, and Salvador Tomas pp 10172–10177 DOI: 10.1021/ja404428u Supporting Info |
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Correction to “Design and Characterization of 1D Nanotubes and 2D Periodic Arrays Self-Assembled from DNA Multi-Helix Bundles” Tong Wang, Daniel Schiffels, Sergio Martinez Cuesta, Deborah Kuchnir Fygenson, and Nadrian C. Seeman pp 10178–10178 DOI: 10.1021/ja403136h Supporting Info |
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Correction to “Better Cycling Performances of Bulk Sb in Na-Ion Batteries Compared to Li-Ion Systems: An Unexpected Electrochemical Mechanism” Ali Darwiche, Cyril Marino, Moulay T. Sougrati, Bernard Fraisse, Lorenzo Stievano, and Laure Monconduit pp 10179–10179 DOI: 10.1021/ja4056195 |
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Correction to “Enhanced Electron-Transfer Reactivity of Nonheme Manganese(IV)–Oxo Complexes by Binding Scandium Ions” Heejung Yoon, Yong-Min Lee, Xiujuan Wu, Kyung-Bin Cho, Ritimukta Sarangi, Wonwoo Nam, and Shunichi Fukuzumi pp 10180–10180 DOI: 10.1021/ja4065014 |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 10181–10182 DOI: 10.1021/ja406852u |
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Highly Z-Selective and Enantioselective Ring-Opening/Cross-Metathesis Catalyzed by a Resolved Stereogenic-at-Ru Complex John Hartung and Robert H. Grubbs pp 10183–10185 DOI: 10.1021/ja4046422 Supporting Info |
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Engineering Chiral Polyoxometalate Hybrid Metal–Organic Frameworks for Asymmetric Dihydroxylation of Olefins Qiuxia Han, Cheng He, Min Zhao, Bo Qi, Jingyang Niu, and Chunying Duan pp 10186–10189 DOI: 10.1021/ja401758c Supporting Info |
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Dual-Stimulus Luminescent Lanthanide Molecular Switch Based on an Unsymmetrical Diarylperfluorocyclopentene Hong-Bo Cheng, Heng-Yi Zhang, and Yu Liu pp 10190–10193 DOI: 10.1021/ja4018804 Supporting Info |
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Computational Evidence for Heavy-Atom Tunneling in the Bergman Cyclization of a 10-Membered-Ring Enediyne Edyta M. Greer, Christopher V. Cosgriff, and Charles Doubleday pp 10194–10197 DOI: 10.1021/ja402445a Supporting Info |
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Sc3+-Triggered Oxoiron(IV) Formation from O2 and its Non-Heme Iron(II) Precursor via a Sc3+–Peroxo–Fe3+ Intermediate Feifei Li, Katherine M. Van Heuvelen, Katlyn K. Meier, Eckard Münck, and Lawrence Que, Jr. pp 10198–10201 DOI: 10.1021/ja402645y Supporting Info |
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Crystal Structure of a Human Prion Protein Fragment Reveals a Motif for Oligomer Formation Marcin I. Apostol, Kay Perry, and Witold K. Surewicz pp 10202–10205 DOI: 10.1021/ja403001q Supporting Info |
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Molecular Hydrogen Formation from Photocatalysis of Methanol on TiO2(110) Chenbiao Xu, Wenshao Yang, Qing Guo, Dongxu Dai, Maodu Chen, and Xueming Yang pp 10206–10209 DOI: 10.1021/ja4030963 Supporting Info |
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Immobilizing Metal Nanoparticles to Metal–Organic Frameworks with Size and Location Control for Optimizing Catalytic Performance Qi-Long Zhu, Jun Li, and Qiang Xu pp 10210–10213 DOI: 10.1021/ja403330m Supporting Info |
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Ferroelectric Switchable Behavior through Fast Reversible De/adsorption of Water Spirals in a Chiral 3D Metal–Organic Framework Xi-Yan Dong, Bo Li, Bin-Bin Ma, Shi-Jun Li, Ming-Ming Dong, Yan-Yan Zhu, Shuang-Quan Zang, You Song, Hong-Wei Hou, and Thomas. C. W. Mak pp 10214–10217 DOI: 10.1021/ja403449k Supporting Info |
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Direct Observation of Large Quantum Interference Effect in Anthraquinone Solid-State Junctions Vincent Rabache, Julien Chaste, Philippe Petit, Maria Luisa Della Rocca, Pascal Martin, Jean-Christophe Lacroix, Richard L. McCreery, and Philippe Lafarge pp 10218–10221 DOI: 10.1021/ja403577u Supporting Info |
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Pd-Catalyzed Cascade Crossover Annulation of o-Alkynylarylhalides and Diarylacetylenes Leading to Dibenzo[a,e]pentalenes Jian Zhao, Kazuaki Oniwa, Naoki Asao, Yoshinori Yamamoto, and Tienan Jin pp 10222–10225 DOI: 10.1021/ja403382d Supporting Info |
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GFP Variants with Alternative β-Strands and Their Application as Light-driven Protease Sensors: A Tale of Two Tails Keunbong Do and Steven G. Boxer pp 10226–10229 DOI: 10.1021/ja4037274 Supporting Info |
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An All-Photonic Molecule-Based Parity Generator/Checker for Error Detection in Data Transmission Magnus Bälter, Shiming Li, Jesper R. Nilsson, Joakim Andréasson, and Uwe Pischel pp 10230–10233 DOI: 10.1021/ja403828z Supporting Info |
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Synthesis and Integration of Fe-soc-MOF Cubes into Colloidosomes via a Single-Step Emulsion-Based Approach Maolin Pang, Amy J. Cairns, Yunling Liu, Youssef Belmabkhout, Hua Chun Zeng, and Mohamed Eddaoudi pp 10234–10237 DOI: 10.1021/ja403994u Supporting Info |
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Fabrication of an Efficient BaTaO2N Photoanode Harvesting a Wide Range of Visible Light for Water Splitting Masanobu Higashi, Kazunari Domen, and Ryu Abe pp 10238–10241 DOI: 10.1021/ja404030x Supporting Info |
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Photoelectrochemical Properties of (In,Ga)N Nanowires for Water Splitting Investigated by in Situ Electrochemical Mass Spectroscopy Jumpei Kamimura, Peter Bogdanoff, Jonas Lähnemann, Christian Hauswald, Lutz Geelhaar, Sebastian Fiechter, and Henning Riechert pp 10242–10245 DOI: 10.1021/ja404043k Supporting Info |
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Aryl Nitrene Rearrangements: Spectroscopic Observation of a Benzazirine and Its Ring Expansion to a Ketenimine by Heavy-Atom Tunneling Hiroshi Inui, Kazuhiro Sawada, Shigero Oishi, Kiminori Ushida, and Robert J. McMahon pp 10246–10249 DOI: 10.1021/ja404172s Supporting Info |
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Monocopper Doping in Cd-In-S Supertetrahedral Nanocluster via Two-Step Strategy and Enhanced Photoelectric Response Tao Wu, Qian Zhang, Yang Hou, Le Wang, Chengyu Mao, Shou-Tian Zheng, Xianhui Bu, and Pingyun Feng pp 10250–10253 DOI: 10.1021/ja404181c Supporting Info |
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Real-Time Observation of Multiple-Protein Complex Formation with Single-Molecule FRET Woori Bae, Mal-Gi Choi, Changbong Hyeon, Yeon-Kyun Shin, and Tae-Young Yoon pp 10254–10257 DOI: 10.1021/ja404276g Supporting Info |
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Readily Accessible and Easily Modifiable Ru-Based Catalysts for Efficient and Z-Selective Ring-Opening Metathesis Polymerization and Ring-Opening/Cross-Metathesis R. Kashif M. Khan, Sebastian Torker, and Amir H. Hoveyda pp 10258–10261 DOI: 10.1021/ja404208a Supporting Info |
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Structural Transitions in Nanoparticle Assemblies Governed by Competing Nanoscale Forces Rachelle M. Choueiri, Anna Klinkova, Héloı̈se Thérien-Aubin, Michael Rubinstein, and Eugenia Kumacheva pp 10262–10265 DOI: 10.1021/ja404341r Supporting Info |
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Pruning the ALS-Associated Protein SOD1 for in-Cell NMR Jens Danielsson, Kohsuke Inomata, Shuhei Murayama, Hidehito Tochio, Lisa Lang, Masahiro Shirakawa, and Mikael Oliveberg pp 10266–10269 DOI: 10.1021/ja404425r Supporting Info |
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Entrapment of Metal Clusters in Metal–Organic Framework Channels by Extended Hooks Anchored at Open Metal Sites Shou-Tian Zheng, Xiang Zhao, Samuel Lau, Addis Fuhr, Pingyun Feng, and Xianhui Bu pp 10270–10273 DOI: 10.1021/ja4044642 Supporting Info |
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Enhanced Hydrogen Evolution Catalysis from Chemically Exfoliated Metallic MoS2 Nanosheets Mark A. Lukowski, Andrew S. Daniel, Fei Meng, Audrey Forticaux, Linsen Li, and Song Jin pp 10274–10277 DOI: 10.1021/ja404523s Supporting Info |
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Controlling Self-Assembly of a Peptide-Based Material via Metal-Ion Induced Registry Shift Paolo Anzini, Chunfu Xu, Spencer Hughes, Elizabeth Magnotti, Tao Jiang, Lars Hemmingsen, Borries Demeler, and Vincent P. Conticello pp 10278–10281 DOI: 10.1021/ja404677c Supporting Info |
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Design of a Dynamic Polymer Interface for Chiral Discrimination Atsuomi Shundo, Koichiro Hori, Takuya Ikeda, Nobuo Kimizuka, and Keiji Tanaka pp 10282–10285 DOI: 10.1021/ja404701s Supporting Info |
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Solar Hydrogen Generation by Nanoscale p–n Junction of p-type Molybdenum Disulfide/n-type Nitrogen-Doped Reduced Graphene Oxide Fanke Meng, Jiangtian Li, Scott K. Cushing, Mingjia Zhi, and Nianqiang Wu pp 10286–10289 DOI: 10.1021/ja404851s Supporting Info |
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Ultrafast Excited-State Dynamics in Hexaethyleneglycol-Linked DNA Homoduplexes Made of A·T Base Pairs Jinquan Chen, Arun K. Thazhathveetil, Frederick D. Lewis, and Bern Kohler pp 10290–10293 DOI: 10.1021/ja4049459 Supporting Info |
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Vapor-Phase Metalation by Atomic Layer Deposition in a Metal–Organic Framework Joseph E. Mondloch, Wojciech Bury, David Fairen-Jimenez, Stephanie Kwon, Erica J. DeMarco, Mitchell H. Weston, Amy A. Sarjeant, SonBinh T. Nguyen, Peter C. Stair, Randall Q. Snurr, Omar K. Farha, and Joseph T. Hupp pp 10294–10297 DOI: 10.1021/ja4050828 Supporting Info |
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Silane–Isocyanide Coupling Involving 1,1-Insertion of XylNC into the Si–H Bond of a σ-Silane Ligand Mark C. Lipke and T. Don Tilley pp 10298–10301 DOI: 10.1021/ja404910h Supporting Info |
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Upgrading Light Hydrocarbons via Tandem Catalysis: A Dual Homogeneous Ta/Ir System for Alkane/Alkene Coupling David C. Leitch, Yan Choi Lam, Jay A. Labinger, and John E. Bercaw pp 10302–10305 DOI: 10.1021/ja405191a Supporting Info |
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Hydroalkoxylation of Unactivated Olefins with Carbon Radicals and Carbocation Species as Key Intermediates Hiroki Shigehisa, Tatsuya Aoki, Sumiko Yamaguchi, Nao Shimizu, and Kou Hiroya pp 10306–10309 DOI: 10.1021/ja405219f Supporting Info |
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A Sugar-Functionalized Amphiphilic Pillar[5]arene: Synthesis, Self-Assembly in Water, and Application in Bacterial Cell Agglutination Guocan Yu, Yingjie Ma, Chengyou Han, Yong Yao, Guping Tang, Zhengwei Mao, Changyou Gao, and Feihe Huang pp 10310–10313 DOI: 10.1021/ja405237q Supporting Info |
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Highly Sensitive SERS Quantification of the Oncogenic Protein c-Jun in Cellular Extracts Luca Guerrini, Elena Pazos, Cristina Penas, M. Eugenio Vázquez, Jose Luis Mascareñas, and Ramon A. Alvarez-Puebla pp 10314–10317 DOI: 10.1021/ja405120x Supporting Info |
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Reaction Products and the X-ray Structure of AmpDh2, a Virulence Determinant of Pseudomonas aeruginosa Siseth Martínez-Caballero, Mijoon Lee, Cecilia Artola-Recolons, César Carrasco-López, Dusan Hesek, Edward Spink, Elena Lastochkin, Weilie Zhang, Lance M. Hellman, Bill Boggess, Shahriar Mobashery, and Juan A. Hermoso pp 10318–10321 DOI: 10.1021/ja405464b Supporting Info |
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Distinct Responses to Mechanical Grinding and Hydrostatic Pressure in Luminescent Chromism of Tetrathiazolylthiophene Kazuhiko Nagura, Shohei Saito, Hitoshi Yusa, Hiroshi Yamawaki, Hiroshi Fujihisa, Hiroyasu Sato, Yuichi Shimoikeda, and Shigehiro Yamaguchi pp 10322–10325 DOI: 10.1021/ja4055228 Supporting Info |
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Pd(II)-Catalyzed C–H Iodination Using Molecular I2 as the Sole Oxidant Xiao-Chen Wang, Yi Hu, Samuel Bonacorsi, Yang Hong, Richard Burrell, and Jin-Quan Yu pp 10326–10329 DOI: 10.1021/ja4055492 Supporting Info |
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Silver-Mediated Trifluoromethylation of Aryldiazonium Salts: Conversion of Amino Group into Trifluoromethyl Group Xi Wang, Yan Xu, Fanyang Mo, Guojing Ji, Di Qiu, Jiajie Feng, Yuxuan Ye, Songnan Zhang, Yan Zhang, and Jianbo Wang pp 10330–10333 DOI: 10.1021/ja4056239 Supporting Info |
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Direct Catalytic Anti-Markovnikov Addition of Carboxylic Acids to Alkenes Andrew J. Perkowski and David A. Nicewicz pp 10334–10337 DOI: 10.1021/ja4057294 Supporting Info |
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Catalytic Asymmetric Hydrophosphonylation of Ketimines Liang Yin, Youmei Bao, Naoya Kumagai, and Masakatsu Shibasaki pp 10338–10341 DOI: 10.1021/ja4059316 Supporting Info |
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Dynamically Interchangeable Nanoparticle Superlattices Through the Use of Nucleic Acid-Based Allosteric Effectors Youngeun Kim, Robert J. Macfarlane, and Chad A. Mirkin pp 10342–10345 DOI: 10.1021/ja405988r Supporting Info |
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Reduction of Fluorinated Cyclopropene by Nitrogenase Feng Ni, Chi Chung Lee, Candy S. Hwang, Yilin Hu, Markus W. Ribbe, and Charles E. McKenna pp 10346–10352 DOI: 10.1021/ja3121058 Supporting Info |
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Dibenzosilanorbornadienyl Cations and Their Fragmentation into Silyliumylidenes Claudia Gerdes, Wolfgang Saak, Detlev Haase, and Thomas Müller pp 10353–10361 DOI: 10.1021/ja400306h Supporting Info |
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A General Method for Fluorescent Labeling of the N-Termini of Lanthipeptides and Its Application to Visualize their Cellular Localization Noah A. Bindman and Wilfred A. van der Donk pp 10362–10371 DOI: 10.1021/ja4010706 Supporting Info |
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Blending Through-Space and Through-Bond π–π-Coupling in [2,2′]-Paracyclophane-oligophenylenevinylene Molecular Wires Mateusz Wielopolski, Agustín Molina-Ontoria, Christina Schubert, Johannes T. Margraf, Evangelos Krokos, Johannes Kirschner, Andreas Gouloumis, Timothy Clark, Dirk M. Guldi, and Nazario Martín pp 10372–10381 DOI: 10.1021/ja401239r Supporting Info |
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Symmetry Break of Special Pair: Photochemically Induced Dynamic Nuclear Polarization NMR Confirms Control by Nonaromatic Substituents Karthick Babu Sai Sankar Gupta, A. Alia, Huub J.M. de Groot, and Jörg Matysik pp 10382–10387 DOI: 10.1021/ja402238w Supporting Info |
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Amphidynamic Crystals of a Steroidal Bicyclo[2.2.2]octane Rotor: A High Symmetry Group That Rotates Faster than Smaller Methyl and Methoxy Groups Braulio Rodríguez-Molina, Salvador Pérez-Estrada, and Miguel A. Garcia-Garibay pp 10388–10395 DOI: 10.1021/ja4024463 Supporting Info |
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Ascorbic Acid Enhances Tet-Mediated 5-Methylcytosine Oxidation and Promotes DNA Demethylation in Mammals Ruichuan Yin, Shi-Qing Mao, Bailin Zhao, Zechen Chong, Ying Yang, Chao Zhao, Dapeng Zhang, Hua Huang, Juan Gao, Zheng Li, Yan Jiao, Cuiping Li, Shengquan Liu, Danni Wu, Weikuan Gu, Yun-Gui Yang, Guo-Liang Xu, and Hailin Wang pp 10396–10403 DOI: 10.1021/ja4028346 Supporting Info |
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A Mechanistic Hypothesis for the Aspirin-Induced Switch in Lipid Mediator Production by Cyclooxygenase-2 Paolo Tosco pp 10404–10410 DOI: 10.1021/ja402870k Supporting Info |
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Vacancy Associates Promoting Solar-Driven Photocatalytic Activity of Ultrathin Bismuth Oxychloride Nanosheets Meili Guan, Chong Xiao, Jie Zhang, Shaojuan Fan, Ran An, Qingmei Cheng, Junfeng Xie, Min Zhou, Bangjiao Ye, and Yi Xie pp 10411–10417 DOI: 10.1021/ja402956f Supporting Info |
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A Cyclic Peptide Inhibitor of HIF-1 Heterodimerization That Inhibits Hypoxia Signaling in Cancer Cells Elena Miranda, Ida K. Nordgren, Abigail L. Male, Charlotte E. Lawrence, Franciane Hoakwie, Francesco Cuda, William Court, Keith R. Fox, Paul A. Townsend, Graham K. Packham, Suzanne A. Eccles, and Ali Tavassoli pp 10418–10425 DOI: 10.1021/ja402993u Supporting Info |
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Enzymatic Neutralization of the Chemical Warfare Agent VX: Evolution of Phosphotriesterase for Phosphorothiolate Hydrolysis Andrew N. Bigley, Chengfu Xu, Terry J. Henderson, Steven P. Harvey, and Frank M. Raushel pp 10426–10432 DOI: 10.1021/ja402832z Supporting Info |
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Structural and Thermodynamic Basis of (+)-α-Pinene Binding to Human Cytochrome P450 2B6 P. Ross Wilderman, Manish B. Shah, Hyun-Hee Jang, C. David Stout, and James R. Halpert pp 10433–10440 DOI: 10.1021/ja403042k Supporting Info |
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Post-synthetic Structural Processing in a Metal–Organic Framework Material as a Mechanism for Exceptional CO2/N2 Selectivity Witold M. Bloch, Ravichandar Babarao, Matthew R. Hill, Christian J. Doonan, and Christopher J. Sumby pp 10441–10448 DOI: 10.1021/ja4032049 Supporting Info |
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Proteomics Guided Discovery of Flavopeptins: Anti-proliferative Aldehydes Synthesized by a Reductase Domain-Containing Non-ribosomal Peptide Synthetase Yunqiu Chen, Ryan A. McClure, Yupeng Zheng, Regan J. Thomson, and Neil L. Kelleher pp 10449–10456 DOI: 10.1021/ja4031193 Supporting Info |
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Stabilization of Different Types of Transition States in a Single Enzyme Active Site: QM/MM Analysis of Enzymes in the Alkaline Phosphatase Superfamily Guanhua Hou and Qiang Cui pp 10457–10469 DOI: 10.1021/ja403293d Supporting Info |
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On-Surface Synthesis of Single-Layered Two-Dimensional Covalent Organic Frameworks via Solid–Vapor Interface Reactions Xuan-He Liu, Cui-Zhong Guan, San-Yuan Ding, Wei Wang, Hui-Juan Yan, Dong Wang, and Li-Jun Wan pp 10470–10474 DOI: 10.1021/ja403464h Supporting Info |
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Controlling Conformations of Conjugated Polymers and Small Molecules: The Role of Nonbonding Interactions Nicholas E. Jackson, Brett M. Savoie, Kevin L. Kohlstedt, Monica Olvera de la Cruz, George C. Schatz, Lin X. Chen, and Mark A. Ratner pp 10475–10483 DOI: 10.1021/ja403667s Supporting Info |
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Mechanistic and Preparative Studies of Radical Chain Homolytic Substitution Reactions of N-Heterocyclic Carbene Boranes and Disulfides Xiangcheng Pan, Anne-Laure Vallet, Stéphane Schweizer, Karim Dahbi, Bernard Delpech, Nicolas Blanchard, Bernadette Graff, Steven J. Geib, Dennis P. Curran, Jacques Lalevée, and Emmanuel Lacôte pp 10484–10491 DOI: 10.1021/ja403627k Supporting Info |
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Proton–Electron Transport and Transfer in Electrocatalytic Films. Application to a Cobalt-Based O2-Evolution Catalyst D. Kwabena Bediako, Cyrille Costentin, Evan C. Jones, Daniel G. Nocera, and Jean-Michel Savéant pp 10492–10502 DOI: 10.1021/ja403656w Supporting Info |
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Self-Assembly, Host–Guest Chemistry, and Photophysical Properties of Subphthalocyanine-Based Metallosupramolecular Capsules Irene Sánchez-Molina, Bruno Grimm, Rafael M. Krick Calderon, Christian G. Claessens, Dirk M. Guldi, and Tomas Torres pp 10503–10511 DOI: 10.1021/ja404234n Supporting Info |
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DNA Computation in Mammalian Cells: MicroRNA Logic Operations James Hemphill and Alexander Deiters pp 10512–10518 DOI: 10.1021/ja404350s Supporting Info |
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SSZ-52, a Zeolite with an 18-Layer Aluminosilicate Framework Structure Related to That of the DeNOx Catalyst Cu-SSZ-13 Dan Xie, Lynne B. McCusker, Christian Baerlocher, Stacey I. Zones, Wei Wan, and Xiaodong Zou pp 10519–10524 DOI: 10.1021/ja4043615 Supporting Info |
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Unusual and Highly Tunable Missing-Linker Defects in Zirconium Metal–Organic Framework UiO-66 and Their Important Effects on Gas Adsorption Hui Wu, Yong Shen Chua, Vaiva Krungleviciute, Madhusudan Tyagi, Ping Chen, Taner Yildirim, and Wei Zhou pp 10525–10532 DOI: 10.1021/ja404514r Supporting Info |
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Dynamic Equilibria between Monomeric and Oligomeric Misfolded States of the Mammalian Prion Protein Measured by 19F NMR Sacha Thierry Larda, Karen Simonetti, M. Sameer Al-Abdul-Wahid, Simon Sharpe, and R. Scott Prosser pp 10533–10541 DOI: 10.1021/ja404584s Supporting Info |
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pH-Responsive Supramolecular Vesicles Based on Water-Soluble Pillar[6]arene and Ferrocene Derivative for Drug Delivery Qunpeng Duan, Yu Cao, Yan Li, Xiaoyu Hu, Tangxin Xiao, Chen Lin, Yi Pan, and Leyong Wang pp 10542–10549 DOI: 10.1021/ja405014r Supporting Info |
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Protein–Protein Interaction Regulates the Direction of Catalysis and Electron Transfer in a Redox Enzyme Complex Duncan G. G. McMillan, Sophie J. Marritt, Mackenzie A. Firer-Sherwood, Liang Shi, David J. Richardson, Stephen D. Evans, Sean J. Elliott, Julea N. Butt, and Lars J. C. Jeuken pp 10550–10556 DOI: 10.1021/ja405072z Supporting Info |
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Understanding the Efficiency of Autonomous Nano- and Microscale Motors Wei Wang, Tso-Yi Chiang, Darrell Velegol, and Thomas E. Mallouk pp 10557–10565 DOI: 10.1021/ja405135f Supporting Info |
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Intramolecular RET Enhanced Visible Light-Absorbing Bodipy Organic Triplet Photosensitizers and Application in Photooxidation and Triplet–Triplet Annihilation Upconversion Caishun Zhang, Jianzhang Zhao, Shuo Wu, Zilong Wang, Wanhua Wu, Jie Ma, Song Guo, and Ling Huang pp 10566–10578 DOI: 10.1021/ja405170j Supporting Info |
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Correction to “Using Self-Organization To Control Morphology in Molecular Photovoltaics” Seok Ju Kang, Seokhoon Ahn, Jong Bok Kim, Christine Schenck, Anna M. Hiszpanski, Seokjoon Oh, Theanne Schiros, Yueh-Lin Loo, and Colin Nuckolls pp 10579–10579 DOI: 10.1021/ja404333z |
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Correction to “Hyperstability and Substrate Promiscuity in Laboratory Resurrections of Precambrian β-Lactamases” Valeria A. Risso, Jose A. Gavira, Diego F. Mejia-Carmona, Eric A. Gaucher, and Jose M. Sanchez-Ruiz pp 10580–10580 DOI: 10.1021/ja404387m |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 10581–10581 DOI: 10.1021/ja406854p |
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Maleimide Conjugates of Saxitoxin as Covalent Inhibitors of Voltage-Gated Sodium Channels William H. Parsons and J. Du Bois pp 10582–10585 DOI: 10.1021/ja4019644 Supporting Info |
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Heterogenization of Homogeneous Catalysts in Metal–Organic Frameworks via Cation Exchange Douglas T. Genna, Antek G. Wong-Foy, Adam J. Matzger, and Melanie S. Sanford pp 10586–10589 DOI: 10.1021/ja402577s Supporting Info |
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Secondary Coordination Sphere Influence on the Reactivity of Nonheme Iron(II) Complexes: An Experimental and DFT Approach Sumit Sahu, Leland R. Widger, Matthew G. Quesne, Sam P. de Visser, Hirotoshi Matsumura, Pierre Moënne-Loccoz, Maxime A. Siegler, and David P. Goldberg pp 10590–10593 DOI: 10.1021/ja402688t Supporting Info |
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A Noncovalently Reversible Paramagnetic Switch in Water Alexander T. Buck, Joseph T. Paletta, Shalika A. Khindurangala, Christie L. Beck, and Arthur H. Winter pp 10594–10597 DOI: 10.1021/ja403505z Supporting Info |
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Asymmetric Catalysis with an Inert Chiral-at-Metal Iridium Complex Liang-An Chen, Weici Xu, Biao Huang, Jiajia Ma, Lun Wang, Jianwei Xi, Klaus Harms, Lei Gong, and Eric Meggers pp 10598–10601 DOI: 10.1021/ja403777k Supporting Info |
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Copolymer-Incarcerated Nickel Nanoparticles with N-Heterocyclic Carbene Precursors as Active Cross-Linking Agents for Corriu–Kumada–Tamao Reaction Jean-François Soulé, Hiroyuki Miyamura, and Shu̅ Kobayashi pp 10602–10605 DOI: 10.1021/ja404006w Supporting Info |
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Anthryl-Substituted 3-Silylene-2-silaaziridine Obtained by Isomerization of Disilacyclopropanimine: An Exocyclic Silene Showing a Distinct Intramolecular Charge Transfer Transition Takeaki Iwamoto, Nobuyoshi Ohnishi, Naohiko Akasaka, Koichi Ohno, and Shintaro Ishida pp 10606–10609 DOI: 10.1021/ja404045f Supporting Info |
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Covalent Immobilization of Oriented Photosystem II on a Nanostructured Electrode for Solar Water Oxidation Masaru Kato, Tanai Cardona, A. William Rutherford, and Erwin Reisner pp 10610–10613 DOI: 10.1021/ja404699h Supporting Info |
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Generation of Powerful Tungsten Reductants by Visible Light Excitation Wesley Sattler, Maraia E. Ener, James D. Blakemore, Aaron A. Rachford, Paul J. LaBeaume, James W. Thackeray, James F. Cameron, Jay R. Winkler, and Harry B. Gray pp 10614–10617 DOI: 10.1021/ja4047119 Supporting Info |
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Interfacial Fabrication of Single-Crystalline ZnTe Nanorods with High Blue Fluorescence Linrui Hou, Qiang Zhang, Luting Ling, Chen-Xiong Li, Li Chen, and Su Chen pp 10618–10621 DOI: 10.1021/ja4047476 Supporting Info |
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Efficient Dye-Sensitized Photovoltaic Wires Based on an Organic Redox Electrolyte Shaowu Pan, Zhibin Yang, Houpu Li, Longbin Qiu, Hao Sun, and Huisheng Peng pp 10622–10625 DOI: 10.1021/ja405012w Supporting Info |
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Construction of Vicinal Tertiary and All-Carbon Quaternary Stereocenters via Ir-Catalyzed Regio-, Diastereo-, and Enantioselective Allylic Alkylation and Applications in Sequential Pd Catalysis Wen-Bo Liu, Corey M. Reeves, Scott C. Virgil, and Brian M. Stoltz pp 10626–10629 DOI: 10.1021/ja4052075 Supporting Info |
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Rhodium-Catalyzed Directed C–H Cyanation of Arenes with N-Cyano-N-phenyl-p-toluenesulfonamide Tian-Jun Gong, Bin Xiao, Wan-Min Cheng, Wei Su, Jun Xu, Zhao-Jing Liu, Lei Liu, and Yao Fu pp 10630–10633 DOI: 10.1021/ja405742y Supporting Info |
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A Dual Lewis Base Activation Strategy for Enantioselective Carbene-Catalyzed Annulations Javier Izquierdo, Ane Orue, and Karl A. Scheidt pp 10634–10637 DOI: 10.1021/ja405833m Supporting Info |
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Synthesis of Aryl Sulfonamides via Palladium-Catalyzed Chlorosulfonylation of Arylboronic Acids J. Robb DeBergh, Nootaree Niljianskul, and Stephen L. Buchwald pp 10638–10641 DOI: 10.1021/ja405949a Supporting Info |
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Ligand-Controlled Palladium-Catalyzed Regiodivergent Suzuki–Miyaura Cross-Coupling of Allylboronates and Aryl Halides Yang Yang and Stephen L. Buchwald pp 10642–10645 DOI: 10.1021/ja405950c Supporting Info |
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Femtosecond Electron Solvation at the Ionic Liquid/Metal Electrode Interface Eric A. Muller, Matthew L. Strader, James E. Johns, Aram Yang, Benjamin W. Caplins, Alex J. Shearer, David E. Suich, and Charles B. Harris pp 10646–10653 DOI: 10.1021/ja3108593 |
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Tetrahedral Framework Structures: Polymorphic Phase Transition with Reorientation of Hexagonal Helical Channels in the Zintl Compound Na2ZnSn5 and Its Relation to Na5Zn2+xSn10–x Saskia Stegmaier, Sung-Jin Kim, Alexander Henze, and Thomas F. Fässler pp 10654–10663 DOI: 10.1021/ja401043b Supporting Info |
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Metal–Organic-Frameworks-Derived General Formation of Hollow Structures with High Complexity Lei Zhang, Hao Bin Wu, and Xiong Wen (David) Lou pp 10664–10672 DOI: 10.1021/ja401727n Supporting Info |
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The Role of Reducible Oxide–Metal Cluster Charge Transfer in Catalytic Processes: New Insights on the Catalytic Mechanism of CO Oxidation on Au/TiO2 from ab Initio Molecular Dynamics Yang-Gang Wang, Yeohoon Yoon, Vassiliki-Alexandra Glezakou, Jun Li, and Roger Rousseau pp 10673–10683 DOI: 10.1021/ja402063v Supporting Info |
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Biomimetic Reagents for the Selective Free Radical and Acid–Base Chemistry of Glycans: Application to Glycan Structure Determination by Mass Spectrometry Jinshan Gao, Daniel A. Thomas, Chang Ho Sohn, and J. L. Beauchamp pp 10684–10692 DOI: 10.1021/ja402810t Supporting Info |
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Multiple Pathways for the Primary Step of the Spiropyran Photochromic Reaction: A CASPT2//CASSCF Study Fengyi Liu and Keiji Morokuma pp 10693–10702 DOI: 10.1021/ja402868b Supporting Info |
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Design of Pd/PANI/Pd Sandwich-Structured Nanotube Array Catalysts with Special Shape Effects and Synergistic Effects for Ethanol Electrooxidation An-Liang Wang, Han Xu, Jin-Xian Feng, Liang-Xin Ding, Ye-Xiang Tong, and Gao-Ren Li pp 10703–10709 DOI: 10.1021/ja403101r Supporting Info |
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Formation of Trivalent Zirconocene Complexes from ansa-Zirconocene-Based Olefin-Polymerization Precatalysts: An EPR- and NMR-Spectroscopic Study Taylor N. Lenton, John E. Bercaw, Valentina N. Panchenko, Vladimir A. Zakharov, Dmitrii E. Babushkin, Igor E. Soshnikov, Evgenii P. Talsi, and Hans H. Brintzinger pp 10710–10719 DOI: 10.1021/ja403170u Supporting Info |
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Linear and Nonlinear Two-Coordinate Vanadium Complexes: Synthesis, Characterization, and Magnetic Properties of V(II) Amides Jessica N. Boynton, Jing-Dong Guo, James C. Fettinger, Christopher E. Melton, Shigeru Nagase, and Philip P. Power pp 10720–10728 DOI: 10.1021/ja403244w Supporting Info |
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Oxygen “Getter” Effects on Microstructure and Carrier Transport in Low Temperature Combustion-Processed a-InXZnO (X = Ga, Sc, Y, La) Transistors Jonathan W. Hennek, Jeremy Smith, Aiming Yan, Myung-Gil Kim, Wei Zhao, Vinayak P. Dravid, Antonio Facchetti, and Tobin J. Marks pp 10729–10741 DOI: 10.1021/ja403586x Supporting Info |
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Quantifying the σ and π Interactions between U(V) f Orbitals and Halide, Alkyl, Alkoxide, Amide and Ketimide Ligands Wayne W. Lukens, Norman M. Edelstein, Nicola Magnani, Trevor W. Hayton, Skye Fortier, and Lani A. Seaman pp 10742–10754 DOI: 10.1021/ja403815h Supporting Info |
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Hexagonal Graphene Onion Rings Zheng Yan, Yuanyue Liu, Jian Lin, Zhiwei Peng, Gunuk Wang, Elvira Pembroke, Haiqing Zhou, Changsheng Xiang, Abdul-Rahman O. Raji, Errol L. G. Samuel, Ting Yu, Boris I. Yakobson, and James M. Tour pp 10755–10762 DOI: 10.1021/ja403915m Supporting Info |
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In Situ Synthesis of Thin Zeolitic–Imidazolate Framework ZIF-8 Membranes Exhibiting Exceptionally High Propylene/Propane Separation Hyuk Taek Kwon and Hae-Kwon Jeong pp 10763–10768 DOI: 10.1021/ja403849c Supporting Info |
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Tandem Ring-Opening/Ring-Closing Metathesis Polymerization: Relationship between Monomer Structure and Reactivity Hyeon Park, Ho-Keun Lee, and Tae-Lim Choi pp 10769–10775 DOI: 10.1021/ja4039278 Supporting Info |
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Selective Oxidation of Alcohols to Esters Using Heterogeneous Co3O4–N@C Catalysts under Mild Conditions Rajenahally V. Jagadeesh, Henrik Junge, Marga-Martina Pohl, Jörg Radnik, Angelika Brückner, and Matthias Beller pp 10776–10782 DOI: 10.1021/ja403615c Supporting Info |
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Thioesterase Domains of Fungal Nonreducing Polyketide Synthases Act as Decision Gates during Combinatorial Biosynthesis Yuquan Xu, Tong Zhou, Shuwei Zhang, Li-Jiang Xuan, Jixun Zhan, and István Molnár pp 10783–10791 DOI: 10.1021/ja4041362 Supporting Info |
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Exploiting Hidden Symmetry in Natural Products: Total Syntheses of Amphidinolides C and F Subham Mahapatra and Rich G. Carter pp 10792–10803 DOI: 10.1021/ja404796n Supporting Info |
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Detection of Isomeric Microscopic Host–Guest Complexes. A Time-Evolving Cucurbit[7]uril Complex Mohammad Hossein Tootoonchi, Song Yi, and Angel E. Kaifer pp 10804–10809 DOI: 10.1021/ja404797y Supporting Info |
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Unraveling the Photoluminescence Response of Light-Switching Ruthenium(II) Complexes Bound to Amyloid-β Nathan P. Cook, Mehmet Ozbil, Christina Katsampes, Rajeev Prabhakar, and Angel A. Martí pp 10810–10816 DOI: 10.1021/ja404850u Supporting Info |
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Precise Supramolecular Control of Selectivity in the Rh-Catalyzed Hydroformylation of Terminal and Internal Alkenes Paweł Dydio, Remko J. Detz, and Joost N. H. Reek pp 10817–10828 DOI: 10.1021/ja4046235 Supporting Info |
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Catalyst-Controlled Divergent C–H Functionalization of Unsymmetrical 2-Aryl Cyclic 1,3-Dicarbonyl Compounds with Alkynes and Alkenes Johnathon D. Dooley, Suresh Reddy Chidipudi, and Hon Wai Lam pp 10829–10836 DOI: 10.1021/ja404867k Supporting Info |
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Precursor Transformation during Molecular Oxidation Catalysis with Organometallic Iridium Complexes Ulrich Hintermair, Stafford W. Sheehan, Alexander R. Parent, Daniel H. Ess, David T. Richens, Patrick H. Vaccaro, Gary W. Brudvig, and Robert H. Crabtree pp 10837–10851 DOI: 10.1021/ja4048762 Supporting Info |
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Porphyrins Fused with Strongly Electron-Donating 1,3-Dithiol-2-ylidene Moieties: Redox Control by Metal Cation Complexation and Anion Binding Nathan L. Bill, Masatoshi Ishida, Steffen Bähring, Jong Min Lim, Sangsu Lee, Christina M. Davis, Vincent M. Lynch, Kent A. Nielsen, Jan O. Jeppesen, Kei Ohkubo, Shunichi Fukuzumi, Dongho Kim, and Jonathan L. Sessler pp 10852–10862 DOI: 10.1021/ja404830y Supporting Info |
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Engineering an Enantioselective Amine Oxidase for the Synthesis of Pharmaceutical Building Blocks and Alkaloid Natural Products Diego Ghislieri, Anthony P. Green, Marta Pontini, Simon C. Willies, Ian Rowles, Annika Frank, Gideon Grogan, and Nicholas J. Turner pp 10863–10869 DOI: 10.1021/ja4051235 Supporting Info |
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In Situ AFM Imaging of Li–O2 Electrochemical Reaction on Highly Oriented Pyrolytic Graphite with Ether-Based Electrolyte Rui Wen, Misun Hong, and Hye Ryung Byon pp 10870–10876 DOI: 10.1021/ja405188g Supporting Info |
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Correction to Interaction of Cisplatin with Adenine and Guanine: A Combined IRMPD, MS/MS, and Theoretical Study Barbara Chiavarino, Maria Elisa Crestoni, Simonetta Fornarini, Debora Scuderi, and Jean-Yves Salpin pp 10877–10877 DOI: 10.1021/ja405235n |
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Correction to Isolation of Notoamide E, a Key Precursor in the Biosynthesis of Prenylated Indole Alkaloids in a Marine-Derived Fungus, Aspergillus sp. Sachiko Tsukamoto, Hikaru Kato, Thomas J. Greshock, Hiroshi Hirota, Tomihisa Ohta, and Robert M. Williams pp 10878–10878 DOI: 10.1021/ja405894m |
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Correction to Multisite Prenylation of 4-Substituted Tryptophans by Dimethylallyltryptophan Synthase Jeffrey D. Rudolf, Hong Wang, and C. Dale Poulter pp 10879–10879 DOI: 10.1021/ja405989j |
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Correction to Palladium-Catalyzed Cross-Coupling of Aryl Chlorides and Triflates with Sodium Cyanate: A Practical Synthesis of Unsymmetrical Ureas Ekaterina V. Vinogradova, Brett P. Fors, and Stephen L. Buchwald pp 10880–10880 DOI: 10.1021/ja4058019 |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 10881–10882 DOI: 10.1021/ja4074535 |
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Molybdopterin Biosynthesis: Trapping an Unusual Purine Ribose Adduct in the MoaA-Catalyzed Reaction Angad P. Mehta, Sameh H. Abdelwahed, and Tadhg P. Begley pp 10883–10885 DOI: 10.1021/ja4041048 Supporting Info |
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Enantioselective Total Synthesis of (−)-Citrinadin A and Revision of Its Stereochemical Structure Zhiguo Bian, Christopher C. Marvin, and Stephen F. Martin pp 10886–10889 DOI: 10.1021/ja405547f Supporting Info |
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An Enantioselective Total Synthesis and Stereochemical Revision of (+)-Citrinadin B Ke Kong, John A. Enquist, Jr., Monica E. McCallum, Genessa M. Smith, Takanori Matsumaru, Elnaz Menhaji-Klotz, and John L. Wood pp 10890–10893 DOI: 10.1021/ja405548b Supporting Info |
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Observation of Individual Semiconducting Nanoparticle Collisions by Stochastic Photoelectrochemical Currents Ashantha Fernando, Suman Parajuli, and Mario A. Alpuche-Aviles pp 10894–10897 DOI: 10.1021/ja4007639 Supporting Info |
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Tunable Heparan Sulfate Mimetics for Modulating Chemokine Activity Gloria J. Sheng, Young In Oh, Shuh-Kuen Chang, and Linda C. Hsieh-Wilson pp 10898–10901 DOI: 10.1021/ja4027727 Supporting Info |
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Adaptive Pores: Charge Transfer Modules as Supramolecular Handles for Reversible Pore Engineering of Mesoporous Silica B. V. V. S. Pavan Kumar, K. Venkata Rao, T. Soumya, Subi J. George, and M. Eswaramoorthy pp 10902–10905 DOI: 10.1021/ja4035472 Supporting Info |
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Deconstructing Activation Events in Rhodopsin Elena N. Laricheva, Karunesh Arora, Jennifer L. Knight, and Charles L. Brooks, III pp 10906–10909 DOI: 10.1021/ja4042687 Supporting Info |
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Dehydrocoupling Reactions of Dimethylamine-Borane by Pt(II) Complexes: A New Mechanism Involving Deprotonation of Boronium Cations Marta Roselló-Merino, Joaquín López-Serrano, and Salvador Conejero pp 10910–10913 DOI: 10.1021/ja404655v Supporting Info |
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Selective Synthesis of Co8S15 Cluster in Bowl-Shaped Template of the Pentaaryl[60]fullerene Ligand Masashi Maruyama, Kenta Imoto, Matthias König, Dirk M. Guldi, Shin-ichi Ohkoshi, Eiichi Nakamura, and Yutaka Matsuo pp 10914–10917 DOI: 10.1021/ja405045t Supporting Info |
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Nanoporous Poly(lactide) by Olefin Metathesis Degradation Arthur Bertrand and Marc A. Hillmyer pp 10918–10921 DOI: 10.1021/ja4050532 Supporting Info |
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Patterned Silver Nanoparticles embedded in a Nanoporous Smectic Liquid Crystalline Polymer Network Debarshi Dasgupta, Ivelina K. Shishmanova, Amparo Ruiz-Carretero, Kangbo Lu, Martinus Verhoeven, Huub P. C. van Kuringen, Giuseppe Portale, Philippe Leclère, Cees W. M. Bastiaansen, Dirk J. Broer, and Albertus P. H. J. Schenning pp 10922–10925 DOI: 10.1021/ja404825y Supporting Info |
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Plasmon-Enhanced Photothermoelectric Conversion in Chemical Vapor Deposited Graphene p–n Junctions Di Wu, Kai Yan, Yu Zhou, Huan Wang, Li Lin, Hailin Peng, and Zhongfan Liu pp 10926–10929 DOI: 10.1021/ja404890n Supporting Info |
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Regioselective Carbonylation of trans-Disubstituted Epoxides to β-Lactones: A Viable Entry into syn-Aldol-Type Products Michael Mulzer, Bryan T. Whiting, and Geoffrey W. Coates pp 10930–10933 DOI: 10.1021/ja405151n Supporting Info |
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Overturning Established Chemoselectivities: Selective Reduction of Arenes over Malonates and Cyanoacetates by Photoactivated Organic Electron Donors Eswararao Doni, Bhaskar Mondal, Steven O’Sullivan, Tell Tuttle, and John A. Murphy pp 10934–10937 DOI: 10.1021/ja4050168 Supporting Info |
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Tunable Thioesters as “Reduction” Responsive Functionality for Traceless Reversible Protein PEGylation Jianwei Chen, Mingkun Zhao, Fude Feng, Antons Sizovs, and Jin Wang pp 10938–10941 DOI: 10.1021/ja405261u Supporting Info |
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Engineering the Optical Response of the Titanium-MIL-125 Metal–Organic Framework through Ligand Functionalization Christopher H. Hendon, Davide Tiana, Marc Fontecave, Clément Sanchez, Loïc D’arras, Capucine Sassoye, Laurence Rozes, Caroline Mellot-Draznieks, and Aron Walsh pp 10942–10945 DOI: 10.1021/ja405350u Supporting Info |
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Enantioconvergent Cross-Couplings of Racemic Alkylmetal Reagents with Unactivated Secondary Alkyl Electrophiles: Catalytic Asymmetric Negishi α-Alkylations of N-Boc-pyrrolidine Christopher J. Cordier, Rylan J. Lundgren, and Gregory C. Fu pp 10946–10949 DOI: 10.1021/ja4054114 Supporting Info |
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A Robust Molecular Porous Material with High CO2 Uptake and Selectivity Patrick S. Nugent, Vanessah Lou Rhodus, Tony Pham, Katherine Forrest, Lukasz Wojtas, Brian Space, and Michael J. Zaworotko pp 10950–10953 DOI: 10.1021/ja4054948 Supporting Info |
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Palladium(II)-Catalyzed Direct Carboxylation of Alkenyl C–H Bonds with CO2 Kota Sasano, Jun Takaya, and Nobuharu Iwasawa pp 10954–10957 DOI: 10.1021/ja405503y Supporting Info |
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Bimetallic FeNi Concave Nanocubes and Nanocages Nafiseh Moghimi, Marwa Abdellah, Joseph Palathinkal Thomas, Mamata Mohapatra, and K. T. Leung pp 10958–10961 DOI: 10.1021/ja405504q Supporting Info |
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Spiro-Ring Formation is Catalyzed by a Multifunctional Dioxygenase in Austinol Biosynthesis Yudai Matsuda, Takayoshi Awakawa, Toshiyuki Wakimoto, and Ikuro Abe pp 10962–10965 DOI: 10.1021/ja405518u Supporting Info |
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Highly Ordered Protein Nanorings Designed by Accurate Control of Glutathione S-Transferase Self-Assembly Yushi Bai, Quan Luo, Wei Zhang, Lu Miao, Jiayun Xu, Hongbin Li, and Junqiu Liu pp 10966–10969 DOI: 10.1021/ja405519s Supporting Info |
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Photoselective DNA Hairpin Spin Switches Raanan Carmieli, Arun K. Thazhathveetil, Frederick D. Lewis, and Michael R. Wasielewski pp 10970–10973 DOI: 10.1021/ja4055405 Supporting Info |
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Synthesis and Polymerization of Bicyclic Ketals: A Practical Route to High-Molecular Weight Polyketals Bryan T. Whiting and Geoffrey W. Coates pp 10974–10977 DOI: 10.1021/ja405581r Supporting Info |
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Catalytic Generation of Borenium Ions by Cooperative B–H Bond Activation: The Elusive Direct Electrophilic Borylation of Nitrogen Heterocycles with Pinacolborane Timo Stahl, Kristine Müther, Yasuhiro Ohki, Kazuyuki Tatsumi, and Martin Oestreich pp 10978–10981 DOI: 10.1021/ja405925w Supporting Info |
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Thermodynamic and Kinetic Destabilization of Magnesium Hydride Using Mg–In Solid Solution Alloys Chengshang Zhou, Zhigang Zak Fang, Jun Lu, and Xiaoyi Zhang pp 10982–10985 DOI: 10.1021/ja4058794 Supporting Info |
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Total Synthesis of (+)-Trienomycins A and F via C–C Bond-Forming Hydrogenation and Transfer Hydrogenation David J. Del Valle and Michael J. Krische pp 10986–10989 DOI: 10.1021/ja4061273 Supporting Info |
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Rhodium-Catalyzed Asymmetric Hydroarylation of 3-Pyrrolines Giving 3-Arylpyrrolidines: Protonation as a Key Step Chau Ming So, Satoshi Kume, and Tamio Hayashi pp 10990–10993 DOI: 10.1021/ja406169s Supporting Info |
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Asymmetric Copper(I)-Catalyzed Azide–Alkyne Cycloaddition to Quaternary Oxindoles Feng Zhou, Chen Tan, Jing Tang, Yan-Yan Zhang, Wei-Ming Gao, Hai-Hong Wu, Yi-Hua Yu, and Jian Zhou pp 10994–10997 DOI: 10.1021/ja4066656 Supporting Info |
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Integration of Porous Coordination Polymers and Gold Nanorods into Core–Shell Mesoscopic Composites toward Light-Induced Molecular Release Kira Khaletskaya, Julien Reboul, Mikhail Meilikhov, Masashi Nakahama, Stéphane Diring, Masahiko Tsujimoto, Seiji Isoda, Franklin Kim, Ken-ichiro Kamei, Roland A. Fischer, Susumu Kitagawa, and Shuhei Furukawa pp 10998–11005 DOI: 10.1021/ja403108x Supporting Info |
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Effects of Odd–Even Side Chain Length of Alkyl-Substituted Diphenylbithiophenes on First Monolayer Thin Film Packing Structure Hylke B. Akkerman, Stefan C. B. Mannsfeld, Ananth P. Kaushik, Eric Verploegen, Luc Burnier, Arjan P. Zoombelt, Jonathan D. Saathoff, Sanghyun Hong, Sule Atahan-Evrenk, Xueliang Liu, Alán Aspuru-Guzik, Michael F. Toney, Paulette Clancy, and Zhenan Bao pp 11006–11014 DOI: 10.1021/ja400015e Supporting Info |
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Activatable Oligomerizable Imaging Agents for Photoacoustic Imaging of Furin-Like Activity in Living Subjects Anca Dragulescu-Andrasi, Sri-Rajasekhar Kothapalli, Grigory A. Tikhomirov, Jianghong Rao, and Sanjiv S. Gambhir pp 11015–11022 DOI: 10.1021/ja4010078 Supporting Info |
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Hexagonal-Diamond-like Gold Lattices, Ba and (Au,T)3 Interstitials, and Delocalized Bonding in a Family of Intermetallic Phases Ba2Au6(Au,T)3 (T = Zn, Cd, Ga, In, or Sn) Qisheng Lin, Trinath Mishra, and John D. Corbett pp 11023–11031 DOI: 10.1021/ja401378q Supporting Info |
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Small-Molecule-Induced Clustering of Heparan Sulfate Promotes Cell Adhesion Naohiro Takemoto, Tetsuya Suehara, Heidie L. Frisco, Shin-ichi Sato, Takuhito Sezaki, Kosuke Kusamori, Yoshinori Kawazoe, Sun Min Park, Sayumi Yamazoe, Yoshiyuki Mizuhata, Rintaro Inoue, Gavin J. Miller, Steen U. Hansen, Gordon C. Jayson, John M. Gardiner, Toshiji Kanaya, Norihiro Tokitoh, Kazumitsu Ueda, Yoshinobu Takakura, Noriyuki Kioka, Makiya Nishikawa, and Motonari Uesugi pp 11032–11039 DOI: 10.1021/ja4018682 Supporting Info |
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Direct Observation of Reductive Elimination of MeX (X = Cl, Br, I) from RhIII Complexes: Mechanistic Insight and the Importance of Sterics Moran Feller, Yael Diskin-Posner, Gregory Leitus, Linda J. W. Shimon, and David Milstein pp 11040–11047 DOI: 10.1021/ja401852c Supporting Info |
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Exploiting Localized Surface Binding Effects to Enhance the Catalytic Reactivity of Peptide-Capped Nanoparticles Ryan Coppage, Joseph M. Slocik, Hadi Ramezani-Dakhel, Nicholas M. Bedford, Hendrik Heinz, Rajesh R. Naik, and Marc R. Knecht pp 11048–11054 DOI: 10.1021/ja402215t Supporting Info |
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Designed Synthesis, Structure, and Properties of a Family of Ferecrystalline Compounds [(PbSe)1.00]m(MoSe2)n Colby L. Heideman, Sara Tepfer, Qiyin Lin, Raimar Rostek, Paul Zschack, Michael D. Anderson, Ian M. Anderson, and David C. Johnson pp 11055–11062 DOI: 10.1021/ja402819q |
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Ultrafast Structural Dynamics Inside Planar Phospholipid Multibilayer Model Cell Membranes Measured with 2D IR Spectroscopy Oksana Kel, Amr Tamimi, Megan C. Thielges, and Michael D. Fayer pp 11063–11074 DOI: 10.1021/ja403675x |
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Coexistence of Helical Morphologies in Columnar Stacks of Star-Shaped Discotic Hydrazones Jie Shu, Dmytro Dudenko, Morteza Esmaeili, Jun Ha Park, Sreenivasa Reddy Puniredd, Ji Young Chang, Dag Werner Breiby, Wojciech Pisula, and Michael Ryan Hansen pp 11075–11086 DOI: 10.1021/ja4029186 Supporting Info |
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Partial Oxidation of Ethane to Oxygenates Using Fe- and Cu-Containing ZSM-5 Michael M. Forde, Robert D. Armstrong, Ceri Hammond, Qian He, Robert L. Jenkins, Simon A. Kondrat, Nikolaos Dimitratos, Jose Antonio Lopez-Sanchez, Stuart H. Taylor, David Willock, Christopher J. Kiely, and Graham John Hutchings pp 11087–11099 DOI: 10.1021/ja403060n Supporting Info |
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New Pathways for Formation of Acids and Carbonyl Products in Low-Temperature Oxidation: The Korcek Decomposition of γ-Ketohydroperoxides Amrit Jalan, Ionut M. Alecu, Rubén Meana-Pañeda, Jorge Aguilera-Iparraguirre, Ke R. Yang, Shamel S. Merchant, Donald G. Truhlar, and William H. Green pp 11100–11114 DOI: 10.1021/ja4034439 Supporting Info |
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Inorganic Nanostructures with Sizes down to 1 nm: A Macromolecule Analogue Shi Hu, Huiling Liu, Pengpeng Wang, and Xun Wang pp 11115–11124 DOI: 10.1021/ja403471d Supporting Info |
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Layered Perovskite Oxide: A Reversible Air Electrode for Oxygen Evolution/Reduction in Rechargeable Metal-Air Batteries Tatsuya Takeguchi, Toshiro Yamanaka, Hiroki Takahashi, Hiroshi Watanabe, Tomohiro Kuroki, Haruyuki Nakanishi, Yuki Orikasa, Yoshiharu Uchimoto, Hiroshi Takano, Nobuaki Ohguri, Motofumi Matsuda, Tadatoshi Murota, Kohei Uosaki, and Wataru Ueda pp 11125–11130 DOI: 10.1021/ja403476v Supporting Info |
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Reversible Generation of a Carbon-Centered Radical from Alkyl Iodide Using Organic Salts and Their Application as Organic Catalysts in Living Radical Polymerization Atsushi Goto, Akimichi Ohtsuki, Haruki Ohfuji, Miho Tanishima, and Hironori Kaji pp 11131–11139 DOI: 10.1021/ja4036016 Supporting Info |
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Synthesis and Vaccine Evaluation of the Tumor-Associated Carbohydrate Antigen RM2 from Prostate Cancer Hong-Yang Chuang, Chien-Tai Ren, Chung-An Chao, Chung-Yi Wu, Sachin S. Shivatare, Ting-Jen R. Cheng, Chung-Yi Wu, and Chi-Huey Wong pp 11140–11150 DOI: 10.1021/ja403609x Supporting Info |
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Electron Flow through Nitrotyrosinate in Pseudomonas aeruginosa Azurin Jeffrey J. Warren, Nadia Herrera, Michael G. Hill, Jay R. Winkler, and Harry B. Gray pp 11151–11158 DOI: 10.1021/ja403734n Supporting Info |
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Mesoscale Modulation of Supramolecular Ureidopyrimidinone-Based Poly(ethylene glycol) Transient Networks in Water Roxanne E. Kieltyka, A. C. H. Pape, Lorenzo Albertazzi, Yoko Nakano, Maartje M. C. Bastings, Ilja K. Voets, Patricia Y. W. Dankers, and E. W. Meijer pp 11159–11164 DOI: 10.1021/ja403745w Supporting Info |
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A Metallofullerene Electron Donor that Powers an Efficient Spin Flip in a Linear Electron Donor–Acceptor Conjugate Marc Rudolf, Lai Feng, Zdenek Slanina, Takeshi Akasaka, Shigeru Nagase, and Dirk M. Guldi pp 11165–11174 DOI: 10.1021/ja403763e Supporting Info |
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A Single gD Glycoprotein Can Mediate Infection by Herpes simplex Virus Richard W. Clarke, Anna Drews, Helena Browne, and David Klenerman pp 11175–11180 DOI: 10.1021/ja4038406 Supporting Info |
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Measuring Electrostatic Fields in Both Hydrogen-Bonding and Non-Hydrogen-Bonding Environments Using Carbonyl Vibrational Probes Stephen D. Fried, Sayan Bagchi, and Steven G. Boxer pp 11181–11192 DOI: 10.1021/ja403917z Supporting Info |
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A Bacterial Tyrosine Aminomutase Proceeds through Retention or Inversion of Stereochemistry To Catalyze Its Isomerization Reaction Udayanga Wanninayake and Kevin D. Walker pp 11193–11204 DOI: 10.1021/ja403918w Supporting Info |
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Synthesis, Characterization, and Electrochemical Studies of PPh3–n(dipp)n (dipp = 2,6-Diisopropylphenyl): Steric and Electronic Effects on the Chemical and Electrochemical Oxidation of a Homologous Series of Triarylphosphines and the Reactivities of the Corresponding Phosphoniumyl Radical Cations John P. Bullock, Alan M. Bond, René T. Boeré, Twyla M. Gietz, Tracey L. Roemmele, Sonja D. Seagrave, Jason D. Masuda, and Masood Parvez pp 11205–11215 DOI: 10.1021/ja403555d Supporting Info |
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Herpes Virus Genome, The Pressure Is On David W. Bauer, Jamie B. Huffman, Fred L. Homa, and Alex Evilevitch pp 11216–11221 DOI: 10.1021/ja404008r Supporting Info |
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Scope and Mechanism of the Pt-Catalyzed Enantioselective Diboration of Monosubstituted Alkenes John R. Coombs, Fredrik Haeffner, Laura T. Kliman, and James P. Morken pp 11222–11231 DOI: 10.1021/ja4041016 Supporting Info |
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Biocatalytic Synthesis of Pikromycin, Methymycin, Neomethymycin, Novamethymycin, and Ketomethymycin Douglas A. Hansen, Christopher M. Rath, Eli B. Eisman, Alison R. H. Narayan, Jeffrey D. Kittendorf, Jonathan D. Mortison, Yeo Joon Yoon, and David H. Sherman pp 11232–11238 DOI: 10.1021/ja404134f Supporting Info |
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Realizing Molecular Pixel System for Full-Color Fluorescence Reproduction: RGB-Emitting Molecular Mixture Free from Energy Transfer Crosstalk Ji Eon Kwon, Sanghyuk Park, and Soo Young Park pp 11239–11246 DOI: 10.1021/ja404256s Supporting Info |
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Relation between Structure and Electronic Properties of Amorphous MEH-PPV Polymers Ting Qin and Alessandro Troisi pp 11247–11256 DOI: 10.1021/ja404385y Supporting Info |
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Interfacial Electric Field Effects on a Carbene Reaction Catalyzed by Rh Porphyrins Craig F. Gorin, Eugene S. Beh, Quan M. Bui, Graham R. Dick, and Matthew W. Kanan pp 11257–11265 DOI: 10.1021/ja404394z Supporting Info |
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Reactivity of TEMPO toward 16- and 17-Electron Organometallic Reaction Intermediates: A Time-Resolved IR Study Justin P. Lomont, Son C. Nguyen, and Charles B. Harris pp 11266–11273 DOI: 10.1021/ja404476m Supporting Info |
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Cellular Toxicity Induced by the Photorelease of a Caged Bioactive Molecule: Design of a Potential Dual-Action Ru(II) Complex Mark A. Sgambellone, Amanda David, Robert N. Garner, Kim R. Dunbar, and Claudia Turro pp 11274–11282 DOI: 10.1021/ja4045604 Supporting Info |
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Intercalators as Molecular Chaperones in DNA Self-Assembly Andrea A. Greschner, Katherine E. Bujold, and Hanadi F. Sleiman pp 11283–11288 DOI: 10.1021/ja404402b Supporting Info |
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Unprecedented Boron-Functionalized Carborane Derivatives by Facile and Selective Cobalt-Induced B–H Activation Zhaojin Wang, Hongde Ye, Yuguang Li, Yizhi Li, and Hong Yan pp 11289–11298 DOI: 10.1021/ja4047075 Supporting Info |
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Hydration Layer Coupling and Cooperativity in Phase Behavior of Stimulus Responsive Peptide Polymers Dennis Kurzbach, Wafa Hassouneh, Jonathan R. McDaniel, Eva A. Jaumann, Ashutosh Chilkoti, and Dariush Hinderberger pp 11299–11308 DOI: 10.1021/ja4047872 Supporting Info |
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Unexpected Interaction between PEDOT and Phosphonium Ionic Liquids Vanessa Armel, Jonathan Rivnay, George Malliaras, and Bjorn Winther-Jensen pp 11309–11313 DOI: 10.1021/ja405032c Supporting Info |
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Chemical Sensing of Polyols with Shapeshifting Boronic Acids As a Self-Contained Sensor Array Johannes F. Teichert, Dmitry Mazunin, and Jeffrey W. Bode pp 11314–11321 DOI: 10.1021/ja404981q Supporting Info |
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Quantifying Elongation Rhythm during Full-Length Protein Synthesis Gabriel Rosenblum, Chunlai Chen, Jaskiran Kaur, Xiaonan Cui, Haibo Zhang, Haruichi Asahara, Shaorong Chong, Zeev Smilansky, Yale E. Goldman, and Barry S. Cooperman pp 11322–11329 DOI: 10.1021/ja405205c Supporting Info |
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An Artificial Light-Harvesting Array Constructed from Multiple Bodipy Dyes Raymond Ziessel, Gilles Ulrich, Alexandre Haefele, and Anthony Harriman pp 11330–11344 DOI: 10.1021/ja4049306 Supporting Info |
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Integration of Intrinsic Proton Conduction and Guest-Accessible Nanospace into a Coordination Polymer Daiki Umeyama, Satoshi Horike, Munehiro Inukai, and Susumu Kitagawa pp 11345–11350 DOI: 10.1021/ja4051668 Supporting Info |
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Kinetics and Low Temperature Studies of Electron Transfers in Films of Small (<2 nm) Au Monolayer Protected Clusters Tessa M. Carducci and Royce W. Murray pp 11351–11356 DOI: 10.1021/ja405342r Supporting Info |
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Thermodynamic and Kinetic Study of Cleavage of the N–O Bond of N-Oxides by a Vanadium(III) Complex: Enhanced Oxygen Atom Transfer Reaction Rates for Adducts of Nitrous Oxide and Mesityl Nitrile Oxide Taryn D. Palluccio, Elena V. Rybak-Akimova, Subhojit Majumdar, Xiaochen Cai, Megan Chui, Manuel Temprado, Jared S. Silvia, Anthony F. Cozzolino, Daniel Tofan, Alexandra Velian, Christopher C. Cummins, Burjor Captain, and Carl D. Hoff pp 11357–11372 DOI: 10.1021/ja405395z Supporting Info |
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Synthesis of a Base-Free Hafnium Nitride from N2 Cleavage: A Versatile Platform for Dinitrogen Functionalization Scott P. Semproni and Paul J. Chirik pp 11373–11383 DOI: 10.1021/ja405477m Supporting Info |
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General and Regioselective Synthesis of Pyrroles via Ruthenium-Catalyzed Multicomponent Reactions Min Zhang, Xianjie Fang, Helfried Neumann, and Matthias Beller pp 11384–11388 DOI: 10.1021/ja406666r Supporting Info |
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Combined Charge Carrier Transport and Photoelectrochemical Characterization of BiVO4 Single Crystals: Intrinsic Behavior of a Complex Metal Oxide Alexander J. E. Rettie, Heung Chan Lee, Luke G. Marshall, Jung-Fu Lin, Cigdem Capan, Jeffrey Lindemuth, John S. McCloy, Jianshi Zhou, Allen J. Bard, and C. Buddie Mullins pp 11389–11396 DOI: 10.1021/ja405550k Supporting Info |
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Asymmetric Free-Standing 2-D Photonic Crystal Films and Their Janus Particles Jian-Tao Zhang, Xing Chao, and Sanford A. Asher pp 11397–11401 DOI: 10.1021/ja405629k Supporting Info |
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Asymmetric Cascade Annulation Based on Enantioselective Oxa-Diels–Alder Cycloaddition of in Situ Generated Isochromenyliums by Cooperative Binary Catalysis of Pd(OAc)2 and (S)-Trip Shu-Yan Yu, Hao Zhang, Yang Gao, Lei Mo, Shaozhong Wang, and Zhu-Jun Yao pp 11402–11407 DOI: 10.1021/ja405764p Supporting Info |
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The Mechanism of Photohydrosilylation on Silicon and Porous Silicon Surfaces Kurt W. Kolasinski pp 11408–11412 DOI: 10.1021/ja406063n |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 11413–11413 DOI: 10.1021/ja407725k |
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Sequence-Specific Inhibition of a Nonspecific Protease Leigh A. Logsdon and Adam R. Urbach pp 11414–11416 DOI: 10.1021/ja406032x Supporting Info |
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Nucleation-Controlled Polymerization of Nanoparticles into Supramolecular Structures Jing Wang, Hongwei Xia, Yanfeng Zhang, Hua Lu, Ranjan Kamat, Andrey V. Dobrynin, Jianjun Cheng, and Yao Lin pp 11417–11420 DOI: 10.1021/ja402757e Supporting Info |
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How Far Can We Push Polymer Architectures? Patrick J. M. Stals, Yuanchao Li, Joanna Burdyńska, Renaud Nicolaÿ, Alper Nese, Anja R. A. Palmans, E. W. Meijer, Krzysztof Matyjaszewski, and Sergei S. Sheiko pp 11421–11424 DOI: 10.1021/ja400890v Supporting Info |
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An FeF3·0.5H2O Polytype: A Microporous Framework Compound with Intersecting Tunnels for Li and Na Batteries Chilin Li, Congling Yin, Lin Gu, Robert E. Dinnebier, Xiaoke Mu, Peter A. van Aken, and Joachim Maier pp 11425–11428 DOI: 10.1021/ja402061q Supporting Info |
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Level Alignment of a Prototypical Photocatalytic System: Methanol on TiO2(110) Annapaola Migani, Duncan J. Mowbray, Amilcare Iacomino, Jin Zhao, Hrvoje Petek, and Angel Rubio pp 11429–11432 DOI: 10.1021/ja4036994 Supporting Info |
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Unexpected Catalytic Performance in Silent Tantalum Oxide through Nitridation and Defect Chemistry Yiguo Su, Junyu Lang, Liping Li, Kai Guan, Chunfang Du, Liman Peng, Dan Han, and Xiaojing Wang pp 11433–11436 DOI: 10.1021/ja404239z Supporting Info |
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Design and Synthesis of Metal Sulfide Catalysts Supported on Zeolite Nanofiber Bundles with Unprecedented Hydrodesulfurization Activities Tiandi Tang, Lei Zhang, Wenqian Fu, Yuli Ma, Jin Xu, Jun Jiang, Guoyong Fang, and Feng-Shou Xiao pp 11437–11440 DOI: 10.1021/ja4043388 Supporting Info |
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Bifacial DNA Origami-Directed Discrete, Three-Dimensional, Anisotropic Plasmonic Nanoarchitectures with Tailored Optical Chirality Xiang Lan, Zhong Chen, Gaole Dai, Xuxing Lu, Weihai Ni, and Qiangbin Wang pp 11441–11444 DOI: 10.1021/ja404354c Supporting Info |
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Naphthodithiophenediimide (NDTI): Synthesis, Structure, and Applications Yuta Fukutomi, Masahiro Nakano, Jian-Yong Hu, Itaru Osaka, and Kazuo Takimiya pp 11445–11448 DOI: 10.1021/ja404753r Supporting Info |
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Selective Trapping of Labile S3 in a Porous Coordination Network and the Direct X-ray Observation Hiroyoshi Ohtsu, Wanuk Choi, Nazrul Islam, Yoshitaka Matsushita, and Masaki Kawano pp 11449–11452 DOI: 10.1021/ja4046718 Supporting Info |
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Hybrid Semiconducting Polymer Nanoparticles as Polarization-Sensitive Fluorescent Probes Maxwell B. Zeigler, Wei Sun, Yu Rong, and Daniel T. Chiu pp 11453–11456 DOI: 10.1021/ja404719f Supporting Info |
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Nitrososynthase-Triggered Oxidative Carbon–Carbon Bond Cleavage in Baumycin Biosynthesis Ahmad Al-Mestarihi, Anthony Romo, Hung-wen Liu, and Brian O. Bachmann pp 11457–11460 DOI: 10.1021/ja404987r Supporting Info |
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Charging of Quantum Dots by Sulfide Redox Electrolytes Reduces Electron Injection Efficiency in Quantum Dot Sensitized Solar Cells Haiming Zhu, Nianhui Song, and Tianquan Lian pp 11461–11464 DOI: 10.1021/ja405026x Supporting Info |
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Synthesis Modulation as a Tool To Increase the Catalytic Activity of Metal–Organic Frameworks: The Unique Case of UiO-66(Zr) Frederik Vermoortele, Bart Bueken, Gaëlle Le Bars, Ben Van de Voorde, Matthias Vandichel, Kristof Houthoofd, Alexandre Vimont, Marco Daturi, Michel Waroquier, Veronique Van Speybroeck, Christine Kirschhock, and Dirk E. De Vos pp 11465–11468 DOI: 10.1021/ja405078u Supporting Info |
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Giant Negative Thermal Expansion in NaZn13-Type La(Fe, Si, Co)13 Compounds Rongjin Huang, Yanying Liu, Wei Fan, Jie Tan, Furen Xiao, Lihe Qian, and Laifeng Li pp 11469–11472 DOI: 10.1021/ja405161z Supporting Info |
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Catalytic Asymmetric Three-Component 1,3-Dipolar Cycloaddition of Aldehydes, Hydrazides, and Alkynes Takuya Hashimoto, Yuka Takiguchi, and Keiji Maruoka pp 11473–11476 DOI: 10.1021/ja405444c Supporting Info |
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A Synthetic Zipper Peptide Motif Orchestrated via Co-operative Interplay of Hydrogen Bonding, Aromatic Stacking, and Backbone Chirality Roshna V. Nair, Sanjeev Kheria, Suresh Rayavarapu, Amol S. Kotmale, Bharatam Jagadeesh, Rajesh G. Gonnade, Vedavati G. Puranik, Pattuparambil R. Rajamohanan, and Gangadhar J. Sanjayan pp 11477–11480 DOI: 10.1021/ja405455g Supporting Info |
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Dioxygen-Triggered Oxidative Radical Reaction: Direct Aerobic Difunctionalization of Terminal Alkynes toward β-Keto Sulfones Qingquan Lu, Jian Zhang, Ganglu Zhao, Yue Qi, Huamin Wang, and Aiwen Lei pp 11481–11484 DOI: 10.1021/ja4052685 Supporting Info |
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Enhanced Rate and Selectivity by Carboxylate Salt as a Basic Cocatalyst in Chiral N-Heterocyclic Carbene-Catalyzed Asymmetric Acylation of Secondary Alcohols Satoru Kuwano, Shingo Harada, Bubwoong Kang, Raphaël Oriez, Yousuke Yamaoka, Kiyosei Takasu, and Ken-ichi Yamada pp 11485–11488 DOI: 10.1021/ja4055838 Supporting Info |
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Plasmonically Nanoconfined Light Probing Invisible Phonon Modes in Defect-Free Graphene Katsuyoshi Ikeda, Mai Takase, Norihiko Hayazawa, Satoshi Kawata, Kei Murakoshi, and Kohei Uosaki pp 11489–11492 DOI: 10.1021/ja4056596 |
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Dinitrogen Reduction by a Chromium(0) Complex Supported by a 16-Membered Phosphorus Macrocycle Michael T. Mock, Shentan Chen, Molly O’Hagan, Roger Rousseau, William G. Dougherty, W. Scott Kassel, and R. Morris Bullock pp 11493–11496 DOI: 10.1021/ja405668u Supporting Info |
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Enantioselective Synthesis of Anti Homoallylic Alcohols from Terminal Alkynes and Aldehydes Based on Concomitant Use of a Cationic Iridium Complex and a Chiral Phosphoric Acid Tomoya Miura, Yui Nishida, Masao Morimoto, and Masahiro Murakami pp 11497–11500 DOI: 10.1021/ja405790t Supporting Info |
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Reorientation of a Single Bond within an Adsorbed Molecule by Tunneling Electrons Jörg Henzl, Konrad Boom, and Karina Morgenstern pp 11501–11504 DOI: 10.1021/ja405809f |
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Triply Stacked Heterogeneous Array of Porphyrins and Phthalocyanine through Stepwise Formation of a Fourfold Rotaxane and an Ionic Complex Yasuyuki Yamada, Nozomi Mihara, Shinya Shibano, Kunihisa Sugimoto, and Kentaro Tanaka pp 11505–11508 DOI: 10.1021/ja405963t Supporting Info |
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Photoreconfigurable Supramolecular Nanotube Toshihiro Sendai, Shuvendu Biswas, and Takuzo Aida pp 11509–11512 DOI: 10.1021/ja4060146 Supporting Info |
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Stepwise Filtering of the Internal Layers of Dendrimers by Transverse-Relaxation-Edited NMR Luiz F. Pinto, Ricardo Riguera, and Eduardo Fernandez-Megia pp 11513–11516 DOI: 10.1021/ja4059348 Supporting Info |
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A Room-Temperature Catalytic Asymmetric Synthesis of Allenes with ECNU-Phos Yuli Wang, Wanli Zhang, and Shengming Ma pp 11517–11520 DOI: 10.1021/ja406135t Supporting Info |
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Enantioselective Direct α-Amination of Aldehydes via a Photoredox Mechanism: A Strategy for Asymmetric Amine Fragment Coupling Giuseppe Cecere, Christian M. König, Jennifer L. Alleva, and David W. C. MacMillan pp 11521–11524 DOI: 10.1021/ja406181e Supporting Info |
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Manganese–Tin Triple Bonds: A New Synthetic Route to the Manganese Stannylidyne Complex Cation trans-[H(dmpe)2Mn≡Sn(C6H3-2,6-Mes2)]+ (dmpe = Me2PCH2CH2PMe2, Mes = 2,4,6-Trimethylphenyl) Alexander C. Filippou, Priyabrata Ghana, Uttam Chakraborty, and Gregor Schnakenburg pp 11525–11528 DOI: 10.1021/ja406290t Supporting Info |
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Dye Stabilization and Enhanced Photoelectrode Wettability in Water-Based Dye-Sensitized Solar Cells through Post-assembly Atomic Layer Deposition of TiO2 Ho-Jin Son, Chaiya Prasittichai, Joseph E. Mondloch, Langli Luo, Jinsong Wu, Dong Wook Kim, Omar K. Farha, and Joseph T. Hupp pp 11529–11532 DOI: 10.1021/ja406538a Supporting Info |
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A Cobalt-Based Catalyst for the Hydrogenation of CO2 under Ambient Conditions Matthew S. Jeletic, Michael T. Mock, Aaron M. Appel, and John C. Linehan pp 11533–11536 DOI: 10.1021/ja406601v Supporting Info |
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Photocurrent Enhancement from Diketopyrrolopyrrole Polymer Solar Cells through Alkyl-Chain Branching Point Manipulation Iain Meager, Raja Shahid Ashraf, Sonya Mollinger, Bob C. Schroeder, Hugo Bronstein, Daniel Beatrup, Michelle S. Vezie, Thomas Kirchartz, Alberto Salleo, Jenny Nelson, and Iain McCulloch pp 11537–11540 DOI: 10.1021/ja406934j Supporting Info |
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First-Principles Characterization of the Energy Landscape and Optical Spectra of Green Fluorescent Protein along the A→I→B Proton Transfer Route Bella L. Grigorenko, Alexander V. Nemukhin, Igor V. Polyakov, Dmitry I. Morozov, and Anna I. Krylov pp 11541–11549 DOI: 10.1021/ja402472y Supporting Info |
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A Generalized Electrochemical Aggregative Growth Mechanism Jon Ustarroz, Joshua A. Hammons, Thomas Altantzis, Annick Hubin, Sara Bals, and Herman Terryn pp 11550–11561 DOI: 10.1021/ja402598k Supporting Info |
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Near-Infrared Absorbing Cu12Sb4S13 and Cu3SbS4 Nanocrystals: Synthesis, Characterization, and Photoelectrochemistry Joel van Embden, Kay Latham, Noel W. Duffy, and Yasuhiro Tachibana pp 11562–11571 DOI: 10.1021/ja402702x Supporting Info |
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Mechanistic Studies of Water Electrolysis and Hydrogen Electro-Oxidation on High Temperature Ceria-Based Solid Oxide Electrochemical Cells Chunjuan Zhang, Yi Yu, Michael E. Grass, Catherine Dejoie, Wuchen Ding, Karen Gaskell, Naila Jabeen, Young Pyo Hong, Andrey Shavorskiy, Hendrik Bluhm, Wei-Xue Li, Gregory S. Jackson, Zahid Hussain, Zhi Liu, and Bryan W. Eichhorn pp 11572–11579 DOI: 10.1021/ja402604u Supporting Info |
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Water Oxidation Catalysis: Electrocatalytic Response to Metal Stoichiometry in Amorphous Metal Oxide Films Containing Iron, Cobalt, and Nickel Rodney D. L. Smith, Mathieu S. Prévot, Randal D. Fagan, Simon Trudel, and Curtis P. Berlinguette pp 11580–11586 DOI: 10.1021/ja403102j Supporting Info |
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Accumulation of Multiple Oxidative Equivalents at a Single Site by Cross-Surface Electron Transfer on TiO2 Wenjing Song, Akitaka Ito, Robert A. Binstead, Kenneth Hanson, Hanlin Luo, M. Kyle Brennaman, Javier J. Concepcion, and Thomas J. Meyer pp 11587–11594 DOI: 10.1021/ja4032538 Supporting Info |
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A Dual-Emission Fluorescent Nanocomplex of Gold-Cluster-Decorated Silica Particles for Live Cell Imaging of Highly Reactive Oxygen Species Tingting Chen, Yihui Hu, Yao Cen, Xia Chu, and Yi Lu pp 11595–11602 DOI: 10.1021/ja4035939 Supporting Info |
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Photoexpulsion of Surface-Grafted Ruthenium Complexes and Subsequent Release of Cytotoxic Cargos to Cancer Cells from Mesoporous Silica Nanoparticles Marco Frasconi, Zhichang Liu, Juying Lei, Yilei Wu, Elena Strekalova, Dmitry Malin, Michael W. Ambrogio, Xinqi Chen, Youssry Y. Botros, Vincent L. Cryns, Jean-Pierre Sauvage, and J. Fraser Stoddart pp 11603–11613 DOI: 10.1021/ja405058y Supporting Info |
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Synergistic Effect in Carbon Coated LiFePO4 for High Yield Spontaneous Grafting of Diazonium Salt. Structural Examination at the Grain Agglomerate Scale Lénaïc Madec, Donatien Robert, Philippe Moreau, Pascale Bayle-Guillemaud, Dominique Guyomard, and Joël Gaubicher pp 11614–11622 DOI: 10.1021/ja405087x Supporting Info |
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In Vivo Activation of the p53 Tumor Suppressor Pathway by an Engineered Cyclotide Yanbin Ji, Subhabrata Majumder, Melissa Millard, Radhika Borra, Tao Bi, Ahmed Y. Elnagar, Nouri Neamati, Alexander Shekhtman, and Julio A. Camarero pp 11623–11633 DOI: 10.1021/ja405108p Supporting Info |
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Synthesis and Crystallographic Analysis of Shape-Controlled SnS Nanocrystal Photocatalysts: Evidence for a Pseudotetragonal Structural Modification Adam J. Biacchi, Dimitri D. Vaughn, II, and Raymond E. Schaak pp 11634–11644 DOI: 10.1021/ja405203e Supporting Info |
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Ideal Polyethylene Nanocrystals Anna Osichow, Christian Rabe, Karsten Vogtt, Theyencheri Narayanan, Ludger Harnau, Markus Drechsler, Matthias Ballauff, and Stefan Mecking pp 11645–11650 DOI: 10.1021/ja4052334 Supporting Info |
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The Unusual and the Expected in the Si/C Phase Diagram Guoying Gao, N. W. Ashcroft, and Roald Hoffmann pp 11651–11656 DOI: 10.1021/ja405359a Supporting Info |
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Folate-Based Near-Infrared Fluorescent Theranostic Gemcitabine Delivery Zhigang Yang, Jae Hong Lee, Hyun Mi Jeon, Ji Hye Han, Nayoung Park, Yanxia He, Hyunseung Lee, Kwan Soo Hong, Chulhun Kang, and Jong Seung Kim pp 11657–11662 DOI: 10.1021/ja405372k Supporting Info |
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An Off–On COX-2-Specific Fluorescent Probe: Targeting the Golgi Apparatus of Cancer Cells Hua Zhang, Jiangli Fan, Jingyun Wang, Shuangzhe Zhang, Bairui Dou, and Xiaojun Peng pp 11663–11669 DOI: 10.1021/ja4056905 Supporting Info |
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Molecular Engineering of Organophosphate Hydrolysis Activity from a Weak Promiscuous Lactonase Template Monika M. Meier, Chitra Rajendran, Christoph Malisi, Nicholas G. Fox, Chengfu Xu, Sandra Schlee, David P. Barondeau, Birte Höcker, Reinhard Sterner, and Frank M. Raushel pp 11670–11677 DOI: 10.1021/ja405911h Supporting Info |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 11679–11679 DOI: 10.1021/ja4081452 |
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Picazoplatin, an Azide-Containing Platinum(II) Derivative for Target Analysis by Click Chemistry Jonathan D. White, Maire F. Osborn, Alan D. Moghaddam, Lindsay E. Guzman, Michael M. Haley, and Victoria J. DeRose pp 11680–11683 DOI: 10.1021/ja402453k Supporting Info |
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A Microporous Hydrogen-Bonded Organic Framework: Exceptional Stability and Highly Selective Adsorption of Gas and Liquid Xu-Zhong Luo, Xin-Jian Jia, Ji-Hua Deng, Jin-Lian Zhong, Hui-Jin Liu, Ke-Jun Wang, and Di-Chang Zhong pp 11684–11687 DOI: 10.1021/ja403002m Supporting Info |
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Stepwise Ligand Exchange for the Preparation of a Family of Mesoporous MOFs Tao Li, Mark T. Kozlowski, Evan A. Doud, Maike N. Blakely, and Nathaniel L. Rosi pp 11688–11691 DOI: 10.1021/ja403810k Supporting Info |
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TEMPO-catalyzed Aerobic Oxygenation and Nitrogenation of Olefins via C═C Double-Bond Cleavage Teng Wang and Ning Jiao pp 11692–11695 DOI: 10.1021/ja403824y Supporting Info |
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Photostable p-Type Dye-Sensitized Photoelectrochemical Cells for Water Reduction Zhiqiang Ji, Mingfu He, Zhongjie Huang, Umit Ozkan, and Yiying Wu pp 11696–11699 DOI: 10.1021/ja404525e Supporting Info |
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Cu-Catalyzed Asymmetric Borylative Cyclization of Cyclohexadienone-Containing 1,6-Enynes Ping Liu, Yuki Fukui, Ping Tian, Zhi-Tao He, Cai-Yun Sun, Nuo-Yi Wu, and Guo-Qiang Lin pp 11700–11703 DOI: 10.1021/ja404593c Supporting Info |
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Ruthenium-Catalyzed Redox-Neutral and Single-Step Amide Synthesis from Alcohol and Nitrile with Complete Atom Economy Byungjoon Kang, Zhenqian Fu, and Soon Hyeok Hong pp 11704–11707 DOI: 10.1021/ja404695t Supporting Info |
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X-ray Crystal Structure of Phosphodiesterase 2 in Complex with a Highly Selective, Nanomolar Inhibitor Reveals a Binding-Induced Pocket Important for Selectivity Jian Zhu, Qiqi Yang, Dandan Dai, and Qiang Huang pp 11708–11711 DOI: 10.1021/ja404449g Supporting Info |
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Conversion of Cyclic Ketones to 2,3-Fused Pyrroles and Substituted Indoles Joshua S. Alford, Jillian E. Spangler, and Huw M. L. Davies pp 11712–11715 DOI: 10.1021/ja405043g Supporting Info |
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Electrodeposition of a Pt Monolayer Film: Using Kinetic Limitations for Atomic Layer Epitaxy Sylvain Brimaud and R. Jürgen Behm pp 11716–11719 DOI: 10.1021/ja4051795 Supporting Info |
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Enhanced Catalytic Activity through the Tuning of Micropore Environment and Supercritical CO2 Processing: Al(Porphyrin)-Based Porous Organic Polymers for the Degradation of a Nerve Agent Simulant Ryan K. Totten, Ye-Seong Kim, Mitchell H. Weston, Omar K. Farha, Joseph T. Hupp, and SonBinh T. Nguyen pp 11720–11723 DOI: 10.1021/ja405495u Supporting Info |
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Impact of Molecular Symmetry on Single-Molecule Conductance Emma J. Dell, Brian Capozzi, Kateri H. DuBay, Timothy C. Berkelbach, Jose Ricardo Moreno, David R. Reichman, Latha Venkataraman, and Luis M. Campos pp 11724–11727 DOI: 10.1021/ja4055367 Supporting Info |
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Direct Microwave-Assisted Hydrothermal Depolymerization of Cellulose Jiajun Fan, Mario De bruyn, Vitaliy L. Budarin, Mark J. Gronnow, Peter S. Shuttleworth, Simon Breeden, Duncan J. Macquarrie, and James H. Clark pp 11728–11731 DOI: 10.1021/ja4056273 Supporting Info |
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The Conformation of P450cam in Complex with Putidaredoxin Is Dependent on Oxidation State William K. Myers, Young-Tae Lee, R. David Britt, and David B. Goodin pp 11732–11735 DOI: 10.1021/ja405751z Supporting Info |
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Rapid, Reversible Heterolytic Cleavage of Bound H2 Elliott B. Hulley, Kevin D. Welch, Aaron M. Appel, Daniel L. DuBois, and R. Morris Bullock pp 11736–11739 DOI: 10.1021/ja405755j Supporting Info |
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Chiral Phosphoric Acid-Catalyzed Oxidative Kinetic Resolution of Indolines Based on Transfer Hydrogenation to Imines Kodai Saito, Yukihiro Shibata, Masahiro Yamanaka, and Takahiko Akiyama pp 11740–11743 DOI: 10.1021/ja406004q Supporting Info |
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Cobalt–Salen Complex-Catalyzed Oxidative Generation of Alkyl Radicals from Aldehydes for the Preparation of Hydroperoxides Eiichi Watanabe, Atsushi Kaiho, Hiroyuki Kusama, and Nobuharu Iwasawa pp 11744–11747 DOI: 10.1021/ja406028c Supporting Info |
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Interplay among Subunit Identity, Subunit Proportion, Chain Length, and Stereochemistry in the Activity Profile of Sequence-Random Peptide Mixtures Zvi Hayouka, Saswata Chakraborty, Runhui Liu, Melissa D. Boersma, Bernard Weisblum, and Samuel H. Gellman pp 11748–11751 DOI: 10.1021/ja406231b Supporting Info |
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Transformation of Pd Nanocubes into Octahedra with Controlled Sizes by Maneuvering the Rates of Etching and Regrowth Maochang Liu, Yiqun Zheng, Lei Zhang, Liejin Guo, and Younan Xia pp 11752–11755 DOI: 10.1021/ja406344j Supporting Info |
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Enantioselective α-Alkenylation of Aldehydes with Boronic Acids via the Synergistic Combination of Copper(II) and Amine Catalysis Jason M. Stevens and David W. C. MacMillan pp 11756–11759 DOI: 10.1021/ja406356c Supporting Info |
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Photocontrol over Cucurbit[8]uril Complexes: Stoichiometry and Supramolecular Polymers Jesús del Barrio, Peter N. Horton, Didier Lairez, Gareth O. Lloyd, Chris Toprakcioglu, and Oren A. Scherman pp 11760–11763 DOI: 10.1021/ja406556h Supporting Info |
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A Unified Strategy to ent-Kauranoid Natural Products: Total Syntheses of (−)-Trichorabdal A and (−)-Longikaurin E John T. S. Yeoman, Victor W. Mak, and Sarah E. Reisman pp 11764–11767 DOI: 10.1021/ja406599a Supporting Info |
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“NMR Chemosensing” Using Monolayer-Protected Nanoparticles as Receptors Barbara Perrone, Sara Springhetti, Federico Ramadori, Federico Rastrelli, and Fabrizio Mancin pp 11768–11771 DOI: 10.1021/ja406688a Supporting Info |
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Diaminophosphine Oxide Ligand Enabled Asymmetric Nickel-Catalyzed Hydrocarbamoylations of Alkenes Pavel A. Donets and Nicolai Cramer pp 11772–11775 DOI: 10.1021/ja406730t Supporting Info |
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Activation of Water, Ammonia, and Other Small Molecules by PCcarbeneP Nickel Pincer Complexes Dmitry V. Gutsulyak, Warren E. Piers, Javier Borau-Garcia, and Masood Parvez pp 11776–11779 DOI: 10.1021/ja406742n Supporting Info |
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The Osmium–Silicon Triple Bond: Synthesis, Characterization, and Reactivity of an Osmium Silylyne Complex Paul G. Hayes, Zhenggang Xu, Chad Beddie, Jason M. Keith, Michael B. Hall, and T. Don Tilley pp 11780–11783 DOI: 10.1021/ja406799y Supporting Info |
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Layered Silicate as an Excellent Partner of a TiO2 Photocatalyst for Efficient and Selective Green Fine-Chemical Synthesis Yusuke Ide, Masato Torii, and Tsuneji Sano pp 11784–11786 DOI: 10.1021/ja406855e Supporting Info |
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New Roles for 1,1-Diamino-2,2-dinitroethene (FOX-7): Halogenated FOX-7 and Azo-bis(diahaloFOX) as Energetic Materials and Oxidizers Thao T. Vo, Jiaheng Zhang, Damon A. Parrish, Brendan Twamley, and Jean’ne M. Shreeve pp 11787–11790 DOI: 10.1021/ja406629g Supporting Info |
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Facile N–H Bond Cleavage of Ammonia by an Iridium Complex Bearing a Noninnocent PNP-Pincer Type Phosphaalkene Ligand Yung-Hung Chang, Yumiko Nakajima, Hiromasa Tanaka, Kazunari Yoshizawa, and Fumiyuki Ozawa pp 11791–11794 DOI: 10.1021/ja407163z Supporting Info |
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A Fragile Zwitterionic Phosphasilene as a Transfer Agent of the Elusive Parent Phosphinidene (:PH) Kerstin Hansen, Tibor Szilvási, Burgert Blom, Shigeyoshi Inoue, Jan Epping, and Matthias Driess pp 11795–11798 DOI: 10.1021/ja4072699 Supporting Info |
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Cyclopropenimine-Catalyzed Enantioselective Mannich Reactions of tert-Butyl Glycinates with N-Boc-Imines Jeffrey S. Bandar and Tristan H. Lambert pp 11799–11802 DOI: 10.1021/ja407277a Supporting Info |
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Experimentally Quantifying Small-Molecule Bond Activation Using Valence-to-Core X-ray Emission Spectroscopy Christopher J. Pollock, Katarzyna Grubel, Patrick L. Holland, and Serena DeBeer pp 11803–11808 DOI: 10.1021/ja3116247 Supporting Info |
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Redox-Dependent Structural Transformations of the [4Fe-3S] Proximal Cluster in O2-Tolerant Membrane-Bound [NiFe]-Hydrogenase: A DFT Study Vladimir Pelmenschikov and Martin Kaupp pp 11809–11823 DOI: 10.1021/ja402159u Supporting Info |
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Mechanisms of Acceleration and Retardation of Water Dynamics by Ions Guillaume Stirnemann, Erik Wernersson, Pavel Jungwirth, and Damien Laage pp 11824–11831 DOI: 10.1021/ja405201s Supporting Info |
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Graphene Oxide/Nucleic-Acid-Stabilized Silver Nanoclusters: Functional Hybrid Materials for Optical Aptamer Sensing and Multiplexed Analysis of Pathogenic DNAs Xiaoqing Liu, Fuan Wang, Ruth Aizen, Omer Yehezkeli, and Itamar Willner pp 11832–11839 DOI: 10.1021/ja403485r Supporting Info |
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Ca1–xRExAg1–ySb (RE = La, Ce, Pr, Nd, Sm; 0 ≤ x ≤1; 0 ≤ y ≤1): Interesting Structural Transformation and Enhanced High-Temperature Thermoelectric Performance Jian Wang, Xiao-Cun Liu, Sheng-Qing Xia, and Xu-Tang Tao pp 11840–11848 DOI: 10.1021/ja403653m Supporting Info |
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Aggregation-Free Gold Nanoparticles in Ordered Mesoporous Carbons: Toward Highly Active and Stable Heterogeneous Catalysts Shuai Wang, Qingfei Zhao, Huimin Wei, Jian-Qiang Wang, Minhyung Cho, Hae Sung Cho, Osamu Terasaki, and Ying Wan pp 11849–11860 DOI: 10.1021/ja403822d Supporting Info |
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Photofunctional Construct That Interfaces Molecular Cobalt-Based Catalysts for H2 Production to a Visible-Light-Absorbing Semiconductor Alexandra Krawicz, Jinhui Yang, Eitan Anzenberg, Junko Yano, Ian D. Sharp, and Gary F. Moore pp 11861–11868 DOI: 10.1021/ja404158r Supporting Info |
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Multiplexed Electrochemistry of DNA-Bound Metalloproteins Catrina G. Pheeney, Anna R. Arnold, Michael A. Grodick, and Jacqueline K. Barton pp 11869–11878 DOI: 10.1021/ja4041779 Supporting Info |
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Mechanical Control of Renilla Luciferase Chiao-Yu Tseng and Giovanni Zocchi pp 11879–11886 DOI: 10.1021/ja4043565 |
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Methane Storage in Metal–Organic Frameworks: Current Records, Surprise Findings, and Challenges Yang Peng, Vaiva Krungleviciute, Ibrahim Eryazici, Joseph T. Hupp, Omar K. Farha, and Taner Yildirim pp 11887–11894 DOI: 10.1021/ja4045289 Supporting Info |
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Hydrogen Activation by Biomimetic [NiFe]-Hydrogenase Model Containing Protected Cyanide Cofactors Brian C. Manor and Thomas B. Rauchfuss pp 11895–11900 DOI: 10.1021/ja404580r Supporting Info |
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Charge Transfer Structure–Reactivity Dependence of Fullerene–Single-Walled Carbon Nanotube Heterojunctions Andrew J. Hilmer, Kevin Tvrdy, Jingqing Zhang, and Michael S. Strano pp 11901–11910 DOI: 10.1021/ja404636b Supporting Info |
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Native Chemical Ligation at Asx-Cys, Glx-Cys: Chemical Synthesis and High-Resolution X-ray Structure of ShK Toxin by Racemic Protein Crystallography Bobo Dang, Tomoya Kubota, Kalyaneswar Mandal, Francisco Bezanilla, and Stephen B. H. Kent pp 11911–11919 DOI: 10.1021/ja4046795 Supporting Info |
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Efficient Energy Sensitization of C60 and Application to Organic Photovoltaics Cong Trinh, Kent O. Kirlikovali, Andrew N. Bartynski, Christopher J. Tassone, Michael F. Toney, George F. Burkhard, Michael D. McGehee, Peter I. Djurovich, and Mark E. Thompson pp 11920–11928 DOI: 10.1021/ja4043356 Supporting Info |
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Molecular Crowding Stabilizes Both the Intrinsically Disordered Calcium-Free State and the Folded Calcium-Bound State of a Repeat in Toxin (RTX) Protein Ana-Cristina Sotomayor-Pérez, Orso Subrini, Audrey Hessel, Daniel Ladant, and Alexandre Chenal pp 11929–11934 DOI: 10.1021/ja404790f Supporting Info |
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Rational Design of DNA Motors: Fuel Optimization through Single-Molecule Fluorescence Toma E. Tomov, Roman Tsukanov, Miran Liber, Rula Masoud, Noa Plavner, and Eyal Nir pp 11935–11941 DOI: 10.1021/ja4048416 Supporting Info |
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Nonlinear Active Materials: An Illustration of Controllable Phase Matchability Hongcheng Lu, Romain Gautier, Martin D. Donakowski, T.Thao Tran, Bryce W. Edwards, Juan C. Nino, P. Shiv Halasyamani, Zhengtang Liu, and Kenneth R. Poeppelmeier pp 11942–11950 DOI: 10.1021/ja4050604 Supporting Info |
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Practical and Highly Selective Sulfur Ylide-Mediated Asymmetric Epoxidations and Aziridinations Using a Cheap and Readily Available Chiral Sulfide: Extensive Studies To Map Out Scope, Limitations, and Rationalization of Diastereo- and Enantioselectivities Ona Illa, Mariam Namutebi, Chandreyee Saha, Mehrnoosh Ostovar, C. Chun Chen, Mairi F. Haddow, Sophie Nocquet-Thibault, Matteo Lusi, Eoghan M. McGarrigle, and Varinder K. Aggarwal pp 11951–11966 DOI: 10.1021/ja405073w Supporting Info |
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Additive Effect on Reductive Decomposition and Binding of Carbonate-Based Solvent toward Solid Electrolyte Interphase Formation in Lithium-Ion Battery Keisuke Ushirogata, Keitaro Sodeyama, Yukihiro Okuno, and Yoshitaka Tateyama pp 11967–11974 DOI: 10.1021/ja405079s Supporting Info |
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Synthesis, Structure, and Optical Activity of HPM-1, a Pure Silica Chiral Zeolite Alex Rojas, Oriol Arteaga, Bart Kahr, and Miguel A. Camblor pp 11975–11984 DOI: 10.1021/ja405088c Supporting Info |
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Synthesis of a Single G-Quartet Platform in Water Grant A. L. Bare, Bo Liu, and John C. Sherman pp 11985–11989 DOI: 10.1021/ja405100z Supporting Info |
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Screening Bicyclic Peptide Libraries for Protein–Protein Interaction Inhibitors: Discovery of a Tumor Necrosis Factor-α Antagonist Wenlong Lian, Punit Upadhyaya, Curran A. Rhodes, Yusen Liu, and Dehua Pei pp 11990–11995 DOI: 10.1021/ja405106u Supporting Info |
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Fast CO2 Sequestration, Activation, and Catalytic Transformation Using N-Heterocyclic Olefins Yan-Bo Wang, Yi-Ming Wang, Wen-Zhen Zhang, and Xiao-Bing Lu pp 11996–12003 DOI: 10.1021/ja405114e Supporting Info |
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Bimetallic Oxidative Addition Involving Radical Intermediates in Nickel-Catalyzed Alkyl–Alkyl Kumada Coupling Reactions Jan Breitenfeld, Jesus Ruiz, Matthew D. Wodrich, and Xile Hu pp 12004–12012 DOI: 10.1021/ja4051923 Supporting Info |
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In Vitro and Cellular Self-Assembly of a Zn-Binding Protein Cryptand via Templated Disulfide Bonds Annette Medina-Morales, Alfredo Perez, Jeffrey D. Brodin, and F. Akif Tezcan pp 12013–12022 DOI: 10.1021/ja405318d Supporting Info |
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Selective Nitrite Reduction at Heterobimetallic CoMg Complexes Christopher Uyeda and Jonas C. Peters pp 12023–12031 DOI: 10.1021/ja4053653 Supporting Info |
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Catalyst-Controlled C–O versus C–N Allylic Functionalization of Terminal Olefins Iulia I. Strambeanu and M. Christina White pp 12032–12037 DOI: 10.1021/ja405394v Supporting Info |
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Discovery and Characterization of an Isopeptidase That Linearizes Lasso Peptides Mikhail O. Maksimov and A. James Link pp 12038–12047 DOI: 10.1021/ja4054256 Supporting Info |
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Toward an Ideal Polymer Binder Design for High-Capacity Battery Anodes Mingyan Wu, Xingcheng Xiao, Nenad Vukmirovic, Shidi Xun, Prodip K. Das, Xiangyun Song, Paul Olalde-Velasco, Dongdong Wang, Adam Z. Weber, Lin-Wang Wang, Vincent S. Battaglia, Wanli Yang, and Gao Liu pp 12048–12056 DOI: 10.1021/ja4054465 Supporting Info |
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Predicting Morphologies of Solution Processed Polymer:Fullerene Blends Sandra Kouijzer, Jasper J. Michels, Mauricio van den Berg, Veronique S. Gevaerts, Mathieu Turbiez, Martijn M. Wienk, and René A. J. Janssen pp 12057–12067 DOI: 10.1021/ja405493j Supporting Info |
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Temperature-Induced Structural Phase Transitions in a Two-Dimensional Self-Assembled Network Matthew O. Blunt, Jinne Adisoejoso, Kazukuni Tahara, Keisuke Katayama, Mark Van der Auweraer, Yoshito Tobe, and Steven De Feyter pp 12068–12075 DOI: 10.1021/ja405585s Supporting Info |
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Insertion of Reactive Rhodium Carbenes into Boron–Hydrogen Bonds of Stable N-Heterocyclic Carbene Boranes Xiben Li and Dennis P. Curran pp 12076–12081 DOI: 10.1021/ja4056245 Supporting Info |
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Toward Oriented Surface Architectures with Three Coaxial Charge-Transporting Pathways Giuseppe Sforazzini, Edvinas Orentas, Altan Bolag, Naomi Sakai, and Stefan Matile pp 12082–12090 DOI: 10.1021/ja405776a Supporting Info |
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Interplay of Self-Association and Solvation in Polar Liquids Valeria Amenta, Joanne L. Cook, Christopher A. Hunter, Caroline M. R. Low, Hongmei Sun, and Jeremy G. Vinter pp 12091–12100 DOI: 10.1021/ja405799q Supporting Info |
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Tuning Uranium–Nitrogen Multiple Bond Formation with Ancillary Siloxide Ligands Clément Camp, Jacques Pécaut, and Marinella Mazzanti pp 12101–12111 DOI: 10.1021/ja405815b Supporting Info |
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Urea-Induced Denaturation of PreQ1-Riboswitch Jeseong Yoon, D. Thirumalai, and Changbong Hyeon pp 12112–12121 DOI: 10.1021/ja406019s Supporting Info |
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Radical-Based Regioselective C–H Functionalization of Electron-Deficient Heteroarenes: Scope, Tunability, and Predictability Fionn O’Hara, Donna G. Blackmond, and Phil S. Baran pp 12122–12134 DOI: 10.1021/ja406223k Supporting Info |
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Stereoselective Synthesis of β-Alkylated α-Amino Acids via Palladium-Catalyzed Alkylation of Unactivated Methylene C(sp3)–H Bonds with Primary Alkyl Halides Shu-Yu Zhang, Qiong Li, Gang He, William A. Nack, and Gong Chen pp 12135–12141 DOI: 10.1021/ja406484v Supporting Info |
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Free Radical Coupling of o-Semiquinones Uncovered Alessandro Pezzella, Orlando Crescenzi, Lucia Panzella, Alessandra Napolitano, Edward J. Land, Vincenzo Barone, and Marco d’Ischia pp 12142–12149 DOI: 10.1021/ja4067332 Supporting Info |
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Addition to “The Role of Arene–Arene Interactions in the Folding of ortho-Phenylenes” Sanyo M. Mathew, James T. Engle, Christopher J. Ziegler, and C. Scott Hartley pp 12150–12150 DOI: 10.1021/ja406543a Supporting Info |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 12151–12151 DOI: 10.1021/ja408390h |
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Characterizing Amosamine Biosynthesis in Amicetin Reveals AmiG as a Reversible Retaining Glycosyltransferase Ruidong Chen, Haibo Zhang, Gaiyun Zhang, Sumei Li, Guangtao Zhang, Yiguang Zhu, Jinsong Liu, and Changsheng Zhang pp 12152–12155 DOI: 10.1021/ja401016e Supporting Info |
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Rapid Cross-Metathesis for Reversible Protein Modifications via Chemical Access to Se-Allyl-selenocysteine in Proteins Yuya A. Lin, Omar Boutureira, Lukas Lercher, Bhaskar Bhushan, Robert S. Paton, and Benjamin G. Davis pp 12156–12159 DOI: 10.1021/ja403191g Supporting Info |
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Procedure-Controlled Enantioselectivity Switch in Organocatalytic 2-Oxazolidinone Synthesis Yukihiro Fukata, Keisuke Asano, and Seijiro Matsubara pp 12160–12163 DOI: 10.1021/ja407027e Supporting Info |
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Metal Ion Sensing Using Ion Chemical Exchange Saturation Transfer 19F Magnetic Resonance Imaging Amnon Bar-Shir, Assaf A. Gilad, Kannie W. Y. Chan, Guanshu Liu, Peter C. M. van Zijl, Jeff W. M. Bulte, and Michael T. McMahon pp 12164–12167 DOI: 10.1021/ja403542g Supporting Info |
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Electron-Deficient Poly(p-phenylene vinylene) Provides Electron Mobility over 1 cm2 V–1 s–1 under Ambient Conditions Ting Lei, Jin-Hu Dou, Xiao-Yu Cao, Jie-Yu Wang, and Jian Pei pp 12168–12171 DOI: 10.1021/ja403624a Supporting Info |
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Molecular Threading and Tunable Molecular Recognition on DNA Origami Nanostructures Na Wu, Daniel M. Czajkowsky, Jinjin Zhang, Jianxun Qu, Ming Ye, Dongdong Zeng, Xingfei Zhou, Jun Hu, Zhifeng Shao, Bin Li, and Chunhai Fan pp 12172–12175 DOI: 10.1021/ja403863a Supporting Info |
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Optical Fusion Assay Based on Membrane-Coated Spheres in a 2D Assembly Chunxiao Bao, Gesa Pähler, Burkhard Geil, and Andreas Janshoff pp 12176–12179 DOI: 10.1021/ja404071z Supporting Info |
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Multi-Armed Micelles and Block Co-micelles via Crystallization-Driven Self-Assembly with Homopolymer Nanocrystals as Initiators Huibin Qiu, Graeme Cambridge, Mitchell A. Winnik, and Ian Manners pp 12180–12183 DOI: 10.1021/ja404100w Supporting Info |
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Introducing Defects into Metal-Seamed Nanocapsules Using Mixed Macrocycles Drew A. Fowler, Asanka S. Rathnayake, Stuart Kennedy, Harshita Kumari, Christine M. Beavers, Simon J. Teat, and Jerry L. Atwood pp 12184–12187 DOI: 10.1021/ja404392m Supporting Info |
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Cyclopentannulation of Conjugated Enones Using a Vinyldiazomethane-Based Reagent Matthew Del Bel, Alexander Rovira, and Carlos A. Guerrero pp 12188–12191 DOI: 10.1021/ja4054866 Supporting Info |
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Palladium-Catalyzed Selective Fluorination of o-Carboranes Zaozao Qiu, Yangjian Quan, and Zuowei Xie pp 12192–12195 DOI: 10.1021/ja405808t Supporting Info |
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Anisotropic Nanoparticles as Shape-Directing Catalysts for the Chemical Etching of Silicon Guoliang Liu, Kaylie L. Young, Xing Liao, Michelle L. Personick, and Chad A. Mirkin pp 12196–12199 DOI: 10.1021/ja4061867 Supporting Info |
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Stereodynamic Chemosensor with Selective Circular Dichroism and Fluorescence Readout for in Situ Determination of Absolute Configuration, Enantiomeric Excess, and Concentration of Chiral Compounds Keith W. Bentley and Christian Wolf pp 12200–12203 DOI: 10.1021/ja406259p Supporting Info |
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Rh(III)-Catalyzed Synthesis of Multisubstituted Isoquinoline and Pyridine N-Oxides from Oximes and Diazo Compounds Zhuangzhi Shi, Dennis C. Koester, Mélissa Boultadakis-Arapinis, and Frank Glorius pp 12204–12207 DOI: 10.1021/ja406338r Supporting Info |
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Murahashi Coupling Polymerization: Nickel(II)–N-Heterocyclic Carbene Complex-Catalyzed Polycondensation of Organolithium Species of (Hetero)arenes Kanta Fuji, Shunsuke Tamba, Keisuke Shono, Atsushi Sugie, and Atsunori Mori pp 12208–12211 DOI: 10.1021/ja406374t Supporting Info |
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Molecular Origin of Rapid versus Slow Intramolecular Electron Transfer in the Catalytic Cycle of the Multicopper Oxidases David E. Heppner, Christian H. Kjaergaard, and Edward I. Solomon pp 12212–12215 DOI: 10.1021/ja4064525 Supporting Info |
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Volatile Heterometallic Precursors for the Low-Temperature Synthesis of Prospective Sodium Ion Battery Cathode Materials Zheng Wei, Alexander S. Filatov, and Evgeny V. Dikarev pp 12216–12219 DOI: 10.1021/ja4069529 Supporting Info |
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Defect-Dominated Shape Recovery of Nanocrystals: A New Strategy for Trimetallic Catalysts Yuen Wu, Dingsheng Wang, Xiaobin Chen, Gang Zhou, Rong Yu, and Yadong Li pp 12220–12223 DOI: 10.1021/ja4068063 Supporting Info |
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Double-Gate Light-Emitting Electrochemical Transistor: Confining the Organic p–n Junction Jiang Liu, Isak Engquist, and Magnus Berggren pp 12224–12227 DOI: 10.1021/ja407049b Supporting Info |
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Single-Molecule Conductance of Functionalized Oligoynes: Length Dependence and Junction Evolution Pavel Moreno-García, Murat Gulcur, David Zsolt Manrique, Thomas Pope, Wenjing Hong, Veerabhadrarao Kaliginedi, Cancan Huang, Andrei S. Batsanov, Martin R. Bryce, Colin Lambert, and Thomas Wandlowski pp 12228–12240 DOI: 10.1021/ja4015293 Supporting Info |
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Biomimetic Crystalline Actuators: Structure–Kinematic Aspects of the Self-Actuation and Motility of Thermosalient Crystals Subash Chandra Sahoo, Manas K. Panda, Naba K. Nath, and Panče Naumov pp 12241–12251 DOI: 10.1021/ja404192g Supporting Info |
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Semisynthetic Lectin–4-Dimethylaminopyridine Conjugates for Labeling and Profiling Glycoproteins on Live Cell Surfaces Takahiro Hayashi, Yedi Sun, Tomonori Tamura, Keiko Kuwata, Zhining Song, Yousuke Takaoka, and Itaru Hamachi pp 12252–12258 DOI: 10.1021/ja4043214 Supporting Info |
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Analyzing Structure–Photophysical Property Relationships for Isolated T8, T10, and T12 Stilbenevinylsilsesquioxanes Joseph C. Furgal, Jae Hwan Jung, Theodore Goodson, III, and Richard M. Laine pp 12259–12269 DOI: 10.1021/ja4043092 Supporting Info |
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Synthesis of Uniform Disk-Shaped Copper Telluride Nanocrystals and Cation Exchange to Cadmium Telluride Quantum Disks with Stable Red Emission Hongbo Li, Rosaria Brescia, Mauro Povia, Mirko Prato, Giovanni Bertoni, Liberato Manna, and Iwan Moreels pp 12270–12278 DOI: 10.1021/ja404694k Supporting Info |
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Insights into the Glycyl Radical Enzyme Active Site of Benzylsuccinate Synthase: A Computational Study Vivek S. Bharadwaj, Anthony M. Dean, and C. Mark Maupin pp 12279–12288 DOI: 10.1021/ja404842r Supporting Info |
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Testing the Polynuclear Hypothesis: Multielectron Reduction of Small Molecules by Triiron Reaction Sites Tamara M. Powers and Theodore A. Betley pp 12289–12296 DOI: 10.1021/ja405057n Supporting Info |
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Extensive Reprogramming of the Genetic Code for Genetically Encoded Synthesis of Highly N-Alkylated Polycyclic Peptidomimetics Takashi Kawakami, Takahiro Ishizawa, and Hiroshi Murakami pp 12297–12304 DOI: 10.1021/ja405044k Supporting Info |
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Precision vs Flexibility in GPCR signaling Matthias Elgeti, Alexander S. Rose, Franz J. Bartl, Peter W. Hildebrand, Klaus-Peter Hofmann, and Martin Heck pp 12305–12312 DOI: 10.1021/ja405133k Supporting Info |
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Clathrate Ba8Au16P30: The “Gold Standard” for Lattice Thermal Conductivity James Fulmer, Oleg I. Lebedev, Vladimir V. Roddatis, Derrick C. Kaseman, Sabyasachi Sen, Juli-Anna Dolyniuk, Kathleen Lee, Andrei V. Olenev, and Kirill Kovnir pp 12313–12323 DOI: 10.1021/ja4052679 Supporting Info |
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Phase Separation Polymerization of Dicyclopentadiene Characterized by In Operando Fluorescence Microscopy Eva M. Hensle and Suzanne A. Blum pp 12324–12328 DOI: 10.1021/ja405283k Supporting Info |
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An Investigation of Thin-Film Ni–Fe Oxide Catalysts for the Electrochemical Evolution of Oxygen Mary W. Louie and Alexis T. Bell pp 12329–12337 DOI: 10.1021/ja405351s Supporting Info |
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Oriented Gold Nanoparticle Aggregation for Colorimetric Sensors with Surprisingly High Analytical Figures of Merit Longhua Guo, Yang Xu, Abdul Rahim Ferhan, Guonan Chen, and Dong-Hwan Kim pp 12338–12345 DOI: 10.1021/ja405371g |
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Complementation of Biotransformations with Chemical C–H Oxidation: Copper-Catalyzed Oxidation of Tertiary Amines in Complex Pharmaceuticals Julien Genovino, Stephan Lütz, Dalibor Sames, and B. Barry Touré pp 12346–12352 DOI: 10.1021/ja405471h Supporting Info |
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Chiral Colloidal Molecules And Observation of The Propeller Effect Debora Schamel, Marcel Pfeifer, John G. Gibbs, Björn Miksch, Andrew G. Mark, and Peer Fischer pp 12353–12359 DOI: 10.1021/ja405705x Supporting Info |
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Development of Fluorogenic Probes for Quick No-Wash Live-Cell Imaging of Intracellular Proteins Yuichiro Hori, Tomoya Norinobu, Motoki Sato, Kyohei Arita, Masahiro Shirakawa, and Kazuya Kikuchi pp 12360–12365 DOI: 10.1021/ja405745v Supporting Info |
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Mycobacterium tuberculosis Shikimate Kinase Inhibitors: Design and Simulation Studies of the Catalytic Turnover Beatriz Blanco, Verónica Prado, Emilio Lence, José M. Otero, Carmela Garcia-Doval, Mark J. van Raaij, Antonio L. Llamas-Saiz, Heather Lamb, Alastair R. Hawkins, and Concepción González-Bello pp 12366–12376 DOI: 10.1021/ja405853p Supporting Info |
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Manifestation of Polar Reaction Pathways of 2,3-Dichloro-5,6-dicyano-p-benzoquinone Xingwei Guo and Herbert Mayr pp 12377–12387 DOI: 10.1021/ja405890d Supporting Info |
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Rational Design of Monocrystalline (InP)yGe5–2y/Ge/Si(100) Semiconductors: Synthesis and Optical Properties Patrick E. Sims, Andrew V.G. Chizmeshya, Liying Jiang, Richard T. Beeler, Christian D. Poweleit, James Gallagher, David J. Smith, José Menéndez, and John Kouvetakis pp 12388–12399 DOI: 10.1021/ja405726b |
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Characterization of Cyclopentyllithium and Cyclopentyllithium Tetrahydrofuran Complex Chicheung Su, Russell Hopson, and Paul G. Williard pp 12400–12406 DOI: 10.1021/ja4059102 Supporting Info |
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Syntheses and Structural Characterizations of Inorganic ansa-Metallocene Analogues: ansa-Ferratricarbadecaboranes Brendan Gleeson, Patrick J. Carroll, and Larry G. Sneddon pp 12407–12413 DOI: 10.1021/ja405977q Supporting Info |
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Asymmetric Catalysis at a Distance: Catalytic, Site-Selective Phosphorylation of Teicoplanin Sunkyu Han and Scott J. Miller pp 12414–12421 DOI: 10.1021/ja406067v Supporting Info |
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Acyclic Germylones: Congeners of Allenes with a Central Germanium Atom Yan Li, Kartik Chandra Mondal, Herbert W. Roesky, Hongping Zhu, Peter Stollberg, Regine Herbst-Irmer, Dietmar Stalke, and Diego M. Andrada pp 12422–12428 DOI: 10.1021/ja406112u Supporting Info |
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A “Turn-On” Fluorescent Sensor for Methylglyoxal Tina Wang, Eugene F. Douglass, Jr., Kelly J. Fitzgerald, and David A. Spiegel pp 12429–12433 DOI: 10.1021/ja406077j Supporting Info |
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Stereoselective Total Synthesis of Hainanolidol and Harringtonolide via Oxidopyrylium-Based [5 + 2] Cycloaddition Min Zhang, Na Liu, and Weiping Tang pp 12434–12438 DOI: 10.1021/ja406255j Supporting Info |
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Catalytic Asymmetric Syntheses of Quinolizidines by Dirhodium-Catalyzed Dearomatization of Isoquinolinium/Pyridinium Methylides–The Role of Catalyst and Carbene Source Xichen Xu, Peter Y. Zavalij, and Michael P. Doyle pp 12439–12447 DOI: 10.1021/ja406482q Supporting Info |
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Iridium(I) Complexes with Anionic N-Heterocyclic Carbene Ligands as Catalysts for the Hydrogenation of Alkenes in Nonpolar Media Eugene L. Kolychev, Sabrina Kronig, Kai Brandhorst, Matthias Freytag, Peter G. Jones, and Matthias Tamm pp 12448–12459 DOI: 10.1021/ja406529c Supporting Info |
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Structures of Oligomers of a Peptide from β-Amyloid Johnny D. Pham, Nicholas Chim, Celia W. Goulding, and James S. Nowick pp 12460–12467 DOI: 10.1021/ja4068854 Supporting Info |
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The Realistic Domain Structure of As-Synthesized Graphene Oxide from Ultrafast Spectroscopy Qun Zhang, Hongjun Zheng, Zhigang Geng, Shenlong Jiang, Jing Ge, Kaili Fan, Sai Duan, Yang Chen, Xiaoping Wang, and Yi Luo pp 12468–12474 DOI: 10.1021/ja407110r Supporting Info |
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Retraction of Highly Enantioselective Radical Addition to N-Benzoyl Hydrazones Using Chiral Ammonium Salts Doo Ok Jang and Sang Yoon Kim pp 12475–12475 DOI: 10.1021/ja406816b |
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Correction to “Integration of Gold Nanoparticles into Bilayer Structures via Adaptive Surface Chemistry” Hee-Young Lee, Sun Hae Ra Shin, Ludmila Abezgauz, Sean A. Lewis, Aaron M. Chirsan, Dganit Danino, and Kyle J. M. Bishop pp 12476–12476 DOI: 10.1021/ja407234h |
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Correction to “Crystallographic Characterization of N-Oxide Tripod Amphiphiles” Pil Seok Chae, Ilia A. Guzei, and Samuel H. Gellman pp 12477–12477 DOI: 10.1021/ja407246v |
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Correction to “Dyotropic Rearrangements of Fused Tricyclic β-Lactones: Application to the Synthesis of (−)-Curcumanolide A and (−)-Curcumalactone” Carolyn A. Leverett, Vikram C. Purohit, Alex G. Johnson, Rebecca L. Davis, Dean J. Tantillo, and Daniel Romo pp 12478–12478 DOI: 10.1021/ja407284g |
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Spotlights on JACS Publications ACS Contributing Correspondents pp 12479–12479 DOI: 10.1021/ja408622p |
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Biocatalysis in Organic Chemistry and Biotechnology: Past, Present, and Future Manfred T. Reetz pp 12480–12496 DOI: 10.1021/ja405051f |
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M12L24 Spheres with Endo and Exo Coordination Sites: Scaffolds for Non-Covalent Functionalization Kate Harris, Qing-Fu Sun, Sota Sato, and Makoto Fujita pp 12497–12499 DOI: 10.1021/ja4043609 Supporting Info |
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Inverse Kinetic Isotope Effect in the Excited-State Relaxation of a Ru(II)–Aquo Complex: Revealing the Impact of Hydrogen-Bond Dynamics on Nonradiative Decay Joshua T. Hewitt, Javier J. Concepcion, and Niels H. Damrauer pp 12500–12503 DOI: 10.1021/ja4037498 Supporting Info |
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Neighboring-Cation Substitution Tuning of Photoluminescence by Remote-Controlled Activator in Phosphor Lattice Siao-Shan Wang, Wei-Ting Chen, Ye Li, Jing Wang, Hwo-Shuenn Sheu, and Ru-Shi Liu pp 12504–12507 DOI: 10.1021/ja404510v Supporting Info |
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Autotransfecting Short Interfering RNA through Facile Covalent Polymer Escorts Saadyah E. Averick, Eduardo Paredes, Sourav K. Dey, Kristin M. Snyder, Nikos Tapinos, Krzysztof Matyjaszewski, and Subha R. Das pp 12508–12511 DOI: 10.1021/ja404520j Supporting Info |
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Mg2+ Tunes the Wettability of Liquid Precursors of CaCO3: Toward Controlling Mineralization Sites in Hybrid Materials John K. Berg, Thomas Jordan, Yvonne Binder, Hans G. Börner, and Denis Gebauer pp 12512–12515 DOI: 10.1021/ja404979z Supporting Info |
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Design of a Photoswitchable Cadherin Ryan S. Ritterson, Kristopher M. Kuchenbecker, Michael Michalik, and Tanja Kortemme pp 12516–12519 DOI: 10.1021/ja404992r Supporting Info |
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Site-Specific Chemistry on the Microtubule Polymer Ralph E. Kleiner, Shih-Chieh Ti, and Tarun M. Kapoor pp 12520–12523 DOI: 10.1021/ja405199h Supporting Info |
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Accessibility, Reactivity, and Selectivity of Side Chains within a Channel of de Novo Peptide Assembly Antony J. Burton, Franziska Thomas, Christopher Agnew, Kieran L. Hudson, Stephen E. Halford, R. Leo Brady, and Derek N. Woolfson pp 12524–12527 DOI: 10.1021/ja4053027 Supporting Info |
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Protein-like Tertiary Folding Behavior from Heterogeneous Backbones Zachary E. Reinert, George A. Lengyel, and W. Seth Horne pp 12528–12531 DOI: 10.1021/ja405422v Supporting Info |
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Copper-Catalyzed Carboarylation of Alkynes via Vinyl Cations Andrew J. Walkinshaw, Wenshu Xu, Marcos G. Suero, and Matthew J. Gaunt pp 12532–12535 DOI: 10.1021/ja405972h Supporting Info |
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A Pd(0)-Catalyzed Direct Dehydrative Coupling of Terminal Alkynes with Allylic Alcohols To Access 1,4-Enynes Yang-Xiong Li, Qing-Qing Xuan, Li Liu, Dong Wang, Yong-Jun Chen, and Chao-Jun Li pp 12536–12539 DOI: 10.1021/ja406025p Supporting Info |
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A Genetically Encoded Fluorescent Probe in Mammalian Cells Abhishek Chatterjee, Jiantao Guo, Hyun Soo Lee, and Peter G. Schultz pp 12540–12543 DOI: 10.1021/ja4059553 Supporting Info |
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Thickness-Controlled Synthesis of Ultrathin Au Sheets and Surface Plasmonic Property Hai Li Qin, Dong Wang, Zeng Li Huang, Dong Min Wu, Zhi Cong Zeng, Bin Ren, Ke Xu, and Jian Jin pp 12544–12547 DOI: 10.1021/ja406107u Supporting Info |
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Facile Synthesis of Unsymmetrical Acridines and Phenazines by a Rh(III)-Catalyzed Amination/Cyclization/Aromatization Cascade Yajing Lian, Joshua R. Hummel, Robert G. Bergman, and Jonathan A. Ellman pp 12548–12551 DOI: 10.1021/ja406131a Supporting Info |
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Protein-Mimetic, Molecularly Imprinted Nanoparticles for Selective Binding of Bile Salt Derivatives in Water Joseph K. Awino and Yan Zhao pp 12552–12555 DOI: 10.1021/ja406089c Supporting Info |
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Shaping Crystals with Light: Crystal-to-Crystal Isomerization and Photomechanical Effect in Fluorinated Azobenzenes Oleksandr S. Bushuyev, Anna Tomberg, Tomislav Friščić, and Christopher J. Barrett pp 12556–12559 DOI: 10.1021/ja4063019 Supporting Info |
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Structure and Chemical State of the Pt(557) Surface during Hydrogen Oxidation Reaction Studied by in Situ Scanning Tunneling Microscopy and X-ray Photoelectron Spectroscopy Zhongwei Zhu, Gérôme Melaet, Stephanus Axnanda, Selim Alayoglu, Zhi Liu, Miquel Salmeron, and Gabor A Somorjai pp 12560–12563 DOI: 10.1021/ja406497s Supporting Info |
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Multiplexed Imaging of Nanoparticles in Tissues Using Laser Desorption/Ionization Mass Spectrometry Bo Yan, Sung Tae Kim, Chang Soo Kim, Krishnendu Saha, Daniel F. Moyano, Yuqing Xing, Ying Jiang, Amy L. Roberts, Felix S. Alfonso, Vincent M. Rotello, and Richard W. Vachet pp 12564–12567 DOI: 10.1021/ja406553f Supporting Info |
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Asymmetric Total Synthesis of Neoxaline Tetsuya Ideguchi, Takeshi Yamada, Tatsuya Shirahata, Tomoyasu Hirose, Akihiro Sugawara, Yoshinori Kobayashi, Satoshi O̅mura, and Toshiaki Sunazuka pp 12568–12571 DOI: 10.1021/ja406657v Supporting Info |
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Catalytic Synthesis of n-Alkyl Arenes through Alkyl Group Cross-Metathesis Graham E. Dobereiner, Jian Yuan, Richard R. Schrock, Alan S. Goldman, and Jason D. Hackenberg pp 12572–12575 DOI: 10.1021/ja4066392 Supporting Info |
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Fe-Catalyzed Regiodivergent [1,2]-Shift of α-Aryl Aldehydes Álvaro Gutiérrez-Bonet, Areli Flores-Gaspar, and Ruben Martin pp 12576–12579 DOI: 10.1021/ja4068707 Supporting Info |
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A CO-Derived Iron Dicarbyne That Releases Olefin upon Hydrogenation Daniel L. M. Suess and Jonas C. Peters pp 12580–12583 DOI: 10.1021/ja406874k Supporting Info |
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Cupration of C2F5H: Isolation, Structure, and Synthetic Applications of [K(DMF)2][(t-BuO)Cu(C2F5)]. Highly Efficient Pentafluoroethylation of Unactivated Aryl Bromides Anton Lishchynskyi and Vladimir V. Grushin pp 12584–12587 DOI: 10.1021/ja407017j Supporting Info |
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Volatile and Thermally Stable Mid to Late Transition Metal Complexes Containing α-Imino Alkoxide Ligands, a New Strongly Reducing Coreagent, and Thermal Atomic Layer Deposition of Ni, Co, Fe, and Cr Metal Films Lakmal C. Kalutarage, Philip D. Martin, Mary Jane Heeg, and Charles H. Winter pp 12588–12591 DOI: 10.1021/ja407014w Supporting Info |
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Mono(imidazolin-2-iminato) Titanium Complexes for Ethylene Polymerization at Low Amounts of Methylaluminoxane Dana Shoken, Manab Sharma, Mark Botoshansky, Matthias Tamm, and Moris S. Eisen pp 12592–12595 DOI: 10.1021/ja406925z Supporting Info |
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Symmetry-Amplified J Splittings for Quadrupolar Spin Pairs: A Solid-State NMR Probe of Homoatomic Covalent Bonds Frédéric A. Perras and David L. Bryce pp 12596–12599 DOI: 10.1021/ja407138b Supporting Info |
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Gold(I)-Catalyzed Enantioselective Carboalkoxylation of Alkynes Weiwei Zi and F. Dean Toste pp 12600–12603 DOI: 10.1021/ja407150h Supporting Info |
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Cell-Wall Remodeling by the Zinc-Protease AmpDh3 from Pseudomonas aeruginosa Mijoon Lee, Cecilia Artola-Recolons, César Carrasco-López, Siseth Martínez-Caballero, Dusan Hesek, Edward Spink, Elena Lastochkin, Weilie Zhang, Lance M. Hellman, Bill Boggess, Juan A. Hermoso, and Shahriar Mobashery pp 12604–12607 DOI: 10.1021/ja407445x Supporting Info |
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Mechanistic Investigation of Photon Upconversion in Nd3+-Sensitized Core–Shell Nanoparticles Xiaoji Xie, Nengyue Gao, Renren Deng, Qiang Sun, Qing-Hua Xu, and Xiaogang Liu pp 12608–12611 DOI: 10.1021/ja4075002 Supporting Info |
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Sulfoxides as Response Elements for Fluorescent Chemosensors Rahul S. Kathayat and Nathaniel S. Finney pp 12612–12614 DOI: 10.1021/ja407099a Supporting Info |
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Water Cluster Confinement and Methane Adsorption in the Hydrophobic Cavities of a Fluorinated Metal–Organic Framework Nour Nijem, Pieremanuele Canepa, Ushasree Kaipa, Kui Tan, Katy Roodenko, Sammer Tekarli, Jason Halbert, Iain W. H. Oswald, Ravi K. Arvapally, Chi Yang, Timo Thonhauser, Mohammad A. Omary, and Yves J. Chabal pp 12615–12626 DOI: 10.1021/ja400754p Supporting Info |
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Ionic Conductor with High Conductivity as Single-Component Electrolyte for Efficient Solid-State Dye-Sensitized Solar Cells Hong Wang, Juan Li, Feng Gong, Gang Zhou, and Zhong-Sheng Wang pp 12627–12633 DOI: 10.1021/ja401827w Supporting Info |
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CO Oxidation on Supported Single Pt Atoms: Experimental and ab Initio Density Functional Studies of CO Interaction with Pt Atom on θ-Al2O3(010) Surface Melanie Moses-DeBusk, Mina Yoon, Lawrence F. Allard, David R. Mullins, Zili Wu, Xiaofan Yang, Gabriel Veith, G. Malcolm Stocks, and Chaitanya K. Narula pp 12634–12645 DOI: 10.1021/ja401847c Supporting Info |
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Complete Protein Characterization Using Top-Down Mass Spectrometry and Ultraviolet Photodissociation Jared B. Shaw, Wenzong Li, Dustin D. Holden, Yan Zhang, Jens Griep-Raming, Ryan T. Fellers, Bryan P. Early, Paul M. Thomas, Neil L. Kelleher, and Jennifer S. Brodbelt pp 12646–12651 DOI: 10.1021/ja4029654 Supporting Info |
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X-ray Crystal Structure of rac-[Ru(phen)2dppz]2+ with d(ATGCAT)2 Shows Enantiomer Orientations and Water Ordering James P. Hall, Daniel Cook, Sara Ruiz Morte, Patrick McIntyre, Katrin Buchner, Hanna Beer, David J. Cardin, John A. Brazier, Graeme Winter, John M. Kelly, and Christine J. Cardin pp 12652–12659 DOI: 10.1021/ja403590e Supporting Info |
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Molecular Orientation of Enzymes Attached to Surfaces through Defined Chemical Linkages at the Solid–Liquid Interface Yuwei Liu, Tadeusz L. Ogorzalek, Pei Yang, McKenna M. Schroeder, E. Neil G. Marsh, and Zhan Chen pp 12660–12669 DOI: 10.1021/ja403672s Supporting Info |
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Mechanisms of the Thermal and Catalytic Redistributions, Oligomerizations, and Polymerizations of Linear Diborazanes Alasdair P. M. Robertson, Erin M. Leitao, Titel Jurca, Mairi F. Haddow, Holger Helten, Guy C. Lloyd-Jones, and Ian Manners pp 12670–12683 DOI: 10.1021/ja404247r Supporting Info |
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Synthetic Self-Localizing Ligands That Control the Spatial Location of Proteins in Living Cells Manabu Ishida, Hideaki Watanabe, Kazumasa Takigawa, Yasutaka Kurishita, Choji Oki, Akinobu Nakamura, Itaru Hamachi, and Shinya Tsukiji pp 12684–12689 DOI: 10.1021/ja4046907 Supporting Info |
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A Reductant-Resistant and Metal-Free Fluorescent Probe for Nitroxyl Applicable to Living Cells Kodai Kawai, Naoya Ieda, Kazuyuki Aizawa, Takayoshi Suzuki, Naoki Miyata, and Hidehiko Nakagawa pp 12690–12696 DOI: 10.1021/ja404757s Supporting Info |
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DNA Switches on the Two-Photon Efficiency of an Ultrabright Triphenylamine Fluorescent Probe Specific of AT Regions Blaise Dumat, Guillaume Bordeau, Elodie Faurel-Paul, Florence Mahuteau-Betzer, Nicolas Saettel, Germain Metge, Céline Fiorini-Debuisschert, Fabrice Charra, and Marie-Paule Teulade-Fichou pp 12697–12706 DOI: 10.1021/ja404422z Supporting Info |
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H4octapa-Trastuzumab: Versatile Acyclic Chelate System for 111In and 177Lu Imaging and Therapy Eric W. Price, Brian M. Zeglis, Jacqueline F. Cawthray, Caterina F. Ramogida, Nicholas Ramos, Jason S. Lewis, Michael J. Adam, and Chris Orvig pp 12707–12721 DOI: 10.1021/ja4049493 Supporting Info |
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Molecular Catch Bonds and the Anti-Hammond Effect in Polymer Mechanochemistry Sai Sriharsha M. Konda, Johnathan N. Brantley, Bibin T. Varghese, Kelly M. Wiggins, Christopher W. Bielawski, and Dmitrii E. Makarov pp 12722–12729 DOI: 10.1021/ja4051108 Supporting Info |
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Molecular Structure and Chemical Property of a Divalent Metallofullerene Yb@C2(13)-C84 Wenjun Zhang, Mitsuaki Suzuki, Yunpeng Xie, Lipiao Bao, Wenting Cai, Zdenek Slanina, Shigeru Nagase, Ming Xu, Takeshi Akasaka, and Xing Lu pp 12730–12735 DOI: 10.1021/ja405223t Supporting Info |
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Ex2Box: Interdependent Modes of Binding in a Two-Nanometer-Long Synthetic Receptor Michal Juríček, Jonathan C. Barnes, Edward J. Dale, Wei-Guang Liu, Nathan L. Strutt, Carson J. Bruns, Nicolaas A. Vermeulen, Kala C. Ghooray, Amy A. Sarjeant, Charlotte L. Stern, Youssry Y. Botros, William A. Goddard, III, and J. Fraser Stoddart pp 12736–12746 DOI: 10.1021/ja4052763 Supporting Info |
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Activated Singlet Exciton Fission in a Semiconducting Polymer Andrew J. Musser, Mohammed Al-Hashimi, Margherita Maiuri, Daniele Brida, Martin Heeney, Giulio Cerullo, Richard H. Friend, and Jenny Clark pp 12747–12754 DOI: 10.1021/ja405427j Supporting Info |
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End Group Characterization of Poly(phthalaldehyde): Surprising Discovery of a Reversible, Cationic Macrocyclization Mechanism Joshua A. Kaitz, Charles E. Diesendruck, and Jeffrey S. Moore pp 12755–12761 DOI: 10.1021/ja405628g Supporting Info |
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Nanomechanics of HaloTag Tethers Ionel Popa, Ronen Berkovich, Jorge Alegre-Cebollada, Carmen L. Badilla, Jaime Andrés Rivas-Pardo, Yukinori Taniguchi, Masaru Kawakami, and Julio M. Fernandez pp 12762–12771 DOI: 10.1021/ja4056382 Supporting Info |
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Dynamics of the His79-Heme Alkaline Transition of Yeast Iso-1-cytochrome c Probed by Conformationally Gated Electron Transfer with Co(II)bis(terpyridine) Melisa M. Cherney, Carolyn C. Junior, Bryan B. Bergquist, and Bruce E. Bowler pp 12772–12782 DOI: 10.1021/ja405725f Supporting Info |
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Threading Polyintercalators with Extremely Slow Dissociation Rates and Extended DNA Binding Sites Amy Rhoden Smith and Brent L. Iverson pp 12783–12789 DOI: 10.1021/ja4057344 Supporting Info |
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Large Molecular Weight Nitroxide Biradicals Providing Efficient Dynamic Nuclear Polarization at Temperatures up to 200 K Alexandre Zagdoun, Gilles Casano, Olivier Ouari, Martin Schwarzwälder, Aaron J. Rossini, Fabien Aussenac, Maxim Yulikov, Gunnar Jeschke, Christophe Copéret, Anne Lesage, Paul Tordo, and Lyndon Emsley pp 12790–12797 DOI: 10.1021/ja405813t Supporting Info |
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A Discrete Three-Layer Stack Aggregate of a Linear Porphyrin Tetramer: Solution-Phase Structure Elucidation by NMR and X-ray Scattering Marie Hutin, Johannes K. Sprafke, Barbara Odell, Harry L. Anderson, and Tim D. W. Claridge pp 12798–12807 DOI: 10.1021/ja406015r Supporting Info |
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Random Walk on a Leash: A Simple Single-Molecule Diffusion Model for Surface-Tethered Redox Molecules with Flexible Linkers Kuan-Chun Huang and Ryan J. White pp 12808–12817 DOI: 10.1021/ja4060788 Supporting Info |
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Ion Dynamics in Porous Carbon Electrodes in Supercapacitors Using in Situ Infrared Spectroelectrochemistry Francis W. Richey, Boris Dyatkin, Yury Gogotsi, and Yossef A. Elabd pp 12818–12826 DOI: 10.1021/ja406120e Supporting Info |
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Formation of S–Cl Phosphorothioate Adduct Radicals in dsDNA S-Oligomers: Hole Transfer to Guanine vs Disulfide Anion Radical Formation Amitava Adhikary, Anil Kumar, Brian J. Palmer, Andrew D. Todd, and Michael D. Sevilla pp 12827–12838 DOI: 10.1021/ja406121x Supporting Info |
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Lanthanide Cofactors Accelerate DNA-Catalyzed Synthesis of Branched RNA Fatemeh Javadi-Zarnaghi and Claudia Höbartner pp 12839–12848 DOI: 10.1021/ja406162z Supporting Info |
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Systematic and Controllable Negative, Zero, and Positive Thermal Expansion in Cubic Zr1–xSnxMo2O8 Sarah E. Tallentire, Felicity Child, Ian Fall, Liana Vella-Zarb, Ivana Radosavljević Evans, Matthew G. Tucker, David A. Keen, Claire Wilson, and John S. O. Evans pp 12849–12856 DOI: 10.1021/ja4060564 Supporting Info |
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Quadruple Anionic Buckybowls by Solid-State Chemistry of Corannulene and Cesium Tobias Bauert, Laura Zoppi, Georg Koller, Jay S. Siegel, Kim K. Baldridge, and Karl-Heinz Ernst pp 12857–12860 DOI: 10.1021/ja4063103 Supporting Info |
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Ir(III)-Catalyzed Mild C–H Amidation of Arenes and Alkenes: An Efficient Usage of Acyl Azides as the Nitrogen Source Jaeyune Ryu, Jaesung Kwak, Kwangmin Shin, Donggun Lee, and Sukbok Chang pp 12861–12868 DOI: 10.1021/ja406383h Supporting Info |
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Selective Detection and Inhibition of Active Caspase-3 in Cells with Optimized Peptides Chris J. Vickers, Gonzalo E. González-Páez, and Dennis W. Wolan pp 12869–12876 DOI: 10.1021/ja406399r Supporting Info |
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Suzuki-Miyaura Cross-Coupling of Unprotected, Nitrogen-Rich Heterocycles: Substrate Scope and Mechanistic Investigation M. Alexander Düfert, Kelvin L. Billingsley, and Stephen L. Buchwald pp 12877–12885 DOI: 10.1021/ja4064469 Supporting Info |
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Ti3+-, V2+/3+-, Cr2+/3+-, Mn2+-, and Fe2+-Substituted MOF-5 and Redox Reactivity in Cr- and Fe-MOF-5 Carl K. Brozek and Mircea Dincă pp 12886–12891 DOI: 10.1021/ja4064475 Supporting Info |
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C-Functionalized, Air- and Water-Stable 9,10-Dihydro-9,10-diboraanthracenes: Efficient Blue to Red Emitting Luminophores Christian Reus, Sabine Weidlich, Michael Bolte, Hans-Wolfram Lerner, and Matthias Wagner pp 12892–12907 DOI: 10.1021/ja406766e Supporting Info |
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Protecting Group-Free Synthesis of 1,2-Azaborines: A Simple Approach to the Construction of BN-Benzenoids Eric R. Abbey, Ashley N. Lamm, Andrew W. Baggett, Lev N. Zakharov, and Shih-Yuan Liu pp 12908–12913 DOI: 10.1021/ja4073436 Supporting Info |
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Functionalization Based on the Substitutional Flexibility: Strong Middle IR Nonlinear Optical Selenides AXII4XIII5Se12 Hua Lin, Ling Chen, Liu-Jiang Zhou, and Li-Ming Wu pp 12914–12921 DOI: 10.1021/ja4074084 Supporting Info |
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Correction to “Tandem Facial Amphiphiles for Membrane Protein Stabilization” Pil Seok Chae, Kamil Gotfryd, Jennifer Pacyna, Larry J. W. Miercke, Søren G. F. Rasmussen, Rebecca A. Robbins, Rohini R. Rana, Claus J. Loland, Brian Kobilka, Robert Stroud, Bernadette Byrne, Ulrik Gether, and Samuel H. Gellman pp 12922–12922 DOI: 10.1021/ja407245m |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 12923–12923 DOI: 10.1021/ja408820k |
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Detection of Dihydrofolate Reductase Conformational Change by FRET Using Two Fluorescent Amino Acids Shengxi Chen, Nour Eddine Fahmi, Lin Wang, Chandrabali Bhattacharya, Stephen J. Benkovic, and Sidney M. Hecht pp 12924–12927 DOI: 10.1021/ja403007r Supporting Info |
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One-Pot Colloidal Chemistry Route to Homogeneous and Doped Colloidosomes Xue-Wei Xu, Xi-Mo Zhang, Chao Liu, Ying-Long Yang, Jian-Wei Liu, Huai-Ping Cong, Chun-Hua Dong, Xi-Feng Ren, and Shu-Hong Yu pp 12928–12931 DOI: 10.1021/ja404880b Supporting Info |
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Atomic Layer Deposition of Platinum Catalysts on Nanowire Surfaces for Photoelectrochemical Water Reduction Neil P. Dasgupta, Chong Liu, Sean Andrews, Fritz B. Prinz, and Peidong Yang pp 12932–12935 DOI: 10.1021/ja405680p Supporting Info |
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Synthesis of Tetrachalcogenide-Substituted Phenalenyl Derivatives: Preparation and Solid-State Characterization of Bis(3,4,6,7-tetrathioalkyl-phenalenyl)boron Radicals Pradip Bag, Sushanta K. Pal, Mikhail E. Itkis, Arindam Sarkar, Fook S. Tham, Bruno Donnadieu, and Robert C. Haddon pp 12936–12939 DOI: 10.1021/ja405814f Supporting Info |
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Synergy of Non-antibiotic Drugs and Pyrimidinethiol on Gold Nanoparticles against Superbugs Yuyun Zhao, Zeliang Chen, Yanfen Chen, Jie Xu, Jinghong Li, and Xingyu Jiang pp 12940–12943 DOI: 10.1021/ja4058635 Supporting Info |
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Protected but Accessible: Oxygen Activation by a Calixarene-Stabilized Undecagold Cluster Xi Chen and Hannu Häkkinen pp 12944–12947 DOI: 10.1021/ja4059074 Supporting Info |
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Stepwise Helicity Inversions by Multisequential Metal Exchange Shigehisa Akine, Shiho Sairenji, Takanori Taniguchi, and Tatsuya Nabeshima pp 12948–12951 DOI: 10.1021/ja405979v Supporting Info |
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A Targeted, Self-Delivered, and Photocontrolled Molecular Beacon for mRNA Detection in Living Cells Liping Qiu, Cuichen Wu, Mingxu You, Da Han, Tao Chen, Guizhi Zhu, Jianhui Jiang, Ruqin Yu, and Weihong Tan pp 12952–12955 DOI: 10.1021/ja406252w Supporting Info |
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A C–C Bonded Phenoxyl Radical Dimer with a Zero Bond Dissociation Free Energy Jessica M. Wittman, Rebecca Hayoun, Werner Kaminsky, Michael K. Coggins, and James M. Mayer pp 12956–12959 DOI: 10.1021/ja406500h Supporting Info |
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Catalytic Enantioselective Dibromination of Allylic Alcohols Dennis X. Hu, Grant M. Shibuya, and Noah Z. Burns pp 12960–12963 DOI: 10.1021/ja4083182 Supporting Info |
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A Concise Total Synthesis of (+)-Scholarisine A Empowered by a Unique C–H Arylation Myles W. Smith and Scott A. Snyder pp 12964–12967 DOI: 10.1021/ja406546k Supporting Info |
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Metal-Free Borane-Catalyzed Highly Stereoselective Hydrogenation of Pyridines Yongbing Liu and Haifeng Du pp 12968–12971 DOI: 10.1021/ja406761j Supporting Info |
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Bilayer Molecular Electronics: All-Carbon Electronic Junctions Containing Molecular Bilayers Made with “Click” Chemistry Sayed Youssef Sayed, Akhtar Bayat, Mykola Kondratenko, Yann Leroux, Philippe Hapiot, and Richard L. McCreery pp 12972–12975 DOI: 10.1021/ja4065443 Supporting Info |
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Facile Catch and Release of Fullerenes Using a Photoresponsive Molecular Tube Norifumi Kishi, Munetaka Akita, Motoshi Kamiya, Shigehiko Hayashi, Hsiu-Fu Hsu, and Michito Yoshizawa pp 12976–12979 DOI: 10.1021/ja406893y Supporting Info |
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Cd2+ as a Ca2+ Surrogate in Protein–Membrane Interactions: Isostructural but Not Isofunctional Krystal A. Morales, Yuan Yang, Zheng Long, Pingwei Li, Alexander B. Taylor, P. John Hart, and Tatyana I. Igumenova pp 12980–12983 DOI: 10.1021/ja406958k Supporting Info |
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Synthesis of (±)-Actinophyllic Acid and Analogs: Applications of Cascade Reactions and Diverted Total Synthesis Brett A. Granger, Ivan T. Jewett, Jeffrey D. Butler, Bruce Hua, Claire E. Knezevic, Elizabeth I. Parkinson, Paul J. Hergenrother, and Stephen F. Martin pp 12984–12986 DOI: 10.1021/ja4070206 Supporting Info |
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Superconducting Fiber with Transition Temperature up to 7.43 K in Nb2PdxS5−δ (0.6 < x <1) Hongyan Yu, Ming Zuo, Lei Zhang, Shun Tan, Changjin Zhang, and Yuheng Zhang pp 12987–12989 DOI: 10.1021/ja4062079 Supporting Info |
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Palladium-Catalyzed Allylic C–H Fluorination Marie-Gabrielle Braun and Abigail G. Doyle pp 12990–12993 DOI: 10.1021/ja407223g Supporting Info |
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Bioconjugation by Native Chemical Tagging of C–H Bonds Qianghui Zhou, Jinghan Gui, Chung-Mao Pan, Earl Albone, Xin Cheng, Edward M. Suh, Luigi Grasso, Yoshihiro Ishihara, and Phil S. Baran pp 12994–12997 DOI: 10.1021/ja407739y Supporting Info |
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Probing the Role of Backbone Hydrogen Bonds in Protein–Peptide Interactions by Amide-to-Ester Mutations Jonas N. N. Eildal, Greta Hultqvist, Thomas Balle, Nicolai Stuhr-Hansen, Shahrokh Padrah, Stefano Gianni, Kristian Strømgaard, and Per Jemth pp 12998–13007 DOI: 10.1021/ja402875h Supporting Info |
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Correlation Effects on the Relative Stabilities of Alkanes William C. McKee and Paul von Ragué Schleyer pp 13008–13014 DOI: 10.1021/ja403934s Supporting Info |
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Antifouling Glycocalyx-Mimetic Peptoids Hyun Ok Ham, Sung Hyun Park, Josh W. Kurutz, Igal G. Szleifer, and Phillip B. Messersmith pp 13015–13022 DOI: 10.1021/ja404681x Supporting Info |
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Across the Structural Re-Entrant Transition in BaFe2(PO4)2: Influence of the Two-Dimensional Ferromagnetism Rénald David, Alain Pautrat, Dmitry Filimonov, Houria Kabbour, Hervé Vezin, Myung-Hwan Whangbo, and Olivier Mentré pp 13023–13029 DOI: 10.1021/ja404697b Supporting Info |
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Mechanistic Studies on Initiation and Propagation of Rare Earth Metal-Mediated Group Transfer Polymerization of Vinylphosphonates Stephan Salzinger, Benedikt S. Soller, Andriy Plikhta, Uwe B. Seemann, Eberhardt Herdtweck, and Bernhard Rieger pp 13030–13040 DOI: 10.1021/ja404457f Supporting Info |
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A Core/Satellite Multifunctional Nanotheranostic for in Vivo Imaging and Tumor Eradication by Radiation/Photothermal Synergistic Therapy Qingfeng Xiao, Xiangpeng Zheng, Wenbo Bu, Weiqiang Ge, Shengjian Zhang, Feng Chen, Huaiyong Xing, Qingguo Ren, Wenpei Fan, Kuaile Zhao, Yanqing Hua, and Jianlin Shi pp 13041–13048 DOI: 10.1021/ja404985w Supporting Info |
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Luminescence Studies of Individual Quantum Dot Photocatalysts Lilac Amirav and A. Paul Alivisatos pp 13049–13053 DOI: 10.1021/ja404918z Supporting Info |
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Effect of a Monofunctional Phenanthriplatin-DNA Adduct on RNA Polymerase II Transcriptional Fidelity and Translesion Synthesis Matthew W. Kellinger, Ga Young Park, Jenny Chong, Stephen J. Lippard, and Dong Wang pp 13054–13061 DOI: 10.1021/ja405475y Supporting Info |
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Noncrystalline-to-Crystalline Transformations in Pt Nanoparticles Long Li, Lin-Lin Wang, Duane D. Johnson, Zhongfan Zhang, Sergio I. Sanchez, Joo H. Kang, Ralph G. Nuzzo, Qi Wang, Anatoly I. Frenkel, Jie Li, James Ciston, Eric A. Stach, and Judith C. Yang pp 13062–13072 DOI: 10.1021/ja405497p Supporting Info |
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Chiroptical Inversion in Helical Si–Si Bond Polymer Aggregates Nozomu Suzuki, Michiya Fujiki, Ruth Kimpinde-Kalunga, and Julian R. Koe pp 13073–13079 DOI: 10.1021/ja405570q Supporting Info |
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Indium-Based Ultraviolet-Transparent Electroconductive Oxyfluoride InOF: Ambient-Pressure Synthesis and Unique Electronic Properties in Comparison with In2O3 Tatsuya Mori, Koichi Kajihara, Kiyoshi Kanamura, Yoshitake Toda, Hidenori Hiramatsu, and Hideo Hosono pp 13080–13088 DOI: 10.1021/ja405889m |
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Magic Number Pt13 and Misshapen Pt12 Clusters: Which One is the Better Catalyst? Takane Imaoka, Hirokazu Kitazawa, Wang-Jae Chun, Saori Omura, Ken Albrecht, and Kimihisa Yamamoto pp 13089–13095 DOI: 10.1021/ja405922m Supporting Info |
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Translation Enhancer Improves the Ribosome Liberation from Translation Initiation Shuntaro Takahashi, Hiroyuki Furusawa, Takuya Ueda, and Yoshio Okahata pp 13096–13106 DOI: 10.1021/ja405967h Supporting Info |
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A Versatile Approach to Ullmann C–N Couplings at Room Temperature: New Families of Nucleophiles and Electrophiles for Photoinduced, Copper-Catalyzed Processes Daniel T. Ziegler, Junwon Choi, José María Muñoz-Molina, Alex C. Bissember, Jonas C. Peters, and Gregory C. Fu pp 13107–13112 DOI: 10.1021/ja4060806 Supporting Info |
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Chemical Synthesis of Highly Congested gp120 V1V2 N-Glycopeptide Antigens for Potential HIV-1-Directed Vaccines Baptiste Aussedat, Yusuf Vohra, Peter K. Park, Alberto Fernández-Tejada, S. Munir Alam, S. Moses Dennison, Frederick H. Jaeger, Kara Anasti, Shelley Stewart, Julie H. Blinn, Hua-Xin Liao, Joseph G. Sodroski, Barton F. Haynes, and Samuel J. Danishefsky pp 13113–13120 DOI: 10.1021/ja405990z Supporting Info |
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Pt-Catalyzed C–C Activation Induced by C–H Activation Miriam A. Bowring, Robert G. Bergman, and T. Don Tilley pp 13121–13128 DOI: 10.1021/ja406260j Supporting Info |
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Relationship between Chemical Structure and Supramolecular Effective Molarity for Formation of Intramolecular H-Bonds Hongmei Sun, Christopher A. Hunter, Cristina Navarro, and Simon Turega pp 13129–13141 DOI: 10.1021/ja406235d Supporting Info |
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Systematic Variation of Metal–Metal Bond Order in Metal–Chromium Complexes Laura J. Clouston, Randall B. Siedschlag, P. Alex Rudd, Nora Planas, Shuxian Hu, Adam D. Miller, Laura Gagliardi, and Connie C. Lu pp 13142–13148 DOI: 10.1021/ja406506m Supporting Info |
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Hemilabile N-Xylyl-N′-methylperimidine Carbene Iridium Complexes as Catalysts for C–H Activation and Dehydrogenative Silylation: Dual Role of N-Xylyl Moiety for ortho-C–H Bond Activation and Reductive Bond Cleavage Gyeongshin Choi, Hayato Tsurugi, and Kazushi Mashima pp 13149–13161 DOI: 10.1021/ja406519u Supporting Info |
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Photoinduced Electron Transfer from PbS Quantum Dots to Cobalt(III) Schiff Base Complexes: Light Activation of a Protein Inhibitor Mark D. Peterson, Robert J. Holbrook, Thomas J. Meade, and Emily A. Weiss pp 13162–13167 DOI: 10.1021/ja4065393 Supporting Info |
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Catalytic Hydrogenation Activity and Electronic Structure Determination of Bis(arylimidazol-2-ylidene)pyridine Cobalt Alkyl and Hydride Complexes Renyuan Pony Yu, Jonathan M. Darmon, Carsten Milsmann, Grant W. Margulieux, S. Chantal E. Stieber, Serena DeBeer, and Paul J. Chirik pp 13168–13184 DOI: 10.1021/ja406608u Supporting Info |
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Stable Uranium(VI) Methyl and Acetylide Complexes and the Elucidation of an Inverse Trans Influence Ligand Series Andrew J. Lewis, Patrick J. Carroll, and Eric J. Schelter pp 13185–13192 DOI: 10.1021/ja406610r Supporting Info |
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Carbene Transfer from Triazolylidene Gold Complexes as a Potent Strategy for Inducing High Catalytic Activity Daniel Canseco-Gonzalez, Ana Petronilho, Helge Mueller-Bunz, Kohsuke Ohmatsu, Takashi Ooi, and Martin Albrecht pp 13193–13203 DOI: 10.1021/ja406999p Supporting Info |
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Synthesis of [closo-B12(OH)11NH3]−: A New Heterobifunctional Dodecaborane Scaffold for Drug Delivery Applications Oleg Bondarev, Aslam A. Khan, Xiaoyan Tu, Yulia V. Sevryugina, Satish S. Jalisatgi, and M. Frederick Hawthorne pp 13204–13211 DOI: 10.1021/ja4069613 Supporting Info |
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Designing and Refining Ni(II)diimine Catalysts Toward the Controlled Synthesis of Electron-Deficient Conjugated Polymers Colin R. Bridges, Theresa M. McCormick, Gregory L. Gibson, Jon Hollinger, and Dwight S. Seferos pp 13212–13219 DOI: 10.1021/ja4073904 Supporting Info |
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Correction to “Single-Molecule Protein Unfolding in Solid State Nanopores” David S. Talaga and Jiali Li pp 13220–13220 DOI: 10.1021/ja405675p |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 13221–13221 DOI: 10.1021/ja409118e |
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Metal–Organic Frameworks as A Tunable Platform for Designing Functional Molecular Materials Cheng Wang, Demin Liu, and Wenbin Lin pp 13222–13234 DOI: 10.1021/ja308229p |
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Exceptional Steric Congestion in an in,in-Bis(hydrosilane) Jie Zong, Joel T. Mague, and Robert A. Pascal, Jr. pp 13235–13237 DOI: 10.1021/ja407398w Supporting Info |
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Allosterically Tunable, DNA-Based Switches Triggered by Heavy Metals Alessandro Porchetta, Alexis Vallée-Bélisle, Kevin W. Plaxco, and Francesco Ricci pp 13238–13241 DOI: 10.1021/ja404653q Supporting Info |
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Significant Enhancement of Energy Barriers in Dinuclear Dysprosium Single-Molecule Magnets Through Electron-Withdrawing Effects Fatemah Habib, Gabriel Brunet, Veacheslav Vieru, Ilia Korobkov, Liviu F. Chibotaru, and Muralee Murugesu pp 13242–13245 DOI: 10.1021/ja404846s Supporting Info |
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Protein Delivery of a Ni Catalyst to Photosystem I for Light-Driven Hydrogen Production Sunshine C. Silver, Jens Niklas, Pingwu Du, Oleg G. Poluektov, David M. Tiede, and Lisa M. Utschig pp 13246–13249 DOI: 10.1021/ja405277g Supporting Info |
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Modulation of Y356 Photooxidation in E. coli Class Ia Ribonucleotide Reductase by Y731 Across the α2:β2 Interface Arturo A. Pizano, Lisa Olshansky, Patrick G. Holder, JoAnne Stubbe, and Daniel G. Nocera pp 13250–13253 DOI: 10.1021/ja405498e Supporting Info |
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Chemical Insight into the Emergence of Influenza Virus Strains That Are Resistant to Relenza Fahimeh S. Shidmoossavee, Jacqueline N. Watson, and Andrew J. Bennet pp 13254–13257 DOI: 10.1021/ja405916q Supporting Info |
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Arene–Metal π-Complexation as a Traceless Reactivity Enhancer for C–H Arylation Paolo Ricci, Katrina Krämer, Xacobe C. Cambeiro, and Igor Larrosa pp 13258–13261 DOI: 10.1021/ja405936s Supporting Info |
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Cluster Size Effects in the Photocatalytic Hydrogen Evolution Reaction Florian F. Schweinberger, Maximilian J. Berr, Markus Döblinger, Christian Wolff, Kai E. Sanwald, Andrew S. Crampton, Claron J. Ridge, Frank Jäckel, Jochen Feldmann, Martin Tschurl, and Ueli Heiz pp 13262–13265 DOI: 10.1021/ja406070q Supporting Info |
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Ring-Shaped Re(I) Multinuclear Complexes with Unique Photofunctional Properties Tatsuki Morimoto, Chiaki Nishiura, Marina Tanaka, Jana Rohacova, Yuki Nakagawa, Yusuke Funada, Kazuhide Koike, Youhei Yamamoto, Sayaka Shishido, Tatsuhiro Kojima, Takuro Saeki, Tomoji Ozeki, and Osamu Ishitani pp 13266–13269 DOI: 10.1021/ja406144h Supporting Info |
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Fast and Persistent Electrocatalytic Water Oxidation by Co–Fe Prussian Blue Coordination Polymers Sara Pintado, Sara Goberna-Ferrón, Eduardo C. Escudero-Adán, and José Ramón Galán-Mascarós pp 13270–13273 DOI: 10.1021/ja406242y Supporting Info |
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Controlled Growth of Atomically Thin In2Se3 Flakes by van der Waals Epitaxy Min Lin, Di Wu, Yu Zhou, Wei Huang, Wei Jiang, Wenshan Zheng, Shuli Zhao, Chuanhong Jin, Yunfan Guo, Hailin Peng, and Zhongfan Liu pp 13274–13277 DOI: 10.1021/ja406351u Supporting Info |
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Pd-Catalyzed Aryl C–H Imidation with Arene as the Limiting Reagent Gregory B. Boursalian, Ming-Yu Ngai, Katarzyna N. Hojczyk, and Tobias Ritter pp 13278–13281 DOI: 10.1021/ja4064926 Supporting Info |
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Switchable Fluorescent Imaging of Intracellular Telomerase Activity Using Telomerase-Responsive Mesoporous Silica Nanoparticle Ruocan Qian, Lin Ding, and Huangxian Ju pp 13282–13285 DOI: 10.1021/ja406532e Supporting Info |
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Mechanistic Insights and Kinetic Analysis for the Oxidative Hydroxylation of Arylboronic Acids by Visible Light Photoredox Catalysis: A Metal-Free Alternative Spencer P. Pitre, Christopher D. McTiernan, Hossein Ismaili, and Juan C. Scaiano pp 13286–13289 DOI: 10.1021/ja406311g Supporting Info |
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Binding of a Structured d-RNA Molecule by an l-RNA Aptamer Jonathan T. Sczepanski and Gerald F. Joyce pp 13290–13293 DOI: 10.1021/ja406634g Supporting Info |
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Asymmetric α-Arylation of Amino Acid Derivatives by Clayden Rearrangement of Ester Enolates via Memory of Chirality Keisuke Tomohara, Tomoyuki Yoshimura, Ryuichi Hyakutake, Pan Yang, and Takeo Kawabata pp 13294–13297 DOI: 10.1021/ja406653n Supporting Info |
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High-Spin Ribbons and Antiferromagnetic Ordering of a MnII-Biradical-MnII Complex Elisabeth M. Fatila, Rodolphe Clérac, Mathieu Rouzières, Dmitriy V. Soldatov, Michael Jennings, and Kathryn E. Preuss pp 13298–13301 DOI: 10.1021/ja4067783 Supporting Info |
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A Single-Molecule Magnet Based on Heptacyanomolybdate with the Highest Energy Barrier for a Cyanide Compound Kun Qian, Xing-Cai Huang, Chun Zhou, Xiao-Zeng You, Xin-Yi Wang, and Kim R. Dunbar pp 13302–13305 DOI: 10.1021/ja4067833 Supporting Info |
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Ring-Opening Polymerization with Zn(C6F5)2-Based Lewis Pairs: Original and Efficient Approach to Cyclic Polyesters Estefanía Piedra-Arroni, Catherine Ladavière, Abderrahmane Amgoune, and Didier Bourissou pp 13306–13309 DOI: 10.1021/ja4069968 Supporting Info |
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Identification of the +2 Oxidation State for Uranium in a Crystalline Molecular Complex, [K(2.2.2-Cryptand)][(C5H4SiMe3)3U] Matthew R. MacDonald, Megan E. Fieser, Jefferson E. Bates, Joseph W. Ziller, Filipp Furche, and William J. Evans pp 13310–13313 DOI: 10.1021/ja406791t Supporting Info |
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Enantioselective Gold(I)-Catalyzed Vinylogous [3 + 2] Cycloaddition between Vinyldiazoacetates and Enol Ethers John F. Briones and Huw M. L. Davies pp 13314–13317 DOI: 10.1021/ja407179c Supporting Info |
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Synthesis of a Rotaxane CuI Triazolide under Aqueous Conditions Joby Winn, Aleksandra Pinczewska, and Stephen M. Goldup pp 13318–13321 DOI: 10.1021/ja407446c Supporting Info |
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Extending Photoinduced Charge Separation Lifetimes by Using Supramolecular Design: Guanine–Perylenediimide G-Quadruplex Yi-Lin Wu, Kristen E. Brown, and Michael R. Wasielewski pp 13322–13325 DOI: 10.1021/ja407648d Supporting Info |
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Selective Turn-On Ammonia Sensing Enabled by High-Temperature Fluorescence in Metal–Organic Frameworks with Open Metal Sites Natalia B. Shustova, Anthony F. Cozzolino, Sebastian Reineke, Marc Baldo, and Mircea Dincă pp 13326–13329 DOI: 10.1021/ja407778a Supporting Info |
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Preparation of Vinyl Silyl Ethers and Disiloxanes via the Silyl-Heck Reaction of Silyl Ditriflates Sara E. S. Martin and Donald A. Watson pp 13330–13333 DOI: 10.1021/ja407748z Supporting Info |
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Domino Michael/Mannich/N-Alkylation Route to the Tetrahydrocarbazole Framework of Aspidosperma Alkaloids: Concise Total Syntheses of (−)-Aspidospermidine, (−)-Tabersonine, and (−)-Vincadifformine Senzhi Zhao and Rodrigo B. Andrade pp 13334–13337 DOI: 10.1021/ja408114u Supporting Info |
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Normal-to-Abnormal Rearrangement and NHC Activation in Three-Coordinate Iron(II) Carbene Complexes Benjamin M. Day, Thomas Pugh, Daniël Hendriks, Célia Fonseca Guerra, David J. Evans, F. Matthias Bickelhaupt, and Richard A. Layfield pp 13338–13341 DOI: 10.1021/ja408589p Supporting Info |
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The Mechanism of Borane–Amine Dehydrocoupling with Bifunctional Ruthenium Catalysts Alexander N. Marziale, Anja Friedrich, Isabel Klopsch, Markus Drees, Vinicius R. Celinski, Jörn Schmedt auf der Günne, and Sven Schneider pp 13342–13355 DOI: 10.1021/ja311092c Supporting Info |
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Enzyme-Catalyzed Oxidation Facilitates the Return of Fluorescence for Single-Walled Carbon Nanotubes Cheuk Fai Chiu, Brian A. Barth, Gregg P. Kotchey, Yong Zhao, Kristy A. Gogick, Wissam A. Saidi, Stéphane Petoud, and Alexander Star pp 13356–13364 DOI: 10.1021/ja400699y Supporting Info |
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pH-Dependent Si-Fluorescein Hypochlorous Acid Fluorescent Probe: Spirocycle Ring-Opening and Excess Hypochlorous Acid-Induced Chlorination Quinn A. Best, Narsimha Sattenapally, Daniel J. Dyer, Colleen N. Scott, and Matthew E. McCarroll pp 13365–13370 DOI: 10.1021/ja401426s Supporting Info |
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Directed ortho-Lithiation: Observation of an Unexpected 1-Lithio to 3-Lithio Conversion of 1-Lithio-naphthyllithium Compounds with an ortho-Directing 2-(Dimethylamino)methyl Group Johann T. B. H. Jastrzebski, Anne M. Arink, Henk Kleijn, Thijs W. Braam, Martin Lutz, Anthony L. Spek, and Gerard van Koten pp 13371–13378 DOI: 10.1021/ja402884y Supporting Info |
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Ferrocenoyl Phenylalanine: A New Strategy Toward Supramolecular Hydrogels with Multistimuli Responsive Properties Zhifang Sun, Zhengyuan Li, Yonghui He, Rujuan Shen, Liu Deng, Minghui Yang, Yizeng Liang, and Yi Zhang pp 13379–13386 DOI: 10.1021/ja403345p Supporting Info |
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Discoipyrroles A–D: Isolation, Structure Determination, and Synthesis of Potent Migration Inhibitors from Bacillus hunanensis Youcai Hu, Malia B. Potts, Dominic Colosimo, Mireya L. Herrera-Herrera, Aaron G. Legako, Muhammed Yousufuddin, Michael A. White, and John B. MacMillan pp 13387–13392 DOI: 10.1021/ja403412y Supporting Info |
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Computational Design of an Unnatural Amino Acid Dependent Metalloprotein with Atomic Level Accuracy Jeremy H. Mills, Sagar D. Khare, Jill M. Bolduc, Farhad Forouhar, Vikram Khipple Mulligan, Scott Lew, Jayaraman Seetharaman, Liang Tong, Barry L. Stoddard, and David Baker pp 13393–13399 DOI: 10.1021/ja403503m Supporting Info |
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Amine Oxidation Mediated by Lysine-Specific Demethylase 1: Quantum Mechanics/Molecular Mechanics Insights into Mechanism and Role of Lysine 661 Bora Karasulu, Mahendra Patil, and Walter Thiel pp 13400–13413 DOI: 10.1021/ja403582u Supporting Info |
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Mimicry of High-Density Lipoprotein: Functional Peptide–Lipid Nanoparticles Based on Multivalent Peptide Constructs Yannan Zhao, Tomohiro Imura, Luke J. Leman, Linda K. Curtiss, Bruce E. Maryanoff, and M. Reza Ghadiri pp 13414–13424 DOI: 10.1021/ja404714a Supporting Info |
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Exploring the Programmable Assembly of a Polyoxometalate–Organic Hybrid via Metal Ion Coordination Panchao Yin, Tao Li, Ross S. Forgan, Claire Lydon, Xiaobing Zuo, Zhaoxiong Norm Zheng, Byeongdu Lee, Deliang Long, Leroy Cronin, and Tianbo Liu pp 13425–13432 DOI: 10.1021/ja404777g Supporting Info |
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Genetically Encoded Light-Activated Transcription for Spatiotemporal Control of Gene Expression and Gene Silencing in Mammalian Cells James Hemphill, Chungjung Chou, Jason W. Chin, and Alexander Deiters pp 13433–13439 DOI: 10.1021/ja4051026 Supporting Info |
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Production of Tartrates by Cyanide-Mediated Dimerization of Glyoxylate: A Potential Abiotic Pathway to the Citric Acid Cycle Christopher Butch, Elizabeth D. Cope, Pamela Pollet, Leslie Gelbaum, Ramanarayanan Krishnamurthy, and Charles L. Liotta pp 13440–13445 DOI: 10.1021/ja405103r Supporting Info |
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Targeted Disruption of Transcriptional Regulators in Chaetomium globosum Activates Biosynthetic Pathways and Reveals Transcriptional Regulator-Like Behavior of Aureonitol Takehito Nakazawa, Kan’ichiro Ishiuchi, Michio Sato, Yuta Tsunematsu, Satoru Sugimoto, Yasutaka Gotanda, Hiroshi Noguchi, Kinya Hotta, and Kenji Watanabe pp 13446–13455 DOI: 10.1021/ja405128k Supporting Info |
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Tuning the Size and Properties of ClyA Nanopores Assisted by Directed Evolution Misha Soskine, Annemie Biesemans, Marc De Maeyer, and Giovanni Maglia pp 13456–13463 DOI: 10.1021/ja4053398 Supporting Info |
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Stabilization of Branched Oligosaccharides: Lewisx Benefits from a Nonconventional C–H···O Hydrogen Bond Mirko Zierke, Martin Smieško, Said Rabbani, Thomas Aeschbacher, Brian Cutting, Frédéric H.-T. Allain, Mario Schubert, and Beat Ernst pp 13464–13472 DOI: 10.1021/ja4054702 Supporting Info |
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Platinum-Coated Copper Nanowires with High Activity for Hydrogen Oxidation Reaction in Base Shaun M. Alia, Bryan S. Pivovar, and Yushan Yan pp 13473–13478 DOI: 10.1021/ja405598a Supporting Info |
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Bimodal Intramolecular Excitation Energy Transfer in a Multichromophore Photosynthetic Model System: Hybrid Fusion Proteins Comprising Natural Phycobilin- and Artificial Chlorophyll-Binding Domains Xiao-Li Zeng, Kun Tang, Nan Zhou, Ming Zhou, Harvey J. M. Hou, Hugo Scheer, Kai-Hong Zhao, and Dror Noy pp 13479–13487 DOI: 10.1021/ja405617c Supporting Info |
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Exploiting Differential Surface Display of Chondroitin Sulfate Variants for Directing Neuronal Outgrowth Vimal P. Swarup, Tony W. Hsiao, Jianxing Zhang, Glenn D. Prestwich, Balagurunathan Kuberan, and Vladimir Hlady pp 13488–13494 DOI: 10.1021/ja4056728 Supporting Info |
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Solution Structure of an Intramolecular (3 + 1) Human Telomeric G-Quadruplex Bound to a Telomestatin Derivative Wan Jun Chung, Brahim Heddi, Masayuki Tera, Keisuke Iida, Kazuo Nagasawa, and Anh Tuân Phan pp 13495–13501 DOI: 10.1021/ja405843r Supporting Info |
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Palladium-Catalyzed Carbene Migratory Insertion Using Conjugated Ene–Yne–Ketones as Carbene Precursors Ying Xia, Shuanglin Qu, Qing Xiao, Zhi-Xiang Wang, Peiyuan Qu, Li Chen, Zhen Liu, Leiming Tian, Zhongxing Huang, Yan Zhang, and Jianbo Wang pp 13502–13511 DOI: 10.1021/ja4058844 Supporting Info |
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Visualization of Peroxynitrite-Induced Changes of Labile Zn2+ in the Endoplasmic Reticulum with Benzoresorufin-Based Fluorescent Probes Wei Lin, Daniela Buccella, and Stephen J. Lippard pp 13512–13520 DOI: 10.1021/ja4059487 Supporting Info |
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Theoretical Investigation of the Activity of Cobalt Oxides for the Electrochemical Oxidation of Water Michal Bajdich, Mónica García-Mota, Aleksandra Vojvodic, Jens K. Nørskov, and Alexis T. Bell pp 13521–13530 DOI: 10.1021/ja405997s Supporting Info |
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Assembly and Fiber Formation of a Gemini-Type Hexathienocoronene Amphiphile for Electrical Conduction Long Chen, Kunal S. Mali, Sreenivasa R. Puniredd, Martin Baumgarten, Khaled Parvez, Wojciech Pisula, Steven De Feyter, and Klaus Müllen pp 13531–13537 DOI: 10.1021/ja4062135 Supporting Info |
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Protic Ionic Liquids as p-Dopant for Organic Hole Transporting Materials and Their Application in High Efficiency Hybrid Solar Cells Antonio Abate, Derek J. Hollman, Joël Teuscher, Sandeep Pathak, Roberto Avolio, Gerardino D’Errico, Giuseppe Vitiello, Simona Fantacci, and Henry J. Snaith pp 13538–13548 DOI: 10.1021/ja406230f Supporting Info |
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Development of Large Band-Gap Conjugated Copolymers for Efficient Regular Single and Tandem Organic Solar Cells Kai Li, Zuojia Li, Kui Feng, Xiaopeng Xu, Lingyan Wang, and Qiang Peng pp 13549–13557 DOI: 10.1021/ja406220a Supporting Info |
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Synthesis, Electrochemistry, and Electrogenerated Chemiluminescence of Two BODIPY-Appended Bipyridine Homologues Honglan Qi, Justin J. Teesdale, Rachel C. Pupillo, Joel Rosenthal, and Allen J. Bard pp 13558–13566 DOI: 10.1021/ja406731f Supporting Info |
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Mechanistic Insight into the Formation of Acetic Acid from the Direct Conversion of Methane and Carbon Dioxide on Zinc-Modified H–ZSM-5 Zeolite Jian-Feng Wu, Si-Min Yu, Wei David Wang, Yan-Xin Fan, Shi Bai, Chuan-Wei Zhang, Qiang Gao, Jun Huang, and Wei Wang pp 13567–13573 DOI: 10.1021/ja406978q Supporting Info |
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Polymerization-Induced Self-Assembly of Galactose-Functionalized Biocompatible Diblock Copolymers for Intracellular Delivery Vincent Ladmiral, Mona Semsarilar, Irene Canton, and Steven P. Armes pp 13574–13581 DOI: 10.1021/ja407033x Supporting Info |
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Lipid Bilayers Significantly Modulate Cross-Fibrillation of Two Distinct Amyloidogenic Peptides Noga Gal, Ahiud Morag, Sofiya Kolusheva, Roland Winter, Meytal Landau, and Raz Jelinek pp 13582–13589 DOI: 10.1021/ja4070427 Supporting Info |
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Association Dynamics and Linear and Nonlinear Optical Properties of an N-Acetylaladanamide Probe in a POPC Membrane N. Arul Murugan, Rossen Apostolov, Zilvinas Rinkevicius, Jacob Kongsted, Erik Lindahl, and Hans Ågren pp 13590–13597 DOI: 10.1021/ja407326n Supporting Info |
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Stress-Responsive Polymers Containing Cyclobutane Core Mechanophores: Reactivity and Mechanistic Insights Zachary S. Kean, Zhenbin Niu, Gihan B. Hewage, Arnold L. Rheingold, and Stephen L. Craig pp 13598–13604 DOI: 10.1021/ja4075997 Supporting Info |
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Directed Nickel-Catalyzed Negishi Cross Coupling of Alkyl Aziridines Daniel K. Nielsen, Chung-Yang (Dennis) Huang, and Abigail G. Doyle pp 13605–13609 DOI: 10.1021/ja4076716 Supporting Info |
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Correction to “Spotlights on Recent JACS Publications” ACS Contributing Correspondents pp 13610–13610 DOI: 10.1021/ja407288b |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 13611–13611 DOI: 10.1021/ja4093727 |
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Enhanced Aqueous Suzuki–Miyaura Coupling Allows Site-Specific Polypeptide 18F-Labeling Zhanghua Gao, Véronique Gouverneur, and Benjamin G. Davis pp 13612–13615 DOI: 10.1021/ja4049114 Supporting Info |
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Nanoreactors for Simultaneous Remote Thermal Activation and Optical Monitoring of Chemical Reactions Carmen Vázquez-Vázquez, Belén Vaz, Vincenzo Giannini, Moisés Pérez-Lorenzo, Ramon A. Alvarez-Puebla, and Miguel A. Correa-Duarte pp 13616–13619 DOI: 10.1021/ja4051873 Supporting Info |
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Poly(iohexol) Nanoparticles As Contrast Agents for in Vivo X-ray Computed Tomography Imaging Qian Yin, Felix Y. Yap, Lichen Yin, Liang Ma, Qin Zhou, Lawrence W. Dobrucki, Timothy M. Fan, Ron C. Gaba, and Jianjun Cheng pp 13620–13623 DOI: 10.1021/ja405196f Supporting Info |
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A Critical Test of the “Tunneling and Coupled Motion” Concept in Enzymatic Alcohol Oxidation Daniel Roston and Amnon Kohen pp 13624–13627 DOI: 10.1021/ja405917m Supporting Info |
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DNA Tetraplexes-Based Toehold Activation for Controllable DNA Strand Displacement Reactions Wei Tang, Huaming Wang, Dingzhong Wang, Yan Zhao, Na Li, and Feng Liu pp 13628–13631 DOI: 10.1021/ja406053b Supporting Info |
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Long-Lived Luminogenic Probe for Detection of RNA in a Crude Solution of Living Bacterial Cells Hisao Saneyoshi, Yoshihiro Ito, and Hiroshi Abe pp 13632–13635 DOI: 10.1021/ja406724k Supporting Info |
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Nickel-Catalyzed Decarbonylative Alkylidenation of Phthalimides with Trimethylsilyl-Substituted Alkynes Takahiro Shiba, Takuya Kurahashi, and Seijiro Matsubara pp 13636–13639 DOI: 10.1021/ja4068172 Supporting Info |
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Synthesis, Electronic Structure, and Magnetism of [Ni(6-Mes)2]+: A Two-Coordinate Nickel(I) Complex Stabilized by Bulky N-Heterocyclic Carbenes Rebecca C. Poulten, Michael J. Page, Andrés G. Algarra, Jennifer J. Le Roy, Isidoro López, Emma Carter, Antoni Llobet, Stuart A. Macgregor, Mary F. Mahon, Damien M. Murphy, Muralee Murugesu, and Michael K. Whittlesey pp 13640–13643 DOI: 10.1021/ja407004y Supporting Info |
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A Cyclochiral Conformational Motif Constructed Using a Robust Hydrogen-Bonding Network Kenji Mishiro, Takumi Furuta, Takahiro Sasamori, Kazuhiro Hayashi, Norihiro Tokitoh, Shiroh Futaki, and Takeo Kawabata pp 13644–13647 DOI: 10.1021/ja407051k Supporting Info |
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Co–C Bond Energies in Adenosylcobinamide and Methylcobinamide in the Gas Phase and in Silico Ilia J. Kobylianskii, Florian J. Widner, Bernhard Kräutler, and Peter Chen pp 13648–13651 DOI: 10.1021/ja406676p Supporting Info |
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Stereoselective Synthesis of 2,3-Dihydropyrroles from Terminal Alkynes, Azides, and α,β-Unsaturated Aldehydes via N-Sulfonyl-1,2,3-triazoles Tomoya Miura, Takamasa Tanaka, Kentaro Hiraga, Scott G. Stewart, and Masahiro Murakami pp 13652–13655 DOI: 10.1021/ja407166r Supporting Info |
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A Bio-Inspired, Small Molecule Electron-Coupled-Proton Buffer for Decoupling the Half-Reactions of Electrolytic Water Splitting Benjamin Rausch, Mark D. Symes, and Leroy Cronin pp 13656–13659 DOI: 10.1021/ja4071893 Supporting Info |
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Experimental Evidence of Ultrafast Quenching of the 3MLCT Luminescence in Ruthenium(II) Tris-bipyridyl Complexes via a 3dd State Qinchao Sun, Sandra Mosquera-Vazquez, Latévi Max Lawson Daku, Laure Guénée, Harold A. Goodwin, Eric Vauthey, and Andreas Hauser pp 13660–13663 DOI: 10.1021/ja407225t Supporting Info |
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Pd-Catalyzed Semmler–Wolff Reactions for the Conversion of Substituted Cyclohexenone Oximes to Primary Anilines Wan Pyo Hong, Andrei V. Iosub, and Shannon S. Stahl pp 13664–13667 DOI: 10.1021/ja4073172 Supporting Info |
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Incorporation and Luminescence of Yb3+ in CdSe Nanocrystals Rosa Martín-Rodríguez, Robin Geitenbeek, and Andries Meijerink pp 13668–13671 DOI: 10.1021/ja4077414 Supporting Info |
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Amplified Halogen Bonding in a Small Space Mohammed G. Sarwar, Dariush Ajami, Giannoula Theodorakopoulos, Ioannis D. Petsalakis, and Julius Rebek, Jr. pp 13672–13675 DOI: 10.1021/ja407815t Supporting Info |
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Tunable Visible Light Emission of Self-Assembled Rhomboidal Metallacycles J. Bryant Pollock, Gregory L. Schneider, Timothy R. Cook, Andrew S. Davies, and Peter J. Stang pp 13676–13679 DOI: 10.1021/ja4079607 Supporting Info |
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Isomeric Cyclopropenes Exhibit Unique Bioorthogonal Reactivities David N. Kamber, Lidia A. Nazarova, Yong Liang, Steven A. Lopez, David M. Patterson, Hui-Wen Shih, K. N. Houk, and Jennifer A. Prescher pp 13680–13683 DOI: 10.1021/ja407737d Supporting Info |
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Total Synthesis of Ecteinascidin 743 Fumiki Kawagishi, Tatsuya Toma, Tomohiko Inui, Satoshi Yokoshima, and Tohru Fukuyama pp 13684–13687 DOI: 10.1021/ja408034x Supporting Info |
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Catalytic Activation of H2 under Mild Conditions by an [FeFe]-Hydrogenase Model via an Active μ-Hydride Species Ning Wang, Mei Wang, Ying Wang, Dehua Zheng, Hongxian Han, Mårten S. G. Ahlquist, and Licheng Sun pp 13688–13691 DOI: 10.1021/ja408376t Supporting Info |
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Universal Aptamer-Based Real-Time Monitoring of Enzymatic RNA Synthesis Katharina Höfer, Lisa V. Langejürgen, and Andres Jäschke pp 13692–13694 DOI: 10.1021/ja407142f Supporting Info |
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“Fibonacci’s Route” to Regioregular Oligo(3-hexylthiophene)s Felix P. V. Koch, Paul Smith, and Martin Heeney pp 13695–13698 DOI: 10.1021/ja4057932 Supporting Info |
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Thermal and Structural Characteristics of Oligo(3-hexylthiophene)s (3HT)n, n = 4–36 Felix Peter Vinzenz Koch, Martin Heeney, and Paul Smith pp 13699–13709 DOI: 10.1021/ja405792b |
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Influenza Virus A M2 Protein Generates Negative Gaussian Membrane Curvature Necessary for Budding and Scission Nathan W. Schmidt, Abhijit Mishra, Jun Wang, William F. DeGrado, and Gerard C. L. Wong pp 13710–13719 DOI: 10.1021/ja400146z Supporting Info |
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Volume Change during Thermal [4 + 4] Cycloaddition of [2.2] (9,10)Anthracenophane Brad Slepetz and Miklos Kertesz pp 13720–13727 DOI: 10.1021/ja402485j Supporting Info |
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Bioanalysis for Biocatalysis: Multiplexed Capillary Electrophoresis–Mass Spectrometry Assay for Aminotransferase Substrate Discovery and Specificity Profiling Gleb G. Mironov, Antony D. St-Jacques, Alexander Mungham, Matthew G. Eason, Roberto A. Chica, and Maxim V. Berezovski pp 13728–13736 DOI: 10.1021/ja407486z Supporting Info |
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Highly Anisotropic Rhenium(IV) Complexes: New Examples of Mononuclear Single-Molecule Magnets José Martínez-Lillo, Teresa F. Mastropietro, Elsa Lhotel, Carley Paulsen, Joan Cano, Giovanni De Munno, Juan Faus, Francesc Lloret, Miguel Julve, Saritha Nellutla, and J. Krzystek pp 13737–13748 DOI: 10.1021/ja403154z Supporting Info |
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Mechanistic Studies on the Pd-Catalyzed Vinylation of Aryl Halides with Vinylalkoxysilanes in Water: The Effect of the Solvent and NaOH Promoter Alvaro Gordillo, Manuel A. Ortuño, Carmen López-Mardomingo, Agustí Lledós, Gregori Ujaque, and Ernesto de Jesús pp 13749–13763 DOI: 10.1021/ja404255u Supporting Info |
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Phosphoryl Transfers of the Phospholipase D Superfamily: A Quantum Mechanical Theoretical Study Nathan J. DeYonker and Charles Edwin Webster pp 13764–13774 DOI: 10.1021/ja4042753 Supporting Info |
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Giant Stretchability and Reversibility of Tightly Wound Helical Carbon Nanotubes Jianyang Wu, Jianying He, Gregory M. Odegard, Shijo Nagao, Quanshui Zheng, and Zhiliang Zhang pp 13775–13785 DOI: 10.1021/ja404330q Supporting Info |
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Multidentate Zwitterionic Ligands Provide Compact and Highly Biocompatible Quantum Dots Naiqian Zhan, Goutam Palui, Malak Safi, Xin Ji, and Hedi Mattoussi pp 13786–13795 DOI: 10.1021/ja405010v Supporting Info |
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Molecular Crowding Drives Active Pin1 into Nonspecific Complexes with Endogenous Proteins Prior to Substrate Recognition Laura M. Luh, Robert Hänsel, Frank Löhr, Donata K. Kirchner, Katharina Krauskopf, Susanne Pitzius, Birgit Schäfer, Peter Tufar, Ivan Corbeski, Peter Güntert, and Volker Dötsch pp 13796–13803 DOI: 10.1021/ja405244v Supporting Info |
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Water Oxidation Mechanism for Synthetic Co–Oxides with Small Nuclearity Xichen Li and Per E. M. Siegbahn pp 13804–13813 DOI: 10.1021/ja4053448 Supporting Info |
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Keys for the Existence of Stable Dimers of Bis-tetrathiafulvalene (bis-TTF)-Functionalized Molecular Clips Presenting [TTF]•+···[TTF]•+ Long, Multicenter Bonds at Room Temperature Maria Fumanal, Marçal Capdevila-Cortada, Joel S. Miller, and Juan J. Novoa pp 13814–13826 DOI: 10.1021/ja405352p Supporting Info |
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Activation of a σ-SnSn Bond at Copper, Followed by Double Addition to an Alkyne Nicolas Lassauque, Pauline Gualco, Sonia Mallet-Ladeira, Karinne Miqueu, Abderrahmane Amgoune, and Didier Bourissou pp 13827–13834 DOI: 10.1021/ja405516j Supporting Info |
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Ligand-Controlled Remarkable Regio- and Stereodivergence in Intermolecular Hydrosilylation of Internal Alkynes: Experimental and Theoretical Studies Shengtao Ding, Li-Juan Song, Lung Wa Chung, Xinhao Zhang, Jianwei Sun, and Yun-Dong Wu pp 13835–13842 DOI: 10.1021/ja405752w Supporting Info |
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Kinematic and Mechanical Profile of the Self-Actuation of Thermosalient Crystal Twins of 1,2,4,5-Tetrabromobenzene: A Molecular Crystalline Analogue of a Bimetallic Strip Subash Chandra Sahoo, Shashi Bhushan Sinha, M. S. R. N. Kiran, Upadrasta Ramamurty, Arcan F. Dericioglu, C. Malla Reddy, and Panče Naumov pp 13843–13850 DOI: 10.1021/ja4056323 Supporting Info |
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Repair of Hydantoin Lesions and Their Amine Adducts in DNA by Base and Nucleotide Excision Repair Paige L. McKibbin, Aaron M. Fleming, Mohammad Atif Towheed, Bennett Van Houten, Cynthia J. Burrows, and Sheila S. David pp 13851–13861 DOI: 10.1021/ja4059469 Supporting Info |
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Establishing the Ground State of the Disjoint Diradical Tetramethyleneethane with Quantum Monte Carlo Zachary D. Pozun, Xiaoge Su, and Kenneth D. Jordan pp 13862–13869 DOI: 10.1021/ja406002n Supporting Info |
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A New High-Energy Cathode for a Na-Ion Battery with Ultrahigh Stability Young-Uk Park, Dong-Hwa Seo, Hyung-Soon Kwon, Byoungkook Kim, Jongsoon Kim, Haegyeom Kim, Inkyung Kim, Han-Ill Yoo, and Kisuk Kang pp 13870–13878 DOI: 10.1021/ja406016j Supporting Info |
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Seed-Mediated Synthesis of Core/Shell FePtM/FePt (M = Pd, Au) Nanowires and Their Electrocatalysis for Oxygen Reduction Reaction Shaojun Guo, Sen Zhang, Dong Su, and Shouheng Sun pp 13879–13884 DOI: 10.1021/ja406091p Supporting Info |
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Site-Specific Antibody–Polymer Conjugates for siRNA Delivery Hua Lu, Danling Wang, Stephanie Kazane, Tsotne Javahishvili, Feng Tian, Frank Song, Aaron Sellers, Barney Barnett, and Peter G. Schultz pp 13885–13891 DOI: 10.1021/ja4059525 Supporting Info |
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Hidden Non-Innocence in an Expanded Porphyrin: Electronic Structure of the Siamese-Twin Porphyrin’s Dicopper Complex in Different Oxidation States Lina K. Blusch, Kathryn E. Craigo, Vlad Martin-Diaconescu, Ashley B. McQuarters, Eckhard Bill, Sebastian Dechert, Serena DeBeer, Nicolai Lehnert, and Franc Meyer pp 13892–13899 DOI: 10.1021/ja406176e Supporting Info |
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Consecutive Thiophene-Annulation Approach to π-Extended Thienoacene-Based Organic Semiconductors with [1]Benzothieno[3,2-b][1]benzothiophene (BTBT) Substructure Takamichi Mori, Takeshi Nishimura, Tatsuya Yamamoto, Iori Doi, Eigo Miyazaki, Itaru Osaka, and Kazuo Takimiya pp 13900–13913 DOI: 10.1021/ja406257u Supporting Info |
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Computational de Novo Design and Characterization of a Protein That Selectively Binds a Highly Hyperpolarizable Abiological Chromophore H. Christopher Fry, Andreas Lehmann, Louise E. Sinks, Inge Asselberghs, Andrey Tronin, Venkata Krishnan, J. Kent Blasie, Koen Clays, William F. DeGrado, Jeffery G. Saven, and Michael J. Therien pp 13914–13926 DOI: 10.1021/ja4067404 Supporting Info |
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Structure-Guided Discovery of New Deaminase Enzymes Daniel S. Hitchcock, Hao Fan, Jungwook Kim, Matthew Vetting, Brandan Hillerich, Ronald D. Seidel, Steven C. Almo, Brian K. Shoichet, Andrej Sali, and Frank M. Raushel pp 13927–13933 DOI: 10.1021/ja4066078 Supporting Info |
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An Exceptionally Stable, Porphyrinic Zr Metal–Organic Framework Exhibiting pH-Dependent Fluorescence Hai-Long Jiang, Dawei Feng, Kecheng Wang, Zhi-Yuan Gu, Zhangwen Wei, Ying-Pin Chen, and Hong-Cai Zhou pp 13934–13938 DOI: 10.1021/ja406844r Supporting Info |
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Sterically Directed Functionalization of the Redox-Active Bis(imino)acenaphthene Ligand Class: An Experimental and Theoretical Investigation Daniel A. Evans, Ignacio Vargas-Baca, and Alan H. Cowley pp 13939–13946 DOI: 10.1021/ja407070y Supporting Info |
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Pressure-Induced Amorphization in Single-Crystal Ta2O5 Nanowires: A Kinetic Mechanism and Improved Electrical Conductivity Xujie Lü, Qingyang Hu, Wenge Yang, Ligang Bai, Howard Sheng, Lin Wang, Fuqiang Huang, Jianguo Wen, Dean J. Miller, and Yusheng Zhao pp 13947–13953 DOI: 10.1021/ja407108u Supporting Info |
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How to Make the σ0π2 Singlet the Ground State of Carbenes Bo Chen, Andrey Yu. Rogachev, David A. Hrovat, Roald Hoffmann, and Weston Thatcher Borden pp 13954–13964 DOI: 10.1021/ja407116e Supporting Info |
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Synthesis and Characterization of Thorium(IV) and Uranium(IV) Corrole Complexes Ashleigh L. Ward, Heather L. Buckley, Wayne W. Lukens, and John Arnold pp 13965–13971 DOI: 10.1021/ja407203s Supporting Info |
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Role of Water in Mukaiyama–Aldol Reaction Catalyzed by Lanthanide Lewis Acid: A Computational Study Miho Hatanaka and Keiji Morokuma pp 13972–13979 DOI: 10.1021/ja407357c Supporting Info |
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Renalase Is an α-NAD(P)H Oxidase/Anomerase Brett A. Beaupre, Brenton R. Carmichael, Matthew R. Hoag, Dhara D. Shah, and Graham R. Moran pp 13980–13987 DOI: 10.1021/ja407384h |
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Controlling Macromolecular Topology with Genetically Encoded SpyTag–SpyCatcher Chemistry Wen-Bin Zhang, Fei Sun, David A. Tirrell, and Frances H. Arnold pp 13988–13997 DOI: 10.1021/ja4076452 Supporting Info |
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Correction to “The Entropies of Adsorbed Molecules” C. T. Campbell and Jason R. V. Sellers pp 13998–13998 DOI: 10.1021/ja407293b |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 13999–13999 DOI: 10.1021/ja4094567 |
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Activation of Snap-Top Capped Mesoporous Silica Nanocontainers Using Two Near-Infrared Photons Tania M. Guardado-Alvarez, Lekshmi Sudha Devi, Melissa M. Russell, Benjamin J. Schwartz, and Jeffrey I. Zink pp 14000–14003 DOI: 10.1021/ja407331n Supporting Info |
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Surface-Supported Supramolecular Pentamers Sujoy Karan, Yongfeng Wang, Roberto Robles, Nicolás Lorente, and Richard Berndt pp 14004–14007 DOI: 10.1021/ja405456k Supporting Info |
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A Universal DNA-Based Protein Detection System Thua N. N. Tran, Jinhui Cui, Mark R. Hartman, Songming Peng, Hisakage Funabashi, Faping Duan, Dayong Yang, John C. March, John T. Lis, Haixin Cui, and Dan Luo pp 14008–14011 DOI: 10.1021/ja405872g Supporting Info |
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Palladium(III)-Catalyzed Fluorination of Arylboronic Acid Derivatives Anthony R. Mazzotti, Michael G. Campbell, Pingping Tang, Jennifer M. Murphy, and Tobias Ritter pp 14012–14015 DOI: 10.1021/ja405919z Supporting Info |
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A Family of Porous Lonsdaleite-e Networks Obtained through Pillaring of Decorated Kagomé Lattice Sheets Alexander Schoedel, Wesley Boyette, Lukasz Wojtas, Mohamed Eddaoudi, and Michael J. Zaworotko pp 14016–14019 DOI: 10.1021/ja406030p Supporting Info |
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Electrochemistry of Aqueous Pyridinium: Exploration of a Key Aspect of Electrocatalytic Reduction of CO2 to Methanol Yong Yan, Elizabeth L. Zeitler, Jing Gu, Yuan Hu, and Andrew B. Bocarsly pp 14020–14023 DOI: 10.1021/ja4064052 Supporting Info |
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Preparation of Non-heme {FeNO}7 Models of Cysteine Dioxygenase: Sulfur versus Nitrogen Ligation and Photorelease of Nitric Oxide Alison C. McQuilken, Yang Ha, Kyle D. Sutherlin, Maxime A. Siegler, Keith O. Hodgson, Britt Hedman, Edward I. Solomon, Guy N. L. Jameson, and David P. Goldberg pp 14024–14027 DOI: 10.1021/ja4064487 Supporting Info |
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Identification of Labile Zn Sites in Drug-Target Proteins Yu-Ming Lee, Yi-Ting Wang, Yulander Duh, Hanna S. Yuan, and Carmay Lim pp 14028–14031 DOI: 10.1021/ja406300c Supporting Info |
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Highly Efficient and Robust Au/MgCuCr2O4 Catalyst for Gas-Phase Oxidation of Ethanol to Acetaldehyde Peng Liu and Emiel J. M. Hensen pp 14032–14035 DOI: 10.1021/ja406820f Supporting Info |
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Hierarchical Self-Assembly: Well-Defined Supramolecular Nanostructures and Metallohydrogels via Amphiphilic Discrete Organoplatinum(II) Metallacycles Xuzhou Yan, Shijun Li, Timothy R. Cook, Xiaofan Ji, Yong Yao, J. Bryant Pollock, Yanhui Shi, Guocan Yu, Jinying Li, Feihe Huang, and Peter J. Stang pp 14036–14039 DOI: 10.1021/ja406877b Supporting Info |
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Single-Molecule Spectroscopy of Cold Denaturation and the Temperature-Induced Collapse of Unfolded Proteins Mikayel Aznauryan, Daniel Nettels, Andrea Holla, Hagen Hofmann, and Benjamin Schuler pp 14040–14043 DOI: 10.1021/ja407009w Supporting Info |
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Asymmetric Cross-Dehydrogenative Coupling Enabled by the Design and Application of Chiral Triazole-Containing Phosphoric Acids Andrew J. Neel, Jörg P. Hehn, Pascal F. Tripet, and F. Dean Toste pp 14044–14047 DOI: 10.1021/ja407410b Supporting Info |
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Aerobic, Transition-Metal-Free, Direct, and Regiospecific Mono-α-arylation of Ketones: Synthesis and Mechanism by DFT Calculations Qing-Long Xu, Hongyin Gao, Muhammed Yousufuddin, Daniel H. Ess, and László Kürti pp 14048–14051 DOI: 10.1021/ja4074563 Supporting Info |
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Catalyst-Controlled Aliphatic C–H Oxidations with a Predictive Model for Site-Selectivity Paul E. Gormisky and M. Christina White pp 14052–14055 DOI: 10.1021/ja407388y Supporting Info |
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Enzyme Sensitive Synthetic Polymer Micelles Based on the Azobenzene Motif Jingyi Rao and Anzar Khan pp 14056–14059 DOI: 10.1021/ja407514z Supporting Info |
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Bidentate Ligands on Osmium(VI) Nitrido Complexes Control Intracellular Targeting and Cell Death Pathways Kogularamanan Suntharalingam, Timothy C. Johnstone, Peter M. Bruno, Wei Lin, Michael T. Hemann, and Stephen J. Lippard pp 14060–14063 DOI: 10.1021/ja4075375 Supporting Info |
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Patchy Particle Self-Assembly via Metal Coordination Yufeng Wang, Andrew D. Hollingsworth, Si Kyung Yang, Sonal Patel, David J. Pine, and Marcus Weck pp 14064–14067 DOI: 10.1021/ja4075979 Supporting Info |
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Robust Cuprous Phenanthroline Sensitizer for Solar Hydrogen Photocatalysis Rony S. Khnayzer, Catherine E. McCusker, Babatunde S. Olaiya, and Felix N. Castellano pp 14068–14070 DOI: 10.1021/ja407816f Supporting Info |
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Crystalline, Lewis Base-Free, Cationic Phosphoranimines (Iminophosphonium Salts) Fabian Dielmann, Curtis E. Moore, Arnold L. Rheingold, and Guy Bertrand pp 14071–14073 DOI: 10.1021/ja4080979 Supporting Info |
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Tetrabenzo[8]circulene: Aromatic Saddles from Negatively Curved Graphene Youichi Sakamoto and Toshiyasu Suzuki pp 14074–14077 DOI: 10.1021/ja407842z Supporting Info |
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Organocatalytic C–H/C–H′ Cross-Biaryl Coupling: C-Selective Arylation of Sulfonanilides with Aromatic Hydrocarbons Motoki Ito, Hiroko Kubo, Itsuki Itani, Koji Morimoto, Toshifumi Dohi, and Yasuyuki Kita pp 14078–14081 DOI: 10.1021/ja407944p Supporting Info |
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Silver-Catalyzed Radical Phosphonofluorination of Unactivated Alkenes Chengwei Zhang, Zhaodong Li, Lin Zhu, Limei Yu, Zhentao Wang, and Chaozhong Li pp 14082–14085 DOI: 10.1021/ja408031s Supporting Info |
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Synthesis, Characterization, and Nonvolatile Ternary Memory Behavior of a Larger Heteroacene with Nine Linearly Fused Rings and Two Different Heteroatoms Pei-Yang Gu, Feng Zhou, Junkuo Gao, Gang Li, Chengyuan Wang, Qing-Feng Xu, Qichun Zhang, and Jian-Mei Lu pp 14086–14089 DOI: 10.1021/ja408208c Supporting Info |
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Single-Operation Deracemization of 3H-Indolines and Tetrahydroquinolines Enabled by Phase Separation Aaron D. Lackner, Andrew V. Samant, and F. Dean Toste pp 14090–14093 DOI: 10.1021/ja4082827 Supporting Info |
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Copper-Catalyzed B–H Bond Insertion Reaction: A Highly Efficient and Enantioselective C–B Bond-Forming Reaction with Amine–Borane and Phosphine–Borane Adducts Qing-Qing Cheng, Shou-Fei Zhu, Yong-Zhen Zhang, Xiu-Lan Xie, and Qi-Lin Zhou pp 14094–14097 DOI: 10.1021/ja408306a Supporting Info |
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Construction of Vicinal All-Carbon Quaternary Stereocenters by Catalytic Asymmetric Alkylation Reaction of 3-Bromooxindoles with 3-Substituted Indoles: Total Synthesis of (+)-Perophoramidine Hailong Zhang, Liang Hong, Hong Kang, and Rui Wang pp 14098–14101 DOI: 10.1021/ja408336v Supporting Info |
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Temperature-Activated Nucleic Acid Nanostructures Ke Zhang, Xiao Zhu, Fei Jia, Evelyn Auyeung, and Chad A. Mirkin pp 14102–14105 DOI: 10.1021/ja408465t Supporting Info |
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Fabrication of Unique Chemical Patterns and Concentration Gradients with Visible Light Brett P. Fors, Justin E. Poelma, Matthew S. Menyo, Maxwell J. Robb, Daniel M. Spokoyny, John W. Kramer, J. Herbert Waite, and Craig J. Hawker pp 14106–14109 DOI: 10.1021/ja408467b Supporting Info |
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Differentiating Homogeneous and Heterogeneous Water Oxidation Catalysis: Confirmation that [Co4(H2O)2(α-PW9O34)2]10– Is a Molecular Water Oxidation Catalyst James W. Vickers, Hongjin Lv, Jordan M. Sumliner, Guibo Zhu, Zhen Luo, Djamaladdin G. Musaev, Yurii V. Geletii, and Craig L. Hill pp 14110–14118 DOI: 10.1021/ja4024868 Supporting Info |
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Nanoscale Phase Separation in Sequence-Defined Peptoid Diblock Copolymers Jing Sun, Alexander A. Teran, Xunxun Liao, Nitash P Balsara, and Ronald N. Zuckermann pp 14119–14124 DOI: 10.1021/ja404233d Supporting Info |
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Functional Near Infrared-Emitting Cr3+/Pr3+ Co-Doped Zinc Gallogermanate Persistent Luminescent Nanoparticles with Superlong Afterglow for in Vivo Targeted Bioimaging Abdukader Abdukayum, Jia-Tong Chen, Qiang Zhao, and Xiu-Ping Yan pp 14125–14133 DOI: 10.1021/ja404243v Supporting Info |
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A Two-Dimensional Polymer from the Anthracene Dimer and Triptycene Motifs Radha Bhola, Payam Payamyar, Daniel J. Murray, Bharat Kumar, Aaron J. Teator, Martin U. Schmidt, Sonja M. Hammer, Animesh Saha, Junji Sakamoto, A. Dieter Schlüter, and Benjamin T. King pp 14134–14141 DOI: 10.1021/ja404351p Supporting Info |
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Control of Plasmonic and Interband Transitions in Colloidal Indium Nitride Nanocrystals Peter K. B. Palomaki, Elisa M. Miller, and Nathan R. Neale pp 14142–14150 DOI: 10.1021/ja404599g Supporting Info |
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Single Lipid Vesicle Assay for Characterizing Single-Enzyme Kinetics of Phospholipid Hydrolysis in a Complex Biological Fluid Seyed R. Tabaei, Michael Rabe, Henrik Zetterberg, Vladimir P. Zhdanov, and Fredrik Höök pp 14151–14158 DOI: 10.1021/ja4046313 Supporting Info |
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Negative Differential Resistance by Molecular Resonant Tunneling between Neutral Tribenzosubporphine Anchored to a Au(111) Surface and Tribenzosubporphine Cation Adsorbed on to a Tungsten Tip Yutaka Majima, Daisuke Ogawa, Masachika Iwamoto, Yasuo Azuma, Eiji Tsurumaki, and Atsuhiro Osuka pp 14159–14166 DOI: 10.1021/ja404512w Supporting Info |
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Structural Evolution of Carbon Dioxide under High Pressure Cheng Lu, Maosheng Miao, and Yanming Ma pp 14167–14171 DOI: 10.1021/ja404854x Supporting Info |
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Very Rapid DNA-Templated Reaction for Efficient Signal Amplification and Its Steady-State Kinetic Analysis of the Turnover Cycle Aya Shibata, Takanori Uzawa, Yuko Nakashima, Mika Ito, Yukiko Nakano, Satoshi Shuto, Yoshihiro Ito, and Hiroshi Abe pp 14172–14178 DOI: 10.1021/ja404743m Supporting Info |
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Electrostatic Control of Peptide Side-Chain Reactivity Using Amphiphilic Homopolymer-Based Supramolecular Assemblies Feng Wang, Andrea Gomez-Escudero, Rajasekhar R. Ramireddy, Gladys Murage, S. Thayumanavan, and Richard W. Vachet pp 14179–14188 DOI: 10.1021/ja404940s Supporting Info |
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Inhibition of Mucin-Type O-Glycosylation through Metabolic Processing and Incorporation of N-Thioglycolyl-d-galactosamine Peracetate (Ac5GalNTGc) Kavita Agarwal, Rachna Kaul, Monika Garg, Asif Shajahan, Saroj Kumar Jha, and Srinivasa-Gopalan Sampathkumar pp 14189–14197 DOI: 10.1021/ja405189k Supporting Info |
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Redox Responsive Release of Hydrophobic Self-Healing Agents from Polyaniline Capsules Li-Ping Lv, Yi Zhao, Nicole Vilbrandt, Markus Gallei, Ashokanand Vimalanandan, Michael Rohwerder, Katharina Landfester, and Daniel Crespy pp 14198–14205 DOI: 10.1021/ja405279t Supporting Info |
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Understanding the Reactivity of Pd0/PR3-Catalyzed Intermolecular C(sp3)–H Bond Arylation Travis M. Figg, Masayuki Wasa, Jin-Quan Yu, and Djamaladdin G. Musaev pp 14206–14214 DOI: 10.1021/ja4053416 Supporting Info |
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Kinetic Rotating Droplet Electrochemistry: A Simple and Versatile Method for Reaction Progress Kinetic Analysis in Microliter Volumes Lylian Challier, Rebeca Miranda-Castro, Damien Marchal, Vincent Noël, François Mavré, and Benoît Limoges pp 14215–14228 DOI: 10.1021/ja405415q Supporting Info |
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Dissociative Photoionization of Glycerol and its Dimer Occurs Predominantly via a Ternary Hydrogen-Bridged Ion–Molecule Complex Franziska Bell, Qiao N. Ruan, Amir Golan, Paul R. Horn, Musahid Ahmed, Stephen R. Leone, and Martin Head-Gordon pp 14229–14239 DOI: 10.1021/ja405511v Supporting Info |
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Understanding the Role of Aqueous Solution Speciation and Its Application to the Directed Syntheses of Complex Oxidic Zr Chlorides and Sulfates Yung-Jin Hu, Karah E. Knope, S. Skanthakumar, Mercouri G. Kanatzidis, John F. Mitchell, and L. Soderholm pp 14240–14248 DOI: 10.1021/ja405555h Supporting Info |
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Probing the Influence of a 4,6-O-Acetal on the Reactivity of Galactopyranosyl Donors: Verification of the Disarming Influence of the trans–gauche Conformation of C5–C6 Bonds Myriame Moumé-Pymbock, Takayuki Furukawa, Sujit Mondal, and David Crich pp 14249–14255 DOI: 10.1021/ja405588x Supporting Info |
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Facile Rearrangement of 3-Oxoalkyl Radicals is Evident in Low-Temperature Gas-Phase Oxidation of Ketones Adam M. Scheer, Oliver Welz, Darryl Y. Sasaki, David L. Osborn, and Craig A. Taatjes pp 14256–14265 DOI: 10.1021/ja405892y Supporting Info |
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The Membrane Protein LeuT in Micellar Systems: Aggregation Dynamics and Detergent Binding to the S2 Site George Khelashvili, Michael V. LeVine, Lei Shi, Matthias Quick, Jonathan A. Javitch, and Harel Weinstein pp 14266–14275 DOI: 10.1021/ja405984v Supporting Info |
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The Chemical Basis of Serine Palmitoyltransferase Inhibition by Myriocin John M. Wadsworth, David J. Clarke, Stephen A. McMahon, Jonathan P. Lowther, Ashley E. Beattie, Pat R. R. Langridge-Smith, Howard B. Broughton, Teresa M. Dunn, James H. Naismith, and Dominic J. Campopiano pp 14276–14285 DOI: 10.1021/ja4059876 Supporting Info |
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Size Effect and Odd–Even Alternation in the Melting of Single and Stacked AgSCn Layers: Synthesis and Nanocalorimetry Measurements Lito P. de la Rama, Liang Hu, Zichao Ye, Mikhail Y. Efremov, and Leslie H. Allen pp 14286–14298 DOI: 10.1021/ja4059958 Supporting Info |
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Electrooxidation of Alcohols Catalyzed by Amino Alcohol Ligated Ruthenium Complexes Kristen R. Brownell, Charles C. L. McCrory, Christopher E. D. Chidsey, Richard H. Perry, Richard N. Zare, and Robert M. Waymouth pp 14299–14305 DOI: 10.1021/ja4055564 Supporting Info |
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Ruthenium-Catalyzed Hydroformylation/Reduction of Olefins to Alcohols: Extending the Scope to Internal Alkenes Lipeng Wu, Ivana Fleischer, Ralf Jackstell, Irina Profir, Robert Franke, and Matthias Beller pp 14306–14312 DOI: 10.1021/ja4060977 Supporting Info |
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Total Synthesis, Relay Synthesis, and Structural Confirmation of the C18-Norditerpenoid Alkaloid Neofinaconitine Yuan Shi, Jeremy T. Wilmot, Lars Ulrik Nordstrøm, Derek S. Tan, and David Y. Gin pp 14313–14320 DOI: 10.1021/ja4064958 Supporting Info |
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Deep-Blue Phosphorescence from Perfluoro Carbonyl-Substituted Iridium Complexes Sunghun Lee, Seul-Ong Kim, Hyun Shin, Hui-Jun Yun, Kiyull Yang, Soon-Ki Kwon, Jang-Joo Kim, and Yun-Hi Kim pp 14321–14328 DOI: 10.1021/ja4065188 Supporting Info |
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Why (1 0 0) Terraces Break and Make Bonds: Oxidation of Dimethyl Ether on Platinum Single-Crystal Electrodes Hongjiao Li, Federico Calle-Vallejo, Manuel J. Kolb, Youngkook Kwon, Yongdan Li, and Marc T.M. Koper pp 14329–14338 DOI: 10.1021/ja406655q Supporting Info |
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Biochemical Determination of Enzyme-Bound Metabolites: Preferential Accumulation of a Programmed Octaketide on the Enediyne Polyketide Synthase CalE8 Katherine Belecki and Craig A. Townsend pp 14339–14348 DOI: 10.1021/ja406697t Supporting Info |
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Combined NMR Analysis of Huge Residual Dipolar Couplings and Pseudocontact Shifts in Terbium(III)-Phthalocyaninato Single Molecule Magnets Marko Damjanovic, Keiichi Katoh, Masahiro Yamashita, and Markus Enders pp 14349–14358 DOI: 10.1021/ja4069485 Supporting Info |
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Proton-Coupled Electron Transfers: pH-Dependent Driving Forces? Fundamentals and Artifacts Julien Bonin, Cyrille Costentin, Marc Robert, Mathilde Routier, and Jean-Michel Savéant pp 14359–14366 DOI: 10.1021/ja406712c Supporting Info |
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Mixed Aggregates of an Alkyl Lithium Reagent and a Chiral Lithium Amide Derived from N-Ethyl-O-triisopropylsilyl Valinol Chicheung Su, Russell Hopson, and Paul G. Williard pp 14367–14379 DOI: 10.1021/ja406912h Supporting Info |
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Nanocrystal Diffusion Doping Vladimir A. Vlaskin, Charles J. Barrows, Christian S. Erickson, and Daniel R. Gamelin pp 14380–14389 DOI: 10.1021/ja4072207 Supporting Info |
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Stereochemical Inversion of a Cyano-Stabilized Grignard Reagent: Remarkable Effects of the Ethereal Solvent Structure and Concentration Ming Gao, Neeraj N. Patwardhan, and Paul R. Carlier pp 14390–14400 DOI: 10.1021/ja407348s Supporting Info |
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Hydrophobic Collapse of Foldamer Capsules Drives Picomolar-Level Chloride Binding in Aqueous Acetonitrile Solutions Yuran Hua, Yun Liu, Chun-Hsing Chen, and Amar H. Flood pp 14401–14412 DOI: 10.1021/ja4074744 Supporting Info |
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Visible-Light Photoredox Catalysis: Selective Reduction of Carbon Dioxide to Carbon Monoxide by a Nickel N-Heterocyclic Carbene–Isoquinoline Complex V. Sara Thoi, Nikolay Kornienko, Charles G. Margarit, Peidong Yang, and Christopher J. Chang pp 14413–14424 DOI: 10.1021/ja4074003 Supporting Info |
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Improved Biocatalysts from a Synthetic Circular Permutation Library of the Flavin-Dependent Oxidoreductase Old Yellow Enzyme Ashley B. Daugherty, Sridhar Govindarajan, and Stefan Lutz pp 14425–14432 DOI: 10.1021/ja4074886 Supporting Info |
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Molecular Iodine Initiates Hydroborations of Alkenes with N-Heterocyclic Carbene Boranes Xiangcheng Pan, Anne Boussonnière, and Dennis P. Curran pp 14433–14437 DOI: 10.1021/ja407678e Supporting Info |
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Experimental and Computational Studies on the [3,3]- and [3,5]-Sigmatropic Rearrangements of Acetoxycyclohexadienones: A Non-ionic Mechanism for Acyl Migration Shikha Sharma, Trideep Rajale, David B. Cordes, Fernando Hung-Low, and David M. Birney pp 14438–14447 DOI: 10.1021/ja4077364 Supporting Info |
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Synthesis of Open-Shell, Bimetallic Mn/Fe Trinuclear Clusters Tamara M. Powers, Nina X. Gu, Alison R. Fout, Anne M. Baldwin, Raúl Hernández Sánchez, Denise M. Alfonso, Yu-Sheng Chen, Shao-Liang Zheng, and Theodore A. Betley pp 14448–14458 DOI: 10.1021/ja408003d Supporting Info |
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Correction to “A Sugar-Functionalized Amphiphilic Pillar[5]arene: Synthesis, Self-Assembly in Water, and Application in Bacterial Cell Agglutination” Guocan Yu, Yingjie Ma, Chengyou Han, Yong Yao, Guping Tang, Zhengwei Mao, Changyou Gao, and Feihe Huang pp 14459–14459 DOI: 10.1021/ja407418m |
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Correction to “Synthesis, Characterization, and Heterobimetallic Cooperation in a Titanium–Chromium Catalyst for Highly Branched Polyethylenes” Shaofeng Liu, Alessandro Motta, Massimiliano Delferro, and Tobin J. Marks pp 14460–14460 DOI: 10.1021/ja4082217 |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 14461–14461 DOI: 10.1021/ja409879f |
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A Vision for Vaccines Built from Fully Synthetic Tumor-Associated Antigens: From the Laboratory to the Clinic Rebecca M. Wilson and Samuel J. Danishefsky pp 14462–14472 DOI: 10.1021/ja405932r |
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Catalysis by Desolvation: The Catalytic Prowess of SAM-Dependent Halide-Alkylating Enzymes Danielle C. Lohman, David R. Edwards, and Richard Wolfenden pp 14473–14475 DOI: 10.1021/ja406381b Supporting Info |
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CdSe–CdS Nanoheteroplatelets with Efficient Photoexcitation of Central CdSe Region through Epitaxially Grown CdS Wings Anatol Prudnikau, Andrey Chuvilin, and Mikhail Artemyev pp 14476–14479 DOI: 10.1021/ja401737z Supporting Info |
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Copper-Catalyzed One-Pot Trifluoromethylation/Aryl Migration/Desulfonylation and C(sp2)–N Bond Formation of Conjugated Tosyl Amides Wangqing Kong, Maria Casimiro, Estı́baliz Merino, and Cristina Nevado pp 14480–14483 DOI: 10.1021/ja403954g Supporting Info |
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An Efficient Light-Driven P450 BM3 Biocatalyst Ngoc-Han Tran, Daniel Nguyen, Sudharsan Dwaraknath, Sruthi Mahadevan, Garrett Chavez, Angelina Nguyen, Thanh Dao, Sarah Mullen, Thien-Anh Nguyen, and Lionel E. Cheruzel pp 14484–14487 DOI: 10.1021/ja409337v Supporting Info |
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Iron(III)-Based Metal–Organic Frameworks As Visible Light Photocatalysts Katrien G. M. Laurier, Frederik Vermoortele, Rob Ameloot, Dirk E. De Vos, Johan Hofkens, and Maarten B. J. Roeffaers pp 14488–14491 DOI: 10.1021/ja405086e Supporting Info |
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Rh(III)-Catalyzed C–H Activation and Double Directing Group Strategy for the Regioselective Synthesis of Naphthyridinones John R. Huckins, Eric A. Bercot, Oliver R. Thiel, Tsang-Lin Hwang, and Matthew M. Bio pp 14492–14495 DOI: 10.1021/ja405140f Supporting Info |
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Temporally Controlled Targeting of 4-Hydroxynonenal to Specific Proteins in Living Cells Xinqiang Fang, Yuan Fu, Marcus J. C. Long, Joseph A. Haegele, Eva J. Ge, Saba Parvez, and Yimon Aye pp 14496–14499 DOI: 10.1021/ja405400k Supporting Info |
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A Photo-driven Polyoxometalate Complex Shuttle and Its Homogeneous Catalysis and Heterogeneous Separation Yang Yang, Bin Zhang, Yizhan Wang, Liang Yue, Wen Li, and Lixin Wu pp 14500–14503 DOI: 10.1021/ja4057882 Supporting Info |
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Borate as a Synergistic Anion for Marinobacter algicola Ferric Binding Protein, FbpA: A Role for Boron in Iron Transport in Marine Life Aruna J. Weerasinghe, Shady A. Amin, Ryan A. Barker, Thaer Othman, Ariel N. Romano, Claire J. Parker Siburt, Jerrell Tisnado, Lisa A. Lambert, Tom Huxford, Carl J. Carrano, and Alvin L. Crumbliss pp 14504–14507 DOI: 10.1021/ja406609s Supporting Info |
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Mechanistic Origin of Chemo- and Regioselectivity of Nickel-Catalyzed [3 + 2 + 2] Cyclization Reaction Shinsuke Komagawa, Chao Wang, Keiji Morokuma, Shinichi Saito, and Masanobu Uchiyama pp 14508–14511 DOI: 10.1021/ja4068468 Supporting Info |
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Controlling Spatial Distributions of Molecules in Multicomponent Organic Crystals, with Quantitative Mapping by Confocal Raman Microspectrometry Benjamin A. Palmer, Annaïg Le Comte, Kenneth D.M. Harris, and François Guillaume pp 14512–14515 DOI: 10.1021/ja406866a Supporting Info |
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Rh2(R-TPCP)4-Catalyzed Enantioselective [3+2]-Cycloaddition between Nitrones and Vinyldiazoacetates Changming Qin and Huw M. L. Davies pp 14516–14519 DOI: 10.1021/ja4069003 Supporting Info |
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Generating Tunable White Light by Resonance Energy Transfer in Transparent Dye-Conjugated Metal Oxide Nanocrystals Ting Wang, Vadim Chirmanov, Wan Hang M. Chiu, and Pavle V. Radovanovic pp 14520–14523 DOI: 10.1021/ja407013z Supporting Info |
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Dissecting the Stereocontrol Elements of a Catalytic Asymmetric Chlorolactonization: Syn Addition Obviates Bridging Chloronium Roozbeh Yousefi, Kumar Dilip Ashtekar, Daniel C. Whitehead, James E. Jackson, and Babak Borhan pp 14524–14527 DOI: 10.1021/ja4072145 Supporting Info |
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Inside versus Outside: Ion Redistribution in Nitric Acid Reacted Sea Spray Aerosol Particles as Determined by Single Particle Analysis Andrew P. Ault, Timothy L. Guasco, Olivia S. Ryder, Jonas Baltrusaitis, Luis A. Cuadra-Rodriguez, Douglas B. Collins, Matthew J. Ruppel, Timothy H. Bertram, Kimberly A. Prather, and Vicki H. Grassian pp 14528–14531 DOI: 10.1021/ja407117x Supporting Info |
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Increasing the Gravimetric Energy Density of Organic Based Secondary Battery Cathodes Using Small Radius Cations (Li+ and Mg2+) Kenneth Hernández-Burgos, Gabriel G. Rodríguez-Calero, Weidong Zhou, Stephen E. Burkhardt, and Héctor D. Abruña pp 14532–14535 DOI: 10.1021/ja407273c Supporting Info |
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A Simple Method to Measure Protein Side-Chain Mobility Using NMR Chemical Shifts Mark V. Berjanskii and David S. Wishart pp 14536–14539 DOI: 10.1021/ja407509z Supporting Info |
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Superconductivity in the Narrow-Gap Semiconductor CsBi4Te6 Christos D. Malliakas, Duck Young Chung, Helmut Claus, and Mercouri G. Kanatzidis pp 14540–14543 DOI: 10.1021/ja407530u Supporting Info |
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Capturing a Sulfenic Acid with Arylboronic Acids and Benzoxaborole C. Tony Liu and Stephen J. Benkovic pp 14544–14547 DOI: 10.1021/ja407628a Supporting Info |
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Design, Preparation, and Implementation of an Imidazole-Based Chiral Biaryl P,N-Ligand for Asymmetric Catalysis Flavio S. P. Cardoso, Khalil A. Abboud, and Aaron Aponick pp 14548–14551 DOI: 10.1021/ja407689a Supporting Info |
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Total Synthesis of Maoecrystal V: Early-Stage C–H Functionalization and Lactone Assembly by Radical Cyclization Ping Lu, Zhenhua Gu, and Armen Zakarian pp 14552–14555 DOI: 10.1021/ja408231t Supporting Info |
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Catalytic Asymmetric Insertion of Diazoesters into Aryl-CHO Bonds: Highly Enantioselective Construction of Chiral All-Carbon Quaternary Centers Lizhu Gao, Byung Chul Kang, and Do Hyun Ryu pp 14556–14559 DOI: 10.1021/ja408196g Supporting Info |
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Order–Disorder Transition of Dipolar Rotor in a Crystalline Molecular Gyrotop and Its Optical Change Wataru Setaka and Kentaro Yamaguchi pp 14560–14563 DOI: 10.1021/ja408405f Supporting Info |
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o-Phenylene Octamers as Surface Modifiers for Homeotropic Columnar Ordering of Discotic Liquid Crystals Takashi Kajitani, Yuki Suna, Atsuko Kosaka, Terutsune Osawa, Shigenori Fujikawa, Masaki Takata, Takanori Fukushima, and Takuzo Aida pp 14564–14567 DOI: 10.1021/ja4087853 Supporting Info |
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An Alkyne–Aspirin Chemical Reporter for the Detection of Aspirin-Dependent Protein Modification in Living Cells Leslie A. Bateman, Balyn W. Zaro, Stephanie M. Miller, and Matthew R. Pratt pp 14568–14573 DOI: 10.1021/ja408322b Supporting Info |
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Catalytic Mechanism of the Glycyl Radical Enzyme 4-Hydroxyphenylacetate Decarboxylase from Continuum Electrostatic and QC/MM Calculations Mikolaj Feliks, Berta M. Martins, and G. Matthias Ullmann pp 14574–14585 DOI: 10.1021/ja402379q Supporting Info |
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Spatial Waves in Synthetic Biochemical Networks Adrien Padirac, Teruo Fujii, André Estévez-Torres, and Yannick Rondelez pp 14586–14592 DOI: 10.1021/ja403584p Supporting Info |
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Deamination, Oxidation, and C–C Bond Cleavage Reactivity of 5-Hydroxymethylcytosine, 5-Formylcytosine, and 5-Carboxycytosine Stefan Schiesser, Toni Pfaffeneder, Keyarash Sadeghian, Benjamin Hackner, Barbara Steigenberger, Arne S. Schröder, Jessica Steinbacher, Gengo Kashiwazaki, Georg Höfner, Klaus T. Wanner, Christian Ochsenfeld, and Thomas Carell pp 14593–14599 DOI: 10.1021/ja403229y Supporting Info |
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Atomic Imaging of the Irreversible Sensing Mechanism of NO2 Adsorption on Copper Phthalocyanine Jun Hong Park, James E. Royer, Evgeniy Chagarov, Tobin Kaufman-Osborn, Mary Edmonds, Tyler Kent, Sangyeob Lee, William C. Trogler, and Andrew C. Kummel pp 14600–14609 DOI: 10.1021/ja403752r Supporting Info |
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Effect of Internal Cavities on Folding Rates and Routes Revealed by Real-Time Pressure-Jump NMR Spectroscopy Julien Roche, Mariano Dellarole, José A. Caro, Douglas R. Norberto, Angel E. Garcia, Bertrand Garcia-Moreno, Christian Roumestand, and Catherine A. Royer pp 14610–14618 DOI: 10.1021/ja406682e Supporting Info |
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Microfluidic Approach toward Continuous and Ultrafast Synthesis of Metal–Organic Framework Crystals and Hetero Structures in Confined Microdroplets Marco Faustini, Jun Kim, Guan-Young Jeong, Jin Yeong Kim, Hoi Ri Moon, Wha-Seung Ahn, and Dong-Pyo Kim pp 14619–14626 DOI: 10.1021/ja4039642 Supporting Info |
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Mechanism of Transient Binding and Release of Substrate Protein during the Allosteric Cycle of the p97 Nanomachine Sam Tonddast-Navaei and George Stan pp 14627–14636 DOI: 10.1021/ja404051b Supporting Info |
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Ultrafast Carbonyl Motion of the Photoactive Yellow Protein Chromophore Probed by Femtosecond Circular Dichroism Lucille Mendonça, François Hache, Pascale Changenet-Barret, Pascal Plaza, Haik Chosrowjan, Seiji Taniguchi, and Yasushi Imamoto pp 14637–14643 DOI: 10.1021/ja404503q Supporting Info |
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Using Reduced Catalysts for Oxidation Reactions: Mechanistic Studies of the “Periana-Catalytica” System for CH4 Oxidation Oleg A. Mironov, Steven M. Bischof, Michael M. Konnick, Brian G. Hashiguchi, Vadim R. Ziatdinov, William A. Goddard, III, Mårten Ahlquist, and Roy A. Periana pp 14644–14658 DOI: 10.1021/ja404895z Supporting Info |
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Nickel Pyridinethiolate Complexes as Catalysts for the Light-Driven Production of Hydrogen from Aqueous Solutions in Noble-Metal-Free Systems Zhiji Han, Luxi Shen, William W. Brennessel, Patrick L. Holland, and Richard Eisenberg pp 14659–14669 DOI: 10.1021/ja405257s Supporting Info |
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A Dinuclear Cobalt Complex Featuring Unprecedented Anodic and Cathodic Redox Switches for Single-Molecule Magnet Activity Skye Fortier, Jennifer J. Le Roy, Chun-Hsing Chen, Veacheslav Vieru, Muralee Murugesu, Liviu F. Chibotaru, Daniel J. Mindiola, and Kenneth G. Caulton pp 14670–14678 DOI: 10.1021/ja405284t Supporting Info |
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Mechanism of Acyl–Enzyme Complex Formation from the Henry–Michaelis Complex of Class C β-Lactamases with β-Lactam Antibiotics Ravi Tripathi and Nisanth N. Nair pp 14679–14690 DOI: 10.1021/ja405319n Supporting Info |
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Nanoscale-Phase-Separated Pd–Rh Boxes Synthesized via Metal Migration: An Archetype for Studying Lattice Strain and Composition Effects in Electrocatalysis Brian T. Sneed, Casey N. Brodsky, Chun-Hong Kuo, Leo K. Lamontagne, Ying Jiang, Yong Wang, Franklin (Feng) Tao, Weixin Huang, and Chia-Kuang Tsung pp 14691–14700 DOI: 10.1021/ja405387q Supporting Info |
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Singlet Exciton Fission in Polycrystalline Thin Films of a Slip-Stacked Perylenediimide Samuel W. Eaton, Leah E. Shoer, Steven D. Karlen, Scott M. Dyar, Eric A. Margulies, Brad S. Veldkamp, Charusheela Ramanan, Daniel A. Hartzler, Sergei Savikhin, Tobin J. Marks, and Michael R. Wasielewski pp 14701–14712 DOI: 10.1021/ja4053174 Supporting Info |
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Electronic and Exchange Coupling in a Cross-Conjugated D–B–A Biradical: Mechanistic Implications for Quantum Interference Effects Martin L. Kirk, David A. Shultz, Daniel E. Stasiw, Diana Habel-Rodriguez, Benjamin Stein, and Paul D. Boyle pp 14713–14725 DOI: 10.1021/ja405354x Supporting Info |
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Improved Quenched Fluorescent Probe for Imaging of Cysteine Cathepsin Activity Martijn Verdoes, Kristina Oresic Bender, Ehud Segal, Wouter A. van der Linden, Salahuddin Syed, Nimali P. Withana, Laura E. Sanman, and Matthew Bogyo pp 14726–14730 DOI: 10.1021/ja4056068 Supporting Info |
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Carbon K-Edge X-ray Absorption Spectroscopy and Time-Dependent Density Functional Theory Examination of Metal–Carbon Bonding in Metallocene Dichlorides Stefan G. Minasian, Jason M. Keith, Enrique R. Batista, Kevin S. Boland, Stosh A. Kozimor, Richard L. Martin, David K. Shuh, Tolek Tyliszczak, and Louis J. Vernon pp 14731–14740 DOI: 10.1021/ja405844j Supporting Info |
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Computational Analysis of the Binding Specificity of Gleevec to Abl, c-Kit, Lck, and c-Src Tyrosine Kinases Yen-Lin Lin and Benoît Roux pp 14741–14753 DOI: 10.1021/ja405939x Supporting Info |
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Room Temperature Dehydrogenation of Ethane, Propane, Linear Alkanes C4–C8, and Some Cyclic Alkanes by Titanium–Carbon Multiple Bonds Marco G. Crestani, Anne K. Hickey, Xinfeng Gao, Balazs Pinter, Vincent N. Cavaliere, Jun-Ichi Ito, Chun-Hsing Chen, and Daniel J. Mindiola pp 14754–14767 DOI: 10.1021/ja4060178 Supporting Info |
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Multiple Unfolding Pathways of Leucine Binding Protein (LBP) Probed by Single-Molecule Force Spectroscopy (SMFS) Hema Chandra Kotamarthi, Riddhi Sharma, Satya Narayan, Sayoni Ray, and Sri Rama Koti Ainavarapu pp 14768–14774 DOI: 10.1021/ja406238q Supporting Info |
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Chemical Analog-to-Digital Signal Conversion Based on Robust Threshold Chemistry and Its Evaluation in the Context of Microfluidics-Based Quantitative Assays Toan Huynh, Bing Sun, Liang Li, Kevin P. Nichols, Jay L. Koyner, and Rustem F. Ismagilov pp 14775–14783 DOI: 10.1021/ja4062882 Supporting Info |
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Versatile Reactivity of a Four-Coordinate Scandium Phosphinidene Complex: Reduction, Addition, and CO Activation Reactions Yingdong Lv, Christos E. Kefalidis, Jiliang Zhou, Laurent Maron, Xuebing Leng, and Yaofeng Chen pp 14784–14796 DOI: 10.1021/ja406413d Supporting Info |
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Ion-Based Materials Derived from Positively and Negatively Charged Chloride Complexes of π-Conjugated Molecules Bin Dong, Tsuneaki Sakurai, Yuya Bando, Shu Seki, Kazuto Takaishi, Masanobu Uchiyama, Atsuya Muranaka, and Hiromitsu Maeda pp 14797–14805 DOI: 10.1021/ja4071333 Supporting Info |
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Kinetic Resolution of Unsaturated Amides in a Chlorocyclization Reaction: Concomitant Enantiomer Differentiation and Face Selective Alkene Chlorination by a Single Catalyst Arvind Jaganathan, Richard J. Staples, and Babak Borhan pp 14806–14813 DOI: 10.1021/ja407241d Supporting Info |
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In-Situ Generation of Differential Sensors that Fingerprint Kinases and the Cellular Response to Their Expression Diana Zamora-Olivares, Tamer S. Kaoud, Kevin N. Dalby, and Eric V. Anslyn pp 14814–14820 DOI: 10.1021/ja407397z Supporting Info |
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Locating Protonated Amines in Clathrates Terrence M. Chang, Richard J. Cooper, and Evan R. Williams pp 14821–14830 DOI: 10.1021/ja407414d Supporting Info |
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Effective Sugar Nucleotide Regeneration for the Large-Scale Enzymatic Synthesis of Globo H and SSEA4 Tsung-I Tsai, Hsin-Yu Lee, Shih-Huang Chang, Chia-Hung Wang, Yu-Chen Tu, Yu-Chen Lin, Der-Ren Hwang, Chung-Yi Wu, and Chi-Huey Wong pp 14831–14839 DOI: 10.1021/ja4075584 Supporting Info |
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Rational Design of a Photomagnetic Chain: Bridging Single-Molecule Magnets with a Spin-Crossover Complex Rodica Ababei, Céline Pichon, Olivier Roubeau, Yang-Guang Li, Nicolas Bréfuel, Lionel Buisson, Philippe Guionneau, Corine Mathonière, and Rodolphe Clérac pp 14840–14853 DOI: 10.1021/ja407570n Supporting Info |
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Born–Haber Cycle for Monolayer Self-Assembly at the Liquid–Solid Interface: Assessing the Enthalpic Driving Force Wentao Song, Natalia Martsinovich, Wolfgang M. Heckl, and Markus Lackinger pp 14854–14862 DOI: 10.1021/ja407698t Supporting Info |
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Nile Blue-Based Nanosized pH Sensors for Simultaneous Far-Red and Near-Infrared Live Bioimaging Jeppe Madsen, Irene Canton, Nicholas J. Warren, Efrosyni Themistou, Adam Blanazs, Burcin Ustbas, Xiaohe Tian, Russell Pearson, Giuseppe Battaglia, Andrew L. Lewis, and Steven P. Armes pp 14863–14870 DOI: 10.1021/ja407380t Supporting Info |
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Asymmetric Epoxidation with H2O2 by Manipulating the Electronic Properties of Non-heme Iron Catalysts Olaf Cussó, Isaac Garcia-Bosch, Xavi Ribas, Julio Lloret-Fillol, and Miquel Costas pp 14871–14878 DOI: 10.1021/ja4078446 Supporting Info |
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Cucurbit[8]uril and Blue-Box: High-Energy Water Release Overwhelms Electrostatic Interactions Frank Biedermann, Michele Vendruscolo, Oren A. Scherman, Alfonso De Simone, and Werner M. Nau pp 14879–14888 DOI: 10.1021/ja407951x Supporting Info |
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Three Distinct Equilibrium States via Self-Assembly: Simple Access to a Supramolecular Ion-Controlled NAND Logic Gate Dong Sub Kim, Vincent M. Lynch, Jung Su Park, and Jonathan L. Sessler pp 14889–14894 DOI: 10.1021/ja4080198 Supporting Info |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 14895–14895 DOI: 10.1021/ja410056x |
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Record High Hole Mobility in Polymer Semiconductors via Side-Chain Engineering Il Kang, Hui-Jun Yun, Dae Sung Chung, Soon-Ki Kwon, and Yun-Hi Kim pp 14896–14899 DOI: 10.1021/ja405112s Supporting Info |
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Reactions of a Chromium(III)-Superoxo Complex and Nitric Oxide That Lead to the Formation of Chromium(IV)-Oxo and Chromium(III)-Nitrito Complexes Atsutoshi Yokoyama, Kyung-Bin Cho, Kenneth D. Karlin, and Wonwoo Nam pp 14900–14903 DOI: 10.1021/ja405891n Supporting Info |
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Modulation of CEST Images in Vivo by T1 Relaxation: A New Approach in the Design of Responsive PARACEST Agents S. James Ratnakar, Todd C. Soesbe, Lloyd Laporca Lumata, Quyen N. Do, Subha Viswanathan, Chien-Yuan Lin, A. Dean Sherry, and Zoltan Kovacs pp 14904–14907 DOI: 10.1021/ja406738y Supporting Info |
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Highly Selective Fluorescent Recognition of Sulfate in Water by Two Rigid Tetrakisimidazolium Macrocycles with Peripheral Chains Hongjun Zhou, Yinsong, Zhao, Ge Gao, Shiqing Li, Jingbo Lan, and Jingsong You pp 14908–14911 DOI: 10.1021/ja406638b Supporting Info |
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One-Electron Oxidation of an Organic Molecule by B(C6F5)3; Isolation and Structures of Stable Non-para-substituted Triarylamine Cation Radical and Bis(triarylamine) Dication Diradicaloid Xin Zheng, Xingyong Wang, Yunfan Qiu, Yuantao Li, Chenkun Zhou, Yunxia Sui, Yizhi Li, Jing Ma, and Xinping Wang pp 14912–14915 DOI: 10.1021/ja407318h Supporting Info |
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Aromatizing Olefin Metathesis by Ligand Isolation inside a Metal– Organic Framework Nicolaas A. Vermeulen, Olga Karagiaridi, Amy A. Sarjeant, Charlotte L. Stern, Joseph T. Hupp, Omar K. Farha, and J. Fraser Stoddart pp 14916–14919 DOI: 10.1021/ja407333q Supporting Info |
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High-Mobility n-Type Conjugated Polymers Based on Electron-Deficient Tetraazabenzodifluoranthene Diimide for Organic Electronics Haiyan Li, Felix Sunjoo Kim, Guoqiang Ren, and Samson A. Jenekhe pp 14920–14923 DOI: 10.1021/ja407471b Supporting Info |
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Surface-Modified Silicon Nanoparticles with Ultrabright Photoluminescence and Single-Exponential Decay for Nanoscale Fluorescence Lifetime Imaging of Temperature Qi Li, Yao He, Jian Chang, Lei Wang, Hongzheng Chen, Yan-Wen Tan, Haiyu Wang, and Zhengzhong Shao pp 14924–14927 DOI: 10.1021/ja407508v Supporting Info |
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DNA Catalysts with Tyrosine Kinase Activity Shannon M. Walsh, Amit Sachdeva, and Scott K. Silverman pp 14928–14931 DOI: 10.1021/ja407586u Supporting Info |
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Hybrid and Nonhybrid Lipids Exert Common Effects on Membrane Raft Size and Morphology Frederick A. Heberle, Milka Doktorova, Shih Lin Goh, Robert F. Standaert, John Katsaras, and Gerald W. Feigenson pp 14932–14935 DOI: 10.1021/ja407624c Supporting Info |
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Conversion of Azides into Diazo Compounds in Water Ho-Hsuan Chou and Ronald T. Raines pp 14936–14939 DOI: 10.1021/ja407822b Supporting Info |
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Genetically Encoded Fluorescent Probe for the Selective Detection of Peroxynitrite Zhi-jie Chen, Wei Ren, Quintin E. Wright, and Hui-wang Ai pp 14940–14943 DOI: 10.1021/ja408011q Supporting Info |
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Intraduplex DNA-Mediated Electrochemistry of Covalently Tethered Redox-Active Reporters Catrina G. Pheeney and Jacqueline K. Barton pp 14944–14947 DOI: 10.1021/ja408135g Supporting Info |
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Enantioselective Intermolecular [2+2] Photocycloadditions of Isoquinolone Mediated by a Chiral Hydrogen-Bonding Template Susannah C. Coote and Thorsten Bach pp 14948–14951 DOI: 10.1021/ja408167r Supporting Info |
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Bulk Synthesis of Exfoliated Two-Dimensional Polymers Using Hydrazone-Linked Covalent Organic Frameworks David N. Bunck and William R. Dichtel pp 14952–14955 DOI: 10.1021/ja408243n Supporting Info |
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Dynamic and Reversible Fluorescence Imaging of Superoxide Anion Fluctuations in Live Cells and in Vivo Wen Zhang, Ping Li, Fan Yang, Xiufen Hu, Chuanzhi Sun, Wei Zhang, Dezhan Chen, and Bo Tang pp 14956–14959 DOI: 10.1021/ja408524j Supporting Info |
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All-Polymer Solar Cells with 3.3% Efficiency Based on Naphthalene Diimide-Selenophene Copolymer Acceptor Taeshik Earmme, Ye-Jin Hwang, Nishit M. Murari, Selvam Subramaniyan, and Samson A. Jenekhe pp 14960–14963 DOI: 10.1021/ja4085429 Supporting Info |
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Assembly of Amphiphilic Baskets into Stimuli-Responsive Vesicles. Developing a Strategy for the Detection of Organophosphorus Chemical Nerve Agents Shigui Chen, Yian Ruan, Jason D. Brown, Judith Gallucci, Veselin Maslak, Christopher M. Hadad, and Jovica D. Badjić pp 14964–14967 DOI: 10.1021/ja408585j Supporting Info |
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Electrophilic Rearrangements of Chiral Amides: A Traceless Asymmetric α-Allylation Bo Peng, Danny Geerdink, and Nuno Maulide pp 14968–14971 DOI: 10.1021/ja408856p Supporting Info |
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C–H Activation by a Diselenido Dinickel(II) Complex Jessica Wallick, Charles G. Riordan, and Glenn P. A. Yap pp 14972–14974 DOI: 10.1021/ja407995r Supporting Info |
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Methyl-Coenzyme M Reductase from Methanogenic Archaea: Isotope Effects on the Formation and Anaerobic Oxidation of Methane Silvan Scheller, Meike Goenrich, Rudolf K. Thauer, and Bernhard Jaun pp 14975–14984 DOI: 10.1021/ja406485z Supporting Info |
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Methyl-Coenzyme M Reductase from Methanogenic Archaea: Isotope Effects on Label Exchange and Ethane Formation with the Homologous Substrate Ethyl-Coenzyme M Silvan Scheller, Meike Goenrich, Rudolf K. Thauer, and Bernhard Jaun pp 14985–14995 DOI: 10.1021/ja4064876 Supporting Info |
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Mechanism and Enantioselectivity in Palladium-Catalyzed Conjugate Addition of Arylboronic Acids to β-Substituted Cyclic Enones: Insights from Computation and Experiment Jeffrey C. Holder, Lufeng Zou, Alexander N. Marziale, Peng Liu, Yu Lan, Michele Gatti, Kotaro Kikushima, K. N. Houk, and Brian M. Stoltz pp 14996–15007 DOI: 10.1021/ja401713g Supporting Info |
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Homogeneous Ice Nucleation at Moderate Supercooling from Molecular Simulation E. Sanz, C. Vega, J. R. Espinosa, R. Caballero-Bernal, J. L. F. Abascal, and C. Valeriani pp 15008–15017 DOI: 10.1021/ja4028814 Supporting Info |
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Mechanistic Study on the Solution-Phase n-Doping of 1,3-Dimethyl-2-aryl-2,3-dihydro-1H-benzoimidazole Derivatives Benjamin D. Naab, Song Guo, Selina Olthof, Eric G. B. Evans, Peng Wei, Glenn L. Millhauser, Antoine Kahn, Stephen Barlow, Seth R. Marder, and Zhenan Bao pp 15018–15025 DOI: 10.1021/ja403906d Supporting Info |
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How Light-Harvesting Semiconductors Can Alter the Bias of Reversible Electrocatalysts in Favor of H2 Production and CO2 Reduction Andreas Bachmeier, Vincent C. C. Wang, Thomas W. Woolerton, Sophie Bell, Juan C. Fontecilla-Camps, Mehmet Can, Stephen W. Ragsdale, Yatendra S. Chaudhary, and Fraser A. Armstrong pp 15026–15032 DOI: 10.1021/ja4042675 Supporting Info |
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Real-Time Observation of the Destruction of Hydration Shells under Electrochemical Force Akira Yamakata, Eiji Soeta, Tatsuya Ishiyama, Masatoshi Osawa, and Akihiro Morita pp 15033–15039 DOI: 10.1021/ja408326d Supporting Info |
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Residue-Dependent Adsorption of Model Oligopeptides on Gold Kenan P. Fears, Thomas D. Clark, and Dmitri Y. Petrovykh pp 15040–15052 DOI: 10.1021/ja404346p Supporting Info |
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Mechanism of Cobalt Self-Exchange Electron Transfer Andrew M. Ullman and Daniel G. Nocera pp 15053–15061 DOI: 10.1021/ja404469y Supporting Info |
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Olefin Hydroaryloxylation Catalyzed by Pincer–Iridium Complexes Michael C. Haibach, Changjian Guan, David Y. Wang, Bo Li, Nicholas Lease, Andrew M. Steffens, Karsten Krogh-Jespersen, and Alan S. Goldman pp 15062–15070 DOI: 10.1021/ja404566v Supporting Info |
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Control of PbSe Nanorod Aspect Ratio by Limiting Phosphine Hydrolysis Janice E. Boercker, Edward E. Foos, Diogenes Placencia, and Joseph G. Tischler pp 15071–15076 DOI: 10.1021/ja404576j Supporting Info |
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Entropic Origin of Cobalt–Carbon Bond Cleavage Catalysis in Adenosylcobalamin-Dependent Ethanolamine Ammonia-Lyase Miao Wang and Kurt Warncke pp 15077–15084 DOI: 10.1021/ja404467d Supporting Info |
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Mechanical Stability of the Antibody Domain CH3 Homodimer in Different Oxidation States Morten Bertz, Johannes Buchner, and Matthias Rief pp 15085–15091 DOI: 10.1021/ja405076j Supporting Info |
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Microscopic Insights into the NMR Relaxation-Based Protein Conformational Entropy Meter Vignesh Kasinath, Kim A. Sharp, and A. Joshua Wand pp 15092–15100 DOI: 10.1021/ja405200u Supporting Info |
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NMR-Based Conformational Ensembles Explain pH-Gated Opening and Closing of OmpG Channel Tiandi Zhuang, Christina Chisholm, Min Chen, and Lukas K. Tamm pp 15101–15113 DOI: 10.1021/ja408206e Supporting Info |
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Identification of a Common Binding Mode for Imaging Agents to Amyloid Fibrils from Molecular Dynamics Simulations Katrine Kirkeby Skeby, Jesper Sørensen, and Birgit Schiøtt pp 15114–15128 DOI: 10.1021/ja405530p Supporting Info |
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Solid Colloids with Surface-Mobile DNA Linkers Stef A. J. van der Meulen and Mirjam E. Leunissen pp 15129–15134 DOI: 10.1021/ja406226b Supporting Info |
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Computational Studies on the Excited States of Luminescent Platinum(II) Alkynyl Systems of Tridentate Pincer Ligands in Radiative and Nonradiative Processes Wai Han Lam, Elizabeth Suk-Hang Lam, and Vivian Wing-Wah Yam pp 15135–15143 DOI: 10.1021/ja406810a Supporting Info |
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Time-Resolved Magnetic Field Effects Distinguish Loose Ion Pairs from Exciplexes Sabine Richert, Arnulf Rosspeintner, Stephan Landgraf, Günter Grampp, Eric Vauthey, and Daniel R. Kattnig pp 15144–15152 DOI: 10.1021/ja407052t Supporting Info |
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Monothiol Glutaredoxins Can Bind Linear [Fe3S4]+ and [Fe4S4]2+ Clusters in Addition to [Fe2S2]2+ Clusters: Spectroscopic Characterization and Functional Implications Bo Zhang, Sibali Bandyopadhyay, Priyanka Shakamuri, Sunil G. Naik, Boi Hanh Huynh, Jérémy Couturier, Nicolas Rouhier, and Michael K. Johnson pp 15153–15164 DOI: 10.1021/ja407059n Supporting Info |
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Molecular Imaging of Labile Iron(II) Pools in Living Cells with a Turn-On Fluorescent Probe Ho Yu Au-Yeung, Jefferson Chan, Teera Chantarojsiri, and Christopher J. Chang pp 15165–15173 DOI: 10.1021/ja4072964 Supporting Info |
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Dangerous Liaisons between Detergents and Membrane Proteins. The Case of Mitochondrial Uncoupling Protein 2 Manuela Zoonens, Jeffrey Comer, Sandrine Masscheleyn, Eva Pebay-Peyroula, Christophe Chipot, Bruno Miroux, and François Dehez pp 15174–15182 DOI: 10.1021/ja407424v Supporting Info |
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Membrane Proteins Can Have High Kinetic Stability Robert E. Jefferson, Tracy M. Blois, and James U. Bowie pp 15183–15190 DOI: 10.1021/ja407232b Supporting Info |
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Dopant-Induced Modification of Active Site Structure and Surface Bonding Mode for High-Performance Nanocatalysts: CO Oxidation on Capping-free (110)-oriented CeO2:Ln (Ln = La–Lu) Nanowires Jun Ke, Jia-Wen Xiao, Wei Zhu, Haichao Liu, Rui Si, Ya-Wen Zhang, and Chun-Hua Yan pp 15191–15200 DOI: 10.1021/ja407616p Supporting Info |
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High Flux Thin Film Nanocomposite Membranes Based on Metal–Organic Frameworks for Organic Solvent Nanofiltration Sara Sorribas, Patricia Gorgojo, Carlos Téllez, Joaquín Coronas, and Andrew G. Livingston pp 15201–15208 DOI: 10.1021/ja407665w Supporting Info |
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The Pivotal Role of Oxyallyl Diradicals in Photo-Favorskii Rearrangements: Transient Spectroscopic and Computational Studies Tomáš Šolomek, Dominik Heger, Bokolombe P. Ngoy, Richard S. Givens, and Petr Klán pp 15209–15215 DOI: 10.1021/ja407588p Supporting Info |
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Nucleophilicity Parameters of Pyridinium Ylides and Their Use in Mechanistic Analyses Dominik S. Allgäuer, Peter Mayer, and Herbert Mayr pp 15216–15224 DOI: 10.1021/ja407885h Supporting Info |
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Lewis Base Mediated β-Elimination and Lewis Acid Mediated Insertion Reactions of Disilazido Zirconium Compounds KaKing Yan, Juan J. Duchimaza Heredia, Arkady Ellern, Mark S. Gordon, and Aaron D. Sadow pp 15225–15237 DOI: 10.1021/ja407950e Supporting Info |
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Multianalyte Sensing of Addictive Over-the-Counter (OTC) Drugs Tsuyoshi Minami, Nina A. Esipenko, Ali Akdeniz, Ben Zhang, Lyle Isaacs, and Pavel Anzenbacher, Jr. pp 15238–15243 DOI: 10.1021/ja407722a Supporting Info |
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Evidence To Challenge the Universality of the Horiuti–Polanyi Mechanism for Hydrogenation in Heterogeneous Catalysis: Origin and Trend of the Preference of a Non-Horiuti–Polanyi Mechanism Bo Yang, Xue-Qing Gong, Hai-Feng Wang, Xiao-Ming Cao, John J. Rooney, and P. Hu pp 15244–15250 DOI: 10.1021/ja408314k Supporting Info |
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Control of Mode/Bond Selectivity and Product Energy Disposal by the Transition State: X + H2O (X = H, F, O(3P), and Cl) Reactions Bin Jiang and Hua Guo pp 15251–15256 DOI: 10.1021/ja408422y Supporting Info |
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Cu-Catalyzed Esterification Reaction via Aerobic Oxygenation and C–C Bond Cleavage: An Approach to α-Ketoesters Chun Zhang, Peng Feng, and Ning Jiao pp 15257–15262 DOI: 10.1021/ja4085463 Supporting Info |
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Composition- and Size-Controlled Cyclic Self-Assembly by Solvent- and C60-Responsive Self-Sorting Qixun Shi, Karl-Erik Bergquist, Ruiping Huo, Jilai Li, Mikael Lund, Robert Vácha, Anders Sundin, Eugenijus Butkus, Edvinas Orentas, and Kenneth Wärnmark pp 15263–15268 DOI: 10.1021/ja408582w Supporting Info |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 15269–15269 DOI: 10.1021/ja4103088 |
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Chirality Transfer in 1D Self-Assemblies: Influence of H-Bonding vs Metal Coordination between Dicyano[7]helicene Enantiomers Aneliia Shchyrba, Manh-Thuong Nguyen, Christian Wäckerlin, Susanne Martens, Sylwia Nowakowska, Toni Ivas, Jesse Roose, Thomas Nijs, Serpil Boz, Michael Schär, Meike Stöhr, Carlo A. Pignedoli, Carlo Thilgen, François Diederich, Daniele Passerone, and Thomas A. Jung pp 15270–15273 DOI: 10.1021/ja407315f Supporting Info |
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Complexin-1 Enhances the On-Rate of Vesicle Docking via Simultaneous SNARE and Membrane Interactions Jiajie Diao, Daniel J. Cipriano, Minglei Zhao, Yunxiang Zhang, Sachi Shah, Mark S. Padolina, Richard A. Pfuetzner, and Axel T. Brunger pp 15274–15277 DOI: 10.1021/ja407392n Supporting Info |
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Histone H3 and H4 N-Terminal Tails in Nucleosome Arrays at Cellular Concentrations Probed by Magic Angle Spinning NMR Spectroscopy Min Gao, Philippe S. Nadaud, Morgan W. Bernier, Justin A. North, P. Chris Hammel, Michael G. Poirier, and Christopher P. Jaroniec pp 15278–15281 DOI: 10.1021/ja407526s Supporting Info |
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Regioselective Allene Hydrosilylation Catalyzed by N-Heterocyclic Carbene Complexes of Nickel and Palladium Zachary D. Miller, Wei Li, Tomás R. Belderrain, and John Montgomery pp 15282–15285 DOI: 10.1021/ja407749w Supporting Info |
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3D Anhydrous Proton-Transporting Nanochannels Formed by Self-Assembly of Liquid Crystals Composed of a Sulfobetaine and a Sulfonic Acid Bartolome Soberats, Masafumi Yoshio, Takahiro Ichikawa, Satomi Taguchi, Hiroyuki Ohno, and Takashi Kato pp 15286–15289 DOI: 10.1021/ja407883b Supporting Info |
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Dynamic Nuclear Polarization NMR Spectroscopy Allows High-Throughput Characterization of Microporous Organic Polymers Frédéric Blanc, Samantha Y. Chong, Tom O. McDonald, Dave J. Adams, Shane Pawsey, Marc A. Caporini, and Andrew I. Cooper pp 15290–15293 DOI: 10.1021/ja408074v Supporting Info |
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Protonation Equilibrium and Hydrogen Production by a Dinuclear Cobalt–Hydride Complex Reduced by Cobaltocene with Trifluoroacetic Acid Sukanta Mandal, Shinya Shikano, Yusuke Yamada, Yong-Min Lee, Wonwoo Nam, Antoni Llobet, and Shunichi Fukuzumi pp 15294–15297 DOI: 10.1021/ja408080z Supporting Info |
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A Structurally Rigid Bis(amido) Ligand Framework in Low-Coordinate Ni(I), Ni(II), and Ni(III) Analogues Provides Access to a Ni(III) Methyl Complex via Oxidative Addition Michael I. Lipschutz, Xinzheng Yang, Ruchira Chatterjee, and T. Don Tilley pp 15298–15301 DOI: 10.1021/ja408151h Supporting Info |
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Magnetic Tuning of Plasmonic Excitation of Gold Nanorods Mingsheng Wang, Chuanbo Gao, Le He, Qipeng Lu, Jinzhong Zhang, Chi Tang, Serkan Zorba, and Yadong Yin pp 15302–15305 DOI: 10.1021/ja408289b Supporting Info |
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Development of a Chiral Bis(guanidino)iminophosphorane as an Uncharged Organosuperbase for the Enantioselective Amination of Ketones Tadahiro Takeda and Masahiro Terada pp 15306–15309 DOI: 10.1021/ja408296h Supporting Info |
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Boryl-Mediated Reversible H2 Activation at Cobalt: Catalytic Hydrogenation, Dehydrogenation, and Transfer Hydrogenation Tzu-Pin Lin and Jonas C. Peters pp 15310–15313 DOI: 10.1021/ja408397v Supporting Info |
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Remarkable Performance of Ir1/FeOx Single-Atom Catalyst in Water Gas Shift Reaction Jian Lin, Aiqin Wang, Botao Qiao, Xiaoyan Liu, Xiaofeng Yang, Xiaodong Wang, Jinxia Liang, Jun Li, Jingyue Liu, and Tao Zhang pp 15314–15317 DOI: 10.1021/ja408574m Supporting Info |
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Menaquinone Biosynthesis: Formation of Aminofutalosine Requires a Unique Radical SAM Enzyme Nilkamal Mahanta, Dmytro Fedoseyenko, Tohru Dairi, and Tadhg P. Begley pp 15318–15321 DOI: 10.1021/ja408594p Supporting Info |
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Fabrication of c-Axis Oriented ZSM-5 Hollow Fibers Based on an in Situ Solid–Solid Transformation Mechanism Kui Shen, Weizhong Qian, Ning Wang, Chang Su, and Fei Wei pp 15322–15325 DOI: 10.1021/ja408624x Supporting Info |
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High-Efficiency Polymer Solar Cells via the Incorporation of an Amino-Functionalized Conjugated Metallopolymer as a Cathode Interlayer Shengjian Liu, Kai Zhang, Junming Lu, Jie Zhang, Hin-Lap Yip, Fei Huang, and Yong Cao pp 15326–15329 DOI: 10.1021/ja408363c Supporting Info |
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Authorizing Multiple Chemical Passwords by a Combinatorial Molecular Keypad Lock Bhimsen Rout, Petr Milko, Mark A. Iron, Leila Motiei, and David Margulies pp 15330–15333 DOI: 10.1021/ja4081748 Supporting Info |
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Disulfonimide-Catalyzed Asymmetric Synthesis of β3-Amino Esters Directly from N-Boc-Amino Sulfones Qinggang Wang, Markus Leutzsch, Manuel van Gemmeren, and Benjamin List pp 15334–15337 DOI: 10.1021/ja408747m Supporting Info |
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Synthesis of a TREN in Which the Aryl Substituents are Part of a 45 Atom Macrocycle Matthew F. Cain, William P. Forrest, Jr., Dmitry V. Peryshkov, Richard R. Schrock, and Peter Müller pp 15338–15341 DOI: 10.1021/ja408964g Supporting Info |
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Direct Construction of Quaternary Carbons from Tertiary Alcohols via Photoredox-Catalyzed Fragmentation of tert-Alkyl N-Phthalimidoyl Oxalates Gregory L. Lackner, Kyle W. Quasdorf, and Larry E. Overman pp 15342–15345 DOI: 10.1021/ja408971t Supporting Info |
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Efficient Chromium(II)-Catalyzed Cross-Coupling Reactions between Csp2 Centers Andreas K. Steib, Olesya M. Kuzmina, Sarah Fernandez, Dietmar Flubacher, and Paul Knochel pp 15346–15349 DOI: 10.1021/ja409076z Supporting Info |
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Fast, Label-Free Force Spectroscopy of Histone–DNA Interactions in Individual Nucleosomes Using Nanopores Andrey Ivankin, Spencer Carson, Shannon R. M. Kinney, and Meni Wanunu pp 15350–15352 DOI: 10.1021/ja408354s Supporting Info |
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Reaction Pathways for Oxygen Evolution Promoted by Cobalt Catalyst Giuseppe Mattioli, Paolo Giannozzi, Aldo Amore Bonapasta, and Leonardo Guidoni pp 15353–15363 DOI: 10.1021/ja401797v Supporting Info |
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Disproportionation in Li–O2 Batteries Based on a Large Surface Area Carbon Cathode Dengyun Zhai, Hsien-Hau Wang, Junbing Yang, Kah Chun Lau, Kaixi Li, Khalil Amine, and Larry A. Curtiss pp 15364–15372 DOI: 10.1021/ja403199d Supporting Info |
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Norovirus Capsid Proteins Self-Assemble through Biphasic Kinetics via Long-Lived Stave-like Intermediates Guillaume Tresset, Clémence Le Coeur, Jean-François Bryche, Mouna Tatou, Mehdi Zeghal, Annie Charpilienne, Didier Poncet, Doru Constantin, and Stéphane Bressanelli pp 15373–15381 DOI: 10.1021/ja403550f Supporting Info |
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Efficient Convergent Synthesis of Bi-, Tri-, and Tetra-antennary Complex Type N-Glycans and Their HIV-1 Antigenicity Sachin S. Shivatare, Shih-Huang Chang, Tsung-I Tsai, Chien-Tai Ren, Hong-Yang Chuang, Li Hsu, Chih-Wei Lin, Shiou-Ting Li, Chung-Yi Wu, and Chi-Huey Wong pp 15382–15391 DOI: 10.1021/ja409097c Supporting Info |
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Origin and Scope of Long-Range Stabilizing Interactions and Associated SOMO–HOMO Conversion in Distonic Radical Anions Ganna Gryn’ova and Michelle L. Coote pp 15392–15403 DOI: 10.1021/ja404279f Supporting Info |
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Identification of an Intermediate Methyl Carrier in the Radical S-Adenosylmethionine Methylthiotransferases RimO and MiaB Bradley J. Landgraf, Arthur J. Arcinas, Kyung-Hoon Lee, and Squire J. Booker pp 15404–15416 DOI: 10.1021/ja4048448 Supporting Info |
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Poly(trehalose): Sugar-Coated Nanocomplexes Promote Stabilization and Effective Polyplex-Mediated siRNA Delivery Antons Sizovs, Lian Xue, Zachary P. Tolstyka, Nilesh P. Ingle, Yaoying Wu, Mallory Cortez, and Theresa M. Reineke pp 15417–15424 DOI: 10.1021/ja404941p Supporting Info |
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Consequences of Metal–Oxide Interconversion for C–H Bond Activation during CH4 Reactions on Pd Catalysts Ya-Huei (Cathy) Chin, Corneliu Buda, Matthew Neurock, and Enrique Iglesia pp 15425–15442 DOI: 10.1021/ja405004m Supporting Info |
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Activity Descriptor Identification for Oxygen Reduction on Nonprecious Electrocatalysts: Linking Surface Science to Coordination Chemistry Nagappan Ramaswamy, Urszula Tylus, Qingying Jia, and Sanjeev Mukerjee pp 15443–15449 DOI: 10.1021/ja405149m Supporting Info |
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Stabilization of a Ruthenium(II) Polypyridyl Dye on Nanocrystalline TiO2 by an Electropolymerized Overlayer Alexander M. Lapides, Dennis L. Ashford, Kenneth Hanson, Daniel A. Torelli, Joseph L. Templeton, and Thomas J. Meyer pp 15450–15458 DOI: 10.1021/ja4055977 Supporting Info |
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Solid-Phase Polarization Matrixes for Dynamic Nuclear Polarization from Homogeneously Distributed Radicals in Mesostructured Hybrid Silica Materials David Gajan, Martin Schwarzwälder, Matthew P. Conley, Wolfram R. Grüning, Aaron J. Rossini, Alexandre Zagdoun, Moreno Lelli, Maxim Yulikov, Gunnar Jeschke, Claire Sauvée, Olivier Ouari, Paul Tordo, Laurent Veyre, Anne Lesage, Chloé Thieuleux, Lyndon Emsley, and Christophe Copéret pp 15459–15466 DOI: 10.1021/ja405822h Supporting Info |
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Intimate Binding Mechanism and Structure of Trigonal Nickel(I) Monocarbonyl Adducts in ZSM-5 Zeolite—Spectroscopic Continuous Wave EPR, HYSCORE, and IR Studies Refined with DFT Quantification of Disentangled Electron and Spin Density Redistributions along σ and π Channels Piotr Pietrzyk, Tomasz Mazur, Katarzyna Podolska-Serafin, Mario Chiesa, and Zbigniew Sojka pp 15467–15478 DOI: 10.1021/ja405874t Supporting Info |
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Gold-Mediated Expulsion of Dinitrogen from Organic Azides Chandrakanta Dash, Muhammed Yousufuddin, Thomas R. Cundari, and H. V. Rasika Dias pp 15479–15488 DOI: 10.1021/ja406027x Supporting Info |
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Facet-Selective Adsorption on Noble Metal Crystals Guided by Electrostatic Potential Surfaces of Aromatic Molecules Chin-Yi Chiu, Hao Wu, Zhaoying Yao, Fei Zhou, Hua Zhang, Vidvuds Ozolins, and Yu Huang pp 15489–15500 DOI: 10.1021/ja406018u Supporting Info |
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Phenylboronic Acid-Installed Polymeric Micelles for Targeting Sialylated Epitopes in Solid Tumors Stephanie Deshayes, Horacio Cabral, Takehiko Ishii, Yutaka Miura, Shutaro Kobayashi, Takashi Yamashita, Akira Matsumoto, Yuji Miyahara, Nobuhiro Nishiyama, and Kazunori Kataoka pp 15501–15507 DOI: 10.1021/ja406406h Supporting Info |
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Investigating the α-Effect in Gas-Phase SN2 Reactions of Microsolvated Anions Ditte L. Thomsen, Jennifer N. Reece, Charles M. Nichols, Steen Hammerum, and Veronica M. Bierbaum pp 15508–15514 DOI: 10.1021/ja4066943 Supporting Info |
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Tryptophan-Accelerated Electron Flow Across a Protein–Protein Interface Kana Takematsu, Heather Williamson, Ana María Blanco-Rodríguez, Lucie Sokolová, Pavle Nikolovski, Jens T. Kaiser, Michael Towrie, Ian P. Clark, Antonín Vlček, Jr., Jay R. Winkler, and Harry B. Gray pp 15515–15525 DOI: 10.1021/ja406830d Supporting Info |
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Crystal Structures of the LsrR Proteins Complexed with Phospho-AI-2 and Two Signal-Interrupting Analogues Reveal Distinct Mechanisms for Ligand Recognition Jung-Hye Ha, Yumi Eo, Alexander Grishaev, Min Guo, Jacqueline A. I. Smith, Herman O. Sintim, Eun-Hee Kim, Hae-Kap Cheong, William E. Bentley, and Kyoung-Seok Ryu pp 15526–15535 DOI: 10.1021/ja407068v Supporting Info |
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Conservation and Functional Importance of Carbon–Oxygen Hydrogen Bonding in AdoMet-Dependent Methyltransferases Scott Horowitz, Lynnette M.A. Dirk, Joseph D. Yesselman, Jennifer S. Nimtz, Upendra Adhikari, Ryan A. Mehl, Steve Scheiner, Robert L. Houtz, Hashim M. Al-Hashimi, and Raymond C. Trievel pp 15536–15548 DOI: 10.1021/ja407140k Supporting Info |
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First-Principles Molecular Dynamics Simulation of Atmospherically Relevant Anion Solvation in Supercooled Water Droplet Yu Zhao, Hui Li, and Xiao Cheng Zeng pp 15549–15558 DOI: 10.1021/ja407286t Supporting Info |
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A Highly Sensitive Mixed Lanthanide Metal–Organic Framework Self-Calibrated Luminescent Thermometer Xingtang Rao, Tao Song, Junkuo Gao, Yuanjing Cui, Yu Yang, Chuande Wu, Banglin Chen, and Guodong Qian pp 15559–15564 DOI: 10.1021/ja407219k Supporting Info |
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Rational Design of Helical Nanotubes from Self-Assembly of Coiled-Coil Lock Washers Chunfu Xu, Rui Liu, Anil K. Mehta, Ricardo C. Guerrero-Ferreira, Elizabeth R. Wright, Stanislaw Dunin-Horkawicz, Kyle Morris, Louise C. Serpell, Xiaobing Zuo, Joseph S. Wall, and Vincent P. Conticello pp 15565–15578 DOI: 10.1021/ja4074529 Supporting Info |
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Water Networks Contribute to Enthalpy/Entropy Compensation in Protein–Ligand Binding Benjamin Breiten, Matthew R. Lockett, Woody Sherman, Shuji Fujita, Mohammad Al-Sayah, Heiko Lange, Carleen M. Bowers, Annie Heroux, Goran Krilov, and George M. Whitesides pp 15579–15584 DOI: 10.1021/ja4075776 Supporting Info |
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Interplay of Charge State, Lability, and Magnetism in the Molecule-like Au25(SR)18 Cluster Sabrina Antonello, Neranjan V. Perera, Marco Ruzzi, José A. Gascón, and Flavio Maran pp 15585–15594 DOI: 10.1021/ja407887d Supporting Info |
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Mechanistic Basis for High Stereoselectivity and Broad Substrate Scope in the (salen)Co(III)-Catalyzed Hydrolytic Kinetic Resolution David D. Ford, Lars P. C. Nielsen, Stephan J. Zuend, Charles B. Musgrave, and Eric N. Jacobsen pp 15595–15608 DOI: 10.1021/ja408027p Supporting Info |
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Highly Ordered Dielectric Mirrors via the Self-Assembly of Dendronized Block Copolymers Victoria A. Piunova, Garret M. Miyake, Christopher S. Daeffler, Raymond A. Weitekamp, and Robert H. Grubbs pp 15609–15616 DOI: 10.1021/ja4081502 |
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From Bis(silylene) and Bis(germylene) Pincer-Type Nickel(II) Complexes to Isolable Intermediates of the Nickel-Catalyzed Sonogashira Cross-Coupling Reaction Daniel Gallego, Andreas Brück, Elisabeth Irran, Florian Meier, Martin Kaupp, Matthias Driess, and John F. Hartwig pp 15617–15626 DOI: 10.1021/ja408137t Supporting Info |
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Correlated Ligand Dynamics in Oxyiron Picket Fence Porphyrins: Structural and Mössbauer Investigations Jianfeng Li, Bruce C. Noll, Allen G. Oliver, Charles E. Schulz, and W. Robert Scheidt pp 15627–15641 DOI: 10.1021/ja408431z Supporting Info |
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Diels–Alder Reactivities of Strained and Unstrained Cycloalkenes with Normal and Inverse-Electron-Demand Dienes: Activation Barriers and Distortion/Interaction Analysis Fang Liu, Robert S. Paton, Seonah Kim, Yong Liang, and K. N. Houk pp 15642–15649 DOI: 10.1021/ja408437u Supporting Info |
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Linear versus Dendritic Molecular Binders for Hydrogel Network Formation with Clay Nanosheets: Studies with ABA Triblock Copolyethers Carrying Guanidinium Ion Pendants Shingo Tamesue, Masataka Ohtani, Kuniyo Yamada, Yasuhiro Ishida, Jason M. Spruell, Nathaniel A. Lynd, Craig J. Hawker, and Takuzo Aida pp 15650–15655 DOI: 10.1021/ja408547g Supporting Info |
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Giant Electroactive M4L6 Tetrahedral Host Self-Assembled with Fe(II) Vertices and Perylene Bisimide Dye Edges Kingsuk Mahata, Peter D. Frischmann, and Frank Würthner pp 15656–15661 DOI: 10.1021/ja4083039 Supporting Info |
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1,6-Carbene Transfer: Gold-Catalyzed Oxidative Diyne Cyclizations Pascal Nösel, Laura Nunes dos Santos Comprido, Tobias Lauterbach, Matthias Rudolph, Frank Rominger, and A. Stephen K. Hashmi pp 15662–15666 DOI: 10.1021/ja4085385 Supporting Info |
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Snapshot of a DNA Polymerase while Incorporating Two Consecutive C5-Modified Nucleotides Samra Obeid, Holger Bußkamp, Wolfram Welte, Kay Diederichs, and Andreas Marx pp 15667–15669 DOI: 10.1021/ja405346s Supporting Info |
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All-Atom Molecular Dynamics Simulation of Photosystem II Embedded in Thylakoid Membrane Koji Ogata, Taichi Yuki, Makoto Hatakeyama, Waka Uchida, and Shinichiro Nakamura pp 15670–15673 DOI: 10.1021/ja404317d Supporting Info |
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Photoinduced Solid State Conversion of a Radical σ-Dimer to a π-Radical Pair Hoa Phan, Kristina Lekin, Stephen M. Winter, Richard T. Oakley, and Michael Shatruk pp 15674–15677 DOI: 10.1021/ja4055806 Supporting Info |
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Isolation of the Large {Actinide}38 Poly-oxo Cluster with Uranium Clément Falaise, Christophe Volkringer, Jean-François Vigier, Arnaud Beaurain, Pascal Roussel, Pierre Rabu, and Thierry Loiseau pp 15678–15681 DOI: 10.1021/ja4067207 Supporting Info |
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Single Vehicular Delivery of siRNA and Small Molecules to Control Stem Cell Differentiation Shreyas Shah, Aniruddh Solanki, Pijus K. Sasmal, and Ki-Bum Lee pp 15682–15685 DOI: 10.1021/ja4071738 Supporting Info |
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Weakly Stabilized Primary Borenium Cations and Their Dicationic Dimers Aleksandrs Prokofjevs, Jeff W. Kampf, Andrey Solovyev, Dennis P. Curran, and Edwin Vedejs pp 15686–15689 DOI: 10.1021/ja407458k Supporting Info |
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Spontaneous Resolution to Absolute Chiral Induction: Pseudo-Kagomé Type Homochiral Zn(II)/Co(II) Coordination Polymers with Achiral Precursors Kamal Kumar Bisht and Eringathodi Suresh pp 15690–15693 DOI: 10.1021/ja4075369 Supporting Info |
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Li10SnP2S12: An Affordable Lithium Superionic Conductor Philipp Bron, Sebastian Johansson, Klaus Zick, Jörn Schmedt auf der Günne, Stefanie Dehnen, and Bernhard Roling pp 15694–15697 DOI: 10.1021/ja407393y Supporting Info |
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Layer-by-Layer Fabrication of Oriented Porous Thin Films Based on Porphyrin-Containing Metal–Organic Frameworks Monica C. So, Shengye Jin, Ho-Jin Son, Gary P. Wiederrecht, Omar K. Farha, and Joseph T. Hupp pp 15698–15701 DOI: 10.1021/ja4078705 Supporting Info |
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Substrate-Directable Electron Transfer Reactions. Dramatic Rate Enhancement in the Chemoselective Reduction of Cyclic Esters Using SmI2–H2O: Mechanism, Scope, and Synthetic Utility Michal Szostak, Malcolm Spain, Kimberly A. Choquette, Robert A. Flowers, II, and David J. Procter pp 15702–15705 DOI: 10.1021/ja4078864 Supporting Info |
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Facile Synthesis of Palladium Right Bipyramids and Their Use as Seeds for Overgrowth and as Catalysts for Formic Acid Oxidation Xiaohu Xia, Sang-Il Choi, Jeffrey A. Herron, Ning Lu, Jessica Scaranto, Hsin-Chieh Peng, Jinguo Wang, Manos Mavrikakis, Moon J. Kim, and Younan Xia pp 15706–15709 DOI: 10.1021/ja408018j Supporting Info |
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Platinum-Catalyzed C–H Arylation of Simple Arenes Anna M. Wagner, Amanda J. Hickman, and Melanie S. Sanford pp 15710–15713 DOI: 10.1021/ja408112j Supporting Info |
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Postsynthetic Functionalization of a Hollow Silica Nanoreactor with Manganese Oxide-Immobilized Metal Nanocrystals Inside the Cavity Soo Min Kim, Mina Jeon, Ki Woong Kim, Jaiwook Park, and In Su Lee pp 15714–15717 DOI: 10.1021/ja4083792 Supporting Info |
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Lithographically Defined Macroscale Modulation of Lateral Fluidity and Phase Separation Realized via Patterned Nanoporous Silica-Supported Phospholipid Bilayers Eric L. Kendall, Viviane N. Ngassam, Sean F. Gilmore, C. Jeffrey Brinker, and Atul N. Parikh pp 15718–15721 DOI: 10.1021/ja408434r Supporting Info |
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Alkahest for V2VI3 Chalcogenides: Dissolution of Nine Bulk Semiconductors in a Diamine-Dithiol Solvent Mixture David H. Webber and Richard L. Brutchey pp 15722–15725 DOI: 10.1021/ja4084336 Supporting Info |
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DNA Protection by the Bacterial Ferritin Dps via DNA Charge Transport Anna R. Arnold and Jacqueline K. Barton pp 15726–15729 DOI: 10.1021/ja408760w Supporting Info |
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Dynamic Kinetic Cross-Coupling Strategy for the Asymmetric Synthesis of Axially Chiral Heterobiaryls Abel Ros, Beatriz Estepa, Pedro Ramírez-López, Eleuterio Álvarez, Rosario Fernández, and José M. Lassaletta pp 15730–15733 DOI: 10.1021/ja4087819 Supporting Info |
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Depolymerization-Powered Autonomous Motors Using Biocompatible Fuel Hua Zhang, Wentao Duan, Lei Liu, and Ayusman Sen pp 15734–15737 DOI: 10.1021/ja4089549 Supporting Info |
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Evidence for Phenylalanine Zipper-Mediated Dimerization in the X-ray Crystal Structure of a Magainin 2 Analogue Zvi Hayouka, David E. Mortenson, Dale F. Kreitler, Bernard Weisblum, Katrina T. Forest, and Samuel H. Gellman pp 15738–15741 DOI: 10.1021/ja409082w Supporting Info |
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Copper(I)/ABNO-Catalyzed Aerobic Alcohol Oxidation: Alleviating Steric and Electronic Constraints of Cu/TEMPO Catalyst Systems Janelle E. Steves and Shannon S. Stahl pp 15742–15745 DOI: 10.1021/ja409241h Supporting Info |
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Enantio- and Regioselective CuH-Catalyzed Hydroamination of Alkenes Shaolin Zhu, Nootaree Niljianskul, and Stephen L. Buchwald pp 15746–15749 DOI: 10.1021/ja4092819 Supporting Info |
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Surface Structure-Dependent Molecular Oxygen Activation of BiOCl Single-Crystalline Nanosheets Kun Zhao, Lizhi Zhang, Jiajun Wang, Qunxiang Li, Weiwei He, and Jun Jie Yin pp 15750–15753 DOI: 10.1021/ja4092903 Supporting Info |
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Detecting Substrates Bound to the Secondary Multidrug Efflux Pump EmrE by DNP-Enhanced Solid-State NMR Yean Sin Ong, Andrea Lakatos, Johanna Becker-Baldus, Klaas M. Pos, and Clemens Glaubitz pp 15754–15762 DOI: 10.1021/ja402605s Supporting Info |
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Elucidating the Breathing of the Metal–Organic Framework MIL-53(Sc) with ab Initio Molecular Dynamics Simulations and in Situ X-ray Powder Diffraction Experiments Linjiang Chen, John P. S. Mowat, David Fairen-Jimenez, Carole A. Morrison, Stephen P. Thompson, Paul A. Wright, and Tina Düren pp 15763–15773 DOI: 10.1021/ja403453g Supporting Info |
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Hydrogen-Bond Dynamics of Water at the Interface with InP/GaP(001) and the Implications for Photoelectrochemistry Brandon C. Wood, Eric Schwegler, Woon Ih Choi, and Tadashi Ogitsu pp 15774–15783 DOI: 10.1021/ja403850s Supporting Info |
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New Dihexadecyldithiophosphate SAMs on Gold Provide Insight into the Unusual Dependence of Adsorbate Chelation on Substrate Morphology in SAMs of Dialkyldithiophosphinic Acids Ronan R. San Juan, Christopher J. Allan, Muhammad Iqbal, S. Holger Eichhorn, Charles L. B. Macdonald, and Tricia Breen Carmichael pp 15784–15793 DOI: 10.1021/ja404798q Supporting Info |
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Self-Decoupled Porphyrin with a Tripodal Anchor for Molecular-Scale Electroluminescence San-E Zhu, Yan-Min Kuang, Feng Geng, Jia-Zhe Zhu, Cong-Zhou Wang, Yun-Jie Yu, Yang Luo, Yang Xiao, Kai-Qing Liu, Qiu-Shi Meng, Li Zhang, Song Jiang, Yang Zhang, Guan-Wu Wang, Zhen-Chao Dong, and J. G. Hou pp 15794–15800 DOI: 10.1021/ja4048569 Supporting Info |
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Substrate-Triggered Addition of Dioxygen to the Diferrous Cofactor of Aldehyde-Deformylating Oxygenase to Form a Diferric-Peroxide Intermediate Maria E. Pandelia, Ning Li, Hanne Nørgaard, Douglas M. Warui, Lauren J. Rajakovich, Wei-chen Chang, Squire J. Booker, Carsten Krebs, and J. Martin Bollinger, Jr. pp 15801–15812 DOI: 10.1021/ja405047b Supporting Info |
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Divergent Mechanisms for Enzymatic Excision of 5-Formylcytosine and 5-Carboxylcytosine from DNA Atanu Maiti, Anna Zhachkina Michelson, Cherece J. Armwood, Jeehiun K. Lee, and Alexander C. Drohat pp 15813–15822 DOI: 10.1021/ja406444x Supporting Info |
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Elucidation of the Selectivity of Proton-Dependent Electrocatalytic CO2 Reduction by fac-Re(bpy)(CO)3Cl John A. Keith, Kyle A. Grice, Clifford P. Kubiak, and Emily A. Carter pp 15823–15829 DOI: 10.1021/ja406456g Supporting Info |
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Dipalladium(I) Terphenyl Diphosphine Complexes as Models for Two-Site Adsorption and Activation of Organic Molecules Sibo Lin, David E. Herbert, Alexandra Velian, Michael W. Day, and Theodor Agapie pp 15830–15840 DOI: 10.1021/ja406696k Supporting Info |
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Structural Evidence for a Two-Regime Photobleaching Mechanism in a Reversibly Switchable Fluorescent Protein Chenxi Duan, Virgile Adam, Martin Byrdin, Jacqueline Ridard, Sylvie Kieffer-Jaquinod, Cécile Morlot, Delphine Arcizet, Isabelle Demachy, and Dominique Bourgeois pp 15841–15850 DOI: 10.1021/ja406860e Supporting Info |
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Circular Dichroism, Magnetic Circular Dichroism, and Variable Temperature Variable Field Magnetic Circular Dichroism Studies of Biferrous and Mixed-Valent myo-Inositol Oxygenase: Insights into Substrate Activation of O2 Reactivity Rae Ana Snyder, Caleb B. Bell, III, Yinghui Diao, Carsten Krebs, J. Martin Bollinger, Jr., and Edward I. Solomon pp 15851–15863 DOI: 10.1021/ja406635k Supporting Info |
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Pt@CeO2 Multicore@Shell Self-Assembled Nanospheres: Clean Synthesis, Structure Optimization, and Catalytic Applications Xiao Wang, Dapeng Liu, Shuyan Song, and Hongjie Zhang pp 15864–15872 DOI: 10.1021/ja4069134 Supporting Info |
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Tunable Cytotoxicity of Rhodamine 6G via Anion Variations Paul K. S. Magut, Susmita Das, Vivian E. Fernand, Jack Losso, Karen McDonough, Brittni M. Naylor, Sita Aggarwal, and Isiah M. Warner pp 15873–15879 DOI: 10.1021/ja407164w Supporting Info |
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Tristability in a Light-Actuated Single-Molecule Magnet Xiaowen Feng, Corine Mathonière, Ie-Rang Jeon, Mathieu Rouzières, Andrew Ozarowski, Michael L. Aubrey, Miguel I. Gonzalez, Rodolphe Clérac, and Jeffrey R. Long pp 15880–15884 DOI: 10.1021/ja407332y Supporting Info |
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Pattern Recognition Correlating Materials Properties of the Elements to Their Kinetics for the Hydrogen Evolution Reaction Kevin C. Leonard and Allen J. Bard pp 15885–15889 DOI: 10.1021/ja407394q Supporting Info |
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The Study of Multireactional Electrochemical Interfaces via a Tip Generation/Substrate Collection Mode of Scanning Electrochemical Microscopy: The Hydrogen Evolution Reaction for Mn in Acidic Solution Kevin C. Leonard and Allen J. Bard pp 15890–15896 DOI: 10.1021/ja407395m Supporting Info |
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Deamidation of Asparagine to Aspartate Destabilizes Cu, Zn Superoxide Dismutase, Accelerates Fibrillization, and Mirrors ALS-Linked Mutations Yunhua Shi, Nicholas R. Rhodes, Alireza Abdolvahabi, Taylor Kohn, Nathan P. Cook, Angel A. Marti, and Bryan F. Shaw pp 15897–15908 DOI: 10.1021/ja407801x Supporting Info |
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Total Synthesis of Vineomycin B2 Shunichi Kusumi, Satoshi Tomono, Shunsuke Okuzawa, Erika Kaneko, Takashi Ueda, Kaname Sasaki, Daisuke Takahashi, and Kazunobu Toshima pp 15909–15912 DOI: 10.1021/ja407827n Supporting Info |
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Core/Shell Colloidal Quantum Dot Exciplex States for the Development of Highly Efficient Quantum-Dot-Sensitized Solar Cells Jin Wang, Iván Mora-Seró, Zhenxiao Pan, Ke Zhao, Hua Zhang, Yaoyu Feng, Guang Yang, Xinhua Zhong, and Juan Bisquert pp 15913–15922 DOI: 10.1021/ja4079804 Supporting Info |
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Selective Formation of Hydrogen and Hydroxyl Radicals by Electron Beam Irradiation and Their Reactivity with Perfluorosulfonated Acid Ionomer Lida Ghassemzadeh, Timothy J. Peckham, Thomas Weissbach, Xiaoyan Luo, and Steven Holdcroft pp 15923–15932 DOI: 10.1021/ja408032p Supporting Info |
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Stability and Dynamic Processes in 16VE Iridium(III) Ethyl Hydride and Rhodium(I) σ-Ethane Complexes: Experimental and Computational Studies Marc D. Walter, Peter S. White, Cynthia K. Schauer, and Maurice Brookhart pp 15933–15947 DOI: 10.1021/ja4079539 Supporting Info |
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Spectral Evolution of a Photochemical Protecting Group for Orthogonal Two-Color Uncaging with Visible Light Jeremy P. Olson, Matthew R. Banghart, Bernardo L. Sabatini, and Graham C. R. Ellis-Davies pp 15948–15954 DOI: 10.1021/ja408225k Supporting Info |
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β-Technetium Dichloride: Solid-State Modulated Structure, Electronic Structure, and Physical Properties Christos D. Malliakas, Frederic Poineau, Erik V. Johnstone, Philippe F. Weck, Eunja Kim, Brian L. Scott, Paul M. Forster, Mercouri G. Kanatzidis, Kenneth R. Czerwinski, and Alfred P. Sattelberger pp 15955–15962 DOI: 10.1021/ja408459k Supporting Info |
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Correction to “Copper-Catalyzed Aerobic Oxidation of Hydroxamic Acids Leads to a Mild and Versatile Acylnitroso Ene Reaction” Charles P. Frazier, Jarred R. Engelking, and Javier Read de Alaniz pp 15963–15963 DOI: 10.1021/ja408353u |
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Correction to “Organocatalytic Oxyamination of Azlactones: Kinetic Resolution of Oxaziridines and Asymmetric Synthesis of Oxazolin-4-ones” Shunxi Dong, Xiaohua Liu, Yin Zhu, Peng He, Lili Lin, and Xiaoming Feng pp 15964–15964 DOI: 10.1021/ja409178p Supporting Info |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 15965–15965 DOI: 10.1021/ja410682n |
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New Two-Dimensional Niobium and Vanadium Carbides as Promising Materials for Li-Ion Batteries Michael Naguib, Joseph Halim, Jun Lu, Kevin M. Cook, Lars Hultman, Yury Gogotsi, and Michel W. Barsoum pp 15966–15969 DOI: 10.1021/ja405735d Supporting Info |
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Membrane Remodeling by α-Synuclein and Effects on Amyloid Formation Zhiping Jiang, Michel de Messieres, and Jennifer C. Lee pp 15970–15973 DOI: 10.1021/ja405993r Supporting Info |
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Structure of Cu(I)-Bound DJ-1 Reveals a Biscysteinate Metal Binding Site at the Homodimer Interface: Insights into Mutational Inactivation of DJ-1 in Parkinsonism M. Rhyan Puno, Nisha A. Patel, Simon Geir Møller, Carol V. Robinson, Peter C. E. Moody, and Mark Odell pp 15974–15977 DOI: 10.1021/ja406010m Supporting Info |
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Photoactivated Colloidal Dockers for Cargo Transportation Jérémie Palacci, Stefano Sacanna, Adrian Vatchinsky, Paul M. Chaikin, and David J. Pine pp 15978–15981 DOI: 10.1021/ja406090s Supporting Info |
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Antimony-Based Ligand Exchange To Promote Crystallization in Spray-Deposited Cu2ZnSnSe4 Solar Cells Alex Carrete, Alexey Shavel, Xavier Fontané, Joana Montserrat, Jiandong Fan, Maria Ibáñez, Edgardo Saucedo, Alejandro Pérez-Rodríguez, and Andreu Cabot pp 15982–15985 DOI: 10.1021/ja4068639 Supporting Info |
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Spin-Crossover Modification through Selective CO2 Sorption Eugenio Coronado, Mónica Giménez-Marqués, Guillermo Mínguez Espallargas, Fernando Rey, and Iñigo J. Vitórica-Yrezábal pp 15986–15989 DOI: 10.1021/ja407135k Supporting Info |
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Formation of a 1,4-Diamino-2,3-disila-1,3-butadiene Derivative Kartik Chandra Mondal, Herbert W. Roesky, Birger Dittrich, Nicole Holzmann, Markus Hermann, Gernot Frenking, and Alke Meents pp 15990–15993 DOI: 10.1021/ja4072139 Supporting Info |
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Metallo-Supramolecular Cyclic Polymers Ke Zhang, Yongping Zha, Bo Peng, Yongming Chen, and Gregory N. Tew pp 15994–15997 DOI: 10.1021/ja407381f Supporting Info |
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Rational Defect Passivation of Cu2ZnSn(S,Se)4 Photovoltaics with Solution-Processed Cu2ZnSnS4:Na Nanocrystals Huanping Zhou, Tze-Bin Song, Wan-Ching Hsu, Song Luo, Shenglin Ye, Hsin-Sheng Duan, Chia-Jung Hsu, Wenbing Yang, and Yang Yang pp 15998–16001 DOI: 10.1021/ja407202u Supporting Info |
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Mesoporous Metal–Nitrogen-Doped Carbon Electrocatalysts for Highly Efficient Oxygen Reduction Reaction Hai-Wei Liang, Wei Wei, Zhong-Shuai Wu, Xinliang Feng, and Klaus Müllen pp 16002–16005 DOI: 10.1021/ja407552k Supporting Info |
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Cation-Dependent Magnetic Ordering and Room-Temperature Bistability in Azido-Bridged Perovskite-Type Compounds Xin-Hua Zhao, Xing-Cai Huang, Shao-Liang Zhang, Dong Shao, Hai-Yan Wei, and Xin-Yi Wang pp 16006–16009 DOI: 10.1021/ja407654n Supporting Info |
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Axially Chiral Dicarboxylic Acid Catalyzed Activation of Quinone Imine Ketals: Enantioselective Arylation of Enecarbamates Takuya Hashimoto, Hiroki Nakatsu, Yuka Takiguchi, and Keiji Maruoka pp 16010–16013 DOI: 10.1021/ja407501h Supporting Info |
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DNA-Catalyzed Hydrolysis of Esters and Aromatic Amides Benjamin M. Brandsen, Anthony R. Hesser, Marissa A. Castner, Madhavaiah Chandra, and Scott K. Silverman pp 16014–16017 DOI: 10.1021/ja4077233 Supporting Info |
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Multicomponent Reactions for de Novo Synthesis of BODIPY Probes: In Vivo Imaging of Phagocytic Macrophages Ana Vázquez-Romero, Nicola Kielland, María J. Arévalo, Sara Preciado, Richard J. Mellanby, Yi Feng, Rodolfo Lavilla, and Marc Vendrell pp 16018–16021 DOI: 10.1021/ja408093p Supporting Info |
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Hydrogenation of Carboxylic Acids Catalyzed by Half-Sandwich Complexes of Iridium and Rhodium Timothy P. Brewster, Alexander J. M. Miller, D. Michael Heinekey, and Karen I. Goldberg pp 16022–16025 DOI: 10.1021/ja408149n Supporting Info |
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P3F92–: An All-Pseudo-π* 2π-Aromatic Chakkingal P. Priyakumari and Eluvathingal D. Jemmis pp 16026–16029 DOI: 10.1021/ja408308g Supporting Info |
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Re-examining the Size/Charge Paradigm: Differing in Vivo Characteristics of Size- and Charge-Matched Mesoporous Silica Nanoparticles Jason L. Townson, Yu-Shen Lin, Jacob O. Agola, Eric C. Carnes, Hon S. Leong, John D. Lewis, Christy L. Haynes, and C. Jeffrey Brinker pp 16030–16033 DOI: 10.1021/ja4082414 Supporting Info |
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An Ultrasensitive Nanowire-Transistor Biosensor for Detecting Dopamine Release from Living PC12 Cells under Hypoxic Stimulation Bor-Ran Li, Ying-Jhu Hsieh, Yan-Xi Chen, Ya-Ting Chung, Chien-Yuan Pan, and Yit-Tsong Chen pp 16034–16037 DOI: 10.1021/ja408485m Supporting Info |
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Rational Design of Porous Coordination Polymers Based on Bis(phosphine)MCl2 Complexes That Exhibit High-Temperature H2 Sorption and Chemical Reactivity Alisha M. Bohnsack, Ilich A. Ibarra, Vladimir I. Bakhmutov, Vincent M. Lynch, and Simon M. Humphrey pp 16038–16041 DOI: 10.1021/ja408508m Supporting Info |
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Morphology-Based Plasmonic Nanoparticle Sensors: Controlling Etching Kinetics with Target-Responsive Permeability Gate Brian Malile and Jennifer I. L. Chen pp 16042–16045 DOI: 10.1021/ja4086269 Supporting Info |
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Size Dependence of the Structure of Organic Aerosol Daniel P. Veghte, Muhammad Bilal Altaf, and Miriam Arak Freedman pp 16046–16049 DOI: 10.1021/ja408903g Supporting Info |
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Squaramide-Catalyzed Enantioselective Michael Addition of Masked Acyl Cyanides to Substituted Enones Kin S. Yang, Antoinette E. Nibbs, Yunus E. Türkmen, and Viresh H. Rawal pp 16050–16053 DOI: 10.1021/ja409012q Supporting Info |
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Synthesis of Enantioenriched Tertiary Boronic Esters by the Lithiation/Borylation of Secondary Alkyl Benzoates Alexander P. Pulis, Daniel J. Blair, Eva Torres, and Varinder K. Aggarwal pp 16054–16057 DOI: 10.1021/ja409100y Supporting Info |
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Iron Oxychloride (FeOCl): An Efficient Fenton-Like Catalyst for Producing Hydroxyl Radicals in Degradation of Organic Contaminants Xue-jing Yang, Xi-meng Xu, Jing Xu, and Yi-fan Han pp 16058–16061 DOI: 10.1021/ja409130c Supporting Info |
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Polyhedral Metal-Imidazolate Cages: Control of Self-Assembly and Cage to Cage Transformation Xiao-Ping Zhou, Yuan Wu, and Dan Li pp 16062–16065 DOI: 10.1021/ja4092984 Supporting Info |
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A Zwitterionic Carbanion Frustrated by Boranes – Dihydrogen Cleavage with Weak Lewis Acids via an “Inverse” Frustrated Lewis Pair Approach Hui Li, Adelia J. A. Aquino, David B. Cordes, Fernando Hung-Low, William L. Hase, and Clemens Krempner pp 16066–16069 DOI: 10.1021/ja409330h Supporting Info |
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Halogen and Chalcogen Cation Pools Stabilized by DMSO. Versatile Reagents for Alkene Difunctionalization Yosuke Ashikari, Akihiro Shimizu, Toshiki Nokami, and Jun-ichi Yoshida pp 16070–16073 DOI: 10.1021/ja4092648 Supporting Info |
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Simple Catalytic Mechanism for the Direct Coupling of α-Carbonyls with Functionalized Amines: A One-Step Synthesis of Plavix Ryan W. Evans, Jason R. Zbieg, Shaolin Zhu, Wei Li, and David W. C. MacMillan pp 16074–16077 DOI: 10.1021/ja4096472 Supporting Info |
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Protonation-Induced Chromism of Pyridylethynyl-Appended [core+exo]-Type Au8 Clusters. Resonance-Coupled Electronic Perturbation through π-Conjugated Group Naoki Kobayashi, Yutaro Kamei, Yukatsu Shichibu, and Katsuaki Konishi pp 16078–16081 DOI: 10.1021/ja4099092 Supporting Info |
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Pearson’s Principle Inspired Generalized Strategy for the Fabrication of Metal Hydroxide and Oxide Nanocages Jianwei Nai, Yu Tian, Xin Guan, and Lin Guo pp 16082–16091 DOI: 10.1021/ja402751r Supporting Info |
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Dynamics of an Intrinsically Disordered Protein Reveal Metastable Conformations That Potentially Seed Aggregation Qin Qiao, Gregory R. Bowman, and Xuhui Huang pp 16092–16101 DOI: 10.1021/ja403147m Supporting Info |
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Bioinspired Artificial Single Ion Pump Huacheng Zhang, Xu Hou, Lu Zeng, Fu Yang, Lin Li, Dadong Yan, Ye Tian, and Lei Jiang pp 16102–16110 DOI: 10.1021/ja4037669 Supporting Info |
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Rational Design of a Colorimetric pH Sensor from a Soluble Retinoic Acid Chaperone Tetyana Berbasova, Meisam Nosrati, Chrysoula Vasileiou, Wenjing Wang, Kin Sing Stephen Lee, Ipek Yapici, James H. Geiger, and Babak Borhan pp 16111–16119 DOI: 10.1021/ja404900k Supporting Info |
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Diagnostic Imaging Agents for Alzheimer’s Disease: Copper Radiopharmaceuticals that Target Aβ Plaques James L. Hickey, SinChun Lim, David J. Hayne, Brett M. Paterson, Jonathan M. White, Victor L. Villemagne, Peter Roselt, David Binns, Carleen Cullinane, Charmaine M. Jeffery, Roger I. Price, Kevin J. Barnham, and Paul S. Donnelly pp 16120–16132 DOI: 10.1021/ja4057807 Supporting Info |
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Structure and Dynamics of Full-Length HIV-1 Capsid Protein in Solution Lalit Deshmukh, Charles D. Schwieters, Alexander Grishaev, Rodolfo Ghirlando, James L. Baber, and G. Marius Clore pp 16133–16147 DOI: 10.1021/ja406246z Supporting Info |
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Access to a CuII–O–CuII Motif: Spectroscopic Properties, Solution Structure, and Reactivity Peter Haack, Anne Kärgel, Claudio Greco, Jadranka Dokic, Beatrice Braun, Florian F. Pfaff, Stefan Mebs, Kallol Ray, and Christian Limberg pp 16148–16160 DOI: 10.1021/ja406721a Supporting Info |
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Details of the Ultrafast DNA Photo-Cross-Linking Reaction of 3-Cyanovinylcarbazole Nucleoside: Cis–Trans Isomeric Effect and the Application for SNP-Based Genotyping Kenzo Fujimoto, Asuka Yamada, Yoshinaga Yoshimura, Tadashi Tsukaguchi, and Takashi Sakamoto pp 16161–16167 DOI: 10.1021/ja406965f Supporting Info |
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Proteins in Action: Femtosecond to Millisecond Structural Dynamics of a Photoactive Flavoprotein Richard Brust, Andras Lukacs, Allison Haigney, Kiri Addison, Agnieszka Gil, Michael Towrie, Ian P. Clark, Gregory M. Greetham, Peter J. Tonge, and Stephen R. Meech pp 16168–16174 DOI: 10.1021/ja407265p Supporting Info |
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Tuning the Reactivity of an Actor Ligand for Tandem CO2 and C–H Activations: From Spectator Metals to Metal-Free Vincent T. Annibale, Daniel A. Dalessandro, and Datong Song pp 16175–16183 DOI: 10.1021/ja4073832 Supporting Info |
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Postclustering Dynamic Covalent Modification for Chirality Control and Chiral Sensing Yang Yang, Xiao-Li Pei, and Quan-Ming Wang pp 16184–16191 DOI: 10.1021/ja4075419 Supporting Info |
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Mechanism and Selectivity in Nickel-Catalyzed Cross-Electrophile Coupling of Aryl Halides with Alkyl Halides Soumik Biswas and Daniel J. Weix pp 16192–16197 DOI: 10.1021/ja407589e Supporting Info |
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Kinetic and Thermodynamic Selectivity of Intermolecular C–H Activation at [Tp′Rh(PMe3)]. How Does the Ancillary Ligand Affect the Metal–Carbon Bond Strength? Yunzhe Jiao, James Morris, William W. Brennessel, and William D. Jones pp 16198–16212 DOI: 10.1021/ja4080985 Supporting Info |
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Hexameric Resorcinarene Capsule is a Brønsted Acid: Investigation and Application to Synthesis and Catalysis Qi Zhang and Konrad Tiefenbacher pp 16213–16219 DOI: 10.1021/ja4080375 Supporting Info |
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Single-Handed Helical Wrapping of Single-Walled Carbon Nanotubes by Chiral, Ionic, Semiconducting Polymers Pravas Deria, Christopher D. Von Bargen, Jean-Hubert Olivier, Amar S. Kumbhar, Jeffery G. Saven, and Michael J. Therien pp 16220–16234 DOI: 10.1021/ja408430v Supporting Info |
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Organic Acid-Catalyzed Polyurethane Formation via a Dual-Activated Mechanism: Unexpected Preference of N-Activation over O-Activation of Isocyanates Haritz Sardon, Amanda C. Engler, Julian M. W. Chan, Jeannette M. García, Daniel J. Coady, Ana Pascual, David Mecerreyes, Gavin O. Jones, Julia E. Rice, Hans W. Horn, and James L. Hedrick pp 16235–16241 DOI: 10.1021/ja408641g Supporting Info |
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Correction to “Real-Time Observation of Multiple-Protein Complex Formation with Single-Molecule FRET” Wooli Bae, Mal-Gi Choi, Changbong Hyeon, Yeon-Kyun Shin, and Tae-Young Yoon pp 16242–16242 DOI: 10.1021/ja409056b |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 16243–16244 DOI: 10.1021/ja411008g |
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Kinetic Solvent Isotope Effect in Human P450 CYP17A1-Mediated Androgen Formation: Evidence for a Reactive Peroxoanion Intermediate Michael C. Gregory, Ilia G. Denisov, Yelena V. Grinkova, Yogan Khatri, and Stephen G. Sligar pp 16245–16247 DOI: 10.1021/ja4086403 Supporting Info |
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A Selective Stepwise Heme Oxygenase Model System: An Iron(IV)-Oxo Porphyrin π-Cation Radical Leads to a Verdoheme-Type Compound via an Isoporphyrin Intermediate Isaac Garcia-Bosch, Savita K. Sharma, and Kenneth D. Karlin pp 16248–16251 DOI: 10.1021/ja405739m Supporting Info |
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Photochemical Reduction of Carbon Dioxide to Methanol and Formate in a Homogeneous System with Pyridinium Catalysts David J. Boston, Chengdong Xu, Daniel W. Armstrong, and Frederick M. MacDonnell pp 16252–16255 DOI: 10.1021/ja406074w Supporting Info |
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Thermochemical Evidence for Strong Iodine Chemisorption by ZIF-8 James T. Hughes, Dorina F. Sava, Tina M. Nenoff, and Alexandra Navrotsky pp 16256–16259 DOI: 10.1021/ja406081r Supporting Info |
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Complexation-Induced Control of Electron Propagation Based on Bounded Diffusion through Nanopore-Tethered Ferrocenes Feng Li and Takashi Ito pp 16260–16263 DOI: 10.1021/ja407002d Supporting Info |
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Decoupling Interfacial Reactions between Plasmas and Liquids: Charge Transfer vs Plasma Neutral Reactions Paul Rumbach, Megan Witzke, R. Mohan Sankaran, and David B. Go pp 16264–16267 DOI: 10.1021/ja407149y Supporting Info |
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Water-Enabled Visual Detection of DNA Yonghui Liu, Huaxin Yao, and Jin Zhu pp 16268–16271 DOI: 10.1021/ja407362c Supporting Info |
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Tuning Omniphobicity via Morphological Control of Metal–Organic Framework Functionalized Surfaces Tristan T. Y. Tan, Michael R. Reithofer, Eric Y. Chen, Ajay G. Menon, T. S. Andy Hor, Jianwei Xu, and Jia Min Chin pp 16272–16275 DOI: 10.1021/ja407896m Supporting Info |
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Microporous Brookite-Phase Titania Made by Replication of a Metal–Organic Framework Anthony Shoji Hall, Atsushi Kondo, Kazuyuki Maeda, and Thomas E. Mallouk pp 16276–16279 DOI: 10.1021/ja4083254 Supporting Info |
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Hollow Carbon-Nanotube/Carbon-Nanofiber Hybrid Anodes for Li-Ion Batteries Yuming Chen, Xiaoyan Li, Kyusung Park, Jie Song, Jianhe Hong, Limin Zhou, Yiu-Wing Mai, Haitao Huang, and John B. Goodenough pp 16280–16283 DOI: 10.1021/ja408421n Supporting Info |
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Crystallographic Dependence of CO Activation on Cobalt Catalysts: HCP versus FCC Jin-Xun Liu, Hai-Yan Su, Da-Peng Sun, Bing-Yan Zhang, and Wei-Xue Li pp 16284–16287 DOI: 10.1021/ja408521w Supporting Info |
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Nickel/Bis(oxazoline)-Catalyzed Asymmetric Negishi Arylations of Racemic Secondary Benzylic Electrophiles to Generate Enantioenriched 1,1-Diarylalkanes Hien-Quang Do, E. R. R. Chandrashekar, and Gregory C. Fu pp 16288–16291 DOI: 10.1021/ja408561b Supporting Info |
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Cu(OTf)2-Mediated Fluorination of Aryltrifluoroborates with Potassium Fluoride Yingda Ye, Sydonie D. Schimler, Patrick S. Hanley, and Melanie S. Sanford pp 16292–16295 DOI: 10.1021/ja408607r Supporting Info |
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Nylon-3 Polymers That Enable Selective Culture of Endothelial Cells Runhui Liu, Xinyu Chen, Samuel H. Gellman, and Kristyn S. Masters pp 16296–16299 DOI: 10.1021/ja408634a Supporting Info |
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CO2-Stimulated Diversiform Deformations of Polymer Assemblies Qiang Yan and Yue Zhao pp 16300–16303 DOI: 10.1021/ja408655n Supporting Info |
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A Nanopore–Nanofiber Mesh Biosensor To Control DNA Translocation Allison H. Squires, Joseph S. Hersey, Mark W. Grinstaff, and Amit Meller pp 16304–16307 DOI: 10.1021/ja408685x Supporting Info |
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Tubular Polymersomes: A Cross-Linker-Induced Shape Transformation Matthijs C. M. van Oers, Floris P. J. T. Rutjes, and Jan C. M. van Hest pp 16308–16311 DOI: 10.1021/ja408754z Supporting Info |
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Dihaloiodoarenes: α,α-Dihalogenation of Phenylacetate Derivatives Jason Tao, Richard Tran, and Graham K. Murphy pp 16312–16315 DOI: 10.1021/ja408678p Supporting Info |
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A Robust Ni(II) α-Diimine Catalyst for High Temperature Ethylene Polymerization Jennifer L. Rhinehart, Lauren A. Brown, and Brian K. Long pp 16316–16319 DOI: 10.1021/ja408905t Supporting Info |
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Ruthenium Catalyzed Hydrohydroxyalkylation of Isoprene with Heteroaromatic Secondary Alcohols: Isolation and Reversible Formation of the Putative Metallacycle Intermediate Boyoung Y. Park, T. Patrick Montgomery, Victoria J. Garza, and Michael J. Krische pp 16320–16323 DOI: 10.1021/ja4087193 Supporting Info |
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Coupled Methyl Group Epimerization and Reduction by Polyketide Synthase Ketoreductase Domains. Ketoreductase-Catalyzed Equilibrium Isotope Exchange Ashish Garg, Chaitan Khosla, and David E. Cane pp 16324–16327 DOI: 10.1021/ja408944s Supporting Info |
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Systematic Modulation of Quantum (Electron) Tunneling Behavior by Atomic Layer Deposition on Nanoparticulate SnO2 and TiO2 Photoanodes Chaiya Prasittichai, Jason R. Avila, Omar K. Farha, and Joseph T. Hupp pp 16328–16331 DOI: 10.1021/ja4089555 Supporting Info |
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Magnetic Poles Determinations and Robustness of Memory Effect upon Solubilization in a DyIII-Based Single Ion Magnet Tamyris T. da Cunha, Julie Jung, Marie-Emmanuelle Boulon, Giulio Campo, Fabrice Pointillart, Cynthia L. M. Pereira, Boris Le Guennic, Olivier Cador, Kevin Bernot, Francesco Pineider, Stéphane Golhen, and Lahcène Ouahab pp 16332–16335 DOI: 10.1021/ja4089956 Supporting Info |
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Single-Crystal Structure of a Covalent Organic Framework Yue-Biao Zhang, Jie Su, Hiroyasu Furukawa, Yifeng Yun, Felipe Gándara, Adam Duong, Xiaodong Zou, and Omar M. Yaghi pp 16336–16339 DOI: 10.1021/ja409033p Supporting Info |
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Cyclopentasilane-Fused Hexasilabenzvalene Akihiro Tsurusaki, Chisato Iizuka, Kyohei Otsuka, and Soichiro Kyushin pp 16340–16343 DOI: 10.1021/ja409074m Supporting Info |
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Pd-Catalyzed Enantioselective C–H Iodination: Asymmetric Synthesis of Chiral Diarylmethylamines Ling Chu, Xiao-Chen Wang, Curtis E. Moore, Arnold L. Rheingold, and Jin-Quan Yu pp 16344–16347 DOI: 10.1021/ja408864c Supporting Info |
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Bifunctional Iminophosphorane Organocatalysts for Enantioselective Synthesis: Application to the Ketimine Nitro-Mannich Reaction Marta G. Núñez, Alistair J. M. Farley, and Darren J. Dixon pp 16348–16351 DOI: 10.1021/ja409121s Supporting Info |
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Oxidant-Free Conversion of Primary Amines to Nitriles Kuei-Nin T. Tseng, Andrew M. Rizzi, and Nathaniel K. Szymczak pp 16352–16355 DOI: 10.1021/ja409223a Supporting Info |
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Metal–Organic Framework-Immobilized Polyhedral Metal Nanocrystals: Reduction at Solid–Gas Interface, Metal Segregation, Core–Shell Structure, and High Catalytic Activity Arshad Aijaz, Tomoki Akita, Nobuko Tsumori, and Qiang Xu pp 16356–16359 DOI: 10.1021/ja4093055 Supporting Info |
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Discovery of a Cyclic Phosphodiesterase That Catalyzes the Sequential Hydrolysis of Both Ester Bonds to Phosphorus Swapnil V. Ghodge, Jennifer A. Cummings, Howard J. Williams, and Frank M. Raushel pp 16360–16363 DOI: 10.1021/ja409376k Supporting Info |
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Ultrafast Charge Separation in Organic Photovoltaics Enhanced by Charge Delocalization and Vibronically Hot Exciton Dissociation Hiroyuki Tamura and Irene Burghardt pp 16364–16367 DOI: 10.1021/ja4093874 Supporting Info |
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DNA Double Strand Cleavage via Interstrand Hydrogen Atom Abstraction Marisa L. Taverna Porro and Marc M. Greenberg pp 16368–16371 DOI: 10.1021/ja409513q Supporting Info |
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An Efficient Generation of a Functionalized Tertiary-Alkyl Radical for Copper-catalyzed Tertiary-Alkylative Mizoroki-Heck type Reaction Takashi Nishikata, Yushi Noda, Ryo Fujimoto, and Tomomi Sakashita pp 16372–16375 DOI: 10.1021/ja409661n Supporting Info |
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Controllable Direct Arylation: Fast Route to Symmetrical and Unsymmetrical 4,7-Diaryl-5,6-difluoro-2,1,3-benzothiadiazole Derivatives for Organic Optoelectronic Materials Junxiang Zhang, Wayne Chen, Anthony J. Rojas, Evgheni V. Jucov, Tatiana V. Timofeeva, Timothy C. Parker, Stephen Barlow, and Seth R. Marder pp 16376–16379 DOI: 10.1021/ja4095878 Supporting Info |
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Brønsted Acid Catalyzed Enantioselective Indole Aza-Claisen Rearrangement Mediated by an Arene CH–O Interaction Pradip Maity, Ryan P. Pemberton, Dean J. Tantillo, and Uttam K. Tambar pp 16380–16383 DOI: 10.1021/ja4095473 Supporting Info |
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Isolation, Structure, and Reactivity of an Arylnickel(II) Pivalate Complex in Catalytic C–H/C–O Biaryl Coupling Kei Muto, Junichiro Yamaguchi, Aiwen Lei, and Kenichiro Itami pp 16384–16387 DOI: 10.1021/ja409803x Supporting Info |
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Simultaneous Dual Protein Labeling Using a Triorthogonal Reagent Mohammad Rashidian, Sidath C. Kumarapperuma, Kari Gabrielse, Adrian Fegan, Carston R. Wagner, and Mark D. Distefano pp 16388–16396 DOI: 10.1021/ja403813b Supporting Info |
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Design and Synthesis of Curcumin Analogues for in Vivo Fluorescence Imaging and Inhibiting Copper-Induced Cross-Linking of Amyloid Beta Species in Alzheimer’s Disease Xueli Zhang, Yanli Tian, Zeng Li, Xiaoyu Tian, Hongbin Sun, Hong Liu, Anna Moore, and Chongzhao Ran pp 16397–16409 DOI: 10.1021/ja405239v Supporting Info |
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Optically Modulatable Blue Fluorescent Proteins Amy E. Jablonski, Russell B. Vegh, Jung-Cheng Hsiang, Bettina Bommarius, Yen-Cheng Chen, Kyril M. Solntsev, Andreas S. Bommarius, Laren M. Tolbert, and Robert M. Dickson pp 16410–16417 DOI: 10.1021/ja405459b Supporting Info |
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Interactions of Bacterial Cell Division Protein FtsZ with C8-Substituted Guanine Nucleotide Inhibitors. A Combined NMR, Biochemical and Molecular Modeling Perspective Filipa Marcelo, Sonia Huecas, Laura B. Ruiz-Ávila, F. Javier Cañada, Almudena Perona, Ana Poveda, Sonsoles Martín-Santamaría, Antonio Morreale, Jesús Jiménez-Barbero, and José M. Andreu pp 16418–16428 DOI: 10.1021/ja405515r Supporting Info |
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Rh(I) Complexes Bearing N,N and N,P Ligands Anchored on Glassy Carbon Electrodes: Toward Recyclable Hydroamination Catalysts Andrey A. Tregubov, Khuong Q. Vuong, Erwann Luais, J. Justin Gooding, and Barbara A. Messerle pp 16429–16437 DOI: 10.1021/ja405783g Supporting Info |
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Noncanonical Self-Assembly of Multifunctional DNA Nanoflowers for Biomedical Applications Guizhi Zhu, Rong Hu, Zilong Zhao, Zhuo Chen, Xiaobing Zhang, and Weihong Tan pp 16438–16445 DOI: 10.1021/ja406115e Supporting Info |
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Red-Light-Controllable Liquid-Crystal Soft Actuators via Low-Power Excited Upconversion Based on Triplet–Triplet Annihilation Zhen Jiang, Ming Xu, Fuyou Li, and Yanlei Yu pp 16446–16453 DOI: 10.1021/ja406020r Supporting Info |
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Stepwise Protonation and Electron-Transfer Reduction of a Primary Copper–Dioxygen Adduct Ryan L. Peterson, Jake W. Ginsbach, Ryan E. Cowley, Munzarin F. Qayyum, Richard A. Himes, Maxime A. Siegler, Cathy D. Moore, Britt Hedman, Keith O. Hodgson, Shunichi Fukuzumi, Edward I. Solomon, and Kenneth D. Karlin pp 16454–16467 DOI: 10.1021/ja4065377 Supporting Info |
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Development of a New Method for Synthesis of Tandem Hairpin Pyrrole–Imidazole Polyamide Probes Targeting Human Telomeres Yusuke Kawamoto, Toshikazu Bando, Fukumi Kamada, Yue Li, Kaori Hashiya, Kazuhiro Maeshima, and Hiroshi Sugiyama pp 16468–16477 DOI: 10.1021/ja406737n Supporting Info |
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Local and Average Structure in Zinc Cyanide: Toward an Understanding of the Atomistic Origin of Negative Thermal Expansion Simon J. Hibble, Ann M. Chippindale, Elena Marelli, Scott Kroeker, Vladimir K. Michaelis, Brandon J. Greer, Pedro M. Aguiar, Edward J. Bilbé, Emma R. Barney, and Alex C. Hannon pp 16478–16489 DOI: 10.1021/ja406848s Supporting Info |
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Morphology Control of Nanofibril Donor–Acceptor Heterojunction To Achieve High Photoconductivity: Exploration of New Molecular Design Rule Helin Huang, Ching-En Chou, Yanke Che, Ligui Li, Chen Wang, Xiaomei Yang, Zhonghua Peng, and Ling Zang pp 16490–16496 DOI: 10.1021/ja407024u Supporting Info |
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Conformational Analysis of Chiral Supramolecular Aggregates: Modeling the Subtle Difference between Hydrogen and Deuterium Yoko Nakano, Albert J. Markvoort, Seda Cantekin, Ivo A. W. Filot, Huub M. M. ten Eikelder, E. W. Meijer, and Anja R. A. Palmans pp 16497–16506 DOI: 10.1021/ja4073645 Supporting Info |
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High-Pressure Synthesis of 5d Cubic Perovskite BaOsO3 at 17 GPa: Ferromagnetic Evolution over 3d to 5d Series Youguo Shi, Yanfeng Guo, Yuichi Shirako, Wei Yi, Xia Wang, Alexei A. Belik, Yoshitaka Matsushita, Hai Luke Feng, Yoshihiro Tsujimoto, Masao Arai, Nanlin Wang, Masaki Akaogi, and Kazunari Yamaura pp 16507–16516 DOI: 10.1021/ja4074408 Supporting Info |
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Translocation of Cationic Amphipathic Peptides across the Membranes of Pure Phospholipid Giant Vesicles Sterling A. Wheaten, Francis D. O. Ablan, B. Logan Spaller, Julie M. Trieu, and Paulo F. Almeida pp 16517–16525 DOI: 10.1021/ja407451c |
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Equatorenes: Synthesis and Properties of Chiral Naphthalene, Phenanthrene, Chrysene, and Pyrene Possessing Bis(1-adamantyl) Groups at the Peri-position Koji Yamamoto, Naohiro Oyamada, Sheng Xia, Yuta Kobayashi, Masahiko Yamaguchi, Hiroaki Maeda, Hiroshi Nishihara, Tadafumi Uchimaru, and Eunsang Kwon pp 16526–16532 DOI: 10.1021/ja407800e Supporting Info |
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Composite Molecular Assemblies: Nanoscale Structural Control and Spectroelectrochemical Diversity Graham de Ruiter, Michal Lahav, Guennadi Evmenenko, Pulak Dutta, Domenico A. Cristaldi, Antonino Gulino, and Milko E. van der Boom pp 16533–16544 DOI: 10.1021/ja407659z Supporting Info |
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Thermoelectric Efficiency of Organometallic Complex Wires via Quantum Resonance Effect and Long-Range Electric Transport Property Hisao Nakamura, Tatsuhiko Ohto, Takao Ishida, and Yoshihiro Asai pp 16545–16552 DOI: 10.1021/ja407662m Supporting Info |
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Redox-Controlled Polymerization of Lactide Catalyzed by Bis(imino)pyridine Iron Bis(alkoxide) Complexes Ashley B. Biernesser, Bo Li, and Jeffery A. Byers pp 16553–16560 DOI: 10.1021/ja407920d Supporting Info |
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A Structural Study of Ion Permeation in OmpF Porin from Anomalous X-ray Diffraction and Molecular Dynamics Simulations Balasundaresan Dhakshnamoorthy, Brigitte K. Ziervogel, Lydia Blachowicz, and Benoît Roux pp 16561–16568 DOI: 10.1021/ja407783a Supporting Info |
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Controlling Carrier Densities in Photochemically Reduced Colloidal ZnO Nanocrystals: Size Dependence and Role of the Hole Quencher Alina M. Schimpf, Carolyn E. Gunthardt, Jeffrey D. Rinehart, James M. Mayer, and Daniel R. Gamelin pp 16569–16577 DOI: 10.1021/ja408030u Supporting Info |
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Foldameric α/β-Peptide Analogs of the β-Sheet-Forming Antiangiogenic Anginex: Structure and Bioactivity Zsófia Hegedüs, Edit Wéber, Éva Kriston-Pál, Ildikó Makra, Ágnes Czibula, Éva Monostori, and Tamás A. Martinek pp 16578–16584 DOI: 10.1021/ja408054f Supporting Info |
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π-Electron Conjugation in Two Dimensions Rico Gutzler and Dmitrii F. Perepichka pp 16585–16594 DOI: 10.1021/ja408355p Supporting Info |
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Recovering a Representative Conformational Ensemble from Underdetermined Macromolecular Structural Data Konstantin Berlin, Carlos A. Castañeda, Dina Schneidman-Duhovny, Andrej Sali, Alfredo Nava-Tudela, and David Fushman pp 16595–16609 DOI: 10.1021/ja4083717 Supporting Info |
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Radical Cyclizations of Cyclic Ene Sulfonamides Occur with β-Elimination of Sulfonyl Radicals to Form Polycyclic Imines Hanmo Zhang, E. Ben Hay, Steven J. Geib, and Dennis P. Curran pp 16610–16617 DOI: 10.1021/ja408387d Supporting Info |
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Detection of Specific Protein–Protein Interactions in Nanocages by Engineering Bipartite FlAsH Binding Sites Thomas A. Cornell, Jing Fu, Stephanie H. Newland, and Brendan P. Orner pp 16618–16624 DOI: 10.1021/ja4085034 Supporting Info |
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Rhodium(III)-Catalyzed Indole Synthesis Using N–N Bond as an Internal Oxidant Baoqing Liu, Chao Song, Chao Sun, Shuguang Zhou, and Jin Zhu pp 16625–16631 DOI: 10.1021/ja408541c Supporting Info |
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Electrochemical Assay for the Signal-On Detection of Human DNA Methyltransferase Activity Natalie B. Muren and Jacqueline K. Barton pp 16632–16640 DOI: 10.1021/ja4085918 |
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Kinetics of Allosteric Transitions in S-adenosylmethionine Riboswitch Are Accurately Predicted from the Folding Landscape Jong-Chin Lin and D. Thirumalai pp 16641–16650 DOI: 10.1021/ja408595e |
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Observing Assembly of Complex Inorganic Materials from Polyoxometalate Building Blocks Yu Hou, Lev N. Zakharov, and May Nyman pp 16651–16657 DOI: 10.1021/ja4086484 Supporting Info |
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Confining the Nucleation and Overgrowth of Rh to the {111} Facets of Pd Nanocrystal Seeds: The Roles of Capping Agent and Surface Diffusion Shuifen Xie, Hsin-Chieh Peng, Ning Lu, Jinguo Wang, Moon J. Kim, Zhaoxiong Xie, and Younan Xia pp 16658–16667 DOI: 10.1021/ja408768e Supporting Info |
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High-Pressure Synthesis and Characterization of Li2Ca3[N2]3—An Uncommon Metallic Diazenide with [N2]2– Ions Sebastian B. Schneider, Markus Seibald, Volker L. Deringer, Ralf P. Stoffel, Rainer Frankovsky, Gina M. Friederichs, Henryk Laqua, Viola Duppel, Gunnar Jeschke, Richard Dronskowski, and Wolfgang Schnick pp 16668–16679 DOI: 10.1021/ja408816t Supporting Info |
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Temperature-Independent Singlet Exciton Fission in Tetracene Mark W. B. Wilson, Akshay Rao, Kerr Johnson, Simon Gélinas, Riccardo di Pietro, Jenny Clark, and Richard H. Friend pp 16680–16688 DOI: 10.1021/ja408854u Supporting Info |
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Enhanced CO Oxidation Rates at the Interface of Mesoporous Oxides and Pt Nanoparticles Kwangjin An, Selim Alayoglu, Nathan Musselwhite, Sheba Plamthottam, Gérôme Melaet, Avery E. Lindeman, and Gabor A. Somorjai pp 16689–16696 DOI: 10.1021/ja4088743 Supporting Info |
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Chemiluminescent Detection of Enzymatically Produced Hydrogen Sulfide: Substrate Hydrogen Bonding Influences Selectivity for H2S over Biological Thiols T. Spencer Bailey and Michael D. Pluth pp 16697–16704 DOI: 10.1021/ja408909h Supporting Info |
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Picomolar Inhibitors of HIV Reverse Transcriptase Featuring Bicyclic Replacement of a Cyanovinylphenyl Group Won-Gil Lee, Ricardo Gallardo-Macias, Kathleen M. Frey, Krasimir A. Spasov, Mariela Bollini, Karen S. Anderson, and William L. Jorgensen pp 16705–16713 DOI: 10.1021/ja408917n Supporting Info |
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Two-Photon Chemistry from Upper Triplet States of Thymine Victoria Vendrell-Criado, Gemma M. Rodríguez-Muñiz, Minoru Yamaji, Virginie Lhiaubet-Vallet, M. Consuelo Cuquerella, and Miguel A. Miranda pp 16714–16719 DOI: 10.1021/ja408997j Supporting Info |
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Rapid Access to Spirocyclic Oxindole Alkaloids: Application of the Asymmetric Palladium-Catalyzed [3 + 2] Trimethylenemethane Cycloaddition Barry M. Trost, Dustin A. Bringley, Ting Zhang, and Nicolai Cramer pp 16720–16735 DOI: 10.1021/ja409013m Supporting Info |
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Yolk–Shell Structure of Polyaniline-Coated Sulfur for Lithium–Sulfur Batteries Weidong Zhou, Yingchao Yu, Hao Chen, Francis J. DiSalvo, and Héctor D. Abruña pp 16736–16743 DOI: 10.1021/ja409508q Supporting Info |
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Asymmetric Organocatalytic Thio-Diels–Alder Reactions via Trienamine Catalysis Hao Jiang, David Cruz Cruz, Yang Li, Vibeke Henriette Lauridsen, and Karl Anker Jørgensen pp 16744–16744 DOI: 10.1021/ja409090j |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 16745–16745 DOI: 10.1021/ja411266n |
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Copper(I) Nitrosyls from Reaction of Copper(II) Thiolates with S-Nitrosothiols: Mechanism of NO Release from RSNOs at Cu Shiyu Zhang, Nihan Çelebi-Ölçüm, Marie M. Melzer, K. N. Houk, and Timothy H. Warren pp 16746–16749 DOI: 10.1021/ja406476y Supporting Info |
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Chemoproteomic Discovery of Cysteine-Containing Human Short Open Reading Frames Adam G. Schwaid, D. Alexander Shannon, Jiao Ma, Sarah A. Slavoff, Joshua Z. Levin, Eranthie Weerapana, and Alan Saghatelian pp 16750–16753 DOI: 10.1021/ja406606j Supporting Info |
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Silver-Mediated Oxidative C–H/P–H Functionalization: An Efficient Route for the Synthesis of Benzo[b]phosphole Oxides Yun-Rong Chen and Wei-Liang Duan pp 16754–16757 DOI: 10.1021/ja407373g Supporting Info |
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A 2.8 Å Fe–Fe Separation in the Fe2III/IV Intermediate, X, from Escherichia coli Ribonucleotide Reductase Laura M. K. Dassama, Alexey Silakov, Courtney M. Krest, Julio C. Calixto, Carsten Krebs, J. Martin Bollinger, Jr., and Michael T. Green pp 16758–16761 DOI: 10.1021/ja407438p Supporting Info |
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Metallic Nanocages: Synthesis of Bimetallic Pt–Pd Hollow Nanoparticles with Dendritic Shells by Selective Chemical Etching Liang Wang and Yusuke Yamauchi pp 16762–16765 DOI: 10.1021/ja407773x Supporting Info |
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Fluorogenic, Two-Photon-Triggered Photoclick Chemistry in Live Mammalian Cells Zhipeng Yu, Tymish Y. Ohulchanskyy, Peng An, Paras N. Prasad, and Qing Lin pp 16766–16769 DOI: 10.1021/ja407867a Supporting Info |
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Electroanalytical Evaluation of Antioxidant Activity of Cerium Oxide Nanoparticles by Nanoparticle Collisions at Microelectrodes Naimish P. Sardesai, Daniel Andreescu, and Silvana Andreescu pp 16770–16773 DOI: 10.1021/ja408087s Supporting Info |
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The Direct Oxidative Addition of O2 to a Mononuclear Cr(I) Complex Is Spin Forbidden Fang Dai, Glenn P. A. Yap, and Klaus H. Theopold pp 16774–16776 DOI: 10.1021/ja408357x Supporting Info |
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Inhibitory Effect of Ethylene in Ene–Yne Metathesis: The Case for Ruthenacyclobutane Resting States Timothy M. Gregg, Jerome B. Keister, and Steven T. Diver pp 16777–16780 DOI: 10.1021/ja4085012 Supporting Info |
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In Situ Imaging of Cu2O under Reducing Conditions: Formation of Metallic Fronts by Mass Transfer Ashleigh E. Baber, Fang Xu, Filip Dvorak, Kumudu Mudiyanselage, Markus Soldemo, Jonas Weissenrieder, Sanjaya D. Senanayake, Jerzy T. Sadowski, José A. Rodriguez, Vladimír Matolín, Michael G. White, and Darío J. Stacchiola pp 16781–16784 DOI: 10.1021/ja408506y Supporting Info |
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A Multistage Volumetric Bar Chart Chip for Visualized Quantification of DNA Yujun Song, Yuanchen Wang, and Lidong Qin pp 16785–16788 DOI: 10.1021/ja4085397 Supporting Info |
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Peptide Nanofibers with Dynamic Instability through Nonequilibrium Biocatalytic Assembly Sisir Debnath, Sangita Roy, and Rein V. Ulijn pp 16789–16792 DOI: 10.1021/ja4086353 Supporting Info |
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Hybrid Bombesin Analogues: Combining an Agonist and an Antagonist in Defined Distances for Optimized Tumor Targeting Carsten Kroll, Rosalba Mansi, Friederike Braun, Stefanie Dobitz, Helmut R. Maecke, and Helma Wennemers pp 16793–16796 DOI: 10.1021/ja4087648 Supporting Info |
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Rhodium-Catalyzed Tandem Annulation and (5 + 1) Cycloaddition: 3-Hydroxy-1,4-enyne as the 5-Carbon Component Xiaoxun Li, Wangze Song, and Weiping Tang pp 16797–16800 DOI: 10.1021/ja408829y Supporting Info |
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Perfluoroalkane Functionalization of NU-1000 via Solvent-Assisted Ligand Incorporation: Synthesis and CO2 Adsorption Studies Pravas Deria, Joseph E. Mondloch, Emmanuel Tylianakis, Pritha Ghosh, Wojciech Bury, Randall Q. Snurr, Joseph T. Hupp, and Omar K. Farha pp 16801–16804 DOI: 10.1021/ja408959g Supporting Info |
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A Cytochrome P450 Serves as an Unexpected Terpene Cyclase during Fungal Meroterpenoid Biosynthesis Yit-Heng Chooi, Young J. Hong, Ralph A. Cacho, Dean J. Tantillo, and Yi Tang pp 16805–16808 DOI: 10.1021/ja408966t Supporting Info |
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In Vitro Reconstitution and Analysis of the 6-Deoxyerythronolide B Synthase Brian Lowry, Thomas Robbins, Chih-Hisang Weng, Robert V. O’Brien, David E. Cane, and Chaitan Khosla pp 16809–16812 DOI: 10.1021/ja409048k Supporting Info |
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Dendronized Organoplatinum(II) Metallacyclic Polymers Constructed by Hierarchical Coordination-Driven Self-Assembly and Hydrogen-Bonding Interfaces Xuzhou Yan, Bo Jiang, Timothy R. Cook, Yanyan Zhang, Jinying Li, Yihua Yu, Feihe Huang, Hai-Bo Yang, and Peter J. Stang pp 16813–16816 DOI: 10.1021/ja4092193 Supporting Info |
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Photolithographic Olefin Metathesis Polymerization Raymond A. Weitekamp, Harry A. Atwater, and Robert H. Grubbs pp 16817–16820 DOI: 10.1021/ja4093083 Supporting Info |
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β-Ketoenamine-Linked Covalent Organic Frameworks Capable of Pseudocapacitive Energy Storage Catherine R. DeBlase, Katharine E. Silberstein, Thanh-Tam Truong, Héctor D. Abruña, and William R. Dichtel pp 16821–16824 DOI: 10.1021/ja409421d Supporting Info |
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CO2 Capture by a Rhenium(I) Complex with the Aid of Triethanolamine Tatsuki Morimoto, Takuya Nakajima, Shuhei Sawa, Ryoichi Nakanishi, Daisuke Imori, and Osamu Ishitani pp 16825–16828 DOI: 10.1021/ja409271s Supporting Info |
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Asymmetric Synthesis of QUINAP via Dynamic Kinetic Resolution Vikram Bhat, Su Wang, Brian M. Stoltz, and Scott C. Virgil pp 16829–16832 DOI: 10.1021/ja409383f Supporting Info |
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Monodisperse Au Nanoparticles for Selective Electrocatalytic Reduction of CO2 to CO Wenlei Zhu, Ronald Michalsky, Önder Metin, Haifeng Lv, Shaojun Guo, Christopher J. Wright, Xiaolian Sun, Andrew A. Peterson, and Shouheng Sun pp 16833–16836 DOI: 10.1021/ja409445p Supporting Info |
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Nucleophile-Catalyzed, Facile, and Highly Selective C–H Activation of Fluoroform with Pd(II) Shin Takemoto and Vladimir V. Grushin pp 16837–16840 DOI: 10.1021/ja409533s Supporting Info |
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A Palladium-Catalyzed Carbonylation Approach to Acid Chloride Synthesis Jeffrey S. Quesnel and Bruce A. Arndtsen pp 16841–16844 DOI: 10.1021/ja4098093 Supporting Info |
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An Azophenine Radical-Bridged Fe2 Single-Molecule Magnet with Record Magnetic Exchange Coupling Ie-Rang Jeon, Jesse G. Park, Dianne J. Xiao, and T. David Harris pp 16845–16848 DOI: 10.1021/ja409927v Supporting Info |
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A Highly Efficient and Enantioselective Intramolecular Cannizzaro Reaction under TOX/Cu(II) Catalysis Pan Wang, Wen-Jie Tao, Xiu-Li Sun, Saihu Liao, and Yong Tang pp 16849–16852 DOI: 10.1021/ja409859x Supporting Info |
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Enediolate–Dilithium Amide Mixed Aggregates in the Enantioselective Alkylation of Arylacetic Acids: Structural Studies and a Stereochemical Model Yun Ma, Craig E. Stivala, Ashley M. Wright, Trevor Hayton, Jun Liang, Ivan Keresztes, Emil Lobkovsky, David B. Collum, and Armen Zakarian pp 16853–16864 DOI: 10.1021/ja403076u Supporting Info |
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Dynamic Anchoring of the 3′-End of the Guide Strand Controls the Target Dissociation of Argonaute–Guide Complex Seung-Ryoung Jung, Eunji Kim, Wonseok Hwang, Soochul Shin, Ji-Joon Song, and Sungchul Hohng pp 16865–16871 DOI: 10.1021/ja403138d Supporting Info |
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Visible-Light-Induced Water Splitting Based on Two-Step Photoexcitation between Dye-Sensitized Layered Niobate and Tungsten Oxide Photocatalysts in the Presence of a Triiodide/Iodide Shuttle Redox Mediator Ryu Abe, Kenichi Shinmei, Nagatoshi Koumura, Kohjiro Hara, and Bunsho Ohtani pp 16872–16884 DOI: 10.1021/ja4048637 |
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Concerted Action of P450 Plus Helper Protein To Form the Amino-hydroxy-piperidone Moiety of the Potent Protease Inhibitor Crocapeptin Konrad Viehrig, Frank Surup, Kirsten Harmrolfs, Rolf Jansen, Brigitte Kunze, and Rolf Müller pp 16885–16894 DOI: 10.1021/ja4047153 Supporting Info |
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‘Naked’ and Hydrated Conformers of the Conserved Core Pentasaccharide of N-linked Glycoproteins and Its Building Blocks Conor S. Barry, Emilio J. Cocinero, Pierre Çarçabal, David P. Gamblin, E. Cristina Stanca-Kaposta, Sarah M. Remmert, María C. Fernández-Alonso, Svemir Rudić, John P. Simons, and Benjamin G. Davis pp 16895–16903 DOI: 10.1021/ja4056678 Supporting Info |
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Microsclerodermins from Terrestrial Myxobacteria: An Intriguing Biosynthesis Likely Connected to a Sponge Symbiont Thomas Hoffmann, Stefan Müller, Suvd Nadmid, Ronald Garcia, and Rolf Müller pp 16904–16911 DOI: 10.1021/ja4054509 Supporting Info |
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Tunable Porous Organic Crystals: Structural Scope and Adsorption Properties of Nanoporous Steroidal Ureas Ramalingam Natarajan, Lydia Bridgland, Anchalee Sirikulkajorn, Ji-Hun Lee, Mairi F. Haddow, Germinal Magro, Bakhat Ali, Sampriya Narayanan, Peter Strickland, Jonathan P. H. Charmant, A. Guy Orpen, Neil B. McKeown, C. Grazia Bezzu, and Anthony P. Davis pp 16912–16925 DOI: 10.1021/ja405701u Supporting Info |
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Ion Mobility Spectrometry Reveals the Mechanism of Amyloid Formation of Aβ(25–35) and Its Modulation by Inhibitors at the Molecular Level: Epigallocatechin Gallate and Scyllo-inositol Christian Bleiholder, Thanh D. Do, Chun Wu, Nicholas J. Economou, Summer S. Bernstein, Steven K. Buratto, Joan-Emma Shea, and Michael T. Bowers pp 16926–16937 DOI: 10.1021/ja406197f Supporting Info |
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Formation of N-Heterocyclic Carbene–Boryl Radicals through Electrochemical and Photochemical Cleavage of the B–S bond in N-Heterocyclic Carbene–Boryl Sulfides Sofia Telitel, Anne-Laure Vallet, Stéphane Schweizer, Bernard Delpech, Nicolas Blanchard, Fabrice Morlet-Savary, Bernadette Graff, Dennis P. Curran, Marc Robert, Emmanuel Lacôte, and Jacques Lalevée pp 16938–16947 DOI: 10.1021/ja4066267 Supporting Info |
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Development of Activity-Based Probes for Ubiquitin and Ubiquitin-like Protein Signaling Pathways Heeseon An and Alexander V. Statsyuk pp 16948–16962 DOI: 10.1021/ja4099643 Supporting Info |
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Pyrogallol[4]arenes as Frustrated Organic Solids Harshita Kumari, Loredana Erra, Alicia C. Webb, Prashant Bhatt, Charles L. Barnes, Carol A. Deakyne, John E. Adams, Leonard J. Barbour, and Jerry L. Atwood pp 16963–16967 DOI: 10.1021/ja406643b Supporting Info |
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Protein Dielectric Constants Determined from NMR Chemical Shift Perturbations Predrag Kukic, Damien Farrell, Lawrence P. McIntosh, Bertrand García-Moreno E., Kristine Steen Jensen, Zigmantas Toleikis, Kaare Teilum, and Jens Erik Nielsen pp 16968–16976 DOI: 10.1021/ja406995j Supporting Info |
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Benchmarking Heterogeneous Electrocatalysts for the Oxygen Evolution Reaction Charles C. L. McCrory, Suho Jung, Jonas C. Peters, and Thomas F. Jaramillo pp 16977–16987 DOI: 10.1021/ja407115p Supporting Info |
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Modulation of Electronics and Thermal Stabilities of Photochromic Phosphino–Aminoazobenzene Derivatives in Weak-Link Approach Coordination Complexes Jung Su Park, Alejo M. Lifschitz, Ryan M. Young, Jose Mendez-Arroyo, Michael R. Wasielewski, Charlotte L. Stern, and Chad A. Mirkin pp 16988–16996 DOI: 10.1021/ja407148n Supporting Info |
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Enhanced Photochemical Hydrogen Production by a Molecular Diiron Catalyst Incorporated into a Metal–Organic Framework Sonja Pullen, Honghan Fei, Andreas Orthaber, Seth M. Cohen, and Sascha Ott pp 16997–17003 DOI: 10.1021/ja407176p Supporting Info |
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Activation of Nitriles by Metal Ligand Cooperation. Reversible Formation of Ketimido- and Enamido-Rhenium PNP Pincer Complexes and Relevance to Catalytic Design Matthias Vogt, Alexander Nerush, Mark A. Iron, Gregory Leitus, Yael Diskin-Posner, Linda J. W. Shimon, Yehoshoa Ben-David, and David Milstein pp 17004–17018 DOI: 10.1021/ja4071859 Supporting Info |
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Pillar[5]arene as a Co-Factor in Templating Rotaxane Formation Chenfeng Ke, Nathan L. Strutt, Hao Li, Xisen Hou, Karel J. Hartlieb, Paul R. McGonigal, Zhidong Ma, Julien Iehl, Charlotte L. Stern, Chuyang Cheng, Zhixue Zhu, Nicolaas A. Vermeulen, Thomas J. Meade, Youssry Y. Botros, and J. Fraser Stoddart pp 17019–17030 DOI: 10.1021/ja407229h Supporting Info |
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A Kinetic Safety Gate Controlling the Delivery of Unnatural Amino Acids to the Ribosome Joerg Mittelstaet, Andrey L. Konevega, and Marina V. Rodnina pp 17031–17038 DOI: 10.1021/ja407511q Supporting Info |
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New Insights on Photocatalytic H2 Liberation from Water Using Transition-Metal Oxides: Lessons from Cluster Models of Molybdenum and Tungsten Oxides Raghunath O. Ramabhadran, Jennifer E. Mann, Sarah E. Waller, David W. Rothgeb, Caroline C. Jarrold, and Krishnan Raghavachari pp 17039–17051 DOI: 10.1021/ja4076309 Supporting Info |
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Assembly of Surface-Confined Homochiral Helicates: Chiral Discrimination of DOPA and Unidirectional Charge Transfer Revital Kaminker, Xavier de Hatten, Michal Lahav, Fabio Lupo, Antonino Gulino, Guennadi Evmenenko, Pulak Dutta, Colm Browne, Jonathan R. Nitschke, and Milko E. van der Boom pp 17052–17059 DOI: 10.1021/ja4077205 Supporting Info |
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Fluorinated Benzothiadiazole-Based Conjugated Polymers for High-Performance Polymer Solar Cells without Any Processing Additives or Post-treatments Ning Wang, Zheng Chen, Wei Wei, and Zhenhua Jiang pp 17060–17068 DOI: 10.1021/ja409881g Supporting Info |
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Short Interfering RNA Guide Strand Modifiers from Computational Screening Kazumitsu Onizuka, Jason G. Harrison, Alexi A. Ball-Jones, José M. Ibarra-Soza, Yuxuan Zheng, Diana Ly, Walter Lam, Stephanie Mac, Dean J. Tantillo, and Peter A. Beal pp 17069–17077 DOI: 10.1021/ja4079754 Supporting Info |
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New Continuous Fluorometric Assay for Bacterial Transglycosylase Using Förster Resonance Energy Transfer Shih-Hsien Huang, Wei-Shen Wu, Lin-Ya Huang, Wen-Feng Huang, Wei-Chen Fu, Po-Ting Chen, Jim-Min Fang, Wei-Chieh Cheng, Ting-Jen R. Cheng, and Chi-Huey Wong pp 17078–17089 DOI: 10.1021/ja407985m Supporting Info |
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Dichotomous Hydrogen Atom Transfer vs Proton-Coupled Electron Transfer During Activation of X–H Bonds (X = C, N, O) by Nonheme Iron–Oxo Complexes of Variable Basicity Dandamudi Usharani, David C. Lacy, A. S. Borovik, and Sason Shaik pp 17090–17104 DOI: 10.1021/ja408073m Supporting Info |
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Construction of Ultrastable Porphyrin Zr Metal–Organic Frameworks through Linker Elimination Dawei Feng, Wan-Chun Chung, Zhangwen Wei, Zhi-Yuan Gu, Hai-Long Jiang, Ying-Pin Chen, Donald J. Darensbourg, and Hong-Cai Zhou pp 17105–17110 DOI: 10.1021/ja408084j Supporting Info |
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Interdomain Dynamics Explored by Paramagnetic NMR Luigi Russo, Mitcheell Maestre-Martinez, Sebastian Wolff, Stefan Becker, and Christian Griesinger pp 17111–17120 DOI: 10.1021/ja408143f Supporting Info |
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Metal–Ligand Covalency of Iron Complexes from High-Resolution Resonant Inelastic X-ray Scattering Marcus Lundberg, Thomas Kroll, Serena DeBeer, Uwe Bergmann, Samuel A. Wilson, Pieter Glatzel, Dennis Nordlund, Britt Hedman, Keith O. Hodgson, and Edward I. Solomon pp 17121–17134 DOI: 10.1021/ja408072q Supporting Info |
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Fluorogenic α-Tocopherol Analogue for Monitoring the Antioxidant Status within the Inner Mitochondrial Membrane of Live Cells Katerina Krumova, Lana E. Greene, and Gonzalo Cosa pp 17135–17143 DOI: 10.1021/ja408227f Supporting Info |
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Superexchange Contributions to Distance Dependence of Electron Transfer/Transport: Exchange and Electronic Coupling in Oligo(para-Phenylene)- and Oligo(2,5-Thiophene)-Bridged Donor–Bridge–Acceptor Biradical Complexes Martin L. Kirk, David A. Shultz, Daniel E. Stasiw, Geoffrey F. Lewis, Guangbin Wang, Candice L. Brannen, Roger D. Sommer, and Paul D. Boyle pp 17144–17154 DOI: 10.1021/ja4081887 Supporting Info |
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Bottom-Up Construction of POM-Based Macrostructures: Coordination Assembled Paddle-Wheel Macroclusters and Their Vesicle-like Supramolecular Aggregation in Solution Yi Zhu, Panchao Yin, Fengping Xiao, Dong Li, Emily Bitterlich, Zicheng Xiao, Jin Zhang, Jian Hao, Tianbo Liu, Yuan Wang, and Yongge Wei pp 17155–17160 DOI: 10.1021/ja408228b Supporting Info |
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Exploitation of Long-Lived 3IL Excited States for Metal–Organic Photodynamic Therapy: Verification in a Metastatic Melanoma Model Richard Lincoln, Lars Kohler, Susan Monro, Huimin Yin, Mat Stephenson, Ruifa Zong, Abdellatif Chouai, Christopher Dorsey, Robie Hennigar, Randolph P. Thummel, and Sherri A. McFarland pp 17161–17175 DOI: 10.1021/ja408426z Supporting Info |
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Chirality Driven Metallic versus Semiconducting Behavior in a Complete Series of Radical Cation Salts Based on Dimethyl-Ethylenedithio-Tetrathiafulvalene (DM-EDT-TTF) Flavia Pop, Pascale Auban-Senzier, Arkadiusz Frąckowiak, Krzysztof Ptaszyński, Iwona Olejniczak, John D. Wallis, Enric Canadell, and Narcis Avarvari pp 17176–17186 DOI: 10.1021/ja408350r Supporting Info |
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The Origin of Relative Intensity Fluctuations in Single-Molecule Tip-Enhanced Raman Spectroscopy Matthew. D. Sonntag, Dhabih Chulhai, Tamar Seideman, Lasse Jensen, and Richard P. Van Duyne pp 17187–17192 DOI: 10.1021/ja408758j Supporting Info |
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Chemical Mustard Containment Using Simple Palladium Pincer Complexes: The Influence of Molecular Walls Qi-Qiang Wang, Rowshan Ara Begum, Victor W. Day, and Kristin Bowman-James pp 17193–17199 DOI: 10.1021/ja408770u Supporting Info |
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Importance of Metal Hydration on the Selectivity of Mg2+ versus Ca2+ in Magnesium Ion Channels Todor Dudev and Carmay Lim pp 17200–17208 DOI: 10.1021/ja4087769 |
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DFT Computational Study of the Methanolytic Cleavage of DNA and RNA Phosphodiester Models Promoted by the Dinuclear Zn(II) Complex of 1,3-Bis(1,5,9-triazacyclododec-1-yl)propane Christopher I. Maxwell, Nicholas J. Mosey, and R. Stan Brown pp 17209–17222 DOI: 10.1021/ja4088264 Supporting Info |
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Site-Specific Protein Transamination Using N-Methylpyridinium-4-carboxaldehyde Leah S. Witus, Chawita Netirojjanakul, Kanwal S. Palla, Ellen M. Muehl, Chih-Hisang Weng, Anthony T. Iavarone, and Matthew B. Francis pp 17223–17229 DOI: 10.1021/ja408868a Supporting Info |
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Ruthenium-Catalyzed Hydrohydroxyalkylation of Acrylates with Diols and α-Hydroxycarbonyl Compounds To Form Spiro- and α-Methylene-γ-butyrolactones Emma L. McInturff, Jeffrey Mowat, Andrew R. Waldeck, and Michael J. Krische pp 17230–17235 DOI: 10.1021/ja410533y Supporting Info |
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Correction to “A Cyclochiral Conformational Motif Constructed Using a Robust Hydrogen-Bonding Network” Kenji Mishiro, Takumi Furuta, Takahiro Sasamori, Kazuhiro Hayashi, Norihiro Tokitoh, Shiroh Futaki, and Takeo Kawabata pp 17236–17236 DOI: 10.1021/ja410281w |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 17237–17237 DOI: 10.1021/ja411538z |
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Tunable, Chemoselective Amination via Silver Catalysis Jared W. Rigoli, Cale D. Weatherly, Juliet M. Alderson, Brian T. Vo, and Jennifer M. Schomaker pp 17238–17241 DOI: 10.1021/ja406654y Supporting Info |
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Efficient Noble Metal-Free (Electro)Catalysis of Water and Alcohol Oxidations by Zinc–Cobalt Layered Double Hydroxide Xiaoxin Zou, Anandarup Goswami, and Tewodros Asefa pp 17242–17245 DOI: 10.1021/ja407174u Supporting Info |
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Photoelectrochemical Behavior of n-Type Si(111) Electrodes Coated With a Single Layer of Graphene Adam C. Nielander, Matthew J. Bierman, Nicholas Petrone, Nicholas C. Strandwitz, Shane Ardo, Fan Yang, James Hone, and Nathan S. Lewis pp 17246–17249 DOI: 10.1021/ja407462g Supporting Info |
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A Dark-Field Scattering Spectroelectrochemical Technique for Tracking the Electrodeposition of Single Silver Nanoparticles Caleb M. Hill and Shanlin Pan pp 17250–17253 DOI: 10.1021/ja4075387 Supporting Info |
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pH Responsive Janus-like Supramolecular Fusion Proteins for Functional Protein Delivery Seah Ling Kuan, David Y. W. Ng, Yuzhou Wu, Christina Förtsch, Holger Barth, Mikheil Doroshenko, Kaloian Koynov, Christoph Meier, and Tanja Weil pp 17254–17257 DOI: 10.1021/ja4084122 Supporting Info |
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Base Metal Catalysts for Photochemical C–H Borylation That Utilize Metal–Metal Cooperativity Thomas J. Mazzacano and Neal P. Mankad pp 17258–17261 DOI: 10.1021/ja408861p Supporting Info |
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Electron Transfer from Hexameric Copper Hydrides Michael S. Eberhart, Jack R. Norton, Ashley Zuzek, Wesley Sattler, and Serge Ruccolo pp 17262–17265 DOI: 10.1021/ja408925m Supporting Info |
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Vicinal Bisheterocyclizations of Alkynes via Nucleophilic Interception of a Catalytic Platinum Carbene Paul A. Allegretti and Eric M. Ferreira pp 17266–17269 DOI: 10.1021/ja408957a Supporting Info |
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Methoxy-Directed Aryl-to-Aryl 1,3-Rhodium Migration Jing Zhang, Jun-Feng Liu, Angel Ugrinov, Anthony F. X. Pillai, Zhong-Ming Sun, and Pinjing Zhao pp 17270–17273 DOI: 10.1021/ja409049t Supporting Info |
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Calculations on Tunneling in the Reactions of Noradamantyl Carbenes Sebastian Kozuch, Xue Zhang, David A. Hrovat, and Weston Thatcher Borden pp 17274–17277 DOI: 10.1021/ja409176u Supporting Info |
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Different Rates of Singlet Fission in Monoclinic versus Orthorhombic Crystal Forms of Diphenylhexatriene Robert J. Dillon, Geoffrey B. Piland, and Christopher J. Bardeen pp 17278–17281 DOI: 10.1021/ja409266s Supporting Info |
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C(sp3)–H Bond Hydroxylation Catalyzed by Myoglobin Reconstituted with Manganese Porphycene Koji Oohora, Yushi Kihira, Eiichi Mizohata, Tsuyoshi Inoue, and Takashi Hayashi pp 17282–17285 DOI: 10.1021/ja409404k Supporting Info |
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Electron-Deficient Triarylborane Block Copolymers: Synthesis by Controlled Free Radical Polymerization and Application in the Detection of Fluoride Ions Fei Cheng, Edward M. Bonder, and Frieder Jäkle pp 17286–17289 DOI: 10.1021/ja409525j Supporting Info |
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Seeing through Bone with Surface-Enhanced Spatially Offset Raman Spectroscopy Bhavya Sharma, Ke Ma, Matthew R. Glucksberg, and Richard P. Van Duyne pp 17290–17293 DOI: 10.1021/ja409378f Supporting Info |
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Lipid Directed Intrinsic Membrane Protein Segregation Jesper S. Hansen, James R. Thompson, Claus Hélix-Nielsen, and Noah Malmstadt pp 17294–17297 DOI: 10.1021/ja409708e Supporting Info |
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Enantio-, Diastereo-, and Regioselective Iridium-Catalyzed Asymmetric Allylic Alkylation of Acyclic β-Ketoesters Wen-Bo Liu, Corey M. Reeves, and Brian M. Stoltz pp 17298–17301 DOI: 10.1021/ja4097829 Supporting Info |
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Copper-Catalyzed gem-Difluoroolefination of Diazo Compounds with TMSCF3 via C–F Bond Cleavage Mingyou Hu, Zhengbiao He, Bing Gao, Lingchun Li, Chuanfa Ni, and Jinbo Hu pp 17302–17305 DOI: 10.1021/ja409941r Supporting Info |
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RuII-Catalyzed Vinylative Dearomatization of Naphthols via a C(sp2)–H Bond Activation Approach Jiang Nan, Zhijun Zuo, Lei Luo, Lu Bai, Huayu Zheng, Yini Yuan, Jingjing Liu, Xinjun Luan, and Yaoyu Wang pp 17306–17309 DOI: 10.1021/ja410060e Supporting Info |
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An Azine-Linked Covalent Organic Framework Sasanka Dalapati, Shangbin Jin, Jia Gao, Yanhong Xu, Atsushi Nagai, and Donglin Jiang pp 17310–17313 DOI: 10.1021/ja4103293 Supporting Info |
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Acylgermanes: Photoinitiators and Sources for Ge-Centered Radicals. Insights into their Reactivity Dmytro Neshchadin, Arnulf Rosspeintner, Markus Griesser, Bernhard Lang, Sandra Mosquera-Vazquez, Eric Vauthey, Vitaly Gorelik, Robert Liska, Christian Hametner, Beate Ganster, Robert Saf, Norbert Moszner, and Georg Gescheidt pp 17314–17321 DOI: 10.1021/ja404433u Supporting Info |
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Conditional Dicer Substrate Formation via Shape and Sequence Transduction with Small Conditional RNAs Lisa M. Hochrein, Maayan Schwarzkopf, Mona Shahgholi, Peng Yin, and Niles A. Pierce pp 17322–17330 DOI: 10.1021/ja404676x Supporting Info |
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Atomic Structure and Special Reactivity Toward Methanol Oxidation of Vanadia Nanoclusters on TiO2(110) Luca Artiglia, Stefano Agnoli, Andrea Vittadini, Alberto Verdini, Albano Cossaro, Luca Floreano, and Gaetano Granozzi pp 17331–17338 DOI: 10.1021/ja404889v Supporting Info |
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Counting the Number of Magnesium Ions Bound to the Surface-Immobilized Thymine Oligonucleotides That Comprise Spherical Nucleic Acids Stephanie R. Walter, Kaylie L. Young, Joseph G. Holland, Richard L. Gieseck, Chad A. Mirkin, and Franz M. Geiger pp 17339–17348 DOI: 10.1021/ja406551k Supporting Info |
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Modular Mesoionics: Understanding and Controlling Regioselectivity in 1,3-Dipolar Cycloadditions of Münchnone Derivatives Marie S. T. Morin, Daniel J. St-Cyr, Bruce A. Arndtsen, Elizabeth H. Krenske, and K. N. Houk pp 17349–17358 DOI: 10.1021/ja406833q Supporting Info |
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Revealing the Binding Structure of the Protein Corona on Gold Nanorods Using Synchrotron Radiation-Based Techniques: Understanding the Reduced Damage in Cell Membranes Liming Wang, Jingyuan Li, Jun Pan, Xiumei Jiang, Yinglu Ji, Yufeng Li, Ying Qu, Yuliang Zhao, Xiaochun Wu, and Chunying Chen pp 17359–17368 DOI: 10.1021/ja406924v Supporting Info |
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New Roles for Icosahedral Clusters in Intermetallic Phases: Micelle-like Segregation of Ca–Cd and Cu–Cd Interactions in Ca10Cd27Cu2 Amelia B. Hadler, Nicholas A. Harris, and Daniel C. Fredrickson pp 17369–17378 DOI: 10.1021/ja407291t Supporting Info |
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Is Dipole Moment a Valid Descriptor of Excited State’s Charge-Transfer Character? Piotr Petelenz and Barbara Pac pp 17379–17386 DOI: 10.1021/ja407379h |
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Enhancement of SERS Background through Charge Transfer Resonances on Single Crystal Gold Surfaces of Various Orientations Katsuyoshi Ikeda, Shuto Suzuki, and Kohei Uosaki pp 17387–17392 DOI: 10.1021/ja407459t Supporting Info |
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Tandem Isomerization/Hydroformylation/Hydrogenation of Internal Alkenes to n-Alcohols Using Rh/Ru Dual- or Ternary-Catalyst Systems Yamato Yuki, Kohei Takahashi, Yoshiyuki Tanaka, and Kyoko Nozaki pp 17393–17400 DOI: 10.1021/ja407523j Supporting Info |
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From 1D Chain to 3D Network: A New Family of Inorganic–Organic Hybrid Semiconductors MO3(L)x (M = Mo, W; L = Organic Linker) Built on Perovskite-like Structure Modules Xiao Zhang, Mehdi Hejazi, Suraj J. Thiagarajan, William R. Woerner, Debasis Banerjee, Thomas J. Emge, Wenqian Xu, Simon J. Teat, Qihan Gong, Ahmad Safari, Ronggui Yang, John B. Parise, and Jing Li pp 17401–17407 DOI: 10.1021/ja4077556 Supporting Info |
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Synthetic Remodeling of the Chartreusin Pathway to Tune Antiproliferative and Antibacterial Activities Nico Ueberschaar, Zhongli Xu, Kirstin Scherlach, Mikko Metsä-Ketelä, Tom Bretschneider, Hans-Martin Dahse, Helmar Görls, and Christian Hertweck pp 17408–17416 DOI: 10.1021/ja4080024 Supporting Info |
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L-Edge X-ray Absorption Spectroscopy and DFT Calculations on Cu2O2 Species: Direct Electrophilic Aromatic Attack by Side-on Peroxo Bridged Dicopper(II) Complexes Munzarin F. Qayyum, Ritimukta Sarangi, Kiyoshi Fujisawa, T. Daniel P. Stack, Kenneth D. Karlin, Keith O. Hodgson, Britt Hedman, and Edward I. Solomon pp 17417–17431 DOI: 10.1021/ja4078717 Supporting Info |
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Substrate Distortion Contributes to the Catalysis of Orotidine 5′-Monophosphate Decarboxylase Masahiro Fujihashi, Toyokazu Ishida, Shingo Kuroda, Lakshmi P. Kotra, Emil F. Pai, and Kunio Miki pp 17432–17443 DOI: 10.1021/ja408197k Supporting Info |
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Remarkable Behavior of a Bifunctional Alkynylborane Zirconocene Complex toward Donor Ligands and Acetylenes Santhosh Kumar Podiyanachari, Gerald Kehr, Christian Mück-Lichtenfeld, Constantin G. Daniliuc, and Gerhard Erker pp 17444–17456 DOI: 10.1021/ja408385h Supporting Info |
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Redox-Induced Ion Pairing of Anionic Surfactants with Ferrocene-Terminated Self-Assembled Monolayers: Faradaic Electrochemistry and Surfactant Aggregation at the Monolayer/Liquid Interface Eric R. Dionne, Tania Sultana, Lana L. Norman, Violeta Toader, and Antonella Badia pp 17457–17468 DOI: 10.1021/ja408512q Supporting Info |
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Fluorescence Discrimination of Cancer from Inflammation by Molecular Response to COX-2 Enzymes Hua Zhang, Jiangli Fan, Jingyun Wang, Bairui Dou, Fan Zhou, Jianfang Cao, Junle Qu, Zhi Cao, Weijie Zhao, and Xiaojun Peng pp 17469–17475 DOI: 10.1021/ja4085308 Supporting Info |
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Toroidal Structure and DNA Cleavage by the CRISPR-Associated [4Fe-4S] Cluster Containing Cas4 Nuclease SSO0001 from Sulfolobus solfataricus Sofia Lemak, Natalia Beloglazova, Boguslaw Nocek, Tatiana Skarina, Robert Flick, Greg Brown, Ana Popovic, Andrzej Joachimiak, Alexei Savchenko, and Alexander F. Yakunin pp 17476–17487 DOI: 10.1021/ja408729b Supporting Info |
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Selective Chromium(VI) Ligands Identified Using Combinatorial Peptoid Libraries Abigail S. Knight, Effie Y. Zhou, Jeffrey G. Pelton, and Matthew B. Francis pp 17488–17493 DOI: 10.1021/ja408788t Supporting Info |
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Visible Light-Promoted Metal-Free C–H Activation: Diarylketone-Catalyzed Selective Benzylic Mono- and Difluorination Ji-Bao Xia, Chen Zhu, and Chuo Chen pp 17494–17500 DOI: 10.1021/ja410815u Supporting Info |
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De Novo Determination of the Crystal Structure of a Large Drug Molecule by Crystal Structure Prediction-Based Powder NMR Crystallography Maria Baias, Jean-Nicolas Dumez, Per H. Svensson, Staffan Schantz, Graeme M. Day, and Lyndon Emsley pp 17501–17507 DOI: 10.1021/ja4088874 Supporting Info |
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Ligand-Accelerated ortho-C–H Alkylation of Arylcarboxylic Acids using Alkyl Boron Reagents Peter S. Thuy-Boun, Giorgio Villa, Devin Dang, Paul Richardson, Shun Su, and Jin-Quan Yu pp 17508–17513 DOI: 10.1021/ja409014v Supporting Info |
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[Cp2TiCH2CHMe(SiMe3)]+, an Alkyl–Titanium Complex Which (a) Exists in Equilibrium between a β-Agostic and a Lower Energy γ-Agostic Isomer and (b) Undergoes Hydrogen Atom Exchange between α-, β-, and γ-Sites via a Combination of Conventional β-Hydrogen Elimination–Reinsertion and a Nonconventional CH Bond Activation Process Which Involves Proton Tunnelling Alexandre F. Dunlop-Brière and Michael C. Baird , Peter H. M. Budzelaar pp 17514–17527 DOI: 10.1021/ja4092775 Supporting Info |
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Dynamics of Excess Electronic Charge in Aliphatic Ionic Liquids Containing the Bis(trifluoromethylsulfonyl)amide Anion Changhui Xu, Aleksander Durumeric, Hemant K. Kashyap, Jorge Kohanoff, and Claudio J. Margulis pp 17528–17536 DOI: 10.1021/ja409338z Supporting Info |
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Experimental Analysis of the Catalytic Cycle of the Borane-Promoted Imine Reduction with Hydrosilanes: Spectroscopic Detection of Unexpected Intermediates and a Refined Mechanism Julia Hermeke, Marius Mewald, and Martin Oestreich pp 17537–17546 DOI: 10.1021/ja409344w Supporting Info |
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Universal Binding Behavior for Ionic Alkyl Surfactants with Oppositely Charged Polyelectrolytes Dongcui Li and Norman J. Wagner pp 17547–17555 DOI: 10.1021/ja408587u Supporting Info |
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Synthesis, Characterization and Reactivity of Group 4 Metallocene Bis(diphenylphosphino)acetylene Complexes—A Reactivity and Bonding Study Martin Haehnel, Sven Hansen, Kathleen Schubert, Perdita Arndt, Anke Spannenberg, Haijun Jiao, and Uwe Rosenthal pp 17556–17565 DOI: 10.1021/ja409320k Supporting Info |
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Toward Organometallic 99mTc Imaging Agents: Synthesis of Water-Stable 99Tc–NHC Complexes Michael Benz, Bernhard Spingler, Roger Alberto, and Henrik Braband pp 17566–17572 DOI: 10.1021/ja409499u Supporting Info |
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Geometric and Electronic Structure of the Mn(IV)Fe(III) Cofactor in Class Ic Ribonucleotide Reductase: Correlation to the Class Ia Binuclear Non-Heme Iron Enzyme Yeonju Kwak, Wei Jiang, Laura M. K. Dassama, Kiyoung Park, Caleb B. Bell, III, Lei V. Liu, Shaun D. Wong, Makina Saito, Yasuhiro Kobayashi, Shinji Kitao, Makoto Seto, Yoshitaka Yoda, E. Ercan Alp, Jiyong Zhao, J. Martin Bollinger, Jr., Carsten Krebs, and Edward I. Solomon pp 17573–17584 DOI: 10.1021/ja409510d Supporting Info |
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Computation and Experiment Reveal That the Ring-Rearrangement Metathesis of Himbert Cycloadducts Can Be Subject to Kinetic or Thermodynamic Control Jonathan K. Lam, Hung V. Pham, K. N. Houk, and Christopher D. Vanderwal pp 17585–17594 DOI: 10.1021/ja409618p Supporting Info |
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Surface-Induced Alkene Oligomerization: Does Thermal Hydrosilylation Really Lead to Monolayer Protected Silicon Nanocrystals? Zhenyu Yang, Muhammad Iqbal, Alexander R. Dobbie, and Jonathan G. C. Veinot pp 17595–17601 DOI: 10.1021/ja409657y Supporting Info |
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Raising the pKa Limit of “Soft” Nucleophiles in Palladium-Catalyzed Allylic Substitutions: Application of Diarylmethane Pronucleophiles Sheng-Chun Sha, Jiadi Zhang, Patrick J. Carroll, and Patrick J. Walsh pp 17602–17609 DOI: 10.1021/ja409511n Supporting Info |
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Direct Arylations for Study of the Air-Stable P-Heterocyclic Biradical: From Wide Electronic Tuning to Characterization of the Localized Radicalic Electrons Shigekazu Ito, Yasuhiro Ueta, Trang Thi Thu Ngo, Makoto Kobayashi, Daisuke Hashizume, Jun-ichi Nishida, Yoshiro Yamashita, and Koichi Mikami pp 17610–17616 DOI: 10.1021/ja409625x Supporting Info |
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Polyprodrug Amphiphiles: Hierarchical Assemblies for Shape-Regulated Cellular Internalization, Trafficking, and Drug Delivery Xianglong Hu, Jinming Hu, Jie Tian, Zhishen Ge, Guoying Zhang, Kaifu Luo, and Shiyong Liu pp 17617–17629 DOI: 10.1021/ja409686x Supporting Info |
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Copper Sulfide Nanocrystals with Tunable Composition by Reduction of Covellite Nanocrystals with Cu+ Ions Yi Xie, Andreas Riedinger, Mirko Prato, Alberto Casu, Alessandro Genovese, Pablo Guardia, Silvia Sottini, Claudio Sangregorio, Karol Miszta, Sandeep Ghosh, Teresa Pellegrino, and Liberato Manna pp 17630–17637 DOI: 10.1021/ja409754v Supporting Info |
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Does Nature Click? Theoretical Prediction of an Enzyme-Catalyzed Transannular 1,3-Dipolar Cycloaddition in the Biosynthesis of Lycojaponicumins A and B Elizabeth H. Krenske, Ashay Patel, and K. N. Houk pp 17638–17642 DOI: 10.1021/ja409928z Supporting Info |
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Diels–Alder Reactions of Graphene: Computational Predictions of Products and Sites of Reaction Yang Cao, Sílvia Osuna, Yong Liang, Robert C. Haddon, and K. N. Houk pp 17643–17649 DOI: 10.1021/ja410225u Supporting Info |
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Correction to “Enthalpic Signature of Methonium Desolvation Revealed in a Synthetic Host–Guest System Based on Cucurbit[7]uril” Yi Wang, Jason R. King, Pan Wu, Daniel L. Pelzman, David N. Beratan, and Eric J. Toone pp 17650–17650 DOI: 10.1021/ja408346j |
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Retraction of “Bimetallic Effects for Enhanced Polar Comonomer Enchainment Selectivity in Catalytic Ethylene Polymerization” Brandon A. Rodriguez, Massimiliano Delferro, and Tobin J. Marks pp 17651–17651 DOI: 10.1021/ja409590r |
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Correction to “Activation of Snap-Top Capped Mesoporous Silica Nanocontainers Using Two Near-Infrared Photons” Tania M. Guardado-Alvarez, Lekshmi Sudha Devi, Melissa M. Russell, Benjamin J. Schwartz, and Jeffrey I. Zink pp 17652–17652 DOI: 10.1021/ja410105b |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 17653–17654 DOI: 10.1021/ja411794s |
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Acid-Degradable Polymer-Caged Lipoplex (PCL) Platform for siRNA Delivery: Facile Cellular Triggered Release of siRNA Bong Jin Hong, Anthony J. Chipre, and SonBinh T. Nguyen pp 17655–17658 DOI: 10.1021/ja404491r Supporting Info |
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An Enzymatic Chemical Amplifier Based on Mechanized Nanoparticles Min Xue and Jeffrey I. Zink pp 17659–17662 DOI: 10.1021/ja4066317 Supporting Info |
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Fast Hydrazone Reactants: Electronic and Acid/Base Effects Strongly Influence Rate at Biological pH Eric T. Kool, Do-Hyoung Park, and Pete Crisalli pp 17663–17666 DOI: 10.1021/ja407407h Supporting Info |
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In Situ Assembled Boronate Ester Assisted Chiral Carboxylic Acid Catalyzed Asymmetric Trans-Aziridinations Takuya Hashimoto, Alberto Osuna Gálvez, and Keiji Maruoka pp 17667–17670 DOI: 10.1021/ja407764u Supporting Info |
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Electrochemistry of Acids on Platinum. Application to the Reduction of Carbon Dioxide in the Presence of Pyridinium Ion in Water Cyrille Costentin, Juan Carlos Canales, Baptiste Haddou, and Jean-Michel Savéant pp 17671–17674 DOI: 10.1021/ja407988w Supporting Info |
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Facile and Efficient Preparation of Anisotropic DNA-Functionalized Gold Nanoparticles and Their Regioselective Assembly Li Huey Tan, Hang Xing, Hongyu Chen, and Yi Lu pp 17675–17678 DOI: 10.1021/ja408033e Supporting Info |
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Bio-Inspired Polydopamine: A Versatile and Powerful Platform for Covalent Synthesis of Molecular Sieve Membranes Qian Liu, Nanyi Wang, Jürgen Caro, and Aisheng Huang pp 17679–17682 DOI: 10.1021/ja4080562 Supporting Info |
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A Red-Shifted, Fast-Relaxing Azobenzene Photoswitch for Visible Light Control of an Ionotropic Glutamate Receptor Michael A. Kienzler, Andreas Reiner, Eric Trautman, Stan Yoo, Dirk Trauner, and Ehud Y. Isacoff pp 17683–17686 DOI: 10.1021/ja408104w Supporting Info |
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Tunable Asymmetric Catalysis through Ligand Stacking in Chiral Rigid Rods Matthieu Raynal, François Portier, Piet W. N. M. van Leeuwen, and Laurent Bouteiller pp 17687–17690 DOI: 10.1021/ja408860s Supporting Info |
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A Water-Soluble pH-Triggered Molecular Switch Sergio Grunder, Psaras L. McGrier, Adam C. Whalley, Megan M. Boyle, Charlotte Stern, and J. Fraser Stoddart pp 17691–17694 DOI: 10.1021/ja409006y Supporting Info |
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Nanostar and Nanonetwork Crystals Fabricated by in Situ Nanoparticlization of Fully Conjugated Polythiophene Diblock Copolymers In-Hwan Lee, Pitchamuthu Amaladass, Ki-Young Yoon, Suyong Shin, Yong-Jae Kim, Inhye Kim, Eunji Lee, and Tae-Lim Choi pp 17695–17698 DOI: 10.1021/ja409206p Supporting Info |
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Electrodeposited Cobalt-Sulfide Catalyst for Electrochemical and Photoelectrochemical Hydrogen Generation from Water Yujie Sun, Chong Liu, David C. Grauer, Junko Yano, Jeffrey R. Long, Peidong Yang, and Christopher J. Chang pp 17699–17702 DOI: 10.1021/ja4094764 Supporting Info |
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Water-Soluble Cationic Conjugated Polymers: Response to Electron-Rich Bioanalytes Sébastien Rochat and Timothy M. Swager pp 17703–17706 DOI: 10.1021/ja4095395 Supporting Info |
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Transforming Suzuki–Miyaura Cross-Couplings of MIDA Boronates into a Green Technology: No Organic Solvents Nicholas A. Isley, Fabrice Gallou, and Bruce H. Lipshutz pp 17707–17710 DOI: 10.1021/ja409663q Supporting Info |
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Relaxometry Studies of a Highly Stable Nanoscale Metal–Organic Framework Made of Cu(II), Gd(III), and the Macrocyclic DOTP Arnau Carné-Sánchez, Célia S. Bonnet, Inhar Imaz, Julia Lorenzo, Éva Tóth, and Daniel Maspoch pp 17711–17714 DOI: 10.1021/ja4094378 Supporting Info |
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Carrier Concentration Dependent Conduction in Insulator-Doped Donor/Acceptor Chain Compounds Masaki Nishio, Norihisa Hoshino, Wataru Kosaka, Tomoyuki Akutagawa, and Hitoshi Miyasaka pp 17715–17718 DOI: 10.1021/ja409785a Supporting Info |
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Synthesis and Reactivity of a Transient, Terminal Nitrido Complex of Rhodium Markus G. Scheibel, Yanlin Wu, A. Claudia Stückl, Lennard Krause, Elena Carl, Dietmar Stalke, Bas de Bruin, and Sven Schneider pp 17719–17722 DOI: 10.1021/ja409764j Supporting Info |
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Cooperative Thermodynamic Control of Selectivity in the Self-Assembly of Rare Earth Metal–Ligand Helices Amber M. Johnson, Michael C. Young, Xing Zhang, Ryan R. Julian, and Richard J. Hooley pp 17723–17726 DOI: 10.1021/ja409882k Supporting Info |
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Multistep DNA-Templated Synthesis Using a Universal Template Yizhou Li, Peng Zhao, Mingda Zhang, Xianyuan Zhao, and Xiaoyu Li pp 17727–17730 DOI: 10.1021/ja409936r Supporting Info |
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Programmed Pore Architectures in Modular Quaternary Metal–Organic Frameworks Lujia Liu, Kristina Konstas, Matthew R. Hill, and Shane G. Telfer pp 17731–17734 DOI: 10.1021/ja4100244 Supporting Info |
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Enantioselective Photoredox Catalysis Enabled by Proton-Coupled Electron Transfer: Development of an Asymmetric Aza-Pinacol Cyclization Lydia J. Rono, Hatice G. Yayla, David Y. Wang, Michael F. Armstrong, and Robert R. Knowles pp 17735–17738 DOI: 10.1021/ja4100595 Supporting Info |
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Branched Cylindrical Micelles via Crystallization-Driven Self-Assembly Huibin Qiu, Van An Du, Mitchell A. Winnik, and Ian Manners pp 17739–17742 DOI: 10.1021/ja410176n Supporting Info |
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From 3-Fold Completive Self-Sorting of a Nine-Component Library to a Seven-Component Scalene Quadrilateral Manik Lal Saha and Michael Schmittel pp 17743–17746 DOI: 10.1021/ja410425k Supporting Info |
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Catalytic Direct β-Arylation of Simple Ketones with Aryl Iodides Zhongxing Huang and Guangbin Dong pp 17747–17750 DOI: 10.1021/ja410389a Supporting Info |
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Polydiacetylene-Based Colorimetric and Fluorescent Chemosensor for the Detection of Carbon Dioxide Qingling Xu, Songyi Lee, Yukyung Cho, Myung Hwa Kim, Jean Bouffard, and Juyoung Yoon pp 17751–17754 DOI: 10.1021/ja410557x Supporting Info |
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Iron-Catalyzed Ortho-Allylation of Aromatic Carboxamides with Allyl Ethers Sobi Asako, Laurean Ilies, and Eiichi Nakamura pp 17755–17757 DOI: 10.1021/ja4106368 Supporting Info |
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Interactive Forces between Sodium Dodecyl Sulfate-Suspended Single-Walled Carbon Nanotubes and Agarose Gels Justin G. Clar, Carlos A. Silvera Batista, Sejin Youn, Jean-Claude J. Bonzongo, and Kirk J. Ziegler pp 17758–17767 DOI: 10.1021/ja4052526 Supporting Info |
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A New Synthetic Pathway to the Second and Third Generation of Superbasic Bisphosphazene Proton Sponges: The Run for the Best Chelating Ligand for a Proton Julius F. Kögel, Benjamin Oelkers, Borislav Kovačević, and Jörg Sundermeyer pp 17768–17774 DOI: 10.1021/ja409760z Supporting Info |
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13C and 63,65Cu ENDOR studies of CO Dehydrogenase from Oligotropha carboxidovorans. Experimental Evidence in Support of a Copper–Carbonyl Intermediate Muralidharan Shanmugam, Jarett Wilcoxen, Diana Habel-Rodriguez, George E. Cutsail III, Martin L. Kirk, Brian M. Hoffman, and Russ Hille pp 17775–17782 DOI: 10.1021/ja406136f Supporting Info |
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Single Molecule Force Spectroscopy Reveals the Molecular Mechanical Anisotropy of the FeS4 Metal Center in Rubredoxin Peng Zheng, Chih-Chung Chou, Ying Guo, Yanyan Wang, and Hongbin Li pp 17783–17792 DOI: 10.1021/ja406695g Supporting Info |
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Magic Angle Spinning NMR Reveals Sequence-Dependent Structural Plasticity, Dynamics, and the Spacer Peptide 1 Conformation in HIV-1 Capsid Protein Assemblies Yun Han, Guangjin Hou, Christopher L. Suiter, Jinwoo Ahn, In-Ja L. Byeon, Andrew S. Lipton, Sarah Burton, Ivan Hung, Peter L. Gor′kov, Zhehong Gan, William Brey, David Rice, Angela M. Gronenborn, and Tatyana Polenova pp 17793–17803 DOI: 10.1021/ja406907h Supporting Info |
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Contributions of the S100A9 C-Terminal Tail to High-Affinity Mn(II) Chelation by the Host-Defense Protein Human Calprotectin Megan Brunjes Brophy, Toshiki G. Nakashige, Aleth Gaillard, and Elizabeth M. Nolan pp 17804–17817 DOI: 10.1021/ja407147d Supporting Info |
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Molecular Dynamics Simulations of Gas Selectivity in Amorphous Porous Molecular Solids Shan Jiang, Kim E. Jelfs, Daniel Holden, Tom Hasell, Samantha Y. Chong, Maciej Haranczyk, Abbie Trewin, and Andrew I. Cooper pp 17818–17830 DOI: 10.1021/ja407374k Supporting Info |
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Core-Shell Nanostructured “Black” Rutile Titania as Excellent Catalyst for Hydrogen Production Enhanced by Sulfur Doping Chongyin Yang, Zhou Wang, Tianquan Lin, Hao Yin, Xujie Lü, Dongyun Wan, Tao Xu, Chong Zheng, Jianhua Lin, Fuqiang Huang, Xiaoming Xie, and Mianheng Jiang pp 17831–17838 DOI: 10.1021/ja4076748 Supporting Info |
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Hemichelation, a Way To Stabilize Electron-Unsaturated Complexes: The Case of T-Shaped Pd and Pt Metallacycles. Christophe Werlé, Corinne Bailly, Lydia Karmazin-Brelot, Xavier-Frédéric Le Goff, Louis Ricard, and Jean-Pierre Djukic pp 17839–17852 DOI: 10.1021/ja4076327 Supporting Info |
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Chemically Stable Multilayered Covalent Organic Nanosheets from Covalent Organic Frameworks via Mechanical Delamination Suman Chandra, Sharath Kandambeth, Bishnu P. Biswal, Binit Lukose, Shrikant M. Kunjir, Minakshi Chaudhary, Ravichandar Babarao, Thomas Heine, and Rahul Banerjee pp 17853–17861 DOI: 10.1021/ja408121p Supporting Info |
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Loop Interactions and Dynamics Tune the Enzymatic Activity of the Human Histone Deacetylase 8 Micha B. A. Kunze, David W. Wright, Nicolas D. Werbeck, John Kirkpatrick, Peter V. Coveney, and D. Flemming Hansen pp 17862–17868 DOI: 10.1021/ja408184x Supporting Info |
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Stilbene Vinyl Sulfonamides as Fluorogenic Sensors of and Traceless Covalent Kinetic Stabilizers of Transthyretin That Prevent Amyloidogenesis Eul Hyun Suh, Yu Liu, Stephen Connelly, Joseph C. Genereux, Ian A. Wilson, and Jeffery W. Kelly pp 17869–17880 DOI: 10.1021/ja408230k Supporting Info |
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Controllable Disorder Engineering in Oxygen-Incorporated MoS2 Ultrathin Nanosheets for Efficient Hydrogen Evolution Junfeng Xie, Jiajia Zhang, Shuang Li, Fabian Grote, Xiaodong Zhang, Hao Zhang, Ruoxing Wang, Yong Lei, Bicai Pan, and Yi Xie pp 17881–17888 DOI: 10.1021/ja408329q Supporting Info |
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Solubilizing the Most Easily Ionized Molecules and Generating Powerful Reducing Agents Gina M. Chiarella, F. Albert Cotton, Jason C. Durivage, Dennis L. Lichtenberger, and Carlos A. Murillo pp 17889–17896 DOI: 10.1021/ja408291k Supporting Info |
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Catalytic Production of Hydrogen Peroxide and Water by Oxygen-Tolerant [NiFe]-Hydrogenase during H2 Cycling in the Presence of O2 Lars Lauterbach and Oliver Lenz pp 17897–17905 DOI: 10.1021/ja408420d Supporting Info |
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Discovery and Synthetic Refactoring of Tryptophan Dimer Gene Clusters from the Environment Fang-Yuan Chang, Melinda A. Ternei, Paula Y. Calle, and Sean F. Brady pp 17906–17912 DOI: 10.1021/ja408683p Supporting Info |
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Toward a Single-Layer Two-Dimensional Honeycomb Supramolecular Organic Framework in Water Kang-Da Zhang, Jia Tian, David Hanifi, Yuebiao Zhang, Andrew Chi-Hau Sue, Tian-You Zhou, Lei Zhang, Xin Zhao, Yi Liu, and Zhan-Ting Li pp 17913–17918 DOI: 10.1021/ja4086935 Supporting Info |
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Hydrogen-Bond Networks: Strengths of Different Types of Hydrogen Bonds and An Alternative to the Low Barrier Hydrogen-Bond Proposal Alireza Shokri, Yanping Wang, George A. O’Doherty, Xue-Bin Wang, and Steven R. Kass pp 17919–17924 DOI: 10.1021/ja408762r Supporting Info |
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Organocatalytic Conjugate-Addition Polymerization of Linear and Cyclic Acrylic Monomers by N-Heterocyclic Carbenes: Mechanisms of Chain Initiation, Propagation, and Termination Yuetao Zhang, Meghan Schmitt, Laura Falivene, Lucia Caporaso, Luigi Cavallo, and Eugene Y.-X. Chen pp 17925–17942 DOI: 10.1021/ja4088677 Supporting Info |
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Bipodal Surface Organometallic Complexes with Surface N-Donor Ligands and Application to the Catalytic Cleavage of C–H and C–C Bonds in n-Butane Anissa Bendjeriou-Sedjerari, Joachim M. Azzi, Edy Abou-Hamad, Dalaver H. Anjum, Fahran A. Pasha, Kuo-Wei Huang, Lyndon Emsley, and Jean-Marie Basset pp 17943–17951 DOI: 10.1021/ja407902g Supporting Info |
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Magnetic Blocking at 10 K and a Dipolar-Mediated Avalanche in Salts of the Bis(η8-cyclooctatetraenide) Complex [Er(COT)2]− Katie R. Meihaus and Jeffrey R. Long pp 17952–17957 DOI: 10.1021/ja4094814 Supporting Info |
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From a Zwitterionic Phosphasilene to Base Stabilized Silyliumylidene-Phosphide and Bis(silylene) Complexes Nora C. Breit, Tibor Szilvási, Tsuyoshi Suzuki, Daniel Gallego, and Shigeyoshi Inoue pp 17958–17968 DOI: 10.1021/ja409720c Supporting Info |
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Benzimidazole-Based Ratiometric Two-Photon Fluorescent Probes for Acidic pH in Live Cells and Tissues Hyung Joong Kim, Cheol Ho Heo, and Hwan Myung Kim pp 17969–17977 DOI: 10.1021/ja409971k Supporting Info |
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Tandem Dienone Photorearrangement–Cycloaddition for the Rapid Generation of Molecular Complexity Pieter H. Bos, Mitchell T. Antalek, John A. Porco, Jr., and Corey R. J. Stephenson pp 17978–17982 DOI: 10.1021/ja409992m Supporting Info |
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Enantioselective Functionalization of Allylic C–H Bonds Following a Strategy of Functionalization and Diversification Ankit Sharma and John F. Hartwig pp 17983–17989 DOI: 10.1021/ja409995w Supporting Info |
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Asymmetric Synthesis of the Aminocyclitol Pactamycin, a Universal Translocation Inhibitor Robert J. Sharpe, Justin T. Malinowski, and Jeffrey S. Johnson pp 17990–17998 DOI: 10.1021/ja409944u Supporting Info |
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High-Fidelity Stereochemical Memory in a FeII4L4 Tetrahedral Capsule Ana M. Castilla, Naoki Ousaka, Rana A. Bilbeisi, Elisa Valeri, Tanya K. Ronson, and Jonathan R. Nitschke pp 17999–18006 DOI: 10.1021/ja410117q Supporting Info |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 18007–18007 DOI: 10.1021/ja411877u |
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Light-Emitting Electrochemical Cells Using Cyanine Dyes as the Active Components Antonio Pertegás, Daniel Tordera, Juan J. Serrano-Pérez, Enrique Ortí, and Henk J. Bolink pp 18008–18011 DOI: 10.1021/ja407515w Supporting Info |
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A 18F-Labeled Saxitoxin Derivative for in Vivo PET-MR Imaging of Voltage-Gated Sodium Channel Expression Following Nerve Injury Aileen Hoehne, Deepak Behera, William H. Parsons, Michelle L. James, Bin Shen, Preeti Borgohain, Deepika Bodapati, Archana Prabhakar, Sanjiv S. Gambhir, David C. Yeomans, Sandip Biswal, Frederick T. Chin, and J. Du Bois pp 18012–18015 DOI: 10.1021/ja408300e Supporting Info |
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Specific Binding of Modified RGG Domain in TLS/FUS to G-Quadruplex RNA: Tyrosines in RGG Domain Recognize 2′-OH of the Riboses of Loops in G-Quadruplex Kentaro Takahama and Takanori Oyoshi pp 18016–18019 DOI: 10.1021/ja4086929 Supporting Info |
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Organocatalytic Enantioselective Synthesis of 2,3-Allenoates by Intermolecular Addition of Nitroalkanes to Activated Enynes Hui Qian, Xiuzhao Yu, Junliang Zhang, and Jianwei Sun pp 18020–18023 DOI: 10.1021/ja409080v Supporting Info |
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Side Chain Dynamics of Carboxyl and Carbonyl Groups in the Catalytic Function of Escherichia coli Ribonuclease H Kate A. Stafford, Fabien Ferrage, Jae-Hyun Cho, and Arthur G. Palmer, III pp 18024–18027 DOI: 10.1021/ja409479y Supporting Info |
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A Transition Metal Carbonyl Probe for Use in a Highly Specific and Sensitive SERS-Based Assay for Glucose Kien Voon Kong, Zhiyong Lam, Weber Kam On Lau, Weng Kee Leong, and Malini Olivo pp 18028–18031 DOI: 10.1021/ja409230g Supporting Info |
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Flavin-Linked Oxidase Catalyzes Pyrrolizine Formation of Dichloropyrrole-Containing Polyketide Extender Unit in Chlorizidine A Simone M. Mantovani and Bradley S. Moore pp 18032–18035 DOI: 10.1021/ja409520v Supporting Info |
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Metal-Free Enantioselective Hydroxyamination of Aldehydes with Nitrosocarbonyl Compounds Catalyzed by an Axially Chiral Amine Taichi Kano, Fumitaka Shirozu, and Keiji Maruoka pp 18036–18039 DOI: 10.1021/ja4099627 Supporting Info |
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Dynamic Breathing of CO2 by Hydrotalcite Shinsuke Ishihara, Pathik Sahoo, Kenzo Deguchi, Shinobu Ohki, Masataka Tansho, Tadashi Shimizu, Jan Labuta, Jonathan P. Hill, Katsuhiko Ariga, Ken Watanabe, Yusuke Yamauchi, Shigeru Suehara, and Nobuo Iyi pp 18040–18043 DOI: 10.1021/ja4099752 Supporting Info |
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In Situ-Formed Li2S in Lithiated Graphite Electrodes for Lithium–Sulfur Batteries Yongzhu Fu, Chenxi Zu, and Arumugam Manthiram pp 18044–18047 DOI: 10.1021/ja409705u Supporting Info |
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Alkene Oxyalkylation Enabled by Merging Rhenium Catalysis with Hypervalent Iodine(III) Reagents via Decarboxylation Yin Wang, Lei Zhang, Yunhui Yang, Ping Zhang, Zhenting Du, and Congyang Wang pp 18048–18051 DOI: 10.1021/ja410195j Supporting Info |
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Chirality Sensing of Amines, Diamines, Amino Acids, Amino Alcohols, and α-Hydroxy Acids with a Single Probe Keith W. Bentley, Yea G. Nam, Jaslynn M. Murphy, and Christian Wolf pp 18052–18055 DOI: 10.1021/ja410428b Supporting Info |
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Cross-Coupling of Remote meta-C–H Bonds Directed by a U-Shaped Template Li Wan, Navid Dastbaravardeh, Gang Li, and Jin-Quan Yu pp 18056–18059 DOI: 10.1021/ja410760f Supporting Info |
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Weak Ferromagnetic Ordering of the Li+[TCNE]•– (TCNE = Tetracyanoethylene) Organic Magnet with an Interpenetrating Diamondoid Structure Jae-Hyuk Her, Peter W. Stephens, Royce A. Davidson, Kil Sik Min, Joshua D. Bagnato, Kipp van Schooten, Christoph Boehme, and Joel S. Miller pp 18060–18063 DOI: 10.1021/ja410818e Supporting Info |
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Hydrogen-Bonded Capsules in Water Kang-Da Zhang, Dariush Ajami, and Julius Rebek pp 18064–18066 DOI: 10.1021/ja410644p Supporting Info |
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Semiring Chemistry of Au25(SR)18: Fragmentation Pathway and Catalytic Active site Chunyan Liu, Sisi Lin, Yong Pei, and Xiao Cheng Zeng pp 18067–18079 DOI: 10.1021/ja404957t Supporting Info |
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Design Space for Complex DNA Structures Bryan Wei, Mingjie Dai, Cameron Myhrvold, Yonggang Ke, Ralf Jungmann, and Peng Yin pp 18080–18088 DOI: 10.1021/ja4062294 Supporting Info |
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Inhibition of Microtubule Assembly by a Complex of Actin and Antitumor Macrolide Aplyronine A Masaki Kita, Yuichiro Hirayama, Kozo Yoneda, Kota Yamagishi, Takumi Chinen, Takeo Usui, Eriko Sumiya, Motonari Uesugi, and Hideo Kigoshi pp 18089–18095 DOI: 10.1021/ja406580w Supporting Info |
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De Novo-Designed Metallopeptides with Type 2 Copper Centers: Modulation of Reduction Potentials and Nitrite Reductase Activities Fangting Yu, James E. Penner-Hahn, and Vincent L. Pecoraro pp 18096–18107 DOI: 10.1021/ja406648n Supporting Info |
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Bis-N-Heterocyclic Carbene (NHC) Stabilized η6-Arene Iron(0) Complexes: Synthesis, Structure, Reactivity, and Catalytic Activity Burgert Blom, Gengwen Tan, Stephan Enthaler, Shigeyoshi Inoue, Jan Dirk Epping, and Matthias Driess pp 18108–18120 DOI: 10.1021/ja410234x Supporting Info |
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Metal Oxide Nanoparticle Growth on Graphene via Chemical Activation with Atomic Oxygen James E. Johns, Justice M. P. Alaboson, Sameer Patwardhan, Christopher R. Ryder, George C. Schatz, and Mark C. Hersam pp 18121–18125 DOI: 10.1021/ja408248z Supporting Info |
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Tuning the Ferroelectric Polarization in a Multiferroic Metal–Organic Framework Domenico Di Sante, Alessandro Stroppa, Prashant Jain, and Silvia Picozzi pp 18126–18130 DOI: 10.1021/ja408283a Supporting Info |
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Defining the Value of Injection Current and Effective Electrical Contact Area for EGaIn-Based Molecular Tunneling Junctions Felice C. Simeone, Hyo Jae Yoon, Martin M. Thuo, Jabulani R. Barber, Barbara Smith, and George M. Whitesides pp 18131–18144 DOI: 10.1021/ja408652h Supporting Info |
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Nitric Oxide Releasing Materials Triggered by Near-Infrared Excitation Through Tissue Filters Peter T. Burks, John V. Garcia, Ricardo GonzalezIrias, Jason T. Tillman, Mutong Niu, Alexander A. Mikhailovsky, Jinping Zhang, Fan Zhang, and Peter C. Ford pp 18145–18152 DOI: 10.1021/ja408516w Supporting Info |
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Staurosporine-Derived Inhibitors Broaden the Scope of Analog-Sensitive Kinase Technology Michael S. Lopez, Jonathan W. Choy, Ulf Peters, Martin L. Sos, David O. Morgan, and Kevan M. Shokat pp 18153–18159 DOI: 10.1021/ja408704u Supporting Info |
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NMR Studies of Protonation and Hydrogen Bond States of Internal Aldimines of Pyridoxal 5′-Phosphate Acid–Base in Alanine Racemase, Aspartate Aminotransferase, and Poly-l-lysine Monique Chan-Huot, Alexandra Dos, Reinhard Zander, Shasad Sharif, Peter M. Tolstoy, Shara Compton, Emily Fogle, Michael D. Toney, Ilya Shenderovich, Gleb S. Denisov, and Hans-Heinrich Limbach pp 18160–18175 DOI: 10.1021/ja408988z Supporting Info |
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Nanowire Templated Semihollow Bicontinuous Graphene Scrolls: Designed Construction, Mechanism, and Enhanced Energy Storage Performance Mengyu Yan, Fengchao Wang, Chunhua Han, Xinyu Ma, Xu Xu, Qinyou An, Lin Xu, Chaojiang Niu, Yunlong Zhao, Xiaocong Tian, Ping Hu, Hengan Wu, and Liqiang Mai pp 18176–18182 DOI: 10.1021/ja409027s Supporting Info |
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Probing Adsorption Interactions in Metal–Organic Frameworks using X-ray Spectroscopy Walter S. Drisdell, Roberta Poloni, Thomas M. McDonald, Jeffrey R. Long, Berend Smit, Jeffrey B. Neaton, David Prendergast, and Jeffrey B. Kortright pp 18183–18190 DOI: 10.1021/ja408972f Supporting Info |
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Reconciliation of Chemical, Enzymatic, Spectroscopic and Computational Data To Assign the Absolute Configuration of the DNA Base Lesion Spiroiminodihydantoin Aaron M. Fleming, Anita M. Orendt, Yanan He, Judy Zhu, Rina K. Dukor, and Cynthia J. Burrows pp 18191–18204 DOI: 10.1021/ja409254z Supporting Info |
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High-Spin S = 2 Ground State Aminyl Tetraradicals Andrzej Rajca, Arnon Olankitwanit, Ying Wang, Przemysław J. Boratyński, Maren Pink, and Suchada Rajca pp 18205–18215 DOI: 10.1021/ja409472f Supporting Info |
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Three-Dimensional Metallic Boron Nitride Shunhong Zhang, Qian Wang, Yoshiyuki Kawazoe, and Puru Jena pp 18216–18221 DOI: 10.1021/ja410088y Supporting Info |
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Optical Properties and Electronic Energy Relaxation of Metallic Au144(SR)60 Nanoclusters Chongyue Yi, Marcus A. Tofanelli, Christopher J. Ackerson, and Kenneth L. Knappenberger, Jr. pp 18222–18228 DOI: 10.1021/ja409998j Supporting Info |
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Dibenzoheptazethrene Isomers with Different Biradical Characters: An Exercise of Clar’s Aromatic Sextet Rule in Singlet Biradicaloids Zhe Sun, Sangsu Lee, Kyu Hyung Park, Xiaojian Zhu, Wenhua Zhang, Bin Zheng, Pan Hu, Zebing Zeng, Soumyajit Das, Yuan Li, Chunyan Chi, Run-Wei Li, Kuo-Wei Huang, Jun Ding, Dongho Kim, and Jishan Wu pp 18229–18236 DOI: 10.1021/ja410279j Supporting Info |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 18237–18237 DOI: 10.1021/ja412289s |
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Making Sense of the Mayhem behind Shape Control in the Synthesis of Gold Nanoparticles Michelle L. Personick and Chad A. Mirkin pp 18238–18247 DOI: 10.1021/ja408645b |
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A New, Energy-Efficient Chemical Pathway for Extracting Ti Metal from Ti Minerals Zhigang Zak Fang, Scott Middlemas, Jun Guo, and Peng Fan pp 18248–18251 DOI: 10.1021/ja408118x Supporting Info |
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Ab Initio Modeling of Excitonic and Charge-Transfer States in Organic Semiconductors: The PTB1/PCBM Low Band Gap System Itamar Borges, Jr., Adélia J. A. Aquino, Andreas Köhn, Reed Nieman, William L. Hase, Lin X. Chen, and Hans Lischka pp 18252–18255 DOI: 10.1021/ja4081925 Supporting Info |
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Solution Synthesis and Reactivity of Colloidal Fe2GeS4: A Potential Candidate for Earth Abundant, Nanostructured Photovoltaics Sarah J. Fredrick and Amy L. Prieto pp 18256–18259 DOI: 10.1021/ja408333y Supporting Info |
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An Optical Trap Combined with Three-Color FRET Sanghwa Lee and Sungchul Hohng pp 18260–18263 DOI: 10.1021/ja408767p Supporting Info |
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Nonsuperatomic [Au23(SC6H11)16]− Nanocluster Featuring Bipyramidal Au15 Kernel and Trimeric Au3(SR)4 Motif Anindita Das, Tao Li, Katsuyuki Nobusada, Chenjie Zeng, Nathaniel L. Rosi, and Rongchao Jin pp 18264–18267 DOI: 10.1021/ja409177s Supporting Info |
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Propeller-Shaped Fused Oligothiophenes: A Remarkable Effect of the Topology of Sulfur Atoms on Columnar Stacking Qi Xiao, Tsuneaki Sakurai, Takahiro Fukino, Kouki Akaike, Yoshihito Honsho, Akinori Saeki, Shu Seki, Kenichi Kato, Masaki Takata, and Takuzo Aida pp 18268–18271 DOI: 10.1021/ja4092769 Supporting Info |
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Synthesis and Reactivity of Two-Coordinate Ni(I) Alkyl and Aryl Complexes Carl A. Laskowski, Donald J. Bungum, Steven M. Baldwin, Sarah A. Del Ciello, Vlad M. Iluc, and Gregory L. Hillhouse pp 18272–18275 DOI: 10.1021/ja4095236 Supporting Info |
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Rolling Up the Sheet: Constructing Metal–Organic Lamellae and Nanotubes from a [{Mn3(propanediolato)2}(dicyanamide)2]n Honeycomb Skeleton Gang Wu, Jiaquan Bai, Yuan Jiang, Guanghua Li, Jian Huang, Yi Li, Christopher E. Anson, Annie K. Powell, and Shilun Qiu pp 18276–18279 DOI: 10.1021/ja409569q Supporting Info |
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Synthesis of Biologically Active N- and O-Linked Glycans with Multisialylated Poly-N-acetyllactosamine Extensions Using P. damsela α2-6 Sialyltransferase Corwin M. Nycholat, Wenjie Peng, Ryan McBride, Aristotelis Antonopoulos, Robert P. de Vries, Zinaida Polonskaya, M.G. Finn, Anne Dell, Stuart M. Haslam, and James C. Paulson pp 18280–18283 DOI: 10.1021/ja409781c Supporting Info |
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Room-Temperature Synthesis of Trisubstituted Allenylsilanes via Regioselective C–H Functionalization Rong Zeng, Shangze Wu, Chunling Fu, and Shengming Ma pp 18284–18287 DOI: 10.1021/ja409861s Supporting Info |
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Noncovalent Immobilization of Electrocatalysts on Carbon Electrodes for Fuel Production James D. Blakemore, Ayush Gupta, Jeffrey J. Warren, Bruce S. Brunschwig, and Harry B. Gray pp 18288–18291 DOI: 10.1021/ja4099609 Supporting Info |
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Nano-Chemical Infrared Imaging of Membrane Proteins in Lipid Bilayers Samuel Berweger, Duc M. Nguyen, Eric A. Muller, Hans A. Bechtel, Thomas T. Perkins, and Markus B. Raschke pp 18292–18295 DOI: 10.1021/ja409815g Supporting Info |
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Cobalt Fluorocarbenes: Cycloaddition Reactions with Tetrafluoroethylene and Reactivity of the Perfluorometallacyclic Products Daniel J. Harrison, Graham M. Lee, Matthew C. Leclerc, Ilia Korobkov, and R. Tom Baker pp 18296–18299 DOI: 10.1021/ja411503c Supporting Info |
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Sol–Gel Design Strategy for Ultradispersed TiO2 Nanoparticles on Graphene for High-Performance Lithium Ion Batteries Wei Li, Fei Wang, Shanshan Feng, Jinxiu Wang, Zhenkun Sun, Bin Li, Yuhui Li, Jianping Yang, Ahmed A. Elzatahry, Yongyao Xia, and Dongyuan Zhao pp 18300–18303 DOI: 10.1021/ja4100723 Supporting Info |
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Ultrathin Pt–Cu Nanosheets and Nanocones Faisal Saleem, Zhicheng Zhang, Biao Xu, Xiaobin Xu, Peilei He, and Xun Wang pp 18304–18307 DOI: 10.1021/ja4101968 Supporting Info |
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Olefin Isomerization and Hydrosilylation Catalysis by Lewis Acidic Organofluorophosphonium Salts Manuel Pérez, Lindsay J. Hounjet, Christopher B. Caputo, Roman Dobrovetsky, and Douglas W. Stephan pp 18308–18310 DOI: 10.1021/ja410379x Supporting Info |
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Redox Transitions in an Electrolyte-Free Myoglobin Fluid Kamendra P. Sharma, Kieren Bradley, Alex P. S. Brogan, Stephen Mann, Adam W. Perriman, and David J. Fermin pp 18311–18314 DOI: 10.1021/ja4104606 Supporting Info |
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A Dihydrodisilene Transition Metal Complex from an N-Heterocyclic Carbene-Stabilized Silylene Monohydride Shigeyoshi Inoue and Carsten Eisenhut pp 18315–18318 DOI: 10.1021/ja410528y Supporting Info |
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Deep-Ultraviolet Nonlinear Optical Materials: Na2Be4B4O11 and LiNa5Be12B12O33 Hongwei Huang, Lijuan Liu, Shifeng Jin, Wenjiao Yao, Yihe Zhang, and Chuangtian Chen pp 18319–18322 DOI: 10.1021/ja410543w Supporting Info |
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Direct β-Functionalization of Cyclic Ketones with Aryl Ketones via the Merger of Photoredox and Organocatalysis Filip R. Petronijević, Manuel Nappi, and David W. C. MacMillan pp 18323–18326 DOI: 10.1021/ja410478a Supporting Info |
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Palladium-Catalyzed Difunctionalization of Enol Ethers to Amino Acetals with Aminals and Alcohols Yinjun Xie, Jianhua Hu, Pan Xie, Bo Qian, and Hanmin Huang pp 18327–18330 DOI: 10.1021/ja410611b Supporting Info |
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Silicon Ring Strain Creates High-Conductance Pathways in Single-Molecule Circuits Timothy A. Su, Jonathan R. Widawsky, Haixing Li, Rebekka S. Klausen, James L. Leighton, Michael L. Steigerwald, Latha Venkataraman, and Colin Nuckolls pp 18331–18334 DOI: 10.1021/ja410656a Supporting Info |
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Cyclization of Squalene from Both Termini: Identification of an Onoceroid Synthase and Enzymatic Synthesis of Ambrein Daijiro Ueda, Tsutomu Hoshino, and Tsutomu Sato pp 18335–18338 DOI: 10.1021/ja4107226 Supporting Info |
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Regulation of Light Harvesting in the Green Alga Chlamydomonas reinhardtii: The C-Terminus of LHCSR Is the Knob of a Dimmer Switch Nicoletta Liguori, Laura M. Roy, Milena Opacic, Grégory Durand, and Roberta Croce pp 18339–18342 DOI: 10.1021/ja4107463 Supporting Info |
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Enzyme Architecture: The Activating Oxydianion Binding Domain for Orotidine 5′-Monophophate Decarboxylase Krisztina Spong, Tina L. Amyes, and John P. Richard pp 18343–18346 DOI: 10.1021/ja4107513 Supporting Info |
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Palladium-Catalyzed Cross-Coupling of N-Sulfonylaziridines with Boronic Acids Megan L. Duda and Forrest E. Michael pp 18347–18349 DOI: 10.1021/ja410686v Supporting Info |
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Ortho vs Ipso: Site-Selective Pd and Norbornene-Catalyzed Arene C–H Amination Using Aryl Halides Zhe Dong and Guangbin Dong pp 18350–18353 DOI: 10.1021/ja410823e Supporting Info |
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Facet-Selective Growth on Nanowires Yields Multi-Component Nanostructures and Photonic Devices Thomas J. Kempa, Sun-Kyung Kim, Robert W. Day, Hong-Gyu Park, Daniel G. Nocera, and Charles M. Lieber pp 18354–18357 DOI: 10.1021/ja411050r Supporting Info |
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β-Lactamase Inhibition by 7-Alkylidenecephalosporin Sulfones: Allylic Transposition and Formation of an Unprecedented Stabilized Acyl-Enzyme Elizabeth A. Rodkey, David C. McLeod, Christopher R. Bethel, Kerri M. Smith, Yan Xu, Weirui Chai, Tao Che, Paul R. Carey, Robert A. Bonomo, Focco van den Akker, and John D. Buynak pp 18358–18369 DOI: 10.1021/ja403598g Supporting Info |
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Solvent Wrapped Metastable Colloidal Crystals: Highly Mutable Colloidal Assemblies Sensitive to Weak External Disturbance Dongpeng Yang, Siyun Ye, and Jianping Ge pp 18370–18376 DOI: 10.1021/ja405670r Supporting Info |
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Phase-Controlled Synthesis of Cu2ZnSnS4 Nanocrystals: The Role of Reactivity between Zn and S Yu Zou, Xiong Su, and Jiang Jiang pp 18377–18384 DOI: 10.1021/ja405962k Supporting Info |
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New Basic Insight into Reductive Functionalization Sequences of Single Walled Carbon Nanotubes (SWCNTs) Ferdinand Hof, Sebastian Bosch, Siegfried Eigler, Frank Hauke, and Andreas Hirsch pp 18385–18395 DOI: 10.1021/ja4063713 Supporting Info |
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Mechanistic Insights into the Gold(I)-Catalyzed Activation of Glycosyl ortho-Alkynylbenzoates for Glycosidation Yu Tang, Jiakun Li, Yugen Zhu, Yao Li, and Biao Yu pp 18396–18405 DOI: 10.1021/ja4064316 Supporting Info |
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Uncovering the Selection Criteria for the Emergence of Multi-Building-Block Replicators from Dynamic Combinatorial Libraries Morteza Malakoutikhah, Jérôme J.-P. Peyralans, Mathieu Colomb-Delsuc, Hugo Fanlo-Virgós, Marc C. A. Stuart, and Sijbren Otto pp 18406–18417 DOI: 10.1021/ja4067805 Supporting Info |
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Direct Spectroscopic Evidence of Ultrafast Electron Transfer from a Low Band Gap Polymer to CdSe Quantum Dots in Hybrid Photovoltaic Thin Films Elsa Couderc, Matthew J. Greaney, Richard L. Brutchey, and Stephen E. Bradforth pp 18418–18426 DOI: 10.1021/ja406884h Supporting Info |
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Topological Effects and Binding Modes Operating with Multivalent Iminosugar-Based Glycoclusters and Mannosidases Yoan Brissonnet, Carmen Ortiz Mellet, Sandrine Morandat, M. Isabel Garcia Moreno, David Deniaud, Susan E. Matthews, Sébastien Vidal, Sergej Šesták, Karim El Kirat, and Sébastien G. Gouin pp 18427–18435 DOI: 10.1021/ja406931w Supporting Info |
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Structural Characterization of Native Autoinducing Peptides and Abiotic Analogues Reveals Key Features Essential for Activation and Inhibition of an AgrC Quorum Sensing Receptor in Staphylococcus aureus Yftah Tal-Gan, Monika Ivancic, Gabriel Cornilescu, Claudia C. Cornilescu, and Helen E. Blackwell pp 18436–18444 DOI: 10.1021/ja407533e Supporting Info |
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Intracellular pH Measurements Using Perfluorocarbon Nanoemulsions Michael J. Patrick, Jelena M. Janjic, Haibing Teng, Meredith R. O’Hear, Cortlyn W. Brown, Jesse A. Stokum, Brigitte F. Schmidt, Eric T. Ahrens, and Alan S. Waggoner pp 18445–18457 DOI: 10.1021/ja407573m Supporting Info |
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Epitope Fluctuations in the Human Papillomavirus Are Under Dynamic Allosteric Control: A Computational Evaluation of a New Vaccine Design Strategy Abhishek Singharoy, Abhigna Polavarapu, Harshad Joshi, Mu-Hyun Baik, and Peter Ortoleva pp 18458–18468 DOI: 10.1021/ja407489r Supporting Info |
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Selective NO Trapping in the Pores of Chain-Type Complex Assemblies Based on Electronically Activated Paddlewheel-Type [Ru2II,II]/[Rh2II,II] Dimers Wataru Kosaka, Kayo Yamagishi, Akihiro Hori, Hiroshi Sato, Ryotaro Matsuda, Susumu Kitagawa, Masaki Takata, and Hitoshi Miyasaka pp 18469–18480 DOI: 10.1021/ja4076056 Supporting Info |
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Success in Making Zn+ from Atomic Zn0 Encapsulated in an MFI-Type Zeolite with UV Light Irradiation Akira Oda, Hiroe Torigoe, Atsushi Itadani, Takahiro Ohkubo, Takashi Yumura, Hisayoshi Kobayashi, and Yasushige Kuroda pp 18481–18489 DOI: 10.1021/ja4077342 Supporting Info |
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Minimal Proton Channel Enables H2 Oxidation and Production with a Water-Soluble Nickel-Based Catalyst Arnab Dutta, Sheri Lense, Jianbo Hou, Mark H. Engelhard, John A. S. Roberts, and Wendy J. Shaw pp 18490–18496 DOI: 10.1021/ja407826d Supporting Info |
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Bromine-Catalyzed Conversion of CO2 and Epoxides to Cyclic Carbonates under Continuous Flow Conditions Jennifer A. Kozak, Jie Wu, Xiao Su, Fritz Simeon, T. Alan Hatton, and Timothy F. Jamison pp 18497–18501 DOI: 10.1021/ja4079094 Supporting Info |
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Broadband Ultrafast Photoluminescence Spectroscopy Resolves Charge Photogeneration via Delocalized Hot Excitons in Polymer:Fullerene Photovoltaic Blends Kai Chen, Alex J. Barker, Matthew E. Reish, Keith C. Gordon, and Justin M. Hodgkiss pp 18502–18512 DOI: 10.1021/ja408235h Supporting Info |
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A Photoactive Porphyrin-Based Periodic Mesoporous Organosilica Thin Film Yan Li, Florian Auras, Florian Löbermann, Markus Döblinger, Jörg Schuster, Laurence Peter, Dirk Trauner, and Thomas Bein pp 18513–18519 DOI: 10.1021/ja4082028 Supporting Info |
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Controlled Electrodeposition of Bismuth Nanocatalysts for the Solution–Liquid–Solid Synthesis of CdSe Nanowires on Transparent Conductive Substrates Natalia Reim, Alexander Littig, Dino Behn, and Alf Mews pp 18520–18527 DOI: 10.1021/ja408265s |
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Differentiating Amino Acid Residues and Side Chain Orientations in Peptides Using Scanning Tunneling Microscopy Shelley A. Claridge, John C. Thomas, Miles A. Silverman, Jeffrey J. Schwartz, Yanlian Yang, Chen Wang, and Paul S. Weiss pp 18528–18535 DOI: 10.1021/ja408550a Supporting Info |
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Ligand Exchange and the Stoichiometry of Metal Chalcogenide Nanocrystals: Spectroscopic Observation of Facile Metal-Carboxylate Displacement and Binding Nicholas C. Anderson, Mark P. Hendricks, Joshua J. Choi, and Jonathan S. Owen pp 18536–18548 DOI: 10.1021/ja4086758 Supporting Info |
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Robust Affinity Standards for Cu(I) Biochemistry Pritha Bagchi, M. Thomas Morgan, John Bacsa, and Christoph J. Fahrni pp 18549–18559 DOI: 10.1021/ja408827d Supporting Info |
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CsPbCO3F: A Strong Second-Harmonic Generation Material Derived from Enhancement via p−π Interaction Guohong Zou, Ling Huang, Ning Ye, Chensheng Lin, Wendan Cheng, and Hui Huang pp 18560–18566 DOI: 10.1021/ja408982d Supporting Info |
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Carbonylation Reactions of Intramolecular Vicinal Frustrated Phosphane/Borane Lewis Pairs Muhammad Sajid, Arunlibertsen Lawzer, Weishi Dong, Christoph Rosorius, Wolfram Sander, Birgitta Schirmer, Stefan Grimme, Constantin G. Daniliuc, Gerald Kehr, and Gerhard Erker pp 18567–18574 DOI: 10.1021/ja408815k Supporting Info |
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HIV-1 Nucleocapsid Proteins as Molecular Chaperones for Tetramolecular Antiparallel G-Quadruplex Formation Arivazhagan Rajendran, Masayuki Endo, Kumi Hidaka, Phong Lan Thao Tran, Jean-Louis Mergny, Robert J. Gorelick, and Hiroshi Sugiyama pp 18575–18585 DOI: 10.1021/ja409085j Supporting Info |
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Transition-State Enthalpy and Entropy Effects on Reactivity and Selectivity in Hydrogenolysis of n-Alkanes David W. Flaherty and Enrique Iglesia pp 18586–18599 DOI: 10.1021/ja4093743 Supporting Info |
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Direct Measurement of the Mn(II) Hydration State in Metal Complexes and Metalloproteins through 17O NMR Line Widths Eric M. Gale, Jiang Zhu, and Peter Caravan pp 18600–18608 DOI: 10.1021/ja4094132 Supporting Info |
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Relative Unidirectional Translation in an Artificial Molecular Assembly Fueled by Light Hao Li, Chuyang Cheng, Paul R. McGonigal, Albert C. Fahrenbach, Marco Frasconi, Wei-Guang Liu, Zhixue Zhu, Yanli Zhao, Chenfeng Ke, Juying Lei, Ryan M. Young, Scott M. Dyar, Dick T. Co, Ying-Wei Yang, Youssry Y. Botros, William A. Goddard, III, Michael R. Wasielewski, R. Dean Astumian, and J. Fraser Stoddart pp 18609–18620 DOI: 10.1021/ja4094204 Supporting Info |
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Antiferromagnetic Iron Nanocolloids: A New Generation in Vivo T1 MRI Contrast Agent Yung-Kang Peng, Chien-Liang Liu, Hsieh-Chih Chen, Shang-Wei Chou, Wei-Hsuan Tseng, Yu-Jui Tseng, Chia-Cheng Kang, Jong-Kai Hsiao, and Pi-Tai Chou pp 18621–18628 DOI: 10.1021/ja409490q Supporting Info |
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Unexpected Chirality of Nanoparticle Dimers and Ultrasensitive Chiroplasmonic Bioanalysis Xiaoling Wu, Liguang Xu, Liqiang Liu, Wei Ma, Honghong Yin, Hua Kuang, Libing Wang, Chuanlai Xu, and Nicholas A. Kotov pp 18629–18636 DOI: 10.1021/ja4095445 Supporting Info |
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Structural Insights into DNA Replication without Hydrogen Bonds Karin Betz, Denis A. Malyshev, Thomas Lavergne, Wolfram Welte, Kay Diederichs, Floyd E. Romesberg, and Andreas Marx pp 18637–18643 DOI: 10.1021/ja409609j Supporting Info |
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Building a Multifunctional Aptamer-Based DNA Nanoassembly for Targeted Cancer Therapy Cuichen Wu, Da Han, Tao Chen, Lu Peng, Guizhi Zhu, Mingxu You, Liping Qiu, Kwame Sefah, Xiaobing Zhang, and Weihong Tan pp 18644–18650 DOI: 10.1021/ja4094617 Supporting Info |
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Thioamide Quenching of Fluorescent Probes through Photoinduced Electron Transfer: Mechanistic Studies and Applications Jacob M. Goldberg, Solongo Batjargal, Benson S. Chen, and E. James Petersson pp 18651–18658 DOI: 10.1021/ja409709x Supporting Info |
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Superbases in Confined Space: Control of the Basicity and Reactivity of the Proton Transfer Bastien Chatelet, Heinz Gornitzka, Véronique Dufaud, Erwann Jeanneau, Jean-Pierre Dutasta, and Alexandre Martinez pp 18659–18664 DOI: 10.1021/ja409444s Supporting Info |
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Nanosecond Time Scale Motions in Proteins Revealed by High-Resolution NMR Relaxometry Cyril Charlier, Shahid Nawaz Khan, Thorsten Marquardsen, Philippe Pelupessy, Volker Reiss, Dimitris Sakellariou, Geoffrey Bodenhausen, Frank Engelke, and Fabien Ferrage pp 18665–18672 DOI: 10.1021/ja409820g Supporting Info |
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Naturally Split Inteins Assemble through a “Capture and Collapse” Mechanism Neel H. Shah, Ertan Eryilmaz, David Cowburn, and Tom W. Muir pp 18673–18681 DOI: 10.1021/ja4104364 Supporting Info |
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Interplay of Hydrogen Bonds and n→π* Interactions in Proteins Gail J. Bartlett, Robert W. Newberry, Brett VanVeller, Ronald T. Raines, and Derek N. Woolfson pp 18682–18688 DOI: 10.1021/ja4106122 Supporting Info |
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Increased Dynamic Effects in a Catalytically Compromised Variant of Escherichia coli Dihydrofolate Reductase J. Javier Ruiz-Pernia, Louis Y. P. Luk, Rafael García-Meseguer, Sergio Martí, E. Joel Loveridge, Iñaki Tuñón, Vicent Moliner, and Rudolf K. Allemann pp 18689–18696 DOI: 10.1021/ja410519h Supporting Info |
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A Chiral Sulfoxide-Ligated Ruthenium Complex for Asymmetric Catalysis: Enantio- and Regioselective Allylic Substitution Barry M. Trost, Meera Rao, and André P. Dieskau pp 18697–18704 DOI: 10.1021/ja411310w Supporting Info |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 18705–18705 DOI: 10.1021/ja4124016 |
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Asymmetric Substitution at the Tetrasubstituted Chiral Carbon: Catalytic Ring-Opening Alkylation of Racemic 2,2-Disubstituted Aziridines with 3-Substituted Oxindoles Kohsuke Ohmatsu, Yuichiro Ando, and Takashi Ooi pp 18706–18709 DOI: 10.1021/ja411647x Supporting Info |
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Enzyme-Directed Assembly of Nanoparticles in Tumors Monitored by in Vivo Whole Animal Imaging and ex Vivo Super-Resolution Fluorescence Imaging Miao-Ping Chien, Andrea S. Carlini, Dehong Hu, Christopher V. Barback, Anthony M. Rush, David J. Hall, Galya Orr, and Nathan C. Gianneschi pp 18710–18713 DOI: 10.1021/ja408182p Supporting Info |
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Synthesis, Structure, and Reactivity of a Terminal Organozinc Fluoride Compound: Hydrogen Bonding, Halogen Bonding, and Donor–Acceptor Interactions Wesley Sattler, Serge Ruccolo, and Gerard Parkin pp 18714–18717 DOI: 10.1021/ja408733f Supporting Info |
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Photodegradable Supramolecular Hydrogels with Fluorescence Turn-On Reporter for Photomodulation of Cellular Microenvironments Mingtao He, Jinbo Li, Subee Tan, Ruzhi Wang, and Yan Zhang pp 18718–18721 DOI: 10.1021/ja409000b Supporting Info |
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Biphasic Self-Assembly Pathways and Size-Dependent Photophysical Properties of Perylene Bisimide Dye Aggregates Franziska Fennel, Steffen Wolter, Zengqi Xie, Per-Arno Plötz, Oliver Kühn, Frank Würthner, and Stefan Lochbrunner pp 18722–18725 DOI: 10.1021/ja409597x Supporting Info |
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Acceptorless Dehydrogenation of C–C Single Bonds Adjacent to Functional Groups by Metal–Ligand Cooperation Shuhei Kusumoto, Midori Akiyama, and Kyoko Nozaki pp 18726–18729 DOI: 10.1021/ja409672w Supporting Info |
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Design, Generation, and Synthetic Application of Borylzincate: Borylation of Aryl Halides and Borylzincation of Benzynes/Terminal Alkyne Yuki Nagashima, Ryo Takita, Kengo Yoshida, Keiichi Hirano, and Masanobu Uchiyama pp 18730–18733 DOI: 10.1021/ja409748m Supporting Info |
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Closer to Photosystem II: A Co4O4 Cubane Catalyst with Flexible Ligand Architecture Fabio Evangelisti, Robin Güttinger, René Moré, Sandra Luber, and Greta R. Patzke pp 18734–18737 DOI: 10.1021/ja4098302 Supporting Info |
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Zwitterionic Polymerization to Generate High Molecular Weight Cyclic Poly(Carbosiloxane)s Hayley A. Brown, Young A. Chang, and Robert M. Waymouth pp 18738–18741 DOI: 10.1021/ja409843v Supporting Info |
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Three-Component [2+2+1] Cross-cyclotrimerization of Carboryne, Unactivated Alkene, and Trimethylsilylalkyne Co-mediated by Zr and Ni Yangjian Quan, Jiji Zhang, and Zuowei Xie pp 18742–18745 DOI: 10.1021/ja410233e Supporting Info |
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Long-Lived Nuclear Spin States in Methyl Groups and Quantum-Rotor-Induced Polarization Benno Meier, Jean-Nicolas Dumez, Gabriele Stevanato, Joseph T. Hill-Cousins, Soumya Singha Roy, Pär Håkansson, Salvatore Mamone, Richard C. D. Brown, Giuseppe Pileio, and Malcolm H. Levitt pp 18746–18749 DOI: 10.1021/ja410432f Supporting Info |
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Insights into Caerulomycin A Biosynthesis: A Two-Component Monooxygenase CrmH-Catalyzed Oxime Formation Yiguang Zhu, Qingbo Zhang, Sumei Li, Qinheng Lin, Peng Fu, Guangtao Zhang, Haibo Zhang, Rong Shi, Weiming Zhu, and Changsheng Zhang pp 18750–18753 DOI: 10.1021/ja410513g Supporting Info |
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Synthesis of Convex Hexoctahedral Pt Micro/Nanocrystals with High-Index Facets and Electrochemistry-Mediated Shape Evolution Jing Xiao, Shuo Liu, Na Tian, Zhi-You Zhou, Hai-Xia Liu, Bin-Bin Xu, and Shi-Gang Sun pp 18754–18757 DOI: 10.1021/ja410583b Supporting Info |
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Nitrite Activation to Nitric Oxide via One-fold Protonation of Iron(II)-O,O-nitrito Complex: Relevance to the Nitrite Reductase Activity of Deoxyhemoglobin and Deoxyhemerythrin Chih-Chin Tsou, Wan-Lin Yang, and Wen-Feng Liaw* pp 18758–18761 DOI: 10.1021/ja4105864 Supporting Info |
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Self-Assembly of Left- and Right-Handed Molecular Screws Fei Xu, I. John Khan, Kenneth McGuinness, Avanish S. Parmar, Teresita Silva, N. Sanjeeva Murthy, and Vikas Nanda pp 18762–18765 DOI: 10.1021/ja4106545 Supporting Info |
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Bottleable (Amino)(Carboxy) Radicals Derived from Cyclic (Alkyl)(Amino) Carbenes Janell K. Mahoney, David Martin, Curtis E. Moore, Arnold L. Rheingold, and Guy Bertrand pp 18766–18769 DOI: 10.1021/ja4104765 Supporting Info |
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Detection and Differentiation of Neutral Organic Compounds by 19F NMR with a Tungsten Calix[4]arene Imido Complex Yanchuan Zhao and Timothy M. Swager pp 18770–18773 DOI: 10.1021/ja4106804 Supporting Info |
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Chemical Dynamics of the First Proton-Coupled Electron Transfer of Water Oxidation on TiO2 Anatase Jia Chen, Ye-Fei Li, Patrick Sit, and Annabella Selloni pp 18774–18777 DOI: 10.1021/ja410685m Supporting Info |
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Meta-Selective C–H Functionalization Using a Nitrile-Based Directing Group and Cleavable Si-Tether Sunggi Lee, Hyelee Lee, and Kian L. Tan pp 18778–18781 DOI: 10.1021/ja4107034 Supporting Info |
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Photochemical Electronic Doping of Colloidal CdSe Nanocrystals Jeffrey D. Rinehart, Alina M. Schimpf, Amanda L. Weaver, Alicia W. Cohn, and Daniel R. Gamelin pp 18782–18785 DOI: 10.1021/ja410825c Supporting Info |
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Targeting Human Telomeric Higher-Order DNA: Dimeric G-Quadruplex Units Serve as Preferred Binding Site Chuanqi Zhao, Li Wu, Jinsong Ren, Yan Xu, and Xiaogang Qu pp 18786–18789 DOI: 10.1021/ja410723r Supporting Info |
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A C60-Templated Tetrameric Porphyrin Barrel Complex via Zinc-Mediated Self-Assembly Utilizing Labile Capping Ligands Takashi Nakamura, Hitoshi Ube, Ryosuke Miyake, and Mitsuhiko Shionoya pp 18790–18793 DOI: 10.1021/ja4110446 Supporting Info |
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Four-Component Supramolecular Nanorotors Soumen K. Samanta and Michael Schmittel pp 18794–18797 DOI: 10.1021/ja411011a Supporting Info |
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Elucidation of Carbene Ambiphilicity Leading to the Discovery of Reversible Ammonia Activation Jonathan P. Moerdyk, Garrett A. Blake, Daniel T. Chase, and Christopher W. Bielawski pp 18798–18801 DOI: 10.1021/ja411467p Supporting Info |
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Chiral Amide Directed Assembly of a Diastereo- and Enantiopure Supramolecular Host and its Application to Enantioselective Catalysis of Neutral Substrates Chen Zhao, Qing-Fu Sun, William M. Hart-Cooper, Antonio G. DiPasquale, F. Dean Toste, Robert G. Bergman, and Kenneth N. Raymond pp 18802–18805 DOI: 10.1021/ja411631v Supporting Info |
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Efficient Synthesis and In Vivo Incorporation of Acridon-2-ylalanine, a Fluorescent Amino Acid for Lifetime and Förster Resonance Energy Transfer/Luminescence Resonance Energy Transfer Studies Lee C. Speight, Anand K. Muthusamy, Jacob M. Goldberg, John B. Warner, Rebecca F. Wissner, Taylor S. Willi, Bradley F. Woodman, Ryan A. Mehl, and E. James Petersson pp 18806–18814 DOI: 10.1021/ja403247j Supporting Info |
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Polycationic Ligands in Gold Catalysis: Synthesis and Applications of Extremely π-Acidic Catalysts Javier Carreras, Gopinadhanpillai Gopakumar, Liangu Gu, Ana Gimeno, Pawel Linowski, Jekaterina Petuškova, Walter Thiel, and Manuel Alcarazo pp 18815–18823 DOI: 10.1021/ja411146x Supporting Info |
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Independent Ordering of Two Interpenetrating Magnetic Sublattices in the Double Perovskite Sr2CoOsO6 Ryan Morrow, Rohan Mishra, Oscar D. Restrepo, Molly R. Ball, Wolfgang Windl, Sabine Wurmehl, Ulrike Stockert, Bernd Büchner, and Patrick M. Woodward pp 18824–18830 DOI: 10.1021/ja407342w Supporting Info |
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Glycoside Hydrolase Processivity Is Directly Related to Oligosaccharide Binding Free Energy Christina M. Payne, Wei Jiang, Michael R. Shirts, Michael E. Himmel, Michael F. Crowley, and Gregg T. Beckham pp 18831–18839 DOI: 10.1021/ja407287f Supporting Info |
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The Designability of Protein Switches by Chemical Rescue of Structure: Mechanisms of Inactivation and Reactivation Yan Xia, Nina DiPrimio, Theodore R. Keppel, Binh Vo, Keith Fraser, Kevin P. Battaile, Chet Egan, Christopher Bystroff, Scott Lovell, David D. Weis, J. Christopher Anderson, and John Karanicolas pp 18840–18849 DOI: 10.1021/ja407644b Supporting Info |
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Cell-Specific and pH-Activatable Rubyrin-Loaded Nanoparticles for Highly Selective Near-Infrared Photodynamic Therapy against Cancer Jiangwei Tian, Lin Ding, Hai-Jun Xu, Zhen Shen, Huangxian Ju, Li Jia, Lei Bao, and Jun-Sheng Yu pp 18850–18858 DOI: 10.1021/ja408286k Supporting Info |
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Electronic and Chemical Properties of a Surface-Terminated Screw Dislocation in MgO Keith P. McKenna pp 18859–18865 DOI: 10.1021/ja408342z |
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Evolution of Physical and Electronic Structures of Bilayer Graphene upon Chemical Functionalization Qing Hua Wang, Chih-Jen Shih, Geraldine L. C. Paulus, and Michael S. Strano pp 18866–18875 DOI: 10.1021/ja4083914 Supporting Info |
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Two-Electron HCl to H2 Photocycle Promoted by Ni(II) Polypyridyl Halide Complexes David C. Powers, Bryce L. Anderson, and Daniel G. Nocera pp 18876–18883 DOI: 10.1021/ja408787k Supporting Info |
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The Mechanism of Denaturation and the Unfolded State of the α-Helical Membrane-Associated Protein Mistic Tomas Jacso, Benjamin Bardiaux, Jana Broecker, Sebastian Fiedler, Tom Baerwinkel, Andi Mainz, Uwe Fink, Carolyn Vargas, Hartmut Oschkinat, Sandro Keller, and Bernd Reif pp 18884–18891 DOI: 10.1021/ja408644f Supporting Info |
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Defects Are Needed for Fast Photo-Induced Electron Transfer from a Nanocrystal to a Molecule: Time-Domain Ab Initio Analysis Run Long, Niall J. English, and Oleg V. Prezhdo pp 18892–18900 DOI: 10.1021/ja408936j Supporting Info |
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Enantioselective Polymerization of Epoxides Using Biaryl-Linked Bimetallic Cobalt Catalysts: A Mechanistic Study Syud M. Ahmed, Albert Poater, M. Ian Childers, Peter C. B. Widger, Anne M. LaPointe, Emil B. Lobkovsky, Geoffrey W. Coates, and Luigi Cavallo pp 18901–18911 DOI: 10.1021/ja409521z Supporting Info |
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Ligand Noninnocence of Thiolate/Disulfide in Dinuclear Copper Complexes: Solvent-Dependent Redox Isomerization and Proton-Coupled Electron Transfer Andrew M. Thomas, Bo-Lin Lin, Erik C. Wasinger, and T. Daniel P. Stack pp 18912–18919 DOI: 10.1021/ja409603m Supporting Info |
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In Vivo Multimodality Imaging and Cancer Therapy by Near-Infrared Light-Triggered trans-Platinum Pro-Drug-Conjugated Upconverison Nanoparticles Yunlu Dai, Haihua Xiao, Jianhua Liu, Qinghai Yuan, Ping’an Ma, Dongmei Yang, Chunxia Li, Ziyong Cheng, Zhiyao Hou, Piaoping Yang, and Jun Lin pp 18920–18929 DOI: 10.1021/ja410028q Supporting Info |
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Electrochemical Evidence for Intermolecular Proton-Coupled Electron Transfer through a Hydrogen Bond Complex in a p-Phenylenediamine-Based Urea. Introduction of the “Wedge Scheme” as a Useful Means To Describe Reactions of This Type Laurie A. Clare, An T. Pham, Francine Magdaleno, Jaqueline Acosta, Jessica E. Woods, Andrew L. Cooksy, and Diane K. Smith pp 18930–18941 DOI: 10.1021/ja410061x Supporting Info |
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Universal Correlation between Fibril Width and Quantum Efficiency in Diketopyrrolopyrrole-Based Polymer Solar Cells Weiwei Li, Koen H. Hendriks, Alice Furlan, W. S. Christian Roelofs, Martijn M. Wienk, and René A. J. Janssen pp 18942–18948 DOI: 10.1021/ja4101003 Supporting Info |
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Total Synthesis and Anti-Hepatitis C Virus Activity of MA026 Satomi Shimura, Masahiro Ishima, Syo Nakajima, Toshitaka Fujii, Natsumi Himeno, Kentaro Ikeda, Jesus Izaguirre-Carbonell, Hiroshi Murata, Toshifumi Takeuchi, Shinji Kamisuki, Takahiro Suzuki, Kouji Kuramochi, Koichi Watashi, Susumu Kobayashi, and Fumio Sugawara pp 18949–18956 DOI: 10.1021/ja410145x Supporting Info |
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Modulation of Quinone PCET Reaction by Ca2+ Ion Captured by Calix[4]quinone in Water Yang-Rae Kim, R. Soyoung Kim, Sun Kil Kang, Myung Gil Choi, Hong Yeong Kim, Daeheum Cho, Jin Yong Lee, Suk-Kyu Chang, and Taek Dong Chung pp 18957–18967 DOI: 10.1021/ja410406e Supporting Info |
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In Situ NMR Spectroscopy of Supercapacitors: Insight into the Charge Storage Mechanism Hao Wang, Alexander C. Forse, John M. Griffin, Nicole M. Trease, Lorie Trognko, Pierre-Louis Taberna, Patrice Simon, and Clare P. Grey pp 18968–18980 DOI: 10.1021/ja410287s Supporting Info |
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Cocrystals of Nicotinamide and (R)-Mandelic Acid in Many Ratios with Anomalous Formation Properties Si-Wei Zhang, Michelle T. Harasimowicz, Melgardt M. de Villiers, and Lian Yu pp 18981–18989 DOI: 10.1021/ja4103887 Supporting Info |
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Superhydrophobic Photosensitizers. Mechanistic Studies of 1O2 Generation in the Plastron and Solid/Liquid Droplet Interface David Aebisher, Dorota Bartusik, Yang Liu, Yuanyuan Zhao, Mark Barahman, QianFeng Xu, Alan M. Lyons, and Alexander Greer pp 18990–18998 DOI: 10.1021/ja410529q Supporting Info |
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Influence of Side Chain Conformation and Configuration on Glycosyl Donor Reactivity and Selectivity as Illustrated by Sialic Acid Donors Epimeric at the 7-Position Pavan K. Kancharla and David Crich pp 18999–19007 DOI: 10.1021/ja410683y Supporting Info |
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Reversible Insertion of Carbenes into Ruthenium–Silicon Bonds María J. Bernal, Olga Torres, Marta Martı́n, and Eduardo Sola pp 19008–19015 DOI: 10.1021/ja410822p Supporting Info |
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Tuning Reactivity and Electronic Properties through Ligand Reorganization within a Cerium Heterobimetallic Framework Jerome R. Robinson, Zachary Gordon, Corwin H. Booth, Patrick J. Carroll, Patrick J. Walsh, and Eric J. Schelter pp 19016–19024 DOI: 10.1021/ja410688w Supporting Info |
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Brightness Enhanced DNA FIT-Probes for Wash-Free RNA Imaging in Tissue Felix Hövelmann, Imre Gaspar, Anne Ephrussi, and Oliver Seitz pp 19025–19032 DOI: 10.1021/ja410674h Supporting Info |
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Understanding the Photophysics of the Spinach–DFHBI RNA Aptamer–Fluorogen Complex To Improve Live-Cell RNA Imaging Kyu Young Han, Benjamin J. Leslie, Jingyi Fei, Jichuan Zhang, and Taekjip Ha pp 19033–19038 DOI: 10.1021/ja411060p Supporting Info |
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Strong Photon Energy Dependence of the Photocatalytic Dissociation Rate of Methanol on TiO2(110) Chengbiao Xu, Wenshao Yang, Zefeng Ren, Dongxu Dai, Qing Guo, Timothy K. Minton, and Xueming Yang pp 19039–19045 DOI: 10.1021/ja4114598 Supporting Info |
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Correction to “Stereospecific Substitution of Allylic Alcohols To Give Optically Active Primary Allylic Amines: Unique Reactivity of a (P,alkene)Ir Complex Modulated by Iodide” Markus Roggen and Erick M. Carreira pp 19046–19046 DOI: 10.1021/ja412119q Supporting Info |
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Spotlights on Recent JACS Publications ACS Contributing Correspondents pp 19047–19047 DOI: 10.1021/ja4125912 |
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Plant Biomass Recalcitrance: Effect of Hemicellulose Composition on Nanoscale Forces that Control Cell Wall Strength Rodrigo L. Silveira, Stanislav R. Stoyanov, Sergey Gusarov, Munir S. Skaf, and Andriy Kovalenko pp 19048–19051 DOI: 10.1021/ja405634k Supporting Info |
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A Cascade Cross-Coupling Hydrogen Evolution Reaction by Visible Light Catalysis Qing-Yuan Meng, Jian-Ji Zhong, Qiang Liu, Xue-Wang Gao, Hui-Hui Zhang, Tao Lei, Zhi-Jun Li, Ke Feng, Bin Chen, Chen-Ho Tung, and Li-Zhu Wu pp 19052–19055 DOI: 10.1021/ja408486v Supporting Info |
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Photon Upconverting Liquids: Matrix-Free Molecular Upconversion Systems Functioning in Air Pengfei Duan, Nobuhiro Yanai, and Nobuo Kimizuka pp 19056–19059 DOI: 10.1021/ja411316s Supporting Info |
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Structure Prediction of Au44(SR)28: A Chiral Superatom Cluster Yong Pei, Sisi Lin, Jingcang Su, and Chunyan Liu pp 19060–19063 DOI: 10.1021/ja409788k Supporting Info |
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Spectral Tuning of Ultraviolet Cone Pigments: An Interhelical Lock Mechanism Sivakumar Sekharan, Victoria L. Mooney, Ivan Rivalta, Manija A. Kazmi, Maureen Neitz, Jay Neitz, Thomas P. Sakmar, Elsa C. Y. Yan, and Victor S. Batista pp 19064–19067 DOI: 10.1021/ja409896y Supporting Info |
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A Well-Defined Silica-Supported Tungsten Oxo Alkylidene Is a Highly Active Alkene Metathesis Catalyst Matthew P. Conley, Victor Mougel, Dmitry V. Peryshkov, William P. Forrest, Jr., David Gajan, Anne Lesage, Lyndon Emsley, Christophe Copéret, and Richard R. Schrock pp 19068–19070 DOI: 10.1021/ja410052u Supporting Info |
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Subsecond and in Situ Chemical Speciation of Pt/Al2O3 during Oxidation–Reduction Cycles Monitored by High-Energy Resolution Off-Resonant X-ray Spectroscopy Jakub Szlachetko, Davide Ferri, Valentina Marchionni, Anastasios Kambolis, Olga V. Safonova, Christopher J. Milne, Oliver Kröcher, Maarten Nachtegaal, and Jacinto Sá pp 19071–19074 DOI: 10.1021/ja410146c Supporting Info |
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Heterometallic Triiron-Oxo/Hydroxo Clusters: Effect of Redox-Inactive Metals David E. Herbert, Davide Lionetti, Jonathan Rittle, and Theodor Agapie pp 19075–19078 DOI: 10.1021/ja4104974 Supporting Info |
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Identification of a Selective Polymerase Enables Detection of N6-Methyladenosine in RNA Emily M. Harcourt, Thomas Ehrenschwender, Pedro J. Batista, Howard Y. Chang, and Eric T. Kool pp 19079–19082 DOI: 10.1021/ja4105792 Supporting Info |
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Photoinduced Single-Molecule Magnet Properties in a Four-Coordinate Iron(II) Spin Crossover Complex Corine Mathonière, Hsiu-Jung Lin, Diana Siretanu, Rodolphe Clérac, and Jeremy M. Smith pp 19083–19086 DOI: 10.1021/ja410643s Supporting Info |
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Efficient Inorganic–Organic Hybrid Perovskite Solar Cells Based on Pyrene Arylamine Derivatives as Hole-Transporting Materials Nam Joong Jeon, Jaemin Lee, Jun Hong Noh, Mohammad Khaja Nazeeruddin, Michael Grätzel, and Sang Il Seok pp 19087–19090 DOI: 10.1021/ja410659k Supporting Info |
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How Half-Coated Janus Particles Enter Cells Yuan Gao and Yan Yu pp 19091–19094 DOI: 10.1021/ja410687z Supporting Info |
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Terazulene: A High-Performance n-Type Organic Field-Effect Transistor Based on Molecular Orbital Distribution Control Yuji Yamaguchi, Keisuke Ogawa, Ken-ichi Nakayama, Yoshihiro Ohba, and Hiroshi Katagiri pp 19095–19098 DOI: 10.1021/ja410696j Supporting Info |
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Electrochemical Patterning and Detection of DNA Arrays on a Two-Electrode Platform Ariel Furst, Sally Landefeld, Michael G. Hill, and Jacqueline K. Barton pp 19099–19102 DOI: 10.1021/ja410902j Supporting Info |
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1,5-Rhodium Shift in Rearrangement of N-Arenesulfonylazetidin-3-ols into Benzosultams Naoki Ishida, Yasuhiro Shimamoto, Takaaki Yano, and Masahiro Murakami pp 19103–19106 DOI: 10.1021/ja410910s Supporting Info |
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Bis(imino)pyridine Cobalt-Catalyzed Alkene Isomerization–Hydroboration: A Strategy for Remote Hydrofunctionalization with Terminal Selectivity Jennifer V. Obligacion and Paul J. Chirik pp 19107–19110 DOI: 10.1021/ja4108148 Supporting Info |
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Chemical Excision of Tetrahedral FeSe2 Chains from the Superconductor FeSe: Synthesis, Crystal Structure, and Magnetism of Fe3Se4(en)2 Chongin Pak, Saeed Kamali, Joyce Pham, Kathleen Lee, Joshua T. Greenfield, and Kirill Kovnir pp 19111–19114 DOI: 10.1021/ja410820u Supporting Info |
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Microporous Organic Network Hollow Spheres: Useful Templates for Nanoparticulate Co3O4 Hollow Oxidation Catalysts Narae Kang, Ji Hoon Park, Mingshi Jin, Nojin Park, Sang Moon Lee, Hae Jin Kim, Ji Man Kim, and Seung Uk Son pp 19115–19118 DOI: 10.1021/ja411263h Supporting Info |
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Macrocycle Contraction and Expansion of a Dihydrosapphyrin Isomer Yongshu Xie, Pingchun Wei, Xin Li, Tao Hong, Kai Zhang, and Hiroyuki Furuta pp 19119–19122 DOI: 10.1021/ja4112644 Supporting Info |
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4D Cryo-Electron Microscopy of Proteins Anthony W. P. Fitzpatrick, Ulrich J. Lorenz, Giovanni M. Vanacore, and Ahmed H. Zewail pp 19123–19126 DOI: 10.1021/ja4115055 Supporting Info |
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Enantioselective Total Syntheses of Leuconolam–Leuconoxine–Mersicarpine Group Monoterpene Indole Alkaloids Zhengren Xu, Qian Wang, and Jieping Zhu pp 19127–19130 DOI: 10.1021/ja4115192 Supporting Info |
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Phosphinecarboxamide: A Phosphorus-Containing Analogue of Urea and Stable Primary Phosphine Andrew R. Jupp and Jose M. Goicoechea pp 19131–19134 DOI: 10.1021/ja4115693 Supporting Info |
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Atomic Structure and Handedness of the Building Block of a Biological Assembly Antoine Loquet, Birgit Habenstein, Veniamin Chevelkov, Suresh Kumar Vasa, Karin Giller, Stefan Becker, and Adam Lange pp 19135–19138 DOI: 10.1021/ja411362q Supporting Info |
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Splitting Molecular Oxygen en Route to a Stable Molecule Containing Diphosphorus Tetroxide Yuzhong Wang, Yaoming Xie, Pingrong Wei, Henry F. Schaefer, III, Paul von R. Schleyer, and Gregory H. Robinson pp 19139–19142 DOI: 10.1021/ja411667f Supporting Info |
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A Self-Organizing Chemical Assembly Line Airton G. Salles, Jr., Salvatore Zarra, Richard M. Turner, and Jonathan R. Nitschke pp 19143–19146 DOI: 10.1021/ja412235e Supporting Info |
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From Solution to the Gas Phase: Stepwise Dehydration and Kinetic Trapping of Substance P Reveals the Origin of Peptide Conformations Joshua A. Silveira, Kyle L. Fort, DoYong Kim, Kelly A. Servage, Nicholas A. Pierson, David E. Clemmer, and David H. Russell pp 19147–19153 DOI: 10.1021/ja4114193 Supporting Info |
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Phosphinite-Iminopyridine Iron Catalysts for Chemoselective Alkene Hydrosilylation Dongjie Peng, Yanlu Zhang, Xiaoyong Du, Lei Zhang, Xuebing Leng, Marc D. Walter, and Zheng Huang pp 19154–19166 DOI: 10.1021/ja404963f Supporting Info |
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5-Azido-2-aminopyridine, a New Nitrene/Nitrenium Ion Photoaffinity Labeling Agent That Exhibits Reversible Intersystem Crossing between Singlet and Triplet Nitrenes Maxim S. Panov, Valentyna D. Voskresenska, Mikhail N. Ryazantsev, Alexander N. Tarnovsky, and R. Marshall Wilson pp 19167–19179 DOI: 10.1021/ja405637b Supporting Info |
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Green Emitting Photoproducts from Terrylene Diimide after Red Illumination Zhiyu Liao, Emma N. Hooley, Long Chen, Sebastian Stappert, Klaus Müllen, and Tom Vosch pp 19180–19185 DOI: 10.1021/ja407431w Supporting Info |
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Mixed Close-Packed Cobalt Molybdenum Nitrides as Non-noble Metal Electrocatalysts for the Hydrogen Evolution Reaction Bingfei Cao, Gabriel M. Veith, Joerg C. Neuefeind, Radoslav R. Adzic, and Peter G. Khalifah pp 19186–19192 DOI: 10.1021/ja4081056 Supporting Info |
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Effects of Si/Al Ratio on the Distribution of Framework Al and on the Rates of Alkane Monomolecular Cracking and Dehydrogenation in H-MFI Amber Janda and Alexis T. Bell pp 19193–19207 DOI: 10.1021/ja4081937 Supporting Info |
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Superenantioselective Chiral Surface Explosions Andrew J. Gellman, Ye Huang, Xu Feng, Vladimir V. Pushkarev, Brian Holsclaw, and Bharat S. Mhatre pp 19208–19214 DOI: 10.1021/ja408659v Supporting Info |
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Temporal Variation of a Protein Folding Energy Landscape in the Cell Anna Jean Wirth, Max Platkov, and Martin Gruebele pp 19215–19221 DOI: 10.1021/ja4087165 Supporting Info |
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Atomic Structure of an Ultrathin Fe-Silicate Film Grown on a Metal: A Monolayer of Clay? Radosław Włodarczyk, Joachim Sauer, Xin Yu, Jorge Anibal Boscoboinik, Bing Yang, Shamil Shaikhutdinov, and Hans-Joachim Freund pp 19222–19228 DOI: 10.1021/ja408772p |
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Enhanced Solid-State Order and Field-Effect Hole Mobility through Control of Nanoscale Polymer Aggregation Mark S. Chen, Olivia P. Lee, Jeremy R. Niskala, Alan T. Yiu, Christopher J. Tassone, Kristin Schmidt, Pierre M. Beaujuge, Seita S. Onishi, Michael F. Toney, Alex Zettl, and Jean M. J. Fréchet pp 19229–19236 DOI: 10.1021/ja4088665 Supporting Info |
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Higher Order Amyloid Fibril Structure by MAS NMR and DNP Spectroscopy Galia T. Debelouchina, Marvin J. Bayro, Anthony W. Fitzpatrick, Vladimir Ladizhansky, Michael T. Colvin, Marc A. Caporini, Christopher P. Jaroniec, Vikram S. Bajaj, Melanie Rosay, Cait E. MacPhee, Michele Vendruscolo, Werner E. Maas, Christopher M. Dobson, and Robert G. Griffin pp 19237–19247 DOI: 10.1021/ja409050a Supporting Info |
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Relating Chemical Structure to Device Performance via Morphology Control in Diketopyrrolopyrrole-Based Low Band Gap Polymers Feng Liu, Cheng Wang, Jayanta K. Baral, Lei Zhang, James J. Watkins, Alejandro L. Briseno, and Thomas P. Russell pp 19248–19259 DOI: 10.1021/ja408923y Supporting Info |
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Dynamics of an Ultrafast Folding Subdomain in the Context of a Larger Protein Fold Caitlin M. Davis and R. Brian Dyer pp 19260–19267 DOI: 10.1021/ja409608r Supporting Info |
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Spin Frustration from cis-Edge or -Corner Sharing Metal-Centered Octahedra Romain Gautier, Kengo Oka, Takumi Kihara, Nitesh Kumar, Athinarayanan Sundaresan, Masashi Tokunaga, Masaki Azuma, and Kenneth R. Poeppelmeier pp 19268–19274 DOI: 10.1021/ja409831h Supporting Info |
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Host–Guest Complexes as Water-Soluble High-Performance DNP Polarizing Agents Jiafei Mao, Dmitry Akhmetzyanov, Olivier Ouari, Vasyl Denysenkov, Björn Corzilius, Jörn Plackmeyer, Paul Tordo, Thomas F. Prisner, and Clemens Glaubitz pp 19275–19281 DOI: 10.1021/ja409840y Supporting Info |
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Why Is (SiO)4 Calculated To Be Tetrahedral, Whereas (CO)4 Is Square Planar? A Molecular Orbital Analysis Sebastian Kozuch, David A. Hrovat, and Weston Thatcher Borden pp 19282–19291 DOI: 10.1021/ja409887h Supporting Info |
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Evidence of Entropy-Driven Bistability through 15N NMR Analysis of a Temperature- and Solvent-Induced, Chiroptical Switching Polycarbodiimide James F. Reuther and Bruce M. Novak pp 19292–19303 DOI: 10.1021/ja4098803 Supporting Info |
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Polyoxometalate-Catalyzed Insertion of Oxygen from O2 into Tin–Alkyl Bonds Alexander M. Khenkin, Irena Efremenko, Jan M. L. Martin, and Ronny Neumann pp 19304–19310 DOI: 10.1021/ja409559h Supporting Info |
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Supramolecular Assembly of Multicomponent Photoactive Systems via Cooperatively Coupled Equilibria Miguel Garcı́a-Iglesias, Katrin Peuntinger, Axel Kahnt, Jan Krausmann, Purificación Vázquez, David González-Rodrı́guez, Dirk M. Guldi, and Tomás Torres pp 19311–19318 DOI: 10.1021/ja410114d Supporting Info |
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Crystal Structure of a Promoter Sequence in the B-raf Gene Reveals an Intertwined Dimer Quadruplex Dengguo Wei, Alan K. Todd, Mire Zloh, Mekala Gunaratnam, Gary N. Parkinson, and Stephen Neidle pp 19319–19329 DOI: 10.1021/ja4101358 Supporting Info |
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Stern Layer Formation Induced by Hydrophobic Interactions: A Molecular Level Study Rüdiger Scheu, Yixing Chen, Mireia Subinya, and Sylvie Roke pp 19330–19335 DOI: 10.1021/ja4102858 |
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CO Oxidation on TiO2 (110) Supported Subnanometer Gold Clusters: Size and Shape Effects Lei Li, Yi Gao, Hui Li, Yu Zhao, Yong Pei, Zhongfang Chen, and Xiao Cheng Zeng pp 19336–19346 DOI: 10.1021/ja410292s Supporting Info |
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Base-Excision Repair Activity of Uracil-DNA Glycosylase Monitored Using the Latch Zone of α-Hemolysin Qian Jin, Aaron M. Fleming, Robert P. Johnson, Yun Ding, Cynthia J. Burrows, and Henry S. White pp 19347–19353 DOI: 10.1021/ja410615d Supporting Info |
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Model Peptides Uncover the Role of the β-Secretase Transmembrane Sequence in Metal Ion Mediated Oligomerization Lisa M. Munter, Holger Sieg, Tobias Bethge, Filip Liebsch, Frank S. Bierkandt, Michael Schleeger, Heiko J. Bittner, Joachim Heberle, Norbert Jakubowski, Peter W. Hildebrand, and Gerd Multhaup pp 19354–19361 DOI: 10.1021/ja410812r Supporting Info |
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Correction to “Cyclization Cascades Initiated by 1,6-Conjugate Addition” Joshua L. Brooks and Alison J. Frontier pp 19362–19362 DOI: 10.1021/ja4118363 |